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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 649 records · Page 36
All sourcesNASA NTRSDOE OSTI
DOE OSTI2015

On thermalization of electron-positron-photon plasma

Recently a progress has been made in understanding thermalization mechanism of relativistic plasma starting from a non-equilibrium state. Relativistic Boltzmann equations were solved numerically for homogeneous isotropic plasma with collision integrals for two- and three-particle interactions calculated from the first principles by means of QED matrix elements. All particles were assumed to fulfill Boltzmann statistics. In this work we follow plasma thermalization by accounting for Bose enhancement and Pauli blocking in particle interactions. Our results show that particle in equilibrium reach Bose-Einstein distribution for photons, and Fermi-Dirac one for electrons, respectively.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
NASA NTRS2016

Development of the Model of Galactic Interstellar Emission for Standard Point-Source Analysis of Fermi Large Area Telescope Data

Most of the celestial gamma rays detected by the Large Area Telescope (LAT) on board the Fermi Gamma-ray Space Telescope originate from the interstellar medium when energetic cosmic rays interact with interstellar nucleons and photons. Conventional point-source and extended-source studies rely on the modeling of this diffuse emission for accurate characterization. Here, we describe the development of the Galactic Interstellar Emission Model (GIEM),which is the standard adopted by the LAT Collaboration and is publicly available. This model is based on a linear combination of maps for interstellar gas column density in Galactocentric annuli and for the inverse-Compton emission produced in the Galaxy. In the GIEM, we also include large-scale structures like Loop I and the Fermi bubbles. The measured gas emissivity spectra confirm that the cosmic-ray proton density decreases with Galactocentric distance beyond 5 kpc from the Galactic Center. The measurements also suggest a softening of the proton spectrum with Galactocentric distance. We observe that the Fermi bubbles have boundaries with a shape similar to a catenary at latitudes below 20deg and we observe an enhanced emission toward their base extending in the north and south Galactic directions and located within approximately 4deg of the Galactic Center.

gamma rays: diffuse background – gamma rays: gen↗
DOE OSTI2011

Cosmic rays in the surroundings of SNR G35.6–0.4

HESS J1858+020 is a TeV gamma-ray source that was reported to have no clearly catalogued counterpart at any wavelength. However, it has been recently proposed that this source is indirectly associated with the radio source, re-identified as a supernova remnant (SNR), G35.6–0.4. The latter has been found to be middle-aged (~30 kyr) and to have nearby molecular clouds (MCs). HESS J1858+020 was proposed to be the result of the interaction of protons accelerated in the SNR shell with target ions residing in the clouds. The Fermi Large Area Telescope (LAT) First Source Catalog does not list any source coincident with the position of HESS J1858+020, but some lie close. Here, we analyse more than 2 years of data obtained with the Fermi -LAT for the region of interest, and consider whether it is indeed possible that the closest LAT source, 1FGL J1857.1+0212c, is related to HESS J1858+020. We conclude it is not, and we impose upper limits on the GeV emission originating from HESS J1858+020. Using a simplified 3D model for the cosmic ray propagation out from the shell of the SNR, we consider whether the interaction between SNR G35.6–0.4 and the MCs nearby could give rise to the TeV emission of HESS J1858+020 without producing a GeV counterpart. If so, the pair of SNR/TeV source with no GeV detection would be reminiscent of other similarly aged SNRs, such as some of the TeV hotspots near W28, for which cosmic ray diffusion may be used to explain their multifrequency phenomenology. Furthermore, for HESS J1858+020, we found that although the phase space in principle allows such a GeV–TeV non-correlation to appear, usual and/or observationally constrained values of the parameters (e.g., diffusion coefficients and cloud–SNR likely distances) would disfavour it.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2018

Creating Spin-One Fermions in the Presence of Artificial Spin–Orbit Fields: Emergent Spinor Physics and Spectroscopic Properties

We propose the creation and investigation of a system of spin-one fermions in the presence of artificial spin–orbit coupling, via the interaction of three hyperfine states of fermionic atoms to Raman laser fields. We explore the emergence of spinor physics in the Hamiltonian described by the interaction between light and atoms, and analyze spectroscopic properties such as dispersion relation, Fermi surfaces, spectral functions, spin-dependent momentum distributions and density of states. Connections to spin-one bosons and SU(3) systems is made, as well relations to the Lifshitz transition and Pomeranchuk instability are presented.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2018

Photoexcited Graphene Metasurfaces: Significantly Enhanced and Tunable Magnetic Resonances

