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At least 703 records · Page 39

Establishing gold and platinum standards to 1 terapascal using shockless compression

New techniques are advancing the frontier of high-pressure physics beyond 1 terapascal, leading to new discoveries and offering stringent tests for condensed-matter theory and advanced numerical methods. However, the ability to absolutely determine the pressure state remains challenging, and well-calibrated pressure-density reference materials are required. We conducted shockless dynamic compression experiments at the National Ignition Facility and the Z machine to obtain quasi-absolute, high-precision, pressure-density equation-of-state data for gold and platinum. We derived two experimentally constrained pressure standards to terapascal conditions. Establishing accurate experimental determinations of extreme pressure will facilitate better connections between experiments and theory, paving the way toward improving our understanding of material response to these extreme conditions.

36 MATERIALS SCIENCE↗

Dynamic Strength Characteristics of Materials: Influence of the Specimen Size on Strain Rate

Test results are presented for an additive material prepared of acrylonitrile-butadiene-styrene on a 3D printer. Dynamic tension experiments have been carried out using a tower-type drop hammer with an accelerator. Data obtained from different specimens demonstrate that high-strain-rate tensile experiments are feasible if the working part of the specimen is decreased. A theoretical analysis of test data using the incubation time criterion has been performed, and it has been found that analytical results are in good agreement with experimental data.

36 MATERIALS SCIENCE↗

A Simple Design Erosional Plasma Gun Made of a Coaxial Cable with Polyethylene Insulation

Abstract—: A compact pulsed plasma generator of simple design made of a coaxial cable with polyethylene insulation has been described. A plasma gun generates a cloud of carbon-hydrogen plasma with an electron density of more than 10{sup 13} cm{sup –3}, including in a magnetic field produced of up to 500 G and also in the presence of the background plasma with a density of about 10{sup 12} cm{sup –3}, which is produced by an independent source. The high resource of the gun and stability of plasma parameters from one pulse to another allows using such a gun in laboratory experiments simulating dynamic processes in space.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Human Contribution to the Increasing Summer Precipitation in Central Asia from 1961 to 2013

We report that the ecosystem and societal development over arid Central Asia, the core connecting region of the Silk Road Economic Belt, are highly sensitive to climate change. The results derived from multiobservational datasets show that summer precipitation over Central Asia has significantly increased by 20.78% from 1961 to 2013. It remains unclear whether anthropogenic forcing has contributed to the summer wetting trend or not. In this study, the corresponding physical processes and contributions of anthropogenic forcing are investigated by comparing reanalysis and experiments of the Community Atmosphere Model, version 5.1 (CAM5.1), from the CLIVAR Climate of the Twentieth Century Plus (C20C+) Project. The observed wetting trend is well reproduced in the simulation driven by all radiative forcings (CAM5-All), but poorly reproduced in the simulation with natural forcings only (CAM5-Nat), confirming the important role of human contribution in the observed wetting trend. Moisture budget analysis shows that the observed wetting trend is dominated by the increasing vertical moisture advection term and results from enhanced vertical motion over nearly all of Central Asia. The observed contributions of moisture budget components to the wetting trend are only captured by CAM5-All experiments. The dynamic contribution is determined by the warm advection anomalies in association with a human-induced meridional uneven warm pattern. Finally, human-induced warming increases the specific humidity over all of Central Asia, increasing (decreasing) the precipitation over the climatological ascent (descent) region in eastern (western) Central Asia.

