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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 73 records · Page 4
All sourcesNASA NTRSDOE OSTI
NASA NTRS1997

Laboratory Kinetic Studies of OH and CO2 Relevant to Upper Atmospheric Radiation Balance

The purpose of this project was to quantify the rates of two processes which are crucial to our understanding of radiative energy balance in the upper atmosphere. The first process is radiative emission from vibrationally hot OH radicals following the H + O3 reaction in the upper mesosphere. The importance of this process depends strongly on the OH radiative emission coefficients. Our goal was to measure the OH permanent dipole moment in excited vibrational states and to use these measurements to construct an improved OH dipole moment function and improved radiative emission coefficients. Significant progress was made on these experiments including the construction of a supersonic jet source for vibrationally excited OH radicals. Unfortunately, our efforts to transport the OH radicals into a second lower pressure vacuum chamber were not successful, and we were unable to make improved dipole moment measurements for OH. The second key kinetic process which we attempted to quantify during this project is the rate of relaxation of bend-excited CO2 by oxygen atoms. Since excitation of the bending vibrational mode of CO2 is the major cooling mechanism in the upper mesosphere/lower thermosphere, the cooling rate of this region depends crucially on the rate of energy transfer out of this state. It is believed that the most efficient transfer mechanism is via atomic oxygen but the rate for this process has not been directly measured in the laboratory at appropriate temperatures and even the room temperature rate remains controversial. We attempted to directly measure the relaxation rate Of CO2 (010) by oxygen atoms using the discharge flow technique. This experiment was set up at Aerodyne Research. Again, significant progress was achieved in this experiment. A hot CO2 source was set up, bend excited CO2 was detected and the rate of relaxation of bend excited CO2 by He atoms was measured. Unfortunately, the project ran out of time before the oxygen atom kinetic studies could be implemented.

Nelson, David D.↗
NASA NTRS1979

A GCM simulation of the earth-atmosphere radiation balance for winter and summer

The radiation balance of the earth-atmosphere system simulated by using the general circulation model (GCM) of the Laboratory for Atmospheric Sciences (GLAS) is examined in regards to its graphical distribution, zonally-averaged distribution, and global mean. Most of the main features of the radiation balance at the top of the atmosphere are reasonably simulated, with some differences in the detailed structure of the patterns and intensities for both summer and winter in comparison with values as derived from Nimbus and NOAA (National Oceanic and Atmospheric Administration) satellite observations. Both the capability and defects of the model are discussed.

Wu, M. L. C.↗
NASA NTRS2011

Spectrally-Invariant Approximation Within Atmospheric Radiative Transfer

Certain algebraic combinations of single scattering albedo and solar radiation reflected from, or transmitted through, vegetation canopies do not vary with wavelength. These "spectrally invariant relationships" are the consequence of wavelength independence of the extinction coefficient and scattering phase function in vegetation. In general, this wavelength independence does not hold in the atmosphere, but in cloud~dominated atmospheres the total extinction and total scattering phase function vary only weakly with wavelength. This paper identifies the atmospheric conditions under which the spectrally invariant approximation can accurately describe the extinction. and scattering properties of cloudy atmospheres. The validity of the assumptions and the accuracy of the approximation are tested with ID radiative transfer calculations using publicly available radiative transfer models: Discrete Ordinate Radiative Transfer (DISORT) and Santa Barbara DISORT Atmospheric Radiative Transfer (SBDART). It is shown for cloudy atmospheres with cloud optical depth above 3, and for spectral intervals that exclude strong water vapor absorption, that the spectrally invariant relationships found in vegetation canopy radiative transfer are valid to better than 5%. The physics behind this phenomenon, its mathematical basis, and possible applications to remote sensing and climate are discussed.

Marshak, A.↗
NASA NTRS2011

Spectrally Invariant Approximation within Atmospheric Radiative Transfer

Certain algebraic combinations of single scattering albedo and solar radiation reflected from, or transmitted through, vegetation canopies do not vary with wavelength. These spectrally invariant relationships are the consequence of wavelength independence of the extinction coefficient and scattering phase function in vegetation. In general, this wavelength independence does not hold in the atmosphere, but in cloud-dominated atmospheres the total extinction and total scattering phase function vary only weakly with wavelength. This paper identifies the atmospheric conditions under which the spectrally invariant approximation can accurately describe the extinction and scattering properties of cloudy atmospheres. The validity of the assumptions and the accuracy of the approximation are tested with 1D radiative transfer calculations using publicly available radiative transfer models: Discrete Ordinate Radiative Transfer (DISORT) and Santa Barbara DISORT Atmospheric Radiative Transfer (SBDART). It is shown for cloudy atmospheres with cloud optical depth above 3, and for spectral intervals that exclude strong water vapor absorption, that the spectrally invariant relationships found in vegetation canopy radiative transfer are valid to better than 5%. The physics behind this phenomenon, its mathematical basis, and possible applications to remote sensing and climate are discussed.

