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Analyzing Dynamic Probabilistic Risk Assessment Data through Topology-Based Clustering

We investigate the use of a topology-based clustering technique on the data generated by dynamic event tree methodologies. The clustering technique we utilizes focuses on a domain-partitioning algorithm based on topological structures known as the Morse-Smale complex, which partitions the data points into clusters based on their uniform gradient flow behavior. We perform both end state analysis and transient analysis to classify the set of nuclear scenarios. We demonstrate our methodology on a dataset generated for a sodium-cooled fast reactor during an aircraft crash scenario. The simulation tracks the temperature of the reactor as well as the time for a recovery team to fix the passive cooling system. Combined with clustering results obtained previously through mean shift methodology, we present the user with complementary views of the data that help illuminate key features that may be otherwise hidden using a single methodology. By clustering the data, the number of relevant test cases to be selected for further analysis can be drastically reduced by selecting a representative from each cluster. Identifying the similarities of simulations within a cluster can also aid in the drawing of important conclusions with respect to safety analysis.

97 MATHEMATICS AND COMPUTING↗

Thermal Analysis Evaluations Using the Dry Cask Simulator

Different thermal analysis models were developed to simulate the dry cask simulator (DCS). The DCS is an experiment designed to simulate dry storage of a single boiling water reactor fuel assembly under a variety of heat loads and internal pressures. The DCS was set up and tested in both a vertical and horizontal configuration to determine cladding temperatures in vertical and horizontal dry cask storage systems. The models included a detailed STAR-CCM+ model with the fuel assembly geometry explicitly modeled, a porous STAR-CCM+ model with the fuel assembly geometry modeled as porous media region with calculated effective properties, and a COBRA-SFS model. COBRA-SFS is a thermal-hydraulic code developed for steady-state and transient analysis of multi assembly spent-fuel storage and transportation systems. STAR-CCM+ is a commercial computation fluid dynamics (CFD) code. Both a detailed and porous STARCCM+ model were developed to look at the effective thermal conductivity (keff) approach to modeling a fuel assembly. A keff fuel model is typically model in CFD thermal analyses due to its significantly lower computational costs. The models were run for a combination of low and high canister pressures (100 kPa and 800 kPa) and low and high internal heat loads (0.5 kW and 5 kW). Results from all three models were compared against experimental data taken from the DCS for the peak cladding temperature (PCT) and inlet air mass flow.

Suffield, Sarah R.↗

Experimental Data Sets for CFD Calculations of Flow and Heat Transfer in Deformed Fuel Assemblies

Liquid-metal fast-breeder reactors (LMFBRs) have traditionally used fuel assemblies consisting of a hexagonal array of pins enclosed in a hexagonally shaped duct. Each fuel pin is surrounded by a wire that is wrapped in a helical configuration, which is used to separate the pins sufficiently to allow sodium coolant to flow through the assembly. The helical wire wrap also promotes mixing of the coolant. Experience with these assemblies has shown that they begin to deform with time during normal operation leading to significant changes in core thermal-hydraulics. For example, deformations of assemblies in the Experimental Breeder Reactor-2 and the Fast Flux Test Facility led to pin overheating resulting from pin-to-duct and pin-to-pin contact. This problem is well known and was investigated extensively in the 1970's and early 1980's. This was a period, however, before the development of modern Computational Fluid Dynamics (CFD) computer codes. Therefore, the experiments performed at the time did not record their results in sufficient detail to be useful for compiling validation datasets for CFD codes. Most of the experiments focused only on bulk measurements, such as the pressure drop across the bundle. When the effects of deformation of the fuel assembly were investigated, the studies performed to quantify these effects considered only bare pins without the wire wrap. With the resurgence of interest in LMFBRs in recent years, particularly in designs that leverage long-life performance of the fuel, the need has arisen for data that are suitable for the validation and benchmarking of CFD codes to predict the thermal-hydraulic behavior of flow in wire-wrapped fuel bundles. Such data must include high-resolution, transient, full-field measurements of the fluid velocity and temperature and an accurate record of the test conditions, including a precise description of the geometry. This paper describes a project to produce a validation-quality set of data that can be used to benchmark CFD codes for modeling flow and thermal performance in wire-wrapped fuel assemblies of the kind used by LMFBR designs. In addition, this effort investigates the changes to the flow and other phenomena that occur in the deformed geometries that can form later in a fuel assembly's life. This work is a joint effort of four organizations. The experimental work is being performed by AREVA and Texas A and M University. The computational work, both to support the experiments and to perform blind benchmark calculations, is being done by TerraPower, LLC, and Argonne National Laboratory (ANL). The experiments use a geometry that consists of a complete assembly of 61 wire-wrapped pins, which is surrounded by a hexagonal duct. This configuration is considered the minimum size necessary to adequately capture the important results of interest, such as the thermal gradients across the assembly and the velocity field effects in the assembly resulting from the surrounding duct. These types of effects cannot be captured by a geometry consisting of only a small group of fuel pins. (authors)