54 ENVIRONMENTAL SCIENCES↗

Crystallization kinetics and thermodynamics of an Ag–In–Sb–Te phase change material using complementary in situ microscopic techniques

The crystallization of an amorphous Ag–In–Sb–Te (AIST) phase change material (PCM) is studied using multiple in situ imaging techniques to directly quantify crystal growth rates over a broad range of temperatures. The measurable growth rates span from ≈ 10 –9 to ≈ 20 m/s. Recent results using dynamic transmission electron microscopy (TEM), a photoemission TEM technique, and TEM with sub-framed imaging are reported here and placed into the context of previous growth rate measurements on AIST. Dynamic TEM experiments show a maximum observed crystal growth rate for as-deposited films to be > 20 m/s. It is shown that crystal growth above the glass transition can be imaged in a TEM through use of subframing and a high-frame-rate direct electron detection camera. Challenges associated with the determination of temperature during in situ TEM experiments are described. Finally, preliminary nanocalorimetry results demonstrate the feasibility of collecting thermodynamic data for crystallization of PCMs with simultaneous TEM imaging.

36 MATERIALS SCIENCE↗

Shock and Release Response of Unreacted Epon 828: Shot 2s-905

This document summarizes the shock and release response of Epon 828 measured in the dynamic impact experiment 2s-905. Experimentally, a thin Kel-F impactor backed by a low impedance foam impacted an Epon 828 target with embedded electromagnetic gauges. Computationally, a one dimensional simulation of the impact event was performed, and tracer particles were located at the corresponding electromagnetic gauge locations. The experimental configuration was such that the Epon 828 target was initially shocked, and then allowed to release from the high-pressure state. Comparisons of the experimental gauge and computational tracer data were made to assess the performance of equation of state (EOS) 7603, a SESAME EOS for Epon 828, on and off the principal shock Hugoniot. Results indicate that while EOS 7603 can capture the Hugoniot response to better that 1%, while the sound speeds at pressure are under-predicted by 6 - 7%.

45 MILITARY TECHNOLOGY, WEAPONRY, AND NATIONAL DEF↗

Analytic, empirical and delta method temperature derivatives of D-D and D-T fusion reactivity formulations, as a means of verification

We examine the derivatives with respect to temperature, for various deuterium-tritium (DT) and deuterium-deuterium (D-D) fusion-reactivity formulations. Langenbrunner and Makaruk [1] had studied this as a means of understanding the time and temperature domain of reaction history measured in dynamic fusion experiments. Presently, we consider the temperature derivative dependence of fusion reactivity as a means of exercising and verifying the consistency of the various reactivity formulations.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Early Career: In-situ Monitoring of Dynamic Phenomena during Solidification

Solidification is critical to processes like casting and additive manufacturing and the manufacture of metallic alloy components we use in our everyday lives. State-of-the-art characterization techniques, now available at U.S. DOE User Facilities and in the laboratory, are not only enabling fundamental studies of metallic alloy solidification dynamics, but also in-operando, in-situ deformation, and manufacturing studies. Here we use x-ray, proton, and electron imaging to study solidification dynamics from the micro-scale to the macro-scale, at times ranging from microseconds to minutes. Our experimental results are used to inform, develop, and validate computational models at the same length and time-scales. Integrating in-situ characterization and modeling will yield the prediction and control of metallic alloy solidification dynamics and the creation of microstructures and properties by design with advanced manufacturing. Major research accomplishments during this period include: 1. Exploring dynamical microstructure selection by means of real-time synchrotron x-ray imaging of controlled directional solidification of aluminum alloys and quantitative phase field modeling. 2. In-situ and ex-situ electron microscopy of rapid solidification after laser melting of metallic alloys. 3. Exploring the impact of microstructural heterogeneities that develop during solidification on solid-state phase transitions, with an emphasis on phase growth, (meta)stability, and transition pathways in aluminum alloys. 4. Demonstrations of four-dimensional (three-dimensions plus time) x-ray microscopy during controlled directional solidification and the first quasi-static/dynamic transmission high energy electron microscopy of metallic alloy solidification dynamics. 5. Experiments and modeling of solidification structure evolution and forward modeling and testing of micromechanical behavior.

