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At least 73 records · Page 4

Effect of stratospheric aerosol on ozone profile from BUV measurements

Results of a simulation study on the effects of optically thick stratospheric sulfate aerosol layers on the backscattered ultraviolet radiation (buv) in the range 256-340 nm are presented. In general, the increased Mie scattering produced by the aerosols results in an enhancement of the buv radiation. The increase is approximately linear with optical depth and strongly depends on solar zenith angle and aerosol layer altitude in relation to the ozone maximum. The effect is greatest at those wavelenghts whose contribution functions peak in the vicinity of the densest part of the aerosol layer. The aerosol induced perturbation of the buv field affects the ozone profile retrieval from space measurements by the Solar Backscatter Ultraviolet Experiment (SBUV) experiment. In the tropical stratosphere, the retrieved ozone between 25 and 45 km is underestimated as a result of increased Mie scattering. On the other hand, an algorithm related effect causes the retrieved ozone below 25 km to be overestimated by an amount similar to the stratospheric deficit.

Torres, Omar↗

Parameterizing Single Scattering Properties Across the Electromagnetic Spectrum for Water Cloud Retrieval

Water clouds are composed of spherical water droplets, to which the Mie solution applies for their electromagnetic scattering. The essential variable of Mie solutions is ξ ≡ 𝑚𝑘𝐷 (or equivalently 𝑚𝑘𝑟), where 𝑚 is the complex index of refraction of water, 𝑘 = 2π/λ the angular wavenumber, λ the wavelength, and 𝐷 (𝑟) the diameter (radius) of the water droplet. Consequently, all water-droplet single-scattering properties, such as extinction and scattering efficiencies, i.e., 𝑄 and , are functions of , 𝑒 𝑄𝑠 ξ which provides a convenient pathway to parameterize water-droplet single-scattering properties across the electromagnetic spectrum or spectrum segments. In this paper, we first demonstrate that the numerical Mie solution indeed depends only on ξ. We then present our first attempt to parameterize extinction efficiency across the visible-infrared spectrum.

Kwo-Sen Kuo↗

Time and polarization dependent double scattering calculations of lidar returns from water clouds

We describe and present results of a double scattering lidar model which we use to calculate lidar returns from water clouds. The model is used in conjunction with the Phillips Laboratory's (Geophysics Directorate) low altitude Nd:YAG lidar system to determine microphysical properties of water clouds. The model determines the Stokes parameters of the backscattered lidar radiation, from media composed of spherical particles, as a function of time. The Stokes parameters of the radiation of the lidar return are determined, at each time, by considering all radiation which has traveled the same path length from transmitter to receiver while making two successive single scatters. Each single scatter is considered a Mie scatter. We have also developed a Mie scattering program for use with the double scattering model. Each single scatter takes into account the polarization of the incident and scattered radiation. Inputs to the double scattering mode include the receiver area and field of view, the receiver integration time, the extinction coefficient as a function of distance into the cloud, the particle size distribution (assumed independent of position), and the complex index of refraction of the spherical particles.

Garner, R. C.↗

Experimental Determination of Infrared Extinction Coefficients of Interplanetary Dust Particles

This technique is based on irradiating a single isolated charged dust particle suspended in balance by an electric field, and measuring the scattered radiation as a function of angle. The observed scattered intensity profile at a specific wavelength obtained for a dust particle of known composition is compared with Mie theory calculations, and the variable parameters relating to the particle size and complex refractive index are adjusted for a best fit between the two profiles. This leads to a simultaneous determination of the particle radius, the complex refractive index, and the scattering and extinction coefficients. The results of these experiments can be utilized to examine the IRAS and DIRBE (Diffuse Infrared Background Experiment) infrared data sets in order to determine the dust particle physical characteristics and distributions by using infrared models and inversion techniques. This technique may also be employed for investigation of the rotational bursting phenomena whereby large size cosmic and interplanetary particles are believed to fragment into smaller dust particles.

Spann, J. F., Jr.↗

Implementation of A New Microwave Scattering Database and A Forward Model for Active Microwave Sensors in CRTM