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Development of surface modified Zr cladding by coating technology for ATF

It is expected that the accident tolerance fuels (ATF) will provide an enhanced fuel performance of active cooling in the reactor core for a longer time period during design-basis events as well as maintain or improve the fuel performance during normal operations and operational transients. Thus, various ATF cladding concepts have being suggested and developed in many countries. Among them, the coated cladding concept is studied in this work after the considerations of various performances in both the accidents and normal operation of LWRs. In the surface coated cladding concepts, the combination of coating material and coating method is a very important factor to determine the ATF cladding performance. As a new coating material, Cr-based alloy was developed to increase the corrosion resistance under normal operation as well as the oxidation resistance during an accident. From the high temperature oxidation test at 1200 Celsius degrees, the Cr-based alloy showed a superior oxidation resistance to Zircaloy-4 cladding, and showed more improved corrosion resistance than Zircaloy-4 cladding under 360 Celsius degrees PWR simulated loop conditions. The 3D laser coating and a combination of arc ion plating and laser beam scanning were developed to obtain a good adhesion property of corrosion resistance alloy coated on a Zr substrate. The corrosion resistance alloy (Cr-based alloy and FeCrAl alloy) coated layer used by two types of coating methods was maintained without peeling off during the ring compression test at room temperature, although some cracks were formed on the coated layer. After a high-temperature oxidation test at 1200 Celsius degrees for 2000 s, a very thin oxide layer, which was a few microns, was formed on the corrosion resistance alloy layer. However, the ZrO{sub 2} phase, which was thicker than 100 μm was formed on the Zr alloy cladding surface. Thus, it is known that the high-temperature oxidation resistance of commercial Zr alloy cladding can be considerably improved by the coating of corrosion resistant alloys. In addition, the partial oxide dispersion strengthened (ODS) treatment using a laser beam scanning (LBS) method was applied to decrease the ballooning and rupture opening during accident conditions. (authors)

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Code and Solution Verification Assessment of the CTF Thermal Hydraulic Subchannel Code

CTF is a thermal-hydraulics subchannel code jointly developed by Oak Ridge National Laboratory and North Carolina State University. Over the past seven years, the Consortium for Advanced Simulation of Light Water Reactors (CASL) has made a significant investment in developing CTF so it can be used to model light water reactors, including nominal operating conditions, departure from nucleate boiling analysis, and transients ranging from loss of flow to reactivity insertion accidents. In addition to implementing new modeling capabilities and developing the user input and output interface, extensive work has been performed to improve the code’s quality assurance program, resulting in a development process that conforms with NQA-1 requirements. The CASL program follows the Predictive Capability Maturity Model (PCMM) approach for assessing code quality, which emphasizes performing code verification(ensuring the code converges to the correct answer) and solution verification (ensuring the code converges for the intended application). Code and solution verification are used to identify uncertainty errors introduced by numerical approximations in the code and are important for demonstrating that the model is coded without error, which is an important aspect of the Best Estimate plus Uncertainty method. This paper presents a comprehensive overview of the code and solution verification testing that has been performed on CTF. A top-down approach is taken in which the intended CTF applications are presented, followed by the code features required for their modeling. These features are then linked to the applicable code and solution verification tests that demonstrate proper functioning. Past testing efforts are summarized, and new tests are added to help close gaps in the presented test matrix. Rather than performing “one-off” exercises, these tests are added to the automated CTF regression test suite to ensure continual code quality.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Integrating Sudo-Kaminaga Correlation to the Safety Analysis Code PARET-ANL

