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Technical report with results for 156Eu

The evaluated γ-ray branching ratio values after the decay of 156 Eu are based on measurements done in the 1960s and 1970s which improve upon measurements done back in the 1950s. These experiments, while improving on each other, were not able to produce nearly pure samples and impurities produced along with the sample ( 152 Eu, 154 Eu, and 155 Eu) interfered with the study of the beta spectrum for 156Eu. The values for the branching ratios of 156 Eu from National Nuclear Data Center (NNDC) [4] have uncertainties of ranging from 7-14% for the 10 most intense γ rays and up to 30% for the weaker ones. This work aims to improve the precision on the majority of these γ-ray branches.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Investigating the role of edge neutrals in exciting tearing mode activity and achieving flat temperature profiles in LTX-β

Abstract We present observations, numerical simulations, and analysis from experiments in the Lithium Tokamak Experiment-Beta (LTX- β ) in which the electron temperature profile ( T e ( r )) shifts from flat to peaked and a tearing mode is also destabilized when the average density ( n e ave ) exceeds ∼10 19 m −3 . Flat T e ( r ) is obtained routinely in LTX- β , with a lithium coated, low-recycling first wall, once the external fueling is stopped and density decays [Boyle et al 2023 Nucl. Fusion 63 056020]. In the present experiment, flat T e profiles can be sustained while maintaining constant n e ave below a line averaged density threshold ( n e ave th ) of ∼10 19 m −3 . Above n e ave th , T e ( r ) shifts from flat to peaked and a tearing mode is destabilized. Due to low recycling, the achieved n e ave can be controlled precisely by external fueling and hence, a certain threshold of the edge neutral inventory from the external fueling is experimentally manifested through n e ave th . The goal of the present work is to investigate the role of edge neutrals in determining T e ( r ) and MHD stability in the unique low-recycling regime of LTX- β . Our hypothesis is that the peaking of T e ( r ) beyond n e ave th is due ultimately to the edge cooling by the cold neutrals beyond a critical fueling flux. At lower fueling flux, flat T e ( r ) results in broader pressure profile and lower resistivity, which in turn stabilizes the tearing mode. This hypothesis is supported by edge neutral density estimation by DEGAS 2 code. Mode analysis by singular value decomposition confirms the tearing mode structure to be m / n = 2/1 ( m and n being the poloidal and toroidal mode numbers). Linear tearing stability analysis with M3D-C1 predicts that plasmas with n e ave > 10 19 are highly susceptible to a n = 1 tearing mode. ORBIT simulations, however, confirmed that the tearing modes do not contribute to the loss of fast ions from neutral beam injection. This study shows for the first time that the neutral inventory at the edge could be one of the deciding factors for the achievability of the unique operation regime of flat T e ( r ) and the excitation of tearing activity that could be disruptive for the plasmas.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Evaluation of Attila and MCNP computational methods for dose and exposure estimation

Radiation transport calculations are often used to estimate dose or exposure to components and personnel surrounding a radiation source. The sources for these calculations are decaying radionuclides within various nuclear materials. Historically, dose calculations use MCNP (Monte Carlo N-Particle) transport code as the primary particle transport tool without a secondary computational tool to validate the results from the MCNP simulations [1]. The goal of this study is to make an independent check of the Monte Carlo solution from MCNP6 Version 6.2.1 with the discrete ordinates solution from Attila 10.2.0 Beta 3. As an example problem for this study, water-filled, stainless-steel vessels, modeled with an unstructured mesh (UM) with both MCNP and Attila [2], are exposed to 252Cf and 60Co point sources. This report also includes a discussion of the limitations of unstructured mesh in a MCNP calculation.