Radiative transfer models are extensively used for the assimilation of satellite observations into NWP models as well as retrieving geophysical products from satellite measurements. CRTM is a community model developed by NOAA JCSDA and widely used for different purposes requiring RT calculations. CRTM requires bulk scattering lookup tables in order to perform all-sky RT calculations. However, the current CRTM lookup tables for microwave frequencies were generated based on the Mie theory by assuming spherical frozen particles. The scattering lookup tables generated using the DDA technique has shown to largely improve the RT scattering calculations in the MW region. This presentation targets (i) the implementation and validation of a DDA database that was originally developed for the ARTS RT model into CRTM, and (ii) developing the CRTM active sensor module that takes advantage of the backscattering coefficients computed using the DDA method. The DDA database only provides single scattering properties of different habits, while CRTM requires bulk scattering properties. The CRTM cloud coefficients were previously generated based on the effective radius for representing the size of the particles. However, effective radius is neither measurable nor provided by the NWP models, thus need to be estimated from other geophysical variables such as water content. Therefore, in addition to calculating the CRTM bulk scattering properties from the DDA single scattering database, the CRTM was also largely modified to use cloud water content (kg.m-3), instead of effective radius, for performing the interpolation over size/mass of the particles. CRTM already requires water content as input, thus no extra variables are required for performing scattering calculations using the new ARTS DDA database. The CRTM scattering modules search for effective radius in cloud coefficient files and will use the cloud water content if the effective radius dimension is not found in the cloud coefficient files. Figure 1 shows the CRTM simulated brightness temperatures computed using different cloud coefficients versus ATMS observed values over Hurricane Irma on September 7, 2017 at 18:00 UTC. We used all the cloud water content values included in ERA5 with default CRTM/DDA habits for water, rain, snow, ice, hail, and graupel. ERA5 does not provide separate water content values for ice, hail, and graupel, thus the ice water content values were divided between ice, hail, and graupel clouds similar to what was explained in the previous section. In channels with a frequency lower than 90 GHz, emission from water and rain clouds can compensate for cloud scattering so that cloud contaminated Tbs are larger than corresponding clear sky Tbs. The DDA simulations for channels 1-7 largely perform better than the Mie simulations. The DDA simulations show a mix of small negative and positive simulated minus observed values, while the Mie results show large negative biases. The weighting functions for some of the ATMS temperature sounding channels (channels 9-15) peak mostly above the clouds, therefore the measured Tbs become less sensitive to clouds so that the results of both Mie and DDA become very similar. The Mie lookup tables generate excessive scattering for channel 16, but not enough scattering for the water vapor channels. In the specific case of Hurricane Maria, the DDA lookup tables do not generate enough scattering for channel 16, but the DDA results are much more consistent with observations for water vapor channels than for channel 16. It should be noted that the results may vary if we use other habits to represent snow, hail, and graupel in the DDA simulations. Although these results clearly show the advantage of the DDA database over the Mie dataset, different error sources such as error in the observations, displacement of clouds in the ERA5 reanalysis, and also lack of convective clouds or in general errors in the input atmospheric and cloud profiles contribute to the differences between the simulated and observed values. Aside from the improvements in the simulations, a major advantage of the new dataset is a large number of habits that can be used to tune the data assimilation systems to perform well in different weather conditions.

Isaac Moradi↗

Cloud Liquid Water, Mean Droplet Radius and Number Density Measurements Using a Raman Lidar

A new technique for measuring cloud liquid water, mean droplet radius and droplet number density is outlined. The technique is based on simultaneously measuring Raman and Mie scattering from cloud liquid droplets using a Raman lidar. Laboratory experiments on liquid micro-spheres have shown that the intensity of Raman scattering is proportional to the amount of liquid present in the spheres. This fact is used as a constraint on calculated Mie intensity assuming a gamma function particle size distribution. The resulting retrieval technique is shown to give stable solutions with no false minima. It is tested using Raman lidar data where the liquid water signal was seen as an enhancement to the water vapor signal. The general relationship of retrieved average radius and number density is consistent with traditional cloud physics models. Sensitivity to the assumed maximum cloud liquid water amount and the water vapor mixing ratio calibration are tested. Improvements to the technique are suggested.

Whiteman, David N.↗

Forwardscattering corrections for optical extinction measurements in aerosol media. I - Monodispersions

A parametric investigation of forwardscattering corrections applicable to experimentally determined optical extinction coefficients in homogeneous aerosol media is discussed for the case of monodispersion. Assuming forwardscattering to be a single-scattering phenomenon, corrections are made by two methods: one employing the exact Mie theory, the other employing the approximate Rayleigh diffraction formula. The corrections are evaluated as functions of particle size, the real and imaginary parts of the complex refractive index, and the half-angle of the detector view cone.

Deepak, A.↗

Fresnel diffraction by spherical obstacles

Lommel functions were used to solve the Fresnel-Kirchhoff diffraction integral for the case of a spherical obstacle. Comparisons were made between Fresnel diffraction theory and Mie scattering theory. Fresnel theory is then compared to experimental data. Experiment and theory typically deviated from one another by less than 10 percent. A unique experimental setup using mercury spheres suspended in a viscous fluid significantly reduced optical noise. The major source of error was due to the Gaussian-shaped laser beam.

