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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 73 records · Page 4

Radon emanation rate measurements using liquid scintillation counting

This article describes a radon emanation measurement technique using liquid scintillator counting. A model for radon loading and transport is described, along with its calibration. Detector background and blank have been studied and quantified. The Minimal detectable activity has been determined for the counting setup using a toy Monte Carlo simulation. Here, the measurement technique is validated using a butyl rubber sample previously used for cross-calibration between different radon counting facilities.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Extracting the Galactic Center excess’ source-count distribution with neural nets

The two leading hypotheses for the Galactic Center excess (GCE) in the Fermi data are an unresolved population of faint millisecond pulsars (MSPs) and dark-matter (DM) annihilation. The dichotomy between these explanations is typically reflected by modeling them as two separate emission components. However, point sources (PSs) such as MSPs become statistically degenerate with smooth Poisson emission in the ultrafaint limit (formally where each source is expected to contribute much less than one photon on average), leading to an ambiguity that can render questions such as whether the emission is PS-like or Poissonian in nature ill defined. We present a conceptually new approach that describes the PS and Poisson emission in a unified manner and only afterwards derives constraints on the Poissonian component from the so obtained results. For the implementation of this approach, we leverage deep learning techniques, centered around a neural network-based method for histogram regression that expresses uncertainties in terms of quantiles. We demonstrate that our method is robust against a number of systematics that have plagued previous approaches, in particular DM/PS misattribution. In the Fermi data, we find a faint GCE described by a median source-count distribution (SCD) peaked at a flux of ~ 4 x 10 -11 counts cm -2 s -1 (corresponding to ~ 3-4 expected counts per PS), which would require N ~ $\mathscr{O}$(10 4 ) sources to explain the entire excess (median value N = 29,300 across the sky). Although faint, this SCD allows us to derive the constraint η ρ ≤ 66% for the Poissonian fraction of the GCE flux η ρ at 95% confidence, suggesting that a substantial amount of the GCE flux is due to PSs.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Reduced Dynamics of Full Counting Statistics

We present a theory of modified reduced dynamics in the presence of counting fields. Reduced dynamics techniques are useful for describing open quantum systems at long emergent timescales when the memory timescales are short. However, they can be difficult to formulate for observables spanning the system and its environment, such as those characterizing transport properties. A large variety of mixed system--environment observables, as well as their statistical properties, can be evaluated by considering counting fields. Given a numerical method able to simulate the field-modified dynamics over the memory timescale, we show that the long-lived full counting statistics can be efficiently obtained from the reduced dynamics. We demonstrate the utility of the technique by computing the long-time current in the nonequilibrium Anderson impurity model from short-time Monte Carlo simulations.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Radiation Transport Simulation of the Sulfur Counting System in the Radiation Metrology Laboratory (RML)

At the request of staff members from the Radiation Metrology Laboratory (RML), a series of Monte Carlo radiation transport calculations were performed using two different models of the detector geometry of the RMLs sulfur counting system. The fraction of electrons from each β-decay of 32 P in the sulfur pellet that enter the window of the sulfur counting system was calculated with both MCNP and ITS. In addition, the differential energy distributions of the electrons entering the counting system window were computed. There was significant agreement between the integral and differential quantities calculated by the two transport codes. Summary tables are for the integral efficiency values are found in the body of the report.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Identification of background limitations to ultra-sensitive $\mathrm{LSC}$ counting through $\mathrm{ICP}$-$\mathrm{MS}$ assay of $\mathrm{LSC}$ cocktails

We report the performance of LSC cocktails in ultra-sensitive applications was evaluated. Backgrounds from radioactive contaminations in commercially available and in-house developed liquid scintillation cocktails were measured and compared to the predicted background levels of the ultra-low background liquid scintillation counter. Through the ICP-MS assay of the cocktails and their constituents, potassium impurities in the surfactant component were identified as a significant source of background, potentially limiting the use of LSC counting in ultra-sensitive applications. This work lays the groundwork for future research towards ultrapure LSC cocktails for ultrasensitive LSC counting

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Photon counting with intensified charge coupled device (ICCD) – II. Laser induced breakdown spectroscopy (LIBS) spectral measurement

