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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 73 records · Page 4
All sourcesNASA NTRSDOE OSTI
DOE OSTI2026

Millimeter-wave Detections of Symbiotic Stars in SPT and ACT Data

We present the results of a joint targeted search of candidate symbiotic stars at millimeter wavelengths using the South Pole Telescope (SPT) and the Atacama Cosmology Telescope (ACT). Candidates are selected from the New Online Database of Symbiotic Variables, restricting to objects that are within either the SPT-3G or ACT~DR6 footprint, covering most of the southern hemisphere and up to a declination of $+20^\circ$. Forced photometry on the 828 candidate symbiotic star locations in SPT and ACT data results in 31 unique objects detected with more than a $3σ$ significance using two frequency bands: 18 confirmed and 13 suspected symbiotic stars. We provide the SPT and ACT 95/98, 150, and 220~GHz light curves, along with optical and infrared light curves from 2016--2026, as well as spectral energy distributions, physical parameters from the literature, and brief summaries regarding the nature of each individual object. Using Herschel SPIRE data from 2013, we place upper limits on millimeter flux for CN Cha near the beginning of the optical rise in its 2012/2013 nova, which suggests a strong variability and lag at millimeter wavelengths and results in a rare observance of a Galactic millimeter slow transient. In addition, we provide coadded thumbnails and light curves for the remaining 797 candidate symbiotic stars that did not pass our detection thresholds. Millimeter-wave emission from symbiotic stars is primarily a combination of free-free emission of the ionization region and optically thick blackbody emission of the cooler dust components of the system. When combined with contemporaneous multi-wavelength observations, millimeter-wave observations can be used to test binary models of symbiotic stars and provide insight on the geometry and physical properties of these systems.

Tandoi, C. [Illinois U., Urbana, Astron. Dept.] (O↗
DOE OSTI2021

Transparent window 2D IR spectroscopy of proteins

Proteins are complex, heterogeneous macromolecules that exist as ensembles of interconverting states on a complex energy landscape. A complete, molecular-level understanding of their function requires experimental tools to characterize them with high spatial and temporal precision. Infrared (IR) spectroscopy has an inherently fast time scale that can capture all states and their dynamics with, in principle, bond-specific spatial resolution. Two-dimensional (2D) IR methods that provide richer information are becoming more routine but remain challenging to apply to proteins. Spectral congestion typically prevents selective investigation of native vibrations; however, the problem can be overcome by site-specific introduction of amino acid side chains that have vibrational groups with frequencies in the “transparent window” of protein spectra. This Perspective provides an overview of the history and recent progress in the development of transparent window 2D IR of proteins.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2021

Infrared Light-Emitting Devices from Antenna-Coupled Luttinger Liquid Plasmons In Carbon Nanotubes

Electrically driven light-emitting devices provide highly energy-efficient lighting at visible wavelengths, and they have transformed photonic and electronic lighting applications. Efficient infrared light-emitting devices, however, have been challenging because band gap emission from semiconductors becomes inefficient in the mid-infrared to far-infrared spectral range. Here, in this paper, we investigate infrared light-emitting devices (IRLEDs) based on Luttinger liquid (LL) plasmons in one-dimensional (1D) metallic carbon nanotubes. Elementary excitations in LL are characterized by collective charge and spin excitations, i.e., plasmons and spinons. Consequently, electrons injected into the nanotubes transform efficiently into LL plasmons, a hybrid excitation of electromagnetic fields and electrons. We design nanoantennas coupled to the carbon nanotube to radiate LL plasmons into the far field. LL-based IRLEDs can be designed to selectively emit at wavelengths across the far- and mid-infrared spectra. An electrical-to-optical power conversion efficiency up to 3.2% may be achieved. Such efficient and narrowband LL-based IRLEDs can enable novel infrared nanophotonic applications.