36 MATERIALS SCIENCE↗

A Correct Flat Field Model For DARHT

The forward modeling approach has been utilized to obtain the density distribution during dynamic radiographic experiments using the Bayesian Inference Engine (BIE) at the Dual Axis Radiographic Hydrodynamic Test Facility (DARHT) for over two decades. The forward modeling approach attempts to incorporate all of the known physics to obtain the transmission, from an unknown density field. The density field is then optimized in an attempt to match the flat-fielded radiographic image using a Chi-squared comparison. A depiction of the forward modeling approach implemented in the BIE is given.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Physics Flash Fall 2020

The Fall 2020 edition of Physics Flash includes article briefs on: Patrick Younk, Fusing concepts, technology to past performance of nuclear explosives; LANL inertial confinement fusion programs aims to develop burning plasma for weapons science; Lab's high energy nuclear physics explored at international conference; and, Novel study reveals new details on the impact of thermal interfaces in dynamic compression experiments.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Physical Sciences Vistas (Issue 3 2020)

In this issue, highlights of our outstanding R&D supporting the Laboratory’s nuclear security mission include the following. 1. The essential nuclear materials science contributions of MST’s Materials Properties Team to a range of Lab missions, operations, and initiatives. 2. Work in the Sigma Complex supporting NNSA’s Advanced Manufacturing Development milestones by members of Sigma Division and colleagues across the Laboratory and other NNSA sites. 3. Greg Dale’s role in the Lab’s molybdenum program and today as a technical lead on the Scorpius project. 4. Measurements that reveal the role thermal interfaces play in dynamic compression experiments. 5. The first-ever synthesis of an actinide framework, which offers opportunities for understanding these structures as potential radioactive waste forms and provides new models of actinide species transport in the environment. This issue also showcases, as part of our commitment to simultaneous excellence in mission operations and community relations, the successful high-hazard repair of the LANSCE accelerator, which resulted in a large team Laboratory Distinguished Performance Award, and a virtual Summer Physics Camp for Young Women that brought together participants from around the world, even as COVID kept them socially distant in their homes.

36 MATERIALS SCIENCE↗

Multiple Frame Radiography to Study Material Properties

Poster to be displayed at the upcoming SPIE job fair (August 28-Sept. 1) and recruiting trip to the Colorado School of Mines (Sept. 15). This poster will then also be used as a lab display at NMO.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Modification of Χ c1 (3872) and ψ(2S) Production in p Pb Collisions at $\sqrt{S_{NN}}$ = 8.16 TeV

The LHCb Collaboration measures production of the exotic hadron Χ c1 (3872) in proton-nucleus collisions for the first time. Comparison with the charmonium state ψ(2S) suggests that the exotic Χ c1 (3872) experiences different dynamics in the nuclear medium than conventional hadrons, and comparison with data from proton-proton collisions indicates that the presence of the nucleus may modify Χ c1 (3872) production rates. This is the first measurement of the nuclear modification factor of an exotic hadron.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Chemical controls on the propagation and healing of subcritical fractures

Human activities involving subsurface reservoirs—resource extraction, carbon and nuclear waste storage—alter thermal, mechanical, and chemical steady-state conditions in these systems. Because these systems exist at lithostatic pressures, even minor chemical changes can cause chemically assisted deformation. Therefore, understanding how chemical effects control geomechanical properties is critical to optimizing engineering activities. The grand challenge in predicting the effect of chemical processes on mechanical properties lays in the fact that these phenomena take place at molecular scales, while they manifest all the way to reservoir scales. To address this fundamental challenge, we investigated chemical effects on deformation in model and real systems spanning molecular- to centimeter scales. We used theory, experiment, molecular dynamics simulation, and statistical analysis to (1) identify the effect of simple reactions, such as hydrolysis, on molecular structures in interfacial regions of stressed geomaterials; (2) quantify chemical effects on the bulk mechanical properties, fracture and displacement for granular rocks and single crystals; (3) develop initial understanding of universal scaling for individual displacement events in layered geomaterials; and (4) develop analytic approximations for the single-chain mechanical response utilizing asymptotically correct statistical thermodynamic theory. Taken together, these findings advance the challenging field of chemo-mechanics.

