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Load following capability of CANDLE reactor by adjusting coolant operation condition

The load following capability of CANDLE reactor is investigated in the condition that the control rods are unavailable. Both sodium cooled metallic fuel fast reactor (SFR) and {sup 208}Pb cooled metallic fuel fast reactor (LFR) are investigated for their performance in power rate changing by changing its coolant operation condition; either coolant flow rate or coolant inlet temperature. The change by coolant flow rate is difficult especially for SFR because the maximum temperature criteria on cladding material may be violated. The power rate can be changed for its full range easily by changing the coolant temperature at the core inlet. LFR can reduce the same amount of power rate by smaller change of temperature than SFR. However, the coolant output temperature is generally decreased for this method and the thermal efficiency becomes worse.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Characteristics of TRU Fueled SFR Core during the Transition with Partially Loaded LEU Assemblies

The fast reactor (FR) fuels typically require higher fissile content than the thermal reactor fuels because the cross sections of the fissile isotopes are smaller relative to the fertile isotopes and higher neutron leakage from the reactor core. The medium-sized high-burnup sodium-cooled fast reactors (SFRs) in the framework of uranium-plutonium/transuranic (U/Pu or U/TRU) fuel-cycle can be optimized to operate with less than 17 % of Pu/TRU content in the driver fuel while having higher TRU conversion ratios (CR~1.0) [1]. However, possible shortage or inaccessibility to TRU based fuel could be accommodated by the use of uranium-based fuels on demand such as low enriched uranium (LEU) having significantly higher 235U content than used in the commercial light water reactors (LWRs), which is defined as high-assay LEU. The reactor systems having low TRU conversion ratio are commonly categorized as burner reactors, which include LWRs and even can be achieved by FRs with designed to utilize higher TRU fractions (e.g., increased neutron leakage and lower fuel volume fractions). Such reactor systems need to be initially loaded with high excess reactivity, which decreases toward the end of cycle, in order to achieve target burnup conditions. Therefore, in order to offset the excess reactivity, neutron absorbing materials need to be inserted into the core to compensate (e.g., control rods). By reducing the neutron leakage (e.g., increasing the fuel volume fraction or thicker blankets), the TRU conversion ratio in the FR can be increased. If the TRU conversion ratio becomes 1.0 (technically slightly greater than 1.0 to account for process losses during recycle), the reactor is in the condition known as “breakeven”, in which fuel contains the same amount of fissile material after recycling that was used to fuel the reactor. In such a condition, combined with the fact that fission products do not have strong poisoning effects in FRs, the reactivity swing becomes smaller than that of burner type reactors. For breeders, the reactivity can increase toward the end of the cycle because more fissile material is produced than consumed. In this regard, the breakeven FR core is implicitly optimized in a sense by eliminating the large insertion of control elements to offset the reactivity during the normal operation. However, the breakeven condition here is assumed to be achieved only by the TRU based fuel. Possible lack of TRU based fuel needs to be compensated by available LEU resources containing equivalent amount of fissile (i.e., 235U). The use of LEU will have some impact on important safety parameters that need to be evaluated. U-235 has a higher effective delayed neutron fraction than Pu-239. Also, the number of neutrons produced by fissions per neutron absorption (i.e. ?) of 235U in the fast energy range (>1e4 eV) is lower than that of 239Pu, which may lead to the poor fissile conversion when LEU is used as a high-conversion FR fuel. The full-paper presents the study of the impact of partially loaded LEU fuels within TRU fueled breakeven SFR on the transition of nuclide evolutions and core characteristics particularly focusing on the burnup reactivity swing. The full paper analyzes how the large reactivity swing occurs during the LEU loading and addresses possible options to reduce it to the level equivalent to that of the TRU fueled SFR core.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Nuclear Safety [Vol. 32, No. 1, January-March 1991]