This study explores the application of photon counting (PC) to enhance the resolution of spectra acquired by an intensified charge-coupled device (ICCD) detector, with a focus on analytical atomic emission spectrometry using laser-induced breakdown spectroscopy (LIBS) as a use-case example. It demonstrates that, for spectra obtained with the same spectrometer–ICCD system, PC provides higher spectral resolution compared to conventional analog detector readout. This enhancement is particularly evident in the line wings of spectral peaks, facilitating better discrimination of isotopic peaks in the measured spectra. Although PC does not improve the resolution of an optical spectrometer directly, it rectifies the resolution lost caused by signal spreading in conventional ICCD analog measurement. However, similar to other counting techniques, excessive photons compromise detector linearity due to signal pileup. A correction model is proposed to mitigate the pileup effect, resulting in improved linearity and dynamic range in PC measurements. Additionally, the study reveals unexpected periodic structures in the flatfield image of the ICCD, which cause non-uniform detector gain in conventional analog as well as PC measurement modes and must be addressed for high-precision measurements.

47 OTHER INSTRUMENTATION↗

In Situ Ion Counting for Improved Implanted Ion Error Rate and Silicon Vacancy Yield Uncertainty

An in situ counted ion implantation experiment improving the error on the number of ions required to form a single optically active silicon vacancy (SiV) defect in diamond 7-fold compared to timed implantation is presented. Here, traditional timed implantation relies on a beam current measurement followed by implantation with a preset pulse duration. It is dominated by Poisson statistics, resulting in large errors for low ion numbers. Instead, our in situ detection, measuring the ion number arriving at the substrate, results in a 2-fold improvement of the error on the ion number required to generate a single SiV compared to timed implantation. Through postimplantation analysis, the error is improved 7-fold compared to timed implantation. SiVs are detected by photoluminescence spectroscopy, and the yield of 2.98% is calculated through the photoluminescence count rate. Hanbury–Brown–Twiss interferometry is performed on locations potentially hosting single-photon emitters, confirming that 82% of the locations exhibit single photon emission statistics.

77 NANOSCIENCE AND NANOTECHNOLOGY↗

Quantum nondemolition photon counting with a hybrid electromechanical probe

Quantum nondemolition (QND) measurements of photons is a much pursued endeavor in the field of quantum optics and quantum information processing. Here, we propose a hybrid optoelectromechanical platform that integrates a cavity system with a hybrid electromechanical probe for QND photon counting. Building upon a mechanical-mode-mediated nonperturbative electro-optical dispersive coupling, our protocol performs the QND photon counting measurement by means of the current-voltage characteristics of the probe. In particular, we show that the peak voltage shift of the differential conductance is linearly dependent on the photon occupation number, thus providing a sensitive measure of the photon number, especially in the strong optomechanical coupling regime. Here, given that our proposed hybrid system is compatible with state-of-the-art experimental techniques, we discuss its implementations and anticipate applications in quantum optics and polariton physics.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Distinct universality classes of diffusive transport from full counting statistics

The hydrodynamic transport of local conserved densities furnishes an effective coarse-grained description of the dynamics of a many-body quantum system. However, the full quantum dynamics contains much more structure beyond the simplified hydrodynamic description. Here we show that systems with the same hydrodynamics can nevertheless belong to distinct dynamical universality classes, as revealed by new classes of experimental observables accessible in synthetic quantum systems, which can, for instance, measure simultaneous site-resolved snapshots of all of the particles in a system. Specifically, we study the full counting statistics of spin transport, whose first moment is related to linear-response transport, but the higher moments go beyond. We present an analytic theory of the full counting statistics of spin transport in various integrable and nonintegrable anisotropic one-dimensional spin models, including the XXZ spin chain. We find that spin transport, while diffusive on average, is governed by a distinct non-Gaussian dynamical universality class in the models considered. We consider a setup in which the left and right half of the chain are initially created at different magnetization densities, and consider the probability distribution of the magnetization transferred between the two half-chains. We derive a closed-form expression for the probability distribution of the magnetization transfer, in terms of random walks on the half-line. We show that this distribution strongly violates the large-deviation form expected for diffusive chaotic systems, and explain the physical origin of this violation. Here, we discuss the crossovers that occur as the initial state is brought closer to global equilibrium. Our predictions can directly be tested in experiments using quantum gas microscopes or superconducting qubit arrays.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

