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At least 73 records · Page 4

SAM 2 measurements of the polar stratospheric aerosol, volume 2

The Stratospheric Aerosol Measurement (SAM) 2 sensor aboard Nimbus 7 is providing extinction measurements of Antarctic and Arctic stratospheric aerosols with a vertical resolution of 1 km. Representative examples and weekly averages including corresponding temperature profiles provided by NOAA for the time and place of each SAM 2 measurement (Oct. 1981 - Apr. 1982) are presented. Contours of aerosol extinction as a function of altitude and longitude or time are plotted, and aerosol optical depths are calculated for each week. Typical values of aerosol extinction at 1.0 micron in the main lower stratospheric aerosol layer for this time period are 2 to 4 times 10 to the -4 power/km. for the Antarctic region and 0.5 to 1 times 10 to the -3 power/km. for the Arctic region. Stratospheric optical depths are about 0.001 to 0.004 for the Antarctic region and 0.003 to 0.004 at the beginning to about 0.006 at the end of the time period for the Arctic region. Polar stratospheric clouds (PSC's) were observed during the Arctic winter, as expected. This report provides, in a ready-to-use format, a representative sample of the seventh semester of data to be used in atmospheric and climatic studies.

Mccormick, M. P.↗

Radiative Forcing From the 2014–2022 Volcanic and Wildfire Injections

Abstract Volcanic and wildfire events between 2014 and 2022 injected ∼3.2 Tg of sulfur dioxide and 0.8 Tg of smoke aerosols into the stratosphere. With injections at higher altitudes and lower latitudes, the simulated stratospheric lifetime of the 2014–2022 injections is about 50% longer than the volcanic 2005–2013 injections. The simulated global mean effective radiative forcing (ERF) of 2014–2022 is −0.18 W m −2 , ∼40% of the ERF of the period of 1991–1999 with a large‐magnitude volcanic eruption (Pinatubo). Our climate model suggests that the stratospheric smoke aerosols generate ∼60% more negative ERF than volcanic sulfate per unit aerosol optical depth. Studies that fail to account for the different radiative properties of wildfire smoke relative to volcanic sulfate will likely underestimate the negative stratospheric forcings. Our analysis suggests that stratospheric injections offset 20% of the increase in global mean surface temperature between 2014–2022 and 1999–2002.

54 ENVIRONMENTAL SCIENCES↗

Understanding Model-Observation Discrepancies in Satellite Retrievals of Atmospheric Temperature Using GISS ModelE

We examine multiple factors in the representation of satellite-retrieved atmospheric temperature diagnostics in historical simulations of climate change during the satellite era (specifically 1979–2021) using GISS ModelE contributions to the Coupled Model Intercomparison Project (Phase 6) (CMIP6). The tropospheric and stratospheric trends in these diagnostics are affected by greenhouse gases (notably carbon dioxide and ozone), coupling with the ocean, volcanic aerosols, solar activity and compositional and dynamic feedbacks. We explore the impacts of internal variability, changing forcing specifications, composition interactivity, the quality of the stratospheric circulation, vertical resolution, and possible impacts of the mis-specification of volcanic aerosol optical depths. Overall temperature trends throughout the satellite period are well captured, but discrepancies at all levels exist and have multiple distinct causes. We find that stratospheric comparisons (using Stratospheric Sounding Unit (SSU) retrievals and successor instruments) are most affected by variations in the representation of ozone depletion and feedbacks, followed by the volcanic signals. Tropospheric skill (using the Microwave Sounding Unit (MSU) retrievals) is affected by the trends in ocean heat uptake and tropospheric aerosols, but also by the representation of stratospheric processes through the impact of the Brewer-Dobson circulation on the height of the tropical tropopause. We demonstrate that no single factor is the dominant cause of the discrepancies and that almost all observations lie within the broad envelope of structural uncertainty.