The accuracy and reliability of the reactor safety analysis code are critical because the specifications of the safety systems will depend on the analytical results for initiating events that could occur to the reactor. In safety analyses for power reactors, there exist many proficient and applicable computer codes such as RELAP5, CATHARE, RETRAN, or CATHENA. For non-power research reactors, an issue arises, however, due to lacking of such specialized codes. As a result, computer codes developed for the transient analysis of power reactors need to be applied carefully after proving their applicability to a specified research reactor. The safety analysis discussed in this paper concerns the prevention of fuel damage in hypothetical accidental scenarios for the new research reactor design at National Institute of Standards and Technology (NIST). One fuel integrity criterion is analyzed by investigating the Minimum Critical Heat Flux Ratio (MCHFR) in the core during the accidental transients. Some previous studies develop a relationship that correlates the nominal value of the minimum CHFR with the probability of CHF occurring and causing fuel damage. Using a statistical approach, the nominal value of the MCHFR for the low-enriched uranium (LEU) reactor needs to remain above the recommended limiting value to better ensure the safety of the research reactor. The probability of no fuel failure increases as the MCHFR increases. More importantly, as long as the MCHFR remains above the recommended limiting value of 1.301, the reactor will have a 90% probability that CHF is not reached. The safety analysis program PARET, developed by Argonne National Laboratory (ANL), is employed to obtain the CHFR information in this study. PARET/ANL is a digital computer programming code intended primarily for the analysis of test and research reactors that use plate-type (flat) fuel elements. This program has its own set of correlations that are used to calculate the CHFR. One of them is the Mirshak correlation, which was believed to provide the best estimation of the critical heat flux under the operating conditions of the new reactor at the time. Following the critical heat flux (CHF) experiments for vertical rectangular channels in the JRR-3 (Japan Research Reactor unit 3), the CHF calculations now use the Sudo- Kaminaga correlation. This correlation is of our interest because this method has an enhanced geometric similarity and an increased range of applicability that are more representative of the actual operating conditions of our current design, and has a more mechanistic approach [9]. Since the source code of PARET/ANL is inaccessible, a MATLAB-based utility has been written to integrate the Sudo-Kaminaga correlation as a substitute for the Mirshak correlation in the code. As a result, both the Mirshak and the Sudo-Kaminaga correlations are used to analyze the standard output from the PARET program to calculate the CHFR.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Comparison of Calibration of Sensors Used for the Quantification of Nuclear Energy Rate Deposition

This present work deals with a collaborative program called GAMMA-MAJOR 'Development and qualification of a deterministic scheme for the evaluation of GAMMA heating in MTR reactors with exploitation as example MARIA reactor and Jules Horowitz Reactor' between the National Centre for Nuclear Research of Poland, the French Atomic Energy and Alternative Energies Commission and Aix Marseille University. One of main objectives of this program is to optimize the nuclear heating quantification thanks to calculation validated from experimental measurements of radiation energy deposition carried out in irradiation reactors. The quantification of the nuclear heating is a key data especially for the thermal, mechanical design and sizing of irradiation experimental devices in specific irradiated conditions and locations. The determination of this data is usually performed by differential calorimeters and gamma thermometers such as used in the experimental multi-sensors device called CARMEN 'Calorimetric en Reacteur et Mesures des Emissions Nucleaires'. In the framework of the GAMMA-MAJOR program a new calorimeter was designed for the nuclear energy deposition quantification. It corresponds to a single-cell calorimeter and it is called KAROLINA. This calorimeter was recently tested during an irradiation campaign inside MARIA reactor in Poland. This new single-cell calorimeter differs from previous CALMOS or CARMEN type differential calorimeters according to three main points: its geometry, its preliminary out-of-pile calibration, and its in-pile measurement method. The differential calorimeter, which is made of two identical cells containing heaters, has a calibration method based on the use of steady thermal states reached by simulating the nuclear energy deposition into the calorimeter sample by Joule effect; whereas the single-cell calorimeter, which has no heater, is calibrated by using the transient thermal response of the sensor (heating and cooling steps). The paper will concern these two kinds of calorimetric sensors. It will focus in particular on studies on their out-of-pile calibrations. Firstly, the characteristics of the sensor designs will be detailed (such as geometry, dimension, material sample, assembly, instrumentation). Then the out-of-pile calibration methods will be described. Furthermore numerical results obtained thanks to 2D axisymmetrical thermal simulations (Finite Element Method, CAST3M) and experimental results will be presented for each sensor. A comparison of the two different thermal sensor behaviours will be realized. To conclude a discussion of the advantages and the drawbacks of each sensor will be performed especially regarding measurement methods. (authors)

