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NASA NTRS2020

The NANOGrav 11 yr Data Set: Contraints on Planetary Masses Around 45 Millisecond Pulsars

We search for extrasolar planets around millisecond pulsars using pulsar timing data and seek to determine the minimum detectable planetary masses as a function of orbital period. Using the 11 yr data set from the North American Nanohertz Observatory for Gravitational Waves (NANOGrav), we look for variations from our models of pulse arrival times due to the presence of exoplanets. No planets are detected around the millisecond pulsars in the NANOGrav 11 yr data set, but taking into consideration the noise levels of each pulsar and the sampling rate of our observations, we develop limits that show we are sensitive to planetary masses as low as that of the moon. We analyzed potential planet periods, P, in the range 7 days < P < 2000 days, with somewhat smaller ranges for some binary pulsars. The planetary-mass limit for our median-sensitivity pulsar within this period range is 1 Mmoon (P 100 days)-2/3.

E A Behrens↗

DOE OSTI2021

Discovery and Timing of Three Millisecond Pulsars in Radio and Gamma-Rays with the Giant Metrewave Radio Telescope and Fermi Large Area Telescope

In this work, we performed deep observations to search for radio pulsations in the directions of 375 unassociated Fermi Large Area Telescope γ-ray sources using the Giant Metrewave Radio Telescope (GMRT) at 322 and 607 MHz. In this paper we report the discovery of three millisecond pulsars (MSPs), PSR J0248+4230, PSR J1207–5050, and PSR J1536–4948. We conducted follow-up timing observations for ~5 yr with the GMRT and derived phase-coherent timing models for these MSPs. PSR J0248+4230 and J1207–5050 are isolated MSPs having periodicities of 2.60 ms and 4.84 ms. PSR J1536–4948 is a 3.07 ms pulsar in a binary system with an orbital period of ~62 days about a companion of a minimum mass of 0.32 M⊙. We also present multifrequency pulse profiles of these MSPs from the GMRT observations. PSR J1536–4948 is an MSP with an extremely wide pulse profile having multiple components. Using the radio timing ephemeris we subsequently detected γ-ray pulsations from these three MSPs, confirming them as the sources powering the γ-ray emission. For PSR J1536–4948 we performed combined radio–γ-ray timing using ~11.6 yr of γ-ray pulse times of arrival (TOAs) along with the radio TOAs. PSR J1536–4948 also shows evidence for pulsed γ-ray emission out to above 25 GeV, confirming earlier associations of this MSP with a ≥10 GeV point source. The multiwavelength pulse profiles of all three MSPs offer challenges to models of radio and γ-ray emission in pulsar magnetospheres.

79 ASTRONOMY AND ASTROPHYSICS↗

NASA NTRS2021

Discovery and Timing of Three Millisecond Pulsars in Radio and Gamma-Rays with the Giant Metrewave Radio Telescope and Fermi Large Area Telescope

We performed deep observations to search for radio pulsations in the directions of 375 unassociated Fermi Large Area Telescope γ-ray sources using the Giant Metrewave Radio Telescope (GMRT) at 322 and 607 MHz. In this paper we report the discovery of three millisecond pulsars (MSPs), PSR J0248+4230, PSR J1207–5050, and PSR J1536–4948. We conducted follow-up timing observations for ∼5 yr with the GMRT and derived phase-coherent timing models for these MSPs. PSR J0248+4230 and J1207–5050 are isolated MSPs having periodicities of 2.60 ms and 4.84 ms. PSR J1536–4948 is a 3.07 ms pulsar in a binary system with an orbital period of ∼62 days about a companion of a minimum mass of 0.32 M⊙. We also present multifrequency pulse profiles of these MSPs from the GMRT observations. PSR J1536–4948 is an MSP with an extremely wide pulse profile having multiple components. Using the radio timing ephemeris we subsequently detected γ-ray pulsations from these three MSPs, confirming them as the sources powering the γ-ray emission. For PSR J1536–4948 we performed combined radio–γ-ray timing using ∼11.6 yr of γ-ray pulse times of arrival (TOAs) along with the radio TOAs. PSR J1536–4948 also shows evidence for pulsed γ-ray emission out to above 25 GeV, confirming earlier associations of this MSP with a ≥10 GeV point source. The multiwavelength pulse profiles of all three MSPs offer challenges to models of radio and γ-ray emission in pulsar magnetospheres.

