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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 703 records · Page 39
All sourcesNASA NTRSDOE OSTI
DOE OSTI2016

Low-energy enhancement in the γ -ray strength functions of Ge 73 , 74

Here, t≤he γ-ray strength functions and level densities of 73,74 Ge have been extracted up to the neutron-separation energy S n from particle-γ coincidence data using the Oslo method. Moreover, the γ-ray strength function of 74 Ge above S n has been determined from photoneutron measurements; hence these two experiments cover the range of Eγ ≈ 1–13 MeV for 74 Ge. The obtained data show that both 73,74 Ge display an increase in strength at low γ energies. The experimental γ-ray strength functions are compared with M1 strength functions deduced from average B(M1) values calculated within the shell model for a large number of transitions. The observed low-energy enhancements in 73,74 Ge are adopted in the calculations of the 72,73 Ge(n,γ) cross sections, where there are no direct experimental data. Calculated reaction rates for more neutron-rich germanium isotopes are shown to be strongly dependent on the presence of the low-energy enhancement.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2017

Measurement of the Bi 209 ( n , 4 n ) Bi 206 and Tm 169 ( n , 3 n ) Tm 167 cross sections between 23.5 and 30.5 MeV relevant to reaction-in-flight neutron studies at the National Ignition Facility

At the National Ignition Facility, experiments are being performed to measure charged-particle stopping powers in the previously unexplored warm dense plasma regime. These measurements are done using reaction-in-flight (RIF) neutrons from an inertial confinement fusion system. RIF neutrons are produced with a continuum of energies up to 30 MeV. By making activation measurements utilizing threshold reactions for neutrons in the energy range of 15 < E n < 30 MeV , the number of RIF neutrons can be determined and from this the stopping power of the deuterium and tritium ions that produced the RIF neutrons can be inferred. Currently, the 169 Tm ( n , 3 n ) 167 Tm reaction has been used. However, in an effort to provide a secondary complimentary measurement, efforts are underway to make use of the 209 Bi ( n , 4 n ) 206 Bi reaction, with a threshold of 22.5 MeV. The cross sections were measured at the 10 MV tandem Van De Graaff accelerator at the Triangle Universities Nuclear Laboratory with quasimonoenergetic neutrons between 23.5 and 30.5 MeV, where few previous measurements have been made. Cross-section data are compared to calculations and other available measurements.

42 ENGINEERING↗
DOE OSTI2018

Accurate measurement of the first excited nuclear state in U 235

In this paper, we have used superconducting high-resolution radiation detectors to measure the energy level of metastable $^{235m}\mathrm{U}$ as 76.737 ± 0.018 eV. The $^{235m}\mathrm{U}$ isomer is created from the α decay of $^{239}\mathrm{Pu}$ and embedded directly into the detector. When the $^{235m}\mathrm{U}$ subsequently decays, the energy is fully contained within the detector and is independent of the decay mode or the chemical state of the uranium. The detector is calibrated using an energy comb from a pulsed UV laser. Finally, a comparable measurement of the metastable $^{229m}\mathrm{Th}$ nucleus would enable a laser search for the exact transition energy in $^{229}\mathrm{Th}{-}^{229m}\mathrm{Th}$ as a step towards developing the first ever nuclear (baryonic) clock.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2017

Sensitivity and discovery potential of nEXO to neutrinoless double beta decay

The next-generation Enriched Xenon Observatory (nEXO) is a proposed experiment to search for neutrinoless double beta (0νββ) decay in 136 Xe with a target half-life sensitivity of approximately 10 28 years using 5 × 10 3 kg of isotopically enriched liquid-xenon in a time projection chamber. This improvement of two orders of magnitude in sensitivity over current limits is obtained by a significant increase of the 136 Xe mass, the monolithic and homogeneous configuration of the active medium, and the multi-parameter measurements of the interactions enabled by the time projection chamber. Furthermore, the detector concept and anticipated performance are presented based upon demonstrated realizable background rates.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2018

Compton scattering from the deuteron above pion-production threshold

The electromagnetic polarizabilities of the nucleon are fundamental nucleon-structure observables that characterize its response to external electromagnetic fields. The neutron polarizabilities can be accessed from Compton-scattering data on light nuclear targets. Recent measurements of the differential cross section for Compton scattering on the deuteron below the pion-production threshold have decreased the uncertainties in the neutron polarizabilities, yet the proton polarizabilities remain known substantially more accurately. Here, as the sensitivity of the cross section to the polarizabilities increases with incident photon energy, measurements above the pion threshold may offer a way for an improved determination of the neutron polarizabilities. In this work, the first measurement of the cross section for Compton scattering on the deuteron above the pion-production threshold is presented.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2018

Mass measurement of 51 Fe for the determination of the 51 Fe($p, γ$) 52 Co reaction rate