36 MATERIALS SCIENCE↗
DOE OSTI2020

Anisotropic Fano resonance in the Weyl semimetal candidate LaAlSi

Topological Weyl semimetal (WSM) is a solid-state realization of chiral Weyl fermions, whose phonon behaviors provide in-depth knowledge of their electronic properties. In this work, anisotropic Fano resonance is observed in a type-II WSM candidate LaAlSi by polarized Raman spectroscopy. The asymmetric line shape occurs for the $B^2_1$ phonon mode of LaAlSi only for 488- and 532-nm laser excitations but not for 364-, 633-, and 785-nm excitations, suggesting the excitation selectivity. The asymmetry, frequency, and linewidth of the $B^2_1$ phonon mode, along with the spectral background, all show fourfold rotational symmetry as a function of the polarization angle in the polarized Raman spectra. While the shift of Raman frequency in a metal or semimetal is typically attributed to Kohn anomaly, here we show that the anisotropic frequency shift in LaAlSi cannot be explained by the effect of Kohn anomaly, but potentially by the anisotropic scattering background of Fano resonance. Origins of the excitation-energy dependence and anisotropic behavior of the Fano resonance are discussed by the first-principles calculated electronic band structure and phonon dispersion.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2023

A novel Doppler backscattering (DBS) system to simultaneously measure radio frequency plasma fluctuations and low frequency turbulence

A novel quadrature Doppler Backscattering (DBS) system has been developed and optimized for the E-band (60–90 GHz) frequency range using either O-mode or X-mode polarization in DIII-D plasmas. In general, DBS measures the amplitude of density fluctuations and their velocity in the lab frame. The system can simultaneously monitor both low-frequency turbulence (f < 10 MHz) and radiofrequency plasma density fluctuations over a selectable frequency range (20–500 MHz). Detection of high-frequency fluctuations has been demonstrated for low harmonics of the ion cyclotron frequency (e.g., 2f ci ~ 23 MHz) and externally driven high-frequency helicon waves (f = 476 MHz) using an adjustable frequency down conversion system. Importantly, this extends the application of DBS to a high-frequency spectral domain while maintaining important turbulence and flow measurement capabilities. This unique system has low phase noise, good temporal resolution (sub-millisecond), and excellent wavenumber coverage (k θ ~ 1–20 cm –1 and kr ≲ 30 cm –1 ). As a demonstration, localized internal DIII-D plasma measurements are presented from turbulence (f ≤ 5 MHz), Alfvenic waves (f ~ 6.5 MHz), ion cyclotron waves (f ≥ 20 MHz), as well as fluctuations around 476 MHz driven by an external high-power 476 MHz helicon wave antenna. In the future, helicon measurements will be used to validate GENRAY and AORSA modeling tools for prediction of helicon wave propagation, absorption, and current drive location for the newly installed helicon current drive system on DIII-D.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2023

Validation of the Cloud_CCI (Cloud Climate Change Initiative) cloud products in the Arctic

The role of clouds in the Arctic radiation budget is not well understood. Ground-based and airborne measurements provide valuable data to test and improve our understanding. However, the ground-based measurements are intrinsically sparse, and the airborne observations are snapshots in time and space. Passive remote sensing measurements from satellite sensors offer high spatial coverage and an evolving time series, having lengths potentially of decades. However, detecting clouds by passive satellite remote sensing sensors is challenging over the Arctic because of the brightness of snow and ice in the ultraviolet and visible spectral regions and because of the small brightness temperature contrast to the surface. Consequently, the quality of the resulting cloud data products needs to be assessed quantitatively. In this study, we validate the cloud data products retrieved from the Advanced Very High Resolution Radiometer (AVHRR) post meridiem (PM) data from the polar-orbiting NOAA-19 satellite and compare them with those derived from the ground-based instruments during the sunlit months. The AVHRR cloud data products by the European Space Agency (ESA) Cloud Climate Change Initiative (Cloud_CCI) project uses the observations in the visible and IR bands to determine cloud properties. The ground-based measurements from four high-latitude sites have been selected for this investigation: Hyytiälä (61.84°N, 24.29°E), North Slope of Alaska (NSA; 71.32°N, 156.61°W), Ny-Ålesund (Ny-Å; 78.92°N, 11.93°E), and Summit (72.59°N, 38.42°W). The liquid water path (LWP) ground-based data are retrieved from microwave radiometers, while the cloud top height (CTH) has been determined from the integrated lidar–radar measurements. The quality of the satellite products, cloud mask and cloud optical depth (COD), has been assessed using data from NSA, whereas LWP and CTH have been investigated over Hyytiälä, NSA, Ny-Å, and Summit.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2023