High energy astrophysics↗

NASA NTRS2022

Discovery, Timing, and Multiwavelength Observations of the Black Widow Millisecond Pulsar PSR J1555–2908

We report the discovery of PSR J1555−2908, a 1.79 ms radio and gamma-ray pulsar in a 5.6 hr binary system with a minimum companion mass of 0.052 M⊙. This fast and energetic ((E =3 ×10(exp 35)) ̇ erg s(exp -1) millisecond pulsar was first detected as a gamma-ray point source in Fermi Large Area Telescope (LAT) sky survey observations. Guided by a steep-spectrum radio point source in the Fermi error region, we performed a search at 820 MHz with the Green Bank Telescope that first discovered the pulsations. The initial radio pulse timing observations provided enough information to seed a search for gamma-ray pulsations in the LAT data, from which we derive a timing solution valid for the full Fermi mission. In addition to the discovery and timing of radio and gamma-ray pulsations, we searched for X-ray pulsations using NICER but no significant pulsations were detected. We also obtained time-series r-band photometry that indicates strong heating of the companion star by the pulsar wind. Material blown off the heated companion eclipses the 820 MHz radio pulse during inferior conjunction of the companion for ≈10% of the orbit, which is twice the angle subtended by its Roche lobe in an edge-on system.

Millisecond pulsars↗

DOE OSTI2025

Millisecond Phase Transition Kinetics of Lyotropic Liquid Crystalline Nanoparticles Observed by Time‐Resolved Small Angle X‐ray Solution Scattering

This study investigates the dynamic behavior of lyotropic liquid crystal nanoparticles (LCNPs), which are widely recognized for their applications in drug delivery. By employing nanosecond near‐infrared laser pulse‐induced temperature jump (T‐jump) and time‐resolved X‐ray solution scattering, the structural dynamics of phase transitions in phytantriol‐based cubosomes and hexosomes are revealed. Both cubosome and hexosome LCNPs undergo phase transitions into noncrystalline phases at high temperatures. Their phase transition kinetics, occurring within milliseconds (ms) and involving one intermediate structure, are captured. Additionally, the reverse self‐assembly processes of LCNPs were observed, occurring on the timescale of a few hundred ms. To our knowledge, this is the first observation of LCNP T‐jump induced phase transitions on the ms timescale and their reverse self‐assembly. These findings provide valuable insights into the LCNP phase transition processes, with potential implications for drug delivery applications.

Chemistry↗

DOE OSTI2021

Enabling AI-Accelerated Multiscale Modeling of Thrombogenesis at Millisecond and Molecular Resolutions on Supercomputers

We report the first congruent integration of HPC, AI, and multiscale modeling (MSM) for solving a mainstream biomechanical problem of thrombogenesis involving 6 million particles at record molecular-scale resolutions in space and at simulation rates of milliseconds per day. The two supercomputers, the IBM Summit-like AiMOS and our University’s SeaWulf, are used for scalability analysis of, and production runs with, the LAMMPS with our customization and AI augmentation and they attained optimal simulation speeds of 3,077 µs/day and 266 µs/day respectively. The long-time and large scales simulations enable the first study of the integrated platelet flowing, flipping, aggregating dynamics in one dynamically-coupled production run. The platelets’ angular and translational speeds, membrane particles’ speeds, and the membrane stress distributions are presented for the analysis of platelets’ aggregations.

