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At least 73 records · Page 4

Investigating effects of relativistic kinematics, dimensionality, interactions, and short-range correlations on the ratio of quartic over quadratic nuclear symmetry energies

While ample evidence for the so-called empirical parabolic law of the Equation of State (EOS) of isospin asymmetric nuclear matter (ANM) has been obtained in many studies within both non-relativistic and relativistic nuclear many-body theories using various interactions, it has been unclear if there is any fundamental physics reason for the small quartic symmetry energy compared to the quadratic one even as the ANM approaches pure neutron matter. Within both relativistic and non-relativistic Free Fermi Gas (FFG) models in coordinate spaces of arbitrary dimension d with and without considering Short-Range Correlations (SRC) as well as non-linear Relativistic Mean Field (RMF) models, we study effects of relativistic kinematics, dimensionality, interactions and SRC on the ratio Ψ(ρ) of quartic over quadratic symmetry energies in ANM EOSs. We found that the ratio Ψ(ρ) in the FFG model depends strongly on the dimension d. While it is very small already in the normal 3D space, it could be even smaller in spaces with reduced dimensions for sub-systems of particles in heavy-ion reactions and/or whole neutron stars due to constraints, collectivities and/or symmetries. Here, we also found that the ratio Ψ(ρ) could theoretically become very large only at the ultra-relativistic limit far above the density reachable in neutron stars. On the other hand, nuclear interaction directly and/or indirectly through SRC-induced high-momentum nucleons affect significantly the density dependence of Ψ(ρ) compared to the relativistic FFG model prediction. The SRC affects significantly not only the kinetic energy of symmetric nuclear matter but also the ratio Ψ(ρ) while the relativistic corrections are found negligible. The results may help better understand the EOS of dense neutron-rich matter.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Joint LLNL, LANL, SNL, and IRSN High Multiplication Subcritical (Multiplicity) Benchmark Integral Experiment Execution (CED-3b Report)

This report documents the experimental configurations and measurements for IER-518: Joint LLNL, LANL, SNL, and IRSN High Multiplication Subcritical (Multiplicity) Benchmark Experiments. These measurements involved a series of subcritical configurations at the Sandia Critical Experiments (SCX) facility at Sandia National Laboratories (SNL). The purpose of these measurements was to produce time tagged neutron count data of configurations that exceed a subcritical multiplication of 20, which is the high end of the fundamental physics benchmarks currently available in the International Criticality Safety Benchmark Evaluation Project Handbook (ICSBEP). These measurements leverage experimental configurations 1 and detector systems 2 from previously accepted ICSBEP benchmark evaluations, allowing evaluations of these measurements to be performed at greatly reduced cost.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Equivalent Fundamental-Mode Source Simulations for Spherical Uranium and Plutonium Systems [Abstract]

The equivalent fundamental-mode source refers to a “source” which is identically distributed in space, energy, and angle as that of a fundamental-mode fission source distribution. It has previously been shown that the system fixed source multiplication ($M_{fs}$) relates to the effective multiplication factor ($\kappa_{eff}$) as $M_{fs} = \frac{g^*}{1-k_{eff}}$ The term $\mathcal{g}$* therefore relates the system source distribution to the system equivalent fundamental-mode source. As previously shown, the $\mathcal{g}$* term is approximately 1 for deeply subcritical systems and then diverges as the system multiplication increases. For a system with a point source located in the center of an assembly (such a sphere), $\mathcal{g}$* will be greater than 1; this happens because there is a higher probability of induced fission when all of the starter neutrons originate from the center of the sphere. For a uniform source, $\mathcal{g}$* is less than 1, but does not diverge from 1 as dramatically as seen by a point source. One reason that $\mathcal{g}$* is an important parameter is that it is used in measurement methods to infer reactor kinetics parameters ($β_{eff}$ being one example). This work will discuss multiple ways to simulate $\mathcal{g}$* using MCNP®6.2, which include use of traditional methods versus a single input file method that was recently published. A discussion related to methods to simulate $M_{fs}$ will be presented. Spherical systems of Highly Enriched Uranium (HEU) will be compared with previous works. In addition, results of plutonium including multiple reflector materials will be investigated. Simulated systems will include both parametric studies as well as configurations used in recent experiments performed at the National Criticality Experiments Research Center (NCERC). These studies will include subtleties associated with system geometry that have not been previously shown. Last, this work will investigate the relationship between $\mathcal{g}$* and reactor kinetics parameters (such as $β_{eff}$).