Artificially constructed metamaterials or metasurfaces with tailored resonant elements provide a revolutionary platform for controlling light at the subwavelength scale. Switchable or frequency-agile meta-devices are highly desirable in achieving more flexible functionalities and have been explored extensively by incorporating various materials, which respond to external stimuli. Graphene, a two-dimensional material showing extraordinary physical properties, has been found very promising for tunable meta-devices. However, the high intrinsic loss of graphene severely obstructs us from achieving high-quality resonance in various graphene metamaterials and metasurfaces, and the loss compensation can be considered as a straightforward strategy to take further advantages of enhanced light–graphene interactions. Here, we demonstrate that the photoexcited graphene, in which the quasi-Fermi energy of graphene changes corresponding to optical pumping, can boost the originally extremely weak magnetic resonance in a graphene split-ring metasurface, showing remarkable modulations in the transmission. In conclusion, our work pioneers the possibilities of optically pumped graphene metasurfaces for significant enhancement of resonances and feasible modulations.

36 MATERIALS SCIENCE↗
DOE OSTI2021

Evidence of a coupled electron-phonon liquid in NbGe 2

Whereas electron-phonon scattering relaxes the electron’s momentum in metals, a perpetual exchange of momentum between phonons and electrons may conserve total momentum and lead to a coupled electron-phonon liquid. Such a phase of matter could be a platform for observing electron hydrodynamics. Here we present evidence of an electron-phonon liquid in the transition metal ditetrelide, NbGe 2 , from three different experiments. First, quantum oscillations reveal an enhanced quasiparticle mass, which is unexpected in NbGe 2 with weak electron-electron correlations, hence pointing at electron-phonon interactions. Second, resistivity measurements exhibit a discrepancy between the experimental data and standard Fermi liquid calculations. Third, Raman scattering shows anomalous temperature dependences of the phonon linewidths that fit an empirical model based on phonon-electron coupling. We discuss structural factors, such as chiral symmetry, short metallic bonds, and a low-symmetry coordination environment as potential design principles for materials with coupled electron-phonon liquid.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2021

Charge density waves in cuprate superconductors beyond the critical doping

The unconventional normal-state properties of the cuprates are often discussed in terms of emergent electronic order that onsets below a putative critical doping of x c ≈ 0.19. Charge density wave (CDW) correlations represent one such order; however, experimental evidence for such order generally spans a limited range of doping that falls short of the critical value x c , leading to questions regarding its essential relevance. Here, we use X-ray diffraction to demonstrate that CDW correlations in La 2–x Sr x CuO 4 persist up to a doping of at least x = 0.21. The correlations show strong changes through the superconducting transition, but no obvious discontinuity through x c ≈ 0.19, despite changes in Fermi surface topology and electronic transport at this doping. These results demonstrate the interaction between CDWs and superconductivity even in overdoped cuprates and prompt a reconsideration of the role of CDW correlations in the high-temperature cuprate phase diagram.

36 MATERIALS SCIENCE↗
DOE OSTI2021

Solution-phase p-type doping of highly enriched semiconducting single-walled carbon nanotubes for thermoelectric thin films

Single-walled carbon nanotubes (SWCNTs) are attractive materials for next-generation energy-harvesting technologies, including thermoelectric generators, due to their tunable opto-electronic properties and high charge carrier mobilities. Controlling the Fermi level within these unique 1D nanomaterials is often afforded by charge transfer interactions between SWCNTs and electron or hole accepting species. Conventional methods to dope SWCNT networks typically involve the diffusion of molecular redox dopant species into solid-state thin films, but solution-phase doping could potentially provide routes and/or benefits for charge carrier transport, scalability, and stability. Here, we develop a methodology for solution-phase doping of polymer-wrapped, highly enriched semiconducting SWCNTs using a p-type charge transfer dopant, F4TCNQ. This allows doped SWCNT inks to be cast into thin films without the need for additional post-deposition doping treatments. We demonstrate that the introduction of the dopant at varying stages of the SWCNT dispersion process impacts the ultimate thermoelectric performance and observe that the dopant alters the polymer selectivity for semiconducting vs metallic SWCNTs. In contrast to dense semiconducting polymer films, where solution-phase doping typically leads to disrupted morphologies and poorer TE performance than solid-state doping, thin films of solution-doped s-SWCNTs perform similarly to their solid-state doped counterparts. Interestingly, our results also suggest that solution-phase F4TCNQ doping leads to fully ionized and dimerized F4TCNQ anions in solid-state films that are not observed in films doped with F4TCNQ after deposition. Our results provide a framework for the application of solution-phase doping to a broad array of high-performance SWCNT-based thermoelectric materials and devices that may require high-throughput deposition techniques.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2015

