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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 73 records · Page 4
All sourcesNASA NTRSDOE OSTI
DOE OSTI2024

Universal framework for simultaneous tomography of quantum states and SPAM noise

We present a general denoising algorithm for performing simultaneous tomography of quantum states and measurement noise. This algorithm allows us to fully characterize state preparation and measurement (SPAM) errors present in any quantum system. Our method is based on the analysis of the properties of the linear operator space induced by unitary operations. Given any quantum system with a noisy measurement apparatus, our method can output the quantum state and the noise matrix of the detector up to a single gauge degree of freedom. We show that this gauge freedom is unavoidable in the general case, but this degeneracy can be generally broken using prior knowledge on the state or noise properties, thus fixing the gauge for several types of state-noise combinations with no assumptions about noise strength. Such combinations include pure quantum states with arbitrarily correlated errors, and arbitrary states with block independent errors. This framework can further use available prior information about the setting to systematically reduce the number of observations and measurements required for state and noise detection. Our method effectively generalizes existing approaches to the problem, and includes as special cases common settings considered in the literature requiring an uncorrelated or invertible noise matrix, or specific probe states.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2019

Stratified manifold of quantum states, actions of the complex special linear group

We review the geometry of the space of quantum states S(H) of a finite-level quantum system with Hilbert space H from a group-theoretical point of view. This space carries two stratifications generated by the action of two different Lie groups, namely, the special unitary group SU(H) and its complexification SL(H), the complex special linear group. A stratum of the stratification generated by SU(H) is composed of isospectral states, that is, density operators with the same spectrum. A stratum of the stratification generated by SL(H) is composed of quantum states with the same rank. We prove that on every submanifold of isospectral quantum states there is also a canonical left action of SL(H) which is related with the canonical Kähler structure on isospectral quantum states. The fundamental vector fields of this SL(H)-action are divided into Hamiltonian and gradient vector fields. The former give rise to invertible maps on S that preserve the von Neumann entropy and the convex structure of S(H), while the latter give rise to invertible maps on S(H) that preserve the von Neumann entropy but not the convex structure of S(H). A similar decomposition is given for the fundamental vector fields of the SL(H)-action generating the stratification of S(H) into manifolds of quantum states with the same rank. However, in this case, the gradient vector fields preserve the rank but do not preserve entropy. Finally, some comments on multipartite quantum systems are made, and it is proved that the sets of product states of a multipartite quantum system are homogeneous manifolds for the local action of the complex special linear group associated with the partition.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2011

Quantum key distribution with a reference quantum state

A new quantum key distribution protocol stable at arbitrary losses in a quantum communication channel has been proposed. For the stability of the protocol, it is of fundamental importance that changes in states associated with losses in the communication channel (in the absence of the eavesdropper) are included in measurements.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2014

An impurity-induced gap system as a quantum data bus for quantum state transfer

We introduce a tight-binding chain with a single impurity to act as a quantum data bus for perfect quantum state transfer. Our proposal is based on the weak coupling limit of the two outermost quantum dots to the data bus, which is a gapped system induced by the impurity. By connecting two quantum dots to two sites of the data bus, the system can accomplish a high-fidelity and long-distance quantum state transfer. Numerical simulations for finite system show that the numerical and analytical results of the effective coupling strength agree well with each other. Moreover, we study the robustness of this quantum communication protocol in the presence of disorder in the couplings between the nearest-neighbor quantum dots. We find that the gap of the system plays an important role in robust quantum state transfer.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2026

Vibrational Quantum-State-Controlled Reactivity in the O 2 + + C 3 H 4 Reaction

Quantum-state-controlled reactivity is a long-standing goal in the field of physical chemistry. In this work, we explore the vibrational-state-dependent behavior of the ion–molecule reaction between O 2 + in distinct vibrational states and two isomers of C 3 H 4 , allene (H 2 C 3 H 2 ) and propyne (H 3 C 3 H). While most products are formed regardless of the vibrational state of O 2 + , the branching ratios are influenced by vibrational excitation, and a new product, C 2 O + , appears exclusively in the excited-state reactions. This selective formation of C 2 O + demonstrates that vibrational excitation can effectively activate a reaction pathway, providing direct evidence of quantum-state control in the reactivity. These results represent an important step toward the goal of quantum-state-controlled chemistry in molecular systems.

