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Contribution of IAEA coordinated research projects to light water reactors advanced technology fuel testing and simulation

The Fukushima-Daiichi accident in 2011 highlighted the pressing need for enhanced design and safety analysis of nuclear fuels, especially under accident conditions in nuclear power plants (NPPs). To address this need, the international nuclear fuel community has developed several concepts of Accident Tolerant and Advanced Technology Fuels (ATFs) for light water reactors. The International Atomic Energy Agency (IAEA), at the request of its Member States, has initiated a series of three Coordinated Research Projects (CRPs) to aid in the development and testing of these ATFs. Further, these projects, known as FUMAC, ACTOF, and ATF-TS, focus on the experimentation and simulation of ATFs under various accident conditions, including design basis accidents and design extension conditions. This paper provides a comprehensive overview of the main activities, as well as the achieved or anticipated results of these three CRPs. The insights and advancements gained from these projects will enable IAEA Member States to further refine nuclear fission technology, thereby contributing to efforts aimed at mitigating climate change.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Light Water Reactor Sustainability Program: Complete the weld campaign on Ni-base irradiated materials using stress improved laser welding including the preliminary weld quality inspections

This report summarizes the most recent welding campaign on irradiated Ni-base alloy 182 and the preliminary weld quality inspections at the Radiochemical Engineering Development Center (REDC). Equipment and capabilities were developed jointly by the U.S. Department of Energy, Office of Nuclear Energy, Light Water Reactor Sustainability Program, the Electric Power Research Institute, Long Term Operations Program (and the Welding and Repair Technology Center), and Oak Ridge National Laboratory. Irradiated nickel alloy 182, with target helium contents of 5 atom parts-per million (appm), 10 appm, and 20 appm, were laser welded in the hot cell successfully. The significant, on-going effort to weld irradiated alloys with high helium concentrations and comprehensively analyze the results will eventually yield validated repair techniques and guidelines for use by the nuclear industry in extending the operational lifetimes of nuclear power plants. This report fulfills the FY 2023 milestone M3LW-22OR0406013, “Complete the weld campaign on Ni base irradiated materials using stress improved laser welding including the preliminary weld quality inspections”.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Analysis of Deformation Mechanisms, Strain Localization, and Fracture in Highly Irradiated Austenitic Steels – Light-Water Reactor Core Materials – via Advanced inSEM Techniques

The present report describes the establishing of an advanced experimental approach – high-resolution digital image correlation or µDIC – for testing miniature irradiated specimens in the ORNL’s Low Activation Materials Development and Analysis (LAMDA) facility. As expected, the µDIC approach will allow for studying strain localization inside grains, for instance, during dislocation channel-grain boundary interaction processes. This information is of high importance for understanding degradation processes in irradiated austenitic steels – in-core materials of Light Water Reactors. The Level 4 report provides a brief introduction, lists materials designated for µDIC testing and delivered in LAMDA this FY, discusses methodical concerns and preliminary observations.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

FeCrAl fuel/clad chemical interaction in light water reactor environments

This article investigates the fuel-cladding chemical interaction (FCCI) behavior of two commercial FeCrAl alloys, APMT composition (Fe-21Cr-5Al-3Mo wt.%) and C35M (Fe-13Cr-5Al-2Mo-0.2Si-0.03Y wt.%), after neutron irradiation. “H-cup” diffusion multiples of FeCrAl alloys and ceramic UO 2 fuel were irradiated at a temperature of ~300 °C to a total estimated burnup of 26 GWd/tHM. Post-irradiation Examination results demonstrate the excellent degradation resistance of FeCrAl alloys as accident tolerant fuel (ATF) cladding materials in light water reactor conditions. The study concludes that there was no irradiation-induced defects observed in either of the two commercial FeCrAl claddings. The formation of amorphous Al/U mixed oxide was observed at the fuel-clad interface, which can serve as a tritium permeation barrier and protect against potential chemical attack from the fuel. Finally, the study attributed the formation of amorphous Al/U mixed oxide to the low temperature and limited time of neutron irradiation. APMT forms more distinct Cr and Cr-Fe intermetallic at the FeCrAl-UO 2 interface than C35M due to the higher bulk Cr:Al ratio.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

