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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 73 records · Page 4

FAST Low-Energy Beamline Studies: Toward High-Peak 5D Brightness Beams for FAST-GREENS

The FAST beamline is the injector for the planned Gamma-Ray Electron ENhanced Source (GREENS) program, which aims to achieve the demonstration and first application of a high-efficiency, high-average-power free-electron laser at 515 nm. FAST-GREENS requires high 5D peak brightness; transverse normalized projected emittances of 3 mm-mrad and a peak current of 600 A are the minimum beam requirements for the FEL to reach the 10% efficiency goal. In this work, studies of the low-energy section of the FAST beamline are presented toward these ends, including preliminary measurements of beam compression and beam emittance. An effort toward developing a high-fidelity simulation model that could be later optimized for FAST-GREENS is presented.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Effect of neutron beamline irradiation on hydrogen equilibrium vapor pressure over hydrided Zircaloy-4

Here, the effect of neutron irradiation on the hydrogen equilibrium vapor pressure over hydrided samples of nickel-plated Zircaloy-4 was evaluated at the Washington State University Research Reactor’s epithermal beamline facility. To enable this study, a measurement capability was designed and assembled to obtain low pressure (<0.1 Pa) measurements over the temperature range of interest (i.e., ~300° - 400°C). Measurement results were in good agreement with tends extrapolated from previous data obtained at higher temperatures as well as recent thermodynamic data. No irradiation enhancement of vapor pressure was observed under the incident flux of epithermal neutrons over this temperature range.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Remote and automated high-throughput powder diffraction measurements enabled by a robotic sample changer at SSRL beamline 2-1

The general-purpose powder diffractometer beamline (BL2-1) at the Stanford Synchrotron Radiation Lightsource (SSRL) is described. The evolution of design and performance of BL2-1 are presented, in addition to current operating specifications, applications and measurement capabilities. Recent developments involve a robotic sample changer enabling high-throughput X-ray diffraction measurements, applicable to mail-in and remote operations. In situ and operando capabilities to measure samples with different form factors ( e.g. capillary, flat plate or thin film, and transmission) and under variable experimental conditions are discussed. Several example datasets and accompanying Rietveld refinements are presented.

43 PARTICLE ACCELERATORS↗

Off-axis representation of hyperbolic mirror shapes for X-ray beamlines

Mirror-centered, closed-form expressions for hyperbolic surfaces used in X-ray beamlines have been derived. Hyperbolic mirrors create a virtual focus or source point and can be used to lengthen or shorten the effective focal distance of a compound optical system. The derivations here express off-axis segments of a hyperbolic surface in terms of the real and virtual focal distances and the incident glancing angle at the center of the mirror. Conventional mathematical expressions of hyperbolic shapes describe the surfaces in Cartesian or polar coordinates centered on an axis of symmetry, necessitating cumbersome rotation and translation to mirror-centered coordinates. The representation presented here, with zero slope and the origin at the central point, is most convenient for modeling, metrology, aberration correction, and general surface analysis of off-axis configurations. The direct derivation avoids the need for nested coordinate transforms. A series expansion provides a helpful approximation; the coefficients of the implicit equation are also provided.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Magnetic Designs of New First Target Beamline Magnets for the ORNL SNS Upgrade

The Spallation Neutron Source (SNS) at ORNL currently is being upgraded from 1.0 GeV to 1.3 GeV. Several water-cooled magnets should be upgraded to transport 30% of higher beam energy. New chicane, injection/extraction septum, and Lambertson magnets were designed. Designing the magnets was a challenging task because the new magnets required good combined integrated field quality and needed to occupy the old magnets space but with about 20% greater integrated magnetic field. Additional strong requirements applied to the magnets fringe field do not disturb the circulating beam. The special field profiles had to be provided in foil areas between magnets. The analysis described here was based on OPERA3D simulations. A special technique was used for analyzing the integrated field harmonics. Initially, the particle track was simulated, and integrated field components were calculated along this track for the reference radius, which were used for the harmonics analysis. In addition, 3D field maps were provided for beam optics simulations. The final beamline analysis confirmed good beam transmission and low losses.

