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At least 73 records · Page 4

Effective gravitational couplings of four-dimensional $ \mathcal{N} $ = 2 supersymmetric gauge theories

The low energy effective couplings of a four-dimensional N = 2 supersymmetric gauge theory to topological invariants of the background gravitational field are described by two functions A and B. These two functions play an important role in the study of topologically twisted four-dimensional N = 2 supersymmetric gauge theories and in the computation of central charges of N = 2 superconformal theories. In this paper, we compute A and B from the partition function in the Ω-background for SU(2) gauge theories. Our results not only confirm the predicted expressions of the effective gravitational couplings, but also give the previously undetermined overall multiplicative factors. We also analyze A and B for the SU(N) super-Yang-Mills theory, and confirm all the previous predictions.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Muon g -2 from millicharged hidden confining sector

We provide a novel explanation to the muon g - 2 excess with new physics contributions at the two-loop level. In this scenario, light millicharged particles are introduced to modify the photon vacuum polarization that contributes to muon g - 2 at one additional loop. The muon g - 2 excess can be explained with the millicharged particle mass m χ around 10 MeV and the product of the multiplicity factor and millicharge squared of N χ ε 2 ~ 10 -3 . The minimal model faces severe constraints from direct searches at fixed-target experiments and astrophysical observables. However, if the millicharged particles are also charged under a hidden confining gauge group SU(N χ ) with a confinement scale of MeV, hidden-sector hadrons are unstable and can decay into neutrinos, which makes this scenario consistent with existing constraints. This explanation can be well tested at low-energy lepton colliders such as BESIII and Belle II as well as other proposed fixed-target experiments.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Strategies for thorium fuel cycle transition in the SD-TMSR

Liquid-fueled Molten Salt Reactor (MSR) systems represent advances in safety, economics, and sustainability. The MSR has been designed to operate with a Th/ 233 U fuel cycle with 233 U used as startup fissile material. Since 233 U does not exist in nature, we must examine other available fissile materials to start up these reactor concepts. This work investigates the fuel cycle and neutronics performance of the Single-fluid Double-zone Thorium-based Molten Salt Reactor (SD-TMSR) with different fissile material loadings at startup: High Assay Low Enriched Uranium (HALEU) (19.79%), Pu mixed with HALEU (19.79%), reactor-grade Pu (a mixture of Pu isotopes chemically extracted from Pressurized Water Reactor (PWR) spent nuclear fuel (SNF) with 33 GW d/tHM burnup), transuranic elements (TRU) from Light Water Reactor (LWR) SNF, and 233 U. The MSR burnup routine provided by SERPENT-2 is used to simulate the online reprocessing and refueling in the SD-TMSR. The effective multiplication factor, fuel salt composition evolution, and net production of 233 U are studied in the present work. Additionally, the neutron spectrum shift during the reactor operation is calculated. The results show that the continuous flow of reactorgrade Pu helps transition to the thorium fuel cycle within a relatively short time (≈ 4.5 years) compared to 26 years for 233 U startup fuel. Finally, using TRU as the initial fuel materials offers the possibility of operating the SD-TMSR for an extended period of time (≈ 40 years) without any external feed of 233 U.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Progress on the reevaluation and validation of the n+233U neutron cross sections

The set of 233 U resonance parameters of the ENDF/B-VIII.0 nuclear data library was adopted from the previous ENDF/B-VII.1 evaluation using the external levels to update the thermal values. Adoption of IAEA 2017 thermal standards ( σ f = 533.0 ± 2.2 b, σ c = 44.9 ± 0.9 b, and ν ‾ tot = 2.487 ± 0.011 ) and of the IAEA-recommended thermal-neutron induced prompt fission neutron spectrum (PFNS) with average PFNS energy of 2.030 ± 0.013 MeV requires a re-evaluation of 233 U neutron cross sections in the resolved resonance region. A newly produced evaluation is being tested on benchmarks carefully selected from the Handbook of International Criticality Safety Benchmark Experiments (ICSBEP) which are highly sensitive to 233 U data. An important goal of this work was to eliminate the strong negative gradient of the calculated effective multiplication factors with respect to the epithermal fission fraction observed in the validation of the ENDF/B-VIII.0 library for those assemblies. A significant improvement in integral performance of critical 233 U solutions is observed for the newly proposed evaluation. Further work addressing the fast neutron region is needed.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Total thermal neutron cross section measurements of yttrium hydride from 0.0005 - 3 eV

