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At least 73 records · Page 4

Steady-State Thermal-Hydraulic Analysis of the LEU-Fueled Dalat Nuclear Research Reactor

This paper presents results of steady-state thermal-hydraulic analysis for the designed working core of the Dalat Nuclear Research Reactor (DNRR) using the PLTEMP/ANL code. The core was designed to be loaded with 92 low-enriched uranium (LEU) VVR-M2 fuel bundles (FBs) and 12 beryllium rods surrounding a neutron trap at the core center, for replacement of the previous core with 104 high-enriched uranium (HEU) VVR-M2 FBs. Before using this code for thermohydraulic analysis of the designed LEU working core, it was validated by comparing calculation results with experimental data collected from the HEU working core of the DNRR. The discrepancy between calculated results and measured data was at the maximum about 0.8°C and 1.5°C of fuel cladding and outlet coolant temperatures, respectively. In the design calculation, thermohydraulic safety was confirmed through evaluation of the fuel cladding and coolant temperatures, as well as of other safety parameters such as Departure from Nucleate Boiling Ratio (DNBR) and Onset of Nucleate Boiling Ratio (ONBR). The calculation results showed that, in normal operation conditions at full nominal thermal power of 500 kW without uncertainty parameters, the maximum fuel cladding temperature of the hottest FB was about 90.4°C, which is lower than its limit value of 103°C, the minimum DNBR was 32.0, which is much higher than the recommended value of 1.5, and the minimum ONBR was 1.43, which is higher than the recommended value of 1.4 for VVR-M2 LEU fuel type. When the global and local hot channel factors were taken into account, the maximum temperature of fuel cladding at the hottest FB was about 98.4 °C, for global only, and 114.3°C, for global together with local hot channel factors. The calculation results confirm the safety operation of the designed LEU core loaded with 92 fresh VVR-M2 FBs.

Nguyen, Kien-Cuong↗

Nondestructive measurements of residual 235 U mass of Israeli Research Reactor-1 fuel using the Advanced Experimental Fuel Counter

In 2018, a measurement campaign took place with participants from Los Alamos National Laboratory (LANL), the Nuclear Research Centre-Negev (NRCN) and Soreq Nuclear Research Center (SNRC) at the Israeli Research Reactor-1 (IRR-1) in which 14 of the reactor’s used fuel assemblies (FAs) with varied amount of depletion were measured with the nondestructive assay instrument Advanced Experimental Fuel Counter (AEFC). Designed for safeguards purposes, the AEFC measures both neutrons emitted from the FA (passive neutrons) and fission neutrons induced by an external neutron source (in this experiment, 252 Cf). Signals recorded with the AEFC include total neutron count rates (Singles), time-correlated neutron count rates (Doubles), and total gamma-ray count rates. The 235 U content of the FAs was previously assessed by two independent methods: (1) measurement of the transparency of the FA to low-energy gamma rays from an activated rhenium source (rhenium gamma transmission, or the RGT method) and (2) calculation of the 30-year burnup history of the core using detailed three-dimensional Monte-Carlo core depletion calculations. The results from the FAs that had been measured via the RGT method were used to construct the calibration curves, which translate the AEFC count rates to 235 U mass. Then, the calibration was evaluated using AEFC measurements of six additional FAs that were not measured via the RGT method. From the results, it was determined the Doubles calibration curve was more reliable than that of the Singles and follows a simple second-order polynomial fit for the whole range of residual 235 U mass content, albeit with larger statistical uncertainty. Detailed uncertainties quantification was conducted for both the AEFC Singles and Doubles. This includes the analysis of statistical uncertainties, calibration uncertainty, and random uncertainties due to the sensitivity of the AEFC to several sources of uncertainty, namely the FA position, FA orientation, interrogation source position, and ambient pool temperature. Finally, an overall total uncertainty of 6 g of 235 U is estimated for the Singles and Doubles, which is mainly due to calibration uncertainty (for the Singles) and statistical uncertainty (for the Doubles), and which constitutes 3%–6% of the 235 U total mass in the FAs, depending on their level of depletion.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Purification of U from U-10Mo scrap generated during the fabrication of high performance research reactor fuel