Zhu, Yicong↗

DOE OSTI2021

FAST discovery of an extremely radio-faint millisecond pulsar from the Fermi -LAT unassociated source 3FGL J0318.1+0252

High sensitivity radio searches of unassociated γ-ray sources have proven to be an effective way of finding new pulsars. Using the Five-hundred-meter Aperture Spherical radio Telescope (FAST) during its commissioning phase, we have carried out a number of targeted deep searches of Fermi Large Area Telescope (LAT) γ-ray sources. On February 27, 2018 we discovered an isolated millisecond pulsar (MSP), PSR J0318+0253, coincident with the unassociated γ-ray source 3FGL J0318.1+0252. PSR J0318+0253 has a spin period of 5.19 ms, a dispersion measure (DM) of 26 pc cm –3 corresponding to a DM distance of about 1.3 kpc, and a period-averaged flux density of (~11±2) µJy at L-band (1.05–1.45 GHz). Among all high energy MSPs, PSR J0318+0253 is the faintest ever detected in radio bands, by a factor of at least ~4 in terms of L-band fluxes. With the aid of the radio ephemeris, an analysis of 9.6 years of Fermi-LAT data revealed that PSR J0318+0253 also displays strong γ-ray pulsations. Follow-up observations carried out by both Arecibo and FAST suggest a likely spectral turn-over around 350 MHz. This is the first result from the collaboration between FAST and the Fermi-LAT teams as well as the first confirmed new MSP discovery by FAST, raising hopes for the detection of many more MSPs. Finally, such discoveries will make a significant contribution to our understanding of the neutron star zoo while potentially contributing to the future detection of gravitational waves, via pulsar timing array (PTA) experiments.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2020

Spatiotemporal Formation and Growth Kinetics of Polyelectrolyte Complex Micelles with Millisecond Resolution

We have directly observed the in situ self-assembly kinetics of polyelectrolyte complex (PEC) micelles by synchrotron time-resolved small-angle X-ray scattering, equipped with a stopped-flow device that provides millisecond temporal resolution. A synthesized neutral-charged diblock polycation and homopolyanion that we have previously investigated as a model charge-matched, core-shell micelle system were selected for this work. The initial micellization of the oppositely charged polyelectrolytes was completed within the dead time of mixing of 100 ms, followed by micelle growth and equilibration up to several seconds. By combining the structural evolution of the radius of gyration (R-g) with complementary molecular dynamics simulations, we show how the self-assemblies evolve incrementally in size over time through a two-step kinetic process: first, oppositely charged polyelectrolyte chains pair to form nascent aggregates that immediately assemble into spherical micelles, and second, these PEC micelles grow into larger micellar entities. Furthermore, this work has determined one possible kinetic pathway for the initial formation of PEC micelles, which provides useful physical insights for increasing fundamental understanding self-assembly dynamics, driven by polyelectrolyte complexation that occurs on ultrafast time scales.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

DOE OSTI2021

Millisecond Conversion of Metastable 2D Materials by Flash Joule Heating

Controllable phase engineering is vital for precisely tailoring material properties since different phase structures have various electronic states and atomic arrangements. Rapid synthesis of thermodynamically metastable materials, especially two-dimensional metastable materials, with high efficiency and low cost remains a large challenge. Here we report flash Joule heating (FJH) as an electrothermal method to achieve the bulk conversion of transition metal dichalcogenides, MoS 2 and WS 2 , from 2H phases to 1T phases in milliseconds. The conversions can reach up to 76% of flash MoS 2 using tungsten powder as conductive additive. Different degrees of phase conversion can be realized by controlling the FJH conditions, such as reaction duration and additives, which allows the study of ratio-dependent properties. First-principles calculations confirm that structural processes associated with the FJH, such as vacancy formation and charge accumulation, result in stabilization of the 1T phases. Furthermore, FJH offers rapid access to bulk quantities of the hitherto hard-to-access 1T phases, a promising method for further fundamental research and diverse applications of metastable phases.

