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At least 649 records · Page 36

All sources NASA NTRS DOE OSTI

DOE OSTI2014

Point defect weakened thermal contraction in monolayer graphene

We investigate the thermal expansion behaviors of monolayer graphene and three configurations of graphene with point defects, namely the replacement of one carbon atom with a boron or nitrogen atom, or of two neighboring carbon atoms by boron-nitrogen atoms, based on calculations using first-principles density functional theory. It is found that the thermal contraction of monolayer graphene is significantly decreased by point defects. Moreover, the corresponding temperature for negative linear thermal expansion coefficient with the maximum absolute value is reduced. The cause is determined to be point defects that enhance the mechanical strength of graphene and then reduce the amplitude and phonon frequency of the out-of-plane acoustic vibration mode. Such defect weakening of graphene thermal contraction will be useful in nanotechnology to diminish the mismatching or strain between the graphene and its substrate.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

DOE OSTI2013

Ultrafast spectroscopy of super high frequency mechanical modes of doubly clamped beams

We use ultrafast pump-probe spectroscopy to study the mechanical vibrations in the time domain of doubly clamped silicon nitride beams. Beams with two different clamping conditions are investigated. Finite element method calculations are performed to analyse the mode spectra of both structures. By calculating the strain integral on the surface of the resonators, we are able to reproduce the effect of the detection mechanism and identify all the measured modes. We show that our spectroscopy technique combined with our modelling tools allow the investigation of several different modes in the super high frequency range (3-30 GHz) and above, bringing more information about the vibration modes of nanomechanical resonators.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

DOE OSTI2025

North Pacific meridional mode has larger impacts on El Niño evolution than the March Madden-Julian Oscillation

The El Niño–Southern Oscillation (ENSO) is a key driver of global climate variability. Early-season westerly wind bursts (WWBs) have long been suggested to be important for ENSO evolution and diversity, with the Madden-Julian Oscillation (MJO) among the main sources of WWBs. However, MJO’s contribution to ENSO evolution has been difficult to quantify. Here, using an ensemble hindcast approach specifically designed to isolate internal atmospheric variability, we evaluate the influences of March MJO on subsequent ENSO development. Our results show that the March MJO, under favorable background conditions, by itself has limited impacts on ENSO due to weak equatorial air-sea coupling in spring. In comparison, the North Pacific Oscillation–induced meridional mode exerts a more sustained influence on ENSO evolution. A cyclonic circulation anomaly over Hawaii, associated with the Pacific-North American pattern, also plays a role. These findings suggest that March MJO activity alone may not be a reliable predictor for ENSO evolution, but underscore the importance of North Pacific atmospheric variability.

Science & Technology - Other Topics↗

NASA NTRS1985

Coupled-mode analysis of gain and wavelength oscillation characteristics of diode laser phased arrays

The lasing wavelengths and gain characteristics of the modes of phase-locked arrays of channel-substrate-planar (CSP) lasers are presented. The gain values for the array modes are determined from complex coupling coefficients calculated using the fields of neighboring elements of the array. The computations show that, for index guided lasers which have nearly planar phase fronts, the highest order array mode will be preferred. The 'in-phase' or fundamental mode, which produces only one major lobe in the far-field radiation pattern, has the lowest modal gain of all array modes. The modal gain differential between the highest order and fundamental modes is less than 10/cm for weak coupling between the elements.

Butler, J. K.↗

DOE OSTI2016

Theoretical study of NMR, infrared and Raman spectra on triple-decker phthalocyanines

Electronic structures and magnetic properties of multi-decker phthalocyanines were studied by theoretical calculation. Electronic structures, excited processes at multi-states, isotropic chemical shifts of {sup 13}C, {sup 14}N and {sup 1}H-nuclear magnetic resonance (NMR), principle V-tensor in electronic field gradient (EFG) tensor and asymmetry parameters (η), vibration mode in infrared (IR) and Raman spectra of triple-decker phthalocyanines were calculated by density functional theory (DFT) and time-dependent DFT using B3LYP as basis function. Electron density distribution was delocalized on the phthalocyanine rings with electron static potential. Considerable separation of chemical shifts in {sup 13}C, {sup 14}N and {sup 1}H-NMR was originated from nuclear spin interaction between nitrogen and carbon atoms, nuclear quadrupole interaction based on EFG and η of central metal under crystal field. Calculated optical absorption at multi-excited process was derived from overlapping π-orbital on the phthalocyanine rings. The vibration modes in IR and Raman spectra were based on in-plane deformation and stretching vibrations of metal-ligand coordination bond on the deformed structure.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

