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Gain characterization of LGAD sensors with beta particles and 28-MeV protons

Low Gain Avalanche Diodes, also known as LGADs, are widely considered for fast-timing applications in high energy physics, nuclear physics, space science, medical imaging, and precision measurements of rare processes. Such devices are silicon-based and feature an intrinsic gain due to a p + -doped layer that allows the production of a controlled avalanche of carriers, with multiplication on the order of 10–100. This technology can provide time resolution on the order of 20–30 ps, and variants of this technology can provide precision tracking too. The characterization of LGAD performance has so far primarily been focused on the interaction of minimum ionizing particles for high energy and nuclear physics applications. This article expands the study of LGAD performance to highly-ionizing particles, such as 28-MeV protons, which are relevant for several future scientific applications, e.g. in biology and medical physics, among others. These studies were performed with a beam of 28-MeV protons from a tandem Van de Graaff accelerator at Brookhaven National Laboratory and beta particles from a ^90Sr source; these were used to characterize the response and the gain of an LGAD as a function of bias voltage and collected charge. Here, the experimental results are also compared to TCAD simulations.

47 OTHER INSTRUMENTATION↗

Shock Deformation in Zircon, a Comparison of Results from Shock-Reverberation and Single-Shock Experiments

The utility of the mineral zircon, ZrSiO4, as a shock-metamorphic geobarometer and geochronometer, has been steadily growing within the planetary science community. Zircon is an accessory phase found in many terrestrial rock types, lunar samples, lunar meteorites, martian meteorites and various other achondrites. Because zircon is refractory and has a high closure temperature for Pb diffusion, it has been used to determine the ages of some of the oldest material on Earth and elsewhere in the Solar System. Furthermore, major (O) and trace-element (REE, Ti, Hf) abundances and isotope compositions of zircon help characterize the petrogenetic environments and sources from which they crystallized. The response of zircon to impact-induced shock deformation is predominantly crystallographic, including dislocation creep and the formation of planar and sub-planar, low-angle grain boundaries; the formation of mechanical {112} twins; transformation to the high pressure polymorph reidite; the development of polycrystalline microtextures; and dissociation to the oxide constituents SiO2 and ZrO2. Shock microstructures can also variably affect the U- Pb isotope systematics of zircon and, in some instances, be used to constrain the impact age. While numerous studies have characterized shock deformation in zircon recovered from a variety of terrestrial impact craters and ejecta deposits and Apollo samples, experimental studies of shock deformation in zircon are limited to a handful of examples in the literature. In addition, the formation conditions (e.g., P, T) of various shock microstructures, such as planar-deformation bands, twins, and reidite lamellae, remain poorly con-strained. Furthermore, previous shocked-zircon experimental charges have not been analyzed using modern analytical equipment. This study will therefore under-take an new set of zircon shock experiments, which will then be microstructurally characterized using state-of-the-art instrumentation within the Astromaterials Research and Exploration Science Division (ARES), NASA Johnson Space Center.

Erickon, T. M.↗

Nuclear Interdiction Through Relocatable Detectors

The NNSA Office of Nuclear Smuggling Detection and Deterrence (NSDD) has investigated a set of minimal-infrastructure radiation detection systems as alternatives to fixed Radiation Portal Monitors (RPMs) for nuclear interdiction applications. These versatile and relocatable systems can improve nuclear security in missions or locations that do not warrant or support a standard fixed radiation detection system. Over 2019, a variety of relocatable detectors were characterized at the Interdiction Technologies Integration Laboratory at Pacific Northwest National Laboratory (PNNL). Evaluated detectors were diverse in their size and capabilities, ranging from backpack-sized systems to lane-spanning cargo scanning portals. Both spectroscopic and non-spectroscopic pedestrian and vehicle detection systems were characterized against uranium and plutonium sources. Signatures from the sources were modulated by both shielding and distance to quantify the performance of the relocatable systems as signal strength was decreased. Findings showed that relocatable spectroscopic detectors with isotope identification capabilities could reduce nuisance alarm rates compared to conventional fixed installation, gross-counting, radiation portal monitors. In vehicle scanning applications, detection ability generally trended with detection volume, regardless of spectral capability. In pedestrian scanning applications, several smaller backpack-sized detector systems were found to be more sensitive to detecting material than pedestrian portal monitors. The results of this characterization effort have helped inform the deployment of versatile equipment to improve nuclear security missions.

