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At least 703 records · Page 39

Update on Radiation Testing for Space Fission Power Systems

Radiation effects on materials and electronics is a major topic that needs to be addressed for a nuclear reactor flight demonstration of the Kilopower reactor. The Kilopower project team has taken steps towards developing a standardized radiation environment qualification program for components and materials. Candidate nuclear reactor facilities for both low fluence electronics and high fluence materials irradiations have been identified and approached. Collaborations are being pursued with both NASA and external experts to ensure that the results of the qualification testing are appropriate and relevant to nuclear fission power flight systems.

Chaiken, Max F.↗

Measurements of Proton Displacement Damage in Several Commercial Optocouplers

Proton Displacement Damage (DD) measurements on Isolink OLS049, Micropac 66296-101, 66224-103JANTX, and 66179-003 are reported. The 66179-003 has the worst degradation, 13% of the initial CTR remains when it is used with I(sub F) = 10 mA at 1 x 10(exp 12) 1-MeV n/sq.cm fluence in Silicon. The remaining CTR percentage for OLS049, 66296-101, and 66224-103JANTX are 21%, 32%, and 79% at 2 x 10(exp 12) 1-MeV n/sq.cm fluence in Silicon, respectively.

Irom, Farokh↗

A Search for High-Energy Counterparts to Fast Radio Bursts

We report on a search for high-energy counterparts to fast radio bursts (FRBs) with the Fermi Gamma-ray Burst Monitor, Fermi Large Area Telescope, and the Neil Gehrels Swift Observatory Burst Alert Telescope. We find no significant associations for any of the 23 FRBs in our sample, but report upper limits to the high-energy fluence for each on timescales of 0.1, 1, 10, and 100 s. We report lower limits on the ratio of the radio to high-energy fluence, f(sub r) /f(sub γ), for timescales of 0.1 and 100 s. We discuss the implications of our non-detections on various proposed progenitor models for FRBs, including analogs of giant pulses from the Crab pulsar and hyperflares from magnetars. This work demonstrates the utility of analyses of high-energy data for FRBs in tracking down the nature of these elusive sources..

Cunningham, Virginia↗

The Role of Solar Wind Hydrogen in Space Weathering: Insights from Laboratory-Irradiated Northwest Africa 12008

Micrometeoroid impacts, solar wind plasma interactions, and regolith gardening drive the complicated and nuanced mechanism of space weathering (or optical maturation); a process by which a material’s optical properties are changed as a result of chemical and physical alterations at the surface of grains on airless bodies. Reddened slopes, attenuated absorption bands, and an overall reduction in albedo in the visible and near-IR wavelength ranges are primarily the result of native iron nanoparticle (npFe0) production within glassy rims that form from sputtering and vaporization. The sizes and abundance of these particles provide information about the relative surface exposure age of a particular grain. In addition, many studies have indicated that composition greatly affects the rate at which optical maturation occurs. Despite our understanding of how npFe0 affects optical signatures, the relative roles of micrometeoroid bombardment and solar wind interactions remains undetermined. To simulate the early effects of weathering by the solar wind and to determine thresholds for optical change with respect to a given mineral phase, we irradiated a fine-grained lunar basalt with 1 keV H+ to a fluence of 6.4 x 1016 H+ per sq.cm. Surface alterations within four phases have been evaluated using transmission electron microscopy (TEM). We found that for a given fluence of H+, the extent of damage acquired by each grain was dependent on its composition. No npFe(0) was produced in any of the phases evaluated in this study. These results are consistent with many previous studies conducted using ions of similar energy, but they also provide valuable information about the onset of space weathering and the role of the solar wind during the early stages of optical maturation.

Shusterman, M. L.↗

Inclusion of Radiation Environment Variability for Reliability Estimates for SiC Power MOSFETs

Variability of the solar energetic particle environment is investigated for single-event-burnout reliability of silicon-carbide power metal-oxide-semiconductor field effect transistors. A probabilistic assessment of failure evaluates the benefits of de-rating voltage, shielding, and mission length. The Prediction of Solar particle Yields for Characterizing Integrating Circuits code is used to calculate a cumulative density function for the fluence of the environment. The lethal ion method is then used to determine what proportion of the environment will cause single-event-burnout. The operating voltage determines the lowest linear-energy-transfer particle that will cause single-event-burnout and that should be included in the environment distribution. The shielding and mission length also determine the final environment distribution of the mission fluence. Through calculating the reliability for different operating voltages, shielding, and mission length for a specific device, it is shown that shielding thickness and operating voltage have a large effect on reliability and can be traded off during the design.

