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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 73 records · Page 4

MESOSCALE THERMAL TRANSPORT MEASUREMENTS OF MULTI-PHASE AND POROUS NUCLEAR FUELS USING A SQUARE-WAVE PULSE THERMOREFLECTANCE TECHNIQUE

The safe and efficient operation of nuclear reactors require accurate knowledge of peak temperatures in the fuel assemblies. The temperature profiles are governed by the thermal transport properties of the fuel, namely the thermal conductivities (k) and thermal diffusivities (D). These values can be very difficult to measure as they are known to vary considerably from the measured bulk values of the fresh fuel, and quickly degrade with increasing burnup [1 -3] . Laser-based techniques have been effectively used for non-destructive and non-contact thermal transport measurements of a wide variety of materials, including nuclear materials [4-6] that would otherwise prove too hazardous or difficult to measure otherwise. In this study, a new thermoreflectance technique known as square-pulse transient thermoreflectance (SPTR) is described and used to determine the mesoscale thermal diffusivity of both uranium sesquisilicide (U3Si2) and uranium nitride (UN) phases in a composite fuel with micron level spatial resolution [7]. This technique employs a rapid train of square-wave pulses from an excitation laser to create a periodic heat flux on a gold coated sample surface. Surface adsorption results in transient film temperatures and hence rapid fluctuations in thermoreflectance that can be measured via a detection laser coupled with a digital oscilloscope. The lasers are coaxially focused on the sample surface, allowing for a sample measurement area of a single convolved laser spot size (~2 µm). A sensitivity analysis was conducted to identify key measurement parameters of this technique using reference materials with a range of thermal conductivities comparable to those of both ceramic, composite, and metal nuclear fuel types (1.4 – 27.2 W/m-K). The reference materials were measured using the new technique as well as a spatial-domain thermoreflectance technique (SDTR) previously reported for a comparison [8]. Additionally, measurements of several U3Si2 and UN phase regions of a polished UN/U3Si2 (70/30 vol.%) sample were taken, and the resulting calculated D values are reported, with both techniques showing excellent agreement between samples. This technique was used to scan a multiphase region at 5 micron increments to generate a local diffusivity map, demonstrating the utility of the techniques for measuring thermal transport properties in specimens with precipitates and secondary phases. Furthermore, the technique is currently being applied to measure thermal properties of Fast Flux Test Reactor (FFTR) irradiated metal fuel specimens whose porous microstructure make it very difficult to measure using other techniques. Comparison of the local scale measurements are compared with the pre-irradiated fuel samples to show the degradation of thermal transport in fuels due to pores from fission gas bubbles and other irradiation induced defects.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Laser spot welding of additive manufactured 304L stainless steel

Here, the goal of this work is to understand if an additively manufactured 304L stainless steel exhibits similar spot-welding behavior as wrought 304L stainless steel. Due to the many differences between an additively manufactured component and wrought product, it is important to determine how the material interacts with the laser and how it affects the weld bead morphology. In this paper, the laser coupling efficiency, weld size, and solidification of spot welds produced in wrought and additively manufactured 304L stainless steel were investigated. The coupling efficiency of wrought and additively manufactured 304L stainless steel of similar surface condition were approximately the same over a range of applied laser energies. Laser welding of the untreated (rougher) surface of additively manufactured 304L, however, showed improved coupling efficiency ranging between 3.3 and 100%. The rougher surface traps the incoming light and increases the coupling efficiency at lower laser energies, while at higher energy, the absorption efficiency is dominated by intrinsic absorption from the keyhole formation rather than surface roughness. The resulting spot weld microstructures differed from welds made in wrought 304L and additively manufactured 304L. Welds made in wrought 304L were fully austenitic containing what is suspected to be massive austenite, which suggests that these welds solidified as primary ferrite. Welds made in additively manufactured 304L were also fully austenitic and contained both cellular austenite and what is suspected to be massive austenite. These observations mean that welds made in additively manufactured 304L solidified as primary ferrite and primary austenite. The differences in weld microstructures made in wrought and AM 304L can be attributed to differences in the composition and solidification rate.

