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At least 73 records · Page 4

Investigation of Aerosol Indirect Effects using a Cumulus Microphysics Parameterization in a Regional Climate Model

A new Zhang and McFarlane (ZM) cumulus scheme includes a two-moment cloud microphysics parameterization for convective clouds. This allows aerosol effects to be investigated more comprehensively by linking aerosols with microphysical processes in both stratiform clouds that are explicitly resolved and convective clouds that are parameterized in climate models. This new scheme is implemented in the Weather Research and Forecasting (WRF) model, which is coupled with the physics and aerosol packages from the Community Atmospheric Model version 5 (CAM5). A test case of July 2008 during the East Asian summer monsoon is selected to evaluate the performance of the new ZM scheme and to investigate aerosol effects on monsoon precipitation. The precipitation and radiative fluxes simulated by the new ZM scheme show a better agreement with observations compared to simulations with the original ZM scheme that does not include convective cloud microphysics and aerosol convective cloud interactions. Detailed analysis suggests that an increase in detrained cloud water and ice mass by the new ZM scheme is responsible for this improvement. To investigate precipitation response to increased anthropogenic aerosols, a sensitivity experiment is performed that mimics a clean environment by reducing the primary aerosols and anthropogenic emissions to 30% of that used in the control simulation of a polluted environment. The simulated surface precipitation is reduced by 9.8% from clean to polluted environment and the reduction is less significant when microphysics processes are excluded from the cumulus clouds. Ensemble experiments with ten members under each condition (i.e., clean and polluted) indicate similar response of the monsoon precipitation to increasing aerosols.

aerosol indirect effects↗

A study of cloud microphysics and precipitation over the Tibetan Plateau by radar observations and cloud-resolving model simulations

Cloud microphysical properties and precipitation over the Tibetan Plateau (TP) are unique because of the high terrains, clean atmosphere, and sufficient water vapor. With dual-polarization precipitation radar and cloud radar measurements during the Third Tibetan Plateau Atmospheric Scientific Experiment (TIPEX-III), the simulated microphysics and precipitation by the Weather Research and Forecasting model (WRF) with the Chinese Academy of Meteorological Sciences (CAMS) microphysics and other microphysical schemes are investigated through a typical plateau rainfall event on 22 July 2014. Results show that the WRF-CAMS simulation reasonably reproduces the spatial distribution of 24-h accumulated precipitation, but has limitations in simulating time evolution of precipitation rates. Here, the model-calculated polarimetric radar variables have biases as well, suggesting bias in modeled hydrometeor types. The raindrop sizes in convective region are larger than those in stratiform region indicated by the small intercept of raindrop size distribution in the former. The sensitivity experiments show that precipitation processes are sensitive to the changes of warm rain processes in condensation and nucleated droplet size (but less sensitive to evaporation process). Increasing droplet condensation produces the best area-averaged rain rate during weak convection period compared with the observation, suggesting a considerable bias in thermodynamics in the baseline simulation. Increasing the initial cloud droplet size causes the rain rate reduced by half, an opposite effect to that of increasing droplet condensation.

54 ENVIRONMENTAL SCIENCES↗

Effects of Sea Spray on Microphysics and Intensity of Deep Convective Clouds Under Strong Winds

