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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 73 records · Page 4
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NASA NTRS1996

Regulation of Methane Oxidation in a Freshwater Wetland by Water Table Changes and Anoxia

The effects of water table fluctuations and anoxia on methane emission and methane oxidation were studied in a freshwater marsh. Seasonal aerobic methane oxidation rates varied between 15% and 76% of the potential diffusive methane flux (diffusive flux in the absence of aerobic oxidation). On an annual basis, approximately 43% of the methane diffusing into the oxic zone was oxidized before reaching the atmosphere. The highest methane oxidation was observed when the water table was below the peat surface. This was confirmed in laboratory experiments where short-term decreases in water table levels increased methane oxidation but also net methane emission. Although methane emission was generally not observed during the winter, stems of soft rush (Juncus effusus) emitted methane when the marsh was ice covered. Indigenous methanotrophic bacteria from the wetiand studied were relatively anoxia tolerant. Surface peat incubated under anoxic conditions maintained 30% of the initial methane oxidation capacity after 32 days of anoxia. Methanotrophs from anoxic peat initiated aerobic methane oxidation relatively quickly after oxygen addition (1-7 hours). These results were supported by culture experiments with the methanotroph Methylosinus trichosporium OB3b. This organism maintained a greater capacity for aerobic methane oxidation when starved under anoxic compared to oxic conditions. Anoxic incubation of M. trichosporium OB3b in the presence of sulfide (2 mM) and a low redox potential (-110 mV) did not decrease the capacity for methane oxidation relative to anoxic cultures incubated without sulfide. The results suggest that aerobic methane oxidation was a major regulator of seasonal methane emission front the investigated wetland. The observed water table fluctuations affected net methane oxidation presumably due to associated changes in oxygen gradients. However, changes from oxic to anoxic conditions in situ had relatively little effect on survival of the methanotrophic bacteria and thus on methane oxidation potential per se.

Roslev, Peter↗
NASA NTRS1990

The effects of fire on biogenic emissions of methane and nitric oxide from wetlands

Enhanced emissions of methane (CH4) and nitric oxide (NO) were measured following three controlled burns in a Florida wetlands in 1987 and 1988. Wetlands are the major global source of methane resulting from metabolic activity of methanogenic bacteria. Methanogens require carbon dioxide, acetate, or formate for their growth and the metabolic production of methane. All three water-soluble compounds are produced in large concentrations during biomass burning. Postfire methane emissions exceeded 0.15 g CH 4/sq m per day. Preburn and postburn measurements of soil nutrients indicate significant postburn increases in soil ammonium, from 8.35 to 13.49 parts per million (ppm) in the upper 5 cm of the Juncus marsh and from 8.83 to 23.75 ppm in the upper 5 cm of the Spartina marsh. Soil nitrate concentrations were found to decrease in both marshes after the fire. These measurements indicate that the combustion products of biomass burning exert an important 'fertilizing' effect on the biosphere and on the biogenic production of environmentally significant atmospheric gases.

Levine, Joel S.↗
NASA NTRS2020

Assessment of Lidar XCH4 Measurements During ACT-America 2019 for Boundary Layer Methane and Emission Model Constraint

Atmospheric methane is a potent and abundant greenhouse gas (GHG) with increasing importance due to rising emissions and their subsequent impact on radiative forcing, indicating an important driving role in climate change. The recent Earth Science Decadal Survey called for further understanding of the sources and sinks of atmospheric methane, the processes that will affect their future concentrations, and identified the need for advanced observing capabilities to elucidate these issues. HALO, a combined methane Differential Absorption Lidar and Aerosol/Cloud High Spectral Resolution Lidar participated in the ACT-America summer 2019 campaign to help constrain the emissions and transport of GHGs in the atmosphere to address some of the aforementioned science goals. In this presentation we will discuss the utility of using an in-situ point measurement versus lidar column measurement for inventory and source identification applications. Comparisons between column measurements of methane from in-situ and lidar will be made to assess whether point measurements are useful when the assumption of a well-mixed boundary layer, a practice commonly used in the community, is valid. We will also show that a lidar column measurement can apportion boundary layer methane from the column and has the ability to identify boundary layer methane enhancements in fair weather conditions using atmospheric backscatter signals, a measurement capability that has the potential to transform the observational strategies of future airborne carbon cycle science investigations. We will also present on the differences and utility of constraining emission models using an in-situ versus lidar column and asses the resulting uncertainties of each.