304L stainless steel↗

Development and Optical Testing of the Camera, Hand Lens, and Microscope Probe with Scannable Laser Spectroscopy (CHAMP-SLS)

Conducting high resolution field microscopy with coupled laser spectroscopy that can be used to selectively analyze the surface chemistry of individual pixels in a scene is an enabling capability for next generation robotic and manned spaceflight missions, civil, and military applications. In the laboratory, we use a range of imaging and surface preparation tools that provide us with in-focus images, context imaging for identifying features that we want to investigate at high magnification, and surface-optical coupling that allows us to apply optical spectroscopic analysis techniques for analyzing surface chemistry particularly at high magnifications. The camera, hand lens, and microscope probe with scannable laser spectroscopy (CHAMP-SLS) is an imaging/spectroscopy instrument capable of imaging continuously from infinity down to high resolution microscopy (resolution of approx. 1 micron/pixel in a final camera format), the closer CHAMP-SLS is placed to a feature, the higher the resultant magnification. At hand lens to microscopic magnifications, the imaged scene can be selectively interrogated with point spectroscopic techniques such as Raman spectroscopy, microscopic Laser Induced Breakdown Spectroscopy (micro-LIBS), laser ablation mass-spectrometry, Fluorescence spectroscopy, and/or Reflectance spectroscopy. This paper summarizes the optical design, development, and testing of the CHAMP-SLS optics.

Fluorescence↗

Method and apparatus for a multibeam beacon laser assembly for optical communications

An optical beacon is comprised of a telescope having a primary focal plane or Coud? focal plane, a plurality of fiber coupled laser sources for generating a plurality of beams, a collimator for collimating the plurality of beams, and optics for combining and focusing the plurality of collimated beams onto the primary or Coud? focal plane of the telescope. The telescope propagates the optical beacon, which is arranged into a ring of incoherent plurality of collimated beams. The apparatus further comprises fiber splitters coupled to each laser source to provide at least eight beams from at least four laser sources. The optics comprises a prism assembly, a combiner lens, a focusing lens and a field lens for focusing the plurality of collimated beams onto the primary focal plane or Coud? focal plane of the telescope.

Biswas, Abhijit↗

Investigation of heat transport using directly driven gold spheres

Recently, heat transport was investigated using a directly driven beryllium sphere [Farmer et al., Phys. Plasmas 27, 082701 (2020)]. Models that overly restrict heat transport were rejected. This paper extends work to directly driven gold spheres where radiation loss is more important. Here, gold coated spheres are directly driven at the OMEGA laser facility at intensities of 5×10 14 W/cm 2 . Plasma conditions, laser coupling, and x-ray flux are all measured. Additionally, comparisons to 2D radiation-hydrodynamic simulations are performed. Simulations use three common heat transport models: local transport with flux limiters of f = 0.15 and f = 0.03, and the nonlocal Schurtz–Nicolai–Busquet (SNB) model. It is shown that both the SNB model and f = 0.15 match the measured plasma conditions with the SNB model better capturing the temporal evolution of electron temperature. The f = 0.03 model predicts too low of an electron density and too hot of a temperature. The measured scattered light is roughly 6% of the incident energy, the f = 0.15 and SNB models predict 0.5% uncoupled light, and f = 0.03, 38% uncoupled light. The x-ray fluxes in the f = 0.15 and SNB simulations rise too quickly and are just outside the measurement's error, while the x-ray flux in the f = 0.03 simulation is low by a factor of two-three. For these reasons, the f = 0.03 model is rejected.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Development of a US Gravitational Wave Laser System for LISA

A highly stable and robust laser system is a key component of the space-based LISA mission architecture.In this talk I will describe our plans to demonstrate a TRL 5 LISA laser system at Goddard Space Flight Center by 2016.The laser system includes a low-noise oscillator followed by a power amplifier. The oscillator is a low-mass, compact 10mW External Cavity Laser, consisting of a semiconductor laser coupled to an optical cavity, built by the laser vendorRedfern Integrated Optics. The amplifier is a diode-pumped Yb fiber with 2W output, built at Goddard. I will show noiseand reliability data for the full laser system, and describe our plans to reach TRL 5 by 2016.

Development of a US Gravitational Wave↗

Progress and Plans for a US Laser System for LISA

A highly stable and robust laser system is a key component of the space-based LISA (Laser Interferometer Space Antenna) mission architecture. We describe our progress and plans to demonstrate a TRL (Technology Readiness Level) 5 LISA laser system at Goddard Space Flight Center by 2020. The laser system includes a low-noise oscillator followed by a power fiber amplifier. The oscillator is a low-mass, compact external cavity laser, consisting of a semiconductor laser coupled to an optical cavity, built by the laser vendor Redfern Integrated Optics. The amplifier is a diode-pumped Yb fiber with 2.5 watts output, built at Goddard. We show noise and reliability data for the full laser system, and describe our plans to reach TRL 5.

