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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 685 records · Page 38

Safety Analysis Report For Packaging, Y-12 National Security Complex, Model ES-3100 Package with Bulk HEU Contents

This safety analysis report for packaging (SARP) presents the results of the safety analysis prepared in support of the Consolidated Nuclear Security, LLC (CNS) request for licensing of the Model ES-3100 package with bulk highly enriched uranium (HEU) contents and issuance of a Type B(U) Fissile Material Certificate of Compliance. This SARP, published in the format specified in the U.S. Nuclear Regulatory Commission (NRC) Regulatory Guide 7.9 and using information provided in UCID-21218 and NRC Regulatory Guide 7.10, demonstrates that the Y-12 National Security Complex (Y-12) ES-3100 package with bulk HEU contents meets the established NRC regulations for packaging, preparation for shipment, and transportation of radioactive materials given in Title 10, Part 71, of the Code of Federal Regulations (CFR) [10 CFR 71] as well as U.S. Department of Transportation (DOT) regulations for packaging and shipment of hazardous materials given in Title 49 CFR.

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Development of small particle speciation for nuclear forensics by soft X-ray scanning transmission spectromicroscopy

Synchrotron radiation spectromicroscopy provides a combination of submicron spatial resolution and chemical sensitivity that is well-suited to analysis of heterogeneous nuclear materials. The chemical and physical characteristics determined by scanning transmission X-ray microscopy (STXM) are complementary to information obtained from standard radiochemical analysis methods. In addition, microscopic quantities of radioactive material can be characterized rapidly by STXM with minimal sample handling and intrusion, especially in the case of particulate materials. The STXM can accommodate a diverse range of samples including wet materials, complex mixtures, and small quantities of material contained in a larger matrix. In these cases, the inventory of species present in a sample is likely to carry information on its process history; STXM has the demonstrated capability to identify contaminants and sample matrices. Operating in the soft X-ray regime provides particular sensitivity to the chemical state of specimens containing low-Z materials, via the K-edges of light elements. In this paper, recent developments in forensics-themed spectromicroscopy, sample preparation, and data acquisition methods at the Molecular Environmental Science Beamline 11.0.2 of the Advanced Light Source are described. Results from several initial studies are presented, demonstrating the capability to identify the distribution of the species present in heterogeneous uranium-bearing materials. Finally, future opportunities for STXM forensic studies and potential methodology development are discussed.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Hanford Site Composite Analysis Technical Approach Description: Radionuclide Inventory and Waste Site Selection Process.

The updated Hanford Site Composite Analysis will provide an all-pathways dose projection to a hypothetical future member of the public from all planned low-level radioactive waste disposal facilities and potential contributions from all other projected end-state sources of radioactive material left at Hanford following site closure. Its primary purpose is to support the decision-making process of the U.S. Department of Energy (DOE) under DOE O 435.1-1, Radioactive Waste Management (DOE, 2001), related to managing low-level waste disposal facilities at the Hanford Site.

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Issue focused stakeholder collaboration: reaching consensus on spent nuclear fuel transportation operational practices - 15465

This paper examines stakeholder and issue-focused approaches used by Department of Energy (DOE) programs to collaborate with key stakeholders on transportation practices to ship radioactive material, particularly used nuclear fuel (UNF) and transuranic waste (TRU). In accordance with the Administration's Strategy for the Management and Disposal of Used Nuclear Fuel and High-Level Radioactive Waste, the current effort by DOE to plan for the development of a future transportation system to ship UNF from commercial reactors, with an initial focus on shutdown reactors, is using approaches similar to those used in other successful shipping campaigns to collaborate with stakeholders about sustainable transportation practices. As part of a coordinated approach to stakeholder outreach and collaboration, DOE is currently developing a draft Transportation Planning Framework to provide a template for future shipments of UNF from commercial reactors and is engaged with states and tribes and other stakeholders in discussions on the institutional and operational components of that Framework. (authors)

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Materials and Fuels Complex FY-22 – FY-26 Five-Year Mission Strategy

The Idaho National Laboratory (INL), through its designated mission of advancing innovative nuclear energy solutions, is actively engaged in the research, development, demonstration and deployment of advanced nuclear technology. Key to the success of INL’s mission is the Materials and Fuels Complex (MFC), the only complex in the U.S. that hosts a world-class assemblage of facilities, capabilities and instruments for handling, testing, and characterizing nuclear fuel and radioactive materials. Driven by its mission/vision of “Engineering and Experiments that Drive the World’s Nuclear Energy Future,” MFC is at the center of INL’s – and indeed the Department of Energy’s – advanced nuclear technology development initiatives, providing essential capabilities such as research-scale high-assay low-enriched uranium (HALEU) fuel production, reactor demonstration facilities, post-irradiation examination, and transient irradiation testing. Furthermore, MFC provides an ideal environment for test beds that are utilized for research, development and demonstration (RD&D) activities on used fuel treatment, nuclear non-proliferation, forensics, and nuclear power sources used for space exploration missions conducted by the National Aeronautics and Space Administration (NASA).

