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At least 73 records · Page 4

Detailing Cloud Property Feedbacks with a Regime-Based Decomposition

Diagnosing the root causes of cloud feedback in climate models and reasons for inter-model disagreement is a necessary first step in understanding their wide variation in climate sensitivities. Here we bring together two analysis techniques that illuminate complementary aspects of cloud feedback. The first quantifies feedbacks from changes in cloud amount, altitude, and optical depth, while the second separates feedbacks due to cloud property changes within specific cloud regimes from those due to regime occurrence frequency changes. We find that in the global mean, shortwave cloud feedback averaged across ten models comes solely from a positive within-regime cloud amount feedback countered slightly by a negative within-regime optical depth feedback. These within-regime feedbacks are highly uniform: In nearly all regimes, locations, and models, cloud amount decreases and cloud albedo increases with warming. In contrast, global-mean across-regime components vary widely across models but are very small on average. This component, however, is dominant in setting the geographic structure of the shortwave cloud feedback: Thicker, more extensive cloud types increase at the expense of thinner, less extensive cloud types in the extratropics, and vice versa at low latitudes. The prominent negative extratropical optical depth feedback has contributions from both within- and across-regime components, suggesting that thermodynamic processes affecting cloud properties as well as dynamical processes that favor thicker cloud regimes are important. The feedback breakdown presented herein may provide additional targets for observational constraints by isolating cloud property feedbacks within specific regimes without the obfuscating effects of changing dynamics that may differ across timescales.

climate sensitivity↗

Relaxation oscillations and hierarchy of feedbacks in MAPK signaling

We formulated a computational model for a MAPK signaling cascade downstream of the EGF receptor to investigate how interlinked positive and negative feedback loops process EGF signals into ERK pulses of constant amplitude but dose-dependent duration and frequency. A positive feedback loop involving RAS and SOS, which leads to bistability and allows for switch-like responses to inputs, is nested within a negative feedback loop that encompasses RAS and RAF, MEK, and ERK that inhibits SOS via phosphorylation. This negative feedback, operating on a longer time scale, changes switch-like behavior into oscillations having a period of 1hour or longer. Two auxiliary negative feedback loops, from ERK to MEK and RAF, placed downstream of the positive feedback, shape the temporal ERK activity profile but are dispensable for oscillations. Thus, the positive feedback introduces a hierarchy among negative feedback loops, such that the effect of a negative feedback depends on its position with respect to the positive feedback loop. Furthermore, a combination of the fast positive feedback involving slow-diffusing membrane components with slower negative feedbacks involving faster diffusing cytoplasmic components leads to local excitation/global inhibition dynamics, which allows the MAPK cascade to transmit paracrine EGF signals into spatially non-uniform ERK activity pulses.

59 BASIC BIOLOGICAL SCIENCES↗

Sources of Intermodel Spread in the Lapse Rate and Water Vapor Feedbacks

Abstract Sources of intermodel differences in the global lapse rate (LR) and water vapor (WV) feedbacks are assessed using CO2 forcing simulations from 28 general circulation models. Tropical surface warming leads to significant warming and moistening in the tropical and extratropical upper troposphere, signifying a nonlocal, tropical influence on extratropical radiation and feedbacks. Model spread in the locally defined LR and WV feedbacks is pronounced in the Southern Ocean because of large-scale ocean upwelling, which reduces surface warming and decouples the surface from the tropospheric response. The magnitude of local extratropical feedbacks across models and over time is well characterized using the ratio of tropical to extratropical surface warming. It is shown that model differences in locally defined LR and WV feedbacks, particularly over the southern extratropics, drive model variability in the global feedbacks. The cross-model correlation between the global LR and WV feedbacks therefore does not arise from their covariation in the tropics, but rather from the pattern of warming exerting a common control on extratropical feedback responses. Because local feedbacks over the Southern Hemisphere are an important contributor to the global feedback, the partitioning of surface warming between the tropics and the southern extratropics is a key determinant of the spread in the global LR and WV feedbacks. It is also shown that model Antarctic sea ice climatology influences sea ice area changes and southern extratropical surface warming. As a result, model discrepancies in climatological Antarctic sea ice area have a significant impact on the intermodel spread of the global LR and WV feedbacks.

