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DOE OSTI2026

A fresh perspective on the role of band bending, and related contributors, in light-driven production of electricity and chemicals

It is widely known that semiconductor-based solar energy conversion could power our planet. This is in part because high-quality semiconductor structures are unrivalled in their ability to separate photogenerated electrons and holes. One effective approach to achieving this photoinduced charge separation relies on a phenomenon known as “band bending”. But details to justify why band bending results in photoinduced charge separation are more complex than often appreciated. This underappreciation is an impediment to the rational, hypothesis-driven design of next-generation approaches to solar energy conversion. Herein we show, by means of derivations rooted in physical chemistry, that several phenomena – not just band bending – can facilitate photoinduced charge separation, and that each is influenced by nonequilibrium species concentration and a parameter, such as diffusion coefficient or rate coefficient, that introduces dynamics. To help visualize the impact of each phenomenon, we introduce plots that depict their contributions as free energy, force, flux, force constant, and rate. We reveal that spatial dopant distributions that define band bending are predictors of initial photogenerated species transport rates. But charge separation alone does not guarantee high-efficiency operation. A photogenerated change in energy that is freely available to do useful work is also essential, and is strongly dependent on semiconductor optical properties and reaction kinetics. Notably, this information reveals that specificity of interfacial chemical reactions – even when they are not preceded by charge separation elsewhere – can result in efficient solar energy conversion. We expect that this tutorial will guide researchers in their pursuit to uncover new mechanisms for light to perform useful work.

14 SOLAR ENERGY↗

DOE OSTI2020

Crushing behaviors of unidirectional carbon fiber reinforced plastic composites under dynamic bending and axial crushing loading

The dynamic crushing characteristics of unidirectional carbon fiber reinforced plastic composites under two loading types, dynamic three-point bending and axial crushing, are investigated by experiment and finite element simulation. Hat section samples with two different layup orientations are tested at various impact velocities to investigate its effects. The experiment results show that delamination plays a critical role in dynamic bending deformation. Different layup orientations lead to similar crushing bending behaviors, but remarkable variations in delamination pattern evolutions. In contrast, layup orientation exerts more significant effects on failure modes and energy absorption in axial crushing. A finite element model with multiple layers of thick shell element and cohesive element is established, and simulations are performed for both dynamic three-point bending and axial crushing. The model can capture the crushing behaviors in the two loading types reasonably well. The damage evolution and energy absorption through various mechanisms at different loading conditions are discussed.

42 ENGINEERING↗

DOE OSTI2021

Distributed fiber optic strain sensing of bending deformation of a well mockup in the laboratory

Well integrity is critical to the safety and success of subsurface energy exploration and management, as leakage of fluids from subsurface reservoirs is often induced by compromised wells. This study investigates bending deformation of a mockup of an oil/gas well that is subjected to loads expected in deviated wells under reservoir compaction and assesses the feasibility of utilizing distributed fiber optic strain sensing to monitor the deformation. Here, a well mockup, which consists of outer and inner steel pipes with a cemented annulus, is tested under three-point bending loading and its strain and curvature development is monitored by Brillouin optical time domain reflectometry/analysis (BOTDR/A) as well as optical frequency domain reflectometry (OFDR). The primary objective of this research is to assess the strain sensing performance of newly fabricated fiber optic cables and to identify key cable characteristics which could improve the quality of distributed strain measurements with BOTDR/A. Results show that the tight-buffered cable is best suited for strain sensing as its maximum errors in the strain measurement were -36% and -24% against conventional sensors at the maximum elastic and plastic bending loads, respectively, whereas those of the non-tight-buffered cable were -45% and -71%, respectively. Similar trends were obtained in the bending curvature measurement. The detailed design of the tight-buffered cable is presented to elucidate key characteristics of such a cable, which will facilitate accurate distributed strain sensing in oil and gas wells.

42 ENGINEERING↗

DOE OSTI2025

Reactions of Np(VI) and Pu(VI) with Phenanthroline Result in Bending the [NpVIO2]2+ Unit and a Reduced Pu(V) Species