DOE OSTI2012

Surveillance and diagnostics of the beam mode vibrations of the Ringhals PWRs

Surveillance of core barrel vibrations has been performed in the Swedish Ringhals PWRs for several years. This surveillance is focused mainly on the pendular motion of the core barrel, which is known as the beam mode. The monitoring of the beam mode has suggested that its amplitude increases along the cycle and decreases after refuelling. In the last 5 years several measurements have been taken in order to understand this behaviour. Besides, a non-linear fitting procedure has been implemented in order to better distinguish the different components of vibration. By using this fitting procedure, two modes of vibration have been identified in the frequency range of the beam mode. Several results coming from the trend analysis performed during these years indicate that one of the modes is due to the core barrel motion itself and the other is due to the individual flow induced vibrations of the fuel elements. In this work, the latest results of this monitoring are presented. (authors)

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

NASA NTRS2002

A Solar Model with g-Modes

Good evidence is assembled showing that the Suit's core arid surface vary on time scales from a month to a decade arid that a number of scales are similar. The most plausible source for numerous long time scales and periodicities is long-lived global oscillations. This suggests g-modes (oscillations restored mainly by buoyancy) because they particularly affect the core and base of the convective envelope, which then indirectly modulates the surface. Also, standing g-modes have rotational properties that match many observed periodicities. But the standard solar model (SSM) has a static core and excites few if any g-modes. making new interior structures worth exploring. The model outlined here assumes two well mixed shells near 0.18 and 0.68 R, (13 = solar radius) where sound speed data shows sharp deviations from the SSM. Mixing is sustained by flows driven by the oscillations. The shells form a cavity that excludes g-modes from their main damping region below 0.1 R, assisting their net excitation and increasing their oscillation periods by at least a factor of two and probably much more. In terms of the solar luminosity L, the modes transport up through the cavity a power approx. 0.004 L as a lower limit and 0.11 L as all upper limit. The modes dissipate energy in the outer shell and cool the inner shell, asymmetrically in each case, and this stimulates occasional convective events whose response time is typically 0.8 years longer near the inner shell. Such events cool the core and reduce neutrino flux while heating the envelope and increasing solar activity. This gives a physical basis for a well mixed Sun with low neutrino flux and basis for the observed anticorrelation and lag of neutrino behind surface activity.

Wolff, Charles L.↗

DOE OSTI2016

Theoretical investigation of the dielectric-filled relativistic magnetron

The fundamental mode frequency of a dielectric-filled relativistic magnetron is studied theoretically by the method of the equivalent circuit, and an exact fundamental mode frequency formula is derived. To prove the validity of the theoretical formula, simulation investigation is performed. The simulation results agree well with the theoretical formula, and the relative error does not exceed 3%. The comparative results verify the creditability of the theoretical formula.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

DOE OSTI2011

System studies of rf current drive for MST

Two rf schemes are being studied on the MST reversed field pinch for their potential in current profile control experiments. MHD modeling has shown that a substantial externally-driven off axis parallel current can improve stability of the dominant core tearing modes. A radially localized axisymmetric population of fast electrons has been observed by SXR emission during LH injection (100kW at 800MHz), and is consistent with CQL3D modeling which predicts a small driven current. Computational work suggests that doubling the input power will statistically improve the LH-induced SXR signal to background ratio, and that about 2MW of injected power (an order of magnitude increase) will drive enough current for stabilization of tearing modes. Additionally, a 1 MW 5.5 GHz electron Bernstein wave (EBW) experiment is under construction, which utilizes a very simple and compact antenna compatible with the demands of the RFP. EBW allows access to electron cyclotron heating and current drive in the overdense plasma. Coupling of the external electromagnetic wave to the EBW has been demonstrated, and initial tests at {approx}100kW power have produced a small, localized xray flux consistent with rf heating and high diffusivity of fast electrons. Computational work is currently underway to answer the very important questions of how much power is required, and what level of electron diffusivity is tolerable, to generate a consequential amount of EBW current.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

