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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 73 records · Page 4

Benchmarking fast-neutron response of 7 Li-enriched C 7 LYC scintillators: Simulations and experiment

New insights into the fast neutron response of 7 Li-enriched C 7 LYC scintillators have been obtained through detailed Geant4 simulations of 35 Cl(n,p) and 35 Cl(n, α) reactions that are primarily responsible for the fast neutron response of C 7 LYC. The light output of a 1” x1” C 7 LYC detector was simulated using the Birks equation for light quenching in scintillators. The simulations were benchmarked against neutron scattering data from a 12 C target obtained with a white neutron beam at the Los Alamos LANSCE facility and fourteen 1”x1” C 7 LYC detectors. Incident neutron energies extracted from time-of-flight measurements, and appropriate recoil corrections for the different detector angles were used to map the response of C 7 LYC to mono-energetic neutrons. Resonances in the 35 Cl(n,p) reaction cross-section below 3 MeV incident neutron energy were directly observed in C 7 LYC. The experimental data and simulations are compared with ENDF databases, as well as recent direct cross-section measurements of neutrons scattered from a 35 Cl target. In conclusion, the results suggest a scrutiny of the 35 Cl(n,p) and 35 Cl(n, α) cross sections at low energy in the ENDF library.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Large field-of-view event-mode camera for high-precision epithermal neutron resonance imaging

A large-area event-mode camera system coupled with a 6 LiF-ZnS:Ag scintillator is applied for neutron resonance imaging (NRI) on the energy-resolved neutron imaging (ERNI) flight path, also known as Flight Path 5 (FP5), at the Los Alamos Neutron Science Center (LANSCE). This novel neutron imaging system, featuring a 120 x 120 mm 2 field of view, efficiently captures resonance information across the entire image in a single acquisition, significantly reducing beam time requirements compared to conventional energy-resolved neutron imaging systems. High-quality neutron radiographs with enhanced spatial resolution are achieved through the reconstruction of neutron events based on observations of individual photons emitted from the scintillator. The system demonstrates reduced background through neutron/gamma discrimination capabilities while maintaining sharpness across a large fields of view. In the measurements presented here, a spatial resolution of approximately 340 μm was achieved using center-of-gravity photon cluster centroiding. We demonstrate the system’s capability for quantitatively determining isotopic distributions in various thin samples, as well as automatically reconstructing complex scenes with overlapping resonances from diverse samples. These results are obtained using standard data analysis tools, despite the relatively slow 6 LiF-ZnS:Ag scintillator, which may not be optimal for absorption resonance detection. The capabilities demonstrated here offer a valuable, versatile, and cost-effective solution for high spatial and temporal resolution, large field-of-view energy-resolved neutron imaging, with potential applications across various scientific and industrial domains.

36 MATERIALS SCIENCE↗

Energy-resolved neutron imaging and diffraction including grain orientation mapping using event camera technology

Time-of-flight neutron diffraction and energy-resolved imaging each provide unique perspectives into material properties. Neutron diffraction is useful for assessing microstructural parameters such as phase composition, texture, and dislocation densities, though it typically provides averaged data over the sampled volume. Energy-resolved imaging, on the other hand, offers both spatial and spectral information by detecting Bragg edges and neutron absorption resonances, which enables detailed mapping of microstructure and isotopic composition. When combined, these techniques have the potential to enrich our understanding of material behavior across different scales, enhancing our understanding of complex materials. Traditionally, these modalities are conducted on separate instruments, which is time-consuming and poses challenges for data integration. Here, we report the integration of the LumaCam, an event-mode energy-resolved neutron imaging camera with the HIPPO time-of-flight diffractometer at LANSCE. This integration enables simultaneous diffraction and imaging across the full spectrum, with analysis optimized for diffraction and Bragg-edge imaging in the thermal range (0.45–10 Å) and resonance imaging in the epithermal range (0.5–3000 eV), facilitating comprehensive multi-modal analysis. We demonstrate its capabilities through case studies, including spatial mapping of grain orientations in a steel sample and accurate thickness estimations for irregular samples including a depleted uranium cylinder and a natural silver-containing mineral specimen. The combined setup enhances real-time sample alignment and provides comprehensive data for crystal structure, texture, and isotopic composition analysis. This approach opens new possibilities for advanced applications in nuclear engineering, archaeology, and materials science.

