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DOE OSTI2023

Assessment of Flow-Enhanced Electrochemical Sensor Testing and Deployments for MSRs

This report serves as the deliverable for Milestone M3RS-23AN0401061 that is part of Work Package RS-23AN040106 (Flow Enhanced Sensors for MSRs – ANL). The goal of this milestone was to determine performance of the flow enhanced electrochemical sensor (FEES) and modular flow instrumentation testbed (MFIT) in safeguards relevant scenarios. Flow enhanced electrochemical sensors are a type of electroanalytical sensor that has been developed at Argonne National Laboratory to be installed directly into MSR flow conduits to make measurements of the salt composition. These sensors represent a significant improvement in capabilities compared to earlier electroanalytical sensors that instead can only be operated in quiescent conditions. Previous work has focused on testing of the FEES in flowing conditions provided by the MFIT to assess the accuracy and precision of the sensor measurements. To further improve this capability, in FY23 we undertook a campaign of safeguards relevant scenarios in molten salt containing a range of uranium chloride concentrations (0 to 3 wt%). All the testing carried out in FY23 was aided by a control system designed to automatically actuate flow conditions and collect data. This new automation system is estimated to have increased experimental throughput by a factor of four and enabled testing in a variety of complex conditions. The advancements in throughput and repeatability led to improved quantification of actinide concentrations using the in-flow sensors, with a reduction of the mean absolute relative error from 5.6% in FY22 to 3.1% in FY23. In addition to safeguards scenarios run in the MFIT, FY23 work included deployment of a FEES at a partner institution where it will be tested in a flowing salt loop. The FEES was successfully integrated into that loop and is being tested prior to loop startup. In FY23, work also continued on the smaller flow system that we have named the mini-MFIT. This smaller system is capable of rapid prototyping of new sensor designs prior to installation in the larger MFIT radiological flow system. Work was carried out to test this new system in non-radiological molten salts in a separate glovebox. This work is helping us to enhance the accuracy of our salt monitoring capabilities through the integration of multiple types of sensors. The high degree of accuracy required by 10 CFR 74 represents a significant challenge, and further design evolution and integration of the sensors into multimodal sensing frameworks will be needed to further push the measurement accuracy to the needed level.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

NASA NTRS1978

A demonstration of dual spacecraft tracking conducted with the Viking spacecraft during the approach phase

The potential improvements in navigation capability of dual spacecraft tracking were demonstrated using Viking approach data. Under unfavorable conditions of large plasma noise, low spacecraft declination and large earth-spacecraft distance, the dual spacecraft tracking technique improved the Viking B approach accuracy based on short-arc radio metric data, by a factor of 7, to less than 200 km at Mars orbit insertion minus 3 days. From the results of an analytical expansion and the Viking demonstration with a large intentional error in Mars ephemeris, that dual spacecraft data types are shown to be insensitive to ephemeris error. Results also reveal the potential reduction of tracking time requirements during planet approach.

Chao, C. C.↗

NASA NTRS1987

Galerkin/Runge-Kutta discretizations for parabolic equations with time dependent coefficients

A new class of fully discrete Galerkin/Runge-Kutta methods is constructed and analyzed for linear parabolic initial boundary value problems with time dependent coefficients. Unlike any classical counterpart, this class offers arbitrarily high order convergence while significantly avoiding what has been called order reduction. In support of this claim, error estimates are proved, and computational results are presented. Additionally, since the time stepping equations involve coefficient matrices changing at each time step, a preconditioned iterative technique is used to solve the linear systems only approximately. Nevertheless, the resulting algorithm is shown to preserve the original convergence rate while using only the order of work required by the base scheme applied to a linear parabolic problem with time independent coefficients. Furthermore, it is noted that special Runge-Kutta methods allow computations to be performed in parallel so that the final execution time can be reduced to that of a low order method.

Keeling, Stephen L.↗

NASA NTRS1986

Statistical corrections to numerical predictions. IV

The National Meteorological Center Barotropic-Mesh Model has been used to test a statistical correction procedure, designated as M-II, that was developed in Schemm et al. (1981). In the present application, statistical corrections at 12 h resulted in significant reductions of the mean-square errors of both vorticity and the Laplacian of thickness. Predictions to 48 h demonstrated the feasibility of applying corrections at every 12 h in extended forecasts. In addition to these improvements, however, the statistical corrections resulted in a shift of error from smaller to larger-scale motions, improving the smallest scales dramatically but deteriorating the largest scales. This effect is shown to be a consequence of randomization of the residual errors by the regression equations and can be corrected by spatially high-pass filtering the field of corrections before they are applied.

