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An Evaluation of the Liquid Cloud Droplet Effective Radius Derived from MODIS, Airborne Remote Sensing, and in Situ Measurements from CAMP2Ex

The cloud drop effective radius (Re) of the drop size distribution derived from passive satellite sensors is a key variable used in climate research. Validation of these satellite products has often taken place under stratiform cloud conditions that favor the assumption of cloud horizontal homogeneity used by the retrieval techniques. However, many studies have noted concerns with respect to significant biases in retrieved Re arising from cloud heterogeneity, for example, in cumulus cloud fields. Here, we examine data collected during the 2019 “Cloud, Aerosol and Monsoon Processes Philippines Experiment” (CAMP2Ex), which, in part, targeted the objective of providing the first detailed evaluation of Re retrieved across multiple platforms and techniques in a cumulus and congestus cloud region. Our evaluation consists of cross-comparisons of Re between the Moderate Resolution Imaging Spectroradiometer (MODIS) onboard the Terra satellite, the Research Scanning Polarimeter (RSP) onboard the NASA P-3 aircraft, and in situ measurements from both the NASA P-3 and Learjet aircraft that are all taken in close spatiotemporal proximity to the same cloud fields. A particular advantage of our approach lies in the capability of the RSP to retrieve Re using a bi-spectral MODIS approach and a polarimetric approach, which allows for the evaluation of bi-spectral and polarimetric Re retrievals from an airborne perspective using the same samples. Averaged over all P-3 flight segments examined here for warm clouds, the RSP polarimetric method, the in situ method, and the bias-adjusted MODIS method of Fu et al. (2019) show a comparable median (mean ± standard deviation) for the Re samples of 9.6 (10.2 ± 4.0) µm, 11.0 (13.6 ± 11.3) µm, and 10.4 (10.8 ± 3.8) µm, respectively. These values are far lower than the values of 15.1 (16.2 ± 5.5) µm and 17.2 (17.7 ± 5.7) µm from the bi-spectral retrievals of RSP and MODIS, respectively. Similar results are observed when Re is segregated by cloud-top height and in detailed case studies. The clouds sampled during CAMP2Ex consist of mostly small (mean transect length ∼ 1.4 km) and low clouds (mean cloud-top height ∼ 1 km), which had more numerous small clouds than the trade wind cumuli sampled in past field campaigns such as Rain in Shallow Cumulus over the Ocean (RICO) and the Indian Ocean Experiment (INDOEX). The overestimates of Re from the RSP bi-spectral technique compared with the polarimetric technique increased as cloud size and cloud optical depth decreased. Drizzle, cloud-top bumpiness, and solar zenith angle, however, are not closely correlated with the overestimate of bi-spectral Re. For shallow clouds that dominated the liquid cloud cover for the CAMP2Ex region and period, we show that 3-D radiative transfer and cloud heterogeneity, particularly for the optically thin and small clouds, appear to be the leading cause of the large positive biases in bi-spectral retrievals. Because this bias varies with the underlying structure of the cloud field, caution continues to be warranted in studies that use bi-spectral Re retrievals in cumulus cloud fields.

Cloud microphysics↗

Comparison of Marine Boundary Layer Cloud Properties from CERES-MODIS Edition 4 and DOE ARM AMF Measurements at the Azores