DESI z ≳ 5 Quasar Survey. I. A First Sample of 400 New Quasars at z ~ 4.7–6.6

We report the first results of a high-redshift (z ≳ 5) quasar survey using the Dark Energy Spectroscopic Instrument (DESI). As a DESI secondary target program, this survey is designed to carry out a systematic search and investigation of quasars at 4.8 < z < 6.8. The target selection is based on the DESI Legacy Imaging Surveys (the Legacy Surveys) DR9 photometry, combined with the Pan-STARRS1 data and J-band photometry from public surveys. A first quasar sample has been constructed from the DESI Survey Validation 3 (SV3) and first-year observations until 2022 May. This sample includes more than 400 new quasars at redshift 4.7 ≤ z < 6.6, down to 21.5 magnitude (AB) in the z band, discovered from 35% of the entire target sample. Remarkably, there are 220 new quasars identified at z ≥ 5, more than one-third of existing quasars previously published at this redshift. The observations so far result in an average success rate of 23% at z > 4.7. The current spectral data set has already allowed analysis of interesting individual objects (e.g., quasars with damped Lyα absorbers and broad absorption line features), and statistical analysis will follow the survey's completion. A set of science projects will be carried out leveraging this program, including quasar luminosity function, quasar clustering, intergalactic medium, quasar spectral properties, intervening absorbers, and properties of early supermassive black holes. Additionally, a sample of 38 new quasars at z ~ 3.8–5.7 discovered from a pilot survey in the DESI SV1 is also published in this paper.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2025

Band-Selective Spin-Charge Separation across the Charge Density Wave Transition in Quasi-1D NbSe 3

Non-Fermi liquid (non-FL) phase is a pivotal enigma in understanding intriguing quantum phases in strongly correlated systems, such as high-temperature superconductivity. Tomonaga-Luttinger liquid (TLL) theory, designed for one-dimensional (1D) systems, serves as one of the microscopic frameworks that elucidates non-FL behavior. Despite its theoretical concreteness, comprehensive experimental verification has remained incomplete. In particular, addressing the persistence of the TLL nature within ordered phases, such as charge density wave (CDW), has posed a significant challenge. We report the observation of TLL characteristics across the CDW transitions in a quasi-1D material NbSe 3 using angle-resolved photoemission spectroscopy. Spin-charge separation, a disentanglement of spin and charge degrees of freedom of electrons, is clearly observed within the band, accompanied by the suppression of spectral weight following a power-law behavior with anticipated temperature scaling. Surprisingly, the spin-charge separation persists even below the CDW transition temperatures, indicating the validity of the TLL nature in the CDW phase. In conclusion, our findings offer a unique opportunity to explore the interplay between the TLL and ordered phases, which could be connected to the interplay between non-FL and ordered phases in strongly correlated systems.

1-dimensional systems↗
DOE OSTI2023

eROSITA Final Equatorial-Depth Survey (eFEDS) eFEDS X-ray view of WERGS radio galaxies selected by the Subaru/HSC and VLA/FIRST survey

We constructed the eROSITA X-ray catalog of radio galaxies discovered by the WERGS survey, made by cross-matching the wide area Subaru/Hyper Suprime-Cam (HSC) optical survey and VLA/FIRST 1.4 GHz radio survey. We report finding 393 eROSITA detected radio galaxies in the 0.5-2 keV band in the eFEDS field covering 140 deg 2 . Thanks to the wide and medium depth eFEDS X-ray survey down to f 0.5 - 2 keV = 6.5 × 10 -15 erg s -1 cm -2 , the sample contains the rare and most X-ray luminous radio galaxies above the knee of the X-ray luminosity function, spanning 44 < log(L 0.5-2 keV (abs,corr) /erg s -1 ) < 46.5 at 1 < z < 4. The sample also contains the sources around and below the knee for the sources 41 < log(L 0.5-2 keV (abs,corr) /erg s -1 ) < 45 at z < 1. Based on the X-ray properties obtained by the spectral fitting, 37 sources show obscured active galactic nucleus (AGN) signatures with log(N H /cm -2 ) > 22. These obscured and radio AGN reside in 0.4 < z < 3.2, indicating that they are obscured counterparts of the radio-loud quasar, which were missed in the previous optical quasar surveys. By combining radio and X-ray luminosities, we also investigated the jet production efficiency η jet = η rad P jet /L AGN,bol by utilizing the jet power of P jet . We find that there are 14 sources with extremely high jet production efficiency at η jet ≈ 1. This high η jet value might be a result of the decreased radiation efficiency of η rad < 0.1, due to the low accretion rate for those sources, and/or of the boosting due to the decline of L AGN,bol by a factor of 10-100 by keeping P jet constant in the previous Myr, indicating the experience of the AGN feedback. Finally, inferring the BH masses from the stellar mass, we find that X-ray luminous sources show the excess of the radio emission with respect to the value estimated from the fundamental plane. This radio emission excess cannot be explained by the Doppler boosting alone, and therefore the disk–jet connection of X-ray luminous eFEDS-WERGS is fundamentally different from the conventional fundamental plane which mainly covers the low-accretion regime.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2022