61 RADIATION PROTECTION AND DOSIMETRY↗

Time-Resolved Radioluminescence of the Polynuclear Copper(I) Phosphor Cu4I6²–. Different Temporal responses to Photo, X-Ray, β-Ray and α-Particle Excitation

Described for the first time are the time-resolved radioluminescence (TRRL) properties of the highly luminescent copper(I) cluster Cu4I62– using X-ray, b-ray and a-particle excitation. The copper(I) phosphors are two crystalline salts of this anion, [Na2(18-crown-6)2(H2O)3][Cu4I6] (I) and [Li(benzo-15-crown-5)2(H2O)]2[Cu4I6] (II), that had been shown to display strong photoluminescence (PL) when excited with ultraviolet light. The integrated radioluminescence (RL) spectra observed when pulsed X-rays were used as the excitation source are virtually the same as the PL spectra under comparable conditions. These temporal RL spectra are invariant at all observation times indicating that the observed scintillation occurs from a common excited state (or set of excited states). When the TRRL is collected from excitation with a pulsed X-ray source, b-ray decay from 90Sr or a-decay from 244Cm, the longer components (>2 μs) of the TRRL displayed (in each case) lifetimes comparable to those of the strictly exponential PL decays recorded under pulsed laser UV excitation. However, at shorter observation times (< 500 ns), the RL decay deviated from the exponential model, indicating a markedly different temporal luminescence behavior when these materials were excited with pulsed high energy radiation. Furthermore, this effect was the most pronounced for the a-particle excitation. These results suggest that the absorption of a very high energy X-ray photon, b-ray or a-particle at a site within the crystalline solid leads to a high local density of electronic excited states and that coupling between these states provides an alternative channel for excited state decay. Given that the patterns observed

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗

Low Level Calibration of Liquid Scintillation Counting

Liquid Scintillation Counting (LSC) is an analytical laboratory method that quantifies the concentrations of alpha and beta emitting isotopes. The LSC method can be utilized for the detection of tritium, both environmentally and at nuclear facilities. Most LSC samples are aqueous-based and prepared as a radioactive sample dissolved or suspended in a high efficiency scintillation cocktail that converts radioactive energy into light pulses. When placed in counting vials, the liquid scintillation cocktail allows for optical coupling in which energy is released from the samples radioactive decay, and transferred to the scintillator. That energy is then absorbed to produce excited electrons that fall back to their ground-state and emit a pulse of light that is detected by the liquid scintillation analyzers photomultiplier tubes. Quench is a signal attenuation due to physical, chemical, or color interferences. To compensate for quench, quench standards of a known concentration are implemented at increasing increments of quench per vial to create a quench curve. Quench standards can be purchased pre-made or customized from the manufacturer, however, there are several issues that arise from purchasing the pre-made quench standards. The main issues with ordering pre-made quench standards is that they use higher count values, between 30,000 and 250,000 disintegrations per minute (dpm) of tritium per vial and only come in glass vials. Using higher counting standards in glass vials makes it hard to see lower concentrations in plastic vials. Additionally, when using higher energy standards the accuracy of the calibration readings tend to be lower. On the other hand, making a set of quench standards in-house allows for the customization of the dpm concentration to roughly 1,500-3,000 and preparation in plastic vials. This allows for lower activity readings that results in closer precision of the samples' true concentration. Technical Objectives: Create a quench curve and calibrate the LSA for tritium. Verify the calibration of the quench curve prior to cross sample runs. Check calibration against Quality Control (QC) reference value. Conclusion: a tritium quench curve calibration was performed using a scintillation cocktail with ultima gold (AB and AB/F), acetone (only with AB), and water (only with AB/F). By performing the tritium quench curve calibration, the counting efficiency was correlated to various levels of quench. Calibration checks with quality control standards were also performed to verify that the calibration was correct. The observed results provided acceptable values that matched the quality control standard reference values with an acceptable uncertainty. The next step will be fine tuning and cross comparison checks with legacy instrumentation.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Determination of the 161 Tb half-life

