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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 703 records · Page 39
All sourcesNASA NTRSDOE OSTI
DOE OSTI2017

Superconductivity in three-dimensional spin-orbit coupled semimetals

Here, motivated by the experimental detection of superconductivity in the low-carrier density half-Heusler compound YPtBi, we study the pairing instabilities of three-dimensional strongly spin-orbit coupled semimetals with a quadratic band touching point. In these semimetals the electronic structure at the Fermi energy is described by spin j = 3/2 quasiparticles, which are fundamentally different from those in ordinary metals with spin j = 1/2. For both local and nonlocal pairing channels in j = 3/2 materials we develop a general approach to analyzing pairing instabilities, thereby providing the computational tools needed to investigate the physics of these systems beyond phenomenological considerations. Furthermore, applying our method to a generic density-density interaction, we establish that: (i) The pairing strengths in the different symmetry channels uniquely encode the j = 3/2 nature of the Fermi surface band structure—a manifestation of the fundamental difference with ordinary metals. (ii) The leading odd-parity pairing instabilities are different for electron doping and hole doping. Finally, we argue that polar phonons, i.e., Coulomb interactions mediated by the long-ranged electric polarization of the optical phonon modes, provide a coupling strength large enough to account for a Kelvin-range transition temperature in the s-wave channel, and are likely to play an important role in the overall attraction in non- s -wave channels. Furthermore, the explicit calculation of the coupling strengths allows us to conclude that the two largest non- s-wave contributions occur in nonlocal channels, in contrast with what has been commonly assumed.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2019

High Thermoelectric Power Factor in Intermetallic Co Si Arising from Energy Filtering of Electrons by Phonon Scattering

Intermetallic compounds are usually poor thermoelectrics due to the high electronic densities of states at the Fermi level and concomitantly low Seebeck coefficients. However, intermetallic B20-type CoSi has been experimentally shown to attain remarkably large negative values of the Seebeck coefficient. We provide a theoretical explanation for this surprising fact using state-of-the-art first-principles calculations with explicit treatment of electron-phonon interactions. We find that the unique band structure of CoSi, which has both massless and heavy fermion bands near the Fermi level, facilitates strong scattering of the low-energy electrons by phonons into the heavy band, resulting in effective energy filtering and high thermal voltage. Our study predicts that a very large thermoelectric power factor of 80 μ W cm -1 K -2 or higher is experimentally accessible in the 300–600 K range and highlights a general principle for identifying intermetallic compounds with large thermopower.

36 MATERIALS SCIENCE↗
DOE OSTI2015

FERMI-LAT OBSERVATIONS OF HIGH- AND INTERMEDIATE-VELOCITY CLOUDS: TRACING COSMIC RAYS IN THE HALO OF THE MILKY WAY

It is widely accepted that cosmic rays (CRs) up to at least PeV energies are Galactic in origin. Accelerated particles are injected into the interstellar medium where they propagate to the farthest reaches of the Milky Way, including a surrounding halo. The composition of CRs coming to the solar system can be measured directly and has been used to infer the details of CR propagation that are extrapolated to the whole Galaxy. In contrast, indirect methods, such as observations of γ-ray emission from CR interactions with interstellar gas, have been employed to directly probe the CR densities in distant locations throughout the Galactic plane. In this article we use 73 months of data from the Fermi Large Area Telescope in the energy range between 300 MeV and 10 GeV to search for γ-ray emission produced by CR interactions in several high- and intermediate-velocity clouds (IVCs) located at up to ∼7 kpc above the Galactic plane. We achieve the first detection of IVCs in γ rays and set upper limits on the emission from the remaining targets, thereby tracing the distribution of CR nuclei in the halo for the first time. We find that the γ-ray emissivity per H atom decreases with increasing distance from the plane at 97.5% confidence level. This corroborates the notion that CRs at the relevant energies originate in the Galactic disk. The emissivity of the upper intermediate-velocity Arch hints at a 50% decline of CR densities within 2 kpc from the plane. We compare our results to predictions of CR propagation models.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2025

Non-equilibrium states and interactions in the topological insulator and topological crystalline insulator phases of NaCd4As3

Topological materials are of great interest because they can support metallic edge or surface states that are robust against perturbations, with the potential for technological applications. Here, we experimentally explore the light-induced non-equilibrium properties of two distinct topological phases in NaCd4As3: a topological crystalline insulator (TCI) phase and a topological insulator (TI) phase. This material has surface states that are protected by mirror symmetry in the TCI phase at room temperature, while it undergoes a structural phase transition to a TI phase below 200 K. After exciting the TI phase by an ultrafast laser pulse, we observe a leading band edge shift of >150 meV that slowly builds up and reaches a maximum after ∼0.6 ps and that persists for ∼8 ps. The slow rise time of the excited electron population and electron temperature suggests that the electronic and structural orders are strongly coupled in this TI phase. It also suggests that the directly excited electronic states and the probed electronic states are weakly coupled. Both couplings are likely due to a partial relaxation of the lattice distortion, which is known to be associated with the TI phase. In contrast, no distinct excited state is observed in the TCI phase immediately or after photoexcitation, which we attribute to the low density of states and phase space available near the Fermi level. Our results show how ultrafast laser excitation can reveal the distinct excited states and interactions in phase-rich topological materials.

