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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 73 records · Page 4
All sourcesNASA NTRSDOE OSTI
DOE OSTI2021

Coulomb excitation of 80,82 Kr and a change in structure approaching N = Z = 40

Nuclei approaching N = Z = 40 are known to exhibit strongly deformed structures and are thought to be candidates for shape coexistence. In the krypton isotopes, 80,82 Kr are poorly characterized, preventing an understanding of evolving deformation approaching N = 40. The present work aims to determine electric quadrupole transition strengths and quadrupole moments of 80,82 Kr in order to better characterize their deformation. Sub-barrier Coulomb excitation was employed, impinging the isotopes of krypton on 196 Pt and 208 Pb targets. Utilizing a semiclassical description of the safe Coulomb-excitation process E 2 matrix elements could then be determined. Eleven new or improved matrix elements are determined in 80 Kr and seven in 82 Kr . The new B(E2;0$^+_1$ → 2$^+_1$ ) value in 82 Kr disagrees with the evaluated value by 3σ , which can be explained in terms of deficiencies in a previous Coulomb-excitation analysis. Conclusions: Comparison of measured Q s ( 2$^+_1$ ) and B(E2; 0$^+_1$ → 2$^+_1$ ) values indicates that neutron-deficient ( N ≤ 42 ) isotopes of krypton are closer to axial deformation than other isotopic chains in the mass region. A continuation of this trend to higher Z may result in Sr and Zr isotopes exhibiting near-axial prolate deformation.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2023

Quasiparticle random-phase approximation calculations for M 1 transitions with the noniterative finite-amplitude method and application to neutron radiative capture cross sections

Here, we derive the equations of quasiparticle random-phase approximation (QRPA) based on the finite amplitude method with the Hartree-Fock+Bardeen–Cooper–Schrieffer (HF+BCS) single-particle states, and calculate the magnetic dipole (M⁢1) transition for deformed gadolinium isotopes. Our QRPA calculation shows both large spin-flip transitions in the 5 to 10 MeV excitation energy and the low energy orbital transition that would correspond to the M⁢1 scissors mode observed in nuclear experiments. Then, we calculate neutron capture reactions based on the statistical Hauser-Feshbach theory with the photoabsorption cross sections of even-even nuclei given by QRPA. We find that the capture cross section is enhanced due to the contribution from the low energy M⁢1 transition although the calculated capture cross section still underestimates the experimental data. This issue in the calculated capture cross section could be improved by uncertainties of the low energy E⁢1 transition neglected in our QRPA calculation.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2023

Measurement of the $\textit{B}(\textit{E}2 ↑)$ strengths of 36 Ca and 38 Ca

In this work, the $B(E2, 0^+_1 → 2^+_1)$ strengths of 36 Ca and 38 Ca are measured to be 131(20) $e^2\text{fm}^4$ and 101(11) $e^2\text{fm}^4$, respectively. The $\textit{B}(\textit{E}2)$ value for 36 Ca required a measurement of the p/γ branching ratio because the 2 + state is proton unbound. This branching ratio is $B_p$=0.087(8). These $\textit{B}(\textit{E}2)$ and branching-ratio values can be reproduced in the shell-model with the ZMB2 interaction, an interaction that predicts the $\textit{Z} = 20 \textit{sd}$-shell closure is incomplete with large proton pf-shell occupancies in the ground state. These occupancies are at odds with other shell-model and energy-density-functional calculations of 36 Ca. New data are used to provide an update on constraints of the density dependence of the symmetry energy through mirror charge-radii differences as well as to help reduce uncertainties of the astrophysical important 35 K(p,γ) reaction.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
NASA NTRS1987

Waveguide-Horn-to-Waveguide Transition Assembly

Microstrip-to-waveguide transition integrated with waveguide-horn antenna element. Integrated transition assembly couples electromagnetic energy through horn and transition board to connector.

