Increasing plant water stress and decreasing summer streamflow in response to a warmer and wetter climate in seasonally snow-covered forests
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Environmental Sciences & Ecology↗
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Mixed imbibition controls the advance of wetting fluid in multiscale geological media
Imbibition plays a central role during multiphase flows in geological media; yet, our understanding of imbibition dynamics across the multiscale features of rocks, including fractures, microcracks, and heterogeneous matrices is limited. Here, we deployed a unique combination of micro- and clinical X-ray CT imaging to probe directly the spatiotemporal evolution of imbibition in a natural, multiscale shale sample. The method enabled unraveling of mixed imbibition behavior, with spontaneous imbibition rates in the matrix pores and microcracks driven by capillarity proceeding as $\propto t^{-1/2}$, whereas pressure-driven flows in the macroscopic fractures yield apparent imbibition rates with $\propto t^{-1}$ scaling. Regardless of the aperture, we showed that spontaneous imbibition proceeds uniformly away from the fractures. The effects of microcracks are further investigated by comparing the dynamics of the imbibition fronts with and without microcracks. Finally, these results highlight the paramount role of microcracks on anomalous front roughening and the need to account for microcracks appropriately in the development of predictive theoretical models.
58 GEOSCIENCES↗
Algal Biomass Conversion to Fuels via Combined Algae Processing (CAP): 2022 State of Technology and Future Research
The annual State of Technology (SOT) assessment is an essential activity for platform research conducted under the Bioenergy Technologies Office (BETO). It allows for the impact of research progress (both directly achieved in-house at NREL and furnished by partner organizations) to be quantified in terms of economic improvements in the overall biofuel production process for a particular biomass processing pathway, whether based on terrestrial or algal biomass feedstocks. As such, initial benchmarks can be established for currently demonstrated performance, and progress can be tracked toward out-year goals to ultimately demonstrate economically viable biofuel technologies. NREL's algae SOT benchmarking efforts focus both on front-end algal biomass production and separately on back-end conversion to fuels through NREL's "combined algae processing" (CAP) pathway. The production model is based on outdoor long-term cultivation data, enabled by comprehensive algal biomass production trials conducted under Development of Integrated Screening, Cultivar Optimization, and Verification Research (DISCOVR) consortium efforts and driven by data furnished by Arizona State University's (ASU's) Arizona Center for Algae Technology and Innovation (AzCATI) test bed site. The CAP model is primarily based on experimental efforts conducted under NREL research and development projects, with some process parameters provided by partner organizations. Assumptions regarding the wet storage of algae use data provided by Idaho National Laboratory (INL), while parts of the polyurethane production process leverage BETO-funded research from collaborators at Algenesis and the University of California, San Diego (UCSD). This report focuses on back-end conversion of algal biomass through the CAP pathway, highlighting the 2022 updates to minimum fuel selling price (MFSP). This update incorporates improvements to fermentation performance for two biological pathways through carboxylic acid and 2,3-butanediol (BDO) intermediates, as demonstrated through parallel research on the biochemical conversion of corn stover. Improvements are applied to the glucose fraction of the biomass only, while parameters regarding the conversion of the mannose fraction (not a significant component in corn stover) are maintained consistently with prior CAP SOTs. Additional parameters are also updated to reflect the most current understanding of each pathway, including an increase in the catalyst loading requirement in the ketonization step of the acids pathway and a decrease in the fermentation productivity in the BDO pathway. Additionally, the biomass feedstock costs (minimum biomass selling price [MBSP]), yields, and seasonal variability from the upstream cultivation SOT model were also incorporated into downstream Aspen Plus CAP models.
09 BIOMASS FUELS↗
Industrial Requirements Status Report and Down-Select of Candidate Technologies
The report discusses the potential for implementing Integrated Energy Systems (IES) using advanced nuclear reactors to provide thermal and electrical energy to carbon-emitting industries while reducing their carbon footprint. Nine different industries were reviewed to determine their decarbonization potential, how nuclear power can fit in, and the carbon footprint of each. The report also identifies specific integration points and streams for most processes, including temperature and pressure requirements of integrating nuclear power with industrial processes. The report also provides insights on advanced nuclear reactors and their potential for us in IES for decarbonization. The target audience for the report is broad, but mainly addressed to the industry leads and nuclear reactor developers. The report recommends that in the short term, a few processes should be identified to continue research and investigation so that front end engineering design work can provide technical analysis for integrating nuclear heat and replacing existing carbon-emitting thermal sources. The work emphasized the significant decarbonization opportunity across each of the technologies looked at as well as how novel and useful nuclear integration is to reduce the environmental impact of these significant industries.