A low enriched U-Mo alloy fuel is under development to replace highly enriched U fuels currently used in United States high performance research reactors. The alloy casting and fuel fabrication processes will generate scrap streams containing low enriched U (LEU) which must be recovered. Solvent extraction processes were designed using the Argonne Model for Universal Solvent Extraction (AMUSE) to purify solutions containing 20 and 50 g/L U. The feed for the solvent extraction processes was prepared from solutions generated from the dissolution of U-10Mo-Zr foils and U-10Mo-Zr-Al mini-plates. The U purification processes were demonstrated using two, 16-stage banks of miniature mixer-settlers. The solvent extraction experiments demonstrated that all design objectives for the U purification processes could be met. The U recovery in the product stream for each flowsheet was ≥99.9%. The flowsheet demonstrations also showed that the purity of the U Product will meet the requirements of the ASTM International C1462-21 specification for LEU metal enriched to less than 20% 235 U. In conclusion, the AMUSE modeling for both flowsheet demonstrations was validated by comparing predicted and measured concentrations of U, Mo, and Zr in the exit streams and stage samples at steady-state conditions in the mixer-settlers.

modified PUREX process↗

Transition Core Analysis for HEU to LEU Fuel Conversion at the University of Missouri Research Reactor

A new type of low-enriched uranium (LEU) fuel based on an alloy of uranium and molybdenum is expected to allow the conversion of U.S. domestic high-performance research and test reactors requiring high density fuel from highly enriched uranium (HEU) to LEU. The University of Missouri Research Reactor (MURR (R)) has undergone design and performance calculations for conversion to this LEU fuel. Presented in this paper is the analysis of a crucial step in the conversion process: the sequence of MURR transition cores from all fresh to equilibrium burnup LEU operations. During the initial conversion from HEU to LEU fuel, MURR will operate atypically due to the lack of burned LEU elements. Given the constraints of MURR operation and experiments, a proposed transition scheme minimizes the time MURR operates atypically compared to the prototypic cycles currently run with HEU fuel and moves quickly to the same sort of equilibrium cycles for the LEU fuel.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Simulations of neutron noise in the research reactor AKR-2: comparison between a discrete ordinates and a diffusion-based method

A diffusion-based and a discrete ordinates method are used to simulate a neutron noise experiment in the research reactor AKR-2 at the Technical University in Dresden, Germany. The AKR-2 reactor provides an interesting case for the comparison between the two methods because it is characterized by large heterogeneities and regions with low macroscopic neutron cross-sections. For the calculations, the same spatial discretization and the same set of two-energy macroscopic neutron cross-sections with isotropic scattering are used. Significant discrepancies between the diffusion-based and discrete ordinates methods are found in regions of the systems where the diffusion approximation is expected to be inaccurate in reproducing characteristics of the static neutron flux and neutron noise. (authors)

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Fuel Design and Fabrication: Research Reactor Fuel

The objective of this chapter is to inform the reader on the essential aspects of design and fabrication of nuclear fuel systems utilized in research and test reactors. Fuel attributes of interest include mechanical, physical, and thermal properties as well as overall manufacturability. The chapter focuses primarily on plate-type fuels utilized in the highest power research reactors where design and function are critical to operational safety and successfully meeting each reactor’s unique mission.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Uranium–Molybdenum Alloy Critical Experiments for the Design of the Health Physics Research Reactor