Marshak, A.↗
NASA NTRS2021

Solving Global Cirrus Cloud Top-of-the-Atmosphere Radiative Forcing from Satellite Lidar

We estimate top-of-the-atmosphere (TOA) cirrus cloud radiative forcing from satellite lidar observations. We describe the technical innovations necessary to conduct this experiment. Specifically, we highlight advances in broadband radiative transfer modeling, and the optical and physical parameterizations necessary to run them. We present two years of results, across two decades (2008 vs. 2018), highlighting seasonal and annual differences. The goal of this endeavor is to standardize mechanics for transitioning this work to operational Level 2 ground and satellite lidar products moving forward. However, the unique TOA forcing characteristics of cirrus clouds are also discussed, including specifically daytime characteristics than can oscillate between warming and cooling regionally.

James R Campbell↗
NASA NTRS1988

Effects of cirrus composition on atmospheric radiation budgets

A radiative transfer model that can be used to determine the change in solar and infrared fluxes caused by variations in the composition of cirrus clouds was used to investigate the importance of particle size and shape on the radiation budget of the Earth-atmosphere system. Even though the cloud optical thickness dominates the radiative properties of ice clouds, the particle size and nonsphericity of ice crystals are also important in calculations of the transfer of near-IR solar wavelengths. Results show that, for a given optical thickness, ice clouds composed of larger particles would produce larger greenhouse effects than those composed of smaller particles. Moreover, spherical particles with equivalent surface areas, frequently used for ice crystal clouds, would lead to an overestimation of the greenhouse effect.

Kinne, Stefan↗
NASA NTRS2021

Less Atmospheric Radiative Heating By Dust Due to the Synergy of Coarser Size and Aspherical Shape

Mineral dust aerosols cool and warm the atmosphere by scattering and absorbing solar (shortwave: SW) and thermal (longwave: LW) radiation. However, significant uncertainties remain in dust radiative effects, largely due to differences in the dust size distribution and spectral optical properties simulated in Earth system models. Dust models typically underestimate the coarse dust load (more than 2.5 µm in diameter) and assume a spherical shape, which leads to an overestimate of the fine dust load (less than 2.5 µm) after the dust emissions in the models are scaled to match observed dust aerosol optical depth at 550 nm (DAOD550). Here, we improve the simulated dust properties with data sets that leverage measurements of size-resolved dust concentration, asphericity factor, and refractive index in a coupled global chemical transport model with a radiative transfer module. After the adjustment of size-resolved dust concentration and spectral optical properties, the global and annual average of DAOD550 from the simulation increases from 0.023 to 0.029 and falls within the range of a semi-observationally based estimate (0.030 ± 0.005). The reduction of fine dust load after the adjustment leads to a reduction of the SW cooling at the top of the atmosphere (TOA). To improve agreement against a semi-observationally based estimate of the radiative effect efficiency at TOA, we find that a less absorptive SW dust refractive index is required for coarser aspherical dust. Thus, only a minor difference is estimated for the net global dust radiative effect at TOA (−0.08 vs. −0.00 W m−2 on a global scale). Conversely, our sensitivity simulations reveal that the surface warming is substantially enhanced near the strong dust source regions (less cooling to −0.23 from −0.60 W m−2 on a global scale). Thus, less atmospheric radiative heating is estimated near the major source regions (less heating to 0.15 from 0.59 W m−2 on a global scale), because of enhanced LW warming at the surface by the synergy of coarser size and aspherical shape.