54 ENVIRONMENTAL SCIENCES↗

The Atlantic Meridional Overturning Circulation’s Response to CO2 Increase: Assessing the Roles of Surface Flux and Oceanic Advection Feedbacks

Abstract The Atlantic meridional overturning circulation (AMOC) is projected to slow down in climate models due to greenhouse gas emissions. However, the physical mechanisms determining the rate of the projected AMOC slowdown remain unclear. Accordingly, this study isolates the roles of oceanic advection and surface flux feedbacks that might accelerate or decelerate the AMOC’s weakening using carbon dioxide (CO 2 ) quadrupling simulations in the CESM1.2 model. Surface flux feedbacks are isolated in partially coupled experiments in which either all surface flux components or the momentum flux responses to AMOC’s weakening that might provide feedback are suppressed, while a tracer decomposition of ocean density anomalies isolates the advection feedbacks. Comparing the ocean density components in the experiments shows that the AMOC’s response is initially determined by CO 2 -induced anomalous surface heat fluxes, and afterward, feedbacks determine its response. In the fully coupled case, surface heat flux feedback strongly promotes AMOC slowdown and causes its near shutdown, while a weaker but active AMOC is maintained when the surface flux feedback is inhibited in the partially coupled case. The positive surface heat flux feedback works by canceling out the negative oceanic heat advection feedback on deep-water formation in the subpolar North Atlantic (SPNA). With the heat advection feedback thus reduced, the positive salinity advection feedback becomes the dominant contributor to SPNA density changes and deep-water formation. In the partially coupled case, negative ocean heat advection feedback and the CO 2 -induced subtropical Atlantic saline anomalies imported into the SPNA play a stabilizing role. The results highlight the importance of SPNA salinity gradients and gyre circulation strength in determining the AMOC’s response rate or recovery.

54 ENVIRONMENTAL SCIENCES↗

Feedback Control of Plasma Instabilities with Charged Particle Beams and Study of Plasma Turbulence

A new non-perturbing technique for feedback control of plasma instabilities has been developed in the Columbia Linear Machine (CLM). The feedback control scheme involves the injection of a feedback modulated ion beam as a remote suppressor. The ion beam was obtained from a compact ion beam source which was developed for this purpose. A Langmuir probe was used as the feedback sensor. The feedback controller consisted of a phase-shifter and amplifiers. This technique was demonstrated by stabilizing various plasma instabilities to the background noise level, like the trapped particle instability, the ExB instability and the ion-temperature-gradient (ITG) driven instability. An important feature of this scheme is that the injected ion beam is non-perturbing to the plasma equilibrium parameters. The robustness of this feedback stabilization scheme was also investigated. The principal result is that the scheme is fairly robust, tolerating about 100% variation about the nominal parameter values. Next, this scheme is extended to the unsolved general problem of controlling multimode plasma instabilities simultaneously with a single sensor-suppressor pair. A single sensor-suppressor pair of feedback probes is desirable to reduce the perturbation caused by the probes. Two plasma instabilities the ExB and the ITG modes, were simultaneously stabilized. A simple 'state' feedback type method was used where more state information was generated from the single sensor Langmuir probe by appropriate signal processing, in this case, by differentiation. This proof-of-principle experiment demonstrated for the first time that by designing a more sophisticated electronic feedback controller, many plasma instabilities may be simultaneously controlled. Simple theoretical models showed generally good agreement with the feedback experimental results. On a parallel research front, a better understanding of the saturated state of a plasma instability was sought partly with the help of feedback. A plasma instability is usually observed in its saturated state and appears as a single feature in the frequency spectrum with a single azimuthal and parallel wavenumbers. The physics of the non-zero spectral width was investigated in detail because the finite spectral width can cause "turbulent" transport. One aspect of the "turbulence" was investigated by obtaining the scaling of the linear growth rate of the instabilities with the fluctuation levels. The linear growth rates were measured with the established gated feedback technique. The research showed that the ExB instability evolves into a quasi-coherent state when the fluctuation level is high. The coherent aspects were studied with a bispectral analysis. Moreover, the single spectral feature was discovered to be actually composed of a few radial harmonics. The radial harmonics play a role in the nonlinear saturation of the instability via three-wave coupling.

