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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 73 records · Page 4

Non-destructive depth-resolved characterization of residual strain fields in high electron mobility transistors using differential aperture x-ray microscopy

Localized residual stress and elastic strain concentrations in microelectronic devices often affect the electronic performance, resistance to thermomechanical damage, and, likely, radiation tolerance. A primary challenge for the characterization of these concentrations is that they exist over sub-μm length-scales, precluding their characterization by more traditional residual stress measurement techniques. Here, in this study, we demonstrate the use of synchrotron x-ray-based differential aperture x-ray microscopy (DAXM) as a viable, non-destructive means to characterize these stress and strain concentrations in a depth-resolved manner. DAXM is used to map two-dimensional strain fields between the source and the drain in a gallium nitride (GaN) layer within high electron mobility transistors (HEMTs) with sub-μm spatial resolution. Strain fields at various positions in both pristine and irradiated HEMT specimens are presented in addition to a preliminary stress analysis to estimate the distribution of various stress components within the GaN layer. γ-irradiation is found to significantly reduce the lattice plane spacing in the GaN along the sample normal direction, which is attributed to radiation damage in transistor components bonded to the GaN during irradiation.

42 ENGINEERING↗

Radio frequency electrical resistance measurement under destructive pulsed magnetic fields

We developed a resistance measurement using radio frequency reflection to investigate the electrical transport characteristics under destructive pulsed magnetic fields above 100 T. A sample stage consisting of a homemade flexible printed circuit reduced the noise caused by the induced voltage from the pulsed magnetic fields, improving the accuracy of the measurements of the reflected waves. From the obtained reflectance data, the absolute value of the magnetoresistance was successfully determined by analyzing the phase with admittance charts. In conclusion, these developments enable more accurate and comprehensive measurements of electrical resistance in pulsed magnetic fields.

47 OTHER INSTRUMENTATION↗

Destruction of absorbing metal films during laser printing with gel microdroplets

The degree of destruction and evaporation of metal films (Au and Ti, thickness ∼50 nm) with a gel layer during laser transfer of small volumes of a gel substrate is estimated depending on the laser fluence value. The dynamics of these processes for dry films and films with a gel layer at fluences close to threshold values is investigated using a probe beam of a He – Ne laser. It is shown that the presence of a gel leads to an increase in the ablation threshold, but the time during which the process of structural changes in the film material is completed does not change significantly. The results obtained can be used to improve the laser bioprinting technology. (interaction of laser radiation with matter)

36 MATERIALS SCIENCE↗

Model-based, in-situ, non-destructive qualification and certification of parts made by autonomous additive manufacturing

To address the significant productivity challenges associated with the qualification and certification (Q&C) tasks of additively manufactured (AM) parts, which have traditionally relied on rigorous post‐build inspection and testing, we propose an integrated framework that combines model‐based qualification and certification (MBQ&C) with autonomous additive manufacturing (AAM). MBQ&C employs high‐fidelity predictive models, developed within the Integrated Computational Materials Engineering (ICME) paradigm, to simulate process–structure–property–performance relationships for assessing a part’s fitness for use. Since predictive models are commonly machine learning (ML)-based or reduced-order surrogates of validated physics models, they run efficiently, enabling timely inference. In parallel, the self-driving AAM utilises ML-based adaptive, closed‐loop control strategies to avoid, mitigate, or repair defects and anomalies during fabrication, thereby increasing the likelihood of producing acceptable parts. A key feature of the combined AAM-MBQ&C framework is that predictive models explicitly incorporate defects or anomalies that persist after the build, using instance-specific data captured via in-situ sensing. This customisation enables a build‐specific assessment of fitness for use, rather than relying on nominal or generic parameters. Such individualised evaluation provides a robust basis for Q&C-related acceptance decisions relating to each build. Additionally, the rapid solution capabilities of ML or reduced-order models enable the determination of a part’s suitability for service shortly after build completion. As the framework matures, it has the potential to substantially reduce reliance on conventional point‐design approaches—such as time‐consuming post‐build computed tomography scanning and costly destructive testing. Thus, the AAM-MBQ&C framework represents a transformative, scalable strategy for quality assurance of AM components, as parts produced within a stable, validated, and certified envelope can be certified with reduced testing. Key benefits include: (1) significant gains in Q&C productivity through efficient, model-centric assessment; (2) performance-based classification of defects into critical and non-critical categories; (3) the ability to predict potential deviations in the performance of parts affected by real-time, adaptive process control interventions relative to those produced under a certified process, and (4) the enabling of virtual Q&C for service environments that are difficult, hazardous, or impractical to access or reproduce experimentally. Collectively, these capabilities strengthen the business case for AM, particularly for high‐consequence and mission‐critical applications. Finally, although this work focuses on powder-based AM, the proposed techniques could be extended to AM processes employing alternative feedstock forms.