Despite decades of actinyl chemistry, genuinely bent actinyl structures remain rare beyond uranium. We report the first crystallographic characterization of a bent neptunyl(VI) complex, NpO 2 Cl 2 (phen) 2, along with a linear plutonyl species that, unexpectedly, adopts the +V oxidation state. Coordination of two 1,10-phenanthroline ligands to NpO 2 2+ enforces pronounced bending of the O yl –Np–O yl unit to 162° through steric clashes with the axial phenathroline ligand, representing the sharpest angle reported for any neptunyl(VI) complex. In contrast, synthesis with PuO 2 2+ produces a reduced linear Pu(V) species, PuO 2 Cl(phen) 2, underscoring the redox lability and the reluctance of plutonium to distort. Raman and IR spectra yield the first experimental stretching and interaction force constants for plutonyl(V). Comparison with values for plutonyl(VI) and bent and linear uranyl(VI) and neptunyl(VI) compounds shows that reduction perturbs the actinyl bond more than bending within one oxidation state. Electrochemical and spectroscopic studies clarify phenanthroline binding to Pu(VI) and the system’s reactivity. Quantum chemical calculations indicate that bending is energetically favored in the U–Np–Pu series, but the stabilization energy decreases as the actinide atomic number increases. NBO and QTAIM analyses reveal systematic trends: increasing 5f occupancy and decreasing An–O yl bond covalency from U to Pu. These results demonstrate that ligand-induced bending in neptunyl(VI) species is not only electronically feasible but also synthetically achievable, though plutonyl(VI) is constrained by redox reactivity. This work expands the frontier of nonlinear actinyl chemistry and illuminates how structure, oxidation state, and electronic configuration interrelate across the actinyl series.

actinides↗

DOE OSTI2024

A bending test protocol for characterizing the mechanical performance of flexible photovoltaics

Flexible photovoltaics (PV) represents a promising research field with great potential for wearable, portable, and indoor applications. Significant progress has been made in recent years, with flexible emerging PV reporting power conversion efficiency (PCE) over 24%. Yet, there is a need for a unifying protocol to assess PV performance, compare research results, and evaluate the state- of-the-art achievements in flexible PV. In this paper, a consensus protocol is presented for measuring PCE over 1,000 bending cycles under 1% strain. Moreover, several good practice guidelines are proposed including bending procedures, flexibility testing with and without encapsulation, and ambient conditions during testing (e.g., temperature, humidity, illumination). Notably, the importance of uniform application of bending radius and the testing of parallel and perpendicular orientations of bending axis with respect to the direction of the electric current are emphasized. These recommendations aim to promote consistency in device comparison and allow for better reproducibility.

Fukuda, Kenjiro↗

DOE OSTI2025

Exact statistics of helical wormlike chains with twist-bend coupling

Here, we present a solution for the Green's function for the general case of a helical wormlike chain with twist-bend coupling and demonstrate the applicability of our solution for evaluating general structural and mechanical chain properties. We find that twist-bend coupling renormalizes the persistence length and the force-extension curves relative to wormlike chains. Analysis of intrinsically twisted polymers shows that incorporation of twist-bend coupling results in the oscillatory behavior in principal tangent correlations that are observed in some studies of synthetic polymers. The exact nature of our solution provides a framework to evaluate the role of twist-bend coupling on polymer properties, such as DNA bound to histones and motivates the reinterpretation of existing biopolymer experimental data.

Ghosh, Ashesh [University of California, Berkeley,↗

DOE OSTI2022

Methodology for designing Complex Bend lattice

In this note we are discussing the approach of designing the Triple Complex Bend Achromat lattice. The benefits of the Complex Bend (CB) approach include: 1) the promise of reaching ultra-low emittance and, thus, high brightness and 2) compact arrangement of the lattice components, based on grouping several strong focusing and bending poles into a single element, i.e. Complex Bend. In this note, we are presenting an approach of designing the ring lattice from CB elements in a way of minimizing the number of free variables to simultaneously satisfy constraints of low emittance, low chromaticity, long straight sections and maximum of free space inside the lattice.

43 PARTICLE ACCELERATORS↗

DOE OSTI2023

Stratospheric temperature measurements from nanosatellite stellar occultation observations of refractive bending

Abstract. Stellar occultation observations from space can probe the stratosphere and mesosphere at a fine vertical scale around the globe. Unlike other measurement techniques like radiosondes and aircraft, stellar occultation has the potential to observe the atmosphere above 30 km, and unlike radio occultation, stellar occultation probes fine-scale phenomena with potential to observe atmospheric turbulence. We imaged the refractive bending angle of a star centroid for a series of occultations by the atmosphere. Atmospheric refractivity, density, and then temperature are retrieved from the bending observations with the Abel transformation and Edlén's law, the hydrostatic equation, and the ideal gas law. The retrieval technique is applied to data collected by two nanosatellites operated by Terran Orbital. Measurements were primarily taken by the GEOStare SV2 mission, with a dedicated imaging telescope, supplemented with images captured by spacecraft bus sensors, namely the star trackers on other Terran Orbital missions. The bending angle noise floor is 10 and 30 arcsec for the star tracker and GEOStare SV2 data, respectively. The most significant sources of uncertainty are due to centroiding errors due to the fairly low-resolution stellar images and telescope pointing knowledge derived from noisy satellite attitude sensors. The former mainly affects the star tracker data, while the latter limits the GEOStare SV2 accuracy, with both providing low vertical resolution. This translates to a temperature profile retrieval up to roughly 20 km for both star tracker and GEOStare SV2 datasets. In preparation of an upcoming 2023 mission designed to correct these deficiencies, SOHIP, we simulated bending angle measurements with varying magnitudes of error. The expected maximum altitude of retrieved temperature is 41 km on average for these simulated measurements with a noise floor of 0.39 arcsec. Our work highlights the capabilities of stellar occultation observations from nanosatellites for atmospheric sounding. Future work will investigate high-frequency observations of atmospheric gravity waves and turbulence, mitigating the major uncertainties observed in these datasets.