Davidson, Shayla E.↗
DOE OSTI2022

Robust ab initio prediction of nuclear electric quadrupole observables by scaling to the charge radius

Meaningful predictions for electric quadrupole (E2) observables from ab initio nuclear theory are necessary, if the ab initio description of collective correlations is to be confronted with experiment, as well as to provide predictive power for unknown E2 observables. However, converged results for E2 observables are notoriously challenging to obtain in ab initio no-core configuration interaction (NCCI) approaches. Matrix elements of the E2 operator are sensitive to the large-distance tails of the nuclear wave function, which converge slowly in an oscillator basis expansion. Similar convergence challenges beset ab initio prediction of the nuclear charge radius. We demonstrate that the convergence patterns of the E2 and radius observables are strongly correlated, and that meaningful predictions for the absolute scale of E2 observables may be made by calibrating to the experimentally-known ground-state charge radius. Here, we illustrate by providing robust ab initio predictions for several E2 transition strengths and quadrupole moments in p-shell nuclei, in cases where experimental results are available for comparison.

6 ≤ A ≤ 19↗
DOE OSTI2022

Ab initio estimation of E 2 strengths in Li 8 and its neighbors by normalization to the measured quadrupole moment

For electric quadrupole (E2) observables, which depend on the large-distance tails of the nuclear wave function, ab initio no-core configuration interaction (NCCI) calculations converge slowly, making meaningful predictions challenging to obtain. Nonetheless, the calculated values for different E2 matrix elements, particularly those involving levels with closely-related structure (e.g., within the same rotational band) are found to be robustly proportional. This observation suggests that a known value for one observable may be used to determine the overall scale of E2 strengths, and thereby provide predictions for others. In particular, we demonstrate that meaningful predictions for E2 transitions may be obtained by calibration to the ground-state quadrupole moment. Here, we test this approach for well-measured low-lying E2 transitions in 7 Li and 9 Be, then provide predictions for transitions in 8 Li and 9 Li. In particular, we address the 2 + → 1 + transition in 8 Li, for which the reported measured strength exceeds ab initio Green's function Monte Carlo (GFMC) predictions by over an order of magnitude.

6 ≤ A ≤ 19↗
DOE OSTI2021

Lifetime measurements in the even-even Cd 102 – 108 isotopes

The heaviest T z = 0 doubly-magic nucleus, Sn 100 , and the neighboring nuclei offer unique opportunities to investigate the properties of nuclear interaction. For instance, the structure of light-Sn nuclei has been shown to be affected by the delicate balance between nuclear-interaction components, such as pairing and quadrupole correlations. From Cd to Te, many common features and phenomena have been observed experimentally along the isotopic chains, leading to theoretical studies devoted to a more general and comprehensive study of the region. In this context, having only two proton holes in the Z = 50 shell, the Cd isotopes are expected to present properties similar to those found in the Sn isotopic chain. The aim of this work was to measure lifetimes of excited states in neutron-deficient nuclei in the vicinity of Sn 100 . Here, the neutron-deficient nuclei in the N ≈ Z ≈ 50 region were populated using a multinucleon transfer reaction with a Cd 106 beam and a Mo 92 target. The beamlike products were identified by the VAMOS + + spectrometer, while the γ rays were detected using the AGATA array. Lifetimes of excited states were determined using the recoil distance Doppler-shift method, employing the Cologne differential plunger. Lifetimes of low-lying states were measured in the even-mass Cd 102 – 108 isotopes. In particular, multiple states with excitation energy up to ≈ 3 MeV, belonging to various bands, were populated in Cd 106 via inelastic scattering. The transition strengths corresponding to the measured lifetimes were compared with those resulting from state-of-the-art beyond-mean-field calculations using the symmetry-conserving configuration-mixing approach. Conclusions: Despite the similarities in the electromagnetic properties of the low-lying states, there is a fundamental structural difference between the ground-state bands in the Z = 48 and Z = 50 isotopes. The comparison between experimental and theoretical results revealed a rotational character of the Cd nuclei, which have prolate-deformed ground states with β 2 ≈ 0.2 . At this deformation Z = 48 becomes a closed-shell configuration, which is favored with respect to the spherical one.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2021

Independent normalization for γ -ray strength functions: The shape method

Here, the shape method, a novel approach to obtain the functional form of the γ-ray strength function (γSF), is introduced. In connection with the Oslo method the slope of the nuclear level density (NLD) and γSF can be obtained simultaneously even in the absence of neutron resonance spacing data. The foundation of the shape method lies in the primary γ-ray transitions which preserve information on the functional form of the γSF. The shape method has been applied to 56 Fe, 92 Zr, and 164 Dy, which are representative cases for the variety of situations encountered in typical NLD and γSF studies. The comparisons of results from the shape method to those from the Oslo method demonstrate that the functional form of the γSF is retained regardless of nuclear structure details or J π values of the states fed by the primary transitions.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2025