02 PETROLEUM↗
Numerical Optimization of the Thermal Field in Bridgman Detached Growth
The global modeling of the thermal field in two vertical Bridgman-like crystal growth configurations, has been performed to get optimal thermal conditions for a successful detached growth of Ge and CdTe crystals. These computations are performed using the CrysMAS code and expand upon our previous analysis [1] that propose a new mechanism involving the thermal field and meniscus position to explain stable conditions for dewetted Bridgman growth. The analysis of the vertical Bridgman configuration with two heaters, used by Palosz et al. for the detached growth of Ge, shows, consistent with their results, that the large wetting angle of germanium on boron nitride surfaces was an important factor to promote a successful detached growth. Our computations predict that by initiating growth much higher into the hot zone of the furnace, the thermal conditions will be favorable for continued detachment even for systems that did not exhibit high contact angles. The computations performed for a vertical gradient freeze configuration with three heaters representative of that used for the detached growth of CdTe, show favorable thermal conditions for dewetting during the entirely growth run described. Improved thermal conditions are also predicted for coated silica crucibles when the solid-liquid interface advances higher into the hot zone during the solidification process. The second set of experiments on CdTe growth described elsewhere has shown the reattachment of the crystal to the crucible after few centimeters of dewetted growth. The thermal modeling of this configuration shows a second solidification front appearing at the top of the sample and approaching the middle line across the third heater. In these conditions, the crystal grows detached from the bottom, but will be attached to the crucible in the upper part because of the solidification without gap in this region. The solidification with two interfaces can be avoided when the top of the sample is positioned below the middle position of the third furnace.
Stelian, C.↗
Amapari Marker Band Metal‐Enrichments: Potential Mechanisms and Implications for Surface and Subsurface Water and Weathering in Gale Crater
NASA's Curiosity rover is exploring a 5 km tall sedimentary mound that is hypothesized to record the transition from a warm and wet (phyllosilicate-rich) to a cold and drier (sulfate-rich) Mars. Evidence of magnesium sulfate-bearing rock has shown that Curiosity has crossed through this phyllosilicate-sulfate transition. Recently, Curiosity arrived at the Amapari Marker Band, a darker, indurated unit that can be traced laterally for tens of kilometers in orbiter images. Here, Curiosity found evidence for a very broad lake, and bedforms interpreted as wave-ripple laminated sedimentary rock that likely was deposited in shallow water in the explored location, before becoming a deeper lake. These rocks are enriched in Fe, Mn, and Zn which has major implications for groundwater paleohydrology in Gale crater. Three formation hypotheses are considered: concretion formation during early diagenetic alteration of shallow lake sediments, laterization or leaching of the sediments, and addition of Fe, Mn, and Zn by a mildly acidic and reducing groundwater interacting with a redox and/or pH front in a stratified lake. The preferred interpretation of the metal enrichments within the Amapari Marker band sedimentary rocks is that they formed in a shallow water environment at a redox and/or pH front within the ripple unit, which drove precipitation and concentration of metals. If the enrichments are due to groundwater alteration, these processes could link subsurface and surface environments. Water and the presence of high amounts of redox sensitive elements and other metals are favorable indicators for habitability.