TORSIONAL OSCILLATIONS OF NONBARE STRANGE STARS

Strange stars are one of the possible compact stellar objects that can form after a supernova collapse. We consider a model of a strange star having an inner core in the color-flavor locked phase surmounted by a crystalline color superconducting (CCSC) layer. These two phases constitute the quarksphere, which we assume to be the largest and heaviest part of the strange star. The next layer consists of standard nuclear matter forming an ionic crust, hovering on the top of the quarksphere and prevented from falling by a strong dipolar electric field. The dipolar electric field arises because quark matter is confined in the quarksphere by the strong interaction, but electrons can leak outside forming an electron layer a few hundred fermi thick separating the ionic crust from the underlying quark matter. The ionic matter and the CCSC matter constitute two electromagnetically coupled crust layers. We study the torsional oscillations of these two layers. Remarkably, we find that if a fraction larger than 10{sup −4} of the energy of a Vela-like glitch is conveyed to a torsional oscillation, the ionic crust will likely break. The reason is that the very rigid and heavy CCSC crust layer will absorb only a small fraction of the glitch energy, leading to a large-amplitude torsional oscillation of the ionic crust. The maximum stress generated by the torsional oscillation is located inside the ionic crust and is very close to the star’s surface. This peculiar behavior leads to a much easier crust cracking than in standard neutron stars.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2020

Selective hybridization between the main band and the superstructure band in the Bi 2 Sr 2 CaCu 2 O 8 + δ superconductor

High-resolution laser-based angle-resolved photoemission measurements have been carried out on Bi 2 Sr 2 CaCu 2 O 8+δ (Bi2212) and Bi 2 Sr 2–x La x CuO 6+δ (Bi2201) superconductors. Unexpected hybridization between the main band and the superstructure band in Bi2212 is clearly revealed. In the momentum space where one main Fermi surface intersects with one superstructure Fermi surface, four bands are observed instead of two. The hybridization exists in both the superconducting state and the normal state, and in Bi2212 samples with different doping levels. Such a hybridization is not observed in Bi2201. This phenomenon can be understood by considering the bilayer splitting in Bi2212, the selective hybridization of two bands with peculiar combinations, and the altered matrix element effects of the hybridized bands. These observations indicate that the origin of the superstructure bands is intrinsic to the CuO 2 planes. Furthermore, understanding physical properties and superconductivity in Bi2212 should consider the complete Fermi surface topology which involves the main bands, the superstructure bands, and their interactions.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2016

Physical properties of the Ce 2 M Al 7 Ge 4 heavy-fermion compounds ( M = Co , Ir , Ni , Pd )

Here, we report the synthesis, crystal structure, and characterization by means of single-crystal x-ray diffraction, neutron powder diffraction, and magnetic, thermal, and transport measurements of the new heavy-fermion compounds Ce 2 MAl 7 Ge 4 (M=Co,Ir,Ni,Pd). These compounds crystallize in a noncentrosymmetric tetragonal space group P$\bar{4}$2 1 m, consisting of layers of square nets of Ce atoms separated by Ge-Al and M-Al-Ge blocks. Ce 2 CoAl 7 Ge 4 ,Ce 2 IrAl 7 Ge 4 , and Ce 2 NiAl 7 Ge 4 order magnetically below TM=1.8, 1.6, and 0.8 K, respectively. There is no evidence of magnetic ordering in Ce 2 PdAl 7 Ge 4 down to 0.4 K. Furthermore, the small amount of entropy released in the magnetic state of Ce 2 MAl 7 Ge 4 (M = Co, Ir, Ni) and the reduced specific heat jump at T M suggest a strong Kondo interaction in these materials. Ce 2 PdAl 7 Ge 4 shows non-Fermi liquid behavior, possibly due to the presence of a nearby quantum critical point.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2011

Constraints on light WIMP candidates from the isotropic diffuse gamma-ray emission

Motivated by the measurements reported by direct detection experiments, most notably DAMA, CDMS-II, CoGeNT and Xenon10/100, we study further the constraints that might be set on some light dark matter candidates, M{sub DM} ∼ few GeV, using the Fermi-LAT data on the isotropic gamma-ray diffuse emission. In particular, we consider a Dirac fermion singlet interacting through a new Z' gauge boson, and a scalar singlet S interacting through the Higgs portal. Both candidates are WIMP (Weakly Interacting Massive Particles), i.e. they have an annihilation cross-section in the pbarn range. Also they may both have a spin-independent elastic cross section on nucleons in the range required by direct detection experiments. Although being generic WIMP candidates, because they have different interactions with Standard Model particles, their phenomenology regarding the isotropic diffuse gamma-ray emission is quite distinct. In the case of the scalar singlet, the one-to-one correspondence between its annihilation cross-section and its spin-independent elastic scattering cross-section permits to express the constraints from the Fermi-LAT data in the direct detection exclusion plot, σ{sub n}{sup 0}−M{sub DM}. Depending on the astrophysics, we argue that it is possible to exclude the singlet scalar dark matter candidate at 95% confidence level. The constraints on the Dirac singlet interacting through a Z' are comparatively weaker.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2024