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Radioactive satellites - Intact reentry and breakup by debris impact

There is a substantial mass of radioactive material in nuclear reactors or radioisotope thermal generators (RTGs) in orbit about the earth. This paper examines the reentry of intact nuclear fuel cores and RTGs and the fragmentation and subsequent radioactive debris cloud deposition and evolution resulting from the impact of orbital debris upon an orbiting reactor, fuel core, or RTG. To assess the intact reentry, decay rates and a predicted decay date using historical and projected orbital decay data, are estimated. The current NASA debris environment model is utilized to estimate impact rates and debris cloud evolution of a fragmentation event. Results of these analyses are compared and concepts are tendered which would tend to minimize the radiological debris hazard to personnel and structures both on the earth's surface and in low earth orbit.

Anz-Meador, P. D.↗

Special Analysis: 2016-002, Analysis of Cover Erosion and Enhanced Infiltration at Pit 25, TA-54 Area G

The Los Alamos National Laboratory (LANL) generates radioactive waste as a result of various activities. Operational waste is generated from a wide variety of research and development activities including nuclear weapons development, energy production, and medical research. Environmental restoration, and decontamination and decommissioning (D&D) waste is generated as contaminated sites and facilities at LANL undergo cleanup or remediation. The majority of this waste is low-level radioactive waste (LLW) and is disposed of at the Technical Area 54 (TA-54), Area G disposal facility. U.S. Department of Energy (DOE) Order 435.1 (DOE, 2001) requires that radioactive waste be managed in a manner that protects public health and safety, and the environment. To comply with this order, DOE field sites must prepare site-specific radiological performance assessments for LLW disposal facilities that accept waste after September 26, 1988. Furthermore, sites are required to conduct composite analyses that account for the cumulative impacts of all waste that has been (or will be) disposed of at the facilities and other sources of radioactive material that may interact with the facilities.

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RH-72B Packaging Plan Slides for University of Washington [Slides]

This report describes the Shipping Package RH-72B, specially in terms of why this container should be used, its features, how it will be utilized for the shipment of radiation and radioactive material from the University of Washington, and the placement of the 72B for loading.

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Update on Full-Scale Retrieval and Transfer System Testing for Pneumatic Conveyance of High-Level Calcine Waste - 20241

The Idaho National Laboratory processed spent nuclear fuel from 1953 to 1994. The process used solvent extraction to separate uranium, resulting in a liquid waste. A calcination process was used to convert the liquid waste to a high-level radioactive solid powder, referred to as calcine. The calcine is stored in stainless steel bins contained within concrete vaults called the Calcined Solids Storage Facilities. There are a total of seven CSSFs. The Calcine Retrieval Project is tasked with retrieving the calcine from the bins of CSSF 1 and pneumatically transferring it to the bins of CSSF 6. CSSF 1 was constructed to be a final calcine repository with no forethought of retrieval. It represents the greatest technical hurdle to calcine extraction of all the CSSFs. The challenges inherent with accessing the calcine, safely extracting it, and securely transporting it are copious and complex. Once the calcine is removed from CSSF1, that facility may be closed, reducing the footprint of waste storage at the INL. The same process for removing Calcine from CSSF1 may then be utilized to remove the calcine from the remaining CSSFs for final treatment and transport to a long-term storage facility. To overcome these inherent challenges with accessing CSSF 1 and extracting the calcine in a timely manner, a full-scale integrated mockup has been constructed. The mockup includes a full-size model of a concentric group of bins from CSSF 1 and a storage vessel representing CSSF 6. All essential elements of the transport design are represented in the Mockup, including motive and makeup air supply (air compressor), a replica of the CSSF6 cyclone, pre-filter, HEPA filter, vacuum pump, and retrieval control devices. Construction on the Mockup was completed in 2018 and testing began in February 2019. It has already proven very beneficial to the CRP. Experience in running the Mockup have aided in the development of retrieval and transport methodologies and the selection of process parameter values. It has also uncovered some unforeseen technological challenges and will continue to be valuable to the testing team as these hurdles are overcome and the process is proven effective. Operations personnel have also benefitted from its use as a training tool and will continue to use the Mockup as a simulator to reproduce problems encountered during extraction and transfer of Calcine from CSSF 1. The knowledge gained during this process will also be of continued benefit as future work is done to remove various types of calcine from the remaining CSSFs. The methodology of safe and secure transfer of radioactive material may be of benefit to others throughout the U.S. Department of Energy complex. (authors)

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Hanford Site Composite Analysis: Radionuclide Selection for Groundwater Pathway Evaluation.