Hovenac, Edward A.↗

Light scattering by lunar-like particle size distributions

A fundamental input to models of light scattering from planetary regoliths is the mean phase function of the regolith particles. Using the known size distribution for typical lunar soils, the mean phase function and mean linear polarization for a regolith volume element of spherical particles of any composition were calculated from Mie theory. The two contour plots given here summarize the changes in the mean phase function and linear polarization with changes in the real part of the complex index of refraction, n - ik, for k equals 0.01, the visible wavelength 0.55 micrometers, and the particle size distribution of the typical mature lunar soil 72141. A second figure is a similar index-phase surface, except with k equals 0.1. The index-phase surfaces from this survey are a first order description of scattering by lunar-like regoliths of spherical particles of arbitrary composition. They form the basis of functions that span a large range of parameter-space.

Goguen, Jay D.↗

Size distribution and scattering phase function of aerosol particles retrieved from sky brightness measurements

Ground-based measurements of the solar transmission and sky radiance in a horizontal plane through the Sun are taken in several geographical regions and aerosol types: dust in a desert transition zone in Israel, sulfate particles in Eastern and Western Europe, tropical aerosol in Brazil, and mixed continental/maritime aerosol in California. Stratospheric aerosol was introduced after the eruption of Mount Pinatubo in June 1991. Therefore measurements taken before the eruption are used to analyze the properties of tropospheric aerosol; measurements from 1992 are also used to detect the particle size and concentration of stratospheric aerosol. The measurements are used to retrieve the size distribution and the scattering phase function at large scattering angles of the undisturbed aerosol particles. The retrieved properties represent an average on the entire atmospheric column. A comparison between the retrieved phase function for a scattering angle of 120 deg, with phase function predicted from the retrieved size distribution, is used to test the assumption of particle homogeneity and sphericity in radiative transfer models (Mie theory). The effect was found to be small (20% +/- 15%). For the stratospheric aerosol (sulfates), as expected, the phase function was very well predicted using the Mie theory. A model with a power law distribution, based on the spectral dependence of the optical thickness, alpha, cannot estimate accurately the phase function (up to 50% error for lambda = 0.87 microns). Before the Pinatubo eruption the ratio between the volumes of sulfate and coarse particles was very well correlated with alpha. The Pinatubo stratospheric aerosol destroyed this correlation. The aerosol optical properties are compared with analysis of the size, shape, and composition of the individual particles by electron microscopy of in situ samples. The measured volume size distribution before the injection of stratospheric aerosol consistently show two modes, sulfate particles with r(sub m) less than 0.2 microns and coarse paritcles with r(sub m) greater than 0.7 microns. The 'window' in the tropospheric aerosol in this radius range was used to observe a stable stratospheric aerosol in 1992, with r(sub m) approximately 0.5 microns. A combination of such optical thickness and sky measurements can be used to assess the direct forcing and the climatic impact of aerosol. Systematic inversion for the key aerosol types (sulfates, smoke, dust, and maritime aerosol) of the size distribution and phase function can give the relationship between the aerosol physical and optical properties that can be used to compute the radiative forcing. This forcing can be validated in dedicated field experiments.

Kaufman, Y. J.↗

Plasmon Resonances of Metal Nanoparticles in an Absorbing Medium

We study the behavior of plasmon resonances of metal nanospheres embedded in an absorbing medium. First-principles far-field computations based on the general Lorenz–Mie theory show that increasing absorption in the host medium broadens and suppresses plasmon resonances in the extinction and effective scattering efficiency factors and suppresses resonance features in the phase function. These effects of absorption are analogous to those on the morphology-dependent resonances of dielectric particles with large size parameters.

Mishchenko, Michael I.↗

On the mean particle size and water content of polar mesospheric clouds

Results from the ultraviolet spectrometer experiment (UVS) aboard the Solar Mesospheric Explorer, which measures ultraviolet sunlight scattered from air molecules in the mesosphere, are reported and discussed. The UVS experiment, its observing modes, and details of the observing sequence are described. The data are compared with predictions of Mie scattering theory, assuming the size distribution is parameterized by a mean radius and a width parameter. The water ice content, mean particle radius, and column number are calculated as a function of cloud brightness, and in terms of the unknown width parameter. It is concluded that polar mesospheric cloud particles are quite small, having average volume-effective radii less than 70 mm, and that clouds differ in their optical properties mainly as a result of their mean particle size.

Thomas, G. E.↗

Characterization of Surface Reflectance Variation Effects on Remote Sensing

The use of Monte Carlo radiative transfer codes to simulate the effects on remote sensing in visible and infrared wavelengths of variables which affect classification is examined. These variables include detector viewing angle, atmospheric aerosol size distribution, aerosol vertical and horizontal distribution (e.g., finite clouds), the form of the bidirectional ground reflectance function, and horizontal variability of reflectance type and reflectivity (albedo). These simulations are used to characterize the sensitivity of observables (intensity and polarization) to variations in the underlying physical parameters both to improve algorithms for the removal of atmospheric effects and to identify techniques which can improve classification accuracy. It was necessary to revise and validate the simulation codes (CTRANS, ARTRAN, and the Mie scattering code) to improve efficiency and accommodate a new operational environment, and to build the basic software tools for acquisition and off-line manipulation of simulation results. Initial calculations compare cases in which increasing amounts of aerosol are shifted into the stratosphere, maintaining a constant optical depth. In the case of moderate aerosol optical depth, the effect on the spread function is to scale it linearly as would be expected from a single scattering model. Varying the viewing angle appears to provide the same qualitative effect as modifying the vertical optical depth (for Lambertian ground reflectance).