Controlling 4 f antiferromagnetic dynamics via itinerant electronic susceptibility

Optical manipulation of magnetism holds promise for future ultrafast spintronics, especially with lanthanides and their huge, localized 4 f magnetic moments. These moments interact indirectly by spin polarizing the conduction electrons (the Ruderman-Kittel-Kasuya-Yosida exchange interaction), influenced by interatomic orbital overlap, and the conduction electron's susceptibility around the Fermi level. Here, we study this influence in a series of 4 f antiferromagnets, Gd T 2 Si 2 ( T = Co, Rh, Ir), using ultrafast resonant x-ray diffraction. We observe a twofold increase in the ultrafast intersublattice angular momentum transfer rate between the materials, originating from modifications in the conduction electron susceptibility, as confirmed by first-principles calculations. Published by the American Physical Society 2024

36 MATERIALS SCIENCE↗
DOE OSTI2015

Quantum-mechanical approach to predissociation of water dimers in the vibrational adiabatic representation: Importance of channel interactions

The results of application of the quantum-mechanical adiabatic theory to vibrational predissociation (VPD) of water dimers, (H{sub 2}O){sub 2} and (D{sub 2}O){sub 2}, are presented. We consider the VPD processes including the totally symmetric OH mode of the dimer and the bending mode of the fragment. The VPD in the adiabatic representation is induced by breakdown of the vibrational adiabatic approximation, and two types of nonadiabatic coupling matrix elements are involved: one provides the VPD induced by the low-frequency dissociation mode and the other provides the VPD through channel interactions induced by the low-frequency modes. The VPD rate constants were calculated using the Fermi golden rule expression. A closed form for the nonadiabatic transition matrix element between the discrete and continuum states was derived in the Morse potential model. All of the parameters used were obtained from the potential surfaces of the water dimers, which were calculated by the density functional theory procedures. The VPD rate constants for the two processes were calculated in the non-Condon scheme beyond the so-called Condon approximation. The channel interactions in and between the initial and final states were taken into account, and those are found to increase the VPD rates by 3(1) orders of magnitude for the VPD processes in (H{sub 2}O){sub 2} ((D{sub 2}O){sub 2}). The fraction of the bending-excited donor fragments is larger than that of the bending-excited acceptor fragments. The results obtained by quantum-mechanical approach are compared with both experimental and quasi-classical trajectory calculation results.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2011

Renormalization group approach to spinor Bose-Fermi mixtures in a shallow optical lattice

We study a mixture of ultracold spin-half fermionic and spin-one bosonic atoms in a shallow optical lattice where the bosons are coupled to the fermions via both density-density and spin-spin interactions. We consider the parameter regime where the bosons are in a superfluid ground state, integrate them out, and obtain an effective action for the fermions. We carry out a renormalization group analysis of this effective fermionic action at low temperatures, show that the presence of the spinor bosons may lead to a separation of Fermi surfaces of the spin-up and spin-down fermions, and investigate the parameter range where this phenomenon occurs. We also calculate the susceptibilities corresponding to the possible superfluid instabilities of the fermions and obtain their possible broken-symmetry ground states at low temperatures and weak interactions.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2021

Collective states and charge density waves in the group IV transition metal trichalcogenides

It has been nearly a century since the original mechanism for charge density wave (CDW) formation was suggested by Peierls. Since then, the term has come to describe several related concepts in condensed matter physics, having their origin in either the electron–phonon or electron–electron interaction. The vast majority of CDW literature deals with systems that are metallic, where discussions of mechanisms related to the Fermi surface are valid. Recently, it has been suggested that semiconducting systems such as TiS 3 and TiSe 2 exhibit behavior related to CDWs. In such cases, the origin of the behavior is more subtle and intimately tied to electron–electron interactions. We introduce the different classifications of CDW systems that have been proposed and discuss work on the group IV transition metal trichalcogenides (TMTs) (ZrTe 3 , HfTe 3 , TiTe 3 , and TiS 3 ), which are an exciting and emergent material system whose members exhibit quasi-one-dimensional properties. TMTs are van der Waals materials and can be readily studied in the few-layer limit, opening new avenues to manipulating collective states. We emphasize the semiconducting compound TiS 3 and suggest how it can be classified based on available data. Although we can conjecture on the origin of the CDW in TiS 3 , further measurements are required to properly characterize it.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