54 ENVIRONMENTAL SCIENCES↗

NASA NTRS1973

Thermal static bending of deployable interlocked booms

Metal ribbons processed with a heat-forming treatment are enabled to form tubelike structures when deployed from a roll. Deployable booms of this have been utilized for gravity-gradient stabilization on the RAE, ATS, and Nimbus D satellites. An experimental thermal-mechanics test apparatus was developed to measure the thermal static bending and twist of booms up to 3 meters long. The apparatus was calibrated by using the correlation between calculated and observed thermal bending of a seamless tube. Thermal static bending values of 16 interlocked deployable booms were observed to be within a factor of 2.5 of the values calculated from seamless-tube theory. Out-of-Sun-plane thermal bending was caused by complex heat transfer across the interlocked seam. Significant thermal static twisting was not observed.

Staugaitis, C. L.↗

NASA NTRS1974

Research on wood bending in a macrosonic field

Woodworking often requires the wood to be bent into different shapes. In view of the fact that macrosonic waves compress and expand the medium through which they are being propagated we assumed that wood subjected to the action of these waves during the bending process would have enhanced plasticity as a result of the loosening-up that takes place in it, as well as of the reduction in effort. To this effect, the bending of wood plasticized in a macrosonic field was studied. This bending took place under good conditions, and structural analyses conducted with the aid of an electron microscope proved initial premises to be corrent. Applied on an industrial scale, this procedure would contribute to improving the technology of wood bending as well as to eliminating factory spoilage.

Filipovici, J.↗

NASA NTRS1975

Effect of ball geometry on endurance limit in bending of drilled balls

Four designs of drilled (cylindrically hollow) balls were tested for resistance to bending fatigue. Bending fatigue has been demonstrated to be a limiting factor in previous evaluations of the drilled ball concept. A web reinforced drilled ball was most successful in resisting bending fatigue. Another design of through drilled design, involving a heavier wall than the standard reference ball, also showed significant improvement in resistance to bending fatigue.

Munson, H. E.↗

NASA NTRS1979

An analysis of thermal stress and gas bending effects on vibrations of compressor rotor stages

A preliminary study conducted by Kerrebrock et al. (1976) has shown that the torsional rigidity of untwisted thin blades of a transonic compressor can be reduced significantly by transient thermal stresses. The aerodynamic loads have various effects on blade vibration. One effect is that gas bending loads may result in a bending-torsion coupling which may change the characteristics of the torsion and bending vibration of the blade. For a general study of transient-temperature distribution within a rotor stage, a finite-element heat-conduction analysis was developed. The blade and shroud are divided into annular elements. With a temperature distribution obtained from the heat-conduction analysis and a prescribed gas bending load distribution along the blade span, the static deformation and moment distributions of the blade can be solved iteratively using the finite-element method. The reduction of the torsional rigidity of pretwisted blades caused by the thermal stress effect is then computed. The dynamic behavior of the blade is studied by a modified Galerkin's method.

Chen, L.-T.↗

NASA NTRS1982

Fatigue life prediction in bending from axial fatigue information

Bending fatigue in the low cyclic life range differs from axial fatigue due to the plastic flow which alters the linear stress-strain relation normally used to determine the nominal stresses. An approach is presented to take into account the plastic flow in calculating nominal bending stress (S sub bending) based on true surface stress. These functions are derived in closed form for rectangular and circular cross sections. The nominal bending stress and the axial fatigue stress are plotted as a function of life (N sub S) and these curves are shown for several materials of engineering interest.

Manson, S. S.↗

NASA NTRS1985

Bending waves and the structure of Saturn's rings

The surface mass density profiles at four locations within Saturn's rings are calculated using Voyager spacecraft images of spiral bending waves. The identification of a feature in Saturn's outer B ring as Mimas's 4:2 bending waves is confirmed, and these 4:2 waves are analyzed to determine the surface density in Saturn's B ring. A fourth set of bending waves, the Mimas 7:4, located in the inner A ring, is identified and analyzed. Mimas's 5:3 and 8:5 bending waves, observed in the middle and outer A ring respectively, are reanalyzed.