Nuclear Safety is a review journal that covers significant developments in the field of nuclear safety. Its scope includes the analysis and control of hazards associated with nuclear energy, operations involving fissionable materials, and the products of nuclear fission and their effects on the environment. Primary emphasis is on safety in reactor design, construction, and operation; however, the safety aspects of the entire fuel cycle, including fuel fabrication, spent-fuel processing, nuclear waste disposal, handling of radioisotopes, and environmental effects of these operations, are also treated. Table of Contents for this issue follows. GENERAL SAFETY CONSIDERATIONS: 1 The Safety Review and Approval Process for Space Nuclear Power Sources, G. L. Bennett; 19 Report on the American Nuclear Society International Topical Meeting: "The Safety, Status, and Future of Non-Commercial Reactors and Irradiation Facilities", E. G. Silver; 35 Book Review: Fission Product Transport Processes in Reactor Accidents, Proceedings to the International Centre tor Heat and Mass Processes T. S. Kress; 38 Fast Reactor Technology in the 1990s: A Summary of the 1990 International Fast Reactor Safety Meeting, A. E. Levin; ACCIDENT ANALYSIS: 56 Effects of Chemical Phenomena on LWR Severe Accident Fission Product Behavior, A. P. Malinauskas and T. S. Kress; CONTROL AND INSTRUMENTATION: 65 Technical Note: Safety Parameter Display Systems—10 Years Later, R. J. Eckenrode; 68 Potential Application of Neural Networks to the Operation of Nuclear Power Plants, R. E. Uhrig; DESIGN FEATURES: 80 Twenty-First DOE/NRC Nuclear Air-Cleaning Conference, R. R. Bellamy, D. W. Moeller, and M. W. First; 91 Impact of an Apparent Radiation Embrittlement Rate on the Life Expectancy of PWR Vessel Supports, R. D. Cheverton, G. C. Robinson, W. E. Pennell, and R. K. Nanstad; ENVIRONMENTAL EFFECTS: 103 Technical Note: The Impact of Offsite Factors on the Safety Performance of Small Nuclear Power Plants, Yu. D. Baranaev and A. N. Viktorov; WASTE AND SPENT FUEL MANAGEMENT: 109 Activities Related to Waste Management, Compiled by E. G. Silver; OPERATING EXPERIENCES: 118 Reactor Shutdown Experience, Compiled by J. W. Cletcher; 121 Selected Safety-Related Events, Compiled by G. A. Murphy; 123 Operating U.S. Power Reactors, Compiled by E. G. Silver; RECENT DEVELOPMENTS: 140 General Administrative Activities, Compiled by E. G. Silver; 150 Reports, Standards, and Safety Guides, D. S. Queener; 155 Status of Power-Reactor Licensing Activities, Compiled by E. G. Silver; 157 Proposed Rule Changes as of Sept. 30, 1990; ANNOUNCEMENTS: 79 MIT Offers Summer Program on Nuclear Power Reactor Safety; 108 Harvard School of Public Health Offers Several Short Courses; 139 Short Course and Workshop on Nuclear Criticality Safety at University of New Mexico; 160 SCK/CEN Announces Training Course on Emergency Planning and Response; 161 The Authors; 164 Indexes to Nuclear Safety, Volume 31

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Fuel Cycle Study to Developing a Viable Long Term Nuclear Power Scenario for the UK

Within the UK a closed fuel cycle has been in operation for decades but with the introduction of a new build programme to create 16 GWe capacity using LWR technology and with the closure of the UK's reprocessing industry, an open fuel cycle will be implemented beyond 2020. However, it is expected that 16 GWe nuclear capacity will not be enough for the UK to curb greenhouse gas emissions through increased demand for low carbon electricity, and tackle energy security. As such further nuclear expansion scenarios are being considered between 40 and 75 GWe by 2050. This study evaluates a viable 40 GWe UK nuclear scenario, evaluating the extent to which key drivers can impact a future UK nuclear energy strategy, including; the ability to sustain a relatively high nuclear capacity, fresh uranium availability, accumulation of spent fuel at decommissioning nuclear reactor sites and capacity requirements of future GDF host sites. The thermal reactor open fuel cycle is the de-facto standard around the world for many reasons including the reliance on extremely mature technology, significant operational experience and most importantly a relatively low cost. However, the premise that a thermal reactor open fuel cycle is the correct one to adopt long term is dependent on the notion that large quantities of UO{sub 2} spent fuel can eventually be disposed of in a geological disposal facility and the future availability of fresh uranium. The total amount of available uranium is unknown and if extraction from seawater proves to be economic and practical then any future concerns regarding supply disappear. Spent fuel disposability on the other hand has never been performed on a commercial scale and there is some uncertainty when and whether this can be achieved. This paper will follow from previous work already presented in 2013 [REF] which examined UK fuel cycles involving the transition to a closed fast reactor fleet by the end of this century. The revised scenarios now assume fast reactors are required later in the scenario, in-line with other countries. In addition, the new study has used physics methods originally developed by SKB to assess the physical size of the repository required to dispose of all intermediate and high level waste whilst ensuring temperature limits imposed by the engineered barriers and surrounding geology are adhered to. The disposition of less Am-241 in the repository will no doubt lead to a reduction in GDF footprint. However, this may not be important to GDF design and economics. The purpose of this paper is to also critically review the importance of and put into perspective a smaller GDF footprint and lower fissile inventory. (authors)