Camp, J.↗

45 Km horizontal path optical link demonstrations

Observations made during a mountain-top-to-mountain-top horizontal optical link demonstration are described. The optical link spans a range of 45 Km at an average altitude of 2 Km above sea level. A multi-beam beacon comprised of eight laser beams emerging from multi-mode fiber coupled lasers (780 nm) are launched through a 0.6 m diameter telescope located at the JPL Table Mountain Facility (TMF) in Wrightwood, California. The multibeam beacon is received at Strawberry Peak located in the San Bernadino Mountains of California. The NASA, JPL developed optical communications demonstrator (OCD) receives the beacon, senses the atmosphere induced motion and using an upgraded fine steering loop compensates the re-transmission of a communications laser beam (852 nm, 400 Mbps) to TMF. The eight-beam beacon allowed a four reduction in normalized irradiance or scintillation index. This in turn was sufficient to eliminate beacon fades sensed b the OCD and allowed the fine steering loop performance evaluation. The uncompensated tracking error was determined to be 2.2 - 3 prad compared to a model prediction of 3.4 prad. The paper also discusses various auxiliary observations made during the campaign

Page, Norman A.↗

Laser Ignition Technology for Bi-Propellant Rocket Engine Applications

The fiber optically coupled laser ignition approach summarized is under consideration for use in igniting bi-propellant rocket thrust chambers. This laser ignition approach is based on a novel dual pulse format capable of effectively increasing laser generated plasma life times up to 1000 % over conventional laser ignition methods. In the dual-pulse format tinder consideration here an initial laser pulse is used to generate a small plasma kernel. A second laser pulse that effectively irradiates the plasma kernel follows this pulse. Energy transfer into the kernel is much more efficient because of its absorption characteristics thereby allowing the kernel to develop into a much more effective ignition source for subsequent combustion processes. In this research effort both single and dual-pulse formats were evaluated in a small testbed rocket thrust chamber. The rocket chamber was designed to evaluate several bipropellant combinations. Optical access to the chamber was provided through small sapphire windows. Test results from gaseous oxygen (GOx) and RP-1 propellants are presented here. Several variables were evaluated during the test program, including spark location, pulse timing, and relative pulse energy. These variables were evaluated in an effort to identify the conditions in which laser ignition of bi-propellants is feasible. Preliminary results and analysis indicate that this laser ignition approach may provide superior ignition performance relative to squib and torch igniters, while simultaneously eliminating some of the logistical issues associated with these systems. Further research focused on enhancing the system robustness, multiplexing, and window durability/cleaning and fiber optic enhancements is in progress.

Thomas, Matthew E.↗

Laser Ignition Technology for Bi-Propellant Rocket Engine Applications

This viewgraph presentation gives an overview of laser ignition technology for bipropellant rocket engines applications. The objectives of this project include: (1) the selection test chambers and flows; (2) definition of the laser ignition setup; (3) pulse format optimization; (4) fiber optic coupled laser ignition system analysis; and (5) chamber integration issues definition. The testing concludes that rocket combustion chamber laser ignition is imminent. Support technologies (multiplexing, window durability/cleaning, and fiber optic durability) are feasible.

Thomas, Matt↗

Autoionizing Polaritons in Attosecond Atomic Ionization

Light-induced states and Autler-Townes splitting of laser-coupled states are common features in the photoionization spectra of laser-dressed atoms. The entangled light-matter character of metastable Autler-Townes multiplets, which makes them autoionizing polaritons, however, is still largely unexplored. We employ attosecond transient-absorption spectroscopy in argon to study the formation of polariton multiplets between the 3s –1 4p and several light-induced states. We measure a controllable stabilization of the polaritons against ionization, in excellent agreement with ab initio theory. Using an extension of the Jaynes-Cummings model to autoionizing states, we show that this stabilization is due to the destructive interference between the Auger decay and the radiative ionization of the polaritonic components. Furthermore, these results give new insights into the optical control of electronic structure in the continuum and unlock the door to applications of radiative stabilization in metastable polyelectronic systems.

74 ATOMIC AND MOLECULAR PHYSICS↗

Terahertz Quantum Cascade Laser With Efficient Coupling and Beam Profile

Quantum cascade lasers (QCLs) are unipolar semiconductor lasers, where the wavelength of emitted radiation is determined by the engineering of quantum states within the conduction band in coupled multiple-quantum-well heterostructures to have the desired energy separation. The recent development of terahertz QCLs has provided a new generation of solid-state sources for radiation in the terahertz frequency range. Terahertz QCLs have been demonstrated from 0.84 to 5.0 THz both in pulsed mode and continuous wave mode (CW mode). The approach employs a resonant-phonon depopulation concept. The metal-metal (MM) waveguide fabrication is performed using Cu-Cu thermo-compression bonding to bond the GaAs/AlGaAs epitaxial layer to a GaAs receptor wafer.

