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At least 73 records · Page 4

Intensity and polarization of light scattered by size distributions of randomly oriented nonspherical particles

Calculations of light scattering by small particles are important in many diverse fields of science and engineering. In many cases of practical interest, scattering particles are nonspherical and are distributed over sizes and orientations. However, accurate light scattering computations for ensembles of nonspherical particles are difficult and time-consuming, and the literature in which such calculations are reported is rather scarce. In this paper, the T-matrix approach, as extended recently to randomly oriented particles, is used to calculate rigorously light scattering by size distributions of randomly oriented axially symmetric particles. To model the variation of particle sizes in real ensembles, we use a power law distribution typical of some terrestrial aerosols. Contour plots of intensity and degree of linear polarization for polydisperse prolate and oblate spheroids of different aspect ratios and effective equivalent-sphere size parameters from 0 to 10 are calculated and compared with calculations for equivalent spheres. The angular scattering behavior of nonspherical polydispersions is found to be greatly different from that of spheres, while the scattering properties of oblate and prolate spheroids of the same aspect ratio are similar. With increasing particle size, both intensity and polarization become more shape-dependent. In general, nonspherical particles are stronger side scatterers and weaker backscatterers than equivalent spheres. With increasing aspect ratio of nonspherical particles polarization tends to be predominantly positive. Possible effects of particle nonsphericity on optical remote sensing of atmospheric aerosols are discussed.

Mishchenko, M. I.↗

Nonuniform Absorption and Scattered Light in Direct-Drive Implosions Driven by Polarization Smoothing

Laser-direct-drive symmetric implosions on OMEGA illuminate a target with 60 laser beams and are designed to produce spherical implosions. Each beam is smoothed using orthogonal polarizations obtained by passing through distributed polarization rotators (DPR’s). Observations of the scattered light from OMEGA implosions do not show the expected symmetry and have much larger variation than standard predictions. For the first time, we have quantified the scattered-light nonuniformity from individual beams and identified the DPR’s as the source of the enhanced nonuniformity. An instrument was invented that isolated and measured the variation in the intensity and polarization of the light scattered from each OMEGA beam. The asymmetric intensity and polarization measurements are explained when the on-target offsets between the two orthogonal polarizations produced by the DPR’s are modeled using a 3-D cross-beam energy transfer (CBET) code that tracks the polarizations of each beam. The time-integrated nonuniformity in laser absorption and scattered light due to CBET and the DPR polarization offsets during high-performance OMEGA implosions is predicted to be significant and dominated by low spherical harmonic mode numbers. Further, the nonuniformity is predicted to be greatly reduced by replacing the DPR’s with new optics that create smaller offsets.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Multiple-Fiber-Optic Probe For Light-Scattering Measurements

Multiple-fiber-optical probe developed for use in measuring light scattered at various angles from specimens of materials. Designed for both static and dynamic light-scattering measurements of colloidal dispersions. Probe compact, rugged unit containing no moving parts and remains stationary during operation. Not restricted to operation in controlled, research-laboratory environment. Positioned inside or outside light-scattering chamber. Provides simultaneous measurements at small angular intervals over range of angles, made to include small scattering angles by orienting probe in appropriate direction.

Dhadwal, Harbans Singh↗

Laser light scattering as a probe of fractal colloid aggregates

The extensive use of laser light scattering is reviewed, both static and dynamic, in the study of colloid aggregation. Static light scattering enables the study of the fractal structure of the aggregates, while dynamic light scattering enables the study of aggregation kinetics. In addition, both techniques can be combined to demonstrate the universality of the aggregation process. Colloidal aggregates are now well understood and therefore represent an excellent experimental system to use in the study of the physical properties of fractal objects. However, the ultimate size of fractal aggregates is fundamentally limited by gravitational acceleration which will destroy the fractal structure as the size of the aggregates increases. This represents a great opportunity for spaceborne experimentation, where the reduced g will enable the growth of fractal structures of sufficient size for many interesting studies of their physical properties.