2D materials↗

DOE OSTI2026

Hot-Carrier Injection and Millisecond Charge Separation from a Robust Heteroleptic Iron(II) Chromophore Immobilized on TiO 2

The synthesis, spectroscopic characterization, computational analysis, and photoelectrochemical behavior of a new iron-based chromophore, [(Cpy) 2 Fe- (deeb)](PF 6 ) 2 (Fe(Cpy) 2 (deeb)), where Cpy is 1-methyl-3-(2-pyridyl)imidazole and deeb is 4,4’-(CO 2 CH 2 CH 3 ) 2 -2,2’-bipyridine, is reported. Electrochemically reversible waves assigned to a metal-centered E o (Fe III/II ) = +0.48 and a ligand-centered E o (Fe 2+/+ ) = −1.47 V vs Fc +/0 reduction were evident in cyclic voltammetry measurements. The combination of a strong σ-donor and a π-acceptor lowered the energy of the metal-toligand charge-transfer (MLCT) excited state relative to the metal-centered state. Two MLCT transitions appear in the visible region at 424 and 580 nm. TDDFT calculations revealed that the lower-energy band was well formulated as Fe(II)→deeb, and the higher-energy transition was charge transfer to both the deeb and Cpy ligands. Resonance Raman spectroscopy supports these findings showing enhanced deeb vibrational modes with 532 nm excitation, both deeb and Cpy modes with 473 nm excitation, and exclusively Cpy with 405 nm excitation. Ultrafast spectroscopy reveals a short-lived (∼2 ps) MLCT excited state and a longer-lived (∼20 ps) metal-centered state. Efficient methods to deprotect the ester groups and anchor the complex to mesoporous TiO 2 (anatase) thin films in high surface coverages, Fe(Cpy) 2 (dcb)|TiO 2 σ = 3 × 10 −8 mol/cm 2 , were established. Pulsed light excitation of Fe(Cpy) 2 (dcb)|TiO 2 resulted in rapid excited state injection (k inj > 10 8 s −1 ) and formation of a charge-separated state, Fe III (Cpy) 2 (dcb)|TiO 2 (e), which persists on the millisecond time scale before returning cleanly to the ground state with secondorder kinetics. Injection yields measured 50 ns after light excitation were found to double from Φ = 0.15 with green (532 nm) light to 0.30 with blue (457 nm) light excitation. Incident photon-to-current efficiency (% IPCE) measurements as a function of excitation wavelength in a 0.5 M LiI/I 2 /CH 3 CN electrolyte provide clear evidence for band-selective “hot carrier” injection from the remote Cpy-localized excited state. Collectively, the spectroscopic and photoelectrochemical data indicate that a semiconductor can intercept hot electrons from iron chromophores even when the excited-state dipole is oriented away from the surface-anchoring ligand.

Charge transfer↗

DOE OSTI2026

Visualizing Millisecond Atomic Dynamics of Nanocrystals in Liquid

Atomic structures of nanomaterials are inherently dynamic and continuously reshaped through interactions with chemical species and external stimuli. Such dynamics are further amplified as the size and dimensionality of nanomaterials decrease. Despite advances in analytical methods, it remains challenging to capture the structural dynamics of nanomaterials in reactive environments with both atomic spatial resolution and commensurate temporal resolution. Here, in this study, we directly visualize atomic-scale dynamics of gold (Au) nanocrystals in reactive liquid environments with millisecond-speed liquid-cell electron microscopy (EM) and deep-learning denoising. We uncover reversible fluctuations in the local crystallinity of Au nanocrystals dependent on the surrounding chemical environment. These transient fluctuations, driven by interactions at nanocrystal–liquid interfaces, critically influence the dissolution kinetics and grain boundary relaxation. By overcoming the spatiotemporal limitations in conventional liquid-cell EM, our findings provide insights into how transient nanoscale structures dictate the stability and reactivity of nanomaterials.

