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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 73 records · Page 4
All sourcesNASA NTRSDOE OSTI
NASA NTRS1986

Vertical distribution of ozone and the variation of tropopause heights based on ozonesonde and satellite observations

The distribution of atmospheric ozone is nonuniform both in space and time. Local ozone concentration vary with altitude, latitude, longitude, and season. Two year ozonesonde data, January 1981 to December 1982, observed at four Canadian stations and 2.5 year backscattered ultraviolet experiment data on the Nimbus-4 satellite, April 1970 to August 1972, observed over five American stations were used to study the relationship between the total ozone, vertical height distribution of the ozone mixing ratio, vertical height distribution of half total ozone, and the local tropopause height. The results show that there is a postive correlation between total ozone in Dobson Units and the tropopause height in terms of atmospheric pressure. This result suggests that local intrusion of the statosphere into the troposphere, or the local decreasing of tropopause height could occur if there is a local increasing of total ozone. A comparison of the vertical height distribution of the ozone mixing ratio, the modified pressure height of half total ozone and the tropopause height shows that the pressure height of an ozone mixing ratio of 0.3 micrograms/g, and the modified pressure height of half total ozone are very well correlated with the tropopause pressure height.

Hung, R. J.↗
NASA NTRS1985

Vertical distribution of acetonitrile in the atmosphere

The presence of acetonitrile in the atmosphere was confirmed by results of surface and stratospheric investigations. Stratospheric measurements give mixing ratios typically decreasing with height from 3 ppt at 25 km to 0.5 ppt at 40 km. Measurements at the Earth's surface are less unanimous, although a ground level background mixing ratio of a few times 10 ppt seems realistic. Measurements are compatible with a small global surface source of acetonitrile and a small tropospheric loss. The vertical distribution of acetonitrile presented in consistent with general knowledge of its atmospheric chemistry.

Ingels, J.↗
NASA NTRS2015

Using Satellite Observations of Cloud Vertical Distribution to Improve Global Model Estimates of Cloud Radiative Effect on Key Tropospheric Oxidants

Radiative effect of clouds is one of the major factors that affect tropospheric OH. Large differences in cloud distributions among current (chemistry-climate or chemical transport) models could contribute significantly to the wide model spread of tropospheric OH, which was reported by the ACCMIP activity (Voulgarakis et al., ACP 2013). CCCM, a 3-D cloud data product developed at NASA Langley and merged from multiple A-Train satellite observations, provides unprecedentedly strong constraints on the vertical distribution of clouds and therefore simulated effects of clouds on key tropospheric oxidants.

Liu, Hongyu↗
NASA NTRS1998

Vertical Distribution of Saharan Dust from the Goddard Three Dimensional Transport Model: Comparison with LITE Data

Spatial distributions of Saharan dust are simulated by the Goddard 3D chemistry transport model driven by meteorological fields from the Goddard Earth Observing System Data Assimilation System, GEOS-2 DAS. An aerosol module accounts for gravitational settling and the aerosol source function is based on surface moisture content and wind speed. The simulated aerosol fields are compared with Total Ozone Mapping Spectrometer (TOMS) by P. Ginoux in this session. The main focus is how ventilation of the assimilation winds will impact the simulated aerosol vertical distribution. Excessive ventilation would transport too much aerosol in the upper troposphere and lead to errors in the long range transport as well as errors in any radiative forcing calculations derived from the simulated aerosol fields. Simulated aerosol fields using GEOS-1 DAS wind fields for September 1994 will be compared with lidar observations during the Lidar In-space Technology Experiment (LITE). The lidar return signal clearly delineates the vertical extent and horizontal variability of the aerosol layer allowing rigorous comparison with the simulated fields. A second focus is the simulation of aerosol scavenging due to moist processes. Three-dimensional precipitation fields can be derived from two possible sources: Assimilated precipitation fields from GEOS-DAS or fields obtained from the Special Sensor Microwave/imager (SSM/1). Of interest is the sensitivity of the modeled aerosol fields to the different precipitation fields driving the moist scavenging module.

Weaver, Clark J.↗
NASA NTRS2010

A 10-Year Climatology of Cloud Cover and Vertical Distribution Derived from Both Surface and GOES Observations Over the DOE ARM SGP Site

Analysis of a decade of ARM radar-lidar and GOES observations at the SGP site reveal that 0.5 and 4-hr averages of the surface cloud fraction correspond closely to 0.5deg and 2.5deg averages of GOES cloudiness, respectively. The long-term averaged surface and GOES cloud fractions agree to within 0.5%. Cloud frequency increases and cloud amount decreases as the temporal and spatial averaging scales increase. Clouds occurred most often during winter and spring. Single-layered clouds account for 61.5% of the total cloud frequency. There are distinct bimodal vertical distributions of clouds with a lower peak around 1 km and an upper one that varies from 7.5 to 10.8 km between winter and summer, respectively. The frequency of occurrence for nighttime GOES high-cloud tops agree well with the surface observations, but are underestimated during the day.