Robust ab initio predictions for dimensionless ratios of 𝐸⁢2 and radius observables. II. Estimation of 𝐸⁢2 transition strengths by calibration to the charge radius

Converged results for 𝐸⁢2 observables are notoriously challenging to obtain in ab initio no-core configuration interaction approaches. Matrix elements of the 𝐸⁢2 operator are sensitive to the large-distance tails of the nuclear wave function, which converge slowly in an oscillator basis expansion. Similar convergence challenges beset ab initio prediction of the nuclear charge radius. However, we exploit systematic correlations between the calculated 𝐸⁢2 and radius observables to yield meaningful predictions for relations among these observables. In particular, we examine ab initio predictions for dimensionless ratios of the form 𝐵⁡(𝐸⁢2)/(𝑒 2 ⁢𝑟 4 ) for nuclei throughout the 𝑝 shell. Finally, meaningful predictions for 𝐸⁢2 transition strengths may then be made by calibrating to the ground-state charge radius if experimentally known.

ab initio calculations↗
DOE OSTI2021

Nuclear structure and band mixing in Pt 194

We introduce a two-particle, two-hole mixed configuration scheme to fit E2 strengths for the 0 ↔ 2, 2 ↔ 4, and 4 ↔ 6 transitions in 194 Pt. The interaction includes two sets of pairing operators, {S ± (t), S 0 (t)} (t = s, d). Solutions within this framework are used to analyze energy spectra, E2 transitions, and band-mixing features of the model. The results confirm that mixing is small and similar for J = 2, 4, and 6, with the calculated energies and transition matrix elements in excellent agreement with experimental data.

190 ≤ A ≤ 219↗
DOE OSTI2020

New, low-energy excitations in 107 Mo and 109 Mo

New ground-state level with spin-parity 1/2 + is established in 109 Mo, 69.8 keV below the previously reported 5/2(+) ground state in this nucleus, based on precise spectroscopy measurements of gamma radiation following spontaneous fission of 248 Cm performed using the Eurogam2 array of anti-Compton spectrometers. Analogous measurement of gamma radiation following spontaneous fission of 252 Cf, performed using the Gammasphere array, confirms the new 1/2 + ground state of 107 Mo, proposed recently and establishes the isomeric character of the 5/2 + first excited state in 107 Mo. Two beta-decaying isomers are suggested in 111 Mo nucleus based on regular energy systematics, supporting previous predictions. Low-energy excitations in Mo isotopes are interpreted and compared to calculations reported in the literature. The results suggest shape transition from prolate to oblate deformation at N >= 67.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2021

Dipole response in Te 128 , 130 below the neutron threshold

Numerous studies of the ground-state decay of the pygmy dipole resonance (PDR) have been carried out in the past. However, data on the decay of the PDR to low-lying excited states is still very scarce due to limitations of the sensitivity to weak branching transitions of experimental setups. Here, we present a detailed examination of the low-energy dipole response of 128 Te and 130 Te below their neutron separation thresholds of 8.8 and 8.5 MeV, respectively. Photonuclear reactions with the subsequent γ-ray spectroscopy of the decay channel with continuous-energy bremsstrahlung at varying endpoint energies and linearly polarized quasimonochromatic γ-ray beams with energies ranging from 2.7 to 8.9 MeV in steps of roughly 250 keV were used for probing the decay behavior of the low-energy dipole response in 128Te and 130Te. In addition, (γ,γ' γ") reactions were used to study the population of low-lying states of 128 Te. Spin-parity quantum numbers and reduced transition probabilities are determined for individual photo-excited states. The analysis of average decay properties for nuclear levels in narrow excitation-energy bins enable the extraction of photoabsorption cross sections, average branching ratios to the $2$$^{+}_{1}$ state, and the distinction between E1 and M1 transitions to the ground state and to the $2$$^{+}_{1}$ state accounting for resolved and unresolved transitions.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2022

Noniterative finite amplitude methods for E 1 and M 1 giant resonances

The finite amplitude method (FAM) is a very efficient approach for solving the fully self-consistent random-phase approximation (RPA) equations. We use FAM to rederive the RPA matrices for Skyrme functionals, calculate the electric dipole ( E 1) and the magnetic dipole ( M 1) giant resonances, and compare the results with available experimental and evaluated data. For the E 1 transitions in heavy nuclei, the calculations reproduce well the resonance energy of the photoabsorption cross sections. In the case of M 1 transitions, we show that the residual interaction does not affect the transition strength of double-magic nuclei, which suggests that the spin terms in the Skyrme force currently neglected in the present computation could improve the agreement between FAM and experimental data.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2021