A Block-Based Triangle Counting Algorithm on Heterogeneous Environments

Triangle counting is a fundamental building block in graph algorithms. In this article, we propose a block-based triangle counting algorithm to reduce data movement during both sequential and parallel execution. Our block-based formulation makes the algorithm naturally suitable for heterogeneous architectures. The problem of partitioning the adjacency matrix of a graph is well-studied. Our task decomposition goes one step further: it partitions the set of triangles in the graph. By streaming these small tasks to compute resources, we can solve problems that do not fit on a device. We demonstrate the effectiveness of our approach by providing an implementation on a compute node with multiple sockets, cores and GPUs. The current state-of-the-art in triangle enumeration processes the Friendster graph in 2.1 seconds, not including data copy time between CPU and GPU. Using that metric, our approach is 20 percent faster. When copy times are included, our algorithm takes 3.2 seconds. This is 5.6 times faster than the fastest published CPU-only time.

97 MATHEMATICS AND COMPUTING↗

A Bayesian nonparametric analysis for zero-inflated multivariate count data with application to microbiome study

High-throughput sequencing technology has enabled researchers to profile microbial communities from a variety of environments, but analysis of multivariate taxon count data remains challenging. Here, we develop a Bayesian nonparametric (BNP) regression model with zero inflation to analyse multivariate count data from microbiome studies. A BNP approach flexibly models microbial associations with covariates, such as environmental factors and clinical characteristics. The model produces estimates for probability distributions which relate microbial diversity and differential abundance to covariates, and facilitates community comparisons beyond those provided by simple statistical tests. We compare the model to simpler models and popular alternatives in simulation studies, showing, in addition to these additional community-level insights, it yields superior parameter estimates and model fit in various settings. The model's utility is demonstrated by applying it to a chronic wound microbiome data set and a Human Microbiome Project data set, where it is used to compare microbial communities present in different environments.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

A Block-Based Triangle Counting Algorithm on Heterogeneous Environments

Triangle counting is a fundamental building block in graph algorithms. In this paper, we propose a block-based triangle counting algorithm to reduce data movement during both sequential and parallel execution. Our block-based formulation makes the algorithm naturally suitable for heterogeneous architectures. The problem of partitioning the adjacency matrix of a graph is well-studied. Our task decomposition goes one step further: it partitions the set of triangles in the graph. By streaming these small tasks to compute resources, we can solve problems that do not fit on a device. We demonstrate the effectiveness of our approach by providing an implementation on a compute node with multiple sockets, cores and GPUs. The current state-of-the-art in triangle enumeration processes the Friendster graph in 2.1 seconds, not including data copy time between CPU and GPU. Using that metric, our approach is 20 percent faster. When copy times are included, our algorithm takes 3.2 seconds. This is 5.6 times faster than the fastest published CPU-only time.

97 MATHEMATICS AND COMPUTING↗

Demonstration of low-level biogenic fuel content using quench curve and direct liquid scintillation counting (LSC) methods

In this work, an investigation into the direct method for liquid scintillation counting (LSC) quantification of biogenic fuel content in fuel blendstock is presented. This method development intentionally used a colored matrix (~99 wt%), fossil diesel fraction, and low-level biogenic fractions (~1 wt%) to determine the applicability of the LSC technique in colored blend mixtures. LSC procedures for quench correction, including the use of an instrument internal standard (Quantulus SQP values), color quench curves, and an internal 14 C standard spike on samples containing low-level amounts of biogenic gasoline, jet, and diesel mixed with fossil fuel, were compared. Samples were analyzed on both Perkin-Elmer Quantulus and Tri-Carb instruments, and the 14 C contents were compared with those determined by accelerator mass spectrometry (AMS). Results from the Tri-Carb instrument showed that percent differences of <10 % compared to AMS-reported values are achievable at 5-hour count times despite colored samples. A comparison between the impact of chemical and color quenching in the fuel samples showed that color quenching in highly colored samples reduces efficiency significantly more than chemical quenching, indicating that chemical quench curves are not appropriate for highly colored biofuel/fossil-fuel blended samples. Results indicate that both the direct method with internal spike quench correction and the use of a color-quench curve provide accurate results for 1 % biogenic fuel blends. Additionally, we have explored the use of Fourier transform infrared (FTIR) spectroscopy in measuring the biogenic content of the colored blended fuel samples. Preliminary results show the presence of biogenic carbon-derived fingerprints that are absent in fossil-derived sample. However, further work is needed to develop an FTIR-based quantitative method.