DOE OSTI2011

Electron Bernstein Wave Studies in MST

The overdense plasma in an RFP prevents electromagnetic waves from propagating past the edge, however use of the electron Bernstein wave (EBW) has the potential to heat and drive current in the plasma. MHD simulations have demonstrated that resistive tearing mode stability is very sensitive to gradients in the edge current density profile allowing EBW to potentially be a stabilizing influence. A new MW level experiment is being commissioned on MST to evaluate the potential use of the EBW for current profile control on the RFP. The development of new equipment includes a 5.5 GHz klystron driven by a novel switchmode power supply. A quartz window has been constructed and coupling with a cylindrical molybdenum wave guide antenna has been studied. Due to the steep edge density gradient in the RFP, it is possible to efficiently couple to the EBW with O or X mode launch. The EBW is strongly damped at the electron cyclotron resonance where it couples to the electron gyromotion and alters the electron distribution. Either Fisch-Boozer or Ohkawa current drive mechanisms can be activated to drive off axis current in the plasma. Preliminary experiments have been performed to verify high power coupling and understand heating via observed x-ray emission when compared to Fokker-Plank modeling in CQL3D.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

DOE OSTI2016

Tripartite entanglement dynamics of vibrations in triatomic molecules

In the present study, the dynamical behaviors of tripartite entanglement of vibrations in triatomic molecules are studied based on the Lie algebraic models of molecules. The dynamical behaviors of tripartite entanglement of the local mode molecule H{sub 2}O and normal mode molecule NO{sub 2} are comparatively studied for different initial states by employing the general concurrence. Our results show that the dynamics of tripartite entanglement are relied on the dynamics of intramolecular energy distribution. The local mode molecule is more suitable to construct the tripartite entangled states. Also, the greater degree of tripartite entanglement can be obtained if the stretching vibration is first excited. These results shed new light on the understanding of quantum multipartite entanglement of vibrations in the polyatomic molecules.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

DOE OSTI2011

Production of High Energy Tail Electrons by Electron Bernstein Waves during the Current Start-up Discharges in the LATE Device

Toroidal plasma current is started and ramped up by injecting microwave power in the electron cyclotron range of frequency without induction in the LATE device. Radial scanning with hard X-ray pulse height analysis reveals the production of high energy electrons with average energy {approx}100 keV in the radial region from R = 28 cm to 40.5 cm, which are heated by electron Bernstein wave. The radial profile of photon counts in the energy range from 25 to 200 keV is very similar to that of perpendicular pressure obtained by magnetic measurement and equilibrium analysis, suggesting that a significant portion of trapped electrons exists outside the last closed flux surface. The plasma current inside the LCFS is carried mainly by passing electrons, while some portion of the outside current may be generated as a result of the toroidal precession of trapped electrons.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

DOE OSTI2018

Investigation on Vibration Response of Aluminum Foam Beams Using Speckle Interferometry

This paper firstly presents a brief review on the representations of speckle fringe pattern in vibration measurement using time-averaged electronic speckle pattern interference (ESPI) method. Based on laser phase noise, a new representation of speckle fringe intensity generated by real-time subtraction ESPI method for vibrating measurement is then proposed. In the experimental performance, the real-time subtraction ESPI method is employed to inspect the vibrating response of a closed-cell aluminum foam cantilever beam. In contract with the results of the finite elemental method simulation, the vibration mode shapes obtained by the ESPI method are well agreed with numerical prediction. The optical vibration analysis is also carried out to determine the effective Young’s modulus of aluminum foam, and the results verify the validation of the ESPI method for investigation on mechanical properties of metal foam materials.

36 MATERIALS SCIENCE↗

DOE OSTI2013

Vibration responses of h-BN sheet to charge doping and external strain

Based on density functional theory and density functional perturbation theory calculations, we systematically investigate the vibration responses of h-BN sheet to charge doping and external strains. It is found that under hole doping, the phonon frequencies of the ZO and TO branches at different wave vector q shift linearly with different slopes. Under electron doping, although the phonon frequencies shift irregularly, the shifting values are different at different phonon wave vectors. Interestingly, we find that external strain can restrain the irregular vibration responses of h-BN sheet to electron doping. The critical factor is revealed to be the relative position of the nearly free electron and boron p{sub z} states of h-BN sheet. Under external strains, the vibration responses of h-BN sheet are also found to be highly dependent on the phonon branches. Different vibration modes at different q points are revealed to be responsible for the vibration responses of h-BN sheet to charge doping and external strain. Our results point out a new way to detect the doping or strain status of h-BN sheet by measuring the vibration frequencies at different wave vector.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