Chemical reactions↗
DOE OSTI2020

Computationally efficient Bayesian quantum state tomography

We describe a method for Bayesian quantum state estimation combining efficient parameterization, a pseudo-likelihood, and advanced numerical sampling techniques. Examples reveal significant computational speedup, indicating the approach’s promise in practical quantum state tomography.

Lukens, Joseph↗
DOE OSTI2017

Perfect quantum state engineering by the combination of the counterdiabatic driving and the reverse-engineering technique

We propose a method to design shortcuts to adiabaticity for implementing perfect quantum state engineering by the combination of the counterdiabatic driving and the reverse engineering technique. Based on the method, we can design simple schemes to realize the intended dynamics. For the sake of clearness, we apply this method to several examples including two-level, three-level and four-level system. We show that fast quantum state engineering can be realized by utilizing simply-designed auxiliary Hamiltonian. Furthermore, a suitable choice of the control parameters can eliminate the additional couplings in the introduced auxiliary Hamiltonian. Numerical simulation reveals that the constructed scheme is reliable and robust against various dissipation effects and the fluctuations of control parameters in current technology. - Highlights: • Fast and feasible quantum state engineering can be realized by using the method. • The method allows one to control accurately the evolution of the system. • The scheme is fast and robust against dissipation effects and parameter errors. • The scheme can be generalized to realize N-dimensional quantum state engineering.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2011

Tomography of the quantum state of photons entangled in high dimensions

Systems entangled in high dimensions have recently been proposed as important tools for various quantum information protocols, such as multibit quantum key distribution and loophole-free tests of nonlocality. It is therefore important to have precise knowledge of the nature of such entangled quantum states. We tomographically reconstruct the quantum state of the two photons produced by parametric downconversion that are entangled in a d-dimensional orbital angular momentum basis. We determine exactly the density matrix of the entangled two-qudit state with d ranging from 2 to 8. The recording of higher-dimensional states is limited only by the number of data points required and therefore the length of time needed to complete the measurements. We find all the measured states to have fidelities and linear entropies that satisfy the criteria required for a violation of the appropriate high-dimensional Bell inequality. Our results therefore precisely characterize the nature of the entanglement, thus establishing the suitability of such states for applications in quantum information science.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2022

Quantum state preparation by adiabatic evolution with custom gates

Quantum state preparation by adiabatic evolution is currently rendered ineffective by the long implementation times of the underlying quantum circuits, comparable to the decoherence time of present and near-term quantum devices. These implementation times can be significantly reduced by realizing these circuits with custom gates. Using classical computing, we model the output of a realistic two-qubit processor implementing the adiabatic evolution of a two-spin system by means of custom gates. This modeled output is then compared with the results of quantum simulations solving the same problem on IBM Quantum (IBMQ) systems. Additionally, when used to emulate the behavior of the IBMQ quantum circuit, our realistic model yields state fidelities ranging from 65% to 85%, similar to the actual performance of a diverse set of IBMQ devices. When we reduced the implementation time by using custom gates, however, the loss of fidelity was reduced by at least a factor of 4, allowing us to accurately extract the energy of the target state. This improvement is enough to render adiabatic evolution useful for quantum state preparation for small systems or as a preconditioner for other state preparation methods.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2011

Quantum States Probed By Temperature Dependence Capacitance-Voltage Measurements For InP/GaAs Type-II Ultrathin Quantum Well

We report on the temperature dependent capacitance-voltage measurements on InP/GaAs ultrathin quantum well (QW). We observe a peak in apparent carrier distribution (ACD) profile at around the geometrical position of the QW. Peak value of the ACD profile increases, while it's width decreases with reducing temperature indicating that the peak in ACD is due to the accumulation of two dimensional electrons occupying the quantum states in ultrathin QW.