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

At-power subcritical multiplication in the advanced test reactor

The degree to which a given physical subdivision of a critical reactor acts as a neutron source for other lobes is not analytically characterized for general application. ATR and ATRC both operate at power, and individual power-producing lobes rely on each other as neutron sources in order to maintain constant power, which in general requires either exactly critical multiplication within a reactor or an external neutron source. Here, this work shows that lobe powers in ATR or ATRC can be related with subcritical multiplication theory, demonstrating that the lobes are not individually critical. This explanation is significant for ATR due to the desire to irradiate a large variety of experiments simultaneously, each having its impact on the core neutron population. This work also establishes the lack of relationship between experiment reactivity worth and cross-sections calculated from fundamental nuclear data. For any physical subdivision of any other critical reactor, it is likewise true that the subdivision undergoes only subcritical multiplication.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Dynamical Aspects of the Quark Gluon Plasma

Shortly after the Big Bang the entire universe was filled with a nearly perfect fluid known as the Quark Gluon Plasma. Relativistic heavy ion collisions can now reproduce this fluid in the laboratory where the Quark Gluon Plasma exhibits a rapid but smooth cross-over phase transition into hadrons at vanishing net-baryon densities. Recent experiments plan to explore finite baryon densities where a critical point is expected. If found, this would mark the first discovery of a critical point in a relativistic system described by a fundamental theory of nature, which would have far-reaching consequences for high-energy nuclear physics and nuclear astrophysics (such as in neutron star mergers). Characteristic temperatures of equilibrium (e.g. the inflection point of the entropy density) and transport coefficients (e.g. minimum of the shear viscosity over entropy density) vary widely at a cross-over phase transition but converge at a critical point, and extracting the behavior of these characteristic temperatures is a major focal point of this research. Specifically, the interplay between strange and light hadrons is exploited to study the flavor hierarchy in the cross-over region. To investigate this, a viscous relativistic hydrodynamics framework with two conserved charges is being developed into a new open-source code along with initial conditions that contain baryon number and strangeness. Flow observables sensitive to the equation of state and transport coefficients are calculated across beam energies. New techniques are being developed to study this flavor hierarchy from first principles and to extract the characteristic temperatures from experimental data. Through this new dynamical framework, this project provides essential guidance to the Beam Energy Scan II runs at Relativistic Heavy-Ion Collider and the future Facility for Antiproton and Ion Research facility in the search for the Quantum Chromodynamic critical point and subsequent investigation of the baryon-rich Quark Gluon Plasma.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Chapter 10.02 - Neutron Scattering Studies of Materials for Hydrogen Storage

Hydrogen storage presents a significant barrier to the widespread adaptation of hydrogen as an energy source in mobile and stationary applications. The development of new candidate hydrogen storage materials is therefore an outstanding goal in the field of inorganic chemistry. Neutron scattering techniques - including diffraction, inelastic, and quasielastic scattering - are integral in investigating these materials. Here, we review some of the key studies of candidate hydrogen storage materials which have employed neutron scattering techniques. We begin with a brief discussion of hydrogen's current position in the global energy landscape. Next, we provide a brief description of the theory and practical aspects of the neutron scattering techniques germane to the study of hydrogen storage. Then we enumerate the neutron scattering studies of candidate hydrogen storage materials, including metal hydrides, chemical hydrides, and porous compounds. We focus on the studies which helped develop our understanding of hydrogen storage by revealing the underlying fundamental physics and chemistry of hydrogen sorption in these systems. Finally, we provide an outlook to the future of hydrogen storage research.