36 MATERIALS SCIENCE↗

Nuclear Computational Low Energy Initiative (NUCLEI)

The NUCLEI project, as defined by the scope of work, developed, implemented and run codes for large-scale computations of many topics in low-energy nuclear physics. Physics studied include the properties of nuclei and nuclear decays, nuclear structure and reactions, and the properties of nuclear matter. The computational techniques used include Quantum Monte Carlo, Configuration Interaction, Coupled Cluster, and Density Functional methods. The research program emphasized areas of high interest to current and possible future DOE nuclear physics facilities, including ATLAS and FRIB (nuclear structure and reactions, and nuclear astrophysics), TJNAF (neutron distributions in nuclei, few body systems, and electroweak processes), NIF (thermonuclear reactions), MAJORANA and FNPB (neutrinoless double-beta decay and physics beyond the Standard Model), and LANSCE (fission studies).

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Carbon Block Density

Within the framework of the Neutron Target Demonstrator about 1 m 3 of reactor grade graphite is available at LANSCE. In order to evaluate its suitability as a moderator, knowledge about the exact density is important, since it strongly affects the average time neutrons spend in the volume. The graphite is available in different shapes. A brief analysis was done on three different carbon blocks to determine the density of the material as well as the uncertainty in that measurement.

36 MATERIALS SCIENCE↗

Updated background simulations for DANCE, FP-14

With the installation of the Mark-IV target at LANSCE in 2022 significant changes of the beam-related backgrounds at DANCE are observed. The impact on the count rate at DANCE was discussed and simulated in an earlier report [4]. We report here on simulations, which follow the same general idea as in [4].

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

LAMP Technical Readiness Evaluation Report

An internal preliminary evaluation of Critical Technology Elements (CTEs) for the LANSCE Modernization Project (LAMP) was completed in 2023. This included determining corresponding Technical Readiness Levels (TRLs) for all subsystems using the criteria of DOE G 413.3-4A, Technical Readiness Assessment Guide. This revised report includes a summary of the recent design modifications required to meet the project Key Performance Requirements (KPPs), some of which may reduce technical risk to the project. These recent design modifications include: • Further optimization of the low-energy and medium-energy beam transport regions (LEBT and MEBT, respectively), including relocation of various functional elements (ie choppers, kickers, and bunchers). • An additional H - ion source to separate ion-source function based on beam delivery requirements. • A high-repetition-rate pulsed kicker magnet to select/merge the two H ion beams into a common low-energy beam transport. • Modification and further optimization to a more conventional RFQ design. Performance of the RFQ has been optimized to deliver the required three types of beams while meeting the project KPPs. • The addition of a second chopper in the medium-energy beam transport (MEBT) line to reduce the required pulser voltages. The scope of the evaluation was limited to the project Work Breakdown Structure (WBS) elements as defined for the RFQ Injector and Drift Tube Linac (DTL) systems only. Integration of Instrumentation and Controls (I&C) and Safety Systems was not considered, although specific technologies as related to the RFQ and DTL systems were included. Other elements of the project such as Shielding, System Design, Technical Management, and additional facility integration needed to enable off-line testing and pre-installation commissioning were also not evaluated. Each technical subsystem element was evaluated for technical readiness, however, not all were found to meet the criteria for a CTE. Three subsystem elements were determined to meet the CTE criteria. Their associated TRLs are summarized in the table below. These subsystem elements of the project have the lowest technical readiness due to either being new, novel or modified, requiring additional R&D before being capable of meeting the project Key Performance Parameters (KPPs) and subsystem requirements, or present technology exists but has not yet been demonstrated in a relevant environment. All other subsystems were determined to have a TRL of 8, indicating that actual operating systems exist having similar performance requirements as needed for LAMP. Details of the technical readiness evaluation for each subsystem is given in the following sections of this report.

43 PARTICLE ACCELERATORS↗

LEBT Buncher / Feed Forward / Frequency Generation: System Design Document (SDD)

The LAMP Low Energy Beam Transport (LEBT) transfers a continuous beam at 100 keV from the ion source to RFQ in LEBT. A LEBT buncher imposes an energy tilt to initiate velocy bunching in the chopped beam pulse about 25 ns long to form a short MPEG bunch. One possible option for the LEBT buncher based on a two-gap LC-circuit driven structure was considered, which is similar to the existing LANSCE low-frequncy buncher (LFB). Another possible option is a non-resonant element driven by a pulse-forming-network that provides a single pulse at the repetition frequency of MPEG beam, with a period of 1.8 µs. The LEBT operation is synchronized with the accelerator timing system.

