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At least 73 records · Page 4

Overview of Global/Regional Models Used to Evaluate Tropospheric Ozone in North America

Ozone (O3) is an important greenhouse gas, toxic pollutant, and plays a major role in atmospheric chemistry. Tropospheric O3 which resides in the planetary boundary layer (PBL) is highly reactive and has a lifetime on the order of days, however, O3 in the free troposphere and stratosphere has a lifetime on the order of weeks or months. Modeling O3 mixing ratios at and above the surface is difficult due to the multiple formation/destruction processes and transport pathways that cause large spatio-temporal variability in O3 mixing ratios. This talk will summarize in detail the global/regional models that are commonly used to simulate/predict O3 mixing ratios in the United States. The major models which will be focused on are the: 1) Community Multi-scale Air Quality Model (CMAQ), 2) Comprehensive Air Quality Model with Extensions (CAMx), 3) Goddard Earth Observing System with Chemistry (GEOS-Chem), 4) Real Time Air Quality Modeling System (RAQMS), 5) Weather Research and Forecasting/Chemistry (WRF-Chem) model, National Center for Atmospheric Research (NCAR)'s Model for OZone And Related chemical Tracers (MOZART), and 7) Geophysical Fluid Dynamics Laboratory (GFDL) AM3 model. I will discuss the major modeling components which impact O3 mixing ratio calculations in each model and the similarities/differences between these models. This presentation is vital to the 2nd Annual Tropospheric Ozone Lidar Network (TOLNet) Conference as it will provide an overview of tools, which can be used in conjunction with TOLNet data, to evaluate the complex chemistry and transport pathways controlling tropospheric O3 mixing ratios.

Mixing Ratios↗

Exploratory investigation of the need for and feasibility of a Lower Atmosphere Research Satellite (LARS) program

The need for and feasibility of a research satellite program for the intensive study of the lower atmosphere (the troposphere and lower stratosphere) is discussed. The priorities for scientific investigation of the lower atmosphere during the next decade are examined. The findings of the study are concerned with identification of those broad research issues of highest priority and, in particular, with those that are most appropriate for investigation from space platforms.

Source record↗

A comparison of observed (HALOE) and modeled (CCM2) methane and stratospheric water vapor

Recent measurements (21 September-15 October 1992) of methane and water vapor by the Halogen Occultation Experiment (HALOE) on the Upper Atmosphere Research Satellite (UARS) are compared with model results for the same season from a troposphere-middle atmosphere version of the National Center for Atmospheric Research (NCAR) Community Climate Model (CCM2). Several important features of the two constituent fields are well reproduced by the CCM2, despite the use of simplified methane photochemistry in the CCM2 and some notable differences between the model's zonal mean circulation and climatology. Observed features simulated by the model include the following: 1) subsidence over a deep layer in the Southern Hemisphere polar vortex; 2) widespread dehydration in the polar vortex; and 3) existence of a region of low water vapor mixing ratios extending from the Antarctic into the Northern Hemisphere tropics, which suggests that Antarctic dehydration contributes to midlatitude and tropical dryness in the stratosphere.

Mote, Philip W.↗

Monthly Representations of Mid-Tropospheric Carbon Dioxide from the Atmospheric Infrared Sounder

The Atmospheric Infrared Sounder (AIRS) on NASA's Earth Observing System Aqua spacecraft was launched in May of 2002 and acquires hyperspectral infrared spectra used to generate a wide range of atmospheric products including temperature, water vapor, and trace gas species including carbon dioxide. Here we present monthly representations of global concentrations of mid-tropospheric carbon dioxide produced from 8 years of data obtained by AIRS between the years of 2003 and 2010. We define them as "representations" rather than "climatologies" to reflect that the files are produced over a relatively short time period and represent summaries of the Level 3 data. Finally, they have not yet been independently validated. The representations have a horizontal resolution of 2.0 deg x 2.5 deg (Latitude x Longitude) and faithfully reproduce the original 8 years of monthly L3 CO2 concentrations with a standard deviation of 1.48 ppm and less than 2% outliers. The representations are intended for use in studies of the global general circulation of CO2 and identification of anomalies in CO2 typically associated with atmospheric transport. The seasonal variability and trend found in the AIRS CO2 data are discussed.