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Review of thermophysical property methods applied to fueled and un-fueled molten salts

Recent investigation into designs of molten salt reactors (MSR) requires accurate data of candidate salts. Review of the literature shows lacking thermophysical (TP) property data for coolants and fuel-bearing salts of Advanced High Temperature Reactors (AHTR). Measurement uncertainties of current data are even more deficient, and this affects ongoing research where MSR modeling and testing are being performed. Melting temperature, viscosity, density, specific heat capacity, and thermal and electrical conductivity measurements are often not arranged together or discussed in great detail, especially for fuel-bearing salts. Raw data from key findings spanning over 70 years for LiF, LiF-BeF 2 , LiF-NaF-KF, KCl-MgCl 2 , KF-ZrF 4 , and NaF-KF-MgF 2 have been organized and presented here. Brief description of methods used to obtain these results, in addition to the TP data of some of these salts as fuel carriers, has also been discussed. Thermal conductivity data are particularly weak due to older, high-error measurement techniques. More recent measurement systems to evaluate salt thermal conductivity show promise for obtaining consistent absolute values. This work concludes that measurement systems such as transient hot-wire method, forced Rayleigh scattering, and laser flash analysis provide the most promise to fill these data gaps and reduce current uncertainty in thermal conductivity measurements of both fueled and un-fueled molten salts.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Semi-Annual Report for Modular Integrated Gas High Temperature Reactor Development during Performance Period April 2022 - September 2022

Horizontal Compact High Temperature Gas Reactor (HC-HTGR) is being designed by a multidisciplinary team of nuclear, mechanical, and structural engineers under the support of a DOE-NE Advanced Reactor Demonstration Program’s Advanced Reactor Concepts-20 (ARC-20) award. The objective of this ARC-20 project is to deliver a conceptual design for the proposed HC-HTGR in 3 years and support its commercialization as a safe, low-cost HTGR. Argonne National Laboratory (Argonne) is responsible for the design and analysis of the reactor cavity cooling system (RCCS) as a safety system for passive decay heat removal of the reactor concept. Additionally, Argonne is providing analysis of the primary coolant system to ensure temperatures within the core remain below safety margins during steady-state and potential accident scenarios. This second semi-annual report summarized the progress made at Argonne on the two tasks during the second half of FY22. As a part of the RCCS design task, a scoping calculation in estimating HVAC capability for the HC-HTGR reactor building was performed. A water panel modeling study was first performed with the test case, which confirms the capability of the RELAP5-3D modeling approach to explore various design options of the HC-HTGR RCCS under consideration. Then, a reference RELAP5-3D model for the unit geometry of the preliminary design of the HC-HTGR RCCS was developed. A preliminary performance analysis was conducted to evaluate the performances of a single-phase natural circulation and panel conduction in various operating conditions. For the primary coolant system analysis task, preliminary thermal hydraulic analysis of the HC-HTGR core design was performed with a high resolution 1D fluid-3D solid coupled model using the System Analysis Module (SAM) to assess the assembly coolant channel and bypass flow mass flow rate distribution. Some preliminary work on the development of a full core reduced order model was discussed following the assembly level model to predict the core wide coolant flow distribution and to model certain operational and accidental transients.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

