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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 649 records · Page 36

Analysis of loss-of-coolant accident for a fast-spectrum lithium-cooled nuclear reactor for space-power applications

A two-dimensional, transient, heat-transfer analysis was made to determine the temperature response in the core of a conceptual space-power nuclear reactor following a total loss of reactor coolant. With loss of coolant from the reactor, the controlling mode of heat transfer is thermal radiation. In one of the schemes considered for removing decay heat from the core, it was assumed that the 4 pi shield which surrounds the core acts as a constant-temperature sink (temperature, 700 K) for absorption of thermal radiation from the core. Results based on this scheme of heat removal show that melting of fuel in the core is possible only when the emissivity of the heat-radiating surfaces in the core is less than about 0.40. In another scheme for removing the afterheat, the core centerline fuel pin was replaced by a redundant, constant temperature, coolant channel. Based on an emissivity of 0.20 for all material surfaces in the core, the calculated maximum fuel temperature for this scheme of heat removal was 2840 K, or about 90 K less than the melting temperature of the UN fuel.

Turney, G. E.↗

Revisiting the Optical Spectrum of the Plutonyl Ion (PuO 2 ) 2+ in 1 M HClO 4

The analysis of the solution absorption spectrum of the plutonyl ion in an aqueous environment was given by Eisenstein and Pryce (E&P) in 1968. In 2011 a new spectrum was published of the (PuO 2 ) 2+ ion in 1 M HClO 4 . We have been provided with the original data of this spectrum and have found in the data a previously unreported low-lying transition at 7385 cm –1 which we have assigned as a magnetic dipole transition. We have fit most of the near-infrared and optical transitions with Gaussian fits and tabulated a new energy level list up to 22,000 cm –1 which mostly agrees with the data of E&P. We assumed a crystal field of D ∞h (only axial symmetry) and utilized the intensity calculations published for the isoelectronic (NpO 2 ) 1+ ion using a complete basis set for the 5f 2 problem including the Coulombic, spin–orbit as well as the crystal field Hamiltonian. Our results differ substantially from those of E&P. Subsequently, we used a truncated Hamiltonian to try to establish the effects of assuming the σ antibonding orbitals are at such high energies that we can ignore their contributions to the lower lying φ and δ orbitals.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

A Review of the Lawrence Livermore Nuclear Accident Dosimeter 1980s-present

A Nuclear Accident Dosimetry program is a federal requirement for all facilities that have the potential to have a criticality accident. Personnel Nuclear Accident Dosimeter (PNAD) theory and analytical procedures are driven by various scientific needs and interacting regulations. A brief history of the status of USA Department of Energy (DOE) nuclear accident dosimetry regulations, recommendations, and performance testing criteria are given. Then, the history of the Lawrence Livermore National Laboratory (LLNL) PNAD is explored, including changes in the physical dosimeter and adjustments of the analysis method through the last four decades. Finally, the performance of LLNL’s PNAD at criticality accident intercomparison training exercises since 2009 is explored. In general, reported neutron doses have been within or close to DOE-STD-1098 performance criteria while reported gamma doses have been outside of DOE-STD-1098 performance criteria. Reported total absorbed doses have varied in meeting ANSI/HPS N13.3 and ANSI/HPS N13.3 (R2019) performance criteria. Dosimetry staff retirement and turnover have left historical knowledge gaps, yet provided opportunities within the NAD program at LLNL. This review paper serves as an overview of the history and status of the NAD program. Brief technical, procedural and programmatic recommendations to improve LLNL’s NAD program are given. Technical recommendations include investigating orientation factors through modeling or empirical experimentation, investigating gamma dosimetry methods for high-dose scenarios, and exploring other dosimetric methods for simpler, quicker NAD analysis. Procedural recommendations include better documentation of conversion factor (activity-to-fluence and fluence-to-dose) derivations and spectrum uses, and updated analysis spreadsheets or simple Graphic User Interfaces for dose calculations. In conclusion, programmatic recommendations include formalized training for NAD analysts, and having multiple SMEs trained on the NAD program.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Multimodal X-ray nano-spectromicroscopy analysis of chemically heterogeneous systems