There is significant interest in the use of terbium radioisotopes for applications in cancer therapy and diagnosis. Of these, 161 Tb, a medium energy beta- and prolific auger emitter, is being investigated as a potential alternative to 177 Lu. The higher proportion of conversion electron and Auger electron emissions, and variety of low-energy gammas make 161 Tb an attractive targeted theranostic. As a product of nuclear fission, 161 Tb is also of importance to nuclear forensics. The current evaluated half-life of 6.89(2) d has a standard uncertainty that contributes significantly to the standard uncertainty of decay calculated activity determination. Furthermore, the accuracy of this evaluated half-life has been called into question by measurements reported recently at the Institute of Radiation Physics (IRP), Switzerland. In this work, the half-life of 161 Tb was measured at three independent laboratories located in the United Kingdom and United States of America for a total of five determinations using three independent measurement techniques. In conclusion, the half-life determined for 161 Tb of 6.9637(29) d confirms the observed 1 % relative increase observed by IRP, though the reported half-lives in this work and at IRP are significantly different (ζ-score = 3.1).

half-life↗

A new method for quantifying 64 Cu in nuclear debris samples

Quantifying 64 Cu in post-detonation nuclear debris samples can provide important diagnostic information regarding the structural materials used within a nuclear device. However, this task is challenging due to the weak gamma emissions associated with the decay of 64 Cu, its short half-life (12.701 h), and the presence of interfering fission product radioisotopes. Large quantities of debris sample are generally needed to accurately quantify 64 Cu, which can be problematic in sample-limited scenarios where other radiometric analyses are required. Herein, we present a new method for the separation of 64 Cu from solutions of mixed fission products and demonstrate the quantification of its activity through use of gas-flow proportional beta counting. Here, the new method was validated through a series of rigorous tests and was shown to improve the detection limit of 64 Cu by over two orders of magnitude, from 2.5 × 10 6 to 1.3 × 10 4 atoms/sample for 100 min measurements.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗

Jet substructure from dark sector showers

We examine the robustness of collider phenomenology predictions for a dark sector scenario with QCD-like properties. Pair production of dark quarks at the LHC can result in a wide variety of signatures, depending on the details of the new physics model. A particularly challenging signal results when prompt production induces a parton shower that yields a high multiplicity of collimated dark hadrons with subsequent decays to Standard Model hadrons. The final states contain jets whose substructure encodes their non-QCD origin. This is a relatively subtle signature of strongly coupled beyond the Standard Model dynamics, and thus it is crucial that analyses incorporate systematic errors to account for the approximations that are being made when modeling the signal. We estimate theoretical uncertainties for a canonical substructure observable designed to be sensitive to the gauge structure of the underlying object, the two-point energy correlator $ {e}_2^{\left(\beta \right)} $ , by computing envelopes between resummed analytic distributions and numerical results from Pythia. We explore the separability against the QCD background as the confinement scale, number of colors, number of flavors, and dark quark masses are varied. Additionally, we investigate the uncertainties inherent to modeling dark sector hadronization. Simple estimates are provided that quantify one’s ability to distinguish these dark sector jets from the overwhelming QCD background. Such a search would benefit from theory advances to improve the predictions, and the increase in statistics using the data to be collected at the high luminosity LHC.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Collaborative Research: Parametric Instabilities of Alfven Waves in Low‐beta Plasmas

Alfven waves are of fundamental importance in magnetized plasmas. This project aims to advance our understanding of the basic physics of the parametric instabilities of Alfven waves using advanced computer simulations. The results will have implications for important processes in the heliosphere involving Alfven waves, such as coronal heating and solar wind heating.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Improving Fission Products at CARIBU: Near Field Detection (Q1/FY21 Quarterly Progress Report)

After receiving funds at the beginning of FY21 we were able to resume work on the project. We continued data analysis of 156 Eu decay. The project has also gone through an Independent Review in November. Following the previously reported steps in the analysis of 156 Eu, specifically removing random coincidences from the gamma ray spectrum, we look not only at the peak of interest (811 keV) but all other gamma rays that are visible. Determining the area of all gamma ray peaks in this random coincidence free spectrum is not only necessary to calculate the gamma ray branching ratios but combined with the peak areas of the gamma ray singles spectrum we are able to determine experimentally the efficiency of the beta detector.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Assessment of Baseline Monitoring Data for the Remote-Handled Low-Level Waste Disposal Facility at Idaho National Laboratory

