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At least 667 records · Page 37

Superconducting NbTiN thin films for superconducting radio frequency accelerator cavity applications

Current superconducting radio frequency technology, used in various particle accelerator facilities across the world, is reliant upon bulk niobium superconducting cavities. Due to technological advancements in the processing of bulk Nb cavities, the facilities have reached accelerating fields very close to a material-dependent limit, which is close to 50 MV/m for bulk Nb. One possible solution to improve upon this fundamental limitation was proposed a few years ago by Gurevich [Appl. Phys. Lett. 88, 012511 (2006)], consisting of the deposition of alternating thin layers of superconducting and insulating materials on the interior surface of the cavities. The use of type-II superconductors with Tc > Tc Nb and H c > HcNb, (e.g., Nb 3 Sn, NbN, or NbTiN) could potentially greatly reduce the surface resistance (Rs) and enhance the accelerating field, if the onset of vortex penetration is increased above Hc Nb , thus enabling higher field gradients. Although Nb 3 Sn may prove superior, it is not clear that it can be grown as a suitable thin film for the proposed multilayer approach, since very high temperature is typically required for its growth, hindering achieving smooth interfaces and/or surfaces. On the other hand, since NbTiN has a smaller lower critical field (H c1 ) and higher critical temperature (T c ) than Nb and increased conductivity compared to NbN, it is a promising candidate material for this new scheme. Here, the authors present experimental results correlating filmmicrostructure with superconducting properties on NbTiN thin film coupon samples while also comparing filmsgrown with targets of different stoichiometry. In conclusion, it is worth mentioning that the authors have achieved thin films with bulk-like lattice parameter and transition temperature while also achieving H c1 values larger than bulk for films thinner than their London penetration depths.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Superconducting Thin Films for The Enhancement of Superconducting Radio Frequency Accelerator Cavities

Bulk niobium (Nb) superconducting radio frequency (SRF) cavities are currently the preferred method for acceleration of charged particles at accelerating facilities around the world. However, bulk Nb cavities have poor thermal conductance, impose material and design restrictions on other components of a particle accelerator, have low reproducibility and are approaching the fundamental material-dependent accelerating field limit of approximately 50MV/m. Since the SRF phenomena occurs at surfaces within a shallow depth of ~1 μm, a proposed solution to this problem has been to utilize thin film technology to deposit superconducting thin films on the interior of cavities to engineer the active SRF surface in order to achieve cavities with enhanced properties and performance. Two proposed thin film applications for SRF cavities are: 1) Nb thin films coated on bulk cavities made of suitable castable metals (such as copper or aluminum) and 2) multilayer films designed to increase the accelerating gradient and performance of SRF cavities. While Nb thin films on copper (Cu) cavities have been attempted in the past using DC magnetron sputtering (DCMS), such cavities have never performed at the bulk Nb level. However, new energetic condensation techniques for film deposition, such as High Power Impulse Magnetron Sputtering (HiPIMS), offer the opportunity to create suitably thick Nb films with improved density, microstructure and adhesion compared to traditional DCMS. Clearly use of such novel technique requires fundamental studies to assess surface evolution and growth modes during deposition and resulting microstructure and surface morphology and the correlation with RF superconducting properties. Here we present detailed structure-property correlative research studies done on Nb/Cu thin films and NbN- and NbTiN-based multilayers made using HiPIMS and DCMS, respectively. Experiment Numbers:

Burton, Matthew↗

Surface Cracking and Interface Reaction Associated Delamination Failure of Thermal and Environmental Barrier

In this paper, surface cracking and interface reactions of a ZrO2-8wt%Y2O3 and mullite/BSAS/Si thermal and environmental barrier coating system on SiC/SiC ceramic matrix composites were characterized after long-term combined laser thermal gradient and furnace cyclic tests in a water vapor containing environment. The surface cracking was analyzed based on the coating thermal gradient sintering behavior and thermal expansion mismatch stress characteristics under the thermal cyclic conditions. The interface reactions that were largely enhanced by the coating surface cracking in the water vapor environment were investigated in detail, and the reaction phases were identified for the coating system after the long-term exposure. The accelerated coating delamination failure was attributed to the increased delamination driving force under the thermal gradient cyclic loading and the reduced interface adhesion due to the detrimental interface reactions. The coating design issues will also be discussed based on the observed failure mechanisms under the high-heat-flux test conditions.