The ATWS analysis of the HTR-10GT core induced by the earthquake - 18489

The 10 MW High Temperature Gas Cooled Test Reactor (HTR-10) has been built in Institute of Nuclear and New Energy Technology (INET) and has been operating successfully since the beginning of 2003. The core outlet temperature of HTR-10 is 700 deg. C. To verify the technology of gas-turbine direct cycle, at first INET had a plan to increase its core outlet temperature to 750 deg. C and use a helium gas turbine instead of the steam generator (then the reactor is called HTR-10GT). Though HTR-10 has good intrinsic safety, the design basic accidents and beyond design basis accidents of HTR-10GT must be analyzed according to China s nuclear regulations due to changed operation parameters. THERMIX code system is used to study the Anticipated Transient Without Scram (ATWS) caused by an earthquake. The gravity acceleration of the earthquake will make the porosity of the pebble bed smaller, which will thus induce a positive reactivity. The packing fraction of the HTR-10GT core will increase to 0.64 from 0.61, while a reactivity of 1.24% will be inserted into an initial core and 0.788% for an equilibrium core. Then the reactor power increased and the temperature of the core increased. When the neutron flux of power measuring range exceeded 123% and the reactor period becomes less than 20 seconds, the reactor should scram. It was supposed that all the control rods in the reflectors had been blocked and the reactor could not scram. Thus the accident went on and the core temperature and the system pressure increased but the reactor shutdown at last because of its natural negative temperature reactivity feedback mechanism. The residual heat would be removed out of the core by the cavity cooling system. During the accident sequence the maximum fuel temperature was 1223 deg. C. If a temperature coefficient error of 20% was considered during analyzing, the peak temperature of the fuel during the ATWS will reach 1266 deg. C. It was a little higher than 1230 deg. C --the fuel temperature limitation of HTR-10. Now the sphere fuel used in HTR-10GT will also be used in HTR-PM and the temperature limitation has been raised to 1620 deg. C, so the HTR-10GT is safe during the ATWS caused by an earthquake. The paper also compares the analysis result of HTR10-GT to those of HTR-10. The results shows that the HTR-10GT is still safe during the accident though its operating temperature is higher than HTR-10. (authors)

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Nuclear Safety [Vol. 36, No. 2, July-December 1995]

Nuclear Safety is a journal that covers significant issues in the field of nuclear safety. Its primary scope is safety in the design, construction, operation, and decommissioning of nuclear power reactors worldwide and the research and analysis activities that promote this goal, but it also encompasses the safety aspects of the entire nuclear fuel cycle, including fuel fabrication, spent-fuel processing and handling, and nuclear waste disposal, the handling of fissionable materials and radioisotopes, and the environmental effects of all these activities. Table of Contents for this issue follows. THE CHORNOBYL ACCIDENT: 195 The Chornobyl Accident Revisited, Part III: Chernobyl Source Term Release Dynamics and Reconstruction of Events During the Active Phase, A. R. Sich; GENERAL SAFETY CONSIDERATIONS: 218 Second ANS Workshop on the Safety of Soviet-Designed Nuclear Power Plants, R. A. Bari; 234 Elements of a Nuclear Criticality Safety Program, C. M. Hopper; 243 Rickover, Excellence, and Criticality Safety Programs, R. E. Wilson; ACCIDENT ANALYSIS: 249 Transient Analysis of the PIUS Advanced Reactor Design with the TRAC-PF1/MOD2 Code, B. E. Boyack, J. L Steiner, S. C. Harmony, H. J. Stumpf, and J. F. Lime; 278 The Hierarchy-By-Interval Approach to Identifying Important Models that Need Improvement in Severe-Accident Simulation Codes, T. J. Heames, M. Khatib-Rahbar, J. E. Kelly, R. P. Jenks-Johnson, and Y.-S. Chen; 290 RELAP5/MOD3 Code Coupling Model, R. P. Martin; 299 Missiles Caused by Severe Pressurized-Water Reactor Accidents, R. Krieg; DESIGN FEATURES: 310 Validation of COMMIX with Westinghouse AP-600 PCCS Test Data, J. G. Sun, T. H. Chien, J. Ding, and W T. Sha; ENVIRONMENTAL EFFECTS: 321 Spent Nuclear Fuel Characterization for a Bounding Reference Assembly for the Receiving Basin for Off-Site Fuel, S. D. Kahook, R. L. Garrett, L. R. Canas, and M J. Beckum; OPERATING EXPERIENCES: 332 Reactor Shutdown Experience, Compiled by J. W. Cletcher; U.S. NUCLEAR REGULATORY COMMISSION INFORMATION AND ANALYSES: 335 Reactor Coolant System Blowdown at Wolf Creek on September 17, 1994, J. V. Kauffman and S. L. Israel; RECENT DEVELOPMENTS: 344 Reports, Standards, and Safety Guides, D. S. Oueener; 349 Proposed Rule Changes as of June 30, 1995; ANNOUNCEMENTS: 320 Symposium on Acceptability of Risk From Radiation—Application to Manned Space Flight; 320 24th DOE/NRC Nuclear Air Cleaning and Treatment Conference; 361 Radiation Biology and Radiation Protection— Modern Developments and Tendencies in Radiation Biology; 362 1997 IEEE Sixth Conference on Human Factors and Power Plants; 354 The Authors; 360 Reviewers of Nuclear Safety, Vol. 36.