Clean critical experiments with a uranium-molybdenum alloy (average of 10.1616 wt. % Mo with a density of 17.08 g/cm 3 ) were performed at the Oak Ridge Critical Experiments Facility in 1961 to support the design of the Health Physics Research Reactor (HPRR). The HPRR was similar to the Godiva burst reactor at Los Alamos National Laboratory and was designed to produce 50 microseconds burst of 10 17 fission pulses of radiation for dosimetry measurements, initially in support of the determination of the doses from the nuclear detonations in Japan during World War II. These experiments reported here were used to verify the calculational methods used to design the HPRR. These delayed critical measurements were:1) a solid unreflected and unmoderated 8-in.-dimeter U-Mo cylinder, 2) an unmoderated and unreflected annulus with 8-in.-outside diameter, 2-in.-inside diameter cylinder with a central void, 3) an unmoderated and unreflected annulus with 8-in.-outside diameter, 2-in.-inside diameter cylinder with a central void filled with stainless steel, 4) Same as 3) but with 3-in-thick Plexiglas reflector on top with and without cadmium between the reflector and the U-Mo alloy assembly with steel in the center, and 5) an unmoderated and unreflected annulus which was a modification of the second but with the lower 5 inches of the central hole enlarged to 3.5 in. with various reflector conditions. The reflector conditions were: 1-in.-thick Plexiglas on all outer surfaces-void in the center; 1-in.-thick Plexiglas on all outer surfaces-Plexiglas in the center; 2-in.- thick Plexiglas on radial surface-void in the center; 6-in.-thick Plexiglas on the bottom only-Plexiglas in the center; and 6-in.-thick Plexiglas on bottom, 1-in.-thick on top and on the lower 8.25-cm.-section of the radial surface-void in the center. For some of these reflector conditions 0.025-cm.thick cadmium was located between the reflector and the U-Mo alloy. The uranium contained 93.17 wt. % 235 U. Reflection was a safety concern for this unmoderated and unreflected reactor and reduction of reflection effects was also investigated by insertion of neutron absorber around the U-Mo alloy. The stainless steel 304 contained 18% nickel and 8% chromium and the rest iron. The reflector material was a methacrylate plastic (Plexiglas) containing 5.8 x 10 22 atoms/cm 3 of hydrogen and 3.6 x 10 22 atoms/cm 3 of carbon with a density of 1.20 g/cm 3 . The purpose of this report is to document the experimental information for the measurements performed so that at a later date researchers could perform the required uncertainty and calculational analyses and documentation to use these data for an International Nuclear Criticality Safety Benchmark Program (ICSBEP) or a EURATON Nuclear Energy Agency (NEA) benchmark. The data from the experiments described should be acceptable for use as criticality safety benchmark experiments for the ICSBEP and the NEA nuclear criticality safety benchmark program, once the uncertainty analysis is completed. Based on previous ICSBEP benchmarks with this enriched uranium metal at ORCEF, the uncertainties in k eff could be as low as ±0.0002 for some configurations.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Gaseous fuel nuclear reactor research

Gaseous-fuel nuclear reactors are described; their distinguishing feature is the use of fissile fuels in a gaseous or plasma state, thereby breaking the barrier of temperature imposed by solid-fuel elements. This property creates a reactor heat source that may be able to heat the propellant of a rocket engine to 10,000 or 20,000 K. At this temperature level, gas-core reactors would provide the breakthrough in propulsion needed to open the entire solar system to manned and unmanned spacecraft. The possibility of fuel recycling makes possible efficiencies of up to 65% and nuclear safety at reduced cost, as well as high-thrust propulsion capabilities with specific impulse up to 5000 sec.

Schwenk, F. C.↗

Startup Test Plan and Predictions for Highly Enriched Uranium to Low-Enriched Uranium Fuel Conversion at the University of Missouri Research Reactor

Nonpower reactors licensed by the U.S. Nuclear Regulatory Commission require a startup test plan as part of any facility modification to verify operability prior to resumption of operations. In order to support conversion of the University of Missouri Research Reactor from the use of highly enriched uranium to low-enriched uranium (LEU) fuel, a startup test plan has been devised to measure certain reactor physics parameters for the initial all-fresh LEU core licensing documentation that will be submitted. These parameters include the approach to critical, primary coolant void coefficient of reactivity, flux trap void coefficient of reactivity, determination of flux trap sample reactivity worth, radial and axial thermal neutron flux mapping, control blade worth calibration, primary and pool coolant temperature coefficient of reactivity, and flux mapping of experimental positions. Here, predictions for these parameters made using the Monte Carlo N-Particle Version 5 (MCNP5) radiation transport code are reported. These predictions will support the startup tests by providing a baseline set of expectations and additional insight into the performance of the LEU core.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

University of Missouri Research Reactor LEU Fuel Element Flow Test Conceptual Design