Deep convective clouds similar to those arising in the tropical cyclone eyewall are simulated using a parcel model and 2–D slab symmetric cloud model with spectral bin microphysics (the Hebrew University Cloud Model). The size distribution of sea spray particles (SSPs) at cloud base is calculated using the Lagrangian–Eulerian bin microphysics model. The model describes the SSP production, advection, and formation of the size distribution of SSP in the hurricane atmospheric boundary layer at different strong wind speeds. The SSP distributions calculated by the Lagrangian–Eulerian bin microphysics model are used in the parcel model and the Hebrew University Cloud Model to investigate the microphysical and dynamical effects of SSP on clouds. The SSPs ascending in cloud updrafts dramatically increase the number concentration of cloud drops within a wide range of drop sizes. As a result, sea spray creates clouds with unique property combinations of both maritime and continental types. These clouds have droplet size distributions characterized by a high drop concentration and a low effective radius, as in continental clouds. At the same time, the presence of SSP of a few hundred microns in radii triggers intense rain just above the cloud base, which is typical of extreme maritime clouds. In the presence of large sea spray drops, the smallest cloud condensational nuclei, including the smallest SSP, are activated, giving rise to the permanent in–cloud nucleation of small droplets, which produce a high concentration of small ice crystals above the level of homogeneous freezing. We showed that the SSP substantially increased the maximum vertical velocity, cloud water content, and mass contents of ice particles. Here, the results are compared with available observed data.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Impact of a New Cloud Microphysics Parameterization on the Simulations of Mesoscale Convective Systems in E3SM

Abstract Mesoscale convective systems (MCSs) are one of the most climatically significant forms of convection because of their large role in water and energy cycles. The mesoscale features associated with MCS are difficult to represent in climate models because the relevant dynamics and physics are absent or poorly represented with coarse model resolution (∼100 km). Using a regionally refined model (RRM) with 0.25° grid spacing embedded in the Energy Exascale Earth System Model (E3SM), we explore the impact of cloud microphysics parameterizations on the simulation of precipitation, particularly MCS precipitation over the contiguous United States. The Predicted Particle Properties (P3) cloud microphysics scheme has been modified and implemented into E3SM to overcome the limitations of the default Morrison and Gettelman (MG2) scheme in which rimed precipitating ice particles (graupel/hail) are absent and frozen particles are artificially partitioned into cloud ice and snow. We show that P3 improves the simulation of precipitation statistics including frequency distribution compared with MG2 with a limited effect on the diurnal cycle. P3 predicts higher hourly rain rates, resulting in 20% more MCSs and a higher total MCS precipitation (4.4%) compared to MG2, agreeing better with observations. The improvements with P3 mainly result from improved representations of ice microphysics, which not only produces higher rain rates through melting but also leads to a stronger large‐scale ascending motion by releasing more latent heating. This study suggests that improving microphysics parameterization is important for simulating MCS precipitation as future climate model resolutions continue to increase.

54 ENVIRONMENTAL SCIENCES↗

Sensitivity of deep convection and cross-tropopause water transport to microphysical parameterizations in WRF

Deep convective storms can overshoot the tropopause, thus altering the composition of the stratosphere by vertically transporting tropospheric air. The transport of water vapor and ice particles into a sub-saturated environment can hydrate the stratosphere, with implications for radiative forcing and ozone chemistry. Cloud-resolved models, if employed at high spatial resolutions, are used to probe process-level questions about cross-tropopause deep convective hydration and its controls. There is considerable diversity in model representations of processes associated with water transport and transformation, and the choice of a microphysics scheme affects model skill in simulating deep convective events. This motivates our evaluation of state-of-the-art, as well as widely used standard schemes, in a high spatial- and temporal-resolution framework. Six bulk microphysics schemes were employed in a WRF-LES setup, initialized with a sounding profile representative of a tropopause-overshooting storm. Here, we used an idealized framework to isolate the effect of microphysics on the dominant processes that control the reach of deep convection and stratospheric hydration. All schemes produced the highest reaching updrafts 8-12 hours into the simulation but the strength and persistence of updrafts varied across the schemes; maximum storm heights ranged 9.1-12.6 km across the schemes. Varying microphysics produced large differences in the vertical extent and horizontal aggregation of convection, and an order of magnitude spread in above-tropopause water vapor concentrations.

54 ENVIRONMENTAL SCIENCES↗

What Controls Crystal Diversity and Microphysical Variability in Cirrus Clouds?