Zhu, Dongming↗

Conventional and Bimodal Nuclear Thermal Rocket (NTR) Artificial Gravity Mars Transfer Vehicle Concepts

A variety of countermeasures have been developed to address the debilitating physiological effects of zero-gravity (0-g) experienced by cosmonauts and astronauts during their approximately 0.5 to 1.2 year long stays in low Earth orbit (LEO). Longer interplanetary flights, combined with possible prolonged stays in Mars orbit, could subject crewmembers to up to approximately 2.5 years of weightlessness. In view of known and recently diagnosed problems associated with 0-g, an artificial gravity (AG) spacecraft offers many advantages and may indeed be an enabling technology for human flights to Mars. A number of important human factors must be taken into account in selecting the rotation radius, rotation rate, and orientation of the habitation module or modules. These factors include the gravity gradient effect, radial and tangential Coriolis forces, along with cross-coupled acceleration effects. Artificial gravity Mars transfer vehicle (MTV) concepts are presented that utilize both conventional NTR, as well as, enhanced bimodal nuclear thermal rocket (BNTR) propulsion. The NTR is a proven technology that generates high thrust and has a specific impulse (Isp) capability of approximately 900 s-twice that of today's best chemical rockets. The AG/MTV concepts using conventional Nuclear Thermal Propulsion (NTP) carry twin cylindrical International Space Station (ISS)- type habitation modules with their long axes oriented either perpendicular or parallel to the longitudinal spin axis of the MTV and utilize photovoltaic arrays (PVAs) for spacecraft power. The twin habitat modules are connected to a central operations hub located at the front of the MTV via two pressurized tunnels that provide the rotation radius for the habitat modules. For the BNTR AG/MTV option, each engine has its own closed secondary helium(He)-xenon (Xe) gas loop and Brayton Rotating Unit (BRU) that can generate 10s of kilowatts (kWe) of spacecraft electrical power during the mission coast phase eliminating the need for large PVAs. A single inflatable TransHab-type habitation module is also used with multiple vertical floors oriented radial to the MTV spin axis. The BNTR MTV's geometry-long and linear-is naturally compatible with AG operation. By rotating the vehicle about its center-of-mass (CM) and perpendicular to its flight vector at approximately 3.0 to 5.2 rpm, a centrifugal force and AG environment corresponding to approximately 0.38 to 1.0 g can be established to help maintain crew fitness out to Mars and back. Vehicles using NTP/ Bimodal Nuclear Thermal Propulsion (BNTP) can more readily accommodate the heavier payload mass and increased RCS propellant loading associated with AG operation, and can travel faster to and from Mars thereby reducing the crew's exposure to galactic cosmic radiation and solar flares. Mission scenario descriptions, key vehicle features and operational characteristics for each propulsion option are presented using the lift capability and payload volumes estimated for the Space Launch System (SLS)-1B and followon Heavy Lift Vehicle (HLV).

Nuclear Propulsion↗

Advancements in HF-free bipolar pulsed electropolishing for next-generation superconducting cavities

Hydrofluoric acid (HF)-free bipolar pulsed electropolishing (BPEP) offers an environmentally sustainable alternative to conventional Buffered Chemical Polishing (BCP) and Electropolishing (EP) techniques for superconducting radiofrequency (SRF) cavities. Recent studies at Jefferson Lab have demonstrated that a single-cell 1.3 GHz niobium cavity processed using HF-free BPEP achieved an accelerating gradient Eacc of 35 MV/m with a quality factor Q0 of 1E10 at 2 K, following extensive research and optimization. This talk will highlight the challenges encountered in developing this technique, key insights gained from experimental studies, and ongoing efforts to enhance its capabilities. In particular, we will explore its potential for refining Nb3Sn-coated niobium cavities via vapor diffusion techniques and for electroplating Nb3Sn films onto various cavity substrates, contributing to the advancement of high-performance SRF systems.