Angle-resolved photoemission spectroscopy↗
DOE OSTI2014

A hadronic-leptonic model for the Fermi bubbles: Cosmic-rays in the galactic halo and radio emission

We investigate non-thermal emission from the Fermi bubbles in a hadronic model. Cosmic-ray (CR) protons are accelerated at the forward shock of the bubbles. They interact with the background gas in the Galactic halo and create π{sup 0}-decay gamma-rays and secondary electrons through proton-proton interaction. We follow the evolution of the CR protons and electrons by calculating their distribution functions. We find that the spectrum and the intensity profiles of π{sup 0}-decay gamma-rays are consistent with observations. We predict that the shock front is located far ahead of the gamma-ray boundary of the Fermi bubbles. This naturally explains the fact that a clear temperature jump of thermal gas was not discovered at the gamma-ray boundary in recent Suzaku observations. We also consider re-acceleration of the background CRs in the Galactic halo at the shock front. We find that it can significantly affect the gamma-rays from the Fermi bubbles, unless the density of the background CRs is ≲ 10% of that in the Galactic disk. We indicate that secondary electrons alone cannot produce the observed radio emission from the Fermi bubbles. However, the radio emission from the outermost region of the bubbles can be explained if electrons are directly accelerated at the shock front with an efficiency of ∼0.1% of that of protons.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2011

Auxiliary-field quantum Monte Carlo method for strongly paired fermions

We solve the zero-temperature unitary Fermi gas problem by incorporating a BCS importance function into the auxiliary-field quantum Monte Carlo method. We demonstrate that this method does not suffer from a sign problem and that it increases the efficiency of standard techniques by many orders of magnitude for strongly paired fermions. We calculate the ground-state energies exactly for unpolarized systems with up to 66 particles on lattices of up to 27{sup 3} sites, obtaining an accurate result for the universal parameter {xi}. We also obtain results for interactions with different effective ranges and find that the energy is consistent with a universal linear dependence on the product of the Fermi momentum and the effective range. This method will have many applications in superfluid cold atom systems and in both electronic and nuclear structures where pairing is important.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2012

Isospin-Breaking Corrections to Superallowed Fermi Beta Decay in Isospin- and Angular-Momentum-Projected Nuclear Density Functional Theory

Background: Superallowed -decay rates provide stringent constraints on physics beyond the standard model of particle physics. To extract crucial information about the electroweak force, small isospin-breaking corrections to the Fermi matrix element of superallowed transitions must be applied. Purpose: We perform systematic calculations of isospin-breaking corrections to superallowed decays and estimate theoretical uncertainties related to the basis truncation, to time-odd polarization effects related to the intrinsic symmetry of the underlying Slater determinants, and to the functional parametrization. Methods: We use the self-consistent isospin- and angular-momentum-projected nuclear density functional theory employing two density functionals derived from the density-independent Skyrme interaction. Pairing correlations are ignored. Our framework can simultaneously describe various effects that impact matrix elements of the Fermi decay: symmetry breaking, configuration mixing, and long-range Coulomb polarization. Results: Isospin-breaking corrections to the I=0+, T=1 I=0+, T=1 pure Fermi transitions are computed for nuclei from A=10 to A=98 and, for the first time, to the Fermi branch of the I,T=1/2 I, T=1/2 transitions in mirror nuclei from A=11 to A=49. We carefully analyze various model assumptions impacting theoretical uncertainties of our calculations and provide theoretical error bars on our predictions. Conclusions: The overall agreement with empirical isospin-breaking corrections is very satisfactory. Using computed isospin-breaking corrections we show that the unitarity of the CKM matrix is satisfied with a precision of better than 0.1%.