Abstract Variability of ice microphysical properties like crystal size and density in cirrus clouds is important for climate through its impact on radiative forcing, but challenging to represent in models. For the first time, recent laboratory experiments of particle growth (tied to crystal morphology via deposition density) are combined with a state‐of‐the‐art Lagrangian particle‐based microphysics model in large‐eddy simulations to examine sources of microphysical variability in cirrus. Simulated particle size distributions compare well against balloon‐borne observations. Overall, microphysical variability is dominated by variability in the particles' thermodynamic histories. However, diversity in crystal morphology notably increases spatial variability of mean particle size and density, especially at mid‐levels in the cloud. Little correlation between instantaneous crystal properties and supersaturation occurs even though the modeled particle morphology is directly tied to supersaturation based on laboratory measurements. Thus, the individual thermodynamic paths of each particle, not the instantaneous conditions, control the evolution of particle properties.

54 ENVIRONMENTAL SCIENCES↗

A Moment-Based Polarimetric Radar Forward Operator for Rain Microphysics

There is growing interest in combining microphysical models and polarimetric radar observations to improve our understanding of storms and precipitation. Mapping model-predicted variables into the radar observational space necessitates a forward operator, which requires assumptions that introduce uncertainties into model–observation comparisons. These include uncertainties arising from the microphysics scheme a priori assumptions of a fixed drop size distribution (DSD) functional form, whereas natural DSDs display far greater variability. To address this concern, this study presents a moment-based polarimetric radar forward operator with no fundamental restrictions on the DSD form by linking radar observables to integrated DSD moments. The forward operator is built upon a dataset of >200 million realistic DSDs from one-dimensional bin microphysical rain-shaft simulations, and surface disdrometer measurements from around the world. This allows for a robust statistical assessment of forward operator uncertainty and quantification of the relationship between polarimetric radar observables and DSD moments. Comparison of “truth” and forward-simulated vertical profiles of the polarimetric radar variables are shown for bin simulations using a variety of moment combinations. Higher-order moments (especially those optimized for use with the polarimetric radar variables: the sixth and ninth) perform better than the lower-order moments (zeroth and third) typically predicted by many bulk microphysics schemes.

54 ENVIRONMENTAL SCIENCES↗

A Bayesian Approach for Statistical–Physical Bulk Parameterization of Rain Microphysics. Part II: Idealized Markov Chain Monte Carlo Experiments

Observationally informed development of a new framework for bulk rain microphysics, the Bayesian Observationally Constrained Statistical–Physical Scheme (BOSS; described in Part I of this study), is demonstrated. This scheme’s development is motivated by large uncertainties in cloud and weather simulations associated with approximations and assumptions in existing microphysics schemes. Here, a proof-of-concept study is introduced using a Markov chain Monte Carlo sampling algorithm with BOSS to probabilistically estimate microphysical process rates and parameters directly from a set of synthetically generated rain observations. The framework utilized is an idealized steady-state one-dimensional column rainshaft model with specified column-top rain properties and a fixed thermodynamical profile. Different configurations of BOSS—flexibility being a key feature of this approach—are constrained via synthetic observations generated from a traditional three-moment bulk microphysics scheme. The ability to retrieve correct parameter values when the true parameter values are known is illustrated. For cases when there is no set of true parameter values, the accuracy of configurations of BOSS that have different levels of complexity is compared. It is found that addition of the sixth moment as a prognostic variable improves prediction of the third moment (proportional to bulk rain mass) and rain rate. In contrast, increasing process rate formulation complexity by adding more power terms has little benefit—a result that is explained using further-idealized experiments. BOSS rainshaft simulations are shown to well estimate the true process rates from constraint by bulk rain observations, with the further benefit of rigorously quantified uncertainty of these estimates.

58 GEOSCIENCES↗

How Do Microphysical Processes Influence Large-Scale Precipitation Variability and Extremes?