Marine boundary layer (MBL) cloud properties derived from the NASA Clouds and the Earth's Radiant Energy System (CERES) project using Terra and Aqua Moderate Resolution Imaging Spectroradiometer (MODIS) data are compared with observations taken at the Department of Energy Atmospheric Radiation Measurement (ARM) Mobile Facility at the Azores (AMF-Azores) site from June 2009 through December 2010. Cloud properties derived from ARM ground-based observations were averaged over a 1 h interval centered at the satellite overpass time, while the CERES-MODIS (CM) results were averaged within a 30 km×30 km grid box centered over the Azores site. A total of 63 daytime and 92 nighttime single-layered overcast MBL cloud cases were selected from 19 months of ARM radar-lidar and satellite observations. The CM cloud top/base heights (Htop/Hbase) were determined from cloud top/base temperatures (Ttop/Tbase) using a regional boundary layer lapse rate method. For daytime comparisons, the CM-derived Htop (Hbase), on average, is 0.063 km (0.068 km) higher (lower) than its ARM radar-lidar-observed counterpart, and the CM-derived Ttop and Tbase are 0.9 K less and 2.5 K greater than the surface values with high correlations (R(sup 2) = 0.82 and 0.84, respectively). In general, the cloud top comparisons agree better than the cloud base comparisons, because the CM cloud base temperatures and heights are secondary products determined from cloud top temperatures and heights. No significant day-night difference was found in the analyses. The comparisons of MBL cloud microphysical properties reveal that when averaged over a 30 km× 30 km area, the CM-retrieved cloud droplet effective radius (re) at 3.7 micrometers is 1.3 micrometers larger than that from the ARM retrievals (12.8 micrometers), while the CM-retrieved cloud liquid water path (LWP) is 13.5 gm( exp -2) less than its ARM counterpart (114.2 gm( exp-2) due to its small optical depth (9.6 versus 13.7). The differences are reduced by 50% when the CM averages are computed only using the MODIS pixel nearest the AMF site. Using the effective radius retrieved using 2.1 micrometers channel to calculate LWP can reduce the difference between the CM and ARM microwave radiometer retrievals from 13.7 to 2.1 gm2. The 10% differences between the ARM and CERES-MODIS LWP and r(sub e) retrievals are within the uncertainties of the ARM LWP (approximately 20gm( exp -2)) and r(sub e) (approximately 10%) retrievals; however, the 30% difference in optical depth is significant. Possible reasons contributing to this discrepancy are increased sensitivities in optical depth from both surface retrievals when τ is approximately 10 and topography. The τ differences vary with wind direction and are consistent with the island orography.Much better agreement in τ is obtained when using only those data taken when the wind is from the northeast, where topographical effects on the sampled clouds are minimal.

Xi, Baike↗

A Novel Method for Estimating Shortwave Direct Radiative Effect of Above-Cloud Aerosols Using CALIOP and MODIS Data

This paper describes an efficient and unique method for computing the shortwave direct radiative effect (DRE) of aerosol residing above low-level liquid-phase clouds using CALIOP and MODIS data. It addresses the overlap of aerosol and cloud rigorously by utilizing the joint histogram of cloud optical depth and cloud top pressure while also accounting for subgrid-scale variations of aerosols. The method is computationally efficient because of its use of grid-level cloud and aerosol statistics, instead of pixel-level products, and a pre-computed look-up table based on radiative transfer calculations. We verify that for smoke over the southeast Atlantic Ocean the method yields a seasonal mean instantaneous (approximately 1:30PM local time) shortwave DRE of above cloud aerosol (ACA) that generally agrees with more rigorous pixel-level computation within 4 percent. We also estimate the impact of potential CALIOP aerosol optical depth (AOD) retrieval bias of ACA on DRE. We find that the regional and seasonal mean instantaneous DRE of ACA over southeast Atlantic Ocean would increase, from the original value of 6.4 W m(-2) based on operational CALIOP AOD to 9.6 W m(-2) if CALIOP AOD retrieval are biased low by a factor of 1.5 (Meyer et al., 2013) and further to 30.9 W m(-2) if CALIOP AOD retrieval are biased low by a factor of 5 as suggested in (Jethva et al., 2014). In contrast, the instantaneous ACA radiative forcing efficiency (RFE) remains relatively invariant in all cases at about 53 W m(-2) AOD(-1), suggesting a near linear relation between the instantaneous RFE and AOD. We also compute the annual mean instantaneous shortwave DRE of light-absorbing aerosols (i.e., smoke and polluted dust) over global oceans based on 4 years of CALIOP and MODIS data. We find that the variability of the annual mean shortwave DRE of above-cloud light-absorbing aerosol is mainly driven by the optical depth of the underlying clouds. While we demonstrate our method using CALIOP and MODIS data, it can also be extended to other satellite data sets, as well as climate model outputs.