relocatable detectors, Nuclear Security↗

Active Measurement of Plasma Parameters in Over-Dense MFE Reactor Plasma Using High Frequency Beat-Wave Resonantly Generated Thermal Bernstein Waves

UC Davis was funded to explore the combination of beat-wave excitation and laser scattering to make completely non-invasive determination of local plasma conditions. This involves the use of two high frequency mm-wave sources of differing frequencies (the pump waves) to excite plasma waves at the difference of the frequencies, which is known as the beat frequency. The difference frequency or the frequency of the beat wave is chosen so that we produce plasma waves whose fluctuating electron density is a sensitive function of plasma parameters at the location where the source waves overlap. This fluctuation can be detected from outside the plasma, by measuring the deflection of a probe beam directed at the overlap region between the two pump waves (i.e., collective scattering). This work is an extension of mm-wave frequencies of a 10 GHz beat-wave experiment conducted on the DDT toroidal device (see Fig. 1) in a magnetized plasma where the excited Langmuir wave is replaced by the magnetized upper hybrid wave. Here, two high power (> 1 kW) ~94 GHz pump sources will be employed to match the upper hybrid resonance. The primary envisioned experiment is to drive the electron Bernstein wave (EBW) in the interior of a magnetized plasma. The EBW is a hot-plasma electrostatic wave, which cannot propagate in vacuum. Roots of the EBW dispersion relation occur at frequencies slightly higher than harmonics of the electron cyclotron frequency. Use of the EBW has particular advantages for measuring plasma magnetic field in plasmas with relatively high density and low magnetic field, as is the case in spherical tokamaks. This is the “over dense” condition of future efficient high beta magnetic confinement fusion reactors such as the spherical tokamak (STs). The overarching goal of the proposed project is to demonstrate beat wave EBW excitation in low density and temperature parameters that are directly scalable to over-dense spherical tokamaks such as NSTX or MAST, where measurement of magnetic field by electron cyclotron emission (ECE) is experimentally complex, and requires models of plasma profiles in order to interpret results. In such experiments, availability of point measurements of magnetic field strength provided by a beat-wave diagnostic would serve as a powerful independent check on the ECE results, serving to validate the assumed profiles and wave-propagation models used. The first step was to assemble/modify the target chamber in which the beat-wave plasma experiments will take place. Here, the target chamber of the CTIX compact-toroid (spheromak) injector was chosen. At the time that the proposal was submitted, the aim was to conduct the experiments in the CTIX experimental facilities located at the Livermore campus of UC Davis using microwave/mm-wave equipment brought from the main campus., However, by the time DoE funds for this project were awarded, the CTIX experimental facilities located at the Livermore campus of UC Davis were in the process of being shut down due to the closure of the Livermore campus by Lawrence Livermore National Laboratory (LLNL). Consequently, the equipment needed for this project was crated up and shipped from Livermore to Davis as part of the laboratory shutdown after space on campus was secured and College of Engineering approval secured. Once it arrived in Davis on December 20, 2018, work on the project began in earnest with the initial efforts directed toward developing a new plasma target source. Because of the shutdown of the CTIX facility, the scope of the project thus had to be reduced due to the abbreviated amount of time allocated to the project once the shutdown/move had been completed. Chamber modifications have been completed, including the fabrication and installation of a 38 GHz interferometer, as described in Sec. 3. The thermionic plasma source has been tested and characterized. The magnetic field required for the EBW experiments will be generated by permanent magnets mounted on plates positioned above and below the chamber. Magnetic simulations have been performed, and show that a 3-ring magnet arrangement on each plate, with a plate separation of 50 cm, is required to achieve the ~100 G uniform magnetic field in the interaction region that we feel is necessary to ensure good EBW coupling. We proved unable to successfully revive either of Prof. Luhmann’s two high power (≥20 kW) 94 GHz millimeter-wave sources after their extended time in storage and decided to postpone further efforts and concentrate on slightly lower power sources. Consequently, we were successful in reviving a ~2 kW extended klystron amplifier (EIK), which together with a ~2 kW extended interaction oscillator (EIO) will provide the two pump sources required for the project. Safe operation of the EIO requires extensive modifications to one of Prof. Luhmann’s pulse modulators - these modulator modifications are ongoing, which has unfortunately delayed the planned beat-wave experiments. Details of this work are provided in Sec. 3. Even though project funding has now ended, we still plan to proceed to complete the EIO pulse modulator modifications, install the two ~94 GHz pump wave sources on the target chamber, and conduct unmagnetized tests of the beat-wave concept which involve coupling to unmagnetized electron plasma waves rather than magnetized EBWs. Should these experiments prove successful, we plan to submit a follow-up proposal for additional funding which would allow us to undertake the magnetized EBW experiments.