Tian, Hui [Thomas Jefferson National Accelerator F↗

A Kaczmarz-inspired approach to accelerate the optimization of neural network wavefunctions

Neural network wavefunctions optimized using the variational Monte Carlo method have been shown to produce highly accurate results for the electronic structure of atoms and small molecules, but the high cost of optimizing such wavefunctions prevents their application to larger systems. We propose the Subsampled Projected-Increment Natural Gradient Descent (SPRING) optimizer to reduce this bottleneck. SPRING combines ideas from the recently introduced minimum-step stochastic reconfiguration optimizer (MinSR) and the classical randomized Kaczmarz method for solving linear least-squares problems. We demonstrate that SPRING outperforms both MinSR and the popular Kronecker-Factored Approximate Curvature method (KFAC) across a number of small atoms and molecules, given that the learning rates of all methods are optimally tuned. For example, on the oxygen atom, SPRING attains chemical accuracy after forty thousand training iterations, whereas both MinSR and KFAC fail to do so even after one hundred thousand iterations.

97 MATHEMATICS AND COMPUTING↗

Field, frequency, and temperature dependencies of the surface resistance of nitrogen diffused niobium superconducting radio frequency cavities

We investigate the rf performance of several single-cell superconducting radio-frequency cavities subjected to low temperature heat treatment in nitrogen environment. The cavities were treated at temperature 120 – 165 ° C for an extended period of time (24–48 h) either in high vacuum or in a low partial pressure of ultrapure nitrogen. The improvement in Q 0 with a Q rise was observed when nitrogen gas was injected at ∼ 300 ° C during the cavity cooldown from 800 ° C and held at 165 ° C , without any degradation in accelerating gradient over the baseline performance. The treatment was applied to several elliptical cavities with frequency ranging from 0.75 to 3.0 GHz, showing an improved quality factor as a result of low temperature nitrogen treatments. The Q rise feature is similar to that achieved by nitrogen alloying Nb cavities at higher temperature, followed by material removal by electropolishing. The surface modification was confirmed by the change in electronic mean free path and tuned with the temperature and duration of heat treatment. The decrease of the temperature-dependent surface resistance with increasing rf field, resulting in a Q rise, becomes stronger with increasing frequency and decreasing temperature. The data suggest a crossover frequency of ∼ 0.95 GHz above that the Q rise phenomenon occurs at 2 K. Some of these results can be explained qualitatively with an existing model of intrinsic field-dependence of the surface resistance with both equilibrium and nonequilibrium quasiparticle distribution functions. The change in the Q slope below 0.95 GHz may result from masking contribution of trapped magnetic flux to the residual surface resistance. Published by the American Physical Society 2024

43 PARTICLE ACCELERATORS↗

Conventional and Bimodal Nuclear Thermal Rocket (NTR) Artificial Gravity Mars Transfer Vehicle Concepts

A variety of countermeasures have been developed to address the debilitating physiological effects of "zero-gravity" (0-g) experienced by cosmonauts and astronauts during their approximately 0.5-1.2 year long stays in LEO (Low Earth Orbit). Longer interplanetary flights, combined with possible prolonged stays in Mars orbit, could subject crewmembers to up to approximately 2.5 years of weightlessness. In view of known and recently diagnosed problems associated with 0-g, an artificial gravity spacecraft offers many advantages and may indeed be an enabling technology for human flights to Mars. A number of important human factors must be taken into account in selecting the rotation radius, rotation rate, and orientation of the habitation module or modules. These factors include the gravity gradient effect, radial and tangential Coriolis forces, along with cross-coupled acceleration effects. Artificial gravity (AG) Mars transfer vehicle (MTV) concepts are presented that utilize both conventional NTR, as well as, enhanced "bimodal" nuclear thermal rocket (BNTR) propulsion. The NTR is a proven technology that generates high thrust and has a specific impulse (I (sub sp)) capability of approximately 900 s - twice that of today's best chemical rockets. The AG/MTV concepts using conventional NTP carry twin cylindrical "ISS-type" habitation modules with their long axes oriented either perpendicular or parallel to the longitudinal spin axis of the MTV and utilize photovoltaic arrays (PVAs) for spacecraft power. The twin habitat modules are connected to a central operations hub located at the front of the MTV via two pressurized tunnels that provide the rotation radius for the habitat modules. For the BNTR AG/MTV option, each engine has its own "closed" secondary helium-xenon gas loop and Brayton rotating unit that can generate tens of kilowatts (kW (sub e)) of spacecraft electrical power during the mission coast phase eliminating the need for large PVAs. A single inflatable "TransHab-type" habitation module is also used with multiple vertical floors oriented radial to the MTV spin axis. The BNTR MTV's geometry - long and linear - is naturally compatible with AG operation. By rotating the vehicle about its center-of-mass and perpendicular to its flight vector at approximately 3.0 - 5.2 rpm, a centrifugal force and AG environment corresponding to approximately 0.38 - 1.0 g can be established to help maintain crew fitness out to Mars and back. Vehicles using NTP/BNTP can more readily accommodate the heavier payload mass and increased RCS propellant loading associated with AG operation, and can travel faster to and from Mars thereby reducing the crew's exposure to galactic cosmic radiation and solar flares. Mission scenario descriptions, key vehicle features and operational characteristics for each propulsion options are presented using the lift capability and payload volumes estimated for the SLS-1A and HLV.