Convection permitting simulations using the Model for Prediction Across Scales-Atmosphere (MPAS-A) are used to examine how microphysical processes affect large-scale precipitation variability and extremes. An episode of the Madden-Julian Oscillation is simulated using MPAS-A with a refined region at 4-km grid spacing over the Indian Ocean. It is shown that cloud microphysical processes regulate the precipitable water (PW) statistics. Because of the non-linear relationship between precipitation and PW, PW exceeding a certain critical value (PWcr) contributes disproportionately to precipitation variability. However, the frequency of PW exceeding PWcr decreases rapidly with PW, so changes in microphysical processes that shift the column PW statistics relative to PWcr even slightly have large impacts on precipitation variability. Furthermore, precipitation variance and extreme precipitation frequency are approximately linearly related to the difference between the mean and critical PW values. Thus observed precipitation statistics could be used to directly constrain model microphysical parameters as this study demonstrates using radar observations from DYNAMO field campaign.

58 GEOSCIENCES↗

Aerosol Microphysical and Radiative Effects on Continental Cloud Ensembles

Aerosol-cloud-radiation interactions represent one of the largest uncertainties in the current climate assessment. Much of the complexity arises from the non-monotonic responses of clouds, precipitation and radiative fluxes to aerosol perturbations under various meteorological conditions. Here, an aerosol-aware Weather Research and Forecasting (WRF) model is used to investigate the microphysical and radiative effects of aerosols in three weather systems during the March 2000 Cloud Intensive Observational Period campaign at the Southern Great Plains site of the US Atmospheric Radiation Measurement Program. Three cloud ensembles with different meteorological conditions are simulated, including a low-pressure deep convective cloud system, a series of lessprecipitating stratus and shallow cumulus, and a cold frontal passage. The WRF simulations are evaluated by the available observations of cloud fraction, liquid water path, precipitation, and surface temperature. The microphysical properties of cloud hydrometeors, such as their mass and number concentrations, generally show monotonic trends as a function of cloud condensation nuclei concentrations. Aerosol radiative effects do not interfere the trends of cloud microphysics, except for the stratus and shallow cumulus cases where aerosol semi-direct effects are identified. The precipitation changes by aerosols vary with the cloud types and their evolving stages, with more prominent aerosol invigoration effect and associated enhanced precipitation from the convective sources. Furthermore, the simulated aerosol direct effect suppresses precipitation in all three cases but does not overturn the direction of precipitation changes by the aerosol indirect effect. Cloud fraction exhibits much smaller sensitivity (typically less than 2%) to aerosol perturbations than the cloud microphysics, and the responses vary with aerosol concentrations and cloud regimes. The surface shortwave radiation shows a monotonic decrease by increasing aerosols, while the magnitude of the decrease depends on the cloud type. Surface temperature changes closely follow the modulation of the surface radiation fluxes.

54 ENVIRONMENTAL SCIENCES↗

Insensitivity of the Cloud Response to Surface Warming Under Radical Changes to Boundary Layer Turbulence and Cloud Microphysics: Results From the Ultraparameterized CAM

We study the cloud response to a +4K surface warming in a new multi- scale climate model that uses enough interior resolution to begin explicitly resolving boundary layer turbulence (i.e. Ultra-Parameterization or UP), and the associated low clouds. UP's predictions are compared against those from standard Super-Parameterization (SP). The mean global cloud feedback turns out to be remarkably neutral across all of our simulations, despite some radical changes in both cloud microphysical parameter settings and cloud resolving model grid resolution. The overall cloud response to warming is the positive low-cloud feedbacks over land, negative feedbacks at high latitudes, and weak feedbacks over the low-latitude oceans. The most distinct effects of UP appear to be the result of tuning decisions impacting high latitude cloud feedback. UP's microphysics are tuned to optimize the model present-day, top-of-atmosphere radiation fluxes against CERES observations, by lowering the cloud ice-liquid phase-shift temperature ramp, adjusting the ice/liquid autoconversion rate, and increasing the ice fall speed. This reduces baseline high-latitude low cloud amounts, damping the phase change cloud feedback at high latitudes, leading to a slightly more positive global cloud feedback compared to SP. A sensitivity test that isolates these microphysical impacts from UP's grid resolution conrms that the microphysical settings are mostly responsible for the dierences between SP and UP cloud feedback.