Tham, Philip Kin-Wah↗

Assessing Global and Local Radiative Feedbacks Based on AGCM Simulations for 1980–2014/2017

In order to avoid contamination of unobservable and uncertain effective radiative forcing (ERF) on the diagnosis of radiative feedbacks based on short-term climate variability, we verify the Kernel-Gregory feedback calculation method using atmospheric model experiments with prescribed ERF. We show that both clear-sky radiative fluxes and all-sky radiative feedbacks have a closure between model simulations and kernel derivations. A near-zero global mean net cloud feedback is found in the simulation with prescribed ERF, which results in a more negative global net climate feedback, -2 W m -2 K -1 . Consistent with AMIP6 ensemble mean results, the lapse rate feedback is the largest contributor among all feedbacks to temperature amplification over the three poles (Arctic, Antarctic and Tibetan Plateau), followed by surface albedo feedback and Planck feedback deviation from its global mean. Except for the higher surface albedo feedback in the Antarctic, other feedbacks are almost same between the Arctic and Antarctic.

54 ENVIRONMENTAL SCIENCES↗

Evaluating Cloud Feedback Components in Observations and Their Representation in Climate Models

This study quantifies the contribution of individual cloud feedbacks to the total short-term cloud feedback in satellite observations over the period 2002–2014 and evaluates how they are represented in climate models. The observed positive total cloud feedback is primarily due to positive high-cloud altitude, extratropical high- and low-cloud optical depth, and land cloud amount feedbacks partially offset by negative tropical marine low-cloud feedback. Seventeen models from the Atmosphere Model Intercomparison Project of the sixth Coupled Model Intercomparison Project are analyzed. The models generally reproduce the observed moderate positive short-term cloud feedback. However, compared to satellite estimates, the models are systematically high-biased in tropical marine low-cloud and land cloud amount feedbacks and systematically low-biased in high-cloud altitude and extratropical high- and low-cloud optical depth feedbacks. Errors in modeled short-term cloud feedback components identified in this analysis highlight the need for improvements in model simulations of the response of high clouds and tropical marine low clouds. Our results suggest that skill in simulating interannual cloud feedback components may not indicate skill in simulating long-term cloud feedback components.

58 GEOSCIENCES↗

Calculation of top-of-atmosphere, surface and atmospheric cloud radiative kernels and feedbacks based on ISCCP-H datasets

This study aims to create observation-based cloud radiative kernel (CRK) datasets and evaluate them by direct comparison of CRK and the CRK-derived cloud feedback datasets. Based on the International Satellite Cloud Climatology Project (ISCCP) H datasets, we calculate CRKs (called FH CRKs) as 2D joint function/histogram of cloud optical depth and cloud top pressure for shortwave, longwave, and their sum, Net, at the top of atmosphere (TOA), as well as, for the first time, at the surface (SFC) and in the atmosphere (ATM). The direct comparison shows that FH agrees reasonably well with three other TOA CRK datasets. With cloud fraction change (CFC) datasets of the same histogram for doubled-CO2 simulation from 10 CFMIP1 models, we derive all the TOA, SFC and ATM cloud feedback using the FH CRKs. Our TOA cloud feedback is highly similar to the previous counterparts. Based on the comparison for the 4 CRK datasets and the 10 CFC datasets, we estimate the uncertainty budget for the CRK-derived cloud feedback and show that the CFC-associated uncertainty contributes > 98.5% of the total cloud feedback uncertainty while CRK’s is very small. Our preliminary evaluation shows that some near-zero/small cloud feedback in the TOA-alone feedback indeed results from the compensation of sizable cloud feedback of the SFC and ATM feedback, demonstrating that they help reveal some significant surface and atmospheric cloud feedback whose sum appears insignificant in TOA-alone feedback

cloud radiative kernel (CRK) datasets↗

Insights from a refined decomposition of cloud feedbacks

Decomposing cloud feedback into components due to changes in several gross cloud properties provides valuable insights into its physical causes. Here we present a refined decomposition that separately considers changes in free tropospheric and low cloud properties, better connecting feedbacks to individual governing processes and avoiding ambiguities present in a commonly used decomposition. It reveals that three net cloud feedback components are robustly nonzero: positive feedbacks from increasing free tropospheric cloud altitude and decreasing low cloud cover and a negative feedback from increasing low cloud optical depth. Low cloud amount feedback is the dominant contributor to spread in net cloud feedback but its anticorrelation with other components damps overall spread. Furthermore, the ensemble mean free tropospheric cloud altitude feedback is roughly 60% as large as the standard cloud altitude feedback because it avoids aliasing in low cloud reductions. Implications for the “null hypothesis” climate sensitivity from well-understood and robustly simulated feedbacks are discussed.