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Generating unstructured nuclear reactor core meshes in parallel

Recent advances in supercomputers and parallel solver techniques have enabled users to run large simulations problems using millions of processors. Techniques for multiphysics nuclear reactor core simulations are under active development in several countries. Most of these techniques require large unstructured meshes that can be hard to generate in a standalone desktop computers because of high memory requirements, limited processing power, and other complexities. We have previously reported on a hierarchical lattice-based approach for generating reactor core meshes. Here, we describe efforts to exploit coarse-grained parallelism during reactor assembly and reactor core mesh generation processes. We highlight several reactor core examples including a very high temperature reactor, a full-core model of the Korean MONJU reactor, a ¼ pressurized water reactor core, the fast reactor Experimental Breeder Reactor-II core with a XX09 assembly, and an advanced breeder test reactor core. The times required to generate large mesh models, along with speedups obtained from running these problems in parallel, are reported. A graphical user interface to the tools described here has also been developed.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Experimentally Known Properties of U-10Zr Alloys: A Critical Review

More than 14000 U-10Zr fuel rods (alloys of U with 10 wt% Zr) Zr were been irradiated in the Experimental Breeder Reactor II and Fast Flux Test Facility, with some irradiated to burnups of almost 20 at%. However, very little information about properties of un-irradiated U-10Zr alloys is available. This data is needed to help with interpretation of data from irradiated materials, develop and validate phase diagrams and models of U-Zr and more complex systems, develop and validate fuel-performance codes, design fuels for future fast reactors, and design future experimental investigations to fill in crucial gaps in knowledge. This paper provides a summary and critical review of the available experimental data on phases and phase diagrams, electrical properties, thermal expansion, thermal conductivity, heat capacity, mechanical properties, vapor pressures, and thermodynamic properties of un-irradiated U-10Zr alloys. As a result, much of this data was published before ~1970 and is available only in obscure reports.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Simplified Approach for Scoping Assessment of Non-LWR Source Terms

This report describes a structure to aid in evaluation of release mitigation strategies across a range of reactor technologies. The assessment performed for example reactor concepts utilizes previous studies of postulated accident sequences for each reactor concept. This simplified approach classifies release mitigation strategies based on a range of barriers, physical attenuation processes, and system performance. It is not, however, intended to develop quantitative estimates of radiological release magnitudes and compositions to the environment. Rather, this approach is intended to identify the characteristics of a reactor design concepts release mitigation strategies that are most important to different classes of accident scenarios. It uses a scoping methodology to provide an approximate, order-of-magnitude, estimate of the radiological release to the environment and associated off-site consequences. This scoping method is applied to different reactor concepts, considering the performance of barriers to fission product release for these concepts under sample accident scenarios. The accident scenarios and sensitivity evaluations are selected in this report to evaluate the role of different fission product barriers in ameliorating the source term to the environment and associated off-site consequences. This report applies this structure to characterize how release mitigation measures are integrated to define overall release mitigation strategies for High Temperature Gas Reactors (HTGRs), Sodium Fast Reactors (SFRs), and liquid fueled Molten Salt Reactors (MSRs). To support this evaluation framework, factors defining a chain of release attenuation stages, and thus an overall mitigation strategy, must be established through mechanistic source term calculations. This has typically required the application of an integral plant analysis code such as MELCOR. At present, there is insufficient evidence to support a priori evaluation of the effectiveness of a release mitigation strategy for advanced reactor concepts across the spectrum of events that could challenge the radiological containment function. While it is clear that these designs have significant margin to radiological release to the environment for the scenarios comprising the design basis, detailed studies have not yet been performed to assess the risk profile for these plants. Such studies would require extensive evaluation across a reasonably complete spectrum of accident scenarios that could lead to radiological release to the environment.