Nuclear Propulsion↗

Electron Recombination in a Dense Hydrogen Plasma

A high pressure hydrogen gas filled RF cavity was subjected to an intense proton beam to study the evolution of the beam induced plasma inside the cavity. Varying beam intensities, gas pressures and electric fields were tested. Beam induced ionized electrons load the cavity, thereby decreasing the accelerating gradient. The extent and duration of this degradation has been measured. A model of the recombination between ionized electrons and ions is presented, with the intent of producing a baseline for the physics inside such a cavity used in a muon accelerator. Analysis of the data taken during the summer of 2011 shows that self recombination takes place in pure hydrogen gas. The decay of the number of electrons in the cavity once the beam is turned off indicates self recombination rather than attachment to electronegative dopants or impurities. The cross section of electron recombination grows for larger clusters of hydrogen and so at the equilibrium of electron production and recombination in the cavity, processes involving H{sub 5}{sup +} or larger clusters must be taking place. The measured recombination rates during this time match or exceed the analytic predicted values. The accelerating gradient in the cavity recovers fully in time for the next beam pulse of a muon collider. Exactly what the recombination rate is and how much the gradient degrades during the 60 ns muon collider beam pulse will be extrapolated from data taken during the spring of 2012.

43 PARTICLE ACCELERATORS↗

Performance Limiting Effects in X-Band Accelerators

Acceleration gradient is a critical parameter for the design of future TeV-scale linear colliders. The major obstacle to higher gradient in room-temperature accelerators is rf breakdown, which is still a very mysterious phenomenon that depends on the geometry and material of the accelerator as well as the input power and operating frequency. Pulsed heating has been associated with breakdown for many years; however, there have been no experiments that clearly separate field and heating effects on the breakdown rate. Recently, such experiments have been performed at SLAC with both standing-wave and traveling-wave structures. These experiments have demonstrated that pulsed heating is limiting the gradient. Nevertheless the X-band structures breakdown studies show damage to the iris surfaces in locations of high electric field rather than of high magnetic field after thousands of breakdowns. It is not yet clear how the relative roles of electric field, magnetic field, and heating factor into the damage caused by rf breakdown. Thus, a dual-moded cavity has been designed to better study the electric field, magnetic field, and pulsed heating effects on breakdown damage.