Heavy ion↗

The Lowest-frequency Fast Radio Bursts: Sardinia Radio Telescope Detection of the Periodic FRB 180916 at 328 MHz

We report on the lowest-frequency detection to date of three bursts from the fast radio burst FRB 180916.J0158+65, observed at 328 MHz with the Sardinia Radio Telescope (SRT). The SRT observed the periodic repeater FRB 180916.J0158+65 for five days from 2020 February 20 to 24 during a time interval of active radio bursting, and detected the three bursts during the first hour of observations; no more bursts were detected during the remaining ∼30 hr. Simultaneous SRT observations at 1548 MHz did not detect any bursts. Burst fluences are in the range 37 to 13 Jy ms. No relevant scattering is observed for these bursts. We also present the results of the multiwavelength campaign we performed on FRB 180916.J0158+65, during the five days of the active window. Simultaneously with the SRT observations, others with different time spans were performed with the Northern Cross at 408 MHz, with XMM-Newton, NICER, INTEGRAL, AGILE, and with the TNG and two optical telescopes in Asiago, which are equipped with fast photometers. XMM-Newton obtained data simultaneously with the three bursts detected by the SRT, and determined a luminosity upper limit in the 0.3–10 keV energy range of ∼10(exp 45) erg/s for the burst emission. AGILE obtained data simultaneously with the first burst and determined a fluence upper limit in the MeV range for millisecond timescales of 10(exp -8) erg/sq.cm. Our results show that absorption from the circumburst medium does not significantly affect the emission from FRB 180916.J0158+65, thus limiting the possible presence of a superluminous supernova around the source, and indicate that a cutoff for the bursting mechanism, if present, must be at lower frequencies. Our multi-wavelength campaign sensitively constrains the broadband emission from FRB 180916.J0158+65, and provides the best limits so far for the electromagnetic response to the radio bursting of this remarkable source of fast radio bursts.

M. Pilia↗

Neutrino Target-of-Opportunity Observations with Space-based and Suborbital Optical Cherenkov Detectors

Cosmic-ray accelerators capable of reaching ultra-high energies are expected to also produce very high energy neutrinos via hadronic interactions within the source or its surrounding environment. Many of the candidate astrophysical source classes are either transient in nature or exhibit flaring activity. Using the Earth as a neutrino converter, suborbital and space-based optical Cherenkov detectors, such as POEMMA and EUSO-SPB2, will be able to detect upward-moving extensive air showers induced by decaying tau-leptons generated from cosmic tau neutrinos with energies ∼ 10 PeV and above. Both EUSO-SPB2 and POEMMA will be able to quickly repoint, enabling rapid response to astrophysical transient events. We calculate the transient sensitivity and sky coverage for both EUSO-SPB2 and POEMMA, accounting for constraints imposed by the Sun and the Moon on the observation time. We also calculate both detectors’ neutrino horizons for a variety of modeled astrophysical neutrino fluences. We find that both EUSO-SPB2 and POEMMA will achieve transient sensitivities at the level of modeled neutrino fluences for nearby sources. We conclude with a discussion of the prospects of each mission detecting at least one transient event for various modeled astrophysical neutrino sources.

Tonia M Venters↗

Solar Absorptivity Degradation of Spacecraft Materials Due to UV and Charged Particles in the Gateway Environment

