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The consequences of the universally made assumption that the stimulated emission profile is identical to the absorption profile are quantitatively investigated for a two-level atom with Doppler redistribution. The nonlinear terms arising in the source function are evaluated iteratively. We find that the magnitude of the effects is probably completely negligible for visible and UV solar lines.
Resonant absorption in a laser pulse can be reduced to zero if the trailing part induces stimulated emission and returns the absorbed energy back to the pulse. This kind of effect is called Self-Induced Transparency (SIT). Analytic descriptions of short pulse propagation in a resonant medium, based on Slowly Varying Envelope Approximation (SVEA) and in linear media, have been extended in studies of SIT along two principal directions: First, to improve the SVEA by introducing Short Pulse Approximation (SPA); and second, to consider the effect of nonlinear refractive index.
The results of experiments performed to check the possibility of stimulated emission in the extreme vacuum ultraviolet (VUV) by an Al(+3) laser-generated plasma are reported. It is concluded that the spectral line intensity anomalies previously observed are not due to population inversion.
Charge-transfer reactions or Penning ionization reactions are used to produce population inversions between electronic states of molecular ions which should result in stimulated emission in ultraviolet and visible regions. Such lasers could be used in study of short-lived reaction intermediates, crystal structure and scattering, and photolysis.
The fabrication and application of metal-barrier-metal tunneling junctions for radiative interactions are discussed. Particular attention is given to the photolithographic fabrication of small area devices and the coupling to such devices via surface plasmon waves which play an important role at infrared and optical frequencies. It has been shown that the junction electron tunneling currents can be strongly coupled to surface plasmon junction modes, and spontaneous and stimulated emission of the latter are possible as well as nonlinear interactions. Finally, results demonstrating the photo-excitation of electrons with subsequent tunneling induced by ultraviolet radiation are presented. It is estimated that quantum efficiencies of the order of 5% and higher are possible in the ultraviolet region.
The present discussion deals with some theoretical aspects associated with the description of molecular rate processes in the presence of intense laser radiation, where the radiation actually interacts with the molecular dynamics. Whereas for weak and even moderately intense radiation, the absorption and stimulated emission of photons by a molecular system can be described by perturbative methods, for intense radiation, perturbation theory is usually not adequate. Limiting the analysis to the gas phase, an attempt is made to describe nonperturbative approaches applicable to the description of such processes (in the presence of intense laser radiation) as electronic energy transfer in molecular (in particular atom-atom) collisions; collision-induced ionization and emission; and unimolecular dissociation.
The operation of gamma ray lasers (gasers) are studied. It is assumed that the nuclear isomers mentioned in previously published papers have inherent limitations. It is further assumed that the judicious use of Bormann effect or the application of the total external reflection of low energy gamma radiation at grazing angle of incidence may permit the use of a gaser crystal sufficiently long to achieve observable stimulated emission. It is suggested that a long lived 0(+) isomer decaying by low energy gamma ray emission to a short lived 2(+) excited nuclear state would be an attractive gaser candidate. It is also suggested that the nuclear isomer be incorporated in a matrix of refractory material having an electrostatic field gradient whose principal axis lies along the length of the medium. This results in the preferential transmission of electric quadrupole radiation along the length of the medium.
The thermal and mechanical characteristics which will ultimately limit the performance of Nd:BeL at high average power levels were investigated. The output beam characteristics (pulse width, peak power, beam dimensions and collimation) were determined at high repetition rates for both Nd:BeL and Nd:YAG. The output of Nd:BeL was shown to exceed that of Nd:YAG by a factor of 2.7 at low Q-switched repetition rates (1 Hz). This result follows from the smaller stimulated emission cross section of x-axis Nb:BeL compared to that of NdYAG by the same factor. At high repetition rates (10 Hz) the output of Nd:Bel falls to a level of three-fifths of its low repetition rate value while under similar tests the output of Nd:YAG remains essentially constant. A comparison of the measured values of the elasto-optic coefficients, the dn/dT values and the linear expansion coefficients for BeL and YAG failed to provide an explanation for the performance of BeL; however, thermal lensing was observed in Nd:BeL. Results imply that the output of a high repetition rate Q-switched Nd:BeL laser (high thermal loading) could be dramatically increased by utilization of a resonator design to compensate for the thermal lensing effects.
The detection of methyl formate (HCOOCH3) in four transitions toward Orion KL, in two transitions toward Sagitarrius B2, and in one transition toward W51 is reported. The column densities of HCOOCH3 are found to be surprisingly large (2-5 x 10 to the 14th per sq cm) in all three clouds. Stimulated emission in the 18 cm K doublet of HCOOCH3 toward Sagittarius B2 is clearly demonstrated. The relatively large column densities of HCOOCH3 in clouds outside the galactic-center region probably imply that this molecule is widely distributed in the galaxy, but the negative results in other clouds require lower column densities than in Orion by a factor of 0.5 or less. Two unidentified lines were detected in Orion, at approx. 91 and 99 GHz.
The repetitive Q-switched performances of an x-axis neodymium-doped lanthanum beryllate (Nd:BeL) laser and the current state-of-the-art Nd:YAG laser are compared. Output beam pulse energy, peak power, pulse width, beam divergence and mode pattern were measured for a gold-plated single elliptical cavity using a xenon flashlamp for excitation. The output of the Nd:BeL laser is found to exceed that of the Nd:YAG laser by a factor of two at Q-switched repetition rates on the order of 1 Hz, due to the smaller stimulated emission cross section of the x-axis Nd:BeL. When the repetition rate is increased to 10 Hz, the Nd:BeL output falls to a level three fifths lower than its low-rate value, while Nd:YAG output remained essentially constant. Analysis reveals that the decrease in output may be attributed to a depolarization loss due to thermally induced stress birefringence.