Chattopadhyay, Goutam↗

Roof Polishing of Optical Fibers

Bevealed tip gives optimum coupling efficiency. Abrasive tape used to grind tip of optical fiber. Grinding force depends on stiffness of optical fiber. "Roof" shape on end of optical glass fiber increases efficiency which couples laser light. End surface angle of 65 degrees with perpendicular required for optimum coupling. Since fiber and tape are light in weight and compliant, ridge defect-free, and chipping on fiber edge totally eliminated.

Dholakia, A. R.↗

On the minimization of the prime power consumption of a coupling-modulated gas laser transmitter

The prime power requirements of a coupling-modulated gas laser transmitter are presented. The latter consists of a gas discharge tube and electro-optic modulator inside a laser resonator. In performing the calculations, the laser discharge length and the modulator voltage are simultaneously varied so that the transmitted power remains constant. In this way, tradeoffs can be made between the prime power supplied individually to the discharge tube and to the modulator driver to obtain a transmitter configuration which minimizes the total prime power consumption. An analytical expression is derived which describes the effects of information bandwidth and transmitter output power on the prime power requirements. Specific numerical results are obtained for a CO2 laser transmitter based on presently available experimental data.

Degnan, J. J.↗

Frequency stable high power lasers in space

The concept of a laser heterodyne gravity wave antenna that would operate in solar orbit with a one million kilometer path length is discussed. Laser technology that would be appropriate for operation of this space-based gravity wave detector is also discussed. The rapid progress in diode laser coupled with the energy storage and potentially sub-Hertz linewidths of solid state lasers, and the possibility of efficient frequency conversion by nonlinear optical techniques defines a technology that is appropriate for laser interferometry in space. The present status of diode-laser-pumped, solid state lasers is summarized and future progress is projected in areas of linewidth control, high average power, operating efficiency, and operational lifetimes that are essential for space-based applications.

Byer, Robert L.↗

Laser-induced-fluorescence imaging of a spin-polarized ultracold neutral plasma in a magnetic field

In this work, we report Doppler-sensitive laser-induced-fluorescence (LIF) imaging of an ultracold neutral plasma in a magnetic field. Local values of ion density, hydrodynamic fluid velocity, temperature, and spin polarization are obtained using a fluorescence model based on velocity-resolved rate equations (REs) including the transfer of ions between states due to laser coupling and spontaneous emission. The RE approach captures optical pumping of ions into states that are not driven by the LIF excitation laser, and this is validated with experimental data. Combined molecular-dynamics and quantum-trajectories simulations verify that velocity-changing collisions have a negligible impact on the state population evolution for typical experimental conditions. Relative intensities of Zeeman components of the LIF spectra provide clear evidence that the ions are electron-spin-polarized when created by photoionization of magnetically trapped 88 Sr atoms. This probe opens many possibilities for studying thermal transport and the equilibration of neutral plasmas in overlapping regimes of strong coupling and magnetization.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

How Do You Hear a Quantum Computer Whisper?

Quantum transduction is the process of upconverting microwave quantum signals into optical signals to develop quantum networks through optical fibers outside the dilution refrigerator, enabling connections between quantum technologies on the quantum internet. In this project, upconversion is achieved by directing an optical laser and the microwave quantum signal into an electro-optic bulk crystal. The crystal is housed within a Superconducting Radio Frequency (SRF) cavity designed to maximize the overlap between the microwave field and the crystal volume. In the presence of microwaves, the refractive index of the crystal changes through the Pockels effect. This change in refractive index modifies the propagation of the optical field within the crystal, allowing the quantum information carried by the microwave field to be transferred to the optical field. This study focuses on coupling laser light from suspended waveguide chips into the whispering-gallery modes (WGMs) of the crystal to enable transduction. The coupling efficiency between the optical field in the suspended waveguide and the WGM depends on the position of the laser spot on the crystal. To address this challenge, a feedback-based algorithm is being developed to fine-tune the waveguide position so that the optical signal is coupled efficiently into the crystal. After passing through the crystal, the optical signal is detected by a photodiode connected to an oscilloscope. The algorithm evaluates the coupling quality and iteratively adjusts the waveguide position to maximize coupling efficiency. The expected outcome is an automated waveguide alignment method that improves optical coupling and enables more efficient microwave-to-optical quantum transduction.

Karanastasis, Mihael [Fermilab]↗