CALIOP and MODIS↗

A Novel Method for Estimating Shortwave Direct Radiative Effect of Above-Cloud Aerosols Using CALIOP and MODIS Data

This paper describes an efficient and unique method for computing the shortwave direct radiative effect (DRE) of aerosol residing above low-level liquid-phase clouds using CALIOP and MODIS data. It accounts for the overlapping of aerosol and cloud rigorously by utilizing the joint histogram of cloud optical depth and cloud top pressure. Effects of sub-grid scale cloud and aerosol variations on DRE are accounted for. It is computationally efficient through using grid-level cloud and aerosol statistics, instead of pixel-level products, and a pre-computed look-up table in radiative transfer calculations. We verified that for smoke over the southeast Atlantic Ocean the method yields a seasonal mean instantaneous shortwave DRE that generally agrees with more rigorous pixel-level computation within 4. We have also computed the annual mean instantaneous shortwave DRE of light-absorbing aerosols (i.e., smoke and polluted dust) over global ocean based on 4 yr of CALIOP and MODIS data. We found that the variability of the annual mean shortwave DRE of above-cloud light-absorbing aerosol is mainly driven by the optical depth of the underlying clouds.

radiative forcing↗

A Novel Method for Estimating Shortwave Direct Radiative Effect of Above-cloud Aerosols over Ocean Using CALIOP and MODIS Data

This paper describes an efficient and unique method for computing the shortwave direct radiative effect (DRE) of aerosol residing above low-level liquid-phase clouds using CALIOP and MODIS data. It accounts for the overlapping of aerosol and cloud rigorously by utilizing the joint histogram of cloud optical depth and cloud top pressure. Effects of sub-grid scale cloud and aerosol variations on DRE are accounted for. It is computationally efficient through using grid-level cloud and aerosol statistics, instead of pixel-level products, and a pre-computed look-up table in radiative transfer calculations. We verified that for smoke over the southeast Atlantic Ocean the method yields a seasonal mean instantaneous shortwave DRE that generally agrees with more rigorous pixel-level computation within 4%. We have also computed the annual mean instantaneous shortwave DRE of light-absorbing aerosols (i.e., smoke and polluted dust) over global ocean based on 4 yr of CALIOP and MODIS data. We found that the variability of the annual mean shortwave DRE of above-cloud light-absorbing aerosol is mainly driven by the optical depth of the underlying clouds.

CALIOP and MODIS↗

Liquid Water Cloud Measurements Using the Raman Lidar Technique: Current Understanding and Future Research Needs

This paper describes recent work in the Raman lidar liquid water cloud measurement technique. The range-resolved spectral measurements at the National Aeronautics and Space Administration Goddard Space Flight Center indicate that the Raman backscattering spectra measured in and below low clouds agree well with theoretical spectra for vapor and liquid water. The calibration coefficients of the liquid water measurement for the Raman lidar at the Atmospheric Radiation Measurement Program Southern Great Plains site of the U.S. Department of Energy were determined by comparison with the liquid water path (LWP) obtained with Atmospheric Emitted Radiance Interferometer (AERI) and the liquid water content (LWC) obtained with the millimeter wavelength cloud radar and water vapor radiometer (MMCR-WVR) together. These comparisons were used to estimate the Raman liquid water cross-sectional value. The results indicate a bias consistent with an effective liquid water Raman cross-sectional value that is 28%-46% lower than published, which may be explained by the fact that the difference in the detectors' sensitivity has not been accounted for. The LWP of a thin altostratus cloud showed good qualitative agreement between lidar retrievals and AERI. However, the overall ensemble of comparisons of LWP showed considerable scatter, possibly because of the different fields of view of the instruments, the 350-m distance between the instruments, and the horizontal inhomogeneity of the clouds. The LWC profiles for a thick stratus cloud showed agreement between lidar retrievals andMMCR-WVR between the cloud base and 150m above that where the optical depth was less than 3. Areas requiring further research in this technique are discussed.