simulated dust properties↗
NASA NTRS2009

Monitoring Top-of-Atmosphere Radiative Energy Imbalance for Climate Prediction

Large climate feedback uncertainties limit the prediction accuracy of the Earth s future climate with an increased CO2 atmosphere. One potential to reduce the feedback uncertainties using satellite observations of top-of-atmosphere (TOA) radiative energy imbalance is explored. Instead of solving the initial condition problem in previous energy balance analysis, current study focuses on the boundary condition problem with further considerations on climate system memory and deep ocean heat transport, which is more applicable for the climate. Along with surface temperature measurements of the present climate, the climate feedbacks are obtained based on the constraints of the TOA radiation imbalance. Comparing to the feedback factor of 3.3 W/sq m/K of the neutral climate system, the estimated feedback factor for the current climate system ranges from -1.3 to -1.0 W/sq m/K with an uncertainty of +/-0.26 W/sq m/K. That is, a positive climate feedback is found because of the measured TOA net radiative heating (0.85 W/sq m) to the climate system. The uncertainty is caused by the uncertainties in the climate memory length. The estimated time constant of the climate is large (70 to approx. 120 years), implying that the climate is not in an equilibrium state under the increasing CO2 forcing in the last century.

Lin, Bing↗
NASA NTRS2003

Angular Distribution Models for Top-of-Atmosphere Radiative Flux Estimation from the Clouds and the Earth's Radiant Energy System Instrument on the Tropical Rainfall Measuring Mission Satellite: Validation - Part II

Top-of-atmosphere (TOA) radiative fluxes from the Clouds and the Earth s Radiant Energy System (CERES) are estimated from empirical angular distribution models (ADMs) that convert instantaneous radiance measurements to TOA fluxes. This paper evaluates the accuracy of CERES TOA fluxes obtained from a new set of ADMs developed for the CERES instrument onboard the Tropical Rainfall Measuring Mission (TRMM). The uncertainty in regional monthly mean reflected shortwave (SW) and emitted longwave (LW) TOA fluxes is less than 0.5 W/sq m, based on comparisons with TOA fluxes evaluated by direct integration of the measured radiances. When stratified by viewing geometry, TOA fluxes from different angles are consistent to within 2% in the SW and 0.7% (or 2 W/sq m) in the LW. In contrast, TOA fluxes based on ADMs from the Earth Radiation Budget Experiment (ERBE) applied to the same CERES radiance measurements show a 10% relative increase with viewing zenith angle in the SW and a 3.5% (9 W/sq m) decrease with viewing zenith angle in the LW. Based on multiangle CERES radiance measurements, 18 regional instantaneous TOA flux errors from the new CERES ADMs are estimated to be 10 W/sq m in the SW and, 3.5 W/sq m in the LW. The errors show little or no dependence on cloud phase, cloud optical depth, and cloud infrared emissivity. An analysis of cloud radiative forcing (CRF) sensitivity to differences between ERBE and CERES TRMM ADMs, scene identification, and directional models of albedo as a function of solar zenith angle shows that ADM and clear-sky scene identification differences can lead to an 8 W/sq m root-mean-square (rms) difference in 18 daily mean SW CRF and a 4 W/sq m rms difference in LW CRF. In contrast, monthly mean SW and LW CRF differences reach 3 W/sq m. CRF is found to be relatively insensitive to differences between the ERBE and CERES TRMM directional models.

Loeb, N. G.↗
NASA NTRS1990

Calculations of atmospheric radiative flux profiles

Results are presented of experiments with a diagnostic approach to the radiation budget by using all available data sets to describe the properties of the atmosphere, clouds, and surface at each time and place, together with a radiative transfer model that calculates the radiative fluxes using this information. Each parameter in the calculations is represented explicitly, so that improved data sets can be easily substituted. The model and data are combined to calculate profiles of radiative fluxes, including individual flux components, heating/cooling rates, as well as top-of-atmosphere and surface radiation budget components. The advantage of this explicit approach is that all contributions to the radiation budget can be diagnosed separately; in particular, cloud-radiative feedbacks can be isolated from the effects of other atmospheric and surface changes.

Rossow, William B.↗
NASA NTRS1982

A simple method to compute the change in earth-atmosphere radiative balance due to a stratospheric aerosol layer

A computer code was developed in terms of a three-layer model for the earth-atmosphere system, using a two-stream approximation for the troposphere and stratosphere. The analysis was limited to variable atmosphere loading by solar radiation over an unperturbed section of the atmosphere. The scattering atmosphere above a Lambertian ground layer was considered in order to derive the planar albedo and the spherical albedo. Attention was given to the influence of the aerosol optical thickness in the stratosphere, the single scattering albedo and asymmetry factor, and the sublayer albedo. Calculations were performed of the zonal albedo and the planetary radiation balance, taking into account a stratospheric aerosol layer containing H2SO4 droplets and volcanic ash. The resulting ground temperature disturbance was computed using a Budyko (1969) climate model. Local decreases in the albedo in the summer were observed in high latitudes, implying a heating effect of the aerosol. An accompanying energy loss of 23-27 W/sq m was projected, which translates to surface temperature decreases of either 1.1 and 0.45 C, respectively, for background and volcanic aerosols.