Schemm, Jae-Kyung↗

NASA NTRS1989

Galerkin/Runge-Kutta discretizations for parabolic equations with time-dependent coefficients

Keeling, Stephen L.↗

NASA NTRS1989

A summary of precise orbit computation for the Geosat Exact Repeat Mission

Recent efforts to recompute orbits for the Geosat Exact Repeat Mission have resulted in a substantial reduction in the satellite's orbit error. The improved orbits are based on Doppler tracking and on the new earth gravity models being developed at the Goddard Space Flight Center in support of requirements for the TOPEX/Poseidon mission. The first set of orbit solutions based on the Goddard Earth Model (GEM T1) gravity model and tracking data from the U.S. Navy's Operational Network system are accurate to about 85 cm root mean square (rms) in height. Preliminary tests of orbits computed with the GEM-T2 model, along with tracking data from an augmented network consisting of the Navy's Operational Network and selected Tracking Network sites, indicate that radial accuracies of 35 cm rms can be achieved.

Haines, Bruce J.↗

NASA NTRS1990

Minimizing selective availability error on Topex GPS measurements

GPS measurements made at Topex/Poseidon and the accompanying ground tracking sites will be affected by the selective availability. Although in principle the effects may be removed by differencing between receivers observing the same GPS satellites, this requires accurate synchronization of all receiver clocks. In the case of Topex/Poseidon application, there are two sources of imperfect clock synchronization. The first and larger is due to the constantly drifting clock onboard Topex, which may cause a residual effect as large as 10 cm on Topex carrier phase and 1 m on Topex pseudorange. The second is due to light-time differences between receivers observing the same GPS satellites, which may amount to a few mm error. In this paper a data reduction scheme which incorporates a low-order polynomial interpolation and carrier phase smoothing on pseudorange acquired at Topex and ground receivers is described; a simulation analysis is given demonstrating the effectiveness of the scheme for reducing the GPS S/A effects; and comparison with other schemes is discussed.

Wu, S. C.↗

NASA NTRS2002

Telescope Scientist on the Advanced X-Ray Astrophysics Observatory

This period included many scientific observations made with the Chandra Observatory. The results, as is well known, are spectacular. Fortunately, the HRMA performance continues to be essentially identical to that predicted from ground calibration data. The Telescope Scientist Team has improved the mirror model to provide a more accurate description to the Chandra observers and enable them to reduce the systematic errors and uncertainties in their data reduction. There also has been progress in the scientific program. At this time 47 distant clusters of galaxies have been observed. We are performing a systematic analysis of this rather large data set for the purpose of determining absolute distances utilizing the Sunyaev Zel'dovich effect.

VanSpeybroeck, L.↗

NASA NTRS2002

Telescope Scientist on the Advanced X-ray Astrophysics Observatory

This period included many scientific observations made with the Chandra Observatory. The results, as is well known, are spectacular. Fortunately, the High Resolution Mirror Assembly (HRMA) performance continues to be essentially identical to that predicted from ground calibration data. The Telescope Scientist Team has improved the mirror model to provide a more accurate description to the Chandra observers and enable them to reduce the systematic errors and uncertainties in their data reduction. We also have made considerable progress in improving the scattering model. There also has been progress in the scientific program. At this time 58 distant clusters of galaxies have been observed. We are performing a systematic analysis of this rather large data set for the purpose of determining absolute distances utilizing the Sunyaev Zel'dovich effect. These observations also have been used to study the evolution of the cluster baryon mass function and the cosmological constraints which result from this evolution.

VanSpeybroeck, L.↗

NASA NTRS2003

Instrument Reflections and Scene Amplitude Modulation in a Polychromatic Microwave Quadrature Interferometer

A polychromatic microwave quadrature interferometer has been characterized using several laboratory plasmas. Reflections between the transmitter and the receiver have been observed, and the effects of including reflection terms in the data reduction equation have been examined. An error analysis which includes the reflections, modulation of the scene beam amplitude by the plasma, and simultaneous measurements at two frequencies has been applied to the empirical database, and the results are summarized. For reflection amplitudes around 1096, the reflection terms were found to reduce the calculated error bars for electron density measurements by about a factor of 2. The impact of amplitude modulation is also quantified. In the complete analysis, the mean error bar for high- density measurements is 7.596, and the mean phase shift error for low-density measurements is 1.2". .