New Pulsed Neutron Die-Away Experiments in Light Water

Thermal neutron scattering laws are important data for many nuclear science and engineering applications, especially criticality safety. Recently, pulsed-neutron die-away experiments have been proposed and used as an experiment to validate thermal neutron scattering laws. These experiments involve irradiating a target moderating material with pulses of neutrons from a neutron generator. The physics of thermal scattering greatly affect how the neutron population in the target exponentially decays via absorption and leakage. Herein, we present experimental results from a new pulsed-neutron die-away experiment of light water that was performed at Lawrence Livermore National Laboratory. The experiments were done with cylindrical targets of varying dimensions to modulate the experiment’s sensitivity to thermal scattering and to absorption. We compare the measured integral parameter of the experiment to simulations with MCNP6.2 ® and to past experiments in literature. The integral parameters that were more sensitive to TSLs showed a larger bias. This validation study is known to have errors because the model of the experiment lacks key features about the detectors and neutron generator. These features will be included in the final benchmark evaluation of the experiment which will be submitted to the International Criticality Safety Benchmark Evaluation Project.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Light Water Reactor Sustainability Program: Upgrade of EMRALD to a Modern JavaScript-based Framework

Event Modeling Risk Assessment using Linked Diagrams (EMRALD) is a software tool developed at Idaho National Laboratory for researching the capabilities of dynamic probabilistic risk assessment. It provides a simple interface to represent complex interactions often seen when developing dynamic models. EMRALD can also interface with other applications by modifying inputs, running, and using their results within EMRALD for dynamic and integrated assessment. This report goes over the work performed as part of the Risk-Informed Systems Analysis Pathway under the Light Water Reactor Sustainability program to upgrade the EMRALD software.

97 MATHEMATICS AND COMPUTING↗

Uncertainty Quantification of a Light Water Pulsed-Neutron Die-Away Experiment to Thermal Neutron Scattering Laws

Thermal neutron scattering laws are important nuclear data for many nuclear science and engineering applications. Validation helps to ensure that a thermal neutron scattering law has a high quality and often employs critical benchmarks as integral experiments. Recently, pulsed-neutron die-away benchmarks have been used as an experiment to validate thermal neutron scattering laws. Herein, we evidence how this alternative integral experiment has a high sensitivity to these nuclear data by performing an uncertainty quantification analysis. The analysis randomly sampled the nuclear model parameters associated with hydrogen bound in light water thermal neutron scattering law and sampled other nuclear data that influenced the experiment’s integral parameter (e.g., elastic scattering, absorption in hydrogen and oxygen) from their respective covariance matrices. The thermal neutron scattering law caused an uncertainty in the integral parameter that reached 2.67%, which exceeds by an order of magnitude the uncertainties induced in commonly used thermal solution critical benchmarks. The validation performed here, although limited due to a poor description of the historical experiment, indicated that the ENDF/B-VIII.0 thermal neutron scattering law well predicted the integral parameter. These results motivate further benchmark and validation efforts using pulsed-neutron die-away experiments.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Grizzly Development for Light Water Reactor and Advanced Reactor Applications in Fiscal Year 2021

This report summarizes work performed during Fiscal Year (FY) 2021 at Idaho National Laboratory (INL) for the U.S. Department of Energy’s Nuclear Engineering Advanced Modeling and Simulation (NEAMS) program for the Structural Materials and Chemistry Technical Area in the work package entitled “MS-21IN050106 - Structural Materials - INL.” This effort mainly focused on development and application of capabilities for engineering-scale analysis of nuclear reactor structural components in the Grizzly and BlackBear codes. These efforts include performance improvements and application of models for high-temperature component response, cluster dynamics modeling of precipitation in light water reactor pressure vessel steel, engineering-scale capability development in the areas of concrete simulation and reactor pressure vessel analysis, and preparation for and conducting an independent assessment of the adherence of these codes to software quality standards.

36 MATERIALS SCIENCE↗

Feasibility of Recycling Discharged Microreactor Heavy Metal in Light Water and Sodium-Cooled Fast Reactors: A Neutronics Analysis

Nuclear microreactors (MRs) offer unique advantages, such as rapid deployment, potability, low maintenance requirements, and operational flexibility. Their compact size makes them a promising solution for decentralized power generation, particularly in remote areas, military bases, and disaster-stricken regions. However, MRs face challenges, including unutilized fissile material at the end of life, economic inefficiency, increased heavy metal (HM) waste complicating disposal, and the accumulation of plutonium (Pu) with high 239 Pu concentrations raising proliferation risks. Here, this study investigated the neutronics feasibility of a novel three-stage fuel cycle where discharged HM from MRs is recycled and burned in light water reactors and sodium-cooled fast reactors. This approach converts discharged HM into valuable fuel, enhancing the efficiency of MR deployments while improving the safeguardability of their final waste products. Neutronics analysis demonstrated that the safety characteristics of reactor designs in each stage were minimally impacted by the proposed cycle. For two representative MR designs, a fast-spectrum MR with solid pellet fuel and a thermal-spectrum MR with TRISO (TRi-structural-ISOtropic) fuel compacts, the proposed fuel cycle reduced the uranium disposal mass flow rate by ~60%, decreased the 235 U enrichment of the discharge fuel to ~1 wt%, eliminated plutonium disposal, and increased the cumulative fuel burnup to ~580 gigawatt-day per metric ton of initial heavy metal (GWd/t-iHM) or 60% fissions per initial metal atom. Despite the significant differences between the two MR designs, the performance and infrastructure requirements of the developed fuel cycles were remarkably similar, indicating its generalizability to a broader class of MRs.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Security-by-Design: Light Water Small Modular Reactor