05 NUCLEAR FUELS↗

Modeling of the High Temperature Test Facility PG-26 Transient Using RELAP-7

The High Temperature Test Facility (HTTF) is an electrically heated, helium cooled, experimental facility located at Oregon State University (OSU). Modeling of the HTTF PG-26 transient using a multi-app approach utilizing MOOSE and RELAP-7 was conducted. A 3-D model of the HTTF core, reflector, core barrel, and RPV was generated, and 3-D heat conduction throughout the structure was coupled to 1-D fluid flow results from RELAP-7. The model was able to accurately predict peak ceramic core temperatures experienced during the transient which helps validate the capability of RELAP-7 to model advanced gas-cooled nuclear reactors.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Nuclear Safety [Vol. 36, No. 2, July-December 1995]

Nuclear Safety is a journal that covers significant issues in the field of nuclear safety. Its primary scope is safety in the design, construction, operation, and decommissioning of nuclear power reactors worldwide and the research and analysis activities that promote this goal, but it also encompasses the safety aspects of the entire nuclear fuel cycle, including fuel fabrication, spent-fuel processing and handling, and nuclear waste disposal, the handling of fissionable materials and radioisotopes, and the environmental effects of all these activities. Table of Contents for this issue follows. THE CHORNOBYL ACCIDENT: 195 The Chornobyl Accident Revisited, Part III: Chernobyl Source Term Release Dynamics and Reconstruction of Events During the Active Phase, A. R. Sich; GENERAL SAFETY CONSIDERATIONS: 218 Second ANS Workshop on the Safety of Soviet-Designed Nuclear Power Plants, R. A. Bari; 234 Elements of a Nuclear Criticality Safety Program, C. M. Hopper; 243 Rickover, Excellence, and Criticality Safety Programs, R. E. Wilson; ACCIDENT ANALYSIS: 249 Transient Analysis of the PIUS Advanced Reactor Design with the TRAC-PF1/MOD2 Code, B. E. Boyack, J. L Steiner, S. C. Harmony, H. J. Stumpf, and J. F. Lime; 278 The Hierarchy-By-Interval Approach to Identifying Important Models that Need Improvement in Severe-Accident Simulation Codes, T. J. Heames, M. Khatib-Rahbar, J. E. Kelly, R. P. Jenks-Johnson, and Y.-S. Chen; 290 RELAP5/MOD3 Code Coupling Model, R. P. Martin; 299 Missiles Caused by Severe Pressurized-Water Reactor Accidents, R. Krieg; DESIGN FEATURES: 310 Validation of COMMIX with Westinghouse AP-600 PCCS Test Data, J. G. Sun, T. H. Chien, J. Ding, and W T. Sha; ENVIRONMENTAL EFFECTS: 321 Spent Nuclear Fuel Characterization for a Bounding Reference Assembly for the Receiving Basin for Off-Site Fuel, S. D. Kahook, R. L. Garrett, L. R. Canas, and M J. Beckum; OPERATING EXPERIENCES: 332 Reactor Shutdown Experience, Compiled by J. W. Cletcher; U.S. NUCLEAR REGULATORY COMMISSION INFORMATION AND ANALYSES: 335 Reactor Coolant System Blowdown at Wolf Creek on September 17, 1994, J. V. Kauffman and S. L. Israel; RECENT DEVELOPMENTS: 344 Reports, Standards, and Safety Guides, D. S. Oueener; 349 Proposed Rule Changes as of June 30, 1995; ANNOUNCEMENTS: 320 Symposium on Acceptability of Risk From Radiation—Application to Manned Space Flight; 320 24th DOE/NRC Nuclear Air Cleaning and Treatment Conference; 361 Radiation Biology and Radiation Protection— Modern Developments and Tendencies in Radiation Biology; 362 1997 IEEE Sixth Conference on Human Factors and Power Plants; 354 The Authors; 360 Reviewers of Nuclear Safety, Vol. 36.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Validation of MFUEL Metal Fuel Performance Models of SAS4A/SASSYS-1