Xi, Baike↗
NASA NTRS1994

Analysis of a 7 year tropospheric ozone vertical distribution at the Observatoire de Haute Provence

A seven year (1984-90) climatology of tropospheric vertical ozone soundings, performed by electrochemical sondes at the OHP (44 deg N, 6 deg E, 700 m ASL) in Southern France, is presented. Its seasonal variation shows a broad spring/summer maximum in the troposphere. The contribution of photochemical ozone production and transport from the stratosphere to this seasonal variation are studied by a correlative analysis of ozone concentrations and meteorological variables, with emphasis on potential vorticity. This analysis shows the impact of dynamical and photochemical processes on the spatial and temporal ozone variability. In particular, a positive correlation (r = 04.0, significance greater than 99.9 percent) of ozone with potential vorticity is observed in the middle troposphere, reflecting the impact of stratosphere-troposphere exchange on the vertical ozone distribution.

Beekmann, Matthias↗
NASA NTRS1985

Influence of meteorological conditions on aerosol vertical distribution and composition off the northeast American coastline

The size distribution and composition of lower tropospheric aerosols were measured off the northeast American coastline under clear air and disturbed meteorological conditions. Under the clear air conditions observed on 5 August 1982, with air flow from west to east, sulfate-rich stratified layers are the dominant feature of aerosol distribution in the lowest 3000 m of the troposphere. The encroachment of a warm frontal system over the study area on 9 August 1982 resulted in dramatic changes in aerosol distribution and composition prior to any precipitation, probably due to increased vertical mixing and dilution of pollutant aerosols. Chloride becomes the dominant water soluble anion in the lower 3000 m, primarily due to a several fold decrease in sulfate. Although these results are limited to only two sets of measurements, the data indicate the variability which can occur in the tropospheric vertical aerosol distributions at remote locations. A knowledge of the structure and stability of these stratified layers is of particular importance to studies of the ocean-troposphere chemistry problem.

Sebacher, D. I.↗
NASA NTRS2005

Retrieval of Raindrop Size Distribution, Vertical Air Velocity and Water Vapor Attenuation Using Dual-Wavelength Doppler Radar Observations

Two techniques for retrieving the slope and intercept parameters of an assumed exponential raindrop size distribution (RSD), vertical air velocity, and attenuation by precipitation and water vapor in light stratiform rain using observations by airborne, nadir looking dual-wavelength (X-band, 3.2 cm and W-band, 3.2 mm) radars are presented. In both techniques, the slope parameter of the RSD and the vertical air velocity are retrieved using only the mean Doppler velocities at the two wavelengths. In the first method, the intercept of the RSD is estimated from the observed reflectivity at the longer wavelength assuming no attenuation at that wavelength. The attenuation of the shorter wavelength radiation by precipitation and water vapor are retrieved using the observed reflectivity at the shorter wavelength. In the second technique, it is assumed that the longer wavelength suffers attenuation only in the melting band. Then, assuming a distribution of water vapor, the melting band attenuation at both wavelengths and the rain attenuation at the shorter wavelength are retrieved. Results of the retrievals are discussed and several physically meaningful results are presented.

Heymsfield, Gerald M.↗
NASA NTRS2016

What Controls the Vertical Distribution of Aerosol? Relationships Between Process Sensitivity in HadGEM3-UKCA and Inter-Model Variation from AeroCom Phase II

The vertical profile of aerosol is important for its radiative effects, but weakly constrained by observations on the global scale, and highly variable among different models. To investigate the controlling factors in one particular model, we investigate the effects of individual processes in HadGEM3-UKCA and compare the resulting diversity of aerosol vertical profiles with the inter-model diversity from the AeroCom Phase II control experiment. In this way we show that (in this model at least) the vertical profile is controlled by a relatively small number of processes, although these vary among aerosol components and particle sizes. We also show that sufficiently coarse variations in these processes can produce a similar diversity to that among different models in terms of the global-mean profile and, to a lesser extent, the zonal-mean vertical position. However, there are features of certain models' profiles that cannot be reproduced, suggesting the influence of further structural differences between models. In HadGEM3-UKCA, convective transport is found to be very important in controlling the vertical profile of all aerosol components by mass. In-cloud scavenging is very important for all except mineral dust. Growth by condensation is important for sulfate and carbonaceous aerosol (along with aqueous oxidation for the former and ageing by soluble material for the latter). The vertical extent of biomass-burning emissions into the free troposphere is also important for the profile of carbonaceous aerosol. Boundary-layer mixing plays a dominant role for sea salt and mineral dust, which are emitted only from the surface. Dry deposition and below-cloud scavenging are important for the profile of mineral dust only. In this model, the microphysical processes of nucleation, condensation and coagulation dominate the vertical profile of the smallest particles by number (e.g. total CN >3 nm), while the profiles of larger particles (e.g. CN>100 nm) are controlled by the same processes as the component mass profiles, plus the size distribution of primary emissions. We also show that the processes that affect the AOD-normalised radiative forcing in the model are predominantly those that affect the vertical mass distribution, in particular convective transport, in-cloud scavenging, aqueous oxidation, ageing and the vertical extent of biomass-burning emissions.