Lenoble, J.↗
NASA NTRS2015

Next-Generation Angular Distribution Models for Top-of-Atmosphere Radiative Flux Calculation from CERES Instruments: Validation

Radiative fluxes at the top of the atmosphere (TOA) from the Clouds and the Earth's Radiant Energy System (CERES) instrument are fundamental variables for understanding the Earth's energy balance and how it changes with time. TOA radiative fluxes are derived from the CERES radiance measurements using empirical angular distribution models (ADMs). This paper evaluates the accuracy of CERES TOA fluxes using direct integration and flux consistency tests. Direct integration tests show that the overall bias in regional monthly mean TOA shortwave (SW) flux is less than 0.2Wm(exp -2) and the RMSE is less than 1.1Wm(exp -2). The bias and RMSE are very similar between Terra and Aqua. The bias in regional monthly mean TOA LW fluxes is less than 0.5Wm(exp -2) and the RMSE is less than 0.8Wm(exp -)2 for both Terra and Aqua. The accuracy of the TOA instantaneous flux is assessed by performing tests using fluxes inverted from nadir- and oblique-viewing angles using CERES along-track observations and temporally and spatially matched MODIS observations, and using fluxes inverted from multi-angle MISR observations. The averaged TOA instantaneous SW flux uncertainties from these two tests are about 2.3% (1.9Wm(exp -2) over clear ocean, 1.6% (4.5Wm(exp -2) over clear land, and 2.0% (6.0Wm(exp -) over clear snow/ice; and are about 3.3% (9.0Wm(exp -2), 2.7% (8.4Wm(exp -2), and 3.7% (9.9Wm(exp -2) over ocean, land, and snow/ice under all-sky conditions. The TOA SW flux uncertainties are generally larger for thin broken clouds than for moderate and thick overcast clouds. The TOA instantaneous daytime LW flux uncertainties derived from the CERESMODIS test are 0.5% (1.5Wm(exp -2), 0.8% (2.4Wm(exp -2), and 0.7% (1.3Wm(exp -2) over clear ocean, land, and snow/ice; and are about 1.5% (3.5Wm(exp -2), 1.0% (2.9Wm(exp -2), and 1.1% (2.1Wm(exp -2) over ocean, land, and snow/ice under all-sky conditions. The TOA instantaneous nighttime LW flux uncertainties are about 0.5-1% (<2.0Wm(exp -2) for all surface types. Flux uncertainties caused by errors in scene identification are also assessed by using the collocated CALIPSO, CloudSat, CERES and MODIS data product. Errors in scene identification tend to underestimate TOA SW flux by about 0.6Wm(exp -2) and overestimate TOA daytime (nighttime) LW flux by 0.4 (0.2)Wm(exp -2) when all CERES viewing angles are considered.

Su, W.↗
NASA NTRS2007

Atmospheric Radiative Transfer for Satellite Remote Sensing: Validation and Uncertainty

My presentation will begin with the discussion of the Intercomparison of three-dimensional (3D) Radiative Codes (13RC) project that has been started in 1997. I will highlight the question of how well the atmospheric science community can solve the 3D radiative transfer equation. Initially I3RC was focused only on algorithm intercomparison; now it has acquired a broader identity providing new insights and creating new community resources for 3D radiative transfer calculations. Then I will switch to satellite remote sensing. Almost all radiative transfer calculations for satellite remote sensing are one-dimensional (1D) assuming (i) no variability inside a satellite pixel and (ii) no radiative interactions between pixels. The assumptions behind the 1D approach will be checked using cloud and aerosol data measured by the MODerate Resolution Imaging Spectroradiometer (MODIS) on board of two NASA satellites TERRA and AQUA. In the discussion, I will use both analysis technique: statistical analysis over large areas and time intervals, and single scene analysis to validate how well the 1D radiative transfer equation describes radiative regime in cloudy atmospheres.