As part of the U.S. National Nuclear Security Administration’s (NNSA’s) mission to eliminate or minimize the civilian use of weapon-grade highly enriched uranium (HEU) fuels, the NNSA Office of Material Management and Minimization (M 3 ) Conversion Program is collaborating with six U.S. High Performance Research Reactors (USHPRR), including one critical facility, to convert from the use of HEU to low-enriched uranium (LEU) fuel. The M 3 conversion objectives for the USHPRR are to develop LEU fuel-element designs that will ensure safe reactor operations, as well as maintain the existing experimental performance of each facility. The work is being conducted through many interrelated activities that are being completed by stakeholders across organizations.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Irradiation Results of Commercial Neutron and Gamma Sensors at the Ohio State University Research Reactor

This report serves to present the evaluation results of commercial radiation detectors (SPNDs) with the potential to accomplish the data objectives—having sufficient gamma and fast neutron sensitivity—at temperatures near 650°C. The detectors chosen for evaluation are gamma ion chambers from Exosens (previously known as Photonis) models CRGA11 and CRGE32 and tantalum-based self-powered neutron detectors (Ta-SPND) from Mirion. The evaluation was performed in a series of heat irradiations from ambient to 850°C in the 9.5-inch dry tube furnace at the Ohio State University Research Reactor (OSURR). Ion chamber counting curves were measured to evaluate sensor operability at temperature. Detector sensitivity to reactor power and temperature were measured and presented in curve fit parameters. The curve fit equations were used to identify the suggested operational temperatures based on reactor power. Overall, it was evaluated that the CRGA11 was not significantly affected by temperatures up to 650°C and is operable—with higher temperature-contributed signals—up to 700°C. The CRGE32 was more affected by the high temperatures compared to the CRGA11. As a result of increasing temperature, the leakage current was a dominating factor. While the detector can operate up to 600°C and 700°C with lowered high voltage, it is not recommended unless a suitably strong gamma flux field is present. Finally, Ta SPND did not demonstrate good performance beyond 350°C due to the presence of an unknown phenomenon at changing temperatures. The study of the phenomenon is an active research topic outside the scope of this project.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Research Reactors Division Infrastructure Investment Plan for the High Flux Isotope Reactor

The High Flux Isotope Reactor (HFIR) is a unique national asset. Operational for nearly 60 years, continued investment into the aging infrastructure is necessary to ensure operation for another 6 decades. Additionally, growing missions require HFIR as well as important upgrades. Consequently, carefully integrated planning is required to ensure that infrastructure investments are timely executed to ensure long-term, reliable operation of HFIR. Concerns about challenges to the operational reliability of HFIR resulted in a recommendation from the 2023 Operations Review by the US Department of Energy (DOE) Office of Basic Energy Sciences that a HFIR management strategy be developed to address the infrastructure needs. This report defines the investment needs, which are evolving as new upgrade efforts are better defined. HFIR is part of the three-source strategy within the Neutron Sciences Directorate (NScD) and contributes to the five strategic science areas outlined in the NScD 10 Year Strategic Science Plan: quantum materials, soft matter, materials and engineering, chemistry, and biosciences. Fundamental to this strategy are three core values: operational excellence, responsible stewardship, and servant leadership. These values guide our mission of safe and reliable operation of the reactor and require a strong and just nuclear safety culture, a solemn respect for responsible care of the facility, good workforce development, robust procedures and processes, an effective communication strategy, world-class asset management, a determined customer focus, and a commitment to protecting the environment, the safety and health of the public and our people, and the quality of work performed within our facility. These principles are all essential to operate HFIR at a world-class level. The Research Reactors Division (RRD) will lead a new era of neutron science and isotope production at HFIR through responsible and purposeful leadership and unwavering support of the science community. The approach outlined in this plan highlights the direction leadership is taking to ensure that HFIR is ready to support the science challenges and national needs of the future and that the United States maintains world leadership in neutron sciences. The plan is in alignment with the DOE’s desire to continue operating HFIR and with the NScD strategic science goals for the future. HFIR is an aging facility with numerous infrastructure challenges and needs. It has an aging workforce in relation to the general population of Oak Ridge National Laboratory (ORNL), with many expected retirements over the next 5–10 years. With an increase in work scope caused by changing national priorities and science goals, several critical hires have been identified. To manage HFIR’s infrastructure needs, a prioritized list of equipment upgrades has been identified along with an analysis of future staffing requirements. A desire to operate HFIR at eight cycles per year will necessarily require some significant changes to procedures and processes currently in place as well as targeted staffing additions. Many of the equipment upgrades identified in this plan will significantly increase the reliability of the plant, thus contributing to the effort to reach the goal of safely operating eight cycles per year. A plan to attain eight-cycle operation is being prepared in parallel with the activities identified in this plan, although the actions identified to satisfy both plans will overlap. This plan identifies new infrastructure needs—for both plant equipment and staffing—thus necessitating formulation of future budget requests to fund the increased work scope and improvement activities. Some activities are currently being scheduled with the expectation that funding will be received. Any delays to funding or reductions of funding from the identified cost estimations will directly and negatively affect the plan’s implementation.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Short-lived noble gas effluent trends from a research reactor