Abstract Understanding the nanoscale chemical speciation of heterogeneous systems in their native environment is critical for several disciplines such as life and environmental sciences, biogeochemistry, and materials science. Synchrotron-based X-ray spectromicroscopy tools are widely used to understand the chemistry and morphology of complex material systems owing to their high penetration depth and sensitivity. The multidimensional (4D+) structure of spectromicroscopy data poses visualization and data-reduction challenges. This paper reports the strategies for the visualization and analysis of spectromicroscopy data. We created a new graphical user interface and data analysis platform named XMIDAS (X-ray multimodal image data analysis software) to visualize spectromicroscopy data from both image and spectrum representations. The interactive data analysis toolkit combined conventional analysis methods with well-established machine learning classification algorithms (e.g. nonnegative matrix factorization) for data reduction. The data visualization and analysis methodologies were then defined and optimized using a model particle aggregate with known chemical composition. Nanoprobe-based X-ray fluorescence (nano-XRF) and X-ray absorption near edge structure (nano-XANES) spectromicroscopy techniques were used to probe elemental and chemical state information of the aggregate sample. We illustrated the complete chemical speciation methodology of the model particle by using XMIDAS. Next, we demonstrated the application of this approach in detecting and characterizing nanoparticles associated with alveolar macrophages. Our multimodal approach combining nano-XRF, nano-XANES, and differential phase-contrast imaging efficiently visualizes the chemistry of localized nanostructure with the morphology. We believe that the optimized data-reduction strategies and tool development will facilitate the analysis of complex biological and environmental samples using X-ray spectromicroscopy techniques.

36 MATERIALS SCIENCE↗

The completed SDSS-IV extended Baryon Oscillation Spectroscopic Survey: BAO and RSD measurements from the anisotropic power spectrum of the quasar sample between redshift 0.8 and 2.2

ABSTRACT We measure the clustering of quasars of the final data release (DR16) of eBOSS. The sample contains $343\, 708$ quasars between redshifts 0.8 ≤ z ≤ 2.2 over $4699\, \mathrm{deg}^2$. We calculate the Legendre multipoles (0,2,4) of the anisotropic power spectrum and perform a BAO and a Full-Shape (FS) analysis at the effective redshift zeff = 1.480. The errors include systematic errors that amount to 1/3 of the statistical error. The systematic errors comprise a modelling part studied using a blind N-body mock challenge and observational effects studied with approximate mocks to account for various types of redshift smearing and fibre collisions. For the BAO analysis, we measure the transverse comoving distance DM(zeff)/rdrag = 30.60 ± 0.90 and the Hubble distance DH(zeff)/rdrag = 13.34 ± 0.60. This agrees with the configuration space analysis, and the consensus yields: DM(zeff)/rdrag = 30.69 ± 0.80 and DH(zeff)/rdrag = 13.26 ± 0.55. In the FS analysis, we fit the power spectrum using a model based on Regularised Perturbation Theory, which includes redshift space distortions and the Alcock–Paczynski effect. The results are DM(zeff)/rdrag = 30.68 ± 0.90 and DH(zeff)/rdrag = 13.52 ± 0.51 and we constrain the linear growth rate of structure f(zeff)σ8(zeff) = 0.476 ± 0.047. Our results agree with the configuration space analysis. The consensus analysis of the eBOSS quasar sample yields: DM(zeff)/rdrag = 30.21 ± 0.79, DH(zeff)/rdrag = 3.23 ± 0.47, and f(zeff)σ8(zeff) = 0.462 ± 0.045 and is consistent with a flat ΛCDM cosmological model using Planck results.

Neveux, Richard↗

The Spectrum Orbit Utilization Program (SOUP) used for DBS plan analysis at RARC '83

This paper describes the history, functions, and usage of the program that was used to analyze the plans for direct broadcast satellite service developed in the course of the 1983 Regional Administrative Radio Conference for ITU Region 2. Given the requirements for direct broadcast service by the administrations, the conference delegates (1) developed the appropriate technical parameters; (2) made tentative assignments to the orbit locations, frequencies, and polarizations of space stations, (3) calculated the interferences and margins of such assignments through the use of the Spectrum Orbit Utilization Program (SOUP); and (4) iterated this procedure until an acceptable plan was found.

Davidson, J.↗

Rossi-alpha Analysis of CURIE Experiment [Slides]

Critical assembly measurement and operations are crucial to the development of benchmark data. Knowledge of the prompt neutron lifetime informs on the state of the system’s neutron spectrum. Rossi-alpha analysis can give us time-dependent information on the system. Teflon was selected, via genetic algorithm, as a moderator to target the URR in uranium for CURIE. Rossi-alpha measurements of the assembly's approach to critical using He-3 detectors estimated the prompt neutron decay constant (α) at delayed critical. α values of several subcritical measurements were then used to predict the α value at delayed critical.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Analysis of radiative sources with both specular and diffuse characteristics in the visible and infrared spectrum

The application of analytical concepts developed to facilitate the design and analysis of the thermal simulator for the Apollo Soyuz docking module is discussed. The functions used to mathematically formulate the irradiance from a quartzline lamp and reflector are described with examples of applications to other geometries. General information is denoted for utilization of the functions in computer programs with approximate computer storage and statement requirements.