The Gateway Passive Thermal Control System (PTCS) Group has identified charged particle and UV degradation of Gateway materials as a knowledge gap for the Near Rectilinear Halo Orbit (NRHO) and transit environment. Candidate materials and coatings were subjected to expected mission UV and charged particle environments at NASA Goddard Space Flight Center (GSFC). In situ change in reflectivity was observed at specified intervals during testing such that change in solar absorptivity could be plotted as a function of time of solar exposure. Gateway will be an outpost in cislunar space designed to survive a 15-year mission to support human moon landings and future deep space exploration. The Gateway Passive Thermal Control System (PTCS) Group has identified charged particle and UV degradation of potential Gateway materials as a knowledge gap for the Near Rectilinear Halo Orbit (NRHO) and transit environment, especially the slow spiral transit planned for the first two modules. Solar absorptivity degradation is important to quantify because the end-of-life absorptivity impacts thermal performance of the system. To address this, ground testing is being completed at NASA Goddard Space Flight Center in which potential Gateway materials, including radiators, multi-layer insulation (MLI), and structural materials are subjected to the expected transit plus 15-year on-orbit charged particle fluence (9.86x1015 protons/cm2 at 2.5 keV and 3.1x1016 electrons/cm2 at 10 keV) and up to 5000 Equivalent Solar Hours (ESH). Reflectivity of a single sample of each material was measured in atmosphere and in vacuum inside the chamber after exposure to incremental levels of ESH and charged particle fluence. Increase in absorptivity of most samples were seen throughout the test including large differences in absorptivity of materials of the same category. Future testing will validate these results and include additional materials of interest.

materials in the space environment↗

Dragonfly mass spectrometer titan environment optical damage testing

The Dragonfly Mass Spectrometer (DraMS) being developed at NASA’s Goddard Space Flight Center will use a solid-state 266-nm pulsed Nd:YAG laser perform compositional analysis on the surface of Titan. Due to the high fluence of the focused pulse energy on the laser’s beam steering unit (BSU) and the mass spectrometer window, the damage threshold of these optics in a Titan atmosphere needed to be characterized. This paper details the test setup and the successful demonstration of testing the highest fluence optics for the expected mission duration of 2 million laser pulses in a Titan-relevant atmosphere.

Matt Mullin↗

Damage Threshold Testing of UV Optics Under a Titan Environment for NASA’s Dragonfly Mission

The Dragonfly Mass Spectrometer (DraMS) being developed at NASA’s Goddard Space Flight Center will use a solid-state 266-nm pulsed Nd:YAG laser to perform compositional analysis on the surface of Titan. Due to the high fluence of the focused pulse energy on the laser’s beam steering unit (BSU) and the mass spectrometer window, the damage threshold of these optics in a Titan atmosphere needed to be characterized. This paper details the test setup and the successful demonstration of testing the highest fluence optics for the expected mission duration of 2 million laser pulses in a Titan-relevant atmosphere.

Paul R Stysley↗

Solar Absorptivity Degradation of Spacecraft Materials Due to UV and Charged Particles in the Gateway Environment

Gateway will be an outpost in cislunar space designed to survive a 15-year mission to support human Moon landings and future deep space exploration. The Gateway Passive Thermal Control System (PTCS) Group has identified charged particle and UV degradation of potential Gateway materials as a knowledge gap for the Near Rectilinear Halo Orbit (NRHO) and transit environment, especially the slow spiral transit planned for the first two modules. Solar absorptivity degradation is important to quantify because the end-of-life absorptivity impacts thermal performance of the system. To address this, ground testing has been completed at NASA Goddard Space Flight Center in which potential Gateway materials, including radiators, multi-layer insulation (MLI), and structural materials are subjected to the expected transit plus 15-year on-orbit charged particle fluence (9.86x1015 protons/cm2 at 2.5 keV and 3.1x1016 electrons/cm2 at 10 keV) and 5093 Equivalent Solar Hours (ESH). Reflectivity of a single sample of each material was measured in atmosphere and in vacuum inside the chamber after exposure to incremental levels of ESH and charged particle fluence. Increase in absorptivity of most samples were seen throughout the test including large differences in absorptivity of materials of the same category. Future planned testing will validate these results and include additional materials of interest.