The growing demand for nuclear power is increasing pressure to find solutions to cost prohibitive requirements of both construction and security. Offsite response has been proposed as an option to reduce costs associated with training and maintaining an onsite response force. A previous report explored this option and revealed that security could be provided at the required level, but cost savings was not a result of this methodology. An offsite response strategy required costly active and passive delay barriers to provide sufficient time for responders to muster and deploy to a site in time to interrupt a determined and well-equipped adversary. Also, contrary to the hypothesis, the number of responders required for this strategy exceeded that needed for an onsite response force, as the adversaries could avail themselves of advantageous positions within the facility to repel arriving responders. This report builds upon the previous evaluation by using the same hypothetical light water small modular reactor (LWSMR) facility model, but this time an onsite response strategy was assessed. The goal of this analysis was to show that an onsite response strategy could be implemented effectively at a cost point that removes barriers within the industry at this critical time of growth and development. The assessment of the facility design and response strategy was completed through modeling using Scribe3D© and subsequent scenario analysis over the course of a two-day tabletop exercise. Subject matter experts in nuclear security, nuclear facility design, and response strategy and tactics contributed to the effort to ensure accurate representation of hypothetical scenarios. Several adaptations were made to the layout of the LWSMR based on lessons learned during the first day of scenario analysis. The subsequent design evaluated on the second day proved to provide a robust response posture against a large and well-trained adversary force. This report details the process of the analysis and compares the cost of the final facility design with that of the LWSMR model used for evaluation of offsite response. Ultimately, the results of this effort indicate that, when implemented correctly, an onsite response strategy is the best option from a security and cost perspective.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Modernization of Technical Requirements for Licensing of Advanced Non-Light Water Reactors: Risk-Informed and Performance-Based Evaluation of Defense-in-Depth Adequacy

This document supports the work contained in Nuclear Energy Institute (NEI) 18-04 “Risk-Informed Performance-Based Technology Inclusive Guidance for Advanced Reactor Licensing Basis Development” Revision 0. NEI 18-04 presents a modern, technology-inclusive, risk-informed, and performance-based (TI-RIPB) process for selection of Licensing Basis Events (LBEs); safety classification of structures, systems, and components (SSCs) and associated risk-informed special treatments; and determination of defense-in-depth (DID) adequacy for non-LWRs. The NEI guidance document provides one acceptable means for addressing the aforementioned topics as part of demonstrating a specific design provides reasonable assurance of adequate radiological protection. This report provides the framework and associated methodology guidelines and discussion for establishing, then evaluating, confirming, and documenting the adequacy of defense-in-depth (DID) for advanced non-light-water reactor technologies. It was developed as part of the Licensing Modernization Project led by Southern Company and cost-shared by the United States Department of Energy and has benefited from considerable NRC formal reviews and public workshops. The methodology converts the DID philosophy into a structured process that is implementable, embraces existing United States and international definitions and philosophies of DID that set the foundation for the process. It builds on the DID framework developed in the Department of Energy Next Generation Nuclear Plant Project and earlier works on this subject. The approach to establishing DID adequacy involves the incorporation of DID attributes into the plant capabilities and programmatic elements of DID. The integrated evaluation of DID adequacy includes both quantitative elements to incorporate risk-informed and performance-based (RIPB) considerations and qualitative elements that address uncertainties and limitations in the quantitative models and supporting data. Demonstration of DID adequacy ensures that there are multiple layers of defense for risk-significant challenges to the design and that the plant capabilities and programs that support each layer are provided in a manner that minimizes dependencies among these layers. The focus of this report is assurance of DID adequacy with respect to protection of the public from radiological exposures resulting from accidental releases of radioactive material. While other hazards are not specifically addressed, this methodology is expected to be beneficial for determining DID adequacy for them as well. Risk-informed evaluation of DID considers the integrated performance of all plant SSCs and associated programs to manage daily operational activities, transients, and accidents, including the evaluation of strategies for accident prevention and mitigation. The RIPB LBE scenario methodology used in this evaluation defines the challenges to the plant safety features included in the plant design basis and beyond, and the scope of all deterministic and probabilistic safety evaluations. By examining event sequences across the whole spectrum of LBEs, a systematic assessment of DID can be accomplished.