Rory A Barton-Grimley↗
NASA NTRS2014

Retrieval of Methane Source Strengths in Europe Using a Simple Modeling Approach to Assess the Potential of Spaceborne Lidar Observations

We investigate the sensitivity of future spaceborne lidar measurements to changes in surface methane emissions. We use surface methane observations from nine European ground stations and a Lagrangian transport model to infer surface methane emissions for 2010. Our inversion shows the strongest emissions from the Netherlands, the coal mines in Upper Silesia, Poland, and wetlands in southern Finland. The simulated methane surface concentrations capture at least half of the daily variability in the observations, suggesting that the transport model is correctly simulating the regional transport pathways over Europe. With this tool we can test whether proposed methane lidar instruments will be sensitive to changes in surface emissions. We show that future lidar instruments should be able to detect a 50% reduction in methane emissions from the Netherlands and Germany, at least during summer.

surface fluxes↗
NASA NTRS2022

Wetland Emission and Atmospheric Sink Changes Explain Methane Growth in 2020

Atmospheric methane growth reached an exceptionally high rate of 15.1 ± 0.4 parts per billion per year in 2020 despite a probable decrease in anthropogenic methane emissions during COVID-19 lockdowns(1). Here we quantify changes in methane sources and in its atmospheric sink in 2020 compared with 2019. We find that, globally, total anthropogenic emissions decreased by 1.2 ± 0.1 teragrams of methane per year (Tg CH4 yr−1), fire emissions decreased by 6.5 ± 0.1 Tg CH4 yr−1 and wetland emissions increased by 6.0 ± 2.3 Tg CH4 yr−1. Tropospheric OH concentration decreased by 1.6 ± 0.2 per cent relative to 2019, mainly as a result of lower anthropogenic nitrogen oxide (NOx) emissions and associated lower free tropospheric ozone during pandemic lockdowns(2). From atmospheric inversions, we also infer that global net emissions increased by 6.9 ± 2.1 Tg CH4 yr−1 in 2020 relative to 2019, and global methane removal from reaction with OH decreased by 7.5 ± 0.8 Tg CH4 yr−1. Therefore, we attribute the methane growth rate anomaly in 2020 relative to 2019 to lower OH sink (53 ± 10 per cent) and higher natural emissions (47 ± 16 per cent), mostly from wetlands. In line with previous findings(3,4,) our results imply that wetland methane emissions are sensitive to a warmer and wetter climate and could act as a positive feedback mechanism in the future. Our study also suggests that nitrogen oxide emission trends need to be taken into account when implementing the global anthropogenic methane emissions reduction pledge(5).

Shushi Peng↗
NASA NTRS2018

GES DISC Long-Term Data Analysis Services Using AIRS and CMS Methane Data as an Example

NASA Goddard Earth Sciences Data and Information Services Center (GES DISC) archives and distributes rich collections of data on atmospheric greenhouse gases from multiple satellite missions and model results. Among those greenhouse gases, atmospheric methane is a powerful greenhouse gas contributing ~0.5 (W/m^2) to total radiative forcing, and its concentration has increased by about 150% since 1750. Observations or estimates of methane emissions typically have sparse spatial and temporal coverage. The lack of comprehensive spatial and temporal coverage of methane source and sink observations has made analyzing atmospheric methane trends challenging. In this study the GES DISC aims to provide the community with the resources to better understand changes in atmospheric methane concentrations and the underlying causes. We will utilize methane datasets from Atmospheric Infrared Sounder (AIRS) retrieved methane concentration and three Carbon Monitoring System (CMS) methane emission datasets (in regions of North America, Canada, and Mexico) to compare AIRS methane growth with corresponding CMS regional methane emissions. Comparisons of AIRS methane growth rates and CMS methane emissions suggests wetland emissions may impact methane growth rate trends over North America. As the record for CMS methane data is extended, both datasets can be used in conjunction to better understand impacts on atmospheric methane trends. GES DISCs new anomaly tool can also be used on select datasets to further quantify trends in atmospheric greenhouse gases.

long-term data analysis↗