Gunasegaram, Dayalan↗

Low-energy 23 Al β-delayed proton decay and 22 Na destruction in novae

The radionuclide 22 Na is a target of γ-ray astronomy searches, predicted to be produced during thermonuclear runaways driving classical novae. The 22 Na (p, γ) 23 Mg reaction is the main destruction channel of 22 Na during a nova, hence, its rate is needed to accurately predict the 22 Na yield. However, experimental determinations of the resonance strengths have led to inconsistent results. In this Rapid Communication, we report a measurement of the branching ratios of the 23 Al β-delayed protons as a probe of the key 204-keV (center-of-mass) 22 Na (p, γ) 23 Mg resonance strength. We report a factor of 5 lower branching ratio compared to the most recent literature value. The variation in 22 Na yield due to nuclear data inconsistencies was assessed using a series of hydrodynamic nova outburst simulations and has increased to a factor of 3.8, corresponding to a factor of ≈ 2 uncertainty in the maximum detectability distance. Finally, this is the first reported scientific measurement using the Gaseous Detector with Germanium Tagging system.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Dark matter catalyzed baryon destruction

WIMP-type dark matter may have additional interactions that break baryon number, leading to induced nucleon decays which are subject to direct experimental constraints from proton decay experiments. In this work, we analyze the possibility of continuous baryon destruction, deriving strong limits from the dark matter accumulating inside old neutron stars, as such a process leads to excess heat generation. We construct the simplest particle dark matter model that breaks the baryon and lepton numbers separately but conserves B - L. Virtual exchange by DM particles in this model results in dinucleon decay via nn → $n\overline{v}$ and np → ne⁺ processes.

79 ASTRONOMY AND ASTROPHYSICS↗

Destructive Error Interference in Product-Formula Lattice Simulation

Quantum computers can efficiently simulate the dynamics of quantum systems. Here, we study the cost of digitally simulating the dynamics of several physically relevant systems using the first-order product-formula algorithm. We show that the errors from different Trotterization steps in the algorithm can interfere destructively, yielding a much smaller error than previously estimated. In particular, we prove that the total error in simulating a nearest-neighbor interacting system of n sites for time t using the first-order product formula with r time slices is O ( n t / r + n t 3 / r 2 ) when n t 2 / r is less than a small constant. Given an error tolerance ϵ , the error bound yields an estimate of max { O ( n 2 t / ϵ ) , O ( n 2 t 3 / 2 / ϵ 1 / 2 ) } for the total gate count of the simulation. The estimate is tighter than previous bounds and matches the empirical performance observed in Childs et al. [ Proc. Natl. Acad. Sci. U.S.A. 115 , 9456 (2018) ]. We also provide numerical evidence for potential improvements and conjecture an even tighter estimate for the gate count.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

MIND-MAC: Multi-Level In-memory Quasi Non-Destructive MAC Operation in Compact 2T-nC FeRAM for Efficient DNN Accelerator

We present MIND-MAC, a compact 2T-nC FeRAM architecture that performs multi-level, quasi-non-destructive in-memory multiply–accumulate (MAC) for deep neural networks. By exploiting voltage-controlled partial domain switching in MFM capacitors and read-transistor amplification, the cell stores multi-bit weights and gates bit-serial inputs to produce an accumulated current on shared lines. We combine TCAD-extracted parasitics with experimentally calibrated ferroelectric models in SPICE to validate device-/circuit-level behavior, and validate multi-level sensing and QNRO with measurements on a fabricated 2T-3C test vehicle. An analytical system model maps MIND-MAC to a 6-GB main-memory in-memory compute (IMC) architecture and benchmarks VGG13 inference in 61.08 ms at 964.99 mJ. Results indicate high density, reduced rewrite overhead, and energy efficiency, positioning 2T-nC FeRAM as a promising IMC candidate for next-generation AI hardware.