43 PARTICLE ACCELERATORS↗

Preliminary Look at the LBEG & MPEG Beam Transmissions between HPSim and Operation Data

This report summarizes recent work on estimating the transmission of LANSCE H- beams from the end of the present DTL to both the PSR stripper foil (LBEG) and WNR target 4 (MPEG). The LBEG beam might be considered a more typical LINAC beam and lends itself to continuous monitoring of transmission through the various stages of the accelerator. For the MPEG, however, the widely-spaced micropulses and lack of the requisite sensitivity current monitors throughout the accelerator make these measurements extremely difficult and more uncertain. Therefore, to assist in estimating the MPEG beam transmission, beam-dynamics simulations using HPSim were employed. These beam transmission estimates from the end of the Drift Tube Linac (DTL) to Target 4 (MPEG) and the PSR stripper foil (LBEG) are vital to determine the charge requirements for LAMP’s front end. In this technote, we demonstrate three major efforts in determining the transmission: (1) Convert the WNR beamline lattice from TRANSPORT to HPSim for use in the simulation; (2) Simulate the optimization process in the Central Control Room (CCR) that brings down the losses by up to a factor of 4000 between the end of the initial physics-based tuneup phase and production beam operation; (3) Analyze operational data to deduce measured transmissions. Table 1 shows the estimated losses with HPSim and operational analysis. Finally, a better measurement and other improvements to refine the results are also proposed.

43 PARTICLE ACCELERATORS↗

Low-energy H- beam injectors for particle accelerators: upgrade requirements, challenges and future plans [Slides]

High brightness, negative hydrogen ion sources are used extensively in large, accelerator-based, user facilities operating worldwide. Negative hydrogen beams have become the preferred means of filling circular accelerators and storage rings as well as enabling efficient extraction from cyclotrons. Much larger beams of H- ions are also utilized for neutral beams injection into fusion machines and will be discussed in a separate companion presentation. Some of the accelerator facilities include the US Spallation Neutron Source (SNS), Japan Proton Accelerator Research Complex (J-PARC), Rutherford Appleton Laboratory (RAL-ISIS), Los Alamos Neutron Science Center (LANSCE), Fermi National Accelerator Laboratory (FNAL), Brookhaven National Laboratory (BNL), the CERN LHC injector, the Chinese Spallation Neutron Source (CSNS) as well as numerous installations of D-Pace (licenced by TRIUMF) ion sources used mainly with cyclotrons. Many facilities are currently working on various improvement / upgrade projects, both in the near and long term, which are driving further development of their ion source and LEBT (Low Energy Beam Transport) and, in some cases, their overall front end injector system. This report will first provide a simple description of each facilities existing ion source and LEBT and summarize the operational parameters which are currently being routinely injected into their accelerators. Next, the parametric goals of each of the facilities upgrade projects are specified as well as development efforts currently underway to meet these requirement and improvement goals. It is hoped that that this work will not only capture the current state-of-the-art of worldwide H- beam injectors and clarify the research goals and efforts of the community in general but will also encourage further inter laboratory collaborations.

43 PARTICLE ACCELERATORS↗

Dipole Bend Magnets: Design Considerations

This analysis provides a design of a dipole bend magnet for a beamline, stepping through various considerations while assembling a design. This report can be used as a basis of a bending dipole magnet applicable to LANSCE, a scalable point design for other applications, or as a systematic process for developing a magnet design from scratch. The goal is more to answer, 'Is it reasonable?' than to address correction factors. In this specific case, the dipole should provide 3 kG within a 6.35-cm (2.5") gap across an area provided by 25×15-cm pole pieces. This provides roughly 17° and 21° deflection for proton at 3.0 and 2.1 MeV, respectively.

43 PARTICLE ACCELERATORS↗

Temperature of a tungsten spallation target

We discuss the heat load inside a neutron spallation target made of tungsten hit by an 800 MeV proton beam. This problem is important for the Neutron Target project, where a spallation target will be surrounded by an extended graphite or beryllium cube to create a neutron target. The idea of a free-neutron target enables the measurement of neutron-induced reactions in inverse kinematics. This idea is part of the LANSCE strategy to stay a worldwide leader for neutron-induced research.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Record of Decision: H - LEBT Design Modifications

The LAMP Conceptual Design (LCD) is described in the LAMP Conceptual Design Report. The proposed new configuration of the LAMP H - LEBT encompasses multiple changes to the LCD. The new configuration makes use of a single H - source to supply beam to all LANSCE user stations except IPF; this eliminates one of the H - sources in the LCD, and the associated pulsed merger magnet the use of two such sources required. The source current from the sole H - source is gated on a macropulse-by-macropulse basis using techniques demonstrated at SNS (Spallation Neutron Source), specifically, changes to the RF plasma drive power. A pulsed electrode system is used to match the beam into the LEBT transport line, variable on a macropulse-by-macropulse basis to match the source beam current.

43 PARTICLE ACCELERATORS↗

High-Power Amplifier Considerations for testing the LAMP RFQ and first DTL Cavity

As part of the LANSCE Accelerator Modernization Pro ject (LAMP), critical portions of the proposed accelerator will be tested as proof of concept and aid in planning the installation of LAMP at Los Alamos Neutron Science Cen ter. As part of this demonstration, the radio frequency quadrupole (RFQ) and the first drift-tube linac (DTL) cav ity will be tested with beam. For this purpose, high-power RF amplifiers are being designed to meet the testing de mands. This is a description of the requirements of these amplifiers and how the design is intended to meet them.

