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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 73 records · Page 4
All sourcesNASA NTRSDOE OSTI
DOE OSTI2022

Towards computational polar-topotronics: Multiscale neural-network quantum molecular dynamics simulations of polar vortex states in SrTiO3/PbTiO3 nanowires

Recent discoveries of polar topological structures ( e.g ., skyrmions and merons) in ferroelectric/paraelectric heterostructures have opened a new field of polar topotronics. However, how complex interplay of photoexcitation, electric field and mechanical strain controls these topological structures remains elusive. To address this challenge, we have developed a computational approach at the nexus of machine learning and first-principles simulations. Our multiscale neural-network quantum molecular dynamics molecular mechanics approach achieves orders-of-magnitude faster computation, while maintaining quantum-mechanical accuracy for atoms within the region of interest. This approach has enabled us to investigate the dynamics of vortex states formed in PbTiO 3 nanowires embedded in SrTiO 3 . We find topological switching of these vortex states to topologically trivial, uniformly polarized states using electric field and trivial domain-wall states using shear strain. These results, along with our earlier results on optical control of polar topology, suggest an exciting new avenue toward opto-electro-mechanical control of ultrafast, ultralow-power polar topotronic devices.

Linker, Thomas↗
NASA NTRS1976

Astronomical polarization studies at radio and infrared wavelengths. Part 1: Gravitational deflection of polarized radiation

The gravitational field is probed in a search for polarization dependence in the light bending. This involves searching for a splitting of a source image into orthogonal polarizations as the radiation passes through the solar gravitational field. This search was carried out using the techniques of very long and intermediate baseline interferometry, and by seeking a relative phase delay in orthogonal polarizations of microwaves passing through the solar gravitational field. In this last technique a change in the total polarization of the Helios 1 carrier wave was sought as the spacecraft passed behind the sun. No polarization splitting was detected.

Dennison, B. K.↗
NASA NTRS1976

Astronomical polarization studies at radio and infrared wavelengths. Part 2: Far infrared polarization of dust clouds

Far infrared polarization of dust clouds is examined. The recently observed 10 micron polarization of the Orion Nebula and the Galactic Center suggests that far infrared polarization may be found in these objects. Estimates are made of the degree of far infrared polarization that may exist in the Orion Nebula. An attempt to observe far infrared polarization from the Orion Nebula was carried out.

Dennison, B. K.↗
NASA NTRS1977

Transfer of polarized radiation in self-absorbed synchrotron sources. II - Treatment of inhomogeneous media and calculation of emergent polarization

As an extension of previous treatments of polarized radiation transfer in homogeneous synchrotron sources, a transfer procedure is derived, based on the coupled-wave formulation, which allows consideration of inhomogeneous sources. It is shown that plasma characteristic wave eccentricities in a source must be fairly large unless Faraday rotation per absorption depth is very large, and that coupling between characteristic waves can be strong in inhomogeneous self-absorbed sources. Calculations are made of the polarized radiation emergent from a source with a boundary of finite thickness. It is found that neglect of propagation effects in the source boundary introduces no significant errors at optically thin frequencies, but that below the self-absorption turnover the emergent polarization may depend significantly upon such effects. In particular, the sign of the circular polarization and the linear polarization position angle depend upon the absorption depth in the boundary region.

Jones, T. W.↗
NASA NTRS1979

Measurement of the polarization effects of an instrument using partially polarized light

Accuracy of a radiometer is adversely affected by scene polarization if the receiving optical system is sensitive to polarization. It is therefore necessary to specify and measure the sensitivity of the system to polarized light. The Mueller-Stokes matrix of an instrument may be determined experimentally and used to predict the effects of the instrument on any beam. The specification of a maximum polarization sensitivity stated in terms of the degree of polarization produced in an unpolarized beam can be experimentally verified even though an unpolarized beam is not available in the laboratory for direct measurement.

Howell, B. J.↗
NASA NTRS1983

Eddy intrustion of hot plasma into the polar cap and formation of polar-cap arcs

Under the simple postulate that multiple large scale detachable magnetospheric convection eddies can exist in the vicinity of the convection reversal boundary and in the polar cap, by Kelvin-Helmholtz instability or otherwise, it is shown that a number of seemingly disconnected plasma and electric field observations in the polar cap can be organized into a theory of magnetosheath and plasmasheet plasma intrusion into the polar cap. Current theory of inverted V structures then predicts existence of similar, but weaker, structures at the eddy convection reversal boundaries in the polar cap. A possible consequence is that the polar cap auroras are natural offshoots from discrete oval arcs and evidently are formed by similar processes. The two arc systems can occassionally produce an optical image in the form of the theta aurora.