vapor and liquid water↗

Estimating the Direct Radiative Effect of Absorbing Aerosols Overlying Marine Boundary Layer Clouds in the Southeast Atlantic Using MODIS and CALIOP

Absorbing aerosols such as smoke strongly absorb solar radiation, particularly at ultraviolet and visible/near-infrared (VIS/NIR) wavelengths, and their presence above clouds can have considerable implications. It has been previously shown that they have a positive (i.e., warming) direct aerosol radiative effect (DARE) when overlying bright clouds. Additionally, they can cause biased passive instrument satellite retrievals in techniques that rely on VIS/NIR wavelengths for inferring the cloud optical thickness (COT) and effective radius (re) of underlying clouds, which can in turn yield biased above-cloud DARE estimates. Here we investigate Moderate Resolution Imaging Spectroradiometer (MODIS) cloud optical property retrieval biases due to overlying absorbing aerosols observed by Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) and examine the impact of these biases on above-cloud DARE estimates. The investigation focuses on a region in the southeast Atlantic Ocean during August and September (2006-2011), where smoke from biomass burning in southern Africa overlies persistent marine boundary layer stratocumulus clouds. Adjusting for above-cloud aerosol attenuation yields increases in the regional mean liquid COT (averaged over all ocean-only liquid clouds) by roughly 6%; mean re increases by roughly 2.6%, almost exclusively due to the COT adjustment in the non-orthogonal retrieval space. It is found that these two biases lead to an underestimate of DARE. For liquid cloud Aqua MODIS pixels with CALIOP-observed above-cloud smoke, the regional mean above-cloud radiative forcing efficiency (DARE per unit aerosol optical depth (AOD)) at time of observation (near local noon for Aqua overpass) increases from 50.9Wm(sup-2)AOD(sup-1) to 65.1Wm(sup-2)AOD(sup -1) when using bias-adjusted instead of nonadjusted MODIS cloud retrievals.

aerosols↗

Multilayered Clouds Identification and Retrieval for CERES Using MODIS

Traditionally, analyses of satellite data have been limited to interpreting the radiances in terms of single layer clouds. Generally, this results in significant errors in the retrieved properties for multilayered cloud systems. Two techniques for detecting overlapped clouds and retrieving the cloud properties using satellite data are explored to help address the need for better quantification of cloud vertical structure. The first technique was developed using multispectral imager data with secondary imager products (infrared brightness temperature differences, BTD). The other method uses microwave (MWR) data. The use of BTD, the 11-12 micrometer brightness temperature difference, in conjunction with tau, the retrieved visible optical depth, was suggested by Kawamoto et al. (2001) and used by Pavlonis et al. (2004) as a means to detect multilayered clouds. Combining visible (VIS; 0.65 micrometer) and infrared (IR) retrievals of cloud properties with microwave (MW) retrievals of cloud water temperature Tw and liquid water path LWP retrieved from satellite microwave imagers appears to be a fruitful approach for detecting and retrieving overlapped clouds (Lin et al., 1998, Ho et al., 2003, Huang et al., 2005). The BTD method is limited to optically thin cirrus over low clouds, while the MWR method is limited to ocean areas only. With the availability of VIS and IR data from the Moderate Resolution Imaging Spectroradiometer (MODIS) and MW data from the Advanced Microwave Scanning Radiometer EOS (AMSR-E), both on Aqua, it is now possible to examine both approaches simultaneously. This paper explores the use of the BTD method as applied to MODIS and AMSR-E data taken from the Aqua satellite over non-polar ocean surfaces.