A kinetic model for a solar-simulator pumped iodine laser system is developed and compared to an experiment in which the solar simulator output is dispersed over a large active volume (150 cu cm) with low simulator light intensity (approx. 200 solar constants). A trace foreign gas which quenches the upper level is introduced into the model. Furthermore, a constant representing optical absorption of the stimulated emission is introduced, in addition to a constant representing the scattering at each of the mirrors, via the optical cavity time constant. The non-uniform heating of the gas is treated as well as the pressure change as a function of time within the cavity. With these new phenomena introduced into the kinetic model, a best reasonable fit to the experimental data is found by adjusting the reaction rate coefficients within the range of known uncertainty by numerical methods giving a new bound within this range of uncertainty. The experimental parameters modeled are the lasing time, laser pulse energy, and time to laser threshold.
Near-UV and blue fluorescence from the 4D3/2 and 4D5/2 manifolds in Nd:YLF has been observed at room temperature under CW pumping by a rhodamine 590 dye laser. Excitation to these manifolds is attributed to two-step excitation involving excited-state absorption from the 4F3/2 metastable level. A similar phenomenon has also been observed in Nd:YAG and Nd:glass. The effective excited-state absorption cross section is measured to be (2 + or - 1) x 10 to the -20th sq cm at 587.4 nm in the pi polarization, and the peak effective stimulated emission cross section is measured to be 5 x 10 to the -20th sq cm at 411.7 nm, also in the pi polarization. Estimated laser threshold at 411.7 nm for two-step pumping at 587.4 nm is 70 mW.
Volume interchange factors are shown to be convenient in modeling the radiative processes in the wake of a hypersonic vehicle. Use of the factors facilitates calculating not just the radiative heating rates on afterbody surfaces but also the radiative de-excitation rates from stimulated emission and re-excitation rates from absorption in rarefied nonequilibrium flows. Sample calculations of volume interchange factors are presented for volume configurations modeling wake elements, and the numerical results are compared to limiting approximations to clarify the operation of the emission, transmission, and absorption processes.
Spectroscopic measurements and analysis of diode laser-pumped operation of Tm, Ho:YAG at 2.1 microns at room temperature have been performed. The peak effective stimulated emission cross section is measured to be 9 x 10-21 sq cm at 2.091 microns and the upper state lifetime is 8.5 ms. Under diode laser pumping, thresholds of 4.4 mW of absorbed power and slope efficiency of 19 percent have been demonstrated. Calculations of threshold power are performed based on the spectroscopic measurements. An energy transfer upconversion process is identified which leads to a sublinear rise in upper-state population with pump power.
Experimental process makes films with interesting magnetic and magneto-optical properties. Films of dilute magnetic semiconductor alloy Cd1-xMnxTe deposited on glass and GaAs substrates by metalorganic chemical-vapor deposition (MOCVD). Devices made with Cd1-xMnxTe films known to exhibit strong photoluminescence, stimulated emission, and magnetically-tunable lasing action. In addition, energy-band gaps of such material tailored by altering its composition - property giving flexibility in development of high-efficiency cascade solar photovoltaic cells. Performs at atmospheric pressure, resulting in more-uniform films, covering larger area, and enabling higher production rate.
Solid-state lasers pumped by continuous-wave diode lasers can be Q-switched to obtain high peak power output pulses. The dependence of laser-pulse energy, average output power, peak power, and pulse width on pulse-repetition frequency in Q-switched Nd:YAG and Ho:YLF lasers is determined and compared. At low pulse repetition rates, the much longer upper-stage lifetime in Ho:YLF gives a distinct advantage. At higher pulse rates, the overall laser efficiency and the stimulated emission cross section are more important parameters, leading to an advantage for Nd:YAG. The results are of significance for designing lasers for use in space optical communications and remote sensing systems.
The purpose is to attempt a general introduction to pulsed carbon dioxide lasers of the kind used or proposed for laser radar applications. Laser physics is an excellent example of a cross-disciplinary topic, and the molecular spectroscopy, energy transfer, and plasma kinetics of the devices are explored. The concept of stimulated emission and population inversions is introduced, leading on to the molecular spectroscopy of the CO2 molecule. This is followed by a consideration of electron-impact pumping, and the pertinent energy transfer and relaxation processes which go on. Since the devices are plasma pumped, it is necessary to introduce a complex subject, but this is restricted to appropriate physics of glow discharges. Examples of representative devices are shown. The implications of the foregoing to plasma chemistry and gas life are discussed.
Previous solutions for polarization of astrophysical maser radiation due to closed-shell molecules in a magnetic field have potentially serious limitations. These solutions are mostly based on the approximation that the Zeeman frequency g-Omega is much greater than the rate for stimulated emission R and the rate for decay Gamma of the molecular state. Others are asymptotic solutions obtained for an angular momentum J = 1-0 transition. It has been unclear whether the polarizations due to plausible Zeeman splittings are adequately represented by the solutions obtained for g-Omega/Gamma much greater than 1 and g-Omega/R much greater than 1. Actual masing transitions tend to involve molecular states with angular momenta that are higher than J = 1 and 0. Numerical solutions for the linear polarization are presented here which do not have the foregoing restrictions on the g-Omega and which are not limited to a J = 1-0 transition.