Satula, W.↗
DOE OSTI2019

Unidentified gamma-ray sources as targets for indirect dark matter detection with the Fermi -Large Area Telescope

We report that one of the predictions of the ΛCDM cosmological framework is the hierarchical formation of structure, giving rise to dark matter (DM) halos and subhalos. When the latter are massive enough they retain gas (i.e., baryons) and become visible. This is the case of the dwarf satellite galaxies in the Milky Way (MW) . Below a certain mass, halos may not accumulate significant amounts of baryons and remain completely dark. However, if DM particles are Weakly Interacting Massive Particles (WIMPs), we expect them to annihilate in subhalos, producing gamma rays which can be detected with the Fermi satellite. Using the three most recent point-source Fermi Large Area Telescope (LAT) catalogs (3FGL, 2FHL and 3FHL), we search for DM subhalo candidates among the unidentified sources, i.e., sources with no firm association to a known astrophysical object. We apply several selection criteria based on the expected properties of the DM-induced emission from subhalos, which allow us to significantly reduce the list of potential candidates. Then, by characterizing the minimum detection flux of the instrument and comparing our sample to predictions from the Via Lactea II (VL-II) N-body cosmological simulation, we place conservative and robust constraints on the $\langle$σ v$\rangle$-m DM parameter space. For annihilation via the τ + τ - channel, we put an upper limit of 4 × 10 -26 (5 × 10 -25 ) cm 3 s -1 for a mass of 10 (100) GeV . A critical improvement over previous treatments is the repopulation we made to include low-mass subhalos below the VL\nobreakdash-II mass resolution. Finally, with more advanced subhalo candidate filtering the sensitivity reach of our method can potentially improve these constraints by a factor 3 (2) for τ + τ - (b $\bar{b}$ ) channel.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2020

Competing orders at higher-order Van Hove points

Van Hove points are special points in the energy dispersion, where the density of states exhibits analytic singularities. When a Van Hove point is close to the Fermi level, tendencies towards density wave orders, Pomeranchuk orders, and superconductivity can all be enhanced, often in more than one channel, leading to a competition between different orders and unconventional ground states. In this study we consider the effects from higher-order Van Hove points, around which the dispersion is flatter than near a conventional Van Hove point, and the density of states has a power-law divergence. We argue that such points are present in intercalated graphene and other materials. We use an effective low-energy model for electrons near higher-order Van Hove points and analyze the competition between different ordering tendencies using an unbiased renormalization-group approach. For purely repulsive interactions, we find that two key competitors are ferromagnetism and chiral superconductivity. For a small attractive interaction, we find an unconventional spin Pomeranchuk order, in wich the spin oder parameter winds around the Fermi surface. The supermetal state, predicted for a single higher-order Van Hove point, is an unstable fixed point in our case.

36 MATERIALS SCIENCE↗
DOE OSTI2023

Quarkyonic mean field theory

We discuss mean field theory of quarkyonic matter at zero temperature. We treat the nucleons with contact interactions in mean field approximation, discussing both vector and scalar mean field interactions. We treat the quarks without mean field vector interactions, but allow mass terms to be generated consistently from a scalar mean field consistent with the additive quark model for quark masses. Quarkyonic matter is composed of a shell of nucleons that under-occupy the total available phase space associated with the underlying quark degrees of freedom. Here, the fully occupied Fermi sphere beneath this shell of nucleons at high densities is thought of as quarks, but when this fully occupied distribution of states first appears, although the phase space is filled, the matter is at low density. For the transition between this low density and high density saturated matter, we advocate a dual description of the fully filled Fermi sea in terms of hadrons, and make a phenomenological hypothesis for the equation of state of this matter. We then proceed to an example where the mean field interactions are all vector and only associated with the nucleons, ignoring the effects of mass change associated with the scalar interactions. Except for the effects of Pauli blocking, the nucleons and quarks do not interact. To get a reasonable transition to quarkyonic matter the interaction of the quarks among themselves are assumed to be nonperturbative, and a simple phenomenological relation between quark Fermi energy and density is introduced.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2012

FERMI LARGE AREA TELESCOPE DETECTION OF THE YOUNG SUPERNOVA REMNANT TYCHO

After almost three years of data taking in sky-survey mode, the Fermi Large Area Telescope has detected {gamma}-ray emission toward Tycho's supernova remnant (SNR). The Tycho SNR is among the youngest remnants in the Galaxy, originating from a Type Ia Supernova in AD 1572. The {gamma}-ray integral flux from 400 MeV up to 100 GeV has been measured to be (3.5 {+-} 1.1{sub stat} {+-} 0.7{sub syst}) Multiplication-Sign 10{sup -9} cm{sup -2} s{sup -1} with a photon index of 2.3 {+-} 0.2{sub stat} {+-} 0.1{sub syst}. A simple model consistent with TeV, X-ray, and radio data is sufficient to explain the observed emission as originating from {pi}{sup 0} decays as a result of cosmic-ray acceleration and interaction with the ambient medium.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2014