dust↗
NASA NTRS1990

Vertical distribution of water in the atmosphere of Venus - A simple thermochemical explanation

Several lines of evidence concerning the vertical abundance profile of water in the atmosphere of Venus lead to strikingly unusual distributions (the water vapor abundance decreases sharply in the immediate vicinity of the surface) or to serious conflicts in the profiles (different IR bands suggest water abundances that are discrepant by a factor of 2.5 to 10). These data sets can be reconciled if (1) water molecules associate with carbon dioxide and sulfur trioxide to make gaseous carbonic acid and sulfuric acid in the lower atmosphere, and (2) the discrepant 0.94-micrometer water measurements are due to gaseous sulfuric acid, requiring it to be a somewhat stronger absorber than water vapor in this wavelength region. A mean total water abundance of 50 + or - 20 parts/million and a near-surface free water vapor abundance of 10 + or - 4 parts/million are derived.

Lewis, John S.↗
NASA NTRS1994

The 1990 vertical distribution of two important halons (F-12B1 and F-13B1) in the tropics

The first vertical profiles of F-12B1 and F-13B1 had been obtained in the tropical troposphere and stratosphere by us in 1987. The measurement of these substances responsible for almost the entire anthropogenic contribution to the stratospheric BrO(x) budget is important in the tropics, as tropical upwelling provides their injection along with that of other pollutants, into the stratosphere. To ascertain the trends of these distributions and foster the data, the 1987 experiment was repeated in April 1990. Like 1987, the MPAE cryogenic whole air sampler was launched on a balloon from Hyderabad, India (17.5 deg N), and 14 samples were collected between 10 and 35 km altitude. The results obtained by means of GC and GC-MS analyses showed that the atmospheric abundance of both F-12B1 and F-13B1 is increasing at a fast rate, respectively by about 15 percent and 10 percent per year. From 1987 to 1990, F-12B1 and F-13B1 tropospheric mixing ratios have been growing from 1.2 and 1.3 ppt to 1.8 and 1.7 ppt, respectively. The vertical profiles will be discussed.

Singh, O. N.↗
NASA NTRS1995

Ozone vertical distribution retrieval from ground-based high resolution infrared solar spectra

A practical procedure for the retrieval of ozone vertical profiles from ground-based high resolution Fourier transform infrared solar spectra has been developed. The analysis is based on a multilayer line-by-line forward model and a semi-empirical version of the optimal estimation inversion method of Rodgers. The 1002.6-1003.2 cm(exp -1) spectral interval has been selected for the analysis on the basis of synthetic spectrum calculations. This interval contains numerous ozone lines covering a range of intensities and providing retrieval sensitivity from ground level to about 35 km. Characterization of the method and an error analysis have been performed. For a spectral resolution of 0.05-0.01 cm(exp -1) and a signal-to-noise ratio greater than or equal to 100 the retrieval is stable with a vertical resolution of approximately 5 km attainable near the surface degrading to approximately 10 km in the stratosphere. Synthetic spectra studies show that the a priori profile and weak constraints selected for the retrievals introduce no significant biases for a wide range of ozone profiles.

Pougatchev, N. S.↗
NASA NTRS1999

Trends in the Vertical Distribution of Ozone

Analyses of satellite, ground-based, and balloon measurements allow updated estimates of trends in the vertical profile of ozone since 1979. The results show overall consistency among several independent measurement systems, particularly for northern hemisphere midlatitudes where most balloon and ground-based measurements are made. Combined trend estimates over these latitudes for the period 1979-96 show statistically significant negative trends at ail attitudes between 10 and 45 km, with two local extremes: -7.4 +/- 2.0% per decade at 40 km and -7.3 +/- 4.6% per decade at 15 km attitude. There is a strong seasonal variation in trends over northern midlatitudes in the altitude range of 10 to 18 km, with the largest ozone loss during winter and spring. The profile trends are in quantitative agreement with independently measured trends in column ozone, the amount of ozone in a column above the surface. The vertical profiles of ozone trends provide a fingerprint for the mechanisms of ozone depletion over the last two decades.