54 ENVIRONMENTAL SCIENCES↗

Personalized Feedback on Staff Dose in Fluoroscopy-Guided Interventions: A New Era in Radiation Dose Monitoring

PurposeRadiation safety and protection are a key component of fluoroscopy-guided interventions. We hypothesize that providing weekly personal dose feedback will increase radiation awareness and ultimately will lead to optimized behavior. Therefore, we designed and implemented a personalized feedback of procedure and personal doses for medical staff involved in fluoroscopy-guided interventions.Materials and MethodsMedical staff (physicians and technicians, n = 27) involved in fluoroscopy-guided interventions were equipped with electronic personal dose meters (PDMs). Procedure dose data including the dose area product and effective doses from PDMs were prospectively monitored for each consecutive procedure over an 8-month period (n = 1082). A personalized feedback form was designed displaying for each staff individually the personal dose per procedure, as well as relative and cumulative doses. This study consisted of two phases: (1) 1–5th months: Staff did not receive feedback (n = 701) and (2) 6–8th months: Staff received weekly individual dose feedback (n = 381). An anonymous evaluation was performed on the feedback and occupational dose.ResultsPersonalized feedback was scored valuable by 76% of the staff and increased radiation dose awareness for 71%. 57 and 52% reported an increased feeling of occupational safety and changing their behavior because of personalized feedback, respectively. For technicians, the normalized dose was significantly lower in the feedback phase compared to the prefeedback phase: [median (IQR) normalized dose (phase 1) 0.12 (0.04–0.50) µSv/Gy cm{sup 2} versus (phase 2) 0.08 (0.02–0.24) µSv/Gy cm{sup 2}, p = 0.002].ConclusionPersonalized dose feedback increases radiation awareness and safety and can be provided to staff involved in fluoroscopy-guided interventions.

61 RADIATION PROTECTION AND DOSIMETRY↗

Low-Cloud Feedbacks from Cloud-Controlling Factors: A Review

Abstract The response to warming of tropical low-level clouds including both marine stratocumulus and trade cumulus is a major source of uncertainty in projections of future climate. Climate model simulations of the response vary widely, reflecting the difficulty the models have in simulating these clouds. These inadequacies have led to alternative approaches to predict low-cloud feedbacks. Here, we review an observational approach that relies on the assumption that observed relationships between low clouds and the “cloud-controlling factors” of the large-scale environment are invariant across time-scales. With this assumption, and given predictions of how the cloud-controlling factors change with climate warming, one can predict low-cloud feedbacks without using any model simulation of low clouds. We discuss both fundamental and implementation issues with this approach and suggest steps that could reduce uncertainty in the predicted low-cloud feedback. Recent studies using this approach predict that the tropical low-cloud feedback is positive mainly due to the observation that reflection of solar radiation by low clouds decreases as temperature increases, holding all other cloud-controlling factors fixed. The positive feedback from temperature is partially offset by a negative feedback from the tendency for the inversion strength to increase in a warming world, with other cloud-controlling factors playing a smaller role. A consensus estimate from these studies for the contribution of tropical low clouds to the global mean cloud feedback is 0.25 ± 0.18 W m −2 K −1 (90% confidence interval), suggesting it is very unlikely that tropical low clouds reduce total global cloud feedback. Because the prediction of positive tropical low-cloud feedback with this approach is consistent with independent evidence from low-cloud feedback studies using high-resolution cloud models, progress is being made in reducing this key climate uncertainty.