Williams, F. U.↗

Quantifying Polaron Mole Fractions and Interpreting Spectral Changes in Molecularly Doped Conjugated Polymers

Molecular doping of conjugated polymers causes bleaching of the neutral absorbance and results in new polaron absorbance transitions in the mid and near infrared. In this report the concentration dependent changes in the spectra for a series of molecularly doped diketopyrrolopyrrole (DPP) co-polymers with a series of ultra-high electron affinity cyanotrimethylenecyclopropane-based dopants is analyzed. With these strong dopants the polaron mole fraction (Θ) reaches saturation. Analysis of the full spectrum enables separation of neutral and polaron signals and quantification of the polaron mole fraction using a simple noninteracting site model. The peak ratios for both neutral and polaron peaks change systematically with increasing polaron mole fraction for all measured polymers. Analysis of the spectral changes indicates that the polaron mole fraction can be quantified to within 5%. While the total change in the absorbance spectrum with increasing polaron mole fraction is linear, the lowest energy polaron peak (P1) grows nonlinearly, which indicates increased polarization/delocalization. Molecular doping of polymers that form either H- or J-aggregates shows systematically different spectral changes in the vibronic peak ratios of the neutral spectra and provides insights into the polymer configuration at undoped sites in the film.

36 MATERIALS SCIENCE↗

Analysis of Radiological Release From Fueled Irradiation Experiments During Manual Handling (Slides)

Irradiation experiments are manually handled at the Advanced Test Reactor (ATR) by qualified operators using long handled tools. Standard handling evolutions include insertion and removal from the reactor vessel, transfer to/from a storage location or cask in the ATR canal, and handling/reconfigurations at a canal working tray. Such routine handling has the potential to result in mechanical damage to the experiment boundary which is credited to retain fission products. Since damage can occur due to operator error, this is an anticipated occurrence. This work determines the radiological consequences to receptors inside the ATR facility, as well as public receptors. Given the wide variety of fuel types tested at the ATR, a generic approach to the analysis is taken. The radiological inventory is determined to bound a variety of fuel types (e.g., ceramic and molten fuel matrices) and fission powers on the U-235 enrichment spectrum. The source term analysis considers different release fractions to bound different fuel types and burnups. The postulated handling events occur underwater; thus, retention of the released isotopic content is considered within the canal water column. Retention of radionuclides in the water column is determined using a modified approach of United States (US) Nuclear Regulatory Commission (NRC) Regulatory Guide (RG) 1.183. Radiological dose to the facility receptor is determined using a compartment release model. Dose to the public receptor is determined using atmospheric dispersion models using site specific atmospheric conditions with the use of the Radiological Safety Analysis Computer (RSAC) program version 7.2.

21 - SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLAN↗

Analysis of the time-of-flight neutron scattering cross-section data for light water measured at the SEQUOIA spectrometer, Spallation Neutron Source (SNS)

Thermal neutron scattering cross-section data for light water available in the major nuclear data libraries observes significant differences especially at reactor operating temperatures. During the past few years there has been a renewed interest in reviewing the existing thermal scattering models and generating more accurate and reliable thermal scattering cross sections using existing experimental data and in some cases based on Molecular Dynamics (MD) simulations. There is a need for performing new time-of-flight experiments at high temperatures and pressures, to have a better understanding of the physics involved in the scattering process that could help improve the existing TSL data.Lack of experimental thermal scattering data for light water at high temperatures led to a new measurement campaign within the INSIDER project at the Institut de radioprotection et de sûreté nucléaire (IRSN). Double differential scattering cross section for light water have been measured at the SEQUOIA spectrometer based at the Spallation Neutron Source (SNS), Oak Ridge National Laboratory, United States. Several measurements have been carried out at different temperatures and pressures corresponding to liquid light water. Measurements at five different incident neutron energies Ei (8, 60, 160, 280 and 800 meV) have been carried out to help exploring different regions of the frequency spectrum. This paper presents the analysis of the dynamic structure factor and the derived frequency spectrum of light water. The analysis of the experimental data would provide one with better confidence, the behavior of thermal scattering cross sections for light water at high temperatures, knowledge of which is very important for the design of novel reactors as well as existing pressurized water reactors.

Jaiswal, V↗

Failure analysis of a cooling pump using modal and vibration analysis

Four pumps redundantly supply cooling water to a system. All four pumps underwent maintenance during a recently scheduled downtime. During preliminary evaluation following maintenance, one pump, the subject of this document, exhibited higher vibration levels compared to the other three pumps. The pump underwent further performance testing to rule out potential damage resulting from the higher vibration. Vibration analysis and modal analysis including steady state spectrum, operational deflection shape, run up transients, and modal impact have been utilized to identify dynamic characteristics that could contribute to the increased vibration levels. This article will cover the testing setup, methodology, analysis results, and recommendations.