Marshak, Alexander↗
NASA NTRS1998

Tools for Atmospheric Radiative Transfer: Streamer and FluxNet

Two tools for the solution of radiative transfer problems are presented. Streamer is a highly flexible medium spectral resolution radiative transfer model based on the plane-parallel theory of radiative transfer. Capable of computing either fluxes or radiances, it is suitable for studying radiative processes at the surface or within the atmosphere and for the development of remote-sensing algorithms. FluxNet is a fast neural network-based implementation of Streamer for computing surface fluxes. It allows for a sophisticated treatment of radiative processes in the analysis of large data sets and potential integration into geophysical models where computational efficiency is an issue. Documentation and tools for the development of alternative versions of Fluxnet are available. Collectively, Streamer and FluxNet solve a wide variety of problems related to radiative transfer: Streamer provides the detail and sophistication needed to perform basic research on most aspects of complex radiative processes while the efficiency and simplicity of FluxNet make it ideal for operational use.

Key, Jeffrey R.↗
NASA NTRS1990

Mapping transformations for broadband atmospheric radiation calculations

Two methods of mapping the line-by-line absorption coefficient (k) spectrum onto a new variable to produce a set of k coefficients which can be used for accurate and efficient broadband radiative transfer calculations in vertically inhomogeneous, nongray scattering atmospheres are described. These methods are intended for applications for which the less accurate correlated-k method is inadequate. These methods are tested for model atmospheres containing CO2 and H2O, with pressure in the range 0.05-0.9 bar. The results obtained differed by no more than 1 or 2 percent from the line-by-line results if the number of k coefficients was about 100 times less than the number required for the line-by-line calculation. These algorithms can be used for gas mixtures and for a variety of pressure-temperature profiles.

West, Robert↗
NASA NTRS1994

Martian atmospheric radiation budget

A computer model is used to study the radiative transfer of the martian winter-polar atmosphere. Solar heating at winter-polar latitudes is provided predominately by dust. For normal, low-dust conditions, CO2 provides almost as much heating as dust. Most heating by CO2 in the winter polar atmosphere is provided by the 2.7 micron band between 10 km and 30 km altitude, and by the 2.0 micron band below 10 km. The weak 1.3 micron band provides some significant heating near the surface. The minor CO2 bands at 1.4, 1.6, 4.8 and 5.2 micron are all optically thin, and produce negligible heating. O3 provides less than 10 percent of the total heating. Atmospheric cooling is predominantly thermal emission by dust, although CO2 15 micron band emission is important above 20 km altitude.

Lindner, Bernhard Lee↗
NASA NTRS1973

Method and apparatus for measuring solar activity and atmospheric radiation effects

A radiometric measuring system is described for observing solar activity, atmospheric attenuation, and atmospheric emission. Two highly directional microwave antennas are mounted side by-side on an equatorial mount which tracks the sun. One antenna is aimed directly at the sun to provide a sun temperature, and the other antenna is aimed at a slight angle to the sun antenna to provide a sky temperature reference. Signals from the two antennas are compared in a radiometric detecting system and provide information concerning solar activity and atmospheric attenuation and emission.

Haroules, G. G.↗
NASA NTRS1992

Top-of-atmosphere radiative fluxes - Validation of ERBE scanner inversion algorithm using Nimbus-7 ERB data

The ERBE algorithm is applied to the Nimbus-7 earth radiation budget (ERB) scanner data for June 1979 to analyze the performance of an inversion method in deriving top-of-atmosphere albedos and longwave radiative fluxes. The performance is assessed by comparing ERBE algorithm results with appropriate results derived using the sorting-by-angular-bins (SAB) method, the ERB MATRIX algorithm, and the 'new-cloud ERB' (NCLE) algorithm. Comparisons are made for top-of-atmosphere albedos, longwave fluxes, viewing zenith-angle dependence of derived albedos and longwave fluxes, and cloud fractional coverage. Using the SAB method as a reference, the rms accuracy of monthly average ERBE-derived results are estimated to be 0.0165 (5.6 W/sq m) for albedos (shortwave fluxes) and 3.0 W/sq m for longwave fluxes. The ERBE-derived results were found to depend systematically on the viewing zenith angle, varying from near nadir to near the limb by about 10 percent for albedos and by 6-7 percent for longwave fluxes. Analyses indicated that the ERBE angular models are the most likely source of the systematic angular dependences. Comparison of the ERBE-derived cloud fractions, based on a maximum-likelihood estimation method, with results from the NCLE showed agreement within about 10 percent.

Suttles, John T.↗