36 MATERIALS SCIENCE↗
DOE OSTI2011

Quantum-state preparation with universal gate decompositions

In quantum computation every unitary operation can be decomposed into quantum circuits--a series of single-qubit rotations and a single type entangling two-qubit gates, such as controlled-not(cnot) gates. Two measures are important when judging the complexity of the circuit: the total number of cnot gates needed to implement it and the depth of the circuit, measured by the minimal number of computation steps needed to perform it. Here we give an explicit and simple quantum circuit scheme for preparation of arbitrary quantum states, which can directly utilize any decomposition scheme for arbitrary full quantum gates, thus connecting the two problems. Our circuit reduces the depth of the best currently known circuit by a factor of 2. It also reduces the total number of cnot gates from 2{sup n} to (23/24)2{sup n} in the leading order for even number of qubits. Specifically, the scheme allows us to decrease the upper bound from 11 cnot gates to 9 and the depth from 11 to 5 steps for four qubits. Our results are expected to help in designing and building small-scale quantum circuits using present technologies.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2017

Enhancing multi-step quantum state tomography by PhaseLift

Multi-photon system has been studied by many groups, however the biggest challenge faced is the number of copies of an unknown state are limited and far from detecting quantum entanglement. The difficulty to prepare copies of the state is even more serious for the quantum state tomography. One possible way to solve this problem is to use adaptive quantum state tomography, which means to get a preliminary density matrix in the first step and revise it in the second step. In order to improve the performance of adaptive quantum state tomography, we develop a new distribution scheme of samples and extend it to three steps, that is to correct it once again based on the density matrix obtained in the traditional adaptive quantum state tomography. Our numerical results show that the mean square error of the reconstructed density matrix by our new method is improved to the level from 10{sup −4} to 10{sup −9} for several tested states. In addition, PhaseLift is also applied to reduce the required storage space of measurement operator. - Highlights: • PhaseLift is firstly applied in the adaptive quantum state tomography and the required store space of measurement operator is reduced. • Traditional adaptive quantum state tomography is extended to three-step adaptive quantum state tomography. • A new scheme of copy distribution of state is proposed to effectively use the limited copies of state. • For several tested states, the mean square error of the reconstructed state is reduced to 10{sup −9} from 10{sup −4}. • Fidelity is more accurately estimated with limited copies of state compared with traditional adaptive quantum state tomography.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2020

A practical and efficient approach for Bayesian quantum state estimation

Bayesian inference is a powerful paradigm for quantum state tomography, treating uncertainty in meaningful and informative ways. Yet the numerical challenges associated with sampling from complex probability distributions hampers Bayesian tomography in practical settings. In this article, we introduce an improved, self-contained approach for Bayesian quantum state estimation. Leveraging advances in machine learning and statistics, our formulation relies on highly efficient preconditioned Crank–Nicolson sampling and a pseudo-likelihood. We theoretically analyze the computational cost, and provide explicit examples of inference for both actual and simulated datasets, illustrating improved performance with respect to existing approaches.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
NASA NTRS1992

Nonclassical depth of a quantum state

A measure is defined for how nonclassical a quantum state is, with values ranging from 0 to 1. When it is applied to the photon-number states, the calculated value is 1, the maximum possible. For squeezed states, it is a monotonically increasing function of the squeeze parameter with values varying from 0 to 1/2. The physical meaning of the nonclassical depth is found to be just the number of thermal photons necessary to ruin the nonclassical nature of the quantum state.