Optical Property↗

Trace Elemental Abundances in Calcium-Aluminum-Rich Inclusions in CV Chondrites

Introduction: Calcium-aluminum-rich inclusions (CAIs), are the first formed solids that define the age of the Solar System [1,2]. CAIs are thought to have condensed from nebular gas [3,4] within the first <1 Ma of Solar System formation [5,6]. CAIs have experienced numerous early Solar System processes including condensation, evaporation, melting, recrystallization, and aqueous alteration [e.g., 7]. The chemical, mineralogical, and textural diversity among CAIs results from a range of chemical and physical processes recorded during nebular and parent body epoch. This study aims to explore the mineralogical, textural, and chemical compositions of CAIs including the trace elemental abundances in CAI phases to determine the early Solar System processes recorded in them. Samples and Analytical Methods: We analyzed one CAI each from CV3 chondrites Northwest Africa (NWA) 5508 designated as ‘Saguaro’, and Northwest Africa (NWA) 12772 designated as ‘Hoopoe’. Back-scatter electron (BSE) images were collected using a Phenom XL scanning electron microscope (SEM) at the Lunar and Planetary Institute (LPI) and the JEOL JXA-8530F electron probe microanalyzer (EPMA) at Johnson Space Center (JSC)-NASA. Additionally, energy dispersive X-ray spectrometry (EDS) elemental maps of select areas for these samples were collected using a 15.0kV beam energy and a 40µA emission current. Using the EPMA, wavelength-dispersive X-ray spectroscopy (WDS) quantitative data were collected. In-situ trace element measurements for both CAIs were determined at JSC-NASA using a Photon Machines 193nm laser ablation system and a Thermo-Scientific Element-XR inductively coupled plasma mass spectrometer (ICP-MS). Analyses consisted of 30s ablations at 10Hz, spot sizes of 20-25µm, and a fluence of 6.0 J/cm2 for anorthite and melilite, and a 3.5 J/cm2 fluence for all other phases. NIST612 was used to correct for instrument drift, while BHVO-2g was used as a primary calibration standard. BCR-2g and in-house mineral standards were regularly measured as unknowns to ensure accuracy. Results: Saguaro is a coarse-grained CAI, ~11 x 6 mm in dimensions. Saguaro contains spinel, Al-rich pyroxene, anorthite, Mg-rich melilite, and minor perovskite in its interior and is therefore classified as a Type B CAI. Individual melilite grains shows normal compositional zoning with an Ak content ranging from ~24 to 54 with no apparent trend from the core to the edge of the CAI. The spinel appears euhedral and occurs both as clusters and as spinel palisades [8]. Two rim sequences surround most of the sample: the inner rim being a Wark-Lovering (WL) rim (~10-35 µm) containing pyroxene, spinel, and melilite (or anorthite), and the outer rim is a finer-grained, thicker (~100 µm), accretionary rim (Fig. 1). The mineral phases in Saguaro record an overall flat REE pattern with an average negative Eu anomaly in pyroxene, and an average positive Eu anomaly in anorthite and melilite respectively. Anorthite, melilite, and pyroxene have a minor depletion in Tm (Fig. 2). The Hoopoe CAI is a compact, coarse-grained ~6 × 4 mm in size. The major mineralogy includes hibonite, spinel, melilite, anorthite, and perovskite. Therefore, it is classified as a compact transitional type A and B. (?)zoning was observed in some hibonites. Individual melilite grains show both reverse and normal zoning, where the Ak content ranges from ~6- to 28. Melilite shows two distinct textures. One texture consisted of smooth melilite that appeared homogenous, while the second appeared to consist of many fine fractures. The spinel also often appears clustered. The WL-rim sequence surrounding Hoopoe is ~25 µm thick and composed of spinel, perovskite, hibonite, and melilite/anorthite. It is then partially surrounded by an outer accretionary rim (~75µm). Like before, refractory metal nuggets appeared concentrated near the WL rims. Other metal assemblages rich in Fe and Ni were also observed. All major mineral phases in Hoopoe display relatively flat REE patterns, except for varying Eu and Tm between phases (Fig. 2). There is a prominent negative Eu anomaly in perovskite and an average positive Eu anomaly in spinel, anorthite, and hibonite respectively (Fig. 2, 3). The mixed phases along the rim of the CAI also display a negative Eu anomaly, and all phases the CAI were depleted in Pb. Discussion: The CV3 CAIs analyzed in this study were classified based on their mineralogy and textures into Type A versus Type B CAIs [10]. Hibonite appears to be pseudomorphically replacing the spinel, (i.e., is hibonite in composition, but appears in the shape of spinel). Spinel palisades. The presence of spinel palisades present in Saguaro are consistent with the melting and recrystallization experienced by this CAI. Trace elemental analyses. Saguaro and Hoopoe display similar trace element patterns to each other, with both appearing generally flat, with anomalies in Eu, and Tm. Melilite and anorthite display positive Eu anomalies in both CAIs, in addition to the hibonite in Hoopoe (Fig. 2). The phases that are depleted in Eu are pyroxene and perovskite in both Saguaro and Hoopoe, respectively (Fig. 3). Given that Eu is volatile in reducing environments [11], this could possibly indicate reducing conditions at the time anorthite and melilite crystallized, with the gas they formed from containing Eu. As these CAIs continued to form, this gas as a result would become depleted in Eu. This also could be supported by the propensity of anorthite and melilite to take up Eu from its surroundings and incorporate it into their structure [12]. In addition, analyzing the assemblage of the phases in the Saguaro, melilite and anorthite (Eu enriched) often surround the pyroxene (Eu depleted) as they are crystallized. This intergrowth of phases and the proximity of the phases would support that the Eu is being incorporated into some phases, preventing it from incorporating into other. Trace elemental analyses of the CAI rims will be evaluated in more detail, as they are complicated by the transient signal being composed of a mixture of mineral phases. Broadly, however, the patterns in the rims of both CAIs are comparable to each other, and for Hoopoe, to the mixed phase patterns in the core (Fig. 3). Other studies have found that CAI rims can be depleted in Ce and Yb [13], however we did not observe these anomalies in the two CAIs discussed here. Given their similarity, the trace elemental analyses of the mixed interior (i.e. core) and rim phases could be interpreted as forming from similar, if not the same, reservoirs. The REE abundance between the rim and core of Hoopoe are also similar, indicating they may have formed from a gas of the same or similar composition. Acknowledgments: We thank the ASU Center for Meteorite Studies for loaning the samples used in this work and Tabb Prissel for his assistance with the analysis. Mouti Al-Hashimi thanks Sam Crossley and Cyrena Goodrich for their help with the LPI SEM training. This work was supported by the LPI Summer Intern Program in Planetary Science and the LPI Cooperative Agreement. References: [1] Connelly J.N. (2012) Science, 338, 651-655. [2] MacPherson G. J. (2014) Treatise on Geochem., 2, 139-179. [3] Grossman L. (1972) GCA, 36, 597-619. [4] Ebel, D.S. (2006) Meteorites and the Early Solar System II (D. S. Lauretta & H. Y. McSween, Eds.) 253-277. [5] MacPherson G. J. (2012) Earth Planet. Sci. Lett., 331-332, 43-54. [6] MacPherson G.J. (2017) GCA, 201, 65-82. [7] Krot A.N. (1995) Meteoritics & Planet. Sci., 30, 748-775. [8] Wark and Lovering (1982) GCA, 46, 2595-2607. [9] Palme H. and Jones A. (2003) Treatise on Geochemistry (H. D. Holland and K. K. Turekian Eds.), 1, 41-61. [10] Grossman L. (1980) Ann. Rev. Earth Planet. Sci., 8, 559-608. [11] Floss C. et al. (1996) GCA, 60, 1975-1997. [12] Mason B. and Martin P. M. (1974) Earth Planet. Sci. Lett., 22, 141-144. [13] Wark B. and Boynton W. V. (2001) Meteoritics & Planet. Sci., 36, 1135-1166.