Sub-threshold ultrafast one-photon photoemission from a Cu(111) photocathode

Single-photon photoemission of electrons for incident photon energies below the surface work function is reported for a single-crystal Cu(111) photocathode. Spectral characterization of the quantum efficiency and mean transverse energy of the emitted electrons is shown to be consistent with emission from a thermalized hot electron distribution photoexcited on sub-picosecond time scales into an upper conduction band at the L-point of the Brillouin zone of copper. To our knowledge, this is the first time that such excited-state thermionic emission has been observed from a planar metal photocathode, and then from a commonly used photocathode material. The results, therefore, indicate the potential importance of such band structure dependent sub-threshold photoemission mechanisms on the performance of photocathodes employed for the generation of short electron pulses using sub-picosecond laser pulses. Consequently, the combined experimental and theoretical work presented in this paper contributes to solid-state photocathode-based research aimed at our understanding and selection (or discovery) of high brightness photo-electron sources required for many electron-based diffraction, imaging, and accelerator applications.

43 PARTICLE ACCELERATORS↗
DOE OSTI2023

The rebrightening of a ROSAT -selected tidal disruption event: repeated weak partial disruption flares from a quiescent galaxy?

The ROSAT-selected tidal disruption event (TDE) candidate RX J133157.6-324319.7 (J1331) was detected in 1993 as a bright [0.2–2 keV flux of (1.0 ± 0.1) × 10 -12 erg s -1 cm -2 ], ultra-soft (kT = 0.11 ± 0.03 keV) X-ray flare from a quiescent galaxy (z = 0.051 89). During its fifth all-sky survey (eRASS5) in 2022, Spectrum-Roentgen-Gamma (SRG)/ eROSITA detected the repeated flaring of J1331, where it had rebrightened to an observed 0.2–2 keV flux of (6.0 ± 0.7) × 10 -13 erg s -1 cm -2 , with spectral properties (kT = 0.115 ± 0.007 keV) consistent with the ROSAT-observed flare ~30 yr earlier. In this work, we report on X-ray, ultraviolet, optical, and radio observations of this system. During a pointed XMM observation ~17 d after the eRASS5 detection, J1331 was not detected in the 0.2–2 keV band, constraining the 0.2–2 keV flux to have decayed by a factor of ≳40 over this period. Given the extremely low probability (~5 × 10 -6 ) of observing two independent full TDEs from the same galaxy over a 30 yr period, we consider the variability seen in J1331 to be likely caused by two partial TDEs involving a star on an elliptical orbit around a black hole. J1331-like flares show faster rise and decay time-scales [$\mathcal {O}(\mathrm{d})$] compared to standard TDE candidates, with negligible ongoing accretion at late times post-disruption between outbursts.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2024

Quantum sensing effect of electron tunneling in DQD/analyte complex

We investigate electron tunneling between quantum dots and molecules to propose a quantum sensor. This sensor consists of double quantum dots (DQD) with energy levels specifically tailored to mirror those of the target analyte. By analyzing the spectral distribution of electron localizations in the DQD system, we can delineate the analyte’s spectrum and deduce its composition by comparing it with a reference sample. To understand electron tunneling dynamics within the DQD/analyte complex, we performed three-dimensional computational modeling applying the effective potential approach to the InAs/GaAs heterostructure. In this modeling, we mimicked the analyte spectrum by utilizing a quantum well characterized by a quasi-discrete spectrum. Our calculations reveal the inherent potential of utilizing this method as a highly sensitive and selective sensor.