Interaction-induced backscattering in short quantum wires

We study interaction-induced backscattering in clean quantum wires with adiabatic contacts exposed to a voltage bias. Particle backscattering relaxes such systems to a fully equilibrated steady state only on length scales exponentially large in the ratio of bandwidth of excitations and temperature. Here in this paper we focus on shorter wires in which full equilibration is not accomplished. Signatures of relaxation then are due to backscattering of hole excitations close to the band bottom which perform a diffusive motion in momentum space while scattering from excitations at the Fermi level. This is reminiscent to the first passage problem of a Brownian particle and, regardless of the interaction strength, can be described by an inhomogeneous Fokker-Planck equation. From general solutions of the latter we calculate the hole backscattering rate for different wire lengths and discuss the resulting length dependence of interaction-induced correction to the conductance of a clean single channel quantum wire.

36 MATERIALS SCIENCE↗
DOE OSTI2021

Suppression of antiferromagnetic order and strong ferromagnetic spin fluctuations in Ca(Co 1-x Ni x ) 2-y As 2 single crystals

CaCo 2–y As 2 is a unique itinerant system having strong magnetic frustration. Here, we report the effect of electron doping on the physical properties resulting from Ni substitutions for Co. The single crystals of Ca(Co 1–x Ni x ) 2–y As 2 were characterized by single-crystal x-ray diffraction, energy-dispersive x-ray spectroscopy, magnetization M versus temperature T, magnetic field H, time t, and heat capacity C p (H, T) measurements. The A-type antiferromagnetic (AFM) transition temperature T N = 52 K for x = 0 decreases to 22 K with only 3% Ni substitution and is completely suppressed for x > 0.16. For 0.11 ≤ x ≤ 0.52 strong ferromagnetic (FM) fluctuations develop as revealed by magnetic susceptibility χ(T) = M(T) / H measurements. For x = 0.11 and 0.16 competing AFM and FM interactions result in a reentrant spin-glass behavior below T N , as evidenced by the observations of thermomagnetic hysteresis and magnetic relaxation. Enhanced FM fluctuations are also found for the x = 0.21 and 0.31 crystals, where χ c increases significantly at low T. A large χ anisotropy in these compositions where χ c is up to a factor of two larger than χ ab suggests that the FM spin fluctuations are quasi-1D in nature. Weak ferromagnetic contributions to the magnetization are found at T = 2 K for x = 0.11 –0.31. Heat-capacity Cp(T) measurements reveal the presence of FM quantum spin fluctuations for 0.11 ≤ x ≤ 0.52, where a logarithmic T dependence of Cp(T) / T is observed at low T. Here, the suppression of AFM order by the development of strong FM fluctuations in Ca(Co 1–x Ni x ) 2–y As 2 crystals suggests the presence of a FM quantum-critical point at x ≈ 0.20. Our density-functional theory (DFT) calculations confirm that FM fluctuations are enhanced by Ni substitutions for Co in CaCo 2–y As 2 . The Sommerfeld electronic heat-capacity coefficient is enhanced for x = 0, 0.21, and 0.42 by about a factor of two compared to DFT calculations of the density of states (DOS) at the Fermi energy, suggesting an enhancement of the DOS from electron-phonon and/or electron-electron interactions. The crystals with x > 0.52 do not exhibit FM spin fluctuations or magnetic order at T ≥ 1.8 K, which was found from the DFT calculations to arise from a Stoner transition. Superconductivity is not observed above 1.8 K for any of the compositions. Neutron-diffraction studies of crystals with x = 0.11 and 0.16 in the crossover regime (0.1 ≲ x ≲ 0.2) show no evidence of A-type ordering as observed in the parent compound with x = 0. Furthermore, no other common magnetic structures, such as ferromagnetic (FM), helical stacking of in-plane FM layers, or in-plane AFM structure, are found with an ordered moment greater than the uncertainty of 0.05 μ B per transition-metal atom.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2012

Fermi Large Area Telescope Measurements of the Diffuse Gamma-Ray Emission at Intermediate Galactic Latitudes

The diffuse galactic {gamma}-ray emission is produced by cosmic rays (CRs) interacting with the interstellar gas and radiation field. Measurements by the Energetic Gamma-Ray Experiment Telescope (EGRET) instrument on the Compton Gamma-Ray Observatory indicated excess {gamma}-ray emission {ge}1 GeV relative to diffuse galactic {gamma}-ray emission models consistent with directly measured CR spectra (the so-called 'EGRET GeV excess'). The Large Area Telescope (LAT) instrument on the Fermi Gamma-Ray Space Telescope has measured the diffuse {gamma}-ray emission with improved sensitivity and resolution compared to EGRET. We report on LAT measurements for energies 100 MeV to 10 GeV and galactic latitudes 10{sup o} {le} |b| {le} 20{sup o}. The LAT spectrum for this region of the sky is well reproduced by a diffuse galactic {gamma}-ray emission model that is consistent with local CR spectra and inconsistent with the EGRET GeV excess.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2025