54 ENVIRONMENTAL SCIENCES↗

Global Microphysical Sensitivity of Superparameterized Precipitation Extremes

Abstract A recent study found statistically significant differences in extreme precipitation distributions over the contiguous United States (CONUS) when changing the microphysics scheme in a superparameterized global climate model. Here, we repeat the analysis globally and similarly find that differences are widespread when varying the number of predicted moments in the microphysics parameterization, but not when comparing variants of the double‐moment scheme. However, contrary to the previous study in which differences largely disappeared over CONUS when 5‐day simulations were conducted, we found that the signal in these shorter integrations remains within the tropics, implying a direct local effect of microphysics on precipitation extremes in these regions. The effect on precipitation is traced back to changes in vertical velocity profiles changes that are then amplified in the climatological simulations compared to the 5‐day ones. Finally, the superparameterized extremes, regardless of the microphysics scheme, are shown to be larger than those from the Global Precipitation Climatology Project One‐Degree Daily data set and generally smaller than those from the Tropical Rainfall Measuring Mission 3B42 data set.

54 ENVIRONMENTAL SCIENCES↗

An Efficient Bayesian Approach to Learning Droplet Collision Kernels: Proof of Concept Using “Cloudy,” a New n -Moment Bulk Microphysics Scheme

The small-scale microphysical processes governing the formation of precipitation particles cannot be resolved explicitly by cloud resolving and climate models. Instead, they are represented by microphysics schemes that are based on a combination of theoretical knowledge, statistical assumptions, and fitting to data (“tuning”). Historically, tuning was done in an ad hoc fashion, leading to parameter choices that are not explainable or repeatable. Recent work has treated it as an inverse problem that can be solved by Bayesian inference. The posterior distribution of the parameters given the data—the solution of Bayesian inference—is found through computationally expensive sampling methods, which require over $\mathcal{O}$(10 5 ) evaluations of the forward model; this is prohibitive for many models. We present a proof of concept of Bayesian learning applied to a new bulk microphysics scheme named “Cloudy,” using the recently developed Calibrate-Emulate-Sample (CES) algorithm. Cloudy models collision-coalescence and collisional breakup of cloud droplets with an adjustable number of prognostic moments and with easily modifiable assumptions for the cloud droplet mass distribution and the collision kernel. The CES algorithm uses machine learning tools to accelerate Bayesian inference by reducing the number of forward evaluations needed to $\mathcal{O}$(10 2 ). It also exhibits a smoothing effect when forward evaluations are polluted by noise. In a suite of perfect-model experiments, we show that CES enables computationally efficient Bayesian inference of parameters in Cloudy from noisy observations of moments of the droplet mass distribution. In an additional imperfect-model experiment, a collision kernel parameter is successfully learned from output generated by a Lagrangian particle-based microphysics model.

54 ENVIRONMENTAL SCIENCES↗

A Machine Learning Framework for Predicting Microphysical Properties of Ice Crystals From Cloud Particle Imagery

The microphysical properties of ice crystals are important because they significantly alter the radiative properties and spatiotemporal distributions of clouds, which in turn strongly affect Earth's climate. However, it is challenging to measure key properties of ice crystals, such as mass or morphological features. Here, we present a proof-of-concept framework for predicting three-dimensional (3D) microphysical properties of ice crystals from in situ two-dimensional (2D) imagery. First, we computationally generated synthetic ice crystals using 3D modeling software along with geometric parameters estimated from the 2021 Ice Cryo-Encapsulation Balloon (ICEBall) field campaign. Then, we used synthetic crystals to train machine learning (ML) models to predict effective density ($ρ_e$), effective surface area ($A_e$), and number of bullets ($N_b$) from synthetic rosette imagery. On unseen synthetic images, our ML models accurately predicted ice crystal properties. ResNet-18 performed best, achieving $R^2$ values of 0.99 and 0.98 for $ρ_e$ and $A_e$, respectively, and MAE of 0.10 for mathematical equation in single view tasks. Stereo view ResNet-18 further reduced RMSE by 40% for $ρ_e$ and $A_e$ and reduced MAE by 0.08 for $N_b$. This work provides a novel ML-driven framework for estimating ice microphysical properties from in situ imagery, which will allow for downstream constraints on microphysical parameterizations, such as the mass-size relationship.