Lee, Ching Tsung↗
DOE OSTI2017

Average subentropy, coherence and entanglement of random mixed quantum states

Compact expressions for the average subentropy and coherence are obtained for random mixed states that are generated via various probability measures. Surprisingly, our results show that the average subentropy of random mixed states approaches the maximum value of the subentropy which is attained for the maximally mixed state as we increase the dimension. In the special case of the random mixed states sampled from the induced measure via partial tracing of random bipartite pure states, we establish the typicality of the relative entropy of coherence for random mixed states invoking the concentration of measure phenomenon. Our results also indicate that mixed quantum states are less useful compared to pure quantum states in higher dimension when we extract quantum coherence as a resource. This is because of the fact that average coherence of random mixed states is bounded uniformly, however, the average coherence of random pure states increases with the increasing dimension. As an important application, we establish the typicality of relative entropy of entanglement and distillable entanglement for a specific class of random bipartite mixed states. In particular, most of the random states in this specific class have relative entropy of entanglement and distillable entanglement equal to some fixed number (to within an arbitrary small error), thereby hugely reducing the complexity of computation of these entanglement measures for this specific class of mixed states.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2018

Passive state preparation in the Gaussian-modulated coherent-states quantum key distribution

In the Gaussian-modulated coherent-states (GMCS) quantum key distribution (QKD) protocol, Alice prepares quantum states actively: For each transmission, Alice generates a pair of Gaussian-distributed random numbers, encodes them on a weak coherent pulse using optical amplitude and phase modulators, and then transmits the Gaussian-modulated weak coherent pulse to Bob. Here we propose a passive state preparation scheme using a thermal source. In our scheme, Alice splits the output of a thermal source into two spatial modes using a beam splitter. She measures one mode locally using conjugate optical homodyne detectors, and transmits the other mode to Bob after applying appropriate optical attenuation. Under normal conditions, Alice's measurement results are correlated to Bob's, and they can work out a secure key, as in the active state preparation scheme. Given the initial thermal state generated by the source is strong enough, this scheme can tolerate high detector noise at Alice's side. Furthermore, the output of the source does not need to be single mode, since an optical homodyne detector can selectively measure a single mode determined by the local oscillator. Preliminary experimental results suggest that the proposed scheme could be implemented using an off-the-shelf amplified spontaneous emission source.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2025

Classifying One-Dimensional Quantum States Prepared by a Single Round of Measurements

Measurements and feedback have emerged as powerful resources for creating many-body quantum states. However, a detailed understanding has been restricted to fixed-point representatives of phases of matter. Here, we go beyond this and characterize the patterns of many-body entanglement that can be deterministically created from measurement. Focusing on one spatial dimension, a framework is developed for the case where a single round of measurements is the only entangling operation. We show this creates matrix-product states and identify necessary and sufficient tensor conditions for preparability, which uniquely determine the preparation protocol. We use these conditions to both classify preparable quantum states and characterize their physical constraints. In particular, we find a trade-off between the richness of the preparable entanglement spectrum and correlation functions, which leads to a no-go theorem for preparing certain quantum states. More broadly, we connect properties of the preparation protocol to the resulting phase of matter, including trivial, symmetry-breaking, and symmetry-protected topological phases—for both uniform and modulated symmetries. This work offers a resource-theoretic perspective on preparable quantum entanglement and shows how to systematically create states of matter, away from their fixed points, in quantum devices. Published by the American Physical Society 2025

Sahay, Rahul (ORCID:0000000174579826)↗
DOE OSTI2024

Utilizing Quantum Cascade Lasers for Ultranarrow Velocity Resolution and Quantum-State Selectivity in Molecular Beam Scattering and Spectroscopy

Here, we demonstrate the capability of a narrow linewidth quantum cascade laser (QCL) to selectively excite a very narrow velocity range of nitric oxide (σ ≤ 7(3) m/s) with a pure ro-vibrational quantum state. By implementing a counter-propagating geometry, the molecules are selectively excited according to the Doppler shift of the ro-vibrational transition frequency such that the velocity width associated with the excited molecules depends only on the QCL linewidth. We demonstrate a velocity distribution limited by the effective linewidth of our free-running QCL (Γ = 3.2 MHz). Our development provides a cost-effective, flexible approach to resolve quantum-state selective chemical dynamics with excellent velocity resolution in a wide variety of molecules with infrared-active transitions. This technique has been formulated to provide ultrahigh collisional energy resolution in molecular beams to delineate final quantum-state product pairs in studies of molecular collisions.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