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Overview of Advanced Reactor Simulation Capabilities to Support Demonstrations

The Virtual Test Bed (VTB) was established to support the deployment of advanced reactors by facilitating the use of state-of-the-art modeling and simulation capabilities. These tools are able to solve previously prohibitive challenge problems in greater levels of fidelity and in a multi-physics framework. A VTB repository was recently set up to host models for a wide variety of reactor types and using a range of NEAMS-developed software. Table I summarizes the different capabilities already available in the repository and up-and-coming near/long term ones. The repository currently hosts models for a wide variety of reactor types, including High-Temperature Gas Cooled Reactors (HTGR), Sodium Fast Reactors (SFR), Fluoride salt cooled High-temperature Reactors (FHR), Molten Salt Reactors (MSR), and Heat-Pipe Microreactors (HP-MR). It should be noted that work is ongoing for all of the models and each example problem is at a different state of maturity.

99 GENERAL AND MISCELLANEOUS↗

Preliminary Radioisotope Screening for Off-site Consequence Assessment of Advanced Non-LWR Systems

Currently a set of 71 radionuclides are accounted for in off-site consequence analysis for LWRs. Radionuclides of dose consequence are expected to change for non-LWRs, with radionuclides of interest being type-specific. This document identifies an expanded set of radionuclides that may need to be accounted for in multiple non-LWR systems: high temperature gas reactors (HTGRs); fluoride-salt-cooled high-temperature reactors (FHRs); thermal-spectrum fluoride-based molten salt reactors (MSRs); fast-spectrum chloride-based MSRs; and, liquid metal fast reactors with metallic fuel (LMRs) Specific considerations are provided for each reactor type in Chapter 2 through Chapter 5, and a summary of all recommendations is provided in Chapter 6. All identified radionuclides are already incorporated within the MACCS software, yet the development of tritium-specific and carbon-specific chemistry models are recommended.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Thermal Extraction Modeling within HYBRID: Nominal and Extraction Conditions in Advanced Reactor Systems

This document details continuing development of thermal extraction modeling within the HYBRID repository, the modeling repository of the Integrated Energy Systems program at Idaho National Laboratory. The focus of the thermal extraction work is setting up template energy conversion systems for advanced reactor systems. Based on these nominal conditions, the IES team is developing extraction capability maps that present the system thermal-to-electric efficiency of the remaining system and the mass extraction fraction capability of these systems when extracting steam at various pressures to send steam to applications at a lower given pressure. These curves are mapped on what has become termed “whale chart” due to the appearance of the results. Multiple advanced reactor systems are complete, and it is anticipated that all four of the main advanced reactor types: advanced light-water reactors, high temperature gas reactors, liquid metal fast reactors, and molten salt reactors, will be complete by the end of the fiscal year.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Molten Salt Reactor Experiment Simulation using Shift/Griffin

The Department of Energy (DOE)’s NEAMS focuses its efforts on the development of advanced modeling and simulation (M&S) tools for light-water reactors (LWRs) and non–LWRs (i.e., molten salt reactors, high-temperature gas reactors, microreactors, and fast reactors). In the previous fiscal year, the Multiphysics Applications Driver Technical Area funded molten salt reactor (MSR) M&S at Oak Ridge National Laboratory (ORNL) to generate multigroup macroscopic cross sections with Shift for a MSRE 2D lattice model in Griffin. In addition, Shift’s capability to calculate gamma dose rates from activated components in the primary exchangers in a molten salt breeder reactor was also demonstrated. In fiscal year 2023, ORNL generated multigroup macroscopic cross sections using Shift for a 3D MSRE core model. MSRE depletion calculations using Griffin were also demonstrated in this fiscal year. For the depletion calculation, one-group microscopic cross sections for the 3D MSRE core were generated using Shift, and the decay transmutation library from ORIGEN was converted to an ISOXML file, which is required as input in Griffin. Several Monte Carlo codes, such as OpenMC and Serpent, were also used to benchmark and supplement multigroup cross sections generated by Shift. Multigroup libraries were generated with 8 and 20 group structures, and the study found the 8-group structure to be more accurate when comparing Griffin results to continuous energy (CE) Monte Carlo results. The average flux from CE Shift calculations is up to ~6% higher than the CE Serpent calculations because of different values applied for the energy released per fission (κ values). The average flux in the fuel salt calculated by Griffin using cross sections generated with Shift agrees well with the reference CE Shift solution; the same is valid for the corresponding Serpent results. The maximum relative error is ~6% and ~2% compared to the CE Shift and Serpent reference solutions, respectively. Meanwhile, the average flux calculated by Griffin in the graphite moderator shows a higher difference in the thermal range when compared to both reference Monte Carlo solutions; this result suggests a need for improvement in cross section generation for the graphite moderator in the thermal range in both Monte Carlo codes. Griffin depletion calculations using cross sections from Shift and Serpent were performed and compared against ORIGEN calculations, and the nuclide densities calculated by Griffin were found to be generally in agreement with those of ORIGEN. Because a different approach was taken to calculate the energy released per fission ( κ values) in Shift and Serpent, a difference in nuclide densities from differences in the average flux was observed between Griffin using Serpent and Shift cross sections. Griffin calculations with Shift cross sections produced higher average flux in the salt than with Serpent cross sections, leading to higher consumption of 235 U and higher production of 135 Xe. For time-dependent depletion calculations, cross sections were generated with Serpent, and Griffin’s results using these cross sections were compared to CE Serpent depletion results, demonstrating good agreement. The average difference in keff between Serpent and Griffin as a function of burnup is about 155 pcm. Similarly, good agreement with small differences up to ~0.5% was also noticed in the nuclide density of 235 U and 135 Xe. More details regarding the methodologies invoked to generate the cross section to make code-to-code comparisons are discussed further in this report. User feedback on Griffin and Shift capabilities that will enhance these calculations is provided in this report for future consideration. The work performed this fiscal year can be extended further for multiphysics coupling of Griffin-Pronghorn/SAM with Mole to study precursor flow and salt chemistry.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Evaluating High-Halide Waste Form Options for Salt-Based Nuclear Waste Simulants