Ko, J. [Columbia Univ., New York, NY (United State↗

Cold-Season Precipitation Sensitivity to Microphysical Parameterizations: Hydrologic Evaluations Leveraging Snow Lidar Datasets

Abstract Cloud microphysical processes are an important facet of atmospheric modeling, as they can control the initiation and rates of snowfall. Thus, parameterizations of these processes have important implications for modeling seasonal snow accumulation. We conduct experiments with the Weather Research and Forecasting (WRF V4.3.3) Model using three different microphysics parameterizations, including a sophisticated new scheme (ISHMAEL). Simulations are conducted for two cold seasons (2018 and 2019) centered on the Colorado Rockies’ ∼750-km 2 East River watershed. Precipitation efficiencies are quantified using a drying-ratio mass budget approach and point evaluations are performed against three NRCS SNOTEL stations. Precipitation and meteorological outputs from each are used to force a land surface model (Noah-MP) so that peak snow accumulation can be compared against airborne snow lidar products. We find that microphysical parameterization choice alone has a modest impact on total precipitation on the order of ±3% watershed-wide, and as high as 15% for certain regions, similar to other studies comparing the same parameterizations. Precipitation biases evaluated against SNOTEL are 15% ± 13%. WRF Noah-MP configurations produced snow water equivalents with good correlations with airborne lidar products at a 1-km spatial resolution: Pearson’s r values of 0.9, RMSEs between 8 and 17 cm, and percent biases of 3%–15%. Noah-MP with precipitation from the PRISM geostatistical precipitation product leads to a peak SWE underestimation of 32% in both years examined, and a weaker spatial correlation than the WRF configurations. We fall short of identifying a clearly superior microphysical parameterization but conclude that snow lidar is a valuable nontraditional indicator of model performance.

54 ENVIRONMENTAL SCIENCES↗

Evaluation of Physical Microphysical Property Retrieval Algorithms During the 2020 IMPACTS Field Campaign

The NASA Investigation of Microphysics and Precipitation for Atlantic Coast Threatening Snowstorms (IMPACTS) field campaign provides high-quality, high-altitude aircraft lidar (532 nm), radar (W-band) and in-cloud microphysical aircraft data taken during wintertime storm events impacting the United States. This study evaluates two mass-dimensional relationships (Brown and Francis (1995, BF95); Heymsfield (2014, H14) and two lidar-radar microphysical retrieval algorithms (Cloudsat and CALIPSO Ice Cloud Property Product (2C-ICE); VarPy (a variational method derived from the satellite lidar-radar data community)) to estimate aircraft-retrieved volume extinction coefficient (σ), ice water content (IWC), and effective radius (r e ) during the 2020 IMPACTS deployment. BF95 and H14 have a close 1:1 correlation (R 2 = 0.98) with in-situ observations of σ. However, only BF95 displays a linear, consistent, and almost temperature-independent low bias for IWC and r e , which likely arises from the environmental conditions used to determine each. Unlike the field-campaign-derived BF95 and H14 relationships, VarPy and 2C-ICE directly ingest the aircraft-based lidar and radar data to simulate σ, IWC, and r e . For all three microphysical parameters, VarPy and 2C-ICE retrieval errors became notably more pronounced around the dendritic growth zone (-15°C to -10°C) and near freezing (≥-5°C), which suggests that both algorithms experience difficulty addressing riming and aggregation processes and with larger particles (dendrites and plates) due in part to their simplified ice particle assumptions. However, the mean-melt diameter ice-particle assumption did yield more accurate IWC estimates, which led to slightly better overall results for VarPy.