In-beam γ-ray spectroscopy of 62,64 Cr

The region of neutron-rich Cr isotopes has garnered much attention in recent years due to a rapid onset of collectivity near neutron number N = 40. We report here on the first γ-ray spectroscopy beyond the ($4$ $^{+}_{1}$) state in 62,64 Cr, using nucleon removal reactions from several projectiles within a rare-isotope beam cocktail. A candidate for the 6 + state in 64 Cr is presented as well as one for, possibly, the second excited 0 + state in 62 Cr. The results are discussed in comparison to the LNPS shell-model predictions that allow for neutron excitations across the N = 40 harmonic oscillator gap into the g 9/2 and d 5/2 orbitals. Here, the calculated level schemes for 62,64 Cr reveal intriguing collective structures. From the predicted neutron particle-hole character of the low-lying states in these Cr isotopes, 62 Cr emerges as a transitional system on the path to the center of the N = 40 island of inversion.

59 ≤ A ≤ 89↗
DOE OSTI2021

Nucleon-pair approximation for nuclei from spherical to deformed regions

Here we model low-lying states of atomic nuclei in the nucleon-pair approximation of the shell model, using three approaches to select collective nucleon pairs: the generalized seniority scheme, the conjugate gradient method, and the Hartree-Fock approach. We find the collective pairs obtained from the generalized seniority scheme provide a good description for nearly spherical nuclei, and those from the conjugate gradient method or the Hartree-Fock approach work well for transitional and deformed nuclei. Our NPA calculations using collective pairs with angular momenta 0, 2, and 4 (denoted by S D G pairs) reproduce the nuclear shape evolution in the N = 26 isotones, Ca 46 , Ti 48 , Cr 50 , and Fe 52 , and yield good agreement with full configuration-interaction calculations of low-lying states in medium-heavy transitional and deformed nuclei: Ti 44 – 48 , Cr 48 , Cr 50 , Fe 52 , Zn 60 – 64 , Ge 64 , 66 , Mo 84 , and Xe 108 – 112 . Finally, using the S D G I -pair approximation we describe low-lying states of Ba 112 , 114 , cases difficult to reach by conventional configuration-interaction methods.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2021

Structure of rotational bands in 109 Rh

Rotational bands in 109 Rh are investigated in a simple model and in the interacting boson-fermion model. We have developed a solvable extended transitional Hamiltonian by adding a two-configuration mixing term. Results suggest that 109 Rh is a good candidate for triaxiality and shape coexistence. Mixing between 3/2 + states with K = 1/2 and 3/2 is found to be weak, as evidenced by the E2 strengths.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2021

Structure of even-even Sr isotopes with 50 ≤ N ≤ 58 neutrons

Excited levels in Sr 90 , Sr 92 , Sr 94 , and Sr 96 nuclei were reinvestigated using high-statistics multiple- γ coincidence data from neutron-induced fission of U 235 and spontaneous fission of Cf 252 , measured using Exogam at Institut Laue Langevin and Gammasphere arrays, respectively. The experimental goal was the search for new excited levels and firm spin-parity assignments to known levels. A total of 23 new levels with 30 new or corrected decays and 39 new or improved spin-parity assignments were obtained in the four nuclei. Negative-parity structures on top of 3 - excitation were firmly identified and extended to higher spins. New positive-parity structures in Sr 94 and Sr 96 were observed with 3 + excitations characteristic of γ collectivity. The 277.7-keV, E 2 decay from the 1507.0-keV level to the second 0 + level in Sr 96 , found in this paper, completes the coexisting deformed band in this nucleus. To learn about the microscopic structure of levels in the Sr 88 - 96 nuclei, we performed large-scale shell-model calculations. The calculations compared to the experiment, helped the discussion of the evolution of collectivity in strontium isotopes, highlighting the important role of various single-particle excitations in phase transitions and shape coexistence in the region. The special role of the neutron 9 / 2 + [ 404 ] extruder as a catalyst of the deformation change in the region is highlighted.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