In this study, waste forms were being explored for an electrochemical salt simulant, , referred to as ERV3, which is a high-LiCl/KCl salt containing simulated fission products (i.e., Sr, Cs, Nd) and Na to represent bond sodium from Experimental Breeder Reactor-II metallic fast reactor fuel. The goal was to find glassy systems that could be used to immobilize the salt in a single-step process. The envisionment of this process would be find a frit glass that could be added to the salt waste, heat treated, poured into waste canisters, and then stored for disposal. To perform this study, a literature review was conducted, the most promising seven systems were fabricated without the salt, and then mixed with salt simulant and heat treated under different processes. The criteria that were used to screen potential compositions included demonstrated alkali incorporation, could be melted at reasonably low temperature ( T ≤ 1000°C), and if the compositions had some demonstrated data for waste-form-related properties, that was a benefit. High marks were given for compositions that showed amorphous nature after slow cooling of samples containing ERV3.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Steam Generators: Thermal Hydraulic Measurements and Instrumentation

Steam generators are integral components of both conventional and advanced reactors utilizing steam power cycles, as they influence the power conversion performance. Steam generator designs are highly influenced by the type of reactor coolant used, which mainly governs the different control, monitoring, and safety system actuation requirements. Therefore, the present work reviews the thermal hydraulics instrumentation within steam generators designed for pressurized water reactors (PWRs), high-temperature gas-cooled reactors (HTGRs), sodium fast reactors (SFRs), and molten salt cooled reactors (MSRs). Emphasis is given to measurement techniques that are either unique or particularly important to specific reactor types. Lastly, a discussion is provided on the instrumentation and measured parameters. The work identifies standard parameters of interest and is expected to aid the development of test beds and novel measurements techniques.

21 - SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLAN↗

Editorial: Benchmark experiments, development and needs in support of advanced reactor design

Advanced nuclear reactor designs will for the most part be a departure from low enrichment light water reactor (LWR) designs currently operated around the world. Such advanced designs include but are not limited to new TRISO-fueled high temperature gas reactors, heat-pipe cooled micro-reactors, fluoride salt cooled high-temperature reactors, molten salt reactors, lead cooled fast reactors, nuclear thermal propulsion concepts, and include LWR designs with advanced fuel and clad types. Modeling and simulation methods for advanced reactors is necessary for regulators to approve license requests. However, regulators also require that modeling approaches be validated against experimental measurements. Hence, there is a crucial need for data for advanced reactor systems that will support validation of analysis methods. To this end, this Research Topic includes eleven papers organized into topical seven categories relevant for advanced reactor design.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Heat pipe nuclear reactor for space power

A heat-pipe-cooled nuclear reactor has been designed to provide 3.2 MWth to an out-of-core thermionic conversion system. The reactor is a fast reactor designed to operate at a nominal heat-pipe temperature of 1675 K. Each reactor fuel element consists of a hexagonal molybdenum block which is bonded along its axis to one end of a molybdenum/lithium-vapor heat pipe. The block is perforated with an array of longitudinal holes which are loaded with UO2 pellets. The heat pipe transfers heat directly to a string of six thermionic converters which are bonded along the other end of the heat pipe. An assembly of 90 such fuel elements forms a hexagonal core. The core is surrounded by a thermal radiation shield, a thin thermal neutron absorber, and a BeO reflector containing boron-loaded control drums.