54 ENVIRONMENTAL SCIENCES↗

On the Realism of the Rain Microphysics Representation of a Squall Line in the WRF Model. Part I: Evaluation with Multifrequency Cloud Radar Doppler Spectra Observations

This study investigates how multifrequency cloud radar observations can be used to evaluate the representation of rain microphysics in the WRF Model using two bulk microphysics schemes. A squall line observed over Oklahoma on 12 June 2011 is used as a case study. A recently developed retrieval technique combining observations of two vertically pointing cloud radars provides quantitative description of the drop size distribution (DSD) properties of the transition and stratiform regions of the squall-line system. For the first time, the results of this multifrequency cloud radar retrieval are compared to more conventional retrievals from a nearby polarimetric radar, and a supplementary result of this work is that this new methodology provides a much more detailed description of the DSD vertical and temporal variations. While the extent and evolution of the squall line is well reproduced by the model, the 1-h low-reflectivity transition region is not. In the stratiform region, simulations with both schemes are able to reproduce the observed downdraft and the associated significative subsaturation below the melting level, but with a slight overestimation of the relative humidity. Under this subsaturated air, the simulated rain mixing ratio continuously decreases toward the ground, in agreement with the observations. Conversely, the profiles of the mean volume diameter and the concentration parameter of the DSDs are not well reproduced. These discrepancies pinpoint at an issue in the representation of rain microphysics. The companion paper, investigates the sources of the biases in the microphysics processes in the rain layer by performing numerical sensitivity studies.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Final Technical Report for Interagency Agreement No. DE-SC0005453 “Characterizing Aerosol Distributions, Types, and Optical and Microphysical Properties using the NASA Airborne High Spectral Resolution Lidar (HSRL) and the Research Scanning Polarimeter (RSP)”

Measurements of the vertical profile of atmospheric aerosols and aerosol optical and microphysical characteristics are required to: 1) determine aerosol direct and indirect radiative forcing, 2) compute radiative flux and heating rate profiles, 3) assess model simulations of aerosol distributions and types, and 4) establish the ability of surface and space-based remote sensors to measure the indirect effect. Consequently the ASR program calls for a combination of remote sensing and in situ measurements to determine aerosol properties and aerosol influences on clouds and radiation. As part of our previous DOE ASP project, we deployed the NASA Langley airborne High Spectral Resolution Lidar (HSRL) on the NASA B200 King Air aircraft during major field experiments in 2006 (MILAGRO and MaxTEX), 2007 (CHAPS), 2009 (RACORO), and 2010 (CalNex and CARES). The HSRL provided measurements of aerosol extinction (532 nm), backscatter (532 and 1064 nm), and depolarization (532 and 1064 nm). These measurements were typically made in close temporal and spatial coincidence with measurements made from DOE-funded and other participating aircraft and ground sites. On the RACORO, CARES, and CalNEX missions, we also deployed the NASA Goddard Institute for Space Studies (GISS) Research Scanning Polarimeter (RSP). RSP provided intensity and degree of linear polarization over a broad spectral and angular range enabling column-average retrievals of aerosol optical and microphysical properties. Under this project, we analyzed observations and model results from RACORO, CARES, and CalNex and accomplished the following objectives. 1. Identified aerosol types, characterize the vertical distribution of the aerosol types, and partition aerosol optical depth by type, for CARES and CalNex using HSRL data as we have done for previous missions. 2. Investigated aerosol microphysical and macrophysical properties using the RSP. 3. Used the aerosol backscatter and extinction profiles measured by the HSRL to characterize the planetary boundary layer height (PBL) and the transition zone thickness, for the RACORO and CARES and CalNex campaigns as we have done for previous campaigns. 4. Investigated how optical properties measured by HSRL vary near clouds. 5. Assessed model simulations of aerosol spatial distributions and optical and microphysical properties.

54 ENVIRONMENTAL SCIENCES↗