The purpose of this document is to summarize environmental monitoring data collected at the Remote-Handled Low-Level Waste (RHLLW) Disposal Facility during the first four years of facility operations (FY 2019 through FY 2022). This summary provides a “baseline” condition for the facility, which can be used to distinguish contaminant releases from the RHLLW Disposal Facility from pre existing contamination as well as potential future releases from other sources (i.e., upgradient aquifer sources), as specified in the facility monitoring plan. Sufficient data has been collected over the first four years of operation of the RHLLW Disposal Facility to establish baseline conditions for future compliance monitoring of aquifer wells and performance monitoring of vadose zone lysimeters. Except for seven elevated tritium measurements from lysimeter HFEF-South believed to have been impacted by waste disposals, all data was deemed appropriate for establishing baseline concentrations. Monitoring of the aquifer detected indicator analytes gross alpha and gross beta and target analytes tritium and C-14. There were a few C-14 detections prior to an increase in the required detection level (RDL) after the first round of sampling. I-129 and Tc-99 were not detected above RDLs in aquifer samples. Lysimeter samples detected indicator analytes gross alpha and gross beta and target analyte tritium. Target analytes C-14, I-129, and Tc-99 were not detected above RDLs in lysimeter samples. Except for tritium, baseline concentrations of indicator and target analytes measured during the first four years of RHLLW facility operations are expected to represent conditions through the expected 20 year operating period of the facility. Elevated tritium in the aquifer, a result of past discharges of tritium at upgradient facilities, showed a decline over the first four years of operations, and levels are expected to continue to decline with time as a result of dilution and decay. Current tritium levels in lysimeter samples may be elevated due to tritium in the water applied during construction and infiltration testing of the facility. As a result, tritium concentrations in lysimeters may decline with time as a result of dilution and decay. Statistical measures (i.e., mean, standard deviation, and 99% upper confidence level [UCL]) were calculated for all detected analytes using the four years of concentration data. These measures will be used to evaluate future monitoring results and to demonstrate the facility is performing, or not performing, as established in the facility performance assessment (PA). Future monitoring results will also be combined with the baseline data in this report to further establish temporal trends and natural variability in the measurements. Based on the data collected during the baseline period, it is recommended the gross alpha action level for performance monitoring increase from 10 to 20 pCi/L due to several baseline measurements exceeding the preliminary action level of 10. An action level of 20 pCi/L is slightly greater than the 99% UCL, is protective of the aquifer, and would reduce unnecessary sampling. It is also recommended that tritium be added to the lysimeter analyte list for post-baseline period monitoring. Tritium, while not a dose concern, is a good tracer that can provide valuable information on water flow in and around the RHLLW Disposal Facility. Recommendations for a tritium action level are provided if considered necessary.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Characterization of the image plate multi-scan response to mono-energetic x-rays

Image plates (IPs), or phosphor storage screens, are a technology employed frequently in inertial confinement fusion (ICF) and high energy density plasma (HEDP) diagnostics because of their sensitivity to many types of radiation, including, x rays, protons, alphas, beta particles, and neutrons. Prior studies characterizing IPs are predicated on the signal level remaining below the scanner saturation threshold. Since the scanning process removes some signal from the IP via photostimulated luminescence, repeatedly scanning an IP can bring the signal level below the scanner saturation threshold. This process, in turn, raises concerns about the signal response of IPs after an arbitrary number of scans and whether such a process yields, for example, a constant ratio of signal between the nth and n + 1st scan. Here, the sensitivity of IPs is investigated when scanned multiple times. It is demonstrated that the ratio of signal decay is not a constant with the number of scans and that the signal decay depends on the x-ray energy. As such, repeatedly scanning an IP with a mixture of signal types (e.g., x ray, neutron, and protons) enables ICF and HEDP diagnostics employing IPs to better isolate a particular signal type.