Yttrium hydride serves as a neutron moderator material that enables compact, high temperature nuclear reactors. However, in order to accurately design and simulate a nuclear system relying upon yttrium hydride, the fundamental nuclear data of yttrium hydride must be well understood. Thermal neutron scattering law (TSL) evaluations represent an important aspect of nuclear data as thermal scattering can drastically alter the neutron multiplication factor of a system. Therefore, to support evaluation and validation of thermal neutron scattering for yttrium hydride, researchers at Rensselaer Polytechnic Institute (RPI) performed total thermal neutron cross section measurements for YH 1.68 and YH 1.85 over the energy range of 0.0005 - 3 eV. Further, these measurements represent the first total cross section measurements for yttrium hydride that encompass the entire thermal region. Comparisons were made against the ENDF-B/VIII.0, Zerkle & Holmes and Oak Ridge National Laboratory TSL evaluations, where generally good agreement was found.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Utilization of ACE nuclear data file toolkit ACEtk to calculate relative sensitivity coefficients of point-kinetics parameters

Sensitivity and uncertainty methods are quintessential for nuclear criticality safety and experiment design. This type of analysis relies on calculations of sensitivity coefficients; sensitivity coefficients of the effective neutron multiplication factor with respect to some nuclear data are predominantly calculated and used. As a part of the Laboratory Directed Research & Development project EUCLID (Experiments Underpinned by Computational Learning for Improvements in nuclear Data) at Los Alamos National Laboratory, sensitivity coefficients of many radiation detector measurement responses with respect to nuclear data were investigated. Specifically, this paper outlines a method to calculate point-kinetics parameters relative sensitivity coefficients with respect to nuclear data. Point-kinetics parameters such as the prompt neutron decay constant, effective delayed neutron fraction, and neutron generation time are especially important to experimenters and reactor operators designing systems with dynamic neutron populations. This method couples capabilities of the ACE (A Compact ENDF) nuclear data file toolkit, ACEtk, with the ability to load cross sections into the radiation transport code Monte Carlo N-Particle (MCNP). In conclusion, key aspects of optimizing this method for a particular application and sensitivity profiles of the Jezebel criticality experiment are examined and discussed.

98 NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL P↗

Development of a Griffin model of the advanced test reactor

In the pursuit of a higher fidelity deterministic simulation capability of the Advanced Test Reactor, it is important to have a fast yet accurate deterministic neutronics model. Here, to achieve this, we employed an advanced two-step method. The first step involves generating homogenized cross sections using OpenMC, a cutting-edge Monte Carlo neutron transport code. OpenMC offers excellent modular capabilities, allowing for easy component integration and flexibility in incorporating new designs into the model. The second step involves deterministic transport calculations, which are performed using Griffin, a reactor physics application based on the Multiphysics Object-Oriented Simulation Environment (MOOSE). To ensure the accurate spatial resolution and assignment of material cross sections, a Cubit-generated mesh for the Advanced Test Reactor is utilized as an intermediate step between the OpenMC and Griffin models; Griffin utilizes the mesh for its finite element solution, while OpenMC material identifications are written to the mesh file to be used in Griffin material assignments. Additionally, a Python-based script converts the cross sections generated by OpenMC into the ISOXML format required by Griffin. Initial comparisons using the Griffin diffusion solver indicated good agreement between the neutron multiplication factors obtained from the standalone OpenMC model and the Griffin model, with differences of less than 10 pcm in the 2D geometry configuration; it was later determined that this agreement was likely due to compensating effect and was more likely on the order of –700 pcm relative to the OpenMC solution. However, in three-dimensional calculations, an unacceptably large error (almost 8,000 pcm) was found in the Griffin solution with the diffusion solver. Subsequent calculations using Griffin’s discrete ordinates solver demonstrated substantially improved agreement, within 116 pcm of the OpenMC solution used to generate the cross sections for Griffin. Building on this capability, future work will seek to perform more detailed validation calculations. The ultimate goal is to evaluate both transient and multiphysics simulations of the reactor.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Multizonal modeling of SARS-CoV-2 aerosol dispersion in a virtual office building

The dispersion of indoor airborne contaminants across different zones within a mechanically ventilated building is a complex phenomenon driven by multiple factors. In this study, we modeled the indoor dispersion of airborne SARS-CoV-2 aerosols within a US Department of Energy detailed medium office prototype building using CONTAM software. The aim of this study is to improve our understanding about how different parts of a building can experience varying concentrations of the airborne viruses under different circumstances of release and mitigation strategies. Results indicate that unventilated stairwells can have significantly higher concentrations of airborne viruses. The mitigation strategies of morning and evening flushing of conditioned zones were not found to be very effective. Instead, a constant high percentage of outdoor air in the supply mix, and the use of masks, portable HEPA air cleaners, MERV 13 or higher HVAC air filters, and ultraviolet germicidal irradiation disinfection were effective strategies to prevent airborne viral contamination in the majority of the simulated office building.

