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NASA NTRS2014

Aerosol Properties Derived from Airborne Sky Radiance and Direct Beam Measurements in Recent NASA and DoE Field Campaigns

The AERONET (AErosol RObotic NETwork) ground-based suite of sunphotometers provides measurements of spectral aerosol optical depth (AOD), precipitable water and spectral sky radiance, which can be inverted to retrieve aerosol microphysical properties that are critical to assessments of aerosol-climate interactions. Because of data quality criteria and sampling constraints, there are significant limitations to the temporal and spatial coverage of AERONET data and their representativeness for global aerosol conditions.The 4STAR (Spectrometer for Sky-Scanning, Sun-Tracking Atmospheric Research) instrument, jointly developed by NASA Ames and PNNL (Pacific Northwest National Laboratory) with NASA Goddard collaboration, combines airborne sun tracking and AERONET-like sky scanning with spectroscopic detection. Being an airborne instrument, 4STAR has the potential to fill gaps in the AERONET data set. The 4STAR instrument operated successfully in the SEAC4RS (Studies of Emissions and Atmospheric Composition, Clouds and Climate Coupling by Regional Surveys) experiment in Aug./Sep. 2013 aboard the NASA DC-8 and in the DoE (Department of Energy)-sponsored TCAP (Two Column Aerosol Project, July 2012 & Feb. 2013) experiment aboard the DoE G-1 aircraft. 4STAR provided direct beam measurements of hyperspectral AOD, columnar trace gas retrievals (H2O, O3, NO2), and the first ever airborne hyperspectral sky radiance scans, which can be inverted to yield the same products as AERONET ground-based observations. In this presentation, we provide an overview of the new 4STAR capabilities, with an emphasis on 26 high-quality sky radiance measurements carried out by 4STAR in SEAC4RS. We compare collocated 4STAR and AERONET sky radiances, as well as their retrievals of aerosol microphysical properties for a subset of the available case studies. We summarize the particle property and air-mass characterization studies made possible by the combined 4STAR direct beam and sky radiance observations.

DoE↗
DOE OSTI2024

Geometry of Non-Diffusive Tracer Transport in Gridded Atmospheric Models

A first-order linear and