36 MATERIALS SCIENCE↗

Modeling Low Intensity Fires: Lessons Learned from 2012 RxCADRE

Coupled fire-atmosphere models are increasingly being used to study low-intensity fires, such as those that are used in prescribed fire applications. Thus, the need arises to evaluate these models for their ability to accurately represent fire spread in marginal burning conditions. In this study, wind and fuel data collected during the Prescribed Fire Combustion and Atmospheric Dynamics Research Experiments (RxCADRE) fire campaign were used to generate initial and boundary conditions for coupled fire-atmosphere simulations. We present a novel method to obtain fuels representation at the model grid scale using a combination of imagery, machine learning, and field sampling. Several methods to generate wind input conditions for the model from eight different anemometer measurements are explored. We find a strong sensitivity of fire outcomes to wind inputs. This result highlights the critical need to include variable wind fields as inputs in modeling marginal fire conditions. This work highlights the complexities of comparing physics-based model results against observations, which are more acute in marginal burning conditions, where stronger sensitivities to local variability in wind and fuels drive fire outcomes.

54 ENVIRONMENTAL SCIENCES↗

Validating the Use of Gaussian Process Regression for Adaptive Mapping of Residual Stress Fields

Probing the stress state using a high density of measurement points is time intensive and presents a limitation for what is experimentally feasible. Alternatively, individual strain fields used for determining stresses can be reconstructed from a subset of points using a Gaussian process regression (GPR). Results presented in this paper evidence that determining stresses from reconstructed strain fields is a viable approach for reducing the number of measurements needed to fully sample a component’s stress state. The approach was demonstrated by reconstructing the stress fields in wire-arc additively manufactured walls fabricated using either a mild steel or low-temperature transition feedstock. Effects of errors in individual GP reconstructed strain maps and how these errors propagate to the final stress maps were assessed. Implications of the initial sampling approach and how localized strains affect convergence are explored to give guidance on how best to implement a dynamic sampling experiment.

36 MATERIALS SCIENCE↗

The Pseudosynchronization of Binary Stars Undergoing Strong Tidal Interactions

Eccentric binaries known as heartbeat stars experience strong dynamical tides as the stars pass through periastron, providing a laboratory to study tidal interactions. We measure the rotation periods of 24 heartbeat systems, using the Kepler light curves to identify rotation peaks in the Fourier transform. Where possible, we compare the rotation period to the pseudosynchronization period derived by Hut. Few of our heartbeat stars are pseudosynchronized with the orbital period. For four systems, we were able to identify two sets of rotation peaks, which we interpret as the rotation from both stars in the binary. Most stars in our sample have rotation rates larger than the pseudosynchronization period while a single target rotates much faster than this rate. The majority of the systems have a rotation period that is approximately (3/2) times the pseudosynchronization period, suggesting that other physical mechanisms strongly influence the star’s evolution.

79 ASTRONOMY AND ASTROPHYSICS↗

Auger analysis of oxygen and sulfur interactions with various metals and the effect of sliding on these interactions

Various gases were adsorbed to copper, aluminum, and chromium surfaces. The gases included oxygen, hydrogen sulfide, methyl mercaptan, and sulfur dioxide. Chemisorption was conducted on static surfaces and during dynamic friction experiments. An Auger cyclindrical mirror analyzer was used to monitor surface films. The sulfur containing gases adsorbed readily to all surfaces. Exposures of as little as 0.000001 (torr)(sec) (1 langmuir) were sufficient to reduce friction. Sliding contact did not affect chemisorption of copper or aluminum but did affect chemisorption to chromium surfaces. Oxygen removed sulfur films from all surfaces at room temperature (23 C). Gaseous exposures were from 0.000001 to 0.01 (torr)(sec) (1 to 10,000 langmuirs).

Buckley, D. H.↗