Randel, William J.↗
NASA NTRS1999

Trends in the Vertical Distribution of Ozone

Analyses of satellite, ground-based, and balloon measurements allow updated estimates of trends in the vertical profile of ozone since 1979. The results show overall consistency among several independent measurement systems, particularly for northern hemisphere midlatitudes where most balloon and ground-based measurements are made. Combined trend estimates over these latitudes for the period 1979-96 show statistically significant negative trends at all altitudes between 10 and 45 km, with two local extremes: -7.4 plus or minus 2.0% per decade at 40 km and -7.3 plus or minus -4.6% per decade at 15 km altitude. There is a strong seasonal variation in trends over northern midlatitudes in the attitude range of 10 to 18 km, with the largest ozone loss during winter and spring. The profile trends are in quantitative agreement with independently measured trends in column ozone, the amount of ozone in a column above the surface. The vertical profiles of ozone trends provide a fingerprint for the mechanisms of ozone depletion over the last two decades.

Randel, William J.↗
NASA NTRS2002

Trends in the Vertical Distribution of Ozone

Analyses of satellite, ground-based, and balloon measurements allow updated estimates of trends in the vertical profile of ozone since 1979. The results show overall consistency among several independent measurement systems, particularly for northern hemisphere midlatitudes where most balloon and ground-based measurements are made. Combined trend estimates over these latitudes for the period 1979-96 show statistically significant negative trends at all attitudes between 10 and 45 km, with two local extremes: -7.4 +/- 2.0% per decade at 40 km and -7.3 +/- 4.6% per decade at 15 km attitude. There is a strong seasonal variation in trends over northern midlatitudes in the attitude range of 10 to 18 km. with the largest ozone loss during winter and spring. The profile trends are in quantitative agreement with independently measured trends in column ozone, the amount of ozone in a column above the surface. The vertical profiles of ozone trends provide a fingerprint for the mechanisms of ozone depletion over the last two decades,

Cunnold, Derek M.↗
NASA NTRS1998

Trends in the Vertical Distribution of Ozone

Recent reanalyses of satellite, ground-based and balloon measurements allow updated estimates of trends in the vertical profile of ozone during 1980-96. The results show overall consistency between several independent measurement systems, particularly for northern hemisphere mid-latitudes where most ground-based measurements are made. Combined trend estimates over these latitudes show statistically significant negative trends at all altitudes between 10 and 45 km, with two local maxima: -7.4 +/- 2.0%/decade at 40 km and -7.6 +/- 4.6%/decade at 15 km altitude. There is a strong seasonal variation in trends over northern mid-latitudes in the altitude range of 10- 18 km. The profile trends are in quantitative agreement with independently measured trends in column ozone.

Randel, William J.↗
NASA NTRS2018

A Singular Value Decomposition Framework for Retrievals with Vertical Distribution Information from Greenhouse Gas Column Absorption Spectroscopy Measurements

We review the singular value decomposition (SVD) framework and use it for quantifying and discerning vertical information in greenhouse gas retrievals from column integrated absorption measurements. While the commonly used traditional Bayesian optimal estimation (OE) assumes a prior distribution in order to regularize the inversion problem, the SVD approach identifies principal components that can be retrieved from the measurement without explicitly specifying a prior mean and prior covariance matrix. We review the SVD method, explicitly recognize the use of an uninformative prior and show it to incur no bias from the choice of the prior. We also make the connection between the SVD method and the pseudo-inverse, which makes it more intuitive and easy to understand. We illustrate the use of the SVD method on an integrated path differential absorption CO2 lidar measurement model and verify our derivations and bias-free properties versus optimal estimation using numerical simulations. In contrast, traditional OE retrievals exhibit bias when the prior mean used in the retrieval differs from the true mean. Hence, the SVD method is particularly useful for situations in which knowledge of the prior mean and prior covariance of the true state (e.g., greenhouse gas profiles) is inadequate.

Ramanathan, Anand K.↗
NASA NTRS1980

Vertical distribution of aerosol extinction cross section and inference of aerosol imaginary index in the troposphere by lidar technique

The paper reports on vertical profiles of aerosol extinction and backscatter in the troposphere which were obtained from multi zenith angle lidar measurements. It is reported that a direct slant path solution was found to be not possible due to horizontal inhomogeneity of the atmosphere. Attention is given to the use of a regression analysis with respect to zenith angle for a layer integration of the angle dependent lidar equation in order to determine the optical thickness and aerosol extinction-to-backscatter ratio for defined atmospheric layers and the subsequent evaluation of cross-section profiles.

Spinhirne, J. D.↗