Lissauer, J. J.↗

NASA NTRS1986

The predicted effect of aerodynamic detuning on coupled bending-torsion unstalled supersonic flutter

A mathematical model is developed to predict the enhanced coupled bending-torsion unstalled supersonic flutter stability due to alternate circumferential spacing aerodynamic detuning of a turbomachine rotor. The translational and torsional unsteady aerodynamic coefficients are developed in terms of influence coefficients, with the coupled bending-torsion stability analysis developed by considering the coupled equations of motion together with the unsteady aerodynamic loading. The effect of this aerodynamic detuning on coupled bending-torsion unstalled supersonic flutter as well as the verification of the modeling are then demonstrated by considering an unstable 12 bladed rotor, with Verdon's uniformly spaced Cascade B flow geometry as a baseline. However, with the elastic axis and center of gravity at 60 percent of the chord, this type of aerodynamic detuning has a minimal effect on stability. For both uniform and nonuniform circumferentially space rotors, a single degree of freedom torsion mode analysis was shown to be appropriate for values of the bending-torsion natural frequency ratio lower than 0.6 and higher 1.2. When the elastic axis and center of gravity are not coincident, the effect of detuning on cascade stability was found to be very sensitive to the location of the center of gravity with respect to the elastic axis. In addition, it was determined that when the center of gravity was forward of an elastic axis located at midchord, a single degree of freedom torsion model did not accurately predict cascade stability.

Hoyniak, D.↗

NASA NTRS1986

The relationship of intravascular bubbles to bends at altitude

In response to recent findings attesting to a correlation between intravehicular bubbling and decompression sickness at intermediate altitudes, an attempt was made to define a minimum pressure for a pressure suit which would obviate the need for prebreathing 100 percent oxygen prior to extravehicular activity (EVA). Fifty-seven male subjects were exposed to altitudes ranging from 16,000 to 30,000 ft in two separate protocols. The first was designed to determine a pressure at which no bends occurred if a crewmember were decompressed from a sea level space station pressure just prior to EVA without prebreathing 100 percent oxygen. The other study was designed to define an altitude and exercise regimen at which bends-susceptible and bends-resistant crewmembers could be separated. It is shown that the close association which exists between severe bubbling and bends at a pressure altitude of 4.3 psia (30,000 ft) decreases as pressure is increased and essentially disappears at pressures less than or equal to 7.8 psia (16,000 ft).

Krutz, R. W.↗

NASA NTRS1986

The effect of circumferential aerodynamic detuning on coupled bending-torsion unstalled supersonic flutter

A mathematical model developed to predict the enhanced coupled bending-torsion unstalled supersonic flutter stability due to alternate circumferential spacing aerodynamic detuning of a turbomachine rotor. The translational and torsional unsteady aerodynamic coefficients are developed in terms of influence coefficients, with the coupled bending-torsion stability analysis developed by considering the coupled equations of this aerodynamic detuning on coupled bending-torsion unstalled supersonic flutter as well as the verification of the modeling are then demonstrated by considering an unstable 12 bladed rotor, with Verdon's uniformly spaced Cascade B flow geometry as a baseline. However, with the elastic axis and center of gravity at 60 percent of the chord, this type of aerodynamic detuning has a minimal effect on stability. For both uniform and nonuniform circumferentially space rotors, a single degree of freedom torsion mode analysis was shown to be appropriate for values of the bending-torsion natural frequency ratio lower than 0.6 and higher 1.2. When the elastic axis and center of gravity are not coincident, the effect of detuning on cascade stability was found to be very sensitive to the location of the center of gravity with respect to the elastic axis. In addition, it was determined that when the center of gravity was forward of an elastic axis located at midchord, a single degree of freedom torsion model did not accurately predict cascade stability.

Hoyniak, D.↗

NASA NTRS1933

Strength Tests of Thin-walled Duralumin Cylinders in Pure Bending

This report is the third of a series presenting the results of strengths tests on thin-walled cylinders and truncated cones of circular and elliptic section; it includes the results obtained from pure bending tests on 58 thin-walled duralumin cylinders of circular section with ends clamped to rigid bulkheads. The tests show that the stress on the extreme fiber at failure as calculated by the ordinary theory of bending is from 30 to 80 percent greater than the compressive stress at failure for thin-walled cylinders in compression. The tests also show that length/radius ratio has no consistent effect upon the bending strength and that the size of the wrinkles that form on the compression half of a cylinder in bending is approximately equal to the size of the wrinkles that form in the complete circumference of a cylinder of the same dimensions in compression.

CONES, TRUNCATED - STRENGTH TESTS↗