Background: The 51 Fe(p, γ) 52 Co reaction lies along the main rp-process path leading up to the 56 Ni waiting point. The uncertainty in the reaction Q value, which determines the equilibrium between the forward protoncapture and reverse photodisintegration 52 Co(γ,p) 51 Fe reaction, contributes to considerable uncertainty in the reaction rate in the temperature range of interest for Type I x-ray bursts and thus to an ≈10% uncertainty in burst ashes lighter than A = 56. Purpose: With a recent Penning trap mass measurement of 52 Co reducing the uncertainty on its mass to 6.6 keV [Nesterenko et al., J. Phys. G 44, 065103 (2017)], the dominant source of uncertainty in the reaction Q value is now the mass of 51 Fe, reported in the 2016 atomic mass evaluation to a precision of 9 keV [Wang et al., Chin.Phys. C 41, 030003 (2017)]. A new, high-precision Penning trap mass measurement of 51 Fe was performed to allow the determination of an improved precision Q value and thus new reaction rates. Method: 51 Fe was produced using projectile fragmentation at the Coupled Cyclotron Facility at the National Superconducting Cyclotron Laboratory, and separated using the A1900 fragment separator. The resulting secondary beam was then thermalized in the beam stopping area before a mass measurement was performed using the LEBIT 9.4T Penning trap mass spectrometer. Results: The new mass excess, ME = -40189.2(1.6) keV, is sixfold more precise than the current AME value, and 1.6σ less negative. This value was used to calculate a new proton separation energy for 52 Co of 1431(7) keV. New excitation levels were then calculated for 52 Co using the NUSHELLX code with the GXPF1A interaction, and a new reaction rate and burst ash composition was calculated. Conclusions:With a new measured Q value, the uncertainty on the 51 Fe(p, γ ) reaction rate is dominated by the poorly measured 52 Co level structure. Finally, reducing this uncertainty would allow a more precise rate calculation and a better determination of the mass abundances in the burst ashes.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2019

Multisite event discrimination for the majorana demonstrator

The MAJORANA DEMONSTRATOR is searching for neutrinoless double-beta decay($0\nu\beta\beta$) in 76 Ge using arrays of point-contact germanium detectors operating at the Sanford Underground Research Facility. Background results in the $0\nu\beta\beta$ region of interest from data taken during construction, commissioning, and the start of full operations have been recently published. A pulse shape analysis cut applied to achieve this result, named AvsE , is described in this paper. This cut is developed to remove events whose waveforms are typical of multi-site energy deposits while retaining (90 ± 3.5)% of single-site events. This pulse shape discrimination is based on the relationship between the maximum current and energy, and tuned using 228 Th calibration source data. In conclusion, the efficiency uncertainty accounts for variation across detectors, energy, and time, as well as for the position distribution difference between calibration and $0\nu\beta\beta$ events, established using simulations.

59 ≤ A ≤ 89↗
DOE OSTI2017

Large Longitudinal Spin Alignment of Excited Projectiles in Intermediate Energy Inelastic Scattering

Here, we study the sequential breakup of E/A = 24.0 MeV 7 Li projectiles excited through inelastic interactions with C, Be, and Al target nuclei. For peripheral events that do not excite the target, we find very large spin alignment of the excited 7 Li projectiles longitudinal to the beam axis. This spin alignment is independent of the target used, and we propose a simple alignment mechanism that arises from an angular-momentum-excitation-energy mismatch. This mechanism is independent of the potential used for scattering and should be present in many scattering experiments.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2020

Identification of the New Isotope 244 Md

In an experiment performed at Lawrence Berkeley National Laboratory’s 88-inch cyclotron, the isotope Md 244 was produced in the Bi 209 ( Ar 40 , 5 n ) reaction. Decay properties of Md 244 were measured at the focal plane of the Berkeley Gas-filled Separator, and the mass number assignment of A = 244 was confirmed with the apparatus for the identification of nuclide A . The isotope Md 244 is reported to have one, possibly two, α -decaying states with α energies of 8.66(2) and 8.31(2) MeV and half-lives of 0.4 – 0.1 + 0.4 and ~ 6 s , respectively. Furtermore, first evidence of the α decay of Bk 236 was observed and is reported.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗
DOE OSTI2020

Accessing the Single-Particle Structure of the Pygmy Dipole Resonance in 208 Pb

New experimental data on the neutron single-particle character of the Pygmy Dipole Resonance (PDR) in Pb 208 are presented. They were obtained from ( d , p ) and resonant proton scattering experiments performed at the Q3D spectrograph of the Maier-Leibnitz Laboratory in Garching, Germany. The new data are compared to the large suite of complementary, experimental data available for Pb 208 and establish ( d , p ) as an additional, valuable, experimental probe to study the PDR and its collectivity. Furthermore, besides the single-particle character of the states, different features of the strength distributions are discussed and compared to large-scale shell model (LSSM) and energy-density functional plus quasiparticle-phonon model theoretical approaches to elucidate the microscopic structure of the PDR in Pb 208 .