Koening, D. R.↗

Demonstration of ACCERT Software for Nuclear Power Plant Techno-Economics

In the past few years, there has been a renewed interest in the deployment of nuclear power for decarbonizing the electricity grid as well as a range of industrial applications. As the demonstrations of advanced nuclear power plants start to begin, there will likely be a further increase in this interest. As nuclear is being considered as a part of the energy mix, understanding the cost of nuclear energy becomes increasingly important for all stakeholders including advanced reactor vendors (for making design decisions and marketing their designs), users of nuclear energy (e.g., to estimate the cost of decarbonization of other industries using nuclear), and government (e.g., in capacity expansion models that are used in framing policy). In this summary, we demonstrate a software tool called ACCERT that is currently being developed with funding from the Systems Analysis and Integration (SA&I) program under the Department of Energy’s Office of Nuclear Energy (DOE NE). ACCERT is a cost estimation and techno-economics tool for nuclear power plant applications that includes a database of (a) cost estimates of various ‘reference’ nuclear power plant designs gathered from existing literature, and (b) algorithms developed from these costs that can be used extrapolate the existing costs and perform a bottom-up cost estimation of other designs. A companion summary describes the software and its design in more detail and this summary presents a demonstration for four different nuclear power plant designs: a pressurized water reactor (PWR), high-temperature gas reactor (HTGR), sodium fast reactor (SFR), and a heat-pipe microreactor. The demonstrations include the reference cost estimates and the cost estimates of a modified design for each reference case.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Sodium Spray Fire Simulations using CONTAIN-LMR

License applications for sodium fast reactors will include sodium fire analysis and subsequent mitigation strategies. Sodium leaks or ruptures from piping and support systems can lead to significant fires due to the reactive nature of sodium with air and water. Understanding the behavior of sodium fires is crucial for modeling and predicting accidents in sodium fast reactors. This paper describes the initial results of a control volume code, CONTAIN-LMR (CLMR), modeling effort for a sodium spray fire experiment conducted at Sandia National Laboratories (SNL) in Albuquerque, New Mexico in 2010. Additional sodium spray and pool fire tests were conducted at SNL in 2009 and 2010 and will be compared to CLMR results in future papers. The purpose of this analysis was extract information from the evolution of the SNL tests to better understand how to use CLMR in future sodium fire analysis. Thus the following CLMR simulations were not completely the result of blind benchmarking study. (authors)

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Neutron Cross Section Covariances for Structural Materials and Fission Products

We describe neutron cross section covariances for 78 structural materials and fission products produced for the new US evaluated nuclear reaction library ENDF/B-VII.1. Neutron incident energies cover full range from 10{sup -5} eV to 20 MeV and covariances are primarily provided for capture, elastic and inelastic scattering as well as (n,2n). The list of materials follows priorities defined by the Advanced Fuel Cycle Initiative, the major application being data adjustment for advanced fast reactor systems. Thus, in addition to 28 structural materials and 49 fission products, the list includes also {sup 23}Na which is important fast reactor coolant. Due to extensive amount of materials, we adopted a variety of methodologies depending on the priority of a specific material. In the resolved resonance region we primarily used resonance parameter uncertainties given in Atlas of Neutron Resonances and either applied the kernel approximation to propagate these uncertainties into cross section uncertainties or resorted to simplified estimates based on integral quantities. For several priority materials we adopted MF32 covariances produced by SAMMY at ORNL, modified by us by adding MF33 covariances to account for systematic uncertainties. In the fast neutron region we resorted to three methods. The most sophisticated was EMPIRE-KALMAN method which combines experimental data from EXFOR library with nuclear reaction modeling and least-squares fitting. The two other methods used simplified estimates, either based on the propagation of nuclear reaction model parameter uncertainties or on a dispersion analysis of central cross section values in recent evaluated data files. All covariances were subject to quality assurance procedures adopted recently by CSEWG. In addition, tools were developed to allow inspection of processed covariances and computed integral quantities, and for comparing these values to data from the Atlas and the astrophysics database KADoNiS.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