Kang, Sungsu [University of Chicago, IL (United St↗

DOE OSTI2021

New material platform for superconducting transmon qubits with coherence times exceeding 0.3 milliseconds

The superconducting transmon qubit is a leading platform for quantum computing and quantum science. Building large, useful quantum systems based on transmon qubits will require significant improvements in qubit relaxation and coherence times, which are orders of magnitude shorter than limits imposed by bulk properties of the constituent materials. This indicates that relaxation likely originates from uncontrolled surfaces, interfaces, and contaminants. Previous efforts to improve qubit lifetimes have focused primarily on designs that minimize contributions from surfaces. However, significant improvements in the lifetime of two-dimensional transmon qubits have remained elusive for several years. Here, we fabricate two-dimensional transmon qubits that have both lifetimes and coherence times with dynamical decoupling exceeding 0.3 milliseconds by replacing niobium with tantalum in the device. We have observed increased lifetimes for seventeen devices, indicating that these material improvements are robust, paving the way for higher gate fidelities in multi-qubit processors.

36 MATERIALS SCIENCE↗

DOE OSTI2023

Neutron star mass estimates from gamma-ray eclipses in spider millisecond pulsar binaries

Reliable neutron star mass measurements are key to determining the equation of state of cold nuclear matter, but such measurements are rare. Black widows and redbacks are compact binaries consisting of millisecond pulsars and semi-degenerate companion stars. Spectroscopy of the optically bright companions can determine their radial velocities, providing inclination-dependent pulsar mass estimates. Although inclinations can be inferred from subtle features in optical light curves, such estimates may be systematically biased due to incomplete heating models and poorly understood variability. Using data from the Fermi Large Area Telescope, we have searched for gamma-ray eclipses from 49 spider systems, discovering significant eclipses in 7 systems, including the prototypical black widow PSR B1957+20. Gamma-ray eclipses require direct occultation of the pulsar by the companion, and so the detection, or significant exclusion, of a gamma-ray eclipse strictly limits the binary inclination angle, providing new robust, model-independent pulsar mass constraints. For PSR B1957+20, the eclipse implies a much lighter pulsar (1.81 ± 0.07 solar masses) than inferred from optical light curve modelling.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2022

Deep learning-based noise filtering toward millisecond order imaging by using scanning transmission electron microscopy

Application of scanning transmission electron microscopy (STEM) to in situ observation will be essential in the current and emerging data-driven materials science by taking STEM’s high affinity with various analytical options into account. As is well known, STEM’s image acquisition time needs to be further shortened to capture a targeted phenomenon in real-time as STEM’s current temporal resolution is far below the conventional TEM’s. However, rapid image acquisition in the millisecond per frame or faster generally causes image distortion, poor electron signals, and unidirectional blurring, which are obstacles for realizing video-rate STEM observation. Here we show an image correction framework integrating deep learning (DL)-based denoising and image distortion correction schemes optimized for STEM rapid image acquisition. By comparing a series of distortion corrected rapid scan images with corresponding regular scan speed images, the trained DL network is shown to remove not only the statistical noise but also the unidirectional blurring. This result demonstrates that rapid as well as high-quality image acquisition by STEM without hardware modification can be established by the DL. The DL-based noise filter could be applied to in-situ observation, such as dislocation activities under external stimuli, with high spatio-temporal resolution.

47 OTHER INSTRUMENTATION↗

DOE OSTI2021

Cherenkov Telescope Array sensitivity to the putative millisecond pulsar population responsible for the Galactic Centre excess

ABSTRACT The leading explanation of the Fermi Galactic Centre γ-ray excess is the extended emission from an unresolved population of millisecond pulsars (MSPs) in the Galactic bulge. Such a population would, along with the prompt γ-rays, also inject large quantities of electrons/positrons (e±) into the interstellar medium. These e± could potentially inverse-Compton (IC) scatter ambient photons into γ-rays that fall within the sensitivity range of the upcoming Cherenkov Telescope Array (CTA). In this article, we examine the detection potential of CTA to this signature by making a realistic estimation of the systematic uncertainties on the Galactic diffuse emission model at TeV-scale γ-ray energies. We forecast that, in the event that e± injection spectra are harder than E−2, CTA has the potential to robustly discover the IC signature of a putative Galactic bulge MSP population sufficient to explain the Galactic Centre excess for e± injection efficiencies in the range of ≈2.9–74.1 per cent, or higher, depending on the level of mismodelling of the Galactic diffuse emission components. On the other hand, for spectra softer than E−2.5, a reliable CTA detection would require an unphysically large e± injection efficiency of ${\gtrsim} 158{{\ \rm per\ cent}}$. However, even this pessimistic conclusion may be avoided in the plausible event that MSP observational and/or modelling uncertainties can be reduced. We further find that, in the event that an IC signal were detected, CTA can successfully discriminate between an MSP and a dark matter origin for the radiating e±.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2023