X Mouti↗

Space Environmental Exposure of the MISSE 9-15 Polymers and Composites Experiment 1-4 (PCE 1-4)

Spacecraft in low Earth orbit (LEO) are subjected to harsh environmental conditions, including radiation (cosmic rays, ultraviolet (UV), x-ray and charged particle radiation), micrometeoroids and orbital debris, temperature extremes, thermal cycling, and atomic oxygen (AO). These environmental exposures can result in erosion, embrittlement and optical property degradation of susceptible materials threatening spacecraft performance and durability. To increase our understanding of effects such as AO erosion and radiation induced embrittlement of spacecraft materials, NASA Glenn Research Center has developed a series of experiments that were flown as part of the Materials International Space Station Experiment (MISSE) missions on the exterior of the International Space Station (ISS). These experiments have provided critical space environmental durability data such as AO erosion data of polymers and composites, and radiation induced mechanical property degradation of spacecraft insulation materials, after long term space exposure. Recently, four Glenn experiments with 365 flight samples were flown on ISS’s MISSE-Flight Facility (MISSE-FF). These experiments are the Polymers and Composites Experiment-1 (PCE-1) flown as part of the MISSE-9 mission, the PCE-2 flown as part of the MISSE-10 mission, the PCE-3 flown as part of the MISSE-12 and MISSE-15 missions, and the PCE-4 flown as part of the MISSE-13 mission. This paper provides details on the space environment exposure of Glenn’s PCE 1-4 flight samples. Passive samples were flown in each flight orientation for post-flight AO fluence determination and on-orbit contamination analyses. Solar exposure estimates were computed by Aegis Aerospace, Inc. The environment exposure details include the total space vacuum duration, time on the MISSE-FF, the direct space exposure duration, the AO fluence and the computed mission Equivalent Sun Hours (ESH) solar exposure. Typical on-orbit temperatures are also provided along with a summary of analyses of PCE 1-4 contamination witness samples. Knowledge of the space environmental exposure of the PCE 1-4 flight samples is crucial for flight data interpretation.