Instruments & Instrumentation↗

Effects of temperature and density evolution in MHD simulations of HIT-SI

The helicity injected torus-steady inductive (HIT-SI) experiment uses steady inductive helicity injection to form a spheromak equilibrium and sustain the structure against resistive decay. Helicity injection is performed using two half-tori “injectors” connected to the main plasma volume, whose fields are oscillated in an AC manner. The properties of the sustained spheromak equilibrium have been experimentally observed to vary with the frequency of the injector oscillation, producing higher current gains and more-symmetric and outwardly shifted current centroids with higher frequency. A computational scan of injector frequency using the 3D MHD code PSI-Tet, which models the entire HIT-SI plasma volume including the injectors, has been performed, including a comparison of the results using the full Hall MHD model to those obtained using a simplified “zero-beta” (constant temperature and density) model. The results of both PSI-Tet models are also compared with experimental data and with simulations using the NIMROD code, which does not model the injector regions. The results of the PSI-Tet simulations show that the average temperature and current gain increase with injector frequency, in agreement with experimental trends. The simulations also show qualitative changes in the dynamics of several quantities with increasing injector frequency, such as density oscillations and current evolution. However, the outward shift and symmetrizing of the current centroid, observed experimentally, are not observed in these MHD simulations, indicating that unresolved or excluded dynamics may be important.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Search for heavy Higgs bosons decaying to a top quark pair in proton-proton collisions at $ \sqrt{s} $ = 13 TeV

A search is presented for additional scalar (H) or pseudoscalar (A) Higgs bosons decaying to a top quark pair in proton-proton collisions at a center-of-mass energy of 13 TeV. The data set analyzed corresponds to an integrated luminosity of 35.9 fb$^{-1}$ collected by the CMS experiment at the LHC. Final states with one or two charged leptons are considered. The invariant mass of the reconstructed top quark pair system and variables that are sensitive to the spin of the particles decaying into the top quark pair are used to search for signatures of the H or A bosons. The interference with the standard model top quark pair background is taken into account. A moderate signal-like deviation compatible with an A boson with a mass of 400 GeV is observed with a global significance of 1.9 standard deviations. New stringent constraints are reported on the strength of the coupling of the hypothetical bosons to the top quark, with the mass of the bosons ranging from 400 to 750 GeV and their total relative width from 0.5 to 25%. The results of the search are also interpreted in a minimal supersymmetric standard model scenario. Values of $m_\mathrm{A}$ from 400 to 700 GeV are probed, and a region with values of $\tan\beta$ below 1.0 to 1.5, depending on $m_\mathrm{A}$, is excluded at 95% confidence level.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Critical problems of energy frontier Muon Colliders: optics, magnets and radiation

This White Paper brings together our previous studies on a Muon Collider (MC) and presents a design concept of the 6 TeV MC optics, the superconducting (SC) magnets, and a preliminary analysis of the protection system to reduce magnet radiation loads as well as particle backgrounds in the detector. The SC magnets and detector protection considerations impose strict limitations on the lattice choice, hence the design of the collider optics, magnets and Machine Detector Interface (MDI) are closely intertwined. As a first approximation we use the Interaction Region (IR) design with beta-star=3 mm, whereas for the arcs we re-scale the arc cell design of the 3 TeV MC. Traditional cos-theta coil geometry and Nb3Sn superconductor were used to provide field maps for the analysis and optimization of the arc lattice and IR design, as well as for studies of beam dynamics and magnet protection against radiation. The stress management in the coil will be needed to avoid large degradation or even damage of the brittle SC coils. In the assumed IR designs, the dipoles close to the Interaction Point (IP) and tungsten masks in each IR (to protect magnets) help reducing background particle fluxes in the detector by a substantial factor. The tungsten nozzles in the 6 to 600 cm region from the IP, assisted by the detector solenoid field, trap most of the decay electrons created close to the IP as well as most of the incoherent electron-positron pairs generated in the IP. With sophisticated tungsten, iron, concrete and borated polyethylene shielding in the MDI region, the total reduction of background loads by more than three orders of magnitude can be achieved.