chemical hydrides↗

Distinguishing prompt-collapse binary neutron star mergers from binary black Holes: Tidal effects and remnant properties

We study the properties of remnants formed in prompt-collapse binary neutron star mergers. We consider nonspinning neutron star binaries over a range of total masses and mass ratios across a set of 22 equations of state, totaling 107 numerical relativity simulations. We report the final mass and spin of the systems (including the accretion disk and ejecta) to be constrained in a narrow range—0.98 ≲ 𝑀 𝑓 /𝑀 ≲ 0.99 for the mass and 0.85 ≲ 𝑎 𝑓 ≲ 0.95 for the dimensionless spin—regardless of the binary configuration and matter effects. This sets them apart from binary black hole merger remnants. We assess the detectability of the postmerger signal in a future 40 km Cosmic Explorer observatory and find that the signal-to-noise ratio in the postmerger of an optimally located and oriented binary at a distance of 100 Mpc can range from <1 to 8, depending on the binary configuration and equation of state, with a majority of them greater than 4 in the set of simulations that we consider. We also consider the distinguishability between prompt-collapse binary neutron star and binary black hole mergers with the same masses and spins. We find that Cosmic Explorer will be able to distinguish such systems primarily via the measurement of tidal effects in the late inspiral. Neutron star binaries with reduced tidal deformability $\tilde{Λ}$ as small as ∼ 3.5 can be identified up to a distance of 100 Mpc, while neutron star binaries with $\tilde{Λ}$ ∼ 22 can be identified to distances greater than 250 Mpc. This is larger than the distance up to which the postmerger will be visible. Finally, we discuss the possible implications of our findings for the equation of state of neutron stars from the gravitational wave event GW230529.

79 ASTRONOMY AND ASTROPHYSICS↗

Strange Mesons and Gluonic Excitations

In the standard model of particle physics, the interactions between the fundamental constituents of nuclear matter, quarks and gluons, are governed by the theory of Quantum Chromodynamics (QCD). A central goal of nuclear physics is to understand how hadrons, such as protons and neutrons, are formed from these underlying quark and gluon degrees of freedom. A hadron is primarily constructed from three quarks or a quark-antiquark pair; however, the theory of QCD allows for much more exotic configurations. One of the predicted exotic configurations is known as a hybrid meson, which contains an excited gluonic field in addition to the usual quark-antiquark pair. This project aims to search for and study these gluonic excitations using the Gluonic Excitation (GlueX) experiment at Jefferson Lab in Newport News, VA. The discovery potential of the experiment will be significantly extended by studying the quark flavor composition of the meson spectrum through the completion and use of an enhanced detector to identify mesons containing strange quarks. The unprecedented statistical precision of the data collected at GlueX will allow us to search for a pattern of light-quark hybrid mesons, providing new insight into the interactions that bind the fundamental quarks and gluons into the hadrons we observe in nature.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Gravitational wave physics and astronomy in the nascent era

The detections of gravitational waves (GW) by the LIGO/Virgo collaborations provide various possibilities for both physics and astronomy. We are quite sure that GW observations will develop a lot, both in precision and in number, thanks to the continuous work on the improvement of detectors, including the expected new detector, KAGRA, and the planned detector, LIGO-India. On this occasion, we review the fundamental outcomes and prospects of gravitational wave physics and astronomy. We survey the development, focusing on representative sources of gravitational waves: binary black holes, binary neutron stars, and supernovae. We also summarize the role of gravitational wave observations as a probe of new physics.