3d field maps↗

Detector and Beamline Simulation for Next-Generation High Energy Physics Experiments

The success of high energy physics programs relies heavily on accurate detector simulations and beam interaction modeling. The increasingly complex detector geometries and beam dynamics require sophisticated techniques in order to meet the demands of current and future experiments. Common software tools used today are unable to fully utilize modern computational resources, while data-recording rates are often orders of magnitude larger than what can be produced via simulation. In this paper, we describe the state, current and future needs of high energy physics detector and beamline simulations and related challenges, and we propose a number of possible ways to address them.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Beamline Device Designators

LAMP is to replace the front-end of LANSCE. Therefore, the device designators for LAMP needs approval from LANSCE. This document defines the agreed upon device designator names to be used in LAMP and in the prototype beamline LAMP in ADEF Tunnel (LAT).

43 PARTICLE ACCELERATORS↗

Design and commissioning of an e-beam irradiation beamline at the Upgraded Injector Test Facility at Jefferson Lab

We report the Upgraded Injector Test Facility (UITF) at Jefferson Lab is a continuous-wave superconducting linear accelerator capable of providing an electron beam with energy up to 10 MeV. A beamline for electron-beam irradiation has been designed, installed and successfully commissioned at this facility, aimed at the degradation study of 1,4-dioxane and per- and polyfluoroalkyl substances (PFAS) in wastewater treatment. A solenoid with a peak axial magnetic field of up to 0.28 T and a set of raster coils were used to obtain a Gaussian beam profile with a transverse standard deviation of ~ 15.0 mm at the target location. Monte-Carlo simulations using FLUKA were carried out to calculate the total absorbed dose and the dose distribution in the sample volume inside the target cell. The simulations were benchmarked experimentally by dosimetry mapping using optichromic dosimeters. The results of the irradiation experiments showed a ~ 95% reduction of 1,4-dioxane in ultra-pure water for a dose of 1 kGy, demonstrating the potential of electron-beam irradiation towards addressing growing challenges in environmental remediation.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

HERACLES: A high-voltage DC test beamline for high average current photocathodes

Here, we present commissioning results of the High ElectRon Average Current for Lifetime ExperimentS (HERACLES) beamline at Cornell University. 10 mA average beam current at 200 keV was achieved with a Cs3Sb photocathode operated with an Argon laser at 488 nm. HERACLES is intended to be a test facility to improve the robustness of photocathodes developed for high average current beam operation in conjunction with the Cornell photocathode laboratory.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Delivering real-time multi-modal materials analysis with enterprise beamlines

Contemporary advancements in low-cost automation and computation, reduced barrier to entry in developing artificial intelligence/machine learning (AI/ML), and increased ability to represent complex materials in digital form have led to a number of accelerated materials discovery platforms. However, many of these approaches operate with completely rigid vertical integration in an isolated feedback loop using limited modalities. In order to make a substantial impact on discovering new energy materials, AI-driven experiments must operate collaboratively with each other and researchers and over multiple measurement modalities. Herein, we describe the potential for an “internet of things” approach to self-driving enterprise beamlines that merges core information technologies, robotics, and multi-modal AI. The approach will enable full utility of light sources, collaborate effectively with other remote materials acceleration platforms, and help stride toward the world’s energy future.

36 MATERIALS SCIENCE↗

A new platform for ultra-high dose rate radiobiological research using the BELLA PW laser proton beamline

Abstract Radiotherapy is the current standard of care for more than 50% of all cancer patients. Improvements in radiotherapy (RT) technology have increased tumor targeting and normal tissue sparing. Radiations at ultra-high dose rates required for FLASH-RT effects have sparked interest in potentially providing additional differential therapeutic benefits. We present a new experimental platform that is the first one to deliver petawatt laser-driven proton pulses of 2 MeV energy at 0.2 Hz repetition rate by means of a compact, tunable active plasma lens beamline to biological samples. Cell monolayers grown over a 10 mm diameter field were exposed to clinically relevant proton doses ranging from 7 to 35 Gy at ultra-high instantaneous dose rates of 10 7 Gy/s. Dose-dependent cell survival measurements of human normal and tumor cells exposed to LD protons showed significantly higher cell survival of normal-cells compared to tumor-cells for total doses of 7 Gy and higher, which was not observed to the same extent for X-ray reference irradiations at clinical dose rates. These findings provide preliminary evidence that compact LD proton sources enable a new and promising platform for investigating the physical, chemical and biological mechanisms underlying the FLASH effect.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