77 NANOSCIENCE AND NANOTECHNOLOGY↗
DOE OSTI2022

The gMOSS: the galaxy survey and galaxy populations of the large homogeneous field

ABSTRACT We present the gMOSS (Galaxies of Medium-band One-meter Schmidt telescope Survey) catalogue of ∼19 000 galaxies in 20 filters (4 broad-band SDSS and 16 medium-band filters). We observed 2.386 deg2 on the central part of the HS47.5-22 field with the 1-m Schmidt telescope of the Byurakan Astrophysical Observatory. The gMOSS is a complete flux-limited sample of galaxies with a threshold magnitude of r SDSS ≤ 22.5 AB. From photometric measurements with 16 medium-band filters and u SDSS, we get spectral energy distributions for each object in the field, which are used for further analysis. Galaxy classification and photometric redshift estimation based on spectral template matching with zebra software. The obtained redshift accuracy is σNMAD < 0.0043. Using the SED-fitting cigale code, we obtained the main properties of the stellar population of galaxies, such as rest-frame (u − r)res colour, stellar mass, extinction, and mass-weighted age with a precision of 0.16 ± 0.07 mag, 0.14 ± 0.04 dex, 0.27 ± 0.1 mag, and 0.08 ± 0.04 dex, respectively. Using a dust-corrected colour–mass diagram, we divided the full sample into populations of red and blue galaxies and considered the dependencies between stellar mass and age. Throughout cosmic time, red sequence galaxies remain older and more massive than blue cloud galaxies. The star formation history of a complete subsample of galaxies selected in the redshift range 0.05 ≤ z ≤ 0.015 with <$\mathrm{log} M \mathrm{\gt }_\mathrm{[M_\odot ]}$>8.3 shows an increase in the SFRD up to z ∼ 3, under the results obtained in earlier studies.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2020

The Hα Dots Survey. II. A Second List of Faint Emission-line Objects

We present the second catalog of serendipitously discovered compact extragalactic emission-line sources—Hα Dots. These objects have been discovered in searches of moderately deep narrow-band images acquired for the ALFALFA Hα project. In addition to cataloging 119 new Hα Dots, we also present follow-up spectral data for the full sample. These spectra allow us to confirm the nature of these objects as true extragalactic emission-line objects, to classify them in terms of activity type (star-forming or AGN), and to identify the emission line via which they were discovered. We tabulate photometric and spectroscopic data for the all objects, and we present an overview of the properties of the full Hα Dot sample. The Hα Dots represent a broad range of star-forming and active galaxies detected via several different emission lines over a wide range of redshifts. The sample includes Hα-detected blue compact dwarf galaxies at low redshift, [O iii]-detected Seyfert 2 and Green Pea-like galaxies at intermediate redshifts, and QSOs detected via one of several UV emission lines, including Lyα. Despite the heterogeneous appearance of the resulting catalog of objects, we show that our selection method leads to well-defined samples of specific classes of emission-line objects with properties that allow for statistical studies of each class.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2021

Toward white light emission from plasmonic-luminescent hybrid nanostructures

We study the light emission of plasmonic-luminescent hybrid nanostructures consisting of Ag nanoparticles (NPs) embedded in europium oxide (EuO X ). The Ag NPs present a bidimensional organization in the nanostructures and they optically behave as oblate spheroids. The photoluminescence (PL) spectral response of the nanostructures evolves from a narrow red emission characteristic of Eu 3+ ions in absence of Ag NPs to a broad blue-green emission band associated with Eu 2+ ions when the layer of Ag NPs is present. This behavior is not related to a change in the Eu 2+ /Eu 3+ ratio, which is verified by compositional analysis. Instead, a detailed investigation of the PL emission of the nanostructures suggests that the coupling of the Ag NPs to the Eu 2+ ions present in the EuO X layer, which manifests itself in an efficient sensitization of these ions, enhances their broad visible emission. In particular, the longitudinal mode of the Ag NPs surface plasmon is considered to be responsible for the efficient energy transfer for the non-normal incidence excitation PL configuration used. Finally, the use of a capping amorphous Al 2 O 3 layer allows improving the robustness of hybrid nanostructures and further enhances their PL emission. These findings provide a new path to actively control the selective excitation of Eu 2+ and Eu 3+ ions via a controlled coupling with the surface plasmon resonance modes of the Ag NPs and points to these nanostructures as promising building blocks for the development of integrable white light sources.