58 GEOSCIENCES↗

Examining Cloud Feedback Components in the Simple Cloud-Resolving E3SM Atmosphere Model (SCREAM)

Cloud feedback remains the main source of uncertainty in climate sensitivity estimated by global climate models (GCMs), largely because subgrid cloud responses are parameterized in GCMs due to their coarse resolution. Here, this study examines cloud feedback in the global 3.25-km Simple Cloud-Resolving Energy Exascale Earth System Model (E3SM) Atmosphere Model (SCREAM 3 km) through a pair of 1-yr atmosphere-only simulations with control and +4-K sea surface temperature perturbations. SCREAM 3 km produces a positive cloud feedback that falls within but at the upper end of the range of Coupled Model Intercomparison Project phase 5 (CMIP5) and CMIP phase 6 (CMIP6) models and expert judgment. The positive cloud feedback arises from positive contributions from both high- and low-level clouds, with increases in high-cloud altitude and decreases in low-cloud amount and optical depth playing key roles. The stronger-than-CMIP-average feedback is mainly attributable to the high-cloud altitude feedback, owing to cloud tops rising nearly isothermally in SCREAM 3 km. The positive low-cloud amount feedback is weaker in SCREAM than in GCMs because estimated inversion strength (EIS) increases more dramatically with warming. A coarser 12-km resolution version of SCREAM exhibits a weaker positive cloud feedback than SCREAM 3 km, mainly because its low-cloud-radiative flux is more sensitive to EIS, leading to a stronger negative low-cloud amount feedback. With this process-level assessment of cloud feedback, this study reveals where SCREAM aligns with and diverges from conventional GCMs and expert assessment, providing insights to inform further model improvement and future expert assessment.

Cloud radiative effects↗

ENSO Disrupts Boreal Winter CRE Feedback

Twenty years of satellite-based cloud and radiation observations allow us to examine the observed cloud radiative effect (CRE) feedback (i.e., CRE change per unit change in global mean surface temperature). By employing a decomposition method to separate the contribution of “internal changes” and “relative-frequency-of-occurrence (RFO) changes” of distinct cloud regime (CR) groups, notable seasonal contrasts of CRE feedback characteristics emerge. Boreal winter CRE feedback is dominated by the positive shortwave CRE (SWCRE) feedback of oceanic low-thick clouds, due to their decreasing RFO as temperature rises. This signal is most likely due to El Niño-Southern Oscillation (ENSO) activity. When ENSO signals are excluded, boreal winter CRE feedback becomes qualitatively similar to the boreal summer feedback, where several CR groups contribute to the total CRE feedback more evenly. Most CR groups’ CRE feedbacks largely come from changing RFO: e.g., the predominant transition from oceanic cumulus to broken clouds and more occurrences of higher convective clouds with warming temperature. At the same time, low-thick and broken clouds experience optical thinning and decreasing cloud fraction, and these features are more prominent in boreal summer than winter. Overall, the seasonally asymmetric patterns of CRE feedback, primarily due to ENSO, introduce complexity in assessments of CRE feedback.

ENSO↗

Mesoscale system feedback-induced dissipation and noise suppression

A high-gain and low-noise negative feedback control (“feedback control”) system can detect charge transfer in quantum systems at room temperatures. The feedback control system can attenuate dissipative coupling between a quantum system and its thermodynamic environment. The feedback control system can be integrated with standard commercial voltage-impedance measurement system, for example, a potentiostat. In one aspect, the feedback control system includes a plurality of electrodes that are configured to electrically couple to a sample, and a feedback mechanism coupled to a first electrode of the plurality of electrodes. The feedback mechanism is configured to detect a potential associated with the sample via the first electrode. The feedback mechanism provides a feedback signal to the sample via a second electrode of the plurality of electrodes, the feedback signal is configured to provide excitation control of the sample at a third electrode of the plurality of electrode.

Gupta, Chaitanya↗

Decomposing Cloud Radiative Feedbacks by Cloud-Top Phase

Changes in cloud scattering properties and emissivity that arise from atmospheric warming cause substantial radiative feedbacks in model projections of anthropogenic climate change, and the relative importance of the underlying mechanisms is poorly understood. One leading hypothesis is that ice-to-liquid conversions cause clouds to optically thicken, producing a major negative feedback. We test this hypothesis by developing a method to decompose cloud radiative feedbacks by cloud-top phase. The method is applied to an ensemble of six state-of-the-art global climate models run with prescribed sea surface temperature. In these simulations, the global mean of the net cloud scattering and emissivity feedback from cloud-phase conversions ranges from −0.17 to −0.01 W m −2 K −1 , while the overall net cloud feedback ranges from 0.02 to 0.91 W m −2 K −1 . The multimodel mean of the cloud scattering and emissivity feedback from cloud-phase conversions is approximately 19% of the magnitude of the multimodel mean of the overall cloud feedback (−0.10 vs 0.52 W m −2 K −1 ). These results indicate that cloud-phase conversions cause a robust negative feedback by changing cloud scattering and emissivity, but this mechanism makes a modest contribution to the overall cloud feedback at the global scale.