Sun-Mack, Sunny↗

Surface Radiation Budget (SRB) Release 2.5 Longwave cloud props 3 hourly Data in Native Format (SRB_REL2.5_LW_CLDPROPS_3HRLY)

The Surface Radiation Budget (SRB) data set contain 47 surface and cloud properties including cloud fraction, cloud visible optical depth, cloud top temperature, cloud top pressure, cloud base pressure, and cloud water and ice content for each of 5 cloud types and in total. In addition to these cloud properties, the parameters also include surface pressure, total column ozone, day/night flag, and precipitable water. All perameters were measured at three hourly intervals for each day for the entire globe between 07/01/1983 and 06/30/2005 and serve as inputs to the Global Energy and Water-Cycle Experiment (GEWEX) longwave algorithm (GLW). [Location=GLOBAL] [Temporal_Coverage: Start_Date=1998-01-01; Stop_Date=2005-06-30] [Spatial_Coverage: Southernmost_Latitude=-90; Northernmost_Latitude=90; Westernmost_Longitude=-180; Easternmost_Longitude=180] [Data_Resolution: Latitude_Resolution=1 degree; Longitude_Resolution=Ranges from 1 degree (tropics and subtropics) to 120 degrees (the poles).; Temporal_Resolution=3 hourly; Temporal_Resolution_Range=3 hourly].

CLOUD TOP TEMPERATURE↗

Carbon Dioxide Clouds at High Altitude in the Tropics and in an Early Dense Martian Atmosphere

We use a time dependent, microphysical cloud model to study the formation of carbon dioxide clouds in the Martian atmosphere. Laboratory studies by Glandor et al. show that high critical supersaturations are required for cloud particle nucleation and that surface kinetic growth is not limited. These conditions, which are similar to those for cirrus clouds on Earth, lead to the formation of carbon dioxide ice particles with radii greater than 500 micrometers and concentrations of less than 0.1 cm(exp -3) for typical atmospheric conditions. Within the current Martian atmosphere, CO2 cloud formation is possible at the poles during winter and at high altitudes in the tropics during periods of increased atmospheric dust loading. In both cases, temperature perturbations of several degrees below the CO2 saturation temperature are required to nucleate new cloud particles suggesting that dynamical processes are the most common initiators of carbon dioxide clouds rather than diabatic cooling. The microphysical cloud model, coupled to a two-stream radiative transfer model, is used to reexamine the impact of CO2 clouds on the surface temperature within a dense CO2 atmosphere. The formation of carbon dioxide clouds leads to a warmer surface than what would be expected for clear sky conditions. The amount of warming is sensitive to the presence of dust and water vapor in the atmosphere, both of which act to dampen cloud effects. The radiative warming associated with cloud formation, as well as latent heating, work to dissipate the clouds when present. Thus, clouds never last for periods much longer than several days, limiting their overall effectiveness for warming the surface. The time average cloud optical depth is approximately unity leading to a 5-10 K warming, depending on the surface pressure. However, the surface temperature does not rise about the freezing point of liquid water even for pressures as high as 5 bars, at a solar luminosity of 75% the current value.

Colaprete, Anthony↗

A Climatology of Midlatitude Continental Clouds from the ARM SGP Site: Low-Level Cloud Macrophysical, Microphysical, and Radiative Properties - Part I