42 ENGINEERING↗

OSO-7 observations of the X-ray nova 3U 1543-47

The intensity and spectrum of the transient X-ray source 3U 1543-47 were measured by X-ray detectors on the OSO-7 satellite on 13 occasions between November 1971 and December 1972. The results, together with observations of the same object by the Vela and Uhuru satellites, can be described in terms of four qualitatively distinct phases in the X-ray light curve: (1) outburst; (2) relatively steady intensity and spectrum; (3) rapid decrease in intensity and decrease in apparent temperature; and (4) irregular intensity fluctuations with complex spectra. The term 'X-ray nova' is proposed to characterize this and similar transient sources, and a new model for such X-ray novae is proposed.

Li, F. K.↗

Characterizing Wildfires in Western US.: A Cloud-based Case Study for Interdisciplinary Research using NASA Resources

This presentation will demonstrate a case study of interdisciplinary research done in the Amazon Web Services (AWS) cloud platform, in addition to in the local machine. We conduct data analysis next to data by leveraging various cloud-based data in NASA Earthdata Cloud, which are distributed by different missions/NASA Distributed Active Archive Centers (DAACs), and cloud computing resources at NASA. For instance, we directly access multiple datasets stored in the AWS Simple Storage Service (S3) buckets using a Python Jupyter notebook through a JupyterHub interface hosted in AWS (without having to download data), and conduct data analysis next to data in the cloud. We will also show how to share the research results following Open Source policy. This case study characterizes the change in wildfire events in the western United States during the past 20 years. In particular, we focus on the wildfires in California in 2021, one of the most severe wildfire years occurring in the most recent 20 years in California. We will analyze the possible causes of wildfires, such as drought conditions and climate variability, and examine the impacts of wildfires on air quality and atmospheric composition, and on land cover. We will examine the data distributed by the NASA Goddard Earth Sciences Data and Information Services Center (GES DISC), including aerosols and meteorological data from the NASA Modern-Era Retrospective analysis for Research and Applications version 2 (MERRA-2), precipitation from the Global Precipitation Measurement (GPM) and Global Precipitation Climate Project (GPCP), and aerosol index from Ozone Monitoring Instrument (OMI). We also utilize the data distributed by the Physical Oceanography (PO) DAAC, such as Sea Surface Temperature (SST) data from the Group for High Resolution Sea Surface Temperature (GHRSST), and the data distributed by Land Processes (LP) DAAC, such as Normalized Difference Vegetation Index (NDVI).

Xiaohua Pan↗

Discovery of intrinsic linear polarization in SS433

Observations of variable linear polarization in the optical range in the unique radio and X-ray source SS 433, which is characterized by moving emission lines in its visible and near-IR spectra, are reported. The observations were made with an unfiltered GaAs photocathode covering the spectral region 3000-9000 A, with a passband characteristic wavelength near 7000 A. Measurements reveal the presence of both a long-term and a very short time-scale variation in linear polarization in the continuum and in H-alpha, which indicate that a substantial fraction of the polarization is intrinsic to SS 433 and not produced in the interstellar medium. It is suggested that the most likely source of polarization in the optical continuum is electron scattering, and constraints on models of SS 433 implied by the discovery of intrinsic polarization are considered.