Dobson, Chris C.↗

NASA NTRS2004

Telescope Scientist on the Advanced X-ray Astrophysics Observatory

In this period, the Chandra X-ray Observatory continued to perform exceptionally well, with many scientific observations and spectacular results. The HRMA performance continues to be essentially identical to that predicted from ground calibration data. The Telescope Scientist Team has improved the mirror model to provide a more accurate description to the Chandra observers, enabling them to reduce the systematic errors and uncertainties in their data reduction. There also has been good progress in the scientific program. Using the Telescope Scientist GTO time, we carried out an extensive Chandra program to observe distant clusters of galaxies. The goals of this program were to use clusters to derive cosmological constraints and to investigate the physics and evolution of clusters. A total of 71 clusters were observed with ACIS-I; the last observations were completed in December 2003.

Smith, Carl M.↗

NASA NTRS2006

NASA Tech Briefs, June 2006

Topics covered include: Magnetic-Field-Response Measurement-Acquisition System; Platform for Testing Robotic Vehicles on Simulated Terrain; Interferometer for Low-Uncertainty Vector Metrology; Rayleigh Scattering for Measuring Flow in a Nozzle Testing Facility; "Virtual Feel" Capaciflectors; FETs Based on Doped Polyaniline/Polyethylene Oxide Fibers; Miniature Housings for Electronics With Standard Interfaces; Integrated Modeling Environment; Modified Recursive Hierarchical Segmentation of Data; Sizing Structures and Predicting Weight of a Spacecraft; Stress Testing of Data-Communication Networks; Framework for Flexible Security in Group Communications; Software for Collaborative Use of Large Interactive Displays; Microsphere Insulation Panels; Single-Wall Carbon Nanotube Anodes for Lithium Cells; Tantalum-Based Ceramics for Refractory Composites; Integral Flexure Mounts for Metal Mirrors for Cryogenic Use; Templates for Fabricating Nanowire/Nanoconduit- Based Devices; Measuring Vapors To Monitor the State of Cure of a Resin; Partial-Vacuum-Gasketed Electrochemical Corrosion Cell; Theodolite Ring Lights; Integrating Terrain Maps Into a Reactive Navigation Strategy; Reducing Centroid Error Through Model-Based Noise Reduction; Adaptive Modeling Language and Its Derivatives; Stable Satellite Orbits for Global Coverage of the Moon; and Low-Cost Propellant Launch From a Tethered Balloon

Source record↗

NASA NTRS2011

Optimal Asteroid Mass Determination from Planetary Range Observations: A Study of a Simplified Test Model

Mars ranging observations are available over the past 10 years with an accuracy of a few meters. Such precise measurements of the Earth-Mars distance provide valuable constraints on the masses of the asteroids perturbing both planets. Today more than 30 asteroid masses have thus been estimated from planetary ranging data (see [1] and [2]). Obtaining unbiased mass estimations is nevertheless difficult. Various systematic errors can be introduced by imperfect reduction of spacecraft tracking observations to planetary ranging data. The large number of asteroids and the limited a priori knowledge of their masses is also an obstacle for parameter selection. Fitting in a model a mass of a negligible perturber, or on the contrary omitting a significant perturber, will induce important bias in determined asteroid masses. In this communication, we investigate a simplified version of the mass determination problem. Instead of planetary ranging observations from spacecraft or radar data, we consider synthetic ranging observations generated with the INPOP [2] ephemeris for a test model containing ~25000 asteroids. We then suggest a method for optimal parameter selection and estimation in this simplified framework.

asteroids↗

NASA NTRS2010

Advanced Navigation Strategies For Asteroid Sample Return Missions

Flyby and rendezvous missions to asteroids have been accomplished using navigation techniques derived from experience gained in planetary exploration. This paper presents analysis of advanced navigation techniques required to meet unique challenges for precision navigation to acquire a sample from an asteroid and return it to Earth. These techniques rely on tracking data types such as spacecraft-based laser ranging and optical landmark tracking in addition to the traditional Earth-based Deep Space Network radio metric tracking. A systematic study of navigation strategy, including the navigation event timeline and reduction in spacecraft-asteroid relative errors, has been performed using simulation and covariance analysis on a representative mission.