An understanding of anthropogenic sources of radioactive noble gases in the atmosphere is needed to enhance the discrimination ability of the International Monitoring System's sensors. These sources include commercial and research nuclear reactors and medical isotope production facilities. While abiding by local environmental ordinances these facilities all emit noble gas radioisotopes through normal operation. Here, this research presents measurements and analysis of noble gas isotopes ( 41 Ar, 135 Xe, 135m Xe, 137 Xe, 138 Xe, 87 Kr, 88 Kr, and 89 Kr) made directly at the stack of the High Flux Isotope Reactor (HFIR) at Oak Ridge National Laboratory. The Xe and Kr noble gases are concurrently observed with 41 Ar, a neutron activation product, when the reactor is operational. The magnitude of the Xe and Kr noble gases released is not constant over the HFIR cycle, but they temporally match the 41 Ar trend. An isotope activity ratio analysis of these shorter lived isotopes combined with the observation of the cycle's temporal trend helps understand the noble gas production mechanism at the HFIR. Isotopes with short half-lives are not useful for long-range environmental monitoring. However, these measurements could potentially be combined with atmospheric modeling to predict the background source term of the longer-lived Xe ratios at a monitoring station.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

An Evaluation and Qualification of U.S.-Based Research Reactors for Irradiation Capabilities Supporting Advanced Nuclear Systems

Irradiation experiments are a prerequisite for evaluating nuclear reactor system designs, analyzing the performance of these systems, and obtaining licenses. Likewise, irradiation facilities are necessary for producing the radioisotopes used in industrial and medical applications. Recent developments in modeling and simulation capabilities and advancements in computational resources have further enabled the design of irradiation experiments for evaluating radiation-induced phenomena and determining nuclear fuel, material, and system design and safety criteria pertaining to both normal and accident scenarios. These computational tools and models require comprehensive experimental datasets acquired under prototypic radiation conditions—for exploring material and system performance under the uniquely harsh environments found in nuclear reactors—to enable verification and validation for qualification and licensing purposes. However, qualification of irradiation experimental facilities, primarily research and test reactors (RTRs), necessitates that their performance be evaluated based on the irradiation environment (e.g. flux, power, testing capabilities) using an appropriate scoring matrix. Although many university campus RTRs are available for research and development (R&D) activities and initiatives, this study focuses on evaluating and qualifying the irradiation facilities (mostly RTRs) within the United States that are suitable for advanced nuclear fuel, material, and system irradiation experiments aimed at establishing operational-performance limits and informing component and fuel designs so as to improve operational efficiencies and mitigate proliferation vulnerabilities, as well as for radioisotope production aimed at multipurpose applications. As a result, the findings of the present study support the acceleration of nuclear fuel and material qualifications, thus hastening new and advanced nuclear energy system demonstrations and radioisotope production efforts by using extended R&D.

irradiation experiment↗

Impact of boundary layer simulation on predicting radioactive pollutant dispersion: a case study for HANARO Research Reactor using the WRF-MMIF-CALPUFF modeling system