42 ENGINEERING↗

Comparisons of Nodal diffusion and whole-core transport methods for multiple cycles of a small Light water reacto

As part of a cooperative research and development agreement between the US department of Energy's Oak Ridge National Laboratory and Holtec International subsidiary SMR LLC, core simulator models of the SMR-160, a light water-cooled and -moderated, natural circulation, small modular reactor, were developed and compared. The model results indicate pin-by-pin power histories, critical boron concentration, and other key performance indicators useful for developing multi-cycle core loading patterns. One model uses industry standard nodal methods with a simple thermal-hydraulics solution, and the other uses an advanced deterministic neutronics solver with a coupled subchannel calculation. The goals of the comparison are to provide the reactor designer with a detailed and coupled core physics reference solution, inform the reactor designer of nodal model best practices based on the code-to-code comparison, and set up a workflow for performing subsequent detailed core simulator calculations. The results of this work will be used in the development of coupled neutronic, thermal hydraulic, and fuel performance models for advanced analysis of the SMR-160. (authors)

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Techno-Economic Analysis of Synthetic Fuels Pathways Integrated with Light Water Reactors

The purpose of this work is to identify, model, perform techno-economic analysis, and compare two possible synfuel production routes utilizing CO 2 as the feedstock. Heat from an LWR nuclear plant is integrated wherever possible to positively affect the economics of the LWR by converting power to fuels during times of low grid electricity demand. Process and economic modeling for a conceptual synfuel production plant co-located (or in near proximity) with an LWR is presented, including the cost of CO 2 captured from an ethanol plant, compressed, and transported to the LWR hybrid plant, co-electrolysis of the CO 2 with water in a solid oxide electrolyzing cell (SOEC) system to produce syngas, and thermocatalytic conversion of the syngas to transportation fuel. The hybrid LWR/synfuels plant is assumed to be located within 50–150 miles of an ethanol plant (e.g., located in the midwest region of the United States). Performance and nth-plant economics for the co-electrolysis-based processes are evaluated and compared with biomass-gasification-based technology for the synfuel routes considered. Sensitivity analysis around the price of CO 2 and electricity, two of the major cost drivers, is presented for each case. Consideration of a carbon credit is also included in the sensitivity analysis.

10 SYNTHETIC FUELS↗

Scale and Regionality of Nonelectric Markets for U.S. Nuclear Light Water Reactors

This study assesses existing and potential industries that could conceivably be directly coupled to existing nuclear reactors. The goal is to identify the scale, location, and accessibility of the candidate industrial-product markets, as well as process feedstocks that are available near the plants to establish new industries. For example, CO 2 as a feedstock can be combined with H 2 to produce formic acid (FA), transportation fuels, and lubricants. These new plants can be entirely supported with the heat and electricity provided by a nearby NPP. The potential demand for nonelectric industrial products was assessed by documenting current and possible growth of nonelectricity product markets considered. This assessment used DOE- and industry-supported tools, data, and projections to capture regional industrial market opportunities. Electricity-capacity markets that reward large and reliable generators, such as NPPs, were considered because the electricity market will likely continue to be an important revenue source to NPPs. The key is to balance the needs of energy customers so as to optimize revenue for the affiliated energy customers or partners. In most cases, flexible plant energy delivery and power generation for the grid will require either energy storage or a stock of intermediate products to sustain the industrial customers when the NPP dispatches electricity to the grid. A diverse mix of temperate regions with operating NPPs around the U.S.—representing a variety of operating markets, local generation mix, and seasonal climates—were chosen for this market study. Both current and future market opportunities for candidate industrial-product markets surrounding these NPPs were studied. Figure 2 illustrates the regions chosen for this study. The success of developing nonelectric industrial-product markets as alternative revenue-generating sources for LWRs depends, not only on demand from growing existing markets, such as petroleum refining and NH 3 production, but also on the development of new markets such as light-duty (LD) and heavy-duty (HD) hydrogen FCEVs, synfuels, chemical production, biofuels, metal refining, injection of hydrogen into NG pipelines for gas power-generating units, FA, polymers, and close-coupled industrial heat applications, all of which can significantly increase demand relative to current levels while decarbonizing energy sectors. This study also presents a sample analysis of the economics of hydrogen production in an area of Minnesota, considering the capital and operating costs of a hydrogen plant as well as the local market demand for hydrogen. It includes some assumptions on electricity-grid pricing, showing how hydrogen could be integrated with an NPP and be competitive with the incumbent hydrogen-production process, steam methane reforming (SMR). The objectives of this study include: Provide U.S. NPP operators a robust sampling of the market demand location, scale, and accessibility (including storage and transportation) of the wide variety of industrial-product choices that can be produced using nuclear thermal energy and electricity proximate to a subset of U.S. NPPs to inform the industry of the potential opportunity; show examples and trade-off analyses of how U.S. LWR operators can access these markets, including storage and transportation of industrial products to their intended markets; and present a general analysis example for one industrial product (hydrogen) in one region (Minnesota area), including production, storage, and transportation, to show how nuclear-hybrid integrated energy systems (IESs) could access local markets and improve the profitability of an NPP.