Optical spectral observations of three binary millisecond pulsars

We present the results of optical spectroscopy of stellar companions to three binary millisecond pulsars, PSRs J0621+2514, J2317+1439, and J2302+4442, obtained with the Gran Telescopio Canarias. The spectrum of the J0621+2514 companion shows a blue continuum and prominent Balmer absorption lines. The latter are also resolved in the spectrum of the J2317+1439 companion, showing that both are DA-type white dwarfs. No spectral features are detected for the J2302+4442 companion; however, its broad-band magnitudes and the spectral shape of the continuum emission imply that this is also a DA-type white dwarf. Based on the spectral analyses, we conclude that the companions of J0621+2514 and J2317+1439 are relatively hot, with effective temperatures T eff = 8600 ± 200 and 9600 ± 2000 K, respectively, while the J2302+4442 companion is significantly cooler, T eff <6000 K. We also estimated the distance to J0621+2514 of 1.1 ± 0.3 kpc and argue that its companion and the companion of J2317+1439 are He-core white dwarfs providing constraints on their cooling ages of $\lesssim$2 Gyr.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2026

Defect in diamond with millisecond-scale spin relaxation time at room temperature

Spin defects in diamond are promising platforms for quantum sensing. The longest electron spin relaxation times (T1) at room temperature for solid-state defects are observed in nitrogen vacancy centers in diamond, which can reach 6.67 ms [1], and substitutional nitrogen (“P1 centers”) in diamond, which exhibit a T1 of 2 ms [2]. No other solid-state defect has exhibited millisecond-scale spin relaxation times at room temperature thus far. Here, we characterize the spin properties of the WAR5 defect in diamond [3] with pulsed electron spin resonance. The observed T1 is one of the longest for solid-state spin defects: 0.97(27) ms at room temperature and 14.38(19) min at 4 K. The observed coherence time (T2) is 246(7) µs, which can be extended to 6.49(34) ms at 4 K with dynamical decoupling. Finally, we demonstrate optical spin polarization with a range of wavelengths from 405 nm to 500 nm and propose potential zero-phonon line candidates.

36 MATERIALS SCIENCE↗

DOE OSTI2022

Evidence of TeV halos around millisecond pulsars

Using data from the HAWC gamma-ray Telescope, we have studied a sample of 37 millisecond pulsars (MSPs), selected for their spindown power and proximity. From among these MSP, we have identified four which favor the presence of very high-energy gamma-ray emission at a level of (2Δ ln L) 1/2 ≥ 2.5. Adopting a correlation between the spindown power and gamma-ray luminosity of each pulsar, we performed a stacked likelihood analysis of these 37 MSPs, finding that the data supports the conclusion that these sources emit very high-energy gamma-rays at a level of (2Δ ln L) 1/2 = 4.24. Among sets of randomly selected sky locations within HAWC’s field-of-view, less than 1% of such realizations yielded such high statistical significance. Our analysis suggests that MSPs produce very high-energy gamma-ray emission with a similar efficiency to that observed from the Geminga TeV-halo, η MSP = (0.39 - 1.08) x η Geminga . So this conclusion poses a significant challenge for pulsar interpretations of the Galactic Center gamma-ray excess, as it suggests that any population of MSPs potentially capable of producing the GeV excess would also produce TeV-scale emission in excess of that observed by HESS from this region. Future observations by CTA will be able to substantially clarify this situation

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