Atomic oxygen↗

As-Run Physics Analysis for the AGC-4 Experiment Irradiated in the ATR

This Engineering Calculations Analysis Report (ECAR) documents the results of the Advanced Test Reactor (ATR) detailed physics analyses performed to calculate the displacements per atom (DPA) and the fast neutron fluence (E > 0.1 MeV) of the Advanced Graphite Creep (AGC) experiment, AGC-4, irradiated in the ATR East Flux Trap (EFT) (see Figure 1) during ATR Cycle 157D, 158A, 162A, 162B, 164A, 164B, 166A, and Cycle 166B. This ECAR also reports the neutron and photon heat rates for the materials of the AGC-4 experiment for ATR Cycle 158A (timestep 19), which provides to the maximum heating. The results for these evaluations and analysis are reported herein. The AGC-4 as-run specimen neutron fast fluence (E > 0.1 MeV), DPA, and material heat rate calculations were performed using a general-purpose Monte Carlo N-Particle (MCNP) code. All calculated results are tabulated herein.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

AGR-5/6/7 Irradiation As Run Predictions Using PARFUME

The PARticle FUel ModEl (PARFUME), a fuel performance modeling code used for high-temperature gas-cooled reactors, was used to model the Advanced Gas Reactor (AGR)-5/6/7 irradiation test using as-run physics and thermal data. The AGR-5/6/7 irradiation test consists of the combined fifth, sixth, and seventh planned irradiations of the AGR Fuel Development and Qualification Program. The AGR-5/6/7 test train is a multi-capsule, instrumented experiment that is designed for irradiation in the 133.4-mm diameter northeast flux trap position of the Advanced Test Reactor (ATR) at Idaho National Laboratory. Each capsule contains compacts filled with uranium oxycarbide unaltered fuel particles. This report documents the calculations performed to predict the failure probability of tristructural isotropic (TRISO)-coated fuel particles during the AGR-5/6/7 experiment. In addition, this report documents the calculated fission product release fraction from the fuel. The calculations include modeling of the AGR 5/6/7 irradiation that occurred from February 2018 to July 2020 over nine ATR cycles, including six normal cycles and three power axial locator mechanism cycles, for a total of approximately 376 effective full power days (EFPD). The irradiation conditions and material properties of the AGR-5/6/7 test predicted zero fuel particle failures in Capsules 1, 3, and 4. Fuel particle failures were predicted in two of the compacts in Capsule 2 and one particle failure is predicted in each one of the compacts in Capsule 5. All compacts that exhibited fuel particle failures predicted by PARFUME were caused by localized stress concentrations in the silicon carbide (SiC) layer caused by cracking in the inner pyrolytic (IPyC) layer. In addition, shrinkage of the buffer and IPyC layer during irradiation resulted in formation of a buffer-IPyC gap. Compacts with a lower irradiation temperature and fluence experienced the smallest buffer-IPyC gap formation. Conversely, higher irradiated temperature compacts with a high fluence experienced the largest buffer-IPyC gap formation. Compact 3-6-3 experienced the largest buffer IPyC gap formation of just under 21.7 µm. The release fraction of fission products silver (Ag), cesium (Cs), and strontium (Sr) vary depending on capsule location and irradiation temperature. The maximum release fraction of Ag occurs in Capsule 3, reaching up to 59.5% for the TRISO fuel particles (compact 3-6-3). The release fraction of the other two fission products, Cs and Sr, are much smaller. A maximum Cs release fraction of 1.1% occurred in compact 3-4-3 and 4.4% for Sr in compact 3-6-3.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Advanced Graphite Creep Uncertainty Analysis