The fuel characterization models of SAS4A/SASSYS-1 (SAS) have recently been extended to include a new U-Pu-Zr metal fuel model, MFUEL. MFUEL is equipped with mechanistic physics based models to predict the pre-transient characterization and transient response of metal fuel, with emphasis on fuel melting, cladding failure, and the metal fuel’s impact on core reactivity. The MFUEL model will be available in the full version of SAS4A/SASSYS-1 5.7, which is scheduled to be released in June 2023. Fast reactor fuel pins that operated in EBR-II and FFTF with low smear density U-Zr and U-Pu-Zr metal fuels and irradiation resistant ferritic-martensitic cladding showed significant advantages in achieving high burnups and assuring inherent safety characteristics during anticipated transients, design basis events, and beyond design basis events. For safety analysis, a fuel performance model must be able to predict (1) Fuel pin mechanics and compositional and dimensional changes, (2) Clad failure, and (3) Fuel pin thermal resistance. Achieving these high level goals accurately is strongly related to the model performance of individual physical processes taking place within a fuel pin during its lifetime. Metal fuels typically operate above the mid-point temperature of melting during normal, as well as off-normal, conditions. At these elevated temperatures, the availability of thermal activation provides a driving force for various diffusional processes leading to complex phase transformations, micro-structure evolution, significant amounts of fuel swelling, interconnected porosity formation, excessive amounts of fission gas release, and fuel clad chemical interactions. Clad failure in fast reactors primarily occurs as a result of creep rupture augmented by clad wastage formation. The reaction is driven by thermal creep induced dislocation motion, grain boundary cavity nucleation, growth and breakup of grain boundaries. The high level complexity and limited available data requires introducing physics-based modeling approaches to gain extrapolation ability and sensitivity with respect to various conditions. The objective of this report is to perform validation of MFUEL using the experimental data for (1) Normal operation EBR-II fuel behavior, (2) Normal operation PHENIX fuel behavior, (3) HT9 Pressure tube ramp-and-hold creep rupture tests, (4) Whole Pin Furnace (WPF) creep strain, creep rupture and eutectic tests, (5) Fuel Behavior Test Apparatus (FBTA) eutectic tests, and (6) TREAT M5-7 OverPower tests up to clad failure. Section-2 includes a brief description of the MFUEL models. A detailed description of the MFUEL physics-based, semi-empirical models will be presented in the SAS V 5.7 theory manual. Section-3, 4, and 5 describes the validation effort for the pre-transient irradiation, furnace transients, and TREAT M-Series transients, respectively.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Reactivity-initiated accidents in two pressurized water reactor high burnup core designs

Here, this paper presents a safety analysis of two proposed core loadings for 24-month Pressurized Water Reactor (PWR) fuel cycles. This analysis focuses on reactivity-initiated accidents (RIAs) and evaluates core safety performance impacts of rod-averaged burnup limits up to 75 GWD/MTU and less than 7 % enriched UO 2 . The capabilities of Polaris, PARCS, and RELAP5-3D are leveraged to evaluate the core neutronic and thermal–hydraulic behavior for normal-operation, uncontrolled control rod withdrawal (CRW) transients, and control rod ejection (CRE) accidents. The two core designs are compared to identify features of realistic high burnup/extended enrichment core design approaches which have significant safety impact, identify experimental data needs for high-fidelity predictive modeling, and provide recommendations for future high burnup core designs. The first core design evaluated in this study was developed by Southern Nuclear Company and used an ZrB 2 Integral Fuel Burnable Absorber (IFBA) and B 4 C Wet-Annular Burnable Absorber (WABA)-based burnable poison strategy. The second core design assessed in this work used a Gd 2 O 3 -doped UO 2 burnable poison, similar to that used in boiling water reactors or French PWRs. Results indicate that fuel thermal limits are maintained for limiting CRW and hot full power (HFP) CRE transients. Cladding failure is predicted for the highest energy deposition rods in each core during limiting hot zero power (HZP) CRE accidents (where maximum radially averaged enthalpy exceeds 120 cal/g), though licensing may be permissible with a limited number of failed rods. While concerns exist regarding high critical boron concentration during steady state for the IFBA core and large plenum pressures for the gadolinia core design, the analysis demonstrates adequate safety performance during limiting RIA accident scenarios for two representative high burnup core designs. Design changes limiting plenum pressures and implementation of accident tolerant fuel (ATF) cladding features which minimize hydriding and susceptibility to pellet-cladding mechanical interaction (PCMI) are recommended for future high burnup fuel concepts. To support the technical basis for burnup limit increases, high-fidelity fuel performance models are needed to address physical effects not considered in this analysis, and high burnup irradiated fuel tests are required to extend applicability of the fuel failure limits and validate existing and future models.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Used nuclear fuel separations process simulation and testing