satellite retrievals of atmospheric temperature↗

Global distribution of stratospheric aerosols by satellite measurements

A description is given of the first-ever global stratospheric aerosol climatology which is being developed by the earth-orbiting SAM II and SAGE satellite-based sensors. These sensors use the technique of solar occulation; that is, for every spacecraft sunrise and sunset, the modulation of solar intensity caused by the intervening earth-limb is measured. These data are mathematically inverted to yield vertical profiles of aerosol extinction coefficients with 1 km resolution. The data show seasonal variations which are similar in each hemisphere, with strong correlation between aerosol extinction and the corresponding temperature field. Typical values of extinction in the stratosphere are found to be about 0.0001 to 0.0002 per km at 1 micrometer; stratospheric optical depths at this wavelength are about 0.002. The peak extinction in the stratospheric aerosol layer follows the tropopause with altitude, with peak extinction ratios about 10 km above the local tropopause.

Mccormick, M. P.↗

SAM 2 measurements of the polar stratospheric aerosol, volume 8

The Stratospheric Aerosol Measurement (SAM) 2 sensor aboard Nimbus 7 is providing extinction measurements of Antarctic and Arctic stratospheric aerosols with a vertical resolution of 1 km. Representative examples and weekly averages including corresponding temperature profiles provided by NOAA for the time and place of each SAM 2 measurement (Apr. 1982 - Oct. 1982) are presented. Contours of aerosol extinction as a function of altitude and longitude or time are plotted, and aerosol optical depths are calculated for each week. Typical values of aerosol extinction at 1.0 microns in the main stratospheric aerosol layer are approximately 4 to 6 times .0001/km at the beginning to 1 to 2 times .001/km at the end of the time period for the Antarctic region and approximately 1 to 3 times .001/km for the Arctic region throughout the time period. Stratospheric optical depths are about 0.002 to 0.009 for the Antarctic region and about 0.007 at the beginning to 0.024 at the end of the time period for the Arctic region. Polar stratospheric clouds were observed during the Antarctic winter, as expected. This report provides, in a ready-to-use format, a representative sample of the eighth 6 months of data to be used in atmospheric and climatic studies.

Mccormick, M. P.↗

Utilization of SAGE aerosol profiles in the analysis of Mauna Loa stratospheric lidar data

A systematic approach to analyzing lidar data collected at NOAA's Mauna Loa Observatory (MLO) was developed which relies on parameters derived from SAGE satellite extinction profile measurements to verify boundary conditions applied to analysis. The approach also provides a means of assessing the uncertainties associated with the various inputs, so that the accuracy of the analysis of the MLO lidar data is available. The stratosphere during the 1980 to 1981 period was only mildly perturbed and could be easily represented by the SAMII/SAGE background aerosol model. The MLO lidar observations collected during this period provided stratospheric optical depths with uncertainties ranging between 15% and 25%. Uncertainties in the aerosol optical model contribute errors of 3% to 4% in the computed optical depths. Most of the optical depth uncertainty is associated with the calibration assumption in which no marked improvement can be expected.

Fernald, F. G.↗

Planetary Spectroscopy

The goal of this task is to acquire physical data on the atmospheres of the outer planets and Titan by means of ground-based spectroscopy, spectrophotometry, and spectral imaging at visible to near-infrared wavelengths (approximately 0.3 to 2.5 micrometer). These data constrain physical parameters which characterize properties and distribution of aerosols in the atmospheres of these bodies. Reduced spectral imaging of Neptune was accomplished. The data were analyzed in several ways. Direct inspection of images reveals the distribution of discrete clouds in the atmosphere, which indicate that the global distribution of clouds has changed since earlier imaging. Disk-integrated photometry obtained from the images demonstrates that the diurnal variability at methane-band wavelengths is caused by the presence of discrete clouds; short-term variability is also seen in the rotational light curve, providing evidence for modification of cloud structure on the planet. The center-to-limb brightness profiles of the equatorial region of Neptune were analyzed, which provided constraints on the location, albedos, and optical depths of aerosol scattering layers in the troposphere and lower stratosphere.