79 ASTRONOMY AND ASTROPHYSICS↗

Differential analysis of incompressibility in neutron-rich nuclei

Both the incompressibility K A of a finite nucleus of mass A and that (K ∞ ) of infinite nuclear matter are fundamentally important for many critical issues in nuclear physics and astrophysics. While some consensus has been reached about K ∞ , accurate theoretical predictions and experimental extractions of K τ characterizing the isospin dependence of K A have been very difficult. We propose a differential approach to extract K τ and K ∞ independently from the K A data of any two nuclei in a given isotope chain. Applying this method to the K A data from isoscalar giant monopole resonances (ISGMR) in even-even Pb, Sn, Cd, and Ca isotopes taken by Garg et al. at the Research Center for Nuclear Physics (RCNP), Osaka University, Japan, we find that the 106 Cd– 116 Cd and 112 Sn– 124 Sn pairs having the largest differences in isospin asymmetries in their respective isotope chains measured so far provide consistently the most accurate up-to-date K τ value of K τ = –616 ± 59 MeV and K τ =–623 ± 86 MeV, respectively, largely independent of the remaining uncertainties of the surface and Coulomb terms in expanding K A , while the K ∞ values extracted from different isotopes chains are all well within the current uncertainty range of the community consensus for K ∞ . Moreover, the size and origin of the “soft Sn puzzle” is studied with respect to the “stiff Pb phenomenon.” Furthermore, it is found that the latter is favored due to a much larger (by ≈ 380 MeV) K τ for Pb isotopes than for Sn isotopes, while K ∞ from analyzing the K A data of Sn isotopes is only about 5 MeV less than that from analyzing the Pb data.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Neutron spin dynamics in polarized targets

We present neutron elastic scattering amplitude for arbitrary polarized target in irreducible spherical tensor representation. Here, the general approach for the description of neutron spin dynamics for the propagation trough the medium with an arbitrary polarization is discussed in a relation to the search for time reversal invariance violation in neutron scattering.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Joint LLNL, LANL, SNL, and IRSN High Multiplication Subcritical (Multiplicity) Benchmark Experiments Execution Plan (IER-518 CED-3a)

As part of the experiment design and planning, the critical experiment design team (CEDT), as well as additional stakeholders, convened a series of meetings to discuss the goals and requirements of execution for this experiment. The slides from these meetings are attached in Appendix A. The following sections summarize the outcome of those discussions and present the planned experimental configurations and measurements. The stated goals of this experiment are as follows: 1) Measure time-tagged list-mode data for configurations exceeding neutron multiplication of 100; 2) Provide intercomparison between LLNL, LANL, and IRSN detector systems and methodologies; 3) Generate experiment execution report(s) useful to a fundamental physics benchmark for the ICSBEP; 4) Leverage existing critical experiment and detector system benchmarks to limit required modeling and uncertainty analysis.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Relativistic plasma effects and ion acceleration using Scarlet and ELI-NP

High energy density science (HEDS) explores the nature of matter under extreme conditions of temperature and pressure. It has wide ranging fundamental importance from understanding the physical structure of our planet to extreme phenomena in the cosmos. It also has many applications such as facilitating imaging with ions, neutrons, x-rays, gamma rays and more with new applications being developed, including materials processing and medical therapies.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Rheo-Structural Spectroscopy: Fingerprinting the In Situ Response of Fluids to Arbitrary Flow Fields