A new μ -high energy resolution fluorescence detection microprobe imaging spectrometer at the Stanford Synchrotron Radiation Lightsource beamline 6-2

In this report we describe a new synchrotron X-ray Fluorescence (XRF) imaging instrument with an integrated High Energy Fluorescence Detection X-ray Absorption Spectroscopy (HERFD-XAS) spectrometer at the Stanford Synchrotron Radiation Lightsource at beamline 6-2. The X-ray beam size on the sample can be defined via a range of pinhole apertures or focusing optics. XRF imaging is performed using a continuous rapid scan system with sample stages covering a travel range of 250 × 200 mm 2 , allowing for multiple samples and/or large samples to be mounted. The HERFD spectrometer is a Johann-type with seven spherically bent 100 mm diameter crystals arranged on intersecting Rowland circles of 1 m diameter with a total solid angle of about 0.44% of 4π sr. A wide range of emission lines can be studied with the available Bragg angle range of ~64.5°–82.6°. With this instrument, elements in a sample can be rapidly mapped via XRF and then selected features targeted for HERFD-XAS analysis. Furthermore, utilizing the higher spectral resolution of HERFD for XRF imaging provides better separation of interfering emission lines, and it can be used to select a much narrower emission bandwidth, resulting in increased image contrast for imaging specific element species, i.e., sparse excitation energy XAS imaging. This combination of features and characteristics provides a highly adaptable and valuable tool in the study of a wide range of materials.

47 OTHER INSTRUMENTATION↗

A beamline for ultrafast extreme ultraviolet magneto-optical spectroscopy in reflection near the shot noise limit

High harmonic generation (HHG) makes it possible to measure spin and charge dynamics in materials on femtosecond to attosecond timescales. However, the extreme nonlinear nature of the high harmonic process means that intensity fluctuations can limit measurement sensitivity. Here we present a noise-canceled, tabletop high harmonic beamline for time-resolved reflection mode spectroscopy of magnetic materials. We use a reference spectrometer to independently normalize the intensity fluctuations of each harmonic order and eliminate long term drift, allowing us to make spectroscopic measurements near the shot noise limit. Here, these improvements allow us to significantly reduce the integration time required for high signal-to-noise (SNR) measurements of element-specific spin dynamics. Looking forward, improvements in the HHG flux, optical coatings, and grating design can further reduce the acquisition time for high SNR measurements by 1–2 orders of magnitude, enabling dramatically improved sensitivity to spin, charge, and phonon dynamics in magnetic materials.

47 OTHER INSTRUMENTATION↗

Coded-mask-based wavefront sensing technique for APS nanofocusing beamline diagnostics

Here, we extend our recently developed coded-mask wavefront sensing technique to enable single-shot measurements of nanofocused x-ray beams. This method accurately reconstructs the focal beam profile by backpropagating the wavefront measured downstream of the beam focus. To validate its performance, we benchmarked it against the conventional fluorescence wire scan method, successfully measuring ∼120 nm focal spots at the 28-ID-B beamline of the Advanced Photon Source using a polymeric compound refractive lens. The results highlight the effectiveness of coded-mask wavefront sensing for high-precision beam profiling and its application as a real-time wavefront monitoring tool.

Shi, Xianbo [Argonne National Laboratory (ANL), Ar↗

Application and performance of the novel Elcomat 5000 autocollimator in slope-measuring profilometry of beamline optics