36 MATERIALS SCIENCE↗

Direct measurement of fluorocarbon radicals in the thermal destruction of perfluorohexanoic acid using photoionization mass spectrometry

Thermal destruction is a critical cornerstone of addressing the rampant contamination of natural resources with per- and polyfluoroalkyl substances (PFAS). However, grave concerns associated with stack emissions from incineration exist because mechanistic studies have thus far relied on ex situ analyses of end products and theoretical calculations. Here, we used synchrotron-based vacuum ultraviolet photoionization mass spectrometry to study the pyrolysis of a representative PFAS-perfluorohexanoic acid-and provide direct evidence of fluorocarbon radicals and intermediates. A key reaction pathway from perfluorocarboxylic acids to ketenes via acyl fluorides is proposed. We furthermore propose CF2/CF3 radical-centered pyrolysis mechanisms and explain their roles in the formation of other products that may form in full-scale incinerators. These results have not only unveiled the role of radicals and intermediates in thermal PFAS decomposition and recombination mechanisms but also provide unique insight into improving the safety and viability of industrial PFAS incineration.

Xu, Ming-Gao↗

Typha angustifolia non-destructive biomass data from an upland tidal brackish marsh, PIE LTER, Byfield, MA, (2022-2024)

This dataset contains non-destructive measurements of key features of Typha angustifolia samples. These samples were measured during the growing season in 2022, 2023, and 2024 in an upland brackish tidal wetland along the Parker River, Byfield, Massachusetts (MA), which is within the Plum Island Ecosystems Long Term Ecological Research Station (PIE LTER). Measurements were taken to investigate the difference in above ground biomass between two locations, the marsh interior (MI) and the creek bank (CB) and to support an allometric equation used to predict aboveground Typha angustifolia biomass per square meter. No QA/QC procedures were applied to the data. Metadata files Typha_biomass_observations_dd.csv and Typha_biomass_observations_flmd.csv contain detailed information on variable definitions, sampling methods, and the location of the site.

CULM_D_1↗

Non-destructive Examinations of ATF-2 Baseline Rodlets

This report contains the results of non-destructive examinations of Accident Tolerant Fuels 2 (ATF-2) rodlets irradiated in the Advanced Test Reactor (ATR) Loop 2A. The experiment is part of the U.S. Department of Energy Nuclear Technology Research and Development (NTRD) program’s Advanced Fuels Campaign (AFC). The rodlets were composed of UO2 pellets and Zr-4 cladding. The data have been collected to provide baseline PIE data to support future testing in TREAT and to have performance data against which the data of the ATF concepts can be compared directly. The analyses performed included: visual examinations, axial gamma scanning, neutron radiography and profilometry. All the data collected showed a performance consistent with expectations for this fuel system at low burnup.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Applicability of the ARCON96 Code to the Radiological Consequence Analysis of Releases from the Radioassay and Non-Destructive Testing (RANT) Facility

Establish technical justification to demonstrate that the horizontal diffusion parameter (σy) and vertical diffusion parameter (σz) that are embedded in the Nuclear Regulatory Commission (NRC) Atmospheric Relative CONcentrations (ARCON96) code are representative of the meteorological conditions at LANL. Compare the ARCON96 atmospheric diffusion factor ( X /Q) to the MACCS2-calculated X /Q for the determination of radiological consequences of ground releases from the Radioassay and Non-Destructive Testing (RANT) facility on the key receptors, the colocated worker (CW) and Maximally-Effected Offsite Individual (MEOI).

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗

Sister Rod Destructive Examinations (FY20)

As a part of DOE NE High Burnup Spent Fuel Data Project, Oak Ridge National Laboratory (ORNL) is performing destructive examinations (DEs) of high burnup (HBU) (>45 GWd/MTU) spent nuclear fuel (SNF) rods from the North Anna Nuclear Power Station operated by Dominion Energy. The SNF rods, called sister rods or sibling rods, are all HBU and include four different kinds of fuel rod cladding: standard Zircaloy-4 (Zirc-4), low-tin Zirc-4, ZIRLO, and M5. The DEs are being conducted to obtain a baseline of the HBU rod’s condition before dry storage and are focused on understanding overall SNF rod strength and durability. Composite fuel and defueled cladding will be tested to derive material properties. Although the data generated can be used for multiple purposes, one primary goal for obtaining the post-irradiation examination data and the associated measured mechanical properties is to support SNF dry storage licensing and relicensing activities by (1) addressing identified knowledge gaps and (2) enhancing the technical basis for post-storage transportation, handling, and subsequent disposition. This report documents the status of the ORNL Phase I DEs of 8 sister rods and outlines the DE tasks performed and the data collected to date, as guided by the sister rod test plans.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Sister Rod Destructive Examinations (FY20) Appendix A: Full Length Rod Heat Treatments (FHT)