36 MATERIALS SCIENCE↗
DOE OSTI2020

Dark Energy Survey Identification of A Low-Mass Active Galactic Nucleus at Redshift 0.823 from Optical Variability

We report the identification of a low-mass active galactic nucleus (AGN), DES J0218−0430, in a redshift z = 0.823 galaxy in the Dark Energy Survey (DES) Supernova field. We select DES J0218−0430 as an AGN candidate by characterizing its long-term optical variability alone based on DES optical broad-band light curves spanning over 6 yr. An archival optical spectrum from the fourth phase of the Sloan Digital Sky Survey shows both broad Mg ii and broad H β lines, confirming its nature as a broad-line AGN. Archival XMM–Newton X-ray observations suggest an intrinsic hard X-ray luminosity of |$L_{{\rm 2-12\, keV}}\approx 7.6\pm 0.4\times 10^{43}$| erg s^−1, which exceeds those of the most X-ray luminous starburst galaxies, in support of an AGN driving the optical variability. Based on the broad H β from SDSS spectrum, we estimate a virial black hole (BH) mass of M_• ≈ 10^6.43–10^6.72 M_⊙ (with the error denoting the systematic uncertainty from different calibrations), consistent with the estimation from OzDES, making it the lowest mass AGN with redshift > 0.4 detected in optical. We estimate the host galaxy stellar mass to be M_* ≈ 10^10.5 ± 0.3 M_⊙ based on modelling the multiwavelength spectral energy distribution. DES J0218−0430 extends the M_•–M_* relation observed in luminous AGNs at z ∼ 1 to masses lower than being probed by previous work. Our work demonstrates the feasibility of using optical variability to identify low-mass AGNs at higher redshift in deeper synoptic surveys with direct implications for the upcoming Legacy Survey of Space and Time at Vera C. Rubin Observatory.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2021

Electronic Origin of T c in Bulk and Monolayer FeSe

FeSe is classed as a Hund’s metal, with a multiplicity of d bands near the Fermi level. Correlations in Hund’s metals mostly originate from the exchange parameter J, which can drive a strong orbital selectivity in the correlations. The Fe-chalcogens are the most strongly correlated of the Fe-based superconductors, with d xy the most correlated orbital. Yet little is understood whether and how such correlations directly affect the superconducting instability in Hund’s systems. By applying a recently developed ab initio theory, we show explicitly the connections between correlations in d xy and the superconducting critical temperature T c . Starting from the ab initio results as a reference, we consider various kinds of excursions in parameter space around the reference to determine what controls T c . We show small excursions in J can cause colossal changes in T c . Additionally we consider changes in hopping by varying the Fe-Se bond length in bulk, in the free standing monolayer M-FeSe, and M-FeSe on a SrTiO 3 substrate (M-FeSe/STO). The twin conditions of proximity of the dxy state to the Fermi energy, and the strength of J emerge as the primary criteria for incoherent spectral response and enhanced single- and two-particle scattering that in turn controls T c . Using c-RPA, we show further that FeSe in monolayer form (M-FeSe) provides a natural mechanism to enhance J. We explain why M-FeSe/STO has a high T c , whereas M-FeSe in isolation should not. Our study opens a paradigm for a unified understanding what controls Tc in bulk, layers, and interfaces of Hund’s metals by hole pocket and electron screening cloud engineering.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2025

Magnon damping and mode softening in quantum double-exchange ferromagnets

We present a comprehensive analysis of the magnetic excitations and electronic properties of fully quantum double-exchange ferromagnets, i.e. systems where ferromagnetic (FM) ordering emerges from the competition between spin, charge, and orbital degrees of freedom, but without the canonical approximation of using classical localized spins. Specifically, we investigate spin excitations within the Kondo lattice-like model, as well as a two-orbital Hubbard Hamiltonian in proximity to the orbital-selective Mott phase. Computational analysis of the magnon dispersion, damping, and spectral weight within these models reveals unexpected phenomena, such as magnon mode softening and the anomalous decoherence of magnetic excitations as observed in earlier experimental efforts, but explained here without the use of the phononic degrees of freedom. We show that these effects are intrinsically linked to incoherent spectral features near the Fermi level, which arise due to the quantum nature of the local (on-site) triplets. This incoherent spectrum leads to a Stoner-like continuum on which spin excitations scatter, governing magnon lifetime and strongly influencing the dynamical spin structure factor. Our study explores the transition from coherent to incoherent magnon spectra by varying the electron density. Furthermore, we demonstrate that the magnitude of the localized spin mitigates decoherence by suppressing the incoherent spectral contributions near the Fermi level. We also discuss the effective J 1 –J 2 spin Hamiltonian, which can accurately describe the large doping region characterized by the magnon-mode softening. Finally, we show that this behavior is also present in multiorbital models with partially filled orbitals, namely, in systems without localized spin moments, provided that the model is in a strong coupling regime. Our results potentially have far-reaching implications for understanding FM ordering in various multi-band systems. These findings establish a previously unknown direct connection between the electronic correlations of those materials and spin excitations.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