42 ENGINEERING↗

Constraining the baryonic feedback with cosmic shear using the DES Year-3 small-scale measurements

ABSTRACT We use the small scales of the Dark Energy Survey (DES) Year-3 cosmic shear measurements, which are excluded from the DES Year-3 cosmological analysis, to constrain the baryonic feedback. To model the baryonic feedback, we adopt a baryonic correction model and use the numerical package baccoemu to accelerate the evaluation of the baryonic non-linear matter power spectrum. We design our analysis pipeline to focus on the constraints of the baryonic suppression effects, utilizing the implication given by a principal component analysis on the Fisher forecasts. Our constraint on the baryonic effects can then be used to better model and ameliorate the effects of baryons in producing cosmological constraints from the next-generation large-scale structure surveys. We detect the baryonic suppression on the cosmic shear measurements with a ∼2σ significance. The characteristic halo mass for which half of the gas is ejected by baryonic feedback is constrained to be $M_c \gt 10^{13.2} \, h^{-1} \, \mathrm{M}_{\odot }$ (95 per cent C.L.). The best-fitting baryonic suppression is $\sim 5{{\ \rm per\ cent}}$ at $k=1.0 \, {\rm Mpc}\ h^{-1}$ and $\sim 15{{\ \rm per\ cent}}$ at $k=5.0 \, {\rm Mpc} \ h^{-1}$. Our findings are robust with respect to the assumptions about the cosmological parameters, specifics of the baryonic model, and intrinsic alignments.

79 ASTRONOMY AND ASTROPHYSICS↗

Raman scattering in the Jovian atmosphere

On December 8 and 9, 1976, the 1024 channel Reticon silicon photodiode array detector in the coude spectrograph of a 2.7 m telescope was used to obtain spectra of Jupiter and the moon. Three separate data sets were obtained, including one of the Jovian equatorial region, one of the Jovian north polar cap, and one of Mare Serenetatis on the moon. A correlation analysis was conducted. The autocorrelation function of the Jovian spectrum was calculated and the autocorrelation function of the lunar spectrum was subtracted from it. The analysis made it possible to detect Raman scattering by H2 in the atmosphere of Jupiter. The pure rotational H2 S(0) and S(1) lines were detected. The ratio of the relative number of Raman scattered photons in the S(0) and S(1) features indicate that the H2 in the Jovian atmosphere is in the equilibrium, rather than the normal state. Therefore some sort of nonradiative process is responsible for transitions between the ortho and para states of H2.

Cochran, W. D.↗

The MRK 421 Multi-Wavelength Campaign: EUVE Observation

We present the extreme ultraviolet (EUV) spectrum and light curve of the BL Lacertae object Markarian 421, obtained with the Extreme Ultraviolet Explorer (EUVE). The EUVE observation was part of a large multiwavelength campaign covering radio to gamma-ray energies. Preliminary analysis of the EUV spectrum indicates a smooth continuum in the 75-115 A range with no evidence of absorption features. The light curve shows variability of up to factors of two on a time-scale of a few days.

Fruscione, Antonella↗

Rocket observations of the Perseus X-ray source

The spectrum and angular distribution of soft X-ray emission from the source in the Perseus cluster has been observed. A prominent feature of this source is a point-like component at the position of NGC 1275. Preliminary analysis indicates that the spectrum of this source does not rise as steeply at energies below 1 keV as has been reported previously.

Catura, R. C.↗

Development of the NASA/FLAGRO computer program for analysis of airframe structures

The NASA/FLAGRO (NASGRO) computer program was developed for fracture control analysis of space hardware and is currently the standard computer code in NASA, the U.S. Air Force, and the European Agency (ESA) for this purpose. The significant attributes of the NASGRO program are the numerous crack case solutions, the large materials file, the improved growth rate equation based on crack closure theory, and the user-friendly promptive input features. In support of the National Aging Aircraft Research Program (NAARP); NASGRO is being further developed to provide advanced state-of-the-art capability for damage tolerance and crack growth analysis of aircraft structural problems, including mechanical systems and engines. The project currently involves a cooperative development effort by NASA, FAA, and ESA. The primary tasks underway are the incorporation of advanced methodology for crack growth rate retardation resulting from spectrum loading and improved analysis for determining crack instability. Also, the current weight function solutions in NASGRO or nonlinear stress gradient problems are being extended to more crack cases, and the 2-d boundary integral routine for stress analysis and stress-intensity factor solutions is being extended to 3-d problems. Lastly, effort is underway to enhance the program to operate on personal computers and work stations in a Windows environment. Because of the increasing and already wide usage of NASGRO, the code offers an excellent mechanism for technology transfer for new fatigue and fracture mechanics capabilities developed within NAARP.

Forman, R. G.↗