Weitz, David A.↗

A global model–measurement evaluation of particle light scattering coefficients at elevated relative humidity

The uptake of water by atmospheric aerosols has a pronounced effect on particle light scattering properties, which in turn are strongly dependent on the ambient relative humidity (RH). Earth system models need to account for the aerosol water uptake and its influence on light scattering in order to properly capture the overall radiative effects of aerosols. Here we present a comprehensive model–measurement evaluation of the particle light scattering enhancement factor f(RH), defined as the particle light scattering coefficient at elevated RH (here set to 85 %) divided by its dry value. The comparison uses simulations from 10 Earth system models and a global dataset of surface-based in situ measurements. In general, we find a large diversity in the magnitude of predicted f(RH) amongst the different models, which can not be explained by the site types. Based on our evaluation of sea salt scattering enhancement and simulated organic mass fraction, there is a strong indication that differences in the model parameterizations of hygroscopicity and model chemistry are driving at least some of the observed diversity in simulated f(RH). Additionally, a key point is that defining dry conditions is difficult from an observational point of view and, depending on the aerosol, may influence the measured f(RH). The definition of dry also impacts our model evaluation, because several models exhibit significant water uptake between RH = 0 % and 40 %. The multisite average ratio between model outputs and measurements is 1.64 when RH = 0 % is assumed as the model dry RH and 1.16 when RH = 40 % is the model dry RH value. The overestimation by the models is believed to originate from the hygroscopicity parameterizations at the lower RH range which may not implement all phenomena taking place (i.e., not fully dried particles and hysteresis effects). This will be particularly relevant when a location is dominated by a deliquescent aerosol such as sea salt. Our results emphasize the need to consider the measurement conditions in such comparisons and recognize that measurements referred to as dry may not be dry in model terms. Recommendations for future model–measurement evaluation and model improvements are provided.

54 ENVIRONMENTAL SCIENCES↗

Protein crystal nucleation kinetics using relative light-scattering techniques: Center director's discretionary fund

Light-scattering intensity measurements are a sensitive method for following changes in the hydrodynamic radius of particles in solution. The approach used in this report utilizes the light-scattering intensity ratios of a polydisperse to a monodisperse system. By numerically modeling the process, and fitting the model curves to the data, estimates have been obtained for the dimerization equilibrium constant, the dimer + dimer yields tetramer equilibrium constant, and the association rate constant for the dimerization process.

Pusey, Marc Lee↗

In-situ qualification and physics-based process design for aerosol jet printing via spatially correlated light scattering measurements

Aerosol jet printing is a contactless, digital, and additive technique broadly used for manufacturing flexible, hybrid, and conformal electronics. However, batch-to-batch variability has hindered widespread industry adoption and scaling to production volumes. Recently, light scattering measurements have emerged as a tool to measure aerosol volume fraction – a key parameter determining deposition rate – and have proven an effective feedback source for closed loop control on timescales ranging from minutes to hours. Here, the efficacy of light scattering measurements as a tool for in-situ qualification over shorter time durations is explored. To be the linear relationship between light scattering measurements and deposition rate was validated at 500 ms time intervals, allowing deposition rate to be mapped to positional coordinates and providing a new data stream to drive quality control assessments. Because light scattering measurements are indicative of a physical process parameter, they were substituted into equations for resistance and sheet resistance, resulting in predictions nominally within 10% of measured values for sets of printed devices. Finally, to highlight a more active utility, light scattering measurements were employed in a print repair framework, successfully repairing prints with randomly induced defects to within 5% of the measured resistance of a control set.

36 MATERIALS SCIENCE↗

Development of a versatile laser light scattering instrument

A versatile laser light scattering (LLS) instrument is developed for use in microgravity to measure microscopic particles of 30 A to above 3 microns. Since it is an optical technique, LLS does not affect the sample being studied. A LLS instrument built from modules allows several configurations, each optimized for a particular experiment. The multiangle LLS instrument can be mounted in the rack in the Space Shuttle and on Space Station Freedom. It is possible that a Space Shuttle glove-box and a lap-top computer containing a correlator card can be used to perform a number of experiments and to demonstrate the technology needed for more elaborate investigations. This offers simple means of flying a great number of experiments without the additional requirements of full-scale flight hardware experiments.

Meyer, William V.↗

Scattered light in the echelle modes of the Goddard high-resolution spectrograph aboard the Hubble Space Telescope. I - Analysis of prelaunch calibration data

A study of scattered light in the echelle mode of the Goddard high-resolution spectrograph (GHRS), one of the first-generation science instruments aboard the Hubble Space Telescope, is reported. The data analyzed are from the GHRS ground-based test program and include observations with the 500 channel Digicon detectors through the small science aperture of UV emission-line sources, continuum sources, and continuum sources viewed through molecular absorption cells. The two largest contributors to scattered light are the echelle and cross-disperser, the effects of which have been quantified. A computer simulation using the derived scattering functions demonstrates that the combined effects of these sources of scattered light adequately explain the observed level of interorder light when viewing UV continuum sources. Observing strategies and data reduction algorithms for measuring and removing the effects of the scattered light are discussed.