43 PARTICLE ACCELERATORS↗

Assessment of Thin Plastic Scintillation Detectors for Beta-Particle Measurements at the Advanced Test Reactor Critical Facility

The Fission Wire Measurement System is a custom measurement system designed in the 1960s to measure the beta-particle activity of irradiated uranium-aluminum fission wires. This measurement is conducted to determine the fission rate profile of the Advanced Reactor Test Critical facility. The Advanced Test Reactor Critical facility is an open-pool, low-power test reactor used to qualify experiment configurations and verify core models prior to full-power experiment irradiations in the Advanced Test Reactor. Power distribution measurements in ATR-C use uranium-aluminum wires that are distributed throughout the core to validate simulation and modeling results. These measurements require from 340 to 1500 wires to be irradiated and measured within a 12-hour window. The system consists of 4 measurement channels and one reference channel, each with a 2-pi proportional gas flow detector and the measurement channels each have an automated sample changer. The gas flow detectors are of a custom design for this detector system that use methane gas with a large anode wire compared to modern proportional counters. These detectors, which are nearly 60 years old are irreplaceable. The measurements from these gas detectors are affected by the gas flow rate, atmospheric and line pressure, and are very sensitive to the applied high voltage. Recent improvements have been made to the control and data acquisition system, but the detectors have remained the same. The nature of the measurement of the fission product decay activity is such that the energy spectrum of the signal is changing with time. Thin, 250-um thick, plastic scintillators were commercially obtained as a potential replacement for the gas flow detectors. The original calibration of the uranium-aluminum fission wires was conducted in 1965 using a series of irradiations of gold foils and the wires in a well-characterized thermal neutron field. These measurements provided a time-dependent fission rate conversion factor from the gold foil data to calibrate the fission wires based on the response from the 2-pi proportional gas detectors. Transitioning to the new detectors requires qualification and testing. The sensitivity of the scintillators to changes in the energy spectrum of the fission wires and translation of the calibration factor have been completed. These measurements indicated that the sensitivity of the scintillators over time changes at a different rate than the sensitivity of the gas flow detectors. However, the inverse activity of measurements of both detector types is linear with time. Initial results indicate that the scintillator detectors will be a sufficient replacement for the gas detectors with minor adjustments to the fission rate conversion factor. Replacement of the detectors will improve the fission wire measurements and provide a more stable and reliable measurement system.

46 - INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AN↗

Evidence of Quadrupole and Octupole Deformations in Zr 96 + Zr 96 and Ru 96 + Ru 96 Collisions at Ultrarelativistic Energies

In the hydrodynamic model description of heavy-ion collisions, the elliptic flow v 2 and triangular flow v 3 are sensitive to the quadrupole deformation β 2 and octupole deformation β 3 of the colliding nuclei. The relations between v n and β n have recently been clarified and were found to follow a simple parametric form. The STAR Collaboration has just published precision v n data from isobaric Ru 96 + Ru 96 and Zr 96 + Zr 96 collisions, where they observe large differences in central collisions v 2 , Ru > v 2 , Zr and v 3 , Ru < v 3 , Zr . Using a transport model simulation, we show that these orderings are a natural consequence of $\beta_{2,Ru} \gg \beta_{2,Zr}$ and $\beta_{3,Ru} \ll \beta_{3,Zr}$ We reproduce the centrality dependence of the v 2 ratio qualitatively and v 3 ratio quantitatively and extract values of β 2 and β 3 that are consistent with those measured at low-energy nuclear structure experiments. STAR data provide the first direct evidence of strong octupole correlations in the ground state of Zr 96 in heavy-ion collisions. Our analysis demonstrates that flow measurements in high-energy, heavy-ion collisions, especially using isobaric systems, are a new precision tool to study nuclear structure physics.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Updated search for $ {B}_c^{+} $ decays to two charm mesons

A data set corresponding to an integrated luminosity of 9 fb -1 of proton-proton collisions collected by the LHCb experiment has been analysed to search for B c + → D s &lowast; + — D &lowast; 0 decays. The decays are fully or partially reconstructed, where one or two missing neutral pions or photons from the decay of an excited charm meson are allowed. Upper limits for the branching fractions, normalised to B + decays to final states with similar topologies, are obtained for sixteen $ {B}_c^{+} $ decay modes. For the decay $ {B}_c^{+}\to {D}_s^{+}{\overline{D}}^0 $, an excess with a significance of 3.4 standard deviations is found.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