03 NATURAL GAS↗

Light Water Sustainability Program: Optimizing Information Automation Using a New Method Based on System-Theoretic Process Analysis

This report describes the interim progress for research supporting the design and optimization of information automation systems for nuclear power plants. Much of the domestic nuclear fleet is currently focused on modernizing technologies and processes, including transitioning toward digitalization in the control room and elsewhere throughout the plant, along with a greater use of automation, artificial intelligence, robotics, and other emerging technologies. While there are significant opportunities to apply these technologies toward greater plant safety, efficiency, and overall cost-effectiveness, optimizing their design and avoiding potential safety and performance risks depends on ensuring that human-performance-related organizational and technical design issues are identified and addressed. This report describes modeling tools and techniques, based on sociotechnical system theory, to support these design goals and their application in the current research effort. The report is intended for senior nuclear energy stakeholders, including regulators, corporate management, and senior plant management. We have developed and employed a method to design an optimized information automation ecosystem (IAE) based on the systems-theoretic constructs underlying sociotechnical systems theory in general and the Systems-Theoretic Accident Modeling and Processes (STAMP) approach in particular. We argue that an IAE can be modeled as an interactive information control system whose behavior can be understood in terms of dynamic control and feedback relationships amongst the system’s technical and organizational components. Up to this point, we have employed a Causal Analysis based on STAMP (CAST) technique to examine a performance- and safety-related incident at an industry partner’s plant that involved the unintentional activation of an emergency diesel generator. This analysis provided insight into the behavior of the plant’s current information control structure within the context of a specific, significant event. Our ongoing analysis is focused on identifying near-term process improvements and longer-term design requirements for an optimized IAE system. The latter analyses will employ a second STAMP-derived technique, System-Theoretic Process Analysis (STPA). STPA is a useful modeling tool for generating and analyzing actual or potential information control structures. Finally, we have begun modeling plantwide organizational relationships and processes. Organizational system modeling will supplement our CAST and STPA findings and provide a basis for mapping out a plantwide information control architecture. CAST analysis findings indicate an important underlying contributor to the incident under investigation, and a significant risk to information automation system performance, was perceived schedule pressure, which exposed weaknesses in interdepartmental coordination between and within responsible plant organizations and challenged the resilience of established plant processes, until a human caused the initiating event. These findings are discussed in terms of their risk to overall system performance and their implications for information automation system resilience and brittleness. We present two preliminary information automation models. The proactive issue resolution model is a test case of an information automation concept with significant near-term potential for application and subsequent reduction in significant plant events. The IAE model is a more general representation of a broader, plantwide information automation system. From our results, we have generated a set of preliminary system-level requirements and safety constraints. These requirements will be further developed over the remainder of our project in collaboration with nuclear industry subject matter experts and specialists in the technical systems under consideration. Additionally, we will continue to pursue the system analyses initiated in the first part of our effort, with a particular emphasis on STPA as the main tool to identify weak or weakening control structures that affect the resilience of organizations and programs. Our intent is to broaden the scope of the analysis from an individual use case to a related set of use cases (e.g., maintenance tasks, compliance tasks) with similar human-system performance challenges. This will enable more generalized findings to refine the Proactive Issue Resolution and IAE models, as well as their system-level requirements and safety constraints. We will use organizational system modeling analyses to supplement STPA findings and model development. We conclude the report with a set of summary recommendations and an initial draft list of system-level requirements and safety constraints for optimized information automation systems.

99 GENERAL AND MISCELLANEOUS↗