As a part of the US DOE-NE High Burnup Spent Fuel Data Project, ORNL is performing destructive examinations (DEs) of high burnup (HBU) (>45 gigawatt days per metric ton uranium) spent nuclear fuel (SNF) rods from the North Anna Nuclear Power Station operated by Dominion Energy. The SNF rods, called the “sister rods,” are all HBU and include four different kinds of fuel rod cladding: standard Zircaloy-4, low-tin Zircaloy-4, ZIRLO®, and M5®. The DEs are being conducted to obtain a baseline of the HBU rod’s condition prior to dry storage and are focused on understanding overall SNF rod strength and durability. Both composite fuel and empty cladding are being tested. While the data generated can be used for multiple purposes, a primary goal for obtaining the post-irradiation examination data will support SNF dry storage licensing and relicensing activities.This report documents the status of the ORNL Phase 1 DE activities related to full length rod heat treatments (FHT) applied to selected sister rods in Phase 1 of the sister rod test program. The results of this work and detailed examinations are summarized in the Sister Rod DE Status Report.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Sister Rod Destructive Examinations (FY20) Appendix B: Segmentation, Defueling, Metallograhic Data and Total Cladding Hydrogen

As a part of the US DOE-NE High Burnup Spent Fuel Data Project, ORNL is performing destructive examinations (DEs) of high burnup (>45 gigawatt days per metric ton uranium) spent nuclear fuel (SNF) rods from the North Anna Nuclear Power Station operated by Dominion Energy. The SNF rods, called the “sister rods,” are all HBU and include four different kinds of fuel rod cladding: standard Zircaloy-4, low-tin Zircaloy-4, ZIRLO®, and M5®. The DEs are being conducted to obtain a baseline of the HBU rod’s condition prior to dry storage and are focused on understanding overall SNF rod strength and durability. Both composite fuel and empty cladding are being tested. While the data generated can be used for multiple purposes, a primary goal for obtaining the post-irradiation examination data and the associated measured mechanical properties is to support SNF dry storage licensing and relicensing activities.This report documents the status of the ORNL Phase 1 DE activities related to: rough segmentation, defueling, optical microscopy, and cladding total hydrogen measurements for 7 Phase 1 sister rods and outlines the DE tasks performed and the data collected to date. The results of these detailed examinations and others are summarized in the Sister Rod DE Status Report.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Phosgene Neutralization Chemistry for the Explosive Destruction System (EDS)

This report summarizes activities at Sandia National Laboratories as part of the Explosive Destruction System (EDS) Phase 3 (P3) System design. An exploration of chemical neutralization strategies of phosgene was conducted for safe disposal of recovered mortars and M79 1000 lb. bombs filled with carbonyl dichloride "phosgene" or "CG agent" (molecular formula = COCl 2 ). The incumbent strategy utilized aqueous sodium hydroxide was found to be the worst-case scenario, producing enough CO 2 gas that would cause an unacceptable pressure and temperature spike. Several chemical neutralization strategies were evaluated based on criteria set by the operating envelope of the P3 design. In the end, it was determined that a pure solution of N-methyl ethanolamine (MeEA) or 90% monoethanolamine (MEA)(aqueous) provided the best balance reaction profile, cost, and safety.

36 MATERIALS SCIENCE↗

Evaluation of the Impact of Additional Manganese from the Recycle Collection Tank (RCT) Glycolate Destruction Process on Glass Properties

The Defense Waste Processing Facility (DWPF) is planning to implement glycolic acid as a reductant within the waste processing flowsheet. An assessment of the glycolic acid flowsheet has revealed the potential for thermolytic production of hydrogen in the Concentration, Storage and Transfer Facilities (CSTF) from glycolate entrained in the DWPF recycle stream. To mitigate this potential scenario, a glycolate destruction process utilizing sodium permanganate (NaMnO 4 ) is being developed for use in the DWPF Recycle Collection Tank (RCT). The RCT is fed by the Slurry Mix Evaporator Condensate Tank (SMECT) and the Off-Gas Condensate Tank (OGCT). The SMECT could receive glycolate via a foamover from the Sludge Receipt and Adjustment Tank (SRAT) or the Slurry Mix Evaporator (SME), and the OGCT could receive glycolate via carryover of sludge particles in the purge from the melter during surge conditions. The use of NaMnO 4 additions in the RCT will result in additional manganese (Mn) in the waste stream and needs to be evaluated.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