A record of single-layer and overcast low cloud (stratus) properties has been generated using approximately 4000 hours of data collected from January 1997 to December 2002 at the Atmospheric Radiation Measurement (ARM) Southern Great Plains Central Facility (SCF). The cloud properties include liquid-phase and liquid-dominant, mixed-phase, low cloud macrophysical, microphysical, and radiative properties including cloud-base and -top heights and temperatures, and cloud physical thickness derived from a ground-based radar and lidar pair, and rawinsonde sounding; cloud liquid water path (LWP) and content (LWC), and cloud-droplet effective radius (r(sub e)) and number concentration (N) derived from the macrophysical properties and radiometer data; and cloud optical depth (tau), effective solar transmission (gamma), and cloud/top-of-atmosphere albedos (R(sub cldy)/R(sub TOA)) derived from Eppley precision spectral pyranometer measurements. The cloud properties were analyzed in terms of their seasonal, monthly, and hourly variations. In general, more stratus clouds occur during winter and spring than in summer. Cloud-layer altitudes and physical thicknesses were higher and greater in summer than in winter with averaged physical thicknesses of 0.85 km and 0.73 km for day and night, respectively. The seasonal variations of LWP, LWC, N. tau, R(sub cldy), and R(sub TOA) basically follow the same pattern with maxima and minima during winter and summer, respectively. There is no significant variation in mean r(sub e), however, despite a summertime peak in aerosol loading, Although a considerable degree of variability exists, the 6-yr average values of LWP, LWC, r(sub e), N, tau, gamma, R(sub cldy) and R(sub TOA) are 150 gm(exp -2) (138), 0.245 gm(exp -3) (0.268), 8.7 micrometers (8.5), 213 cm(exp -3) (238), 26.8 (24.8), 0.331, 0.672, 0.563 for daytime (nighttime). A new conceptual model of midlatitude continental low clouds at the ARM SGP site has been developed from this study. The low stratus cloud amount monotonically increases from midnight to early morning (0930 LT), and remains large until around local noon, then declines until 1930 LT when it levels off for the remainder of the night. In the morning, the stratus cloud layer is low, warm, and thick with less LWC, while in the afternoon it is high, cold, and thin with more LWC. Future parts of this series will consider other cloud types and cloud radiative forcing at the ARM SCF.

Dong, Xiquan↗

A Variational Method to Retrieve the Extinction Profile in Liquid Clouds Using Multiple Field-of-View Lidar

While liquid clouds playa very important role in the global radiation budget, it's been very difficult to remotely determine their internal cloud structure. Ordinary lidar instruments (similar to radars but using visible light pulses) receive strong signals from such clouds, but the information is limited to a thin layer near the cloud boundary. Multiple field-of-view (FOV) lidars offer some new hope as they are able to isolate photons that were scattered many times by cloud droplets and penetrated deep into a cloud before returning to the instrument. Their data contains new information on cloud structure, although the lack of fast simulation methods made it challenging to interpret the observations. This paper describes a fast new technique that can simulate multiple-FOV lidar signals and can even estimate the way the signals would change in response to changes in cloud properties-an ability that allows quick refinements in our initial guesses of cloud structure. Results for a hypothetical airborne three-FOV lidar suggest that this approach can help determine cloud structure for a deeper layer in clouds, and can reliably determine the optical thickness of even fairly thick liquid clouds. The algorithm is also applied to stratocumulus observations by the 8-FOV airborne "THOR" lidar. These tests demonstrate that the new method can determine the depth to which a lidar provides useful information on vertical cloud structure. This work opens the way to exploit data from spaceborne lidar and radar more rigorously than has been possible up to now.

Pounder, Nicola L.↗

Cirrus cloud statistics: Temperatures and optical depths

Measurements of the upwelling infrared radiance at 10.5 and 6.5 microns were obtained during the FIRE cirrus Intensive Field Observations using a radiometer with a 15 deg cone nadir field-of-view flown on the NASA Ames ER-2. Data are recorded at a frequency of 1 Hz and the radiometer is continuously calibrated with a liquid nitrogen blackbody source, thereby providing a large number of very accurate radiance values during the course of a several hour flight. For this study, the focus is on the statistical properties of the cirrus deck as deduced from the radiance data. The data acquired on 28 October 1986 is stressed, but some data from the other flights are also shown for comparison purposes.