09 BIOMASS FUELS↗

Circulating Lymphocyte Counts Early During Radiation Therapy Are Associated With Recurrence in Pediatric Medulloblastoma

Decreased peripheral lymphocyte counts are associated with survival after radiation therapy (RT) in several solid tumors, although they appear late during or after the radiation course and often correlate with other clinical factors. Here we investigate if absolute lymphocyte counts (ALCs) are independently associated with recurrence in pediatric medulloblastoma early during RT.

62 RADIOLOGY AND NUCLEAR MEDICINE↗

Algorithms of pulse shape analysis for Gammasphere under high count rate conditions

The implementation of digital electronics for the multi-detector Gammasphere array has provided an opportunity to perform experiments which exceed the technical capabilities of its analog counterpart. The pulse shape analysis of HPGe detectors is presented for the purpose of determining the γ-ray energy under high-counting rates and short integration times with the aim of improving the data throughput. A revised trapezoidal algorithm is delineated which is able to determine the γ-ray energies during the offline analysis without being constrained by predetermined parameters. The performance of this algorithm is discussed, and compared with that of the analog system. The measured energy resolution meets expectations for operations with high-counting rates and short integration times.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Absolute decay counting of 146 Sm with 4π cryogenic microcalorimetry

We present a methodology for absolute activity counting of long-lived isotopes based on cryogenic Decay Energy Spectroscopy. A 146 Sm source was produced at the TRIUMF Laboratory and then processed and purified at Lawrence Livermore National Laboratory, yielding a pure sample. The source was embedded within a 4π thermal absorber coupled to a magnetic microcalorimeter achieving nearly 100% counting efficiency. Experimental uncertainties were studied and modeled, including thermal coupling of the source to the absorber, pulse pile-up, trigger, and event selection efficiencies. Here, the absolute activity of the pure 146 Sm source was measured to better than 1% uncertainty.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

The SRG/eROSITA All-Sky Survey: Constraints on ultralight axion dark matter through galaxy cluster number counts

Ultralight axions are hypothetical scalar particles that influence the evolution of large-scale structures of the Universe. Depending on their mass, they can potentially be part of the dark matter component of the Universe as candidates commonly referred to as fuzzy dark matter. While strong constraints have been established for pure fuzzy dark matter models, the more general scenario where ultralight axions constitute only a fraction of the dark matter has been limited to only a few observational probes. In this work, we use the galaxy cluster number counts obtained from the first All-Sky Survey (eRASS1) of the SRG/eROSITA mission together with gravitational weak lensing data from the Dark Energy Survey, the Kilo-Degree Survey, and the Hyper Suprime-Cam to constrain the fraction of ultralight axions in the mass range 10 −32 eV to 10 −24 eV. We put upper bounds on the ultralight axion relic density Ω a in independent logarithmic axion mass bins by performing a full cosmological parameter inference. We find an exclusion region in the intermediate ultralight axion mass regime with the tightest bounds reported so far in the mass bins around m a = 10 −27 eV with Ω a < 0.0035 and m a = 10 −26 eV with Ω a < 0.0079; both are at a 95% confidence level. When combined with cosmic microwave background probes, these bounds are tightened to Ω a < 0.0030 in the m a = 10 −27 eV mass bin and Ω a < 0.0058 in the m a = 10 −26 eV mass bin, with both at a 95% confidence level. This is the first time that constraints on ultralight axions have been obtained using the growth of structure measured by galaxy cluster number counts. These results pave the way for large surveys, which can be utilized to obtain tight constraints on the mass and relic density of ultralight axions with better theoretical modeling of the abundance of halos.

cosmological parameters↗

Counting facilities at the Black Hills Underground Campus

The Black Hills Underground Campus (BHUC) houses a low background counting facility on the 4850’ level of the Sanford Underground Research Facility (SURF) with ~4300 m w.e. of rock overburden. Currently there are five ultra-low-background, high-purity germanium detectors operating inside of a class-1,000 cleanroom at the Davis Campus, with a sixth anticipated to be installed within a year. Here, a robust nitrogen purge system and on-site personnel assistance allow these detectors to run continuously to support groups that need low background counting of materials.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