Pearce, W. A.↗

Experimental investigation of crossflow jet mixing in a rectangular duct

An experimental investigation of the mixing of nonreacting opposed rows of jets injected normal to a confined rectangular crossflow has been conducted. Planar Mie-scattering was used to measure the time-average concentration distribution of the jet fluid in planes perpendicular to the duct axis. The mixing effectiveness of round orifice injectors was measured as a function of orifice spacing and orifice diameter. Mixing effectiveness was determined using a spatial unmixedness parameter based on the variance of mean jet concentration distributions. Optimum mixing was obtained when the spacing-to-duct height ratio was inversely proportional to the square root of the jet-to-mainstream momentum-flux ratio. For opposed rows of round holes with centerlines inline, mixing was similar for blockages up to 75 percent. Lower levels of unmixedness were obtained as a function of downstream location when axial injection length was minimized. Mixing may be enhanced if orifice centerlines of opposed rows are staggered, but note that blockage must be less than 50 percent for this configuration.

Liscinsky, D. S.↗

Experimental investigation of crossflow jet mixing in a rectangular duct

An experimental investigation of the mixing of nonreacting opposed rows of jets injected normal to a confined rectangular crossflow has been conducted. Planar Mie-scattering was used to measure the time-average concentration distribution of the jet fluid in planes perpendicular to the duct axis. The mixing effectiveness of round orifice injectors was measured as a function of orifice spacing and orifice diameter. Mixing effectiveness was determined using a spatial unmixedness parameter based on the variance of mean jet concentration distributions. Optimum mixing was obtained when the spacing-to-duct height ratio was inversely proportional to the square root of the jet-to-mainstream momentum-flux ratio. For opposed rows of round holes with centerlines inline, mixing was similar for blockages up to 75 percent. Lower levels of unmixedness were obtained as a function of downstream location when axial injection length was minimized. Mixing may be enhanced if orifice centerlines of opposed rows are staggered, but note that blockage must be less than 50 percent for this configuration.

Liscinsky, D. S.↗

Scattering by nonspherical particles of size comparable to wavelength - A new semi-empirical theory and its application to tropospheric aerosols

A semiempirical theory is developed which is based on simple physical principles and comparisons with laboratory measurements. The ultimate utility of this approach rests on its ability to successfully reproduce the observed single-scattering phase function for a wide variety of particle shapes, sizes and refractive indices. This approximate theory is developed for evaluating the interaction of randomly oriented, nonspherical particles with the total intensity component of electromagnetic radiation. Mie theory is used when the particle size parameter x (ratio of particle circumference to wavelength) is less than some upper bound x sub zero (about 5). For x greater than x sub zero, the interaction is divided into three components: diffraction, external reflection and transmission. The application of the theory is illustrated by considering the influence of the shape of tropospheric aerosols on their contribution to the earth's global albedo.

Pollack, J. B.↗

Experimental study of cross flow mixing in cylindrical and rectangular ducts

An experimental investigation of non-reacting cross flow jet injection and mixing in cylindrical and rectangular ducts has been conducted with application to a low emissions combustor. Quantitative measurement of injectant concentration distributions perpendicular to the duct axis were obtained by planar digital imaging of the Mie-scattered light from an aerosol seed mixed with the injectant. The flowfield unmixedness was evaluated using (1) a mixing parameter derived from the ratio of the jet concentration fluctuations to the fully mixed concentration, and (2) probability density functions of the concentration distributions. Mixing rate was measured for 45 degree slant slot and round orifice injectors.

Liscinsky, D. S.↗

Far-field Lorenz-Mie Scattering in an Absorbing Host Medium. II: Improved Stability of the Numerical Algorithm

A recently developed FORTRAN program computing far-field optical observables for spherical particles in an absorbing medium has exhibited numerical instability arising when the product of the particle vacuum size parameter and the imaginary part of the refractive index of the host becomes sufficiently large. We offer a simple analytical explanation of this instability and propose a compact numerical algorithm for the stable computation of Lorenz–Mie coefficients based on an upward recursion formula for spherical Hankel functions of a complex argument. Extensive tests confirm an excellent accuracy of this algorithm approaching machine precision. The improved public-domain FORTRAN program is available at https://www.giss.nasa.gov/staff/mmishchenko/Lorenz-Mie.html.

Lorenz-Mie theory↗