Getzandanner, K.↗

NASA NTRS2022

Microstructure Segmentation With Deep Learning Encoders Pre-Trained on a Large Microscopy Dataset

This study examined the improvement of microscopy segmentation intersection over union accuracy by transfer learning from a large dataset of microscopy images called MicroNet. Many neural network encoder architectures were trained on over 100,000 labeled microscopy images from 54 material classes. These pre-trained encoders were then embedded into multiple segmentation architectures including UNet and DeepLabV3+ to evaluate segmentation performance on created benchmark microscopy datasets. Compared to ImageNet pre-training, models pre-trained on MicroNet generalized better to out-of-distribution micrographs taken under different imaging and sample conditions and were more accurate with less training data. When training with only a single Ni-superalloy image, pre-training on MicroNet produced a 72.2% reduction in relative intersection over union error. These results suggest that transfer learning from large in-domain datasets generate models with learned feature representations that are more useful for downstream tasks and will likely improve any microscopy image analysis technique that can leverage pre-trained encoders.

machine learning↗

DOE OSTI2011

Dynamic Aperture and Tolerances for PEP-X Ultimate Storage Ring Design

A lattice for the PEP-X ultimate storage ring light source, having 11 pm-rad natural emittance at a beam energy of 4.5 GeV at zero current, using 90 m of damping wiggler and fitting into the existing 2.2-km PEP-II tunnel, has been recently designed. Such a low emittance lattice requires very strong sextupoles for chromaticity correction, which in turn introduce strong non-linear field effects that limit the beam dynamic aperture. In order to maximize the dynamic aperture we choose the cell phases to cancel the third and fourth order geometric resonances in each 8-cell arc. Four families of chromatic sextupoles and six families of geometric (or harmonic) sextupoles are added to correct the chromatic and amplitude-dependent tunes. To find the best settings of the ten sextupole families, we use a Multi-Objective Genetic Optimizer employing elegant to optimize the beam lifetime and dynamic aperture simultaneously. Then we evaluate dynamic aperture reduction caused by magnetic field multipole errors, magnet fabrication errors and misalignments. A sufficient dynamic aperture is obtained for injection, as well as workable beam lifetime.

43 PARTICLE ACCELERATORS↗

DOE OSTI2013

MULTILEVEL ACCELERATION OF STOCHASTIC COLLOCATION METHODS FOR PDE WITH RANDOM INPUT DATA

Stochastic Collocation (SC) methods for stochastic partial differential equa- tions (SPDEs) suffer from the curse of dimensionality, whereby increases in the stochastic dimension cause an explosion of computational effort. To combat these challenges, multilevel approximation methods seek to decrease computational complexity by balancing spatial and stochastic discretization errors. As a form of variance reduction, multilevel techniques have been successfully applied to Monte Carlo (MC) methods, but may be extended to accelerate other methods for SPDEs in which the stochastic and spatial degrees of freedom are de- coupled. This article presents general convergence and computational complexity analysis of a multilevel method for SPDEs, demonstrating its advantages with regard to standard, single level approximation. The numerical results will highlight conditions under which multilevel sparse grid SC is preferable to the more traditional MC and SC approaches.

Webster, Clayton G↗

DOE OSTI2021

Physics-Guided Machine Learning for Prediction of Cloud Properties in Satellite-Derived Solar Data: Preprint

With over 20 years of high-resolution surface irradiance data covering most of the western hemisphere, the National Solar Radiation Database (NSRDB) is a vital public data asset. The NSRDB uses a two-step Physical Solar Model (PSM) that explicitly considers the effects of clouds and other atmospheric variables on radiative transfer. High-quality physical and optical cloud properties derived from satellite imagery are perhaps the most important data input to the PSM, representing the greatest source of radiation attenuation and scattering. However, traditional methods for cloud property retrieval have their own limitations and are unable to accurately predict cloud properties outside of nominal conditions. We introduce a physics-guided neural network that can accurately predict cloud properties when traditional methods fail or are inaccurate. Using this framework, we show reductions in relative Root Mean Square Error (RMSE) for Global Horizontal Irradiance (GHI) up to 13 percentage points for timesteps that previously had missing or low-quality cloud property data. We expect that this methodology will be effective in improving the quality of cloud property and solar irradiance data in the NSRDB.

41 EE - Solar Energy Technologies Office (EE-4S)↗