Bergstralh, Jay T.↗

Reevaluation of Stratospheric Ozone Trends From SAGE II Data Using a Simultaneous Temporal and Spatial Analysis

This paper details a new method of regression for sparsely sampled data sets for use with time-series analysis, in particular the Stratospheric Aerosol and Gas Experiment (SAGE) II ozone data set. Non-uniform spatial, temporal, and diurnal sampling present in the data set result in biased values for the long-term trend if not accounted for. This new method is performed close to the native resolution of measurements and is a simultaneous temporal and spatial analysis that accounts for potential diurnal ozone variation. Results show biases, introduced by the way data is prepared for use with traditional methods, can be as high as 10%. Derived long-term changes show declines in ozone similar to other studies but very different trends in the presumed recovery period, with differences up to 2% per decade. The regression model allows for a variable turnaround time and reveals a hemispheric asymmetry in derived trends in the middle to upper stratosphere. Similar methodology is also applied to SAGE II aerosol optical depth data to create a new volcanic proxy that covers the SAGE II mission period. Ultimately this technique may be extensible towards the inclusion of multiple data sets without the need for homogenization.

Damadeo, R. P.↗

Major Optical Depth Perturbations to the Stratosphere from Volcanic Eruptions: Stellar-Extinction Period, 1961-1978

A revised chronology of stratospheric aerosol extinction due to volcanic eruptions has been assembled for the period 1961-1978, which immediately precedes the era of dedicated satellite measurements. On the whole, the most accurate data consist of published observations of stellar extinction, supplemented in part by other kinds of observational data. The period covered encompasses the important eruptions of Agung (1963) and Fuego (1974), whose dust veils are discussed with respect to their transport, decay, and total mass. The effective (area-weighted mean) radii of the aerosols for both eruptions are found to be 0.3-0.4 microns. It is confirmed that, among known tropical eruptions, Agung's dust was unique for a low-latitude eruption in remaining almost entirely confined to the hemisphere of its production. A new table of homogeneous visual optical depth perturbations, listed by year and by hemisphere, is provided for the whole period 1881-1978, including the pyrheliometric period before 1961 that was investigated previously.

Stothers, Richard B.↗

Inverse Modeling of the Initial Stage of the 1991 Pinatubo Volcanic Cloud Accounting for Radiative Feedback of Volcanic Ash

The way volcanic clouds evolve is very sensitive to the initial spatial 3D distributions of volcanic materials, which are often unknown. In this study, we conducted inverse modeling of the Mt. Pinatubo cloud using TOMS 2D mapping of Aerosol Index and SO 2 loading during the first three post-eruption days to estimate the time-dependent emissions profiles and initial 3D spatial distributions of volcanic ash and SO 2 . We account for aerosol radiative feedback and dynamic lofting of volcanic ash in the inversion calculations for the first time. This resulted in a lower ash injection height (by 1.5 km for ash) than without ash radiative feedback. The Pinatubo eruption ejected ≈77% of fine ash at 12 to 23 km, ≈65% of SO 2 at 18–25 km. In contrast with previous studies, which suggested that all volcanic materials were emitted above the tropopause, a significant fraction of SO 2 (5.1 of 15.5 Mt) and fine ash (37.2 of 66.5 Mt) were ejected in the troposphere, where SO 2 quickly oxidized into sulfate aerosol that is short-lived in the troposphere. This explains the early presence of sulfate aerosols in the plume and why the models can reproduce the observed volcanic aerosols' optical depth (AOD), assuming lower-than-observed SO 2 emission in the stratosphere. Despite the quicker than in observations build-up of sulfate AOD, in a month after the eruption, the evolution of the Pinatubo AOD simulated using the obtained ash and SO 2 initial distributions converges with the available stratospheric aerosol and gas experiment (SAGE) observations.