42 ENGINEERING↗

LAMP Technical Readiness Evaluation Report: LAMP-ENG-RPT-003 (Revision 2)

An internal preliminary evaluation of Critical Technology Elements (CTEs) for the LANSCE Modernization Project (LAMP) was completed in 2023. This included determining corresponding Technical Readiness Levels (TRLs) for all subsystems using the criteria of DOE G 413.3-4A, Technical Readiness Assessment Guide. This revised report includes a summary of the recent design modifications required to meet the project Key Performance Requirements (KPPs), some of which may reduce technical risks to the project. These recent design modifications are based on the LAMP Conceptual Design which is the design evaluated in this document and include: • Further optimization of the low-energy and medium-energy beam transport regions (LEBT and MEBT, respectively), including relocation of various functional elements (i.e. choppers, kickers, and bunchers). • An additional 100-keV H - ion source to separate ion-source function based on beam delivery requirements. • A high-repetition-rate pulsed kicker magnet to select/merge the two H - ion beams into a common low-energy beam transport. • Modification and further optimization to a more conventional 3-MeV Radio Frequency Quadrupole (RFQ) design. Performance of the RFQ has been optimized to deliver the required three types of beams while meeting the project Key Performance Parameters (KPPs). • The addition of a second chopper in the medium-energy beam transport (MEBT) line to reduce the required pulser voltages.

43 PARTICLE ACCELERATORS↗

Examination of the Atomic Pair Distribution Function (PDF) of SiC Nanocrystals by In-situ High Pressure Diffraction

Key properties of nanocrystals are determined by their real atomic structure, therefore a reasonable understanding and meaningful interpretation of their properties requires a realistic model of the structure. In this paper we present an evidence of a complex response of the lattice distances to external pressure indicating a presence of a complex structure of Sic nanopowders. The experiments were performed on nanocrystalline Sic subjected to hydrostatic or isostatic pressure using synchrotron and neutron powder diffraction. Elastic properties of the samples were examined based on X-ray diffraction data using a Diamond Anvil Cell (DAC) in HASYLAB at DESY. The dependence'of the lattice parameters and of the Bragg reflections width with pressure exhibits a ha1 nature of the properties (compressibilities) of the powders and indicates a complex structure of the grains. We interpreted tws behaviour as originating from different elastic properties of the grain interior and surface. Analysis of the dependence of individual interatomic distances on pressure was based on in-situ neutron diffraction measurements done with HbD diffractometer at LANSCE in Los Alamos National Laboratory with the Paris-Edinburgh cell under pressures up to 8 GPa (Qmax = 26/A). Interatomic distances were obtained by PDF analysis using the PDFgetN program. We have found that the interatomic distances undergo a complex, non-monotonic changes. Even under substantial pressures a considerable relaxation of the lattice may take place: some interatomic distances increase with an increase in pressure. We relate this phenomenon to: (1), changes of the microstructure of the densified material, in particular breaking of its fractal chain structure and, (2), its complex structure resembling that of a material composed of two phases, each with its distinct elastic properties.

Grzanka, E.↗

The Status of Cross Section Measurements for Neutron-induced Reactions Needed for Cosmic Ray Studies

Cosmic ray interactions with lunar rocks and meteorites produce small amounts of radionuclides and stable isotopes. Advances in Accelerator Mass Spectrometry (AMS) allow production rates to be measured routinely in well-documented lunar rocks and meteorites. These measurements are analyzed using theoretical models to learn about the object itself and the history of the cosmic rays that fell on it. Good cross section measurements are essential input to the theoretical calculations. Most primary cosmic ray particles are protons so reliable cross sections for proton-induced reactions are essential. A cross section is deemed accurate if measurements made by different experimenters using different techniques result in consistent values. Most cross sections for proton induced reactions are now well measured. However, good cross section measurements for neutron-induced reactions are still needed. These cross sections are required to fully account for all galactic cosmic ray interactions at depth in an extraterrestrial object. When primary galactic cosmic ray (GCR) particles interact with an object many secondary neutrons are produced, which also initiate spallation reactions. Thus, the total GCR contribution to the overall cosmogenic nuclide archive has to include the contribution from the secondary neutron interactions. Few relevant cross section measurements have been reported for neutron-induced reactions at neutron energies greater than approximately 20 MeV. The status of the cross section measurements using quasi-monoenergetic neutron energies at iThemba LABS, South Africa and white neutron beams at Los Alamos Neutron Science Center (LANSCE), Los Alamos are reported here.

Sisterson, J. M.↗