60 APPLIED LIFE SCIENCES↗

Porosity in nuclear graphite and its impact on nuclear reactor science and criticality safety applications

Porosity in nuclear-grade graphite significantly influences its low-energy neutron scattering, yet its effect on underlying phonon properties remains debated. Here, this work integrates inelastic and small-angle neutron scattering (INS/SANS) experiments, advanced atomistic simulations with a novel machine-learned potential (DeepMD), total cross-section measurements, and neutronics calculations (SCALE, MCNP, OpenMC) to investigate porosity’s impact on neutron thermalization. INS measurements on diverse graphite grades reveal no discernible porosity effect on phonon spectra, which align with crystalline graphite. Conversely, total cross-section data below ≈10 meV show increased scattering attributable to SANS. Our DeepMD simulations demonstrate that realistic micropores do not distort phonon spectra, challenging the assumptions in current ENDF/B-VIII.1 porosity thermal scattering laws (TSLs). These TSLs, based on random atom removal, produce unphysical phonon spectra and inflate inelastic cross-sections. Augmenting a crystalline TSL with an SANS component accurately captures experimental total cross-sections. Neutronics benchmarks (ICSBEP/IRPhE) show ENDF porosity TSLs unphysically increase neutron multiplication factor, keff. Crucially, incorporating SANS physics (NCrystal/OpenMC) indicates accurately modeled porosity negligibly affects keff, reactor physics, or criticality safety.

Critical benchmarks↗

Systematic Evaluation of Atmospheric Forcing, Surface Datasets, and Mesh Effects on Kilometer-Scale Land Surface and River Modeling

Earth system models are advancing toward kilometer-scale resolution to capture local climate impacts and extremes. High-resolution land and river modeling depends on multiple factors, including mesh, surface datasets, and atmospheric forcing, but their relative effects at kilometer scales remain unquantified. We evaluated five Energy Exascale Earth System Model land and river configurations over the Mid-Atlantic region using two mesh (1/8° structured versus variable-resolution unstructured mesh), two surface datasets (default versus newly developed), and three atmospheric forcings (NLDAS2, MSWX, GSWP). Evaluation against satellite, reanalysis, and in situ benchmarks across water, energy, and carbon cycles quantifies how these factors affect model performance. Forcing selection produces the largest bias reductions (12-99% across variables), followed by surface datasets (7-75%) and mesh (up to 21%). Forcing effects vary by variable, with MSWX reducing biases for snow water equivalent, evapotranspiration, albedo, temperature, and gross primary productivity, GSWP for snow cover and runoff, and NLDAS for soil moisture and streamflow. The use of newly developed surface datasets improves gross primary productivity (58% bias reduction) and evapotranspiration but increase soil moisture and albedo biases due to current modeling limitations. Variable-resolution unstructured mesh improves the simulation of small-basin streamflow through better capturing drainage networks, though mesh minimally affects other land variables. These findings provide important guidance for high-resolution modeling development and actionable science.

Land and River modeling↗

Applying a Template of Expected Uncertainties to Updating 239 Pu(n,f) Cross-section Covariances in the Neutron Data Standards Database