Pinatubo volcanic ash and SO2 emissions↗

Latitudinal variation of spectral optical thickness and columnar size distribution of the El Chichon stratospheric aerosol layer

Measurements are presented for the spectral optical thickness of El Chichon's stratospheric aerosol layer, obtained during an airborne latitudinal survey in April and May of 1983. Columnar aerosol size distributions of the stratosphere are derived by inverting the aerosol optical thickness measurements as a function of wavelength and from spectral aerosol depth measurements obtained during an airborne survey in October and November 1982. Spectral optical thickness data and the derived size distributions from both airborne missions show latitidunal regions with similar characteristics. Airborne solar radiometer measurements are shown to be useful in studies of the latitudinal variations of optical and related particle size characteristics of the stratospheric aerosol layer.

Spinhirne, J. D.↗

Physical processes in polar stratospheric ice clouds

A one dimensional model of cloud microphysics was used to simulate the formation and evolution of polar stratospheric ice clouds. Some of the processes which are included in the model are outlined. It is found that the clouds must undergo preferential nucleation upon the existing aerosols just as do tropospheric cirrus clouds. Therefore, there is an energy barrier between stratospheric nitric acid particles and ice particles implying that nitric acid does not form a continuous set of solutions between the trihydrate and ice. The Kelvin barrier is not significant in controlling the rate of formation of ice particles. It was found that the cloud properties are sensitive to the rate at which the air parcels cool. In wave clouds, with cooling rates of hundreds of degrees per day, most of the existing aerosols nucleate and become ice particles. Such clouds have particles with sizes on the order of a few microns, optical depths on order of unity and are probably not efficient at removing materials from the stratosphere. In clouds which form with cooling rates of a few degrees per day or less, only a small fraction of the aerosols become cloud particles. In such clouds the particle radius is larger than 10 microns, the optical depths are low and water vapor is efficiently removed. Seasonal simulations show that the lowest water vapor mixing ratio is determined by the lowest temperature reached, and that the time when clouds disappear is controlled by the time when temperatures begin to rise above the minimum values.

Toon, Owen B.↗

Stratospheric aerosols

The current state of information on stratospheric aerosols is reviewed. Aerosol properties such as size, size distribution, composition, refractive index, number density, extinction, optical depth, and single scattering albedo are considered and generalized as much as possible to be representative of the global aerosol in times of volcanic and nonvolcanic (background) periods. Data are presented that show the global distribution of stratospheric aerosols as measured by the stratospheric aerosol and gas experiment (SAGE) satellite system for background and volcanic (post-Mount St. Helens) conditions. In addition, lidar and dustsonde data are presented that show the changes in stratospheric aerosol over an 8-year period.

Mccormick, M. P.↗

Polar stratospheric optical depth observed between 1978 and 1985

Observations of the stratospheric optical depth at 1.0 micron obtained for high latitudes are presented for a 7-year period. Weekly averaged data determined from measurements made by the Stratospheric Aerosol Measurement experiment from October 1978-1985 show that the overall yearly values in both polar regions are controlled by volcanic perturbations, with most volcanic effects being experienced in Arctic latitudes. Conservatively, peak values found in the Antarctic region were approximately 0.02 and in the Arctic region about 0.55. Probable values for these regions are estimated to be 0.26 and 0.11, respectively. The weekly averaged data also show the seasonal fluctuations due to microphysical and dynamical processes. Comparison of the optical depth record with a weekly averaged 50-mbar temperature record indicates that polar stratospheric clouds are present in the southern high latitudes each year near this level from early June to early September. A depression observed in the optical depth record each austral spring season is believed to be the result of the downward displacement of particles caused by subsidence and sedimentation during the course of winter. Following the breakup of the vortex, optical depth values increase as aerosol is transported poleward. These features are noted to be present in the Arctic region as well, but on a smaller scale because of the satellite sampling methodology and the averaging scheme employed.