58 GEOSCIENCES↗
Plateaus and Sinuous Ridges as the Fingerprints of Lava Flow Inflation in the Eastern Tharsis Plains of Mars
The Tharsis Montes rift aprons are composed of outpourings of lava from chaotic terrains to the northeast and southwest flank of each volcano. Sinuous and branching channel networks that are present on the rift aprons suggest the possibility of fluvial processes in their development, or erosion by rapidly emplaced lavas, but the style of lava flow emplacement throughout rift apron development is not clearly understood. To better characterize the style of lava emplacement and role of fluvial processes in rift apron development, we conducted morphological mapping of the Pavonis Mons southwest rift apron and the eastern Tharsis plains using images from the High Resolution Imaging Science Experiment (HiRISE), Mars Orbiter Camera (MOC), Context Camera (CTX), Thermal Emission Imaging System (THEMIS), and High Resolution Stereo Camera (HRSC) along with the Mars Orbiter Laser Altimeter (MOLA) Precision Experiment Data Records (PEDRs) and gridded data. Our approach was to: (1) search for depositional fans at the slope break between the rift apron and adjacent low slope plains; (2) determine if there is evidence that previously formed deposits might have been buried by plains units; (3) characterize the Tharsis plains morphologies east of Pavonis Mons; and (4) assess their relationship to the rift apron units. We have not identified topographically significant depositional fans, nor did we observe evidence to suggest that plains units have buried older rift apron units. Flow features associated with the rift apron are observed to continue across the slope break onto the plains. In this area, the plains are composed of a variety of small fissures and low shield vents around which broad channel-fed and tube-fed flows have been identified. We also find broad, flat-topped plateaus and sinuous ridges mixed among the channels, tubes and vents. Flat-topped plateaus and sinuous ridges are morphologies that are analogous to those observed on the coastal plain of Hawai'i, where lava flows have advanced from the volcano's several degree flank onto the nearly zero degree coastal plain. When local volumetric flow rates are low, flow fronts tend to spread laterally and often thicken via endogenous growth, or inflation, of the sheet-like flow units. If flow advance is restricted by existing topography into narrow pathways, inflation can be focused into sinuous, elongate ridges. The presence of plateaus and ridges-emplaced from the rift zones, across the plains to the east of Pavonis Mons-and a lack of fan-like features, or evidence for their burial, are consistent with rift apron lavas crossing a slope break with low local volumetric flow rates that led to inflation of sheet-like and tube-fed lava flows.
Bleacher, Jacob E.↗
Defect, Kinetics and Heat Transfer of CDTE Bridgman Growth without Wall Contact
A detached growth mechanism has been proposed, which is similar to that proposed by Duffar et al. and used to study the current detached growth system. From numerical results, we can conclude that detached growth will more likely appear if the growth and wetting angles are large and meniscus is flat. Detached thickness is dependent on growth angle, wetting angle, and gap width and shape of the fins. The model can also explain why the detached growth will not happen for metals in which the growth angle is almost zero. Since the growth angle of CdZnTe cannot be changed, to promote detached growth, the number density of the fins should be low and the wetting angle should be high. Also, a much smaller gap width of the fins should be used in the ground experiment and the detached gap width is much smaller. The shape of the fins has minor influence on detached growth. An integrated numerical model for detached solidification has been developed combining a global heat transfer sub-model and a wall contact sub-model. The global heat transfer sub-model accounts for heat and mass transfer in the multiphase system, convection in the melt, macro-segregation, and interface dynamics. The location and dynamics of the solidification interface are accurately tracked by a multizone adaptive grid generation scheme. The wall contact sub-model accounts for the meniscus dynamics at the three-phase boundary. Simulations have been performed for crystal growth in a conventional ampoule and a designed ampoule to understand the benefits of detached solidification and its impacts on crystalline structural quality, e.g., stoichiometry, macro-segregation, and stress. From simulation results, both the Grashof and Marangoni numbers will have significant effects on the shape of growth front, Zn concentration distribution, and radial segregation. The integrated model can be used in designing apparatus and determining the optimal geometry for detached solidification in space and on the ground.
Larson, D. J., Jr.↗
JMR Noise Diode Stability and Recalibration Methodology after Three Years On-Orbit
The Jason Microwave Radiometer (JMR) is included on the Jason-1 ocean altimeter satellite to measure the wet tropospheric path delay (PD) experienced by the radar altimeter signal. JMR is nadir pointing and measures the radiometric brightness temperature (T(sub B)) at 18.7, 23.8 and 34.0 GHz. JMR is a Dicke radiometer and it is the first radiometer to be flown in space that uses noise diodes for calibration. Therefore, monitoring the long term stability of the noise diodes is essential. Each channel has three redundant noise diodes which are individually coupled into the antenna signal to provide an estimate of the gain. Two significant jumps in the JMR path delays, relative to ground truth, were observed around 300 and 700 days into the mission. Slow drifts in the retrieved products were also evident over the entire mission. During a recalibration effort, it was determined that a single set of calibration coefficients was not able to remove the calibration jumps and drifts, suggesting that there was a change in the hardware and time dependent coefficients would be required. To facilitate the derivation of time dependent coefficients, an optimal estimation based calibration system was developed which iteratively determines that set of calibration coefficients which minimize the RMS difference between the JMR TBs and on-Earth hot and cold absolute references. This optimal calibration algorithm was used to fine tune the front end path loss coefficients and derive a time series of the JMR noise diode brightness temperatures for each of the nine diodes. Jumps and drifts, on the order of 1% to 2%, are observed among the noise diodes in the first three years on-orbit.
Jason 1↗