Radiation damage estimation is an important component of the post irradiation analysis of the Advanced Graphite Creep (AGC) experiment. It depends primarily on the fast fluence, which is determined using well established methods of spectral adjustment. These are based on best estimates from models such as Monte Carlo N-Particle (MCNP), input cross-sections, and measured activities from flux wires in the experiment. Each of these parameters can propagate uncertainties which will affect the uncertainty in the calculated dose levels for AGC, or any experiment irradiated within a reactor. While the methods of propagating uncertainty are well-established, the final uncertainty estimates they provide are only as good as the estimates of uncertainty in the inputs on which they are based. The purpose of this work is to outline some deficiencies in the ways these input uncertainties are presently estimated, and to outline a methodology by which they can be improved. The fast fluence and radiation damage received by graphite specimens irradiated in the Advanced Graphite Creep (AGC) experiments is presently estimated using spectral adjustment methods that are based on both flux wire activity measurements, and MCNP model predictions. This work describes an ongoing effort to quantify and propagate uncertainties in inputs to the spectral adjustment process, and thereby quantify the resultant error in radiation damage (dpa) estimates. The effort is multi-faceted, and we consider the impacts of both the set of flux wires selected, and the counting process. An expanded set of flux wires is identified that provides a more comprehensive data set on the fast spectrum. To address the counting process itself, a series of round-robin measurements in several reactor metrology laboratories across the Department of Energy (DOE) complex and nuclear industry are being undertaken to refine the American Society for Testing and Materials (ASTM) standards for flux wire measurements. To address the contribution of uncertainty in the MCNP model predictions, an uncertainty quantification (UQ) tool has been developed that statistically samples the model input parameters, runs a series of cases, and assimilates the results to provide an overall uncertainty. The impact of the MCNP UQ tool results is demonstrated by re-analyzing previous AGC flux wire and irradiation data. While the expanded flux wire set obviously cannot be added to these experiments retroactively, plans for future graphite irradiations are outlined.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

System and method for ablation assisted nanostructure formation for graded index surfaces for optics

A system and method is disclosed for forming a graded index (GRIN) on a substrate. In one implementation the method may involve applying a metal layer to the substrate. A fluence profile of optical energy applied to the metal layer may be controlled to substantially ablate the metal layer to create a vaporized metal layer. The fluence profile may be further controlled to control a size of metal nanoparticles created from the vaporized metal layer as the vaporized metal layer condenses and forms metal nanoparticles, the metal nanoparticles being deposited back on the substrate to form a GRIN surface on the substrate.

Yoo, Jae Hyuck↗

Modernization of the Radiation Measurements Laboratory at the Advanced Test Reactor Complex

The Advanced Test Reactor (ATR) at the Idaho National Laboratory (INL) is a unique, water-cooled, high-flux test reactor capable of performing tests prototypical of PWR operating conditions. The Radiation Measurements Laboratory (RML) was founded in the 1960s to support reactor operations and to conduct independent scientific research. For nearly six decades RML has performed four primary functions: monitoring of radioactivity by gamma-ray spectroscopy of routine reactor samples, fluence rate determinations for irradiation cycles, fission-rate measurements for the ATR-Critical (ATR-C) Facility, and independent research and development of radiation detection systems and applications. Through the decades, RML has seen technological advancements that have been integrated into each of the critical functions of the laboratory. However, many of the measurement and analysis systems employed to this day can be improved by modernization. Recent progress at RML is improving reliability and accuracy of the radiation measurements performed in support of nuclear energy research for the U.S.A. Department of Energy. The control and data collection systems supporting ATR-C have been upgraded. New High-Purity Germanium (HPGe) spectrometers have been procured with liquid nitrogen recycling capabilities to improve up-time and reduce measurement uncertainties. Fluence-rate measurement techniques are also being improved to ensure accuracy, avoid systemic errors, and identify biases. In a parallel effort, new scientific research avenues are being explored which will provide an opportunity to further enhance the utilization of ATR and ensure the sustainability of the RML as nuclear research continues to evolve. The RML is improving the effectiveness of irradiation services provided by ATR while ensuring a sustainable future for nuclear energy research.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