The objectives of this project were to develop new sample environments, measurement methodologies and associated modeling tools for characterizing the structural response to arbitrarily complex processing flows using small angle scattering, and to apply these new tools for understanding the fundamental physics governing the structuring of anisotropic particulate and polymeric materials under flow histories and conditions relevant to industrial processing flows. The research resulted in the development and implementation of a new sample environment, the fluidic four roll mill (FFoRM), for in situ small angle neutron and X-ray scattering (SANS/SAXS) measurements. These measurements are capable of generating large data sets that “fingerprint” how a complex fluid responds to a wide range of flow histories involving time variations in deformation type and rate. New modeling tools were developed to extract detailed microstructural information from such data sets, including orientation distribution functions and interparticle correlation functions, as well as reduced-order parametric descriptors of these high-dimensional functions that can be used to readily map, visualize and interpret a fluid’s structural response to its flow history. These new tools were applied to a range of model materials involving elongated particle suspensions in order to provide new insights into the physics of how flow couples with orientational and structural order in complex flows, particularly under non-dilute conditions for which no accurate theories currently exist. Using these investigations, we elucidated a number of new insights into the fundamental phenomena driving such process-structure-property relationships. These findings provide guidance for the further development of rheological models, and ultimately can inform the rational and model-based design of flow processes to achieve optimized orientational ordering that is key to the properties and function of a wide range of energy-relevant materials.

36 MATERIALS SCIENCE↗

Capturing dynamical correlations using implicit neural representations

Abstract Understanding the nature and origin of collective excitations in materials is of fundamental importance for unraveling the underlying physics of a many-body system. Excitation spectra are usually obtained by measuring the dynamical structure factor, S ( Q , ω ), using inelastic neutron or x-ray scattering techniques and are analyzed by comparing the experimental results against calculated predictions. We introduce a data-driven analysis tool which leverages ‘neural implicit representations’ that are specifically tailored for handling spectrographic measurements and are able to efficiently obtain unknown parameters from experimental data via automatic differentiation. In this work, we employ linear spin wave theory simulations to train a machine learning platform, enabling precise exchange parameter extraction from inelastic neutron scattering data on the square-lattice spin-1 antiferromagnet La 2 NiO 4 , showcasing a viable pathway towards automatic refinement of advanced models for ordered magnetic systems.

36 MATERIALS SCIENCE↗

Actinides and Neutron Scattering at the Spallation Neutron Source and High Flux Isotope Reactor

The importance of actinides for science, technology, and medicine is widely recognized and does not require a lengthy introduction. However, the fundamental understanding of actinides and their chemical and physical properties lags behind the knowledge of most other elements in the periodic table. Most actinides (89 ≤ Z ≤ 103) are man-made and were produced in particle accelerators or nuclear reactors in the second half of the 20th century. Although trends in bonding and electronic structure are well characterized and documented across the periodic table, fundamental questions remain regarding the chemistry and physics of the actinides. This lack of knowledge is largely because most isotopes of actinides are intensely radioactive, which greatly increases the difficultly in handling them.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Nonequilibrium effects in high-gain inertial confinement fusion

Recent experimental demonstrations of ignition and target gain in inertial confinement fusion (ICF) have stimulated interest in exploring the fundamental physics of violent deuterium-tritium (DT) burn in high-gain ICF targets. A significant DT-burn fraction is a necessary condition for high energy gain and large neutron yields (>100MJ). Using classical molecular-dynamics (MD) simulations and a hybrid fluid-kinetic model, we examine how a large fraction of low-energy 𝛼 particles can kick D and T ions out of equilibrium in high-gain ICF targets. The MD results suggest that (1) temperatures of 𝑇 𝐷 and 𝑇 𝑇 can differ by as much as ∼20% of their mean temperature and (2) the deviation of the DT energy distribution from the Maxwell-Boltzmann function can exceed ∼30%. Some of these MD observations, such as the preferential heating of D ions by low-energy 𝛼 particles and the temperature separation, can be explained by a proposed hybrid fluid-kinetic model. Furthermore, the implication of such nonequilibrium effects on the DT reactivity is also discussed.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

IER 501: Pulsed Neutron Die-Away Experiments at LLNL [Slides]

Pulsed neutron die away experiments occur as follows: (1) a pulse of neutrons is injected into a target material via a D-T neutron generator, (2) neutrons thermalize, (3) neutrons spatially equilibrate, and (4) exponential decay is measured in fundamental mode.

43 PARTICLE ACCELERATORS↗