Templates of uncertainties expected in specific measurement types were recently developed. One aim of these templates is to help evaluators in identifying (1) missing or suspiciously low uncertainties and (2) missing correlations between uncertainties of the same and different experiments, when estimating covariances for experimental data employed in their evaluations. These templates also provide realistic estimates of standard deviations and correlations for a particular uncertainty source and measurement type that can be used by evaluators in situations where they are not supplied by the experimenters. This information allows for a more comprehensive uncertainty analysis across all measurements considered in an evaluation and, thus, more realistic evaluated covariances. Here, in this work, we extend a template that is applicable to uncertainties expected in neutron-induced fission, (n,f), cross-section measurements. It is applied to improving covariances of 239 Pu(n,f) cross-section measurements in the database underlying the Neutron Data Standards evaluations. This particular example was chosen since this evaluation is primarily based on experimental information. Also, some uncertainties of individual 239 Pu(n,f) cross-section experiments in this database were suspected to be underestimated. The evaluated uncertainties obtained after updating the covariances in the database by means of the template indeed do increase compared to their original values. Even more importantly, the evaluated mean values change noticeably. These modified cross sections impact application calculations significantly, as is demonstrated by employing them in simulations of the effective neutron multiplication factor for a few selected critical assemblies. However, this updated evaluated 239 Pu(n,f) cross section should not be interpreted as the final one that should replace values of the current Neutron Data Standards project. Evaluations for the Neutron Data Standards of the 239 Pu(n,f) cross section must be linked to many other observables included in the associated database, most notably to cross sections for 235 U(n,f), but also to those for 10 B(n, α ), 6 Li(n,t), 238 U(n,f), and 238 U(n, γ ), because of included measurements of the 239 Pu(n,f) cross section that appear as ratios to these reactions. Some of these other reactions are correlated to further observables in the database. Hence, updating uncertainties of data sets of any of these observables can potentially impact the 239 Pu(n,f) cross section. Uncertainties for all measurements of these linked physical observables have to be updated before a comprehensive evaluation of the 239 Pu(n,f) cross section and its corresponding uncertainties can be provided.

239Pu Neutron-induced fission cross-section↗

Enhancing nuclear data validation analysis by using machine learning

In this work, we demonstrate how machine learning (ML) techniques can be used as an auxiliary tool for nuclear data validation analysis. The output of the ML analysis can inform evaluators and validators on the quality, or lack thereof, of specific nuclear data and benchmark experiments with respect to simulating these experimental benchmark values. To this end, measured and simulated effective neutron multiplication factors, k eff , of 875 selected ICSBEP critical assemblies and the latter's sensitivities with respect to nuclear data as well as benchmarks' features (e.g., material nuclide, core geometry) are used as input for a random forest (RF) regression model. The RF is used to encode the complex inter-dependencies between thousands of nuclear data features (i.e., sensitivity profiles and aspects describing the measurements) and 875 simulated and experimental k eff values in order to understand what nuclear data features are most informative for predicting bias. The complexity of relationships and high-dimensional space is difficult-to-impossible to search fully using simply expert judgment. As a first proof-of-concept—step, it is demonstrated that this technique is able to correctly trace large discrepancies between simulated and experimental k eff back to fabricated shortcomings in nuclear data that were perturbed to simulated k eff values. In a second, real-case scenario, step, the RF algorithm is used to validate the ENDF/B-VIII.0 library in comparison to ENDF/B-VII.1 nuclear data. One case is showcased where the chosen ML algorithms highlighted nuclear data (the 19 F(n,inl) cross section from 0.4–0.9 MeV) that are shown to be problematic by comparing them to associated differential experimental data and nuclear data from other libraries. In addition to that, it is shown that the RF results point towards poor benchmark experiments and associated underestimated uncertainties (e.g., the PU-SOL-THERM-028 series). However, using the RF algorithm for validating nuclear data with respect to k eff is currently limited to pinpointing groups of questionable nuclear data due to the inherent correlations between features introduced by the nuclear data themselves and how k eff is simulated. Due to this, we recommend that the ML methods presented be used to augment—rather than replace—the expert knowledge of evaluators and validators.

96 KNOWLEDGE MANAGEMENT AND PRESERVATION↗

Rossi-alpha measurements of fast plutonium metal assemblies using organic scintillators

The reactivity and the k-effective multiplication factor (k eff ) of a fissionable assembly are quantities of widespread interest. These values can be inferred from Rossi-alpha measurements of the prompt neutron decay constant (or the inverse:α -1 ). It has been shown that 3 He-gas proportional counter-based detection systems are insensitive to α -1 of fast assemblies (much faster than tens of microseconds). Therefore, it is of interest to investigate fast detection systems such as those based on organic scintillation detectors. In this work, an array of 12 cylindrical, 5.08 cm x 5.08 cm diameter trans-stilbene organic scintillators was used to measure five subcritical assemblies. One assembly was a sphere of approximately 4.5 kg of alpha-phase, weapons-grade plutonium (k eff = 0.773, α -1 = 11.84 ns) known as the BeRP ball encased in a thin stainless-steel clad. The other assemblies used the same encased sphere and 7.62 cm of iron, nickel, copper, or tungsten reflectors (k eff = 0.884, 0.916, 0.924, 0.939, respectively and α -1 = 36.60, 41.56, 49.60, 70.32 ns, respectively). Finally, this work (1) validates Rossi-alpha measurements with organic scintillators by demonstrating good agreement between measurements and simulations; and (2), demonstrates that organic scintillator-based systems are sensitive to α -1 on the order of 10–100 ns.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Validation of the two-region Rossi-alpha model for reflected assemblies