Mclean, I. S.↗

X-ray diagnostics for the cavity-based x-ray free-electron laser project

The success of x-ray free-electron lasers (XFELs) in recent years has greatly advanced many scientific fields. However, most of these XFELs suffer from a low longitudinal coherence and instabilities due to the stochastic start-up process. A cavity-based x-ray free-electron laser (CBXFEL) is a possible future direction in the development of fully coherent and stable x-ray sources. One of the challenges of a CBXFEL is the requirement for the μ⁢m−sized electron bunches to fully overlap in three dimensions with the circulating μ⁢m−sized x-ray pulses in an x-ray cavity tens or hundreds of meters long. We present here the development of an x-ray diagnostics system for accurate alignment of x-ray beams in the CBXFEL cavity. The system was developed within the framework of a CBXFEL research and development collaboration among Argonne National Laboratory, SLAC National Accelerator Laboratory, and Spring-8. All the designed diagnostic components have been fully characterized at the Advanced Photon Source to demonstrate a capability for sub-μ⁢rad angular and μ⁢m spatial alignment of the CBXFEL cavity.

Free-electron lasers↗

X-ray optics for the cavity-based X-ray free-electron laser

A cavity-based X-ray free-electron laser (CBXFEL) is a possible future direction in the development of fully coherent X-ray sources. CBXFELs consist of a low-emittance electron source, a magnet system with several undulators and chicanes, and an X-ray cavity. The X-ray cavity stores and circulates X-ray pulses for repeated FEL interactions with electron pulses until the FEL reaches saturation. CBXFEL cavities require low-loss wavefront-preserving optical components: near-100%-reflectivity X-ray diamond Bragg-reflecting crystals, outcoupling devices such as thin diamond membranes or X-ray gratings, and aberration-free focusing elements. In the framework of the collaborative CBXFEL research and development project of Argonne National Laboratory, SLAC National Accelerator Laboratory and SPring-8, we report here the design, manufacturing and characterization of X-ray optical components for the CBXFEL cavity, which include high-reflectivity diamond crystal mirrors, a diamond drumhead crystal with thin membranes, beryllium refractive lenses and channel-cut Si monochromators. All the designed optical components have been fully characterized at the Advanced Photon Source to demonstrate their suitability for the CBXFEL cavity application.

47 OTHER INSTRUMENTATION↗

Wind Plant Performance Prediction Benchmark Phase 1 (Technical Report)

Financial risk resulting from the uncertainty associated with developing, owning, and operating wind power plants remains a barrier to reducing the levelized cost of energy (LCOE). On average, modern wind power plants in the U.S. underperform their expected annual energy output by 3.5-4.5% , with many underperforming by over 10%. To compensate for this uncertainty, investors require a larger return on investment (ROI) and apply "knock-down" factors that mask much of the underlying sources of uncertainty. Wind energy projects thus have reduced access to low-cost capital. Furthermore, operating wind plants often take a simple approach to estimating operations & maintenance (O&M) costs (e.g. straight-line estimates based on similar plants), which can eat into profits. To overcome these issues, the wind industry must improve the models they use for estimating wind plant performance and operations. An industry consortium (IC) requested that the National Renewable Energy Laboratory (NREL) lead a Department of Energy (DOE) working group to benchmark the accuracy of wind power plant energy predictions against real operational data. The IC was also motivated by DOE and NREL's potential to characterize systematic energy underperformance, identify sources of uncertainty, and explore root causes. The Wind Plant Performance Prediction (WP3) project was created out of this request, and this report represents the successful completion of Phase 1 of the WP3 project. During the project, wind plant owners provided both pre-construction and operational data to NREL. The pre-construction data was provided to wind resource assessment (WRA) consultants so they could conduct energy yield assessments (EYA). NREL took all of the completed EYAs, along with the operational data, and conducted an operational assessment to benchmark the EYA results against actual operational data. Given the large amounts of sensitive data required for this effort, as well as historical opposition to sharing data within industry, successful completion of Phase 1 represents an unprecedented milestone for industry data sharing. To improve the accuracy and confidence of pre-construction EYAs, wind plant owners and investors need better, more certain, energy yield predictions. The WP3 Benchmark Project is an industry-driven response to this reality. For the first time, industry has taken the important step of working together at scale, sharing valuable operational data with DOE and NREL in order to investigate the sources of bias and uncertainty in these energy estimates. This IC provides wind plant preconstruction and operational data to NREL in an organized and documented fashion and provides guidance and feedback as needed. The IC also provides introspection of the design of experiment, key metrics of success, data challenges, analysis best practices, and quality of results.