Valero, Francisco P. J.↗

Assessment of Clear Sky Radiative Forcing in the Caribbean Region Using an Aerosol Dispersion Model and Ground Radiometry During Puerto Rico Dust Experiment

This study investigates the surface and top of the atmosphere solar radiative forcing by long-range transport of Saharan dust. The calculations of radiative forcing are based on measurements collected in the Puerto Rico Dust Experiment (PRIDE) carried out during July, 2000. The purpose of the experiment was the characterization of the Saharan dust plume, which frequently reaches the Caribbean region during the summer. The experiment involved the use of three approaches to study the plume: space and ground based remote sensing, airborne and ground based in-situ measurements and aerosol dispersion modeling. The diversity of measuring platforms provides an excellent opportunity for determination of the direct effect of dust on the clear sky radiative forcing. Specifically, comparisons of heating rates, surface and TOA fluxes derived from the Navy global aerosol dispersion model NAAPS (NRL Aerosol Analysis and Prediction System) and actual measurements of fluxes from ground and space based platforms are shown. In addition, the direct effect of dust on the clear sky radiative forcing is modeled. The extent and time of evolution of the radiative properties of the plume are computed with the aerosol concentrations modeled by NAAPS. Standard aerosol parameterizations, as well as in-situ composition and size distributions measured during PRIDE, are utilized to compute the aerosol optical depth, single scattering albedo and asymmetry factor. Radiative transfer computations are done with an in-house modified spectral radiative transfer code (Fu-Liou). The code includes gas absorption and cloud particles (ice and liquid phase) and it allows the input of meteorological data. The code was modified to include modules for the aerosols contribution to the calculated fluxes. This comparison study helps to narrow the current uncertainty in the dust direct radiative forcing, as recently reported in the 2001 IPCC assessment.

Gasso, Santiago↗

Cloud Thermodynamic Phase Detection with Polarimetrically Sensitive Passive Sky Radiometers

The primary goal of this project has been to investigate if ground-based visible and near-infrared passive radiometers that have polarization sensitivity can determine the thermodynamic phase of overlying clouds, i.e. if they are comprised of liquid droplets or ice particles. While this knowledge is important by itself for our understanding of the global climate, it can also help improve cloud property retrieval algorithms that use total (unpolarized) radiance to determine Cloud Optical Depth (COD). This is a potentially unexploited capability of some instruments in the NASA Aerosol Robotic Network (AERONET), which, if practical, could expand the products of that global instrument network at minimal additional cost. We performed simulations that found, for zenith observations, cloud thermodynamic phase is often expressed in the sign of the Q component of the Stokes polarization vector. We chose our reference frame as the plane containing solar and observation vectors, so the sign of Q indicates the polarization direction, parallel (negative) or perpendicular (positive) to that plane. Since the quantity of polarization is inversely proportional to COD, optically thin clouds are most likely to create a signal greater than instrument noise. Besides COD and instrument accuracy, other important factors for the determination of cloud thermodynamic phase are the solar and observation geometry (scattering angles between 40 and 60 degrees are best), and the properties of ice particles (pristine particles may have halos or other features that make them difficult to distinguish from water droplets at specific scattering angles, while extreme ice crystal aspect ratios polarize more than compact particles). We tested the conclusions of our simulations using data from polarimetrically sensitive versions of the Cimel 318 sun photometerradiometer that comprise AERONET. Most algorithms that exploit Cimel polarized observations use the Degree of Linear Polarization (DoLP), not the individual Stokes vector elements (such as Q). For this reason, we had no information about the accuracy of Cimel observed Q and the potential for cloud phase determination. Indeed, comparisons to ceilometer observations with a single polarized spectral channel version of the Cimel at a site in the Netherlands showed little correlation. Comparisons to Lidar observations with a more recently developed, multi-wavelength polarized Cimel in Maryland, USA, show more promise. This divergence between simulations and observations has prompted us to begin the development of a small test instrument called the Sky Polarization Radiometric Instrument for Test and Evaluation (SPRITE). This instrument is specifically devoted to the accurate observation of Q, and the testing of calibration and uncertainty assessment techniques, with the ultimate goal of understanding the practical feasibility of these measurements.