Carbon Dioxide↗

A study of the mechanism of internal gravity wave generation by quasigeostrophic meteorological motions

Numerous experiments on the detection of atmospheric waves in the frequency range from acoustic to planetary at meteor heights have revealed that important wave sources are meteorological processes in the troposphere (cyclones, atmospheric fronts, jet streams, etc.). A dynamical theory based on the others work include describing the adaptation of meteorological fields to the geostropic equilibrium state. According to this theory, wave motions appear as a result of constant competition between the maladjustment of the wind and pressure fields due to nonlinear effects and the tendency of the atmosphere to establish a quasi-geostrophic equilibrium of these fields. These meteorological fields are discussed.

Medvedev, A. S.↗

NASA plans for spaceborne lidar - The Earth Observing System

The use of laser techniques to observe the earth's atmosphere and surface from space is examined. An Earth Observing System is proposed as the platform for performing lidar observations. The objectives and capabilities of the Lidar Atmospheric Sounder and Altimeter (LASA) are described. The measurement techniques for collecting temperature, pressure, and water vapor profiles, the vertical distribution of ozone in the stratosphere and troposphere, and atmospheric particulates profiles are discussed. The LASA requirements for altimetry and retroranging are considered. The Doppler Lidar Wind Sensor which provides data on wind velocity is analyzed. These laser systems with increased spatial resolution and accuracy form an efficient information system for studying earth science developments.

Curran, R. J.↗

A new numerical model of the middle atmosphere. I - Dynamics and transport of tropospheric source gases

Attention is given to a new model of the middle atmosphere which includes, in addition to the equations governing the zonal mean state, a potential vorticity equation for a single planetary-scale Rossby wave, and an IR radiative transfer code for the stratosphere and lower mesosphere, which replaces the Newtonian cooling parameterization used previously. It is shown that explicit computation of the planetary-scale wave field yields a more realistic representation of the zonal mean dynamics and the distribution of trace chemical species. Wave breaking produces a well-mixed 'surf zone' equatorward of the polar night vortex and drives a meridional circulation with downwelling on the poleward side of the vortex. This combination of mixing and downwelling produces shallow meridional gradients of trace gases in the subtropics and middle latitudes, and very steep gradients at the edge of the polar vortex. Computed distributions of methane and nitrous oxide are shown to agree well with observations.

Garcia, Rolando R.↗

Convective Impact on the Global Lower Stratospheric Water Vapor Budget

Water vapor in the stratosphere is primarily controlled by temperatures in the tropical upper troposphere and lower stratosphere. However, the direct impact of deep convection on the global lower stratospheric water vapor budget is still an actively debated issue. Two complementary modeling approaches are used to investigate the convective impact in boreal winter and summer. Convective influence is diagnosed by tracing trajectories through convective cloud top altitude fields derived from global rainfall and brightness temperature data. Backward trajectory model simulations coupled with a detailed treatment of cloud microphysical processes indicate that convection moistens the global lower stratosphere by approximately 0.3 ppmv in boreal winter and summer 2010. The diurnal peak in convection is responsible for about half of the total convective moistening during winter and nearly all of the convective moistening during summer. Deep convective clouds overshooting the tropopause have relatively minor effect on global lower stratospheric water vapor. A forward trajectory model coupled with a simplified cloud module is used to estimate the relative magnitude of the interannual variability of the convective impact. Combining the results from the two models, we find that the convective impact on the global lower stratospheric water vapor during 2006-2016 is approximately 0.3 ppmv with year-to-year variations of up to 0.1 ppmv. An important mechanism of convective hydration of the lower stratosphere is via the detrainment of saturated air and ice into the tropical uppermost troposphere and the subsequent upward transport of some of these moist air parcels across relatively warm and subsaturated tropopause.