17 WIND ENERGY↗

In-orbit operation of Resolve Filter Wheel and modulated X-ray source

The Resolve soft X-ray spectrometer is a high spectral resolution microcalorimeter spectrometer for the X-ray Imaging and Spectroscopy Mission. In the beam of Resolve, there is a filter wheel containing X-ray filters. In the beam, there is also an active calibration source, the modulated X-ray source (MXS), which can provide pulsed X-rays to facilitate gain calibration. The filter wheel consists of six filter positions. Two open positions, one 55 Fe source to aid in spectrometer characterization during the commissioning phase, and three transmission filters: a neutral density filter, an optical blocking filter, and a beryllium filter. The X-ray intensity, pulse period, and pulse separation of an MXS are highly configurable. Furthermore, the switch-on time is synchronized with the spacecraft’s internal clock to give accurate start and end times of the pulses. One of the issues raised during ground testing was the susceptibility of an MXS at high voltage to ambient light. Although measures were taken to mitigate the light leak, the efficacy of those measures must be verified in orbit. Along with an overview of issues raised during ground testing, we will discuss the calibration source and the filter performance in-flight and compare with the transmission curves present in the Resolve calibration database.

X-ray Imaging and Spectroscopy Mission/Resolve↗

Flux and estimated spectra from a low-intensity laser-driven X-ray source

Laser-driven X-rays as probes for high-energy-density physics spans an extremely large parameter space with laser intensities varying by 8 orders of magnitude. We have built and characterized a soft X-ray source driven by a modest intensity laser of 4 × 10 13 W/cm 2 . Emitted X-rays were measured by diamond radiation detectors and a filtered soft X-ray camera. A material-dependence study on Al, Ti, stainless steel alloy 304, Fe, Cu and Sn targets indicated 5-μm-thick Cu foils produced the highest X-ray yield. X-ray emission in the laser direction and emission in the reverse direction depend strongly on the foil material and the thickness due to the opacity and hydrodynamic disassembly time. The time-varying X-ray signals are used to measure the material thinning rate and is found to be ~1.5 μm/ns for the materials tested implying thermal temperature around 0.6 eV. The X-ray spectra from Cu targets peaks at ~2 keV with no emission >4 keV and was estimated using images with eight different foil filters. One-dimensional hydrodynamic and spectral calculations using HELIOS-CR provide qualitative agreement with experimental results. Modest intensity lasers can be an excellent source for nanosecond bursts of soft X-rays.

47 OTHER INSTRUMENTATION↗

Crowd-based spatial risk assessment of urban flooding: Results from a municipal flood hotline in Detroit, MI

Climate change is increasing the frequency and intensity of extreme precipitation events, raising the risk of urban flood disasters. This study uses a crowd-sourced municipal call database to characterize the spatial distribution of flood risk in Detroit, MI. Call data including dates and addresses were obtained from the City of Detroit Department of Public Works for 2021. Calls were mapped and aggregated to census tract counts and merged with neighborhood-level data. Associations of predictors with flood calls were tested using spatial regression models. Flooding calls were located throughout the city but were concentrated in specific areas. Multivariate models of census tract level call counts indicated that increased poverty and Black, immigrant, and older residents were positively associated with flood calls, while increased elevation was associated with protective effects. Longer distances from waste water interceptors were associated with higher risk for calls. Crowd-sourced flood hotline call data can be used for effective spatial flood risk assessment. Though flooding occurs throughout the city of Detroit, infrastructural, neighborhood, and household factors influence flooding extent. Limitations included the self-reported nature of calls. Future modeling efforts might include input from local stakeholders to improve spatial risk assessment.