Chiu, Y. T.↗
NASA NTRS1986

Simultaneous polar cap and magnetotail observations of intense polar rain

The significance of acceleration processes in accounting for the energies and temperatures of the electrons seen during periods of intense polar rain is investigated along with the role of the IMF and solar wind in controlling the polar rain. Evidence for an acceleration region is sought by comparing DMSP observations of the precipitating electrons over the polar cap with simultaneous ISEE 1 electron measurements in the conjugate tail lobe at distances between 10 and 22.6 earth radii. The second question is explored by examining the solar wind and IMF conditions during which the intense polar rain events occur. It is found that intense polar rain can pass through the tail lobes without undergoing acceleration between 22.6 earth radii and 800 km altitude.

Greenspan, M. E.↗
NASA NTRS1987

Polarized and non-polarized leaf reflectances of Coleus blumei

A polarization photometer has been used to measure the reflectance of three variegated portions of Coleus blumei, Benth. in five wavelength bands of the visible and near-infrared spectrum. The polarized component of the reflectance factor was found to be independent of wavelength, indicating that the polarized reflectance arises from the leaf surface. It is suggested that differences in the polarized component result from variations in surface features. The nonpolarized component of the reflectance factor is shown to be related to the internal leaf structure. The variation of the degree of polarization with wavelength was found to be greatest in the regions of the spectrum where absorption occurs.

Grant, Lois↗
NASA NTRS1992

A technique for measuring vertically and horizontally polarized microwave brightness temperatures using electronic polarization-basis rotation

This technique for electronically rotating the polarization basis of an orthogonal-linear polarization radiometer is based on the measurement of the first three feedhorn Stokes parameters, along with the subsequent transformation of this measured Stokes vector into a rotated coordinate frame. The technique requires an accurate measurement of the cross-correlation between the two orthogonal feedhorn modes, for which an innovative polarized calibration load was developed. The experimental portion of this investigation consisted of a proof of concept demonstration of the technique of electronic polarization basis rotation (EPBR) using a ground based 90-GHz dual orthogonal-linear polarization radiometer. Practical calibration algorithms for ground-, aircraft-, and space-based instruments were identified and tested. The theoretical effort consisted of radiative transfer modeling using the planar-stratified numerical model described in Gasiewski and Staelin (1990).

Gasiewski, Albin J.↗
NASA NTRS1993

Warm O(+) polar wind and the DE-1 polar cap electron density profile

Theoretical steady state semikinetic polar wind density profiles, based on DE1/RIMS polar wind data (up to 3700 km), were obtained which agree very well with the power law electron density profile measured by the DE1/PWI for high altitudes. The polar wind is found to be O(+) dominated for the full altitude range considered (up to 8 R(E)). Multiple solutions are obtained for various combinations of base altitude ion temperatures and electron temperatures, such that the densities fit the Persoon et al. (1983) profile. For example, good fits to measured density profile are found for low base ion temperatures (5000 K) and high electron temperatures (9000 K), and also for unheated H(+) and O(+)(3000 K) with electron temperatures of 11,000 K. Below 2.8 R(E) the theoretical polar wind density deviates somewhat from the r exp -3.85 power law. It is concluded that this theoretical polar wind density profile, with a sum of base electron and ion temperatures of 14,000 K, yields a close match with the measured DE-1 electron density profile.

Ho, C. W.↗
NASA NTRS2012

Characterization of the Morphometry of Impact Craters Hosting Polar Deposits in Mercury's North Polar Region

Earth-based radar images dating back two decades show that the floors of some polar craters on Mercury host radar-bright deposits that have been proposed to consist of frozen volatiles. Several hypotheses have been put forth to explain their source, including volcanic outgassing, chemical sputtering, and deposition of exogenous water ice. Calculations show that volatiles are thermally stable in permanently shadowed areas. An earlier study of the depths of north polar craters determined with photoclinometric techniques applied to Mariner 10 images yielded the conclusion that the mean ratio of crater depth d to rim-crest diameter D for craters hosting polar deposits is two-thirds that of the mean ratio for a comparable population of neighboring craters lacking such deposits. This result could be explained by (though doesn't require) the presence of a thick layer of volatiles within the polar deposit-hosting craters. Here we use altimetric profiles and topographic maps obtained by the Mercury Laser Altimeter (MLA) to revisit this analysis. MLA is an instrument on the MErcury Surface, Space ENvironment, GEochemistry, and Ranging (MESSENGER) spacecraft, which has been orbiting Mercury since March 2011. MLA transmits a 1064-nm laser pulse at 8 Hz during MESSENGER's trajectory over Mercury s surface. The MLA illuminates surface areas averaging between 15 m and 100 m in diameter, spaced approx 400 m apart along the spacecraft ground track. The radial precision of individual measurements is <1 m, and the current accuracy with respect to Mercury s center of mass is better than 20 m. As of mid-December 2011, MLA coverage had reached to 15 S and has yielded a comprehensive map of the topography of Mercury s northern hemisphere. The MLA data are used here to quantify the shapes of craters in the north polar region and to avoid the shadowing bias of photoclinometric techniques.