43 PARTICLE ACCELERATORS↗

A Compact and High Performance Muon Capture Channel for Muon Accelerators

It is widely believed that a neutrino factory would deliver unparallel performance in studying neutrino mixing and would provide tremendous sensitivity to new physics in the neutrino sector. Here we will describe and simulate the front-end of the neutrino factory system, which plays critical role in determining the number of muons that can be accepted by the downstream accelerators. In this system, a proton bunch on a target creates secondaries that drift into a capture transport channel. A sequence of rf cavities forms the resulting muon beams into strings of bunches of differing energies, aligns the bunches to nearly equal central energies, and initiates ionization cooling. For this, the muon beams are transported through sections containing high-gradient cavities and strong focusing solenoids. In this paper we present results of optimization and variation studies toward obtaining the maximum number of muons for a neutrino factory by using a compact transport channel. It has been suggested computationally and experimentally that the maximum achievable gradient is enhanced by introducing an external magnetic field at right angles to the rf electric field since it suppresses field-emission processes. Here, we have discussed a possible scheme for extending the concept of magnetic insulation to capture, transport, and cool muons in a neutrino factory. We incorporated this idea into a new lattice design where the rf cavities are shaped so that their walls were tangential to the magnetic-field lines. We showed that, with magnetic insulation, the field-emitted electrons impact the cavity surface with energies four orders-of-magnitude less than in conventional pillbox cavities; consequently, damage from field-emission is suppressed significantly. While demanding in terms of power requirements, this neutrino factory lattice showed satisfactory performance in both cooling and collecting the accepted muons within the requirements for the IDSNF. Optimizations were also made to reduce heating on the absorber windows minimizing losses in the accepted muon fluxes. The next step for verifying these ideas should be an experimental demonstration of a single muon accelerator magnetically-insulated rf cavity. A successful demonstration will provide us with a new versatile tool for a future muon accelerator.

43 PARTICLE ACCELERATORS↗

Collisionless relativistic magnetic reconnection driven by electron vortices in laser-plasma interaction

Magnetic reconnection (MR) is a fundamental process in space and laboratory plasmas. The appearance of high power lasers opens a new way to investigate MR under the relativistic condition. In this paper, relativistic collisionless MR driven by two ultra-intense lasers and a pair of asymmetric targets is studied numerically via the kinetic simulations. The static magnetic fields produced by the electron vortex structures with opposite magnetic polarities approach each other driven by the magnetic pressure and the density gradient. The antiparallel magnetic fields annihilate accompanied with the topological variation and the corresponding magnetic field energy is being dissipated to the kinetic energy of the nonthermal charged particles. Besides the outflows along the current sheet, a fast particle bunch is accelerated perpendicularly contributed by the displacement current.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Particle-in-cell simulation of x-ray wakefield acceleration and betatron radiation in nanotubes

Though wakefield acceleration in crystal channels has been previously proposed, x-ray wakefield acceleration has only recently become a realistic possibility since the invention of the single-cycled optical laser compression technique. We investigate the acceleration due to a wakefield induced by a coherent, ultrashort x-ray pulse guided by a nanoscale channel inside a solid material. By two-dimensional particle-in-cell computer simulations, we show that an acceleration gradient of TeV/cm is attainable. This is about 3 orders of magnitude stronger than that of the conventional plasma-based wakefield accelerations, which implies the possibility of an extremely compact scheme to attain ultrahigh energies. In addition to particle acceleration, this scheme can also induce the emission of high energy photons at ∼O(10–100) MeV. Our simulations confirm such high energy photon emissions, which is in contrast with that induced by the optical laser driven wakefield scheme. In addition to this, the significantly improved emittance of the energetic electrons has been discussed.

43 PARTICLE ACCELERATORS↗

Reducing field emission in superconducting cavities with ozone

Contaminations on the active surface of high-power microwave resonators, such as radio-frequency accelerator cavities, can greatly enlarge electron field emission and reduce their performance. In this work, we demonstrate the use of ozone to clean the surface of niobium superconducting radio-frequency cavities resulting in reduced field emission and enhanced accelerating gradient before onset of field emission. We report results from processing four cavities.

43 PARTICLE ACCELERATORS↗

STS-40 orbital acceleration research experiment flight results during a typical sleep period

The Orbital Acceleration Research Experiment (OARE), an electrostatic accelerometer package with complete on-orbit calibration capabilities, was flown for the first time aboard the Space Shuttle on STS-40. This is also the first time an accelerometer package with nano-g sensitivity and a calibration facility has flown aboard the Space Shuttle. The instrument is designed to measure and record the Space Shuttle aerodynamic acceleration environment from the free molecule flow regime through the rarified flow transition into the hypersonic continuum regime. Because of its sensitivity, the OARE instrument defects aerodynamic behavior of the Space Shuttle while in low-earth orbit. A 2-hour orbital time period on day seven of the mission, when the crew was asleep and other spacecraft activities were at a minimum, was examined. During the flight, a 'trimmed-mean' filter was used to produce high quality, low frequency data which was successfully stored aboard the Space Shuttle in the OARE data storage system. Initial review of the data indicated that, although the expected precision was achieved, some equipment problems occurred resulting in uncertain accuracy. An acceleration model which includes aerodynamic, gravity-gradient, and rotational effects was constructed and compared with flight data. Examination of the model with the flight data shows the instrument to be sensitive to all major expected low frequency acceleration phenomena; however, some erratic instrument bias behavior persists in two axes. In these axes, the OARE data can be made to match a comprehensive atmospheric-aerodynamic model by making bias adjustments and slight linear corrections for drift. The other axis does not exhibit these difficulties and gives good agreement with the acceleration model.