54 ENVIRONMENTAL SCIENCES↗

Model Simulations of CO2 Transport Using Assimilated Meteorological Fields

The numerical simulation of CO2 transport (and other tracers such as CO, CH4, and biomass burning tracers) in the atmosphere is required to determine the fate of anthropogenic source gases. Estimation of the CO2 exchange between the ocean surface, the terrestrial biosphere, and the atmosphere is of first-order importance to understanding the global carbon cycle and the processes that are most crucial in determining the atmospheric CO2 concentration. Forward transport simulations have been conducted using two-dimensional, time-dependent grids of average surface fluxes (from TRANSCOM) and three-dimensional wind data from a prototype data assimilation system (FV-DAS) run by the Goddard Data Assimilation Office. The objective is to better understand the contribution of meteorological variability to changes in CO2 and other constituents, By accurately accounting for meteorological variability, through use of assimilated winds, we hope to better characterize the distribution of surface sources and sinks (and chemistry where applicable). With assimilated meteorology such chemistry/transport runs provide the basic framework to analyze existing (and proposed) measurement data on a point-by-point, real-time basis. We compare with measured CO2 concentration gradients on a daily, seasonal, regional, and interhemispheric basis to examine the consistency of sources, sinks, and transport formulation. We will also examine the inter-annual variability of atmospheric CO2 due to atmospheric circulation changes using longer runs with assimilated winds.

Kaea, S. R.↗

Synthesis and Characterization of Lignin-grafted-poly(ε-caprolactone) from Different Biomass Sources

Modification of lignin with poly(ε-caprolactone) is a promising approach to valorize industrial low-value lignins and to advance the bioeconomy. We have synthesized lignin grafted poly(ε-caprolactone) (lignin-g-PCL) copolymers via ring-opening polymerization of ε-caprolactone with different types of lignins of varying botanical sources (G-type pine lignin, S/G-type poplar lignin, and C-type Vanilla seeds lignin) and lignin extraction methods (Kraft and ethanol organosolv pulping). The lignin-g-PCL copolymer showed remarkably improved compatibility and dispersion in acetone, chloroform, and toluene in comparison to non-modified lignins. The structure and thermal properties of the lignin-g-PCL were investigated using Fourier-transform infrared spectroscopy (FTIR), 31 P nuclear magnetic resonance (NMR), 2D heteronuclear single quantum correlation (HSQC) NMR, gel permeation chromatography (GPC), and differential scanning calorimetry (DSC). Furthermore, we have found that all the technical lignins were reactive to the copolymerization reaction regardless of their plant source and isolation methods. The molecular weights of the synthesized lignin-g-PCL copolymers were positively correlated with the content of aliphatic lignin hydroxyls, suggesting that the copolymerization reaction tends to occur preferentially at the aliphatic hydroxyls rather than the phenolic hydroxyls of lignin. Thermal analyses of the lignin-g-PCL copolymers were studied, and in general, a reduction of melting temperature and crystallinity percentage in comparison to the neat PCL was observed. However, the thermal behavior of lignin-g-PCL copolymers varied depending on the lignin feedstocks employed in the copolymerization reaction.

59 BASIC BIOLOGICAL SCIENCES↗

Characterization of Spall in Hard Rock from Observations and Simulations of the Source Physics Experiment Phase I

In this work, spall signals from the Source Physics Experiments are presented, analyzed, and modeled for insight to the explosion source. The observed signal is similar in nature to nearby historical nuclear explosions, and the surface force-time history or velocity can be interpreted with the same model. We use the models for peak spall velocity, spalled mass, and spall depth and radius derived from historical nuclear explosions to parameterize the physical force-time history model from Stump (1985) and show that this parameterized model can be used for spall prediction. The spall signal is also investigated with a numerical continuum model that incorporates gravity. Peak velocity and dwell time are well predicted, and the multiple slap-down phases are captured if one includes a weak near-surface layer similar to the geologic observation.

58 GEOSCIENCES↗

Optical Design of the Earth Surface Mineral Dust Source Investigation (EMIT) Imaging Spectrometer

The Earth Surface Mineral Dust Source Investigation (EMIT) instrument is a high fidelity imaging spectrometer developed to characterize surface mineralogy of the Earth’s dust source regions over the spectral range of 380- 2500 nm and spectral sampling of 7.4 nm. EMIT will close the current knowledge gap in dust source mineral composition by collecting over 1 billion high signal-to-noise ratio spectra in this region of our planet. These new measurements will be used in conjunction with state-of-the-art Earth System Models to understand and reduce the uncertainty in the radiative forcing effect of mineral dust aerosols. EMIT will be deployed on the International Space Station that has an orbit that is well suited for measuring the arid land regions of the Earth. The optical design utilizes a Dyson spectrometer to reduce volume and mass for a fast (F/1.8) and wide swath (1240 samples) optical system. An overview of the EMIT optical design, development, and current status are discussed.

Green, Robert O.↗