Cardelli, Jason A.↗

A Layered Debris Disk around M Star TWA 7 in Scattered Light

We have obtained Hubble Space Telescope (HST) coronagraphic observations of the circumstellar disk around M star TWA 7 using the Space Telescope Imaging Spectrograph (STIS) instrument in visible light. Together with archival observations, including HST/NICMOS using the F160W filter and Very Large Telescope/SPHERE at the H-band in polarized light, we investigate the system in scattered light. By studying this nearly face-on system using geometric disk models and Henyey–Greenstein phase functions, we report a new discovery of a tertiary ring and a clump. We identify a layered architecture: three rings, a spiral, and an ≈150 au 2 elliptical clump. The most extended ring peaks at 28 au, and the other components are on its outskirts. Our point-source detection-limit calculations demonstrate the necessity of disk modeling in imaging fainter planets. Morphologically, we witness a clockwise spiral motion, and the motion pattern is consistent with both solid body motion and local Keplerian motion; we also observe underdensity regions for the secondary ring that might result from mean-motion resonance or moving shadows: both call for re-observations to determine their nature. Comparing multi-instrument observations, we obtain blue STIS-NICMOS color, a STIS-SPHERE radial distribution peak difference for the tertiary ring, and a high SPHERE-NICMOS polarization fraction; these aspects indicate that TWA 7 could retain small dust particles. By viewing the debris disk around M star TWA 7 at a nearly face-on vantage point, our study allows for the understanding of such disks in scattered light in both system architecture and dust property.

Debris disks↗

Evaluation of advanced light scattering technology for microgravity experiments

The capabilities of modern light scattering equipment and the uses it might have in studying processes in microgravity are evaluated. Emphasis is on the resolution of polydisperse systems. This choice was made since a major use of light scattering was expected to be the study of crystal growth of macromolecules in low gravity environments. An evaluation of a modern photon correlation spectrometer and a Mie spectrometer is presented.

Fredericks, W. J.↗

Flow Visualization by Elastic Light Scattering in the Boundary Layer of a Supersonic Flow

We demonstrate instantaneous flow visualization of the boundary layer region of a Mach 2.5 supersonic flow over a flat plate that is interacting with an impinging shock wave. Tests were performed in the Unitary Plan Wind Tunnel (UPWT) at NASA Langley Research Center. The technique is elastic light scattering using 10-nsec laser pulses at 532 nm. We emphasize that no seed material of any kind, including water (H2O), is purposely added to the flow. The scattered light comes from a residual impurity that normally exists in the flow medium after the air drying process. Thus, the technique described here differs from the traditional vapor-screen method, which is typically accomplished by the addition of extra H2O vapor to the airflow. The flow is visualized with a series of thin two-dimensional light sheets (oriented perpendicular to the streamwise direction) that are located at several positions downstream of the leading edge of the model. This geometry allows the direct observation of the unsteady flow structure in the spanwise dimension of the model and also allows the indirect observation of the boundary layer growth in the streamwise dimension.

Herring, G. C.↗

DeepGhostBusters: Using Mask R-CNN to Detect and Mask Ghosting and Scattered-Light Artifacts from Optical Survey Images

Wide-field astronomical surveys are often affected by the presence of undesirable reflections (often known as "ghosting artifacts" or "ghosts") and scattered-light artifacts. The identification and mitigation of these artifacts is important for rigorous astronomical analyses of faint and low-surface-brightness systems. However, the identification of ghosts and scattered-light artifacts is challenging due to a) the complex morphology of these features and b) the large data volume of current and near-future surveys. In this work, we use images from the Dark Energy Survey (DES) to train, validate, and test a deep neural network (Mask R-CNN) to detect and localize ghosts and scattered-light artifacts. We find that the ability of the Mask R-CNN model to identify affected regions is superior to that of conventional algorithms and traditional convolutional neural networks methods. We propose that a multi-step pipeline combining Mask R-CNN segmentation with a classical CNN classifier provides a powerful technique for the automated detection of ghosting and scattered-light artifacts in current and near-future surveys.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