Blanchard, R. C.↗

Overview of Mono-Energetic Gamma-Ray Sources and Applications

Recent progress in accelerator physics and laser technology have enabled the development of a new class of tunable gamma-ray light sources based on Compton scattering between a high-brightness, relativistic electron beam and a high intensity laser pulse produced via chirped-pulse amplification (CPA). A precision, tunable Mono-Energetic Gamma-ray (MEGa-ray) source driven by a compact, high-gradient X-band linac is currently under development and construction at LLNL. High-brightness, relativistic electron bunches produced by an X-band linac designed in collaboration with SLAC NAL will interact with a Joule-class, 10 ps, diode-pumped CPA laser pulse to generate tunable {gamma}-rays in the 0.5-2.5 MeV photon energy range via Compton scattering. This MEGaray source will be used to excite nuclear resonance fluorescence in various isotopes. Applications include homeland security, stockpile science and surveillance, nuclear fuel assay, and waste imaging and assay. The source design, key parameters, and current status are presented, along with important applications, including nuclear resonance fluorescence.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Progress and challenges in traveling-wave (TW) SRF cavity

Traveling-wave (TW) technology can push the accelerator field gradient of niobium SRF cavity to 70MV/m or higher beyond the limit of 50~60MV/m in Standing-wave (SW) technology. The early stages of TW SRF cavity developments had been funded by several SBIR grants to Euclid Techlabs and completed in collaboration with Fermilab through a 1-cell prototype and a proof-of-principle 3-cell TW cavity. The TW resonance excitation in the 3-cell TW cavity at 2K was demonstrated through the low power RF test in early 2024. A high-power test of the 3-cell in TW mode being prepared. To advance a design and technology to fabricate a novel high gradient TW SRF cavity, FNAL proposed a half-meter TW RF design and R&Ds to realize that are in progress. Here we will report the recent progress in the 3-cell TW cavity and the challenges towards a half-meter scale TW cavity.

43 PARTICLE ACCELERATORS↗

Development of an X-Ray Talbot-Lau Moire Deflectometer of Fast Density Profile Measurements of Dense Plasmas Generated by Beam Target Interactions

For the first time an x-ray Talbot-Lau moiré deflectometer is being developed that will use a flash tube source and fast detector for dynamic density gradient measurements. In Talbot-Lau moiré deflectometry, an x-ray grating makes an mage of itself on a second grating (the Talbot effect) to produce a moiré pattern on a detector. The test object is placed between these gratings, with variations in index of refraction changing the pattern. A third grating in front of an incoherent x-ray source produces an array of coherent sources. With a 150 kV x-ray flash tube as the source, the gratings are placed in a glancing angle setup for performance at ~60 keV. The detector is a gated CCD with a fast scintillator for x-ray conversion. This diagnostic, designed for the Dual-Axis Radiographic Hydrodynamic Test facility (DARHT) at Los Alamos National Laboratory, measures the density profile of dense plasma plumes ejected from beam-target interactions. DARHT has two high-current, pulsed, inductive linear electron accelerators with bremsstrahlung targets at the end of each beam line to create 2-D radiographic images of hydrodynamic tests. One multipulse accelerator has up to four beam pulses striking the same target within 2 μs. Computer simulations that model target evolution and ejected material between pulses are used to design these targets for optimal radiographic performance; the x-ray deflectometer will directly measure density gradients in the ejected plumes and provide the first experimental constraints to these models. During the first year, currently underway, the diagnostic systems are being designed. In year two, the flash tube and fast detector will be deployed at DARHT for radiographic imaging while the deflectometer is built and tested on the bench with a continuous source. In year three, the fast deflectometer will be installed on DARHT and density measurements will be performed.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