Recent efforts in separations process simulation at Argonne have expanded from the traditional focus on solvent extraction flowsheet design in order to capture process dynamics and to simulate other components, processing and systems of a used nuclear fuel reprocessing plant. For example, the Argonne Model for Universal Solvent Extraction (AMUSE) code has been enhanced to make it both more portable and more readily extensible. Moving away from a spreadsheet environment makes the addition of new species and processes simpler for the expert user, which should enable more rapid implementation of chemical models that simulate evolving processes. The dyAMUSE (dynamic AMUSE) version allows the simulation of transient behavior across an extractor. Electrochemical separations have now been modeled using spreadsheet codes that simulate the electrochemical recycle of fast reactor fuel. The user can follow the evolution of the salt, products, and waste compositions in the electro-refiner, cathode processors, and drawdown as a function of fuel batches treated. To further expand capabilities in integrating multiple unit operations, a platform for linking mathematical models representing the different operations that comprise a reprocessing facility was adapted to enable systems-level analysis and optimization of facility functions. (authors)

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Fuel Performance Evaluation of THOR-C Experiments

The Temperature Heatsink Overpower Response Commissioning (THOR-C) and THOR-Metal (THOR-M) experiments will be performed as part of an ongoing project for testing sodium fast reactor fuels with the Japan Atomic Energy Agency (JAEA). The THOR-C experiments consist of fresh metallic fuel pins and have been analyzed using the ABAQUS, Ansys codes and the BISON fuel performance code. THOR-M-Loss of Flow-1 (THOR-M-LOF-1) is designed to test an EBR-II irradiated fuel pin under LOF conditions. Simulation of the THOR-MLOF-1 experiment required first simulating the base irradiation of the fuel pin in EBR-II. MFUEL module of SAS4A/SASSYS-1 [1] is a physics-based metallic fuel performance model applicable to the normal operation, transient scenarios and fuel failure modeling including scenarios with bulk fuel melting. The model has been validated using EBR-II normal operation, separate effect transient tests as well as TREAT M-Series transient tests [2]. In this study, MFUEL models has been utilized together with a new capsule heat transfer model developed in this project. The new heat transfer model was necessary due to (1) significant amount of heat losses that required 2D heat transfer, (2) the presence of a titanium heat sink, rejecting a significant amount of heat, and (3) stagnant coolant conditions, which are inconsistent with SAS4A/SASSYS-1 (SAS) heat transfer model. Updates to SAS4A/SASSYS-1 and MFUEL has been described below, followed by a preliminary validation effort using the results from THOR-C-2 fresh fuel capsule experiment. A previous study for THOR-C-2 analysis using BISON code is also utilized in this study to model this test [3]. [1] D. O’Grady, A. J. Brunett, L. Ibarra, A. Karahan, T. Kim, T. S. Sumner, R. Thomas, T. H. Fanning, “The SAS4A/SASSYS-2 Version 5.7 Safety Analysis Code System,” Argonne National Laboratory,ANL/NSE-SAS/5.7, (2023). [2] A. Karahan, T. Kim, T. Fanning, D. O’Grady, “Validation of MFUEL Metal Fuel Performance Models of SAS4A/SASSYS-1,” Argonne National Laboratory, ANL/NSE-23/11, (2023). [3] M. Mihelish, A. Zabriskie, K. Paaren, P. Medvedev, C. Jensen, “Fuel Performance Predictions for the TREAT THOR-C Experiments,” Idaho National Laboratory, INL/RPT-23-73397, Revision 0, (2023)

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