Climate change↗

Evaluating Climate Models’ Cloud Feedbacks Against Expert Judgment

Abstract The persistent and growing spread in effective climate sensitivity (ECS) across global climate models necessitates rigorous evaluation of their cloud feedbacks. Here we evaluate several cloud feedback components simulated in 19 climate models against benchmark values determined via an expert synthesis of observational, theoretical, and high‐resolution modeling studies. We find that models with smallest feedback errors relative to these benchmark values generally have moderate total cloud feedbacks (0.4–0.6 W m −2 K −1 ) and ECS (3–4 K). Those with largest errors generally have total cloud feedback and ECS values that are too large or too small. Models tend to achieve large positive total cloud feedbacks by having several cloud feedback components that are systematically biased high rather than by having a single anomalously large component, and vice versa. In general, better simulation of mean‐state cloud properties leads to stronger but not necessarily better cloud feedbacks. The Python code base provided herein could be applied to developmental versions of models to assess cloud feedbacks and cloud errors and place them in the context of other models and of expert judgment in real‐time during model development.

58 GEOSCIENCES↗

Deterministic generation of remote entanglement with active quantum feedback

We develop and study protocols for deterministic remote entanglement generation using quantum feedback, without relying on an entangling Hamiltonian. In order to formulate the most effective experimentally feasible protocol, we introduce the notion of average-sense locally optimal feedback protocols, which do not require real-time quantum state estimation, a difficult component of real-time quantum feedback control. We use this notion of optimality to construct two protocols that can deterministically create maximal entanglement: a semiclassical feedback protocol for low-efficiency measurements and a quantum feedback protocol for high-efficiency measurements. The latter reduces to direct feedback in the continuous-time limit, whose dynamics can be modeled by a Wiseman-Milburn feedback master equation, which yields an analytic solution in the limit of unit measurement efficiency. Our formalism can smoothly interpolate between continuous-time and discrete-time descriptions of feedback dynamics and we exploit this feature to derive a superior hybrid protocol for arbitrary nonunit measurement efficiency that switches between quantum and semiclassical protocols. Lastly, we show using simulations incorporating experimental imperfections that deterministic entanglement of remote superconducting qubits may be achieved with current technology using the continuous-time feedback protocol alone.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Spectral Signatures of Moisture–Convection Feedbacks over the Indian Ocean

Abstract Positive feedbacks between the cloud population and the environmental moisture field are central to theoretical expositions on the Madden–Julian oscillation (MJO). This study investigates the statistical incidence of positive moisture–convection feedbacks across multiple space and time scales over the tropical Indian Ocean. This work uses vertically integrated moisture budget terms from the ECMWF interim reanalysis [ERA-Interim (ERA-I)] in a framework proposed by Hannah et al. Positive moisture–convection feedbacks are primarily a low-frequency, low-wavenumber phenomenon with significant spectral signatures in the 32–48-day time scale. The efficacy of these feedbacks, however, is subject to horizontal moisture advection variations, whose relative importance varies with scale. Wave-filtered Tropical Rainfall Measuring Mission (TRMM) satellite precipitation is used to show that these moisture–convection feedbacks contribute more to moisture increases in the MJO than in other equatorial waves. A moving-window correlation analysis suggests that instances of moisture–convection feedbacks are more frequent in drier conditions, when column water vapor (CWV) is below its climatological mean value, with the implication that positive moisture–convection feedbacks shape the mean CWV field by moistening drier air columns, but that they are less effective in moistening already moist environments. Ground radar observations show that stratiform rain damps local CWV increases on short time scales (<2 days) and therefore precludes positive moisture–convection feedbacks in high-CWV environments. Vertical coherence structures from ERA-I confirm that relatively bottom-heavy cloud ensembles (i.e., peaks between 700 and 850 hPa) are more effective in inducing low-frequency positive moisture–convection feedbacks than ensembles with other vertical structures. Low-frequency horizontal advective drying damps moisture increases and is strongly coherent with upper-level rising motion.

54 ENVIRONMENTAL SCIENCES↗