The updated Hanford Site Composite Analysis (CA) will provide an all-pathways dose projection to a hypothetical future member of the public from all planned low-level radioactive waste disposal facilities and potential contributions from all other projected end-state sources of radioactive material left at the Hanford Site following site closure. Its primary purpose is to support the decision-making process of the U.S. Department of Energy (DOE) under DOE O 435.1-1, Radioactive Waste Management, related to managing low-level waste disposal facilities at the Hanford Site. A key aspect of conducting a CA is selecting the radionuclides to be included in the quantitative analysis.

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Hanford Site Composite Analysis: Radionuclide Selection for Groundwater Pathway Evaluation

The updated Hanford Site Composite Analysis (CA) (DOE/RL-2019-52, Composite Analysis for Low-Level Waste Disposal in the Hanford Site Central Plateau (FY 2020)) provides an all-pathways dose projection to a hypothetical future member of the public from all planned low-level radioactive waste disposal facilities and potential contributions from all other projected end-state sources of radioactive material left at the Hanford Site following site closure. Its primary purpose is to support the decision-making process of the U.S. Department of Energy (DOE) under DOE O 435.1-1, Radioactive Waste Management, related to managing low-level waste disposal facilities at the Hanford Site. A key aspect of conducting a CA is selecting the radionuclides to be analyzed. This document describes the selection process for radionuclides to be included in the quantitative analysis.

07 ISOTOPE AND RADIATION SOURCES↗

HEU Systems at Low Temperatures [Slides]

This project is sponsored by the Nuclear Criticality Safety Program (NCSP) in collaboration with Lawrence Livermore National Laboratory (LLNL) with a novel interest surrounding the transportation of fissile material: there is a concern regarding the inadvertent introduction of the material in a low-temperature environment. The low-temperature environment will be bounded down to temperatures not below -40 ºC, since this is the limit allotted for packages containing general radioactive material exposed to air. Eventually, the goal of the project is to conduct experiments spanning multiple fission energies at these low temperatures, concluding in an International Criticality Safety Benchmark Evaluation Project (ICSBEP) benchmark.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

SAFETY ANALYSIS REPORT FOR PACKAGING SHIELDING & NUCLEAR CRITICALITY SAFETY COURSES DEVELOPED AND CONDUCTED BY OAK RIDGE NATIONAL LABORATORY

The US Department of Energy (DOE) Packaging Certification Program, Office of Packaging and Transportation, is offering Safety Analysis Report for Packaging (SARP) Shielding and Nuclear Criticality Safety (NCS) courses for SARP generalists and analysts. The SARP generalist course is designed for project managers, supervisors, NCS/shielding subject matter experts (SME), and SMEs in non-NCS/shielding technical areas (e.g., structural, thermal, package design) who need to improve their understanding of how NCS/shielding analyses fit into the broader spectrum of SARP documentation. The generalist course provides an overview of the regulations and guidelines for the criticality and shielding analyses included in a SARP, and it illustrates how the NCS/shielding chapters integrate with the other parts of the SARP. After course material is presented, students in the generalist course will review an actual SARP document to examine key elements of the shielding and criticality analyses. The analyst course provides detailed instructions on the radioactive material package shielding analyses and NCS evaluation fundamentals needed by analysts/practitioners, including safety analysts and/or technical reviewers, to prepare and/or review technical analyses for SARP documentation. The analyst course also provides an overview of regulations and guidelines, in addition to detailed in-class exercises associated with package shielding and NCS analyses. Analysis teams will be faced with staged SARP examples in which several important decision processes in the generation of a SARP will be demonstrated and discussed. Both courses are offered at Oak Ridge National Laboratory, and for interested students, the analyst course is offered for one hour of graduate credit (course ME-690) from the University of Nevada at Reno. An overview of the course will be provided to ensure that the NCS community is aware of the course and its intent to support the shielding and NCS aspects of packaging and transportation analyses for SARP activities.