Talpe, Matthieu, J.↗
DOE OSTI2024

Polarization Type Potential Induced Degradation under Positive Bias in a Commercial PERC Module: Preprint

Potential induced degradation of the polarization type (PID-p) can reduce module performance in a relatively short period of time. PID-p can occur at both voltage polarities, but most studies are focused on degradation under a negative bias. This paper uses commercial bifacial passivated emitter and rear contact (PERC) cells within a monofacial glass-backsheet module construction to evaluate the impact of PID-p under a positive bias on the front side. Using the aluminum-foil (Al-foil) method, the module was stressed for PID in an environmental chamber. After the stress, the maximum power (Pmax) showed a decline of 3.1% at 1000 W/m2 and 6.2% at 200 W/m2. Recovery under light was also investigated. Complete recovery was observed at high irradiance, while a partial recovery was seen at lower irradiance. The outcomes of this study can help in understanding PID-p degradation under a positive bias and its recovery under the light.

PERC↗
DOE OSTI2026

Spin Polarization from Circularly Polarized Light Induced Charge Transfer

Here, we show how a spin polarization can be generated through the photoinduced electron transfer of an achiral donor–acceptor complex following chiral light excitation. In particular, we illustrate the basic energetic and symmetry requirements for chirality induced spin selectivity where the chirality emerges from the electronic degrees of freedom following excitation with circularly polarized light. We study this effect in a simple model of a metalloporphyrin complex with an axial acceptor ligand using quantum mechanical rate theories and numerical simulations. We find that the spin polarization emerges due to the selective excitation of a ring current within the porphryin, breaking the degeneracy of the two degenerate spin states. The resultant spin polarization increases with the spin orbit coupling between the metal in the porphyrin and the axial ligand, and is transient, with a lifetime dependent on the rate of dephasing from the Jahn–Teller distortion mode. This proposed effect should be observable in spin-resolved photoemission spectroscopy.

charge transfer↗
DOE OSTI2021

Magnetization distribution in Cu 0.6 Mn 2.4 Ge 2 ferromagnet from polarized and non-polarized neutron powder diffraction aided by density-functional theory calculations

The crystal structure and magnetic properties of Cu 0.6 Mn 2.4 Ge 2 have been re-investigated by a combination of extensive magnetic measurements and neutron scattering experiments, aided by electronic structure calculations. The material is found to be a soft ferromagnet with the ordering temperature T C = 316 K. The magnetocaloric effect evaluated from field-dependent magnetization isotherms is equal to 1.2 J/(kg·K) and 2.5 J/(kg·K) under the maximum applied magnetic field of 2 T and 5 T, respectively. The compound crystallizes in the hexagonal space group P6 3 /mmc. A complex structural disorder necessitated testing of several disorder models against the results of non-polarized and polarized neutron scattering experiments and magnetization measurements. Simulations at the density-functional theory level were also performed to identify the most robust solution that properly described the data observed. The final magnetic structure model reveals non-equal magnetic moments on the Mn1 and Mn2 atoms (2.29(9) µ B and 2.7(1) µ B , respectively) and the presence of vacancies and minor Cu substitution defects in both Mn sites. The work demonstrates how the non-polarized and polarized neutron scattering methods can be combined with electronic structure calculations to establish the microscopic structure of magnetic materials with complex crystallographic disorder.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2021

In situ study of the electronic structure of polar-to-polar SrTiO 3 /($000\bar1$)ZnO heterointerface