Mccormick, M. P.↗

Comparisons of satellite ozone data in the lower stratosphere for 1978/1979

Lower stratospheric zonal mean O3 distributions are compared in both hemispheres from the Nimbus 7 Solar Backscattered Ultraviolet (SBUV) and Limb Infrared Monitor of the Stratosphere (LIMS) data sets. Generally there is very good agreement with regard to individual profile shape and magnitude and with their longitudinal variability about the zonal mean. When the data are considered in terms of Umkehr layer amounts, there are subtle but significant differences in the respective meridional O3 gradients and their variations with time which are probably related to a changing O3 optical depth and constants to an assumed profile climatology in the retrieval. Stratospheric Aerosol and Gas Experiment (SAGE) satellite O3 results are presented which tend to split the differences between SBUV and LIMS. Additional comparisons with electrochemical concentration cell sonde and Mastsonde O3 profiles are presented in order to sort out the more noticeable differences.

Remsberg, Ellis E.↗

Aerosol Optical Depth Measurements by Airborne Sun Photometer in SOLVE II: Comparisons to SAGE III, POAM III and Airborne Spectrometer Measurements

The 14-channel NASA Ames Airborne Tracking Sunphotometer (AATS-14) measured solar-beam transmission on the NASA DC-8 during the Second SAGE III Ozone Loss and Validation Experiment (SOLVE II). This paper presents AATS-14 results for multiwavelength aerosol optical depth (AOD), including its spatial structure and comparisons to results from two satellite sensors and another DC-8 instrument. These are the Stratospheric Aerosol and Gas Experiment III (SAGE III), the Polar Ozone and Aerosol Measurement III (POAM III) and the Direct beam Irradiance Airborne Spectrometer (DIAS).

Russell, P.↗

High-Latitude Stratospheric Aerosol Geoengineering Can Be More Effective if Injection Is Limited to Spring

Stratospheric aerosol geoengineering focused on the Arctic could substantially reduce local and worldwide impacts of anthropogenic global warming. Because the Arctic receives little sunlight during the winter, stratospheric aerosols present in the winter at high latitudes have little impact on the climate, whereas stratospheric aerosols present during the summer achieve larger changes in radiative forcing. Injecting SO 2 in the spring leads to peak aerosol optical depth (AOD) in the summer. We demonstrate that spring injection produces approximately twice as much summer AOD as year-round injection and restores approximately twice as much September sea ice, resulting in less increase in stratospheric sulfur burden, stratospheric heating, and stratospheric ozone depletion per unit of sea ice restored. Furthermore, we also find that differences in AOD between different seasonal injection strategies are small compared to the difference between annual and spring injection.

58 GEOSCIENCES↗

Toba volcano super eruption destroyed the ozone layer and caused a human population bottleneck

Volcanic eruptions trigger a broad spectrum of climatic responses. For example, the Mount Pinatubo eruption in 1991 forced an El Niño and global cooling, and the Tambora eruption in 1815 caused the "Year Without a Summer." Especially grand eruptions such as Toba around 74,000 years ago can push the Earth's climate into a volcanic winter state, significantly lowering the surface temperature and precipitation globally. Here we present a new, previously overlooked element of the volcanic effects spectrum: the radiative mechanism of stratospheric ozone depletion. We found that the volcanic plume of Toba enhanced the UV optical depth and suppressed the primary formation of stratospheric ozone from O2 photolysis. Sulfate aerosols additionally reflect the photons needed to break the O2 bond (λ < 242 nm), otherwise controlled by ozone absorption and Rayleigh scattering alone during volcanically quiescent conditions. Our NASA GISS ModelE simulations of the Toba eruption reveal up to 50% global ozone loss due to the overall photochemistry perturbations of the sulfate aerosols. We also consider and quantify the radiative effects of SO2, which partially compensated for the ozone loss by inhibiting the photolytic O3 sink. Our analysis shows that the magnitude of the ozone loss and UV-induced health-hazardous effects after the Toba eruption are similar to those in the aftermath of a potential nuclear conflict. These findings suggest a “Toba ozone catastrophe" as a likely contributor to the historic population decline in this period, consistent with a genetic bottleneck in human evolution.

Toba volcano↗