DOE OSTI2016

Novel phosphate halides BaMn{sup III}[PO{sub 4}]FCl and BaMn{sup III}[PO{sub 4}]F{sub 2}: Effects of mixed halides on crystal structures and magnetic properties

Two new phosphate halides BaMn{sup III}[PO{sub 4}]FCl (1) and BaMn{sup III}[PO{sub 4}]F{sub 2} (2), have been synthesized under hydrothermal conditions. Structural characterizations show that both new compounds adopt layered structures but with different polyhedral linkages. Introduction of Cl into Compound (1) results in isolated hemimorphic [MnO{sub 4}FCl] octahedra, different from the chain of [MnO{sub 4}F{sub 2}]/[MnO{sub 2}F{sub 4}] octahedra in Compound (2). These compounds have significantly different molecular vibration modes and thermal stabilities. Magnetic measurements reveal that Compound (2) has larger antiferromagnetic interactions than Compound (1), because the former has strong interactions between Mn{sup 3+}-Mn{sup 3+} ions within corner-shared Mn{sup 3+}-octahedral chains whereas the latter only possesses isolated Mn{sup 3+}-octahedra. Both compounds transform to a new orthorhombic compound BaMn{sup II}(PO{sub 4})F (3) after thermal decomposition. - Graphical abstract: The large radius of Cl{sup -} ions makesBaMn{sup III}[PO{sub 4}]FCl to adopt isolated [MnO{sub 4}FCl] rather than corner-sharing octahedra as observed in BaMn{sup III}[PO{sub 4}]F{sub 2}. - Highlights: • Two novel phosphate halides BaMn[PO{sub 4}]FCl and BaMn[PO{sub 4}]F{sub 2} have been prepared. • These new compounds adopt different types of layered structures. • They have different molecular vibration modes and thermal stabilities. • BaMn[PO{sub 4}]FCl has weaker antiferromagnetic interactions than BaMn[PO{sub 4}]F{sub 2}. • The former adopts isolated octahedra whereas the latter adopts octahedral chains.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

DOE OSTI2017

Optimisation of the prism coupling of optical whispering-gallery-mode microcavities

The methods for increasing the coupling efficiency of a prism with spheroidal microcavities, aimed at exciting whispering-gallery modes, have been analytically investigated. Optimal angles of incidence and incident beam parameters are obtained for a spheroidal cavity. The cavity eigenfrequency shift caused by the presence of a prism and the introduced loss by it is calculated. (resonators)

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

DOE OSTI2014

Selective coherent perfect absorption in metamaterials

We show multi-band coherent perfect absorption (CPA) in simple bilayered asymmetrically split ring metamaterials. The selectivity of absorption can be accomplished by separately excited electric and magnetic modes in a standing wave formed by two coherent counterpropagating beams. In particular, each CPA can be completely switched on/off by the phase of a second coherent wave. We propose a practical scheme for realizing multi-band coherent perfect absorption of 100% that is allowed to work from microwave to optical frequency.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

DOE OSTI2012

Superimposed coherent terahertz wave radiation from mono-energetically bunched multi-beam

Intense coherent radiation is obtained from multiple electron beams monochromatically bunched over the wide higher-order-mode (HOM) spectral band in the THz regime. The overmoded waveguide corrugated by dielectric-implanted staggered gratings superimposes evanescent waves emitted from the low energy electron beams. The dispersion and transmission simulations of the three-beam slow wave structure show that the first two fundamental modes ($TE_{10}$ and $TE_{20}$) are considerably suppressed ($\sim-50$ dB) below the multi-beam resonating mode ($TE_{30}$) at the THz regime (0.8–1.24 THz). The theoretical calculations and particle-in-cell simulations show that with significantly higher interaction impedance and power growth rate radiation of the $TE_{30}$ mode is $\sim$23 dBm and $\sim$50 dBm stronger than the $TE_{10}$ and $TE_{20}$ modes around 1 THz, respectively. As a result, this highly selective HOM multi-beam interaction has potential applications for power THz sources and high intensity accelerators.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