Knobelspiesse, Kirk D.↗

CIMEL Measurements of Zenith Radiances at the ARM Site

Starting from October 1, 2001, Cimel at the ARM Central Facility in Oklahoma has been switched to a new "cloud mode." This mode allows taking measurements of zenith radiance when the Sun in blocked by clouds. In this case, every 13 min. Cimel points straight up and takes 10 measurements with 9 sec. time interval. The new Cimel's mode has four filters at 440, 670, 870 and 1020 nm. For cloudy conditions, the spectral contrast in surface albedo dominates over Rayleigh and aerosol effects; this makes normalized zenith radiances at 440 and 670 as well as for 870 and 1020 almost indistinguishable. We compare Cimel measurements with other ARM cart site instruments: Multi-Filter Rotating Shadowband Radiometer (MFRSR), Narrow Field of View (NFOV) sensor, and MicroWave Radiometer(MWR). Based on Cimel and MFRSR 670 and 870 nm channels, we build a normalized difference cloud index (NDCI) for radiances and fluxes, respectively. Radiance NDCI from Cimel and flux NDCI from MFRSR are compared between themselves as well as with cloud Liquid Water Path (LWP) retrieved from MWR. Based on our theoretical calculations and preliminary data analysis,there is a good correlation between NDCIs and LWP for cloudy sky above green vegetation. Based on this correlation, an algorithm to retrieve cloud optical depth from NDCI is proposed.

Marshak, Alexander↗

Satellite-based Assessment of Global Warm Cloud Properties Associated with Aerosols, Atmospheric Stability, and Diurnal Cycle

This study examines variability in marine low cloud properties derived from semi-global observations by the Tropical Rainfall Measuring Mission (TRMM) satellite, as linked to the aerosol index (AI) and lower-tropospheric stability (LTS). AI is derived from the Moderate Resolution Imaging Spectroradiometer (Terra MODIS) sensor and the Goddard Chemistry Aerosol Radiation and Transportation (GOCART) model, and is used to represent column-integrated aerosol concentrations. LTS is derived from the NCEP/NCAR reanalysis, and represents the background thermodynamic environment in which the clouds form. Global statistics reveal that cloud droplet size tends to be smallest in polluted (high-AI) and strong inversion (high-LTS) environments. Statistical quantification shows that cloud droplet size is better correlated with AI than it is with LTS. Simultaneously, the cloud liquid water path (CLWP) tends to decrease as AI increases. This correlation does not support the hypothesis or assumption that constant or increased CLWP is associated with high aerosol concentrations. Global variability in corrected cloud albedo (CCA), the product of cloud optical depth and cloud fraction, is very well explained by LTS, while both AI and LTS are needed to explain local variability in CCA. Most of the local correlations between AI and cloud properties are similar to the results from the global statistics, while weak anomalous aerosol-cloud correlations appear locally in the regions where simultaneous high (low) AI and low (high) LTS compensate each other. Daytime diurnal cycles explain additional variability in cloud properties. CCA has the largest diurnal cycle in high-LTS regions. Cloud droplet size and CLWP have weak diurnal cycles that differ between clean and polluted environments. The combined results suggest that investigations of marine low cloud radiative forcing and its relationship to hypothesized aerosol indirect effects must consider the combined effects of aerosols, thermodynamics, and the diurnal cycle.

Matsui, Toshihisa↗

Heat transfer studies on the liquid droplet radiator

This paper examines radiation transfer in the droplet sheet of a liquid droplet radiator including non-isotropic scattering by the droplets. Non-isotropic scattering becomes significant for small droplets (diameter less than 0.1 mm) and for low emissivity liquids. For droplets with an emittance of 0.1 and for a droplet sheet optical depth or 5, the radiated power varies by about 12 percent, depending on whether scattering is predominantly forward or backward. An experimental measurement of the power emitted by a cylindrical cloud of heated droplets of silicone fluid is also reported. The measured cloud emissivity correlates, within experimental error, with the analytical model.

Mattick, A. T.↗