Correlation control of the Mott transition in LaTiO 3 /SrTiO 3 heterostructures

The Mott metal-insulator transition arises from electron-electron interactions determined by the ratio of Coulomb to kinetic energy scales (U/t). While temperature, pressure, and doping can induce Mott transitions, direct control of U in solid-state systems remains largely unexplored, particularly in the inhomogeneous environments of emerging neuromorphic devices, where conductive filaments create complex gradients of local properties. Here we show that interface-induced screening can continuously tune the electron-electron interaction strength U to drive an isothermal Mott transition. Using thickness-graded LaTiO3/SrTiO3 heterostructures, we used diffraction and photoemission spectroscopy to reveal a continuous, isothermal quantum phase transition from a Fermi liquid quasiparticle with incoherent excitations to a Mott insulator with Hubbard bands. The primary determinant of the transition is the enhanced local screening environment, which directly influences the interaction strength U, driving the system metallic. This demonstrates that interface engineering of the local screening environment provides a promising approach to manipulate Mott physics through correlation control, beyond traditional bandwidth or filling approaches.

Electronic and spintronic devices↗
DOE OSTI2019

Search for plasmons in isotropic Luttinger semimetals

Luttinger semimetals include materials like gray tin (α-Sn) and mercury telluride, which are three-dimensional gapless semiconductors having a quadratic band crossing point (QBCP). Due to a growing interest in QBCPs and new experimental efforts, it is essential to study the finite-temperature properties of such systems. In this paper, we investigate the emergence of plasmons in the presence of Coulomb interactions in isotropic Luttinger semimetals, for zero as well as generic nonzero temperatures. When the Fermi level lies right at the QBCP, which is the point where twofold degenerate conduction and valence bands touch each other quadratically, we find that plasmons cannot appear at zero temperature. However, for nonzero temperatures, thermal plasmons are generated. Whether they are long-lived or not depends on the values of temperature, effective electron mass and effective fine-structure constant, and the number of fermion flavors. We also numerically estimate the behavior of the inelastic scattering rate at nonzero temperatures, as a function of energy, where the signatures of the QBCP thermal plasmons show up as a sharp peak. Our results will thus serve as a guide to experimental probes on these systems.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2013

Revisiting heavy ion collisions under the influence of strong magnetic fields

The quark-gluon plasma (QGP) phase refers to matter where quarks and gluons are believed to be deconfined and it probably takes place at temperatures of the order of 150 to 170 MeV. In large colliders around the world (RHIC/BNL, ALICE/CERN, GSI, etc), physicists are trying to convert hadronic matter at these order of temperatures into QGP by looking at non-central heavy ion collisions. Possible experiments towards this search are Au-Au collisions at RHIC/BNL and Pb-Pb collisions at SPS/CERN, where the hadron abundances and particle ratios are used in order to determine the temperature and baryonic chemical potential of the possibly present hadronic matter-QGP phase transition. The magnetic fields involved in heavy-ion collisions, although time dependent and short-lived, can reach intensities higher than the ones considered in magnetars, around 1.7 Multiplication-Sign 10{sup 19} to 10{sup 20} Gauss. In fact, the densities related to the chemical potentials obtained within the relativistic models framework developed in previous works are very low (of the order of 10{sup -3} fm{sup -3}). At these densities the nuclear interactions are indeed very small and this fact made us consider the possibility of free Fermi and Boson gases under the unfluence of strong magnetic fields. We investigate the effects of magnetic fields of the order of 10{sup 18}, 10{sup 19} and 10{sup 20} G through a {chi}{sup 2} fit to some data sets of the STAR experiment. Our results shown that a field of the order of 10{sup 19} G can produce a much better fit to the experimental data than the calculations without magnetic fields.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2013

Shot-noise at a Fermi-edge singularity: Non-Markovian dynamics

For an InAs quantum dot we study the current shot noise at a Fermi-edge singularity in low temperature cross-correlation measurements. In the regime of the interaction effect the strong suppression of noise observed at zero magnetic field and the sequence of enhancement and suppression in magnetic field go beyond a Markovian master equation model. Qualitative and quantitative agreement can however be achieved by a generalized master equation model taking non-Markovian dynamics into account.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