Autocollimators are used in profilometers for the precise form measurement of beam-shaping optics for synchrotron light sources and x-ray free-electron lasers. This application requires using an aperture stop, typically 2.5 mm in diameter, which limits the footprint of the autocollimator’s measuring beam on the optics to achieve a sufficiently high lateral resolution. Central to the development of profilometry has been the availability of commercial autocollimators, such as the Elcomat 3000 from Möller–Wedel Optical. Although autocollimators are generally not designed for use with small apertures, this device has proven capable and has become the de facto standard. Now that it has been replaced by the Elcomat 5000, we evaluate the performance of several autocollimators of this type at small apertures, including the characterization of instrument transfer functions with a chirped height profile. We demonstrate that the Elcomat 5000 is capable of repeatable angle measurements with a standard deviation of 0.014 arcsec at an aperture diameter of 1.6 mm, whereas the Elcomat 3000 achieves 0.03 arcsec at 2.5 mm, comparing models with modified reticle designs. Here, we also investigate the influence of optical aberrations of the autocollimator’s objective and their changes with the path length to the surface under test. We characterize the sensitivity of the angle measurement to changes in environmental parameters, in particular, barometric pressure. These efforts are aimed at approaching fundamental limits in the characterization of the shape of optical surfaces with autocollimator-based profilometers so that these are ready for characterizing the next generation of synchrotron and XFEL beamline optics.

angle metrology↗

Synchrotron Catalysis Consortium (SCC) at NSLS-II: Dedicated Beamline Facilities for In Situ and Operando Characterization of Catalysts

The Synchrotron Catalysis Consortium (SCC) was funded and established in September 2005 at the National Synchrotron Light Source (NSLS) at Brookhaven National Laboratory (BNL). For more than a decade, the SCC was the first of its kind in the United States, with a mission to promote the utilization of synchrotron techniques for cutting-edge catalysis research under in-situ conditions. The consortium consists of three Principal Investigators (Jingguang Chen, Columbia University, Anatoly Frenkel, Stony Brook University/BNL, and Jose Rodriguez, BNL) and scientific staff member Nebojsa Marinkovic. The initial team also included Radoslav Adzic, BNL, and collaborators from academic, national, and industrial laboratories. During the first decade of its operations at three NSLS beamlines (X18A, X18B, and X19A) until the closing of NSLS on September 30, 2014, the primary goal of the SCC team was to provide assistance and to develop new sciences/techniques to the catalysis community...This report outlines a brief history, specifications, techniques, and training and outreach for the facility.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

The meV-resolved Inelastic X-ray Scattering Beamline at NSLS-II: Design and Performance

The ultrahigh resolution inelastic X-ray scattering (IXS) beamline at NSLS-II is designed and built to achieve sub-meV resolution at a moderate energy of 9.13 keV for IXS experiments with high momentum resolution and high spectral contrast. The key instrument is a novel spectrometer featuring a new type of analyzer optics, which combines post-sample collimation with angular dispersive crystal optics. As the first user instrument of its kind, the spectrometer has demonstrated unique research capabilities in exploring low momentum transfer (Q), THz dynamics in soft material systems characterized by mesoscopic heterogeneity and complexity, such as liquid crystals and bio-membranes. Ongoing efforts to improve performance since the start of user operations have resulted in a state-of-the-art energy resolution in routine operations of less than 1.4 meV, with sharp Gaussian-like tails, making it a premier IXS spectrometer for studying the dynamics of soft materials, while also delivering competitive performance for investigating phonon dynamics in hard condensed matter systems, including a broad range of quantum materials.

43 PARTICLE ACCELERATORS↗

Dynamics of magnetic evaporative beamline cooling for the preparation of cold atomic beams

The most sensitive direct neutrino mass searches today are based on measurement of the end point of the 𝛽 spectrum of tritium to infer limits on the mass of the unobserved neutrino. To avoid the smearing associated with the distribution of molecular final states in the T-He molecule, the next generation of these experiments will need to employ atomic (T) rather than molecular (T 2 ) tritium sources, at currents of at least 10 15 atoms per second. Following production, atomic T can be trapped in gravitational and/or magnetic bottles for 𝛽 spectrum experiments, if and only if it can first be cooled to millikelvin temperatures. Accomplishing this cooling presents substantial technological challenges. The Project 8 collaboration is developing a technique based on magnetic evaporative cooling along a beamline (MECB) for the purpose of cooling T to feed a magnetogravitational trap that also serves as a cyclotron radiation emission spectroscope. Initial tests of the approach are planned in a pathfinder apparatus using atomic Li. Here, this paper presents a method for analyzing the dynamics of the MECB technique and applies these calculations to the design of systems for cooling and slowing of atomic Li and T. A scheme is outlined that could provide a current of T at the millikelvin temperatures required for the Project 8 neutrino mass search.

atom optics↗