Wind plays an important role in cases of unexpected radioactive pollutant dispersion, deciding distribution and concentration of the leaked substance. The accurate prediction of wind has been challenging in numerical weather prediction models, especially near the surface because of the complex interaction between turbulent flow and topographic effect. As such, in this study, we investigated the characteristics of atmospheric dispersion of radioactive material (i.e. 137 Cs) according to the simulated boundary layer around the HANARO research nuclear reactor in Korea using the Weather Research and Forecasting (WRF)-Mesoscale Model Interface (MMIF)-California Puff (CALPUFF) model system. We examined the impacts of orographic drag on wind field, stability calculation methods, and planetary boundary layer parameterizations on the dispersion of radioactive material under a radioactive leaking scenario. We found that inclusion of the orographic drag effect in the WRF model improved the wind prediction most significantly over the complex terrain area, leading the model system to estimate the radioactive concentration near the reactor more conservatively. We also emphasized the importance of the stability calculation method and employing the skillful boundary layer parameterization to ensure more accurate low atmospheric conditions, in order to simulate more feasible spatial distribution of the radioactive dispersion in leaking scenarios.

54 ENVIRONMENTAL SCIENCES↗

The use of U3Si2/Al dispersion fuel for high power research reactors

In order to investigate the irradiation performance of U3Si2/Al dispersion fuel at relatively aggressive reactor conditions, compared to how this fuel is typically used in a research or test reactor, post irradiation examination was performed on two fuel plates that were irradiated at ~270 W/cm2 average surface heat flux and to a maximum local burnup greater than 8 × 1021 fissions/cm3 in the Advanced Test Reactor as part of the RERTR-8 experiment. As part of the non-destructive examinations that were performed on both fuel plates, detailed thickness measurements using a high-fidelity measurement bench were performed on one fuel plate and a segment of the second fuel plate. This paper provides the first reported results of such high-resolution thickness measurements for U3Si2/Al dispersion fuel plates, containing primarily the U3Si2 fuel phase, irradiated at such power levels to high burnup. For destructive examination using optical metallography, samples were generated from both irradiated plates. Localized regions of high swelling (characteristic of internal blistering) were observed on the surface of both fuel plates, suggesting that the performance limits had been reached for each plate. Destructive examinations showed that the fuel particles that are primarily U3Si2, which become amorphous during irradiation, in both plates contained relatively large fission gas bubbles with evidence of fission gas bubble interconnection.

Wachs, Daniel M.↗

High-Temperature Gas-Cooled Reactor Research Survey and Overview: Preliminary Data Platform Construction for the Nuclear Energy University Program

Since the U.S. Department of Energy Office of Nuclear Energy initiated the Nuclear Energy University Program (NEUP) in 2009, there are 29 NEUP projects focusing on high-temperature gas-cooled reactor (HTGR) research up to July 2022. The resultant research product, either experimental or computational, were published as final NEUP reports, journal articles and conference proceedings. However, these federally funded products have been scattered and sometimes cannot be easily accessed. To improve access to this valuable HTGR validation data and optimize the return on the significant investment made by the Department of Energy, the Advanced Reactor Technologies (ART) Gas-Cooled Reactor (GCR) program started a survey of completed and ongoing HTGR NEUP projects to develop a public-access database specific for HTGRs applications that can be used to retrieve computational fluid dynamics and system code validation data. This effort will help guide future NEUP-funded research, define new state of the ART Phenomena Identification and Ranking Table (PIRT), and promote the usage of this data in the codes validation matrices. This report provides an overview of the NEUP-funded HTGR-related research projects from Fiscal Year (FY) 2009–2021 and identifies validation knowledge gaps still existing in HTGR thermal-fluid research. A preliminary data platform has been developed for the 29 NEUP projects investigating HTGR thermal hydraulics, including their final reports as well as the available scientific publications. As an ultimate goal for this work, the ART-GCR program will create a central database at Idaho National Laboratory to identify, organize, and store these datasets generated by experimental investigations or computational models, experimental facility descriptions, and publicly-available academic products from the HTGR-related NEUP projects and provide future guidance for the storage and transmission of important project documentations for later NEUP projects as well.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