Bowen, Douglas G.↗

Simulating Regional Groundwater Flow in the Vicinity of the Nevada National Security Site, Nye County, Nevada - 16104

The Death Valley Regional Groundwater Flow System (DVRFS) occupies an area of about 70,000 km{sup 2} in south-central Nevada and southeastern California. Interest in this system stems from the need to (1) understand the groundwater flow paths and travel times associated with potential migration of radioactive material from the Nevada National Security Site (NNSS) where underground nuclear testing was conducted from 1956 to 1992; (2) characterize the groundwater system in the vicinity of the proposed high-level radioactive waste repository at Yucca Mountain, Nev.; and (3) address a variety of potential effects from NNSS activities on users down gradient from the NNSS and Yucca Mountain. A single groundwater flow model of the DVRFS has been developed that integrates data and results of two previous regional-scale models and supports Department of Energy (DOE) programs at the NNSS. The numerical model was constrained by organizing hydrogeologic data and interpretations in three-dimensional (3D) geographic information systems and constructing a digital three-dimensional (3D) hydrogeologic framework model (HFM) to represent 27 hydrogeologic units (HGUs) and major structures in the DVRFS region. The 3D hydrogeologic data sets were discretized to 1,500 meters (m) grid cell resolution for input arrays required for the model. The DVRFS was simulated using the USGS 3D groundwater-flow modeling code MODFLOW-2000. Two examples showing how the DVRFS regional model is used by the DOE as part of waste management activities at the NNSS: (1) use of the regional model to provide the boundary conditions for site-scale models, and (2) use of the regional model to assess changes in hydraulic gradient and flow paths in the regional flow system resulting from changes in pumping in various areas of interest. (authors)

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Selection of Vadose Zone Flow and Transport Properties with Gravel Fraction Corrections for the Hanford Site Composite Analysis and Cumulative Impact Evaluation

This environmental calculation file (ECF) is a compilation of hydrologic and radiological/chemical properties to be used for the updated Hanford Site Composite Analysis (CA) and Cumulative Impact Evaluation (CIE) vadose zone (VZ) modeling. The CA will provide an all-pathways dose projection to a hypothetical future member of the public from all planned low-level radioactive waste disposal facilities and potential contributions from all other projected end-state sources of radioactive material left at the Hanford Site following site closure. Its primary purpose is to support the decision-making process of the U.S. Department of Energy (DOE) under DOE O 435.1 Chg 1, Radioactive Waste Management, related to managing low-level waste disposal facilities at the Hanford Site. The CIE evaluates the effects of cleanup decisions regarding groundwater quality in the Hanford Site Central Plateau (DOE/RL-2018-69, Cumulative Impact Evaluation Technical Approach Document). Due to the complexity and large number of waste sites in source operable units (OUs), the computational tools used for the CIE must be capable of representing a range of site conditions and source terms in the VZ while also efficiently computing the impact that cleanup decisions have on the underlying aquifer. Waste-site proximity between and within source OUs has resulted in contaminants commingling in the vadose and saturated zones in complex ways. Plume commingling requires cleanup decisions to be evaluated considering the surrounding waste sites and existing groundwater contamination, therefore demonstrating the need to evaluate cumulative impacts from the VZ to groundwater.

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Age Dating of Mixed SNM--Preliminary Investigations

Recently we investigated the nuclear forensics problem of age determination for mixed special nuclear material (SNM). Through limited computational mixing experiments and interactive age analysis, it was observed that age dating results are generally affected by the mixing of samples with different assays or even by small radioactive material contamination. The mixing and contamination can be detected through interactive age analysis, a function provided by the Decay Interaction, Visualization and Analysis (DIVA) software developed by NSTec. It is observed that for mixed SNM with two components, the age estimators typically fall into two distinct clusters on the time axis. This suggests that averaging or other simple statistical methods may not always be suitable for age dating SNM mixtures. Instead, an interactive age analysis would be more suitable for age determination of material components of such SNM mixtures. This work was supported by the National Center for Nuclear Security (NCNS).

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗

International Training Course on Implementing State Systems of Accounting for and Control (SSAC) of Nuclear Material for States with Small Quantity Protocols (SQP): Course Overview and Objectives [Slides]

This course is hosted by Los Alamos National Laboratory on behalf of the U.S. National Nuclear Security Administration (NNSA) in collaboration with the IAEA to support Member States in managing small quantities of nuclear and radioactive materials in a manner that is compliant with their international obligations.

98 NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL P↗

Panel Session 57: Nuclear Power Plant Waste Management - LLW Processor Issues

This panel resulted in senior utility managers discussing issues with commercial LLW processors. LLW processors updated utilities/NPPs on new or different services or technologies being offered to assist in their radioactive waste management goals, changes to their facility license, revisions to their acceptance guidelines, and emerging compliance issues. Presentations proposed include: 1 - EnergySolutions Waste Processing Overview (Joe Heckman, EnergySolutions (USA)); 2 - Perma-Fix: A Nuclear Services and Waste Management Company (John Kelly, Perma-Fix Environmental Services (USA)); 3 - UniTech - 'Expanding to Reduce Costs' LLW Processor Update (Gregg Johnstone, UniTech Services Group, Inc. (USA)); 4 - Low - Level Radioactive Materials Processing (Michael Miller, Veolia Nuclear Solutions (USA))

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