Nuclear criticality safety, nonproliferation and safeguards, emergency response, and stockpile stewardship utilize estimates of the k eff multiplication factor. The value of k eff cannot be directly measured, but it can be inferred from the prompt neutron period. One modality of measuring the prompt neutron period is the Rossi-alpha method, which is predicated on fitting a histogram of detection time differences due to the nonrandom temporal distribution of same-fission-chain neutrons. Recent works have developed the motivation and theory to expand traditional one-region point kinetic models resulting in one-exponential histogram fits to two-region models that result in two-exponential fits. This paper validates the new two-region model using organic scintillator measurements of copper-reflected weapons-grade plutonium (0:83 ≤ k eff ≤ 0:94) and high-density- polyethylene-reflected highly enriched uranium (0:73 ≤ k eff ≤ 0:95). Furthermore, the results show that more thermal systems have shorter prompt neutron periods in the core region due to increased induced-fission probabilities for moderated neutrons. Here, a new parameter introduced by the two- region model is also shown to be correlated to the amount of reflection, and may be used to infer assembly properties such as type and amount of reflector.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Nuclear data uncertainty propagation applied to the versatile test reactor conceptual design

We report the Versatile Test Reactor (VTR) currently under development is a 300 MWth sodium-cooled fast reactor (SFR) fueled with ternary metal alloy fuel, which aims to accelerate the testing of advanced nuclear fuels, materials, instrumentation, and sensors in high flux environments that are necessary to license the next generation of advanced reactor concepts. To support the VTR design process, uncertainties associated with the nuclear data has been propagated through the reactor core neutronics calculation to global parameters of interest, such as the core multiplication factor, kinetic parameters, and various reactivity feedback coefficients, following the sensitivity based uncertainty propagation approach. By folding the sensitivity coefficients, separately computed by the generalized perturbation theory code PERSENT and Monte Carlo code Serpent 2, with the variance-covariance matrices from COMMARA-2.0, we obtain the reaction-wise, isotope-wise, and overall uncertainties for each response of interest due to nuclear data uncertainty. With Serpent 2, the statistical error of the uncertainty is obtained by propagating the statistical error of the sensitivity coefficients through the same process using a newly developed uncertainty propagation method. From both codes, the overall top uncertainty contributors are found to be the cross section of Fe-56 elastic scattering, Na-23 elastic scattering, and U 238 inelastic scattering. The large contributions of the Fe-56 elastic scattering cross sections to global parameters are due to its relatively large relative uncertainty of 5–10% in nuclear data and the large volume of Fe-containing reflector assemblies in the fairly compact VTR core design. Both codes agreed well for the overall uncertainty estimates of all responses of interest, except the delayed neutron fraction, prompt neutron generation time, and the coolant density feedback coefficient, where Serpent 2 yielded a much larger value than PERSENT due to the large statistical error of sensitivity coefficients. The calculated uncertainties are also compared to those associated with other SFR cores. Another outcome of this study is a variance-covariance matrix of reactivity coefficients, which can be used in the subsequent uncertainty propagation to the system level to investigate the impact of identified uncertainties on system responses in the safety analysis.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Evaluation of the spatial self-shielding impact for TRISO-based nuclear fuel depletion

Reactor physics analyses of nuclear cores with nuclear fuel concepts containing tristructural isotropic (TRISO) particles, such as pebbles or compact fuel elements, rely on various degrees of simplification to keep these highly heterogeneous problems computationally tractable. One such limitation regards the level of spatial discretization employed during burnup calculations, where traditionally only a limited number of spatial zones are modeled at the full core level and assume that the spectrum is constant within the fuel elements and TRISO particles in this depletion zone. This type of assumption neglects the impact of spatial self-shielding effect within the kernels (microscale level) as well as within the compact or pebbles (mesoscale level). Furthermore, the Monte Carlo code Serpent 2 contains many relevant features for efficiently modeling this type of geometry, including a collision-based domain decomposition intended for very large burnup calculations, which we leveraged for this work to quantify the impact of capturing neutron flux variations occurring at the micro- and mesoscale level on a series of high-temperature gas-cooled reactor fuel element depletion problems. While spatial self-shielding is observed at both scales, with differences from a volume-averaged burnup of ±7% within the kernels and ±2% between TRISO particles within the fuel element, the conjugated effect on nuclide inventories and multiplication factor are negligible, hence confirming that assuming a single average spectrum value may be sufficient for most applications.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