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2021

Charge Radius of Neutron-Deficient Ni 54 and Symmetry Energy Constraints Using the Difference in Mirror Pair Charge Radii

he nuclear root-mean-square charge radius of Ni 54 was determined with collinear laser spectroscopy to be R ( Ni 54 ) = 3.737 ( 3 ) fm . In conjunction with the known radius of the mirror nucleus Fe 54 , the difference of the charge radii was extracted as Δ R ch = 0.049 ( 4 ) fm . Based on the correlation between Δ R ch and the slope of the symmetry energy at nuclear saturation density ( L ), we deduced 21 ≤ L ≤ 88 MeV . The present result is consistent with the L from the binary neutron star merger GW170817, favoring a soft neutron matter EOS, and barely consistent with the PREX-2 result within 1 σ error bands. Our result indicates the neutron-skin thickness of Ca 48 as 0.15–0.21 fm.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2021

Solving the Puzzles of the Decay of the Heaviest Known Proton-Emitting Nucleus 185 Bi

Two long-standing puzzles in the decay of 185 Bi, the heaviest known proton-emitting nucleus are revisited. These are the non-observation of the 9/2 – state, which is the ground state of all heavier odd-A Bi isotopes, and the hindered nature of proton and α decays of its presumed 60-μs 1/2 + ground state. The 185 Bi nucleus has now been studied with the 95 Mo( 93 Nb; 3n) reaction in complementary experiments using the Fragment Mass Analyzer and Argonne Gas-Filled Analyzer at Argonne National Laboratory’s ATLAS facility. The experiments have established the existence of two states in 185 Bi; the short-lived T 1/2 = $2.8$$^{+2.3}_{–1.0}$ μs, proton- and α-decaying ground state, and a 58(2)–μs γ-decaying isomer, the half-life of which was previously attributed to the ground state. The reassignment of the ground-state lifetime results in a proton-decay spectroscopic factor close to unity and represents the only known example of a ground-state proton decay to a daughter nucleus ( 184 Pb) with a major shell closure. Furthermore, the data also demonstrate that the ordering of low- and high-spin states in 185 Bi is reversed relative to the heavier odd-A Bi isotopes, with the intruder-based 1/2 + configuration becoming the ground state, similar to the lightest At nuclides.

150 ≤ A ≤ 189↗
DOE OSTI2023

Surprising Charge-Radius Kink in the Sc Isotopes at N = 20

For this work, charge radii of neutron deficient 40 Sc and 41 Sc nuclei were determined using collinear laser spectroscopy. With the new data, the chain of Sc charge radii extends below the neutron magic number N=20 and shows a pronounced kink, generally taken as a signature of a shell closure, but one notably absent in the neighboring Ca, K, and Ar isotopic chains. Theoretical models that explain the trend at N=20 for the Ca isotopes cannot reproduce this puzzling behavior.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2024

Proton Shell Gaps in N = 28 Nuclei from the First Complete Spectroscopy Study with FRIB Decay Station Initiator

The first complete measurement of the $β$-decay strength distribution of $_{17}^{45}$Cl 28 was performed at the Facility for Rare Isotope Beams (FRIB) with the FRIB Decay Station Initiator during the second FRIB experiment. The measurement involved the detection of neutrons and $γ$ rays in two focal planes of the FRIB Decay Station Initiator in a single experiment for the first time. This enabled an analytical consistency in extracting the $β$-decay strength distribution over the large range of excitation energies, including neutron unbound states. Here, we observe a rapid increase in the $β$-decay strength distribution above the neutron separation energy in $_{18}^{45}$Ar 27 . This was interpreted to be caused by the transitioning of neutrons into protons excited across the Z = 20 shell gap. The SDPF-MU interaction with reduced shell gap best reproduced the data. The measurement demonstrates a new approach that is sensitive to the proton shell gap in neutron rich nuclei according to SDPF-MU calculations.

39 ≤ A ≤ 58↗
DOE OSTI2024

Quest for Cooper Pair Transfer in Heavy-Ion Reactions: The 206 Pb + 118 Sn Case

In this Letter we report on effects of nucleon-nucleon correlations probed in nucleon transfer reactions with heavy ions. We measured with high efficiency and resolution a complete set of observables for neutron transfer channels in the ²⁰⁶Pb + ¹¹⁸Sn system employing a large solid angle magnetic spectrometer, which allowed us to study a wide range of internuclear distances via a detailed excitation function. The coupled channel theory, based on an independent particle transfer mechanism, follows the experimental transfer probabilities for one- and two-neutron pick-up and stripping channels. The experimental two-neutron transfer cross sections indicate that in reactions between pair-vibrational (closed shell) and pair-rotational (open shell) nuclei, correlations manifest via pair-addition and pair-removal modes, which constitute one of the elementary modes of excitations in nuclei.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