CONVECTION↗

Preface to Special Section: Validation of Atmospheric Infrared Sounder Observations

The papers described below demonstrate that the AIRS calibrated radiances and retrieved geophysical products generally meet or exceed the prelaunch specifications. The retrieved quantities show little variation in uncertainty as a function of cloud amount. However, AIRS retrieval yield is a rapidly decreasing function of cloud amount; at about 80% cloudiness essentially no infrared radiances are used in the retrieval processes. Also, AIRS performance has not been demonstrated for all conditions and products. Calibrated and forward calculated radiances meet performance specifications for conditions varying from the cold poles to warm tropics. The retrieval system performs well over extrapolar land in the free troposphere (~2-15 km above the surface) and over extrapolar oceans at all tropospheric altitudes. The AIRS retrieval algorithms have not been optimized for polar winter conditions, so no such results are presented in these papers.

temperature↗

Response of Earth's Atmosphere to Increases in Solar Flux and Implications for Loss of Water from Venus

A one dimensional radiative convective model is used to compute temperature and water vapor profiles as functions of solar flux for earthlike atmosphere. The troposphere is assumed to be fully saturated with a moist adiabatic lapse rate, and changes in cloudiness are neglected. Predicted surface temperatures increase monotonically from -1 to 111 C as the solar flux is increased from 0.81 to 1.45 times its present value. The results imply that the surface temperature of a primitive water rich Venus should have been at least 80-100 C and may have been much higher, water vapor should have been a major atmospheric constituent at all altitudes, leading to the rapid hydrodynamic escape of hydrogen. The oxygen left behind by this process was presumably consumed by reactions with reduced minerals in the crust.

Kasting, J. F.↗

Studies of thermal wave phenomena on the Jovian planets

Ground based and Voyager observations of Jupiter have provided evidence that the tropospheric temperature shows global scale longitudinal variations which are often wavelike in character. Voyager data are reported to exhibit the presence of slowly moving thermal features, wherein the jovian tropospheric temperature patterns are not advected by the equatorial zonal winds, but are not found to rotate at the System III (interior) rate. Ground based data in a broad infrared band (8 to 13 micron) show a wavelike structure whose amplitude and spatial scale are similar to the reported properties of the slowly moving thermal features. This study is directed toward obtaining additional ground based data in infrared spectral bands whose contribution functions are optimized for specific atmospheric regions (tropospheric at 20 micron, and stratospheric at 7.8 micron), in order to confirm the previous results, and to identify the nature and physical significance of wavelike longitudinal temperature fluctuations on the Jovian planets. A 2-D infrared array detector and low resolution cryogenic grating spectrometer is being adapted to obtain maps in approx. 2/cm bandpasses.

Deming, Drake↗

Response of earth's atmosphere to increases in solar flux and implications for loss of water from Venus

A one-dimensional radiative-convective model is used to compute temperature and water vapor profiles as functions of solar flux for an earthlike atmosphere. The troposphere is assumed to be fully saturated, with a moist adiabatic lapse rate, and changes in cloudiness are neglected. Predicted surface temperatures increase monotonically from -1 to 111 C as the solar flux is increased from 0.81 to 1.45 times its present value. The results imply that the surface temperature of a primitive water-rich Venus should have been at least 80-100 C and may have been much higher. Water vapor should have been a major atmospheric constituent at all altitudes, leading to the rapid hydrodynamic escape of hydrogen. The oxygen left behind by this process was presumably consumed by reactions with reduced minerals in the crust.

Kasting, J. F.↗

The Influence of Tropospheric Processes in Modeling the Middle Atmosphere with Gravity Waves

Our Numerical Spectral Model (NSM) extends from the ground up into the thermosphere and has a vertical grid point resolution of about 0.5 km to resolve the interactions of gravity waves (GWs) described with Hines' Doppler Spread Parameterization (DSP). This model produces in the stratosphere and mesosphere the major features of QBO, SAO, tides, and planetary waves. The purpose of this paper is to discuss results from an initial study with our 3D model that shows how certain tropospheric processes can affect the dynamics of the middle atmosphere. Under the influence of tropospheric heating, and augmented by GW interactions, two distinct but related processes can be identified. (1) A meridional circulation develops in the stratosphere, with rising motions at low latitudes that are in magnitude comparable to the downward propagation of the QBO. As Dunkerton pointed out, a larger GW source is then required to reproduce the observed QBO, which tends to move us closer to the values recommended for the DSP. This has significant consequences for our model results that describe the upper mesosphere, considering the general importance of GWs for this region and in influencing planetary waves (e.g., 2-day wave) and tides in particular. (2) Tropospheric heating produces zonal jets near the tropopause that are related to latitudinal variations in pressure and reversing temperature variations (resembling the dynamical conditions near the mesopause), which in turn is conducive to generate baroclinic instability. Modeling results show that our ability to generate the QBO critically depends on the magnitude of the temperature reversal that is a measure of this instability. Planetary waves are generated in this process, which can apparently interfere with or augment the GW interactions. As originally demonstrated by Lindzen and Holton, the eastward propagating Kelvin waves and westward propagating Rossby gravity waves (generated by tropospheric convection) can in principle provide the acceleration to influence the QBO, and we were able to confirm this with our 3D model.