The SrTiO 3 (STO)/ZnO heterointerface, which is widely used in the fabrication of novel optoelectronic devices, is a classical system combining functional perovskite oxides and wurtzite-structure semiconductor materials. The electronic structure of the heterointerface often plays a significant role in controlling the functions of novel devices. In this study, the electronic structure was explored using in situ photoemission spectroscopy and X-ray absorption spectroscopy. X-ray diffraction results showed the coexistence of (111) STO and (011) STO orientations for the STO film deposited on the ZnO-($000\bar1$) substrate via pulsed laser deposition. High-resolution transmission electron microscopic results revealed two types of polar interfaces: [$11\bar2$][$10\bar1$](111) STO //[$1\bar210$][$10\bar10$]($000\bar1$) ZnO and [111][$2\bar1\bar1$](011) STO //[$10\bar21$][$10\bar10$]($000\bar1$)ZnO. In situ photoemission spectroscopic results revealed downward band bending and the transformation of the valence states of Ti from 4+ to 3+, with extra electrons transferring to the hybridization states between O 2p and Ti t 2g orbitals at the polar-to-polar STO/ZnO interface. We propose that the polar discontinuity drives the electron transfer to the STO/ZnO interface during the growth process. This study provides insight into the electronic structure of the STO/($000\bar1$)ZnO heterointerface.

77 NANOSCIENCE AND NANOTECHNOLOGY↗
DOE OSTI2023

Nonadiabatic Dynamics in a Continuous Circularly Polarized Laser Field with Floquet Phase-Space Surface Hopping

Non-adiabatic chemical reactions involving continuous circularly polarized light (cw CPL) have not attracted as much attention as dynamics in unpolarized/linearly polarized light. However, including circularly (in contrast to linearly) polarized light allows one to effectively introduce a complex-valued time-dependent Hamiltonian, which offers a new path for control or exploration through the introduction of Berry forces. Here, we investigate several inexpensive semiclassical approaches for modeling such nonadiabatic dynamics in the presence of a time-dependent complex-valued Hamiltonian, beginning with a straightforward instantaneous adiabatic fewest-switches surface hopping (IA-FSSH) approach (where the electronic states depend on position and time), continuing to a standard Floquet fewest switches surface hopping (F-FSSH) approach (where the electronic states depend on position and frequency), and ending with an exotic Floquet phase-space surface hopping (F-PSSH) approach (wherethe electronic states depend on position, frequency, and momentum). Using a set of model systems with time-dependent complex-valued Hamiltonians, we show that the Floquet phase- space adiabats are the optimal choice of basis as far as accounting for Berry phase effects and delivering accuracy. Furthermore, the F-PSSH algorithm sets the stage for modeling nonadiabatic dynamics under strong externally pumped circular polarization in the future.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2025

Polarization options in inclusive DIS off tensor polarized deuteron

In the near future, the Jefferson Lab b 1 experiment will provide the second measurement of tensor polarized asymmetries in inclusive DIS on the deuteron. In this asymmetry, 4 independent tensor polarized structure functions contribute. This necessitates systematic approximations in the extraction of the leading twist structure function b 1 from a single tensor asymmetry measurement. Contamination from higher twist structure functions and kinematic effects is discussed here. Using a deuteron convolution model, we quantify the systematic errors from these approximations for two different choices for the target polarization direction (momentum transfer, electron beam direction). For Jefferson Lab 12 GeV kinematics, the systematic error turns out to be comparable between the two polarization options, while at higher Q 2 values the momentum transfer direction is preferred.

Cosyn, Wim [Florida International University, Miam↗
DOE OSTI2021

Superconducting RF Gun with High Current and the Capability to Generate Polarized Electron Beams

High-current low-emittance CW electron beams are indispensable for nuclear and high-energy physics fixed target and collider experiments, cooling high energy hadron beams, generating CW beams of monoenergetic X-rays (in FELs) and gamma-rays (in Compton sources). Polarization of electrons in these beams provides extra value by opening a new set of observables and frequently improving the data quality. We report on the upgrade of the unique and fully functional CW SRF 1.25 MeV SRF gun, built as part of the Coherent electron Cooling (CeC) project, which has demonstrated sustained CW operation with CsK2Sb photocathodes generating electron bunches with record-low transverse emittances and record-high bunch charge exceeding 10 nC. We propose to extend the capabilities of this system to high average current of 100 milliampere in two steps: increasing the current 30-fold at each step with the goal to demonstrate reliable long-term operation of the high-current low-emittance CW SRF guns. We also propose to test polarized GaAs photocathodes in the ultra-high vacuum (UHV) environment of the SRF gun, which has never been successfully demonstrated in RF accelerators.

43 PARTICLE ACCELERATORS↗