Mayr, H. G.↗

ShupeTurner cloud microphysics

This product is the ShupeTurner cloud microphysics product derived for the Multidisciplinary drifting Observatory for the Study of Arctic Climate (MOSAiC) expedition in the central Arctic. The product includes time-height derivations of the cloud type (phase type) and the condensed water content and characteristic effective particle size for liquid and ice hydrometeor populations. Additionally, it includes the vertical integral of the condensed water content for liquid and ice, i.e., the liquid water path and ice water path. These are derived using a combination of sensors, including: cloud radar, depolarization lidar, microwave radiometer, ceilometer, and radiosondes. During MOSAiC, these sensors were installed and operated onboard the Polarstern icebreaker while within the Arctic sea ice. Most data were obtained while Polarstern was moored to the MOSAiC sea ice floe, passively drifting through the Arctic. However, the data from 16 May 2020 - 17 June 2020 and 31 July 2020 - 21 August 2020 were obtained while Polarstern was underway transiting through the sea ice during relocations of the expedition. General details of the retrieval algorithm, its application, and uncertainties are provided in Shupe et al. (2015), with the cloud classification being described in more detail in Shupe (2007). General details about the MOSAiC expedition including instruments, locations, and meteorological context is provided in Shupe et al. (2022).

54 ENVIRONMENTAL SCIENCES↗

NPFTURBULENCE: Best Estimate Aerosol Size Distribution by airborne measurements

The original data were collected during the field campaign of “Turbulent layers promoting New Particle Formation” experiment (NPFTURBULENCE; https://www.arm.gov/research/campaigns/aaf2024npfturbulence) over the Atmospheric Radiation Measurement (ARM) Southern Great Plains (SGP) Atmospheric Observatory (https://www.arm.gov/capabilities/observatories/sgp ) in north-central Oklahoma. The ARM Aerial Facility ArcticShark uncrewed aerial system (UAS) was based at Blackwell–Tonkawa Municipal Airport (IATA: BWL, ICAO: KBKN, FAA LID: BKN, 36.74475° N, 97.34918° W, 313.9 m MSL), for the field campaign from May 5 through May 29, 2024. The ArcticShark UAS performed 11 flights, including 10 research flights over the Central Facility of the ARM SGP to measure atmospheric state, turbulence, surface IT temperature and imagery, aerosol number concentration and size distribution. The current data set presents Best Estimate Aerosol Size Distribution: a merged aerosol size distribution composed of the data from 2 sensors: miniaturized Scanning Electrical Mobility Sizer (mSEMS) and Portable Optical Particle Spectrometer (POPS). The mSEMS data were interpolated to 1 second from “native” time resolution of about 15 second to match the other probe. The POPS data were converted from equivalent optical size into geometric size using value of aerosol refractive index of 1.477 from the HISCALE field campaign (same geographical area, altitudes, and time of year; http://www.arm.gov/campaigns/aaf2016hiscale ).

54 ENVIRONMENTAL SCIENCES↗

CACTI CSAPR2 Taranis Retrievals

Taranis is an end-to-end processing chain for radar data written in Python with C extension for computation performance. Features include: masking for quality control, specific differential phase (Kdp), attenuation correction for reflectivity factor (Z) and differential reflectivity (Zdr) in rain, and additional geophysical retrievals. Retrievals are mostly drawn from literature or open-source software when appropriate, and have been tested, tuned, and modified to work with one another cohesively rather than using isolated off-the-shelf algorithms. Incorporated algorithms include hydrometeor (echo) identification, rain water content, raindrop mass-weighted mean diameter (gamma size distribution assumption), and rainfall rate (QPE). Taranis data sets exist for CSAPR2 PPI, HSRHI, and sector RHI scans. Cartesian-gridded data sets were also produced as well as a near-surface rain rate retrieval. More details can be found in the README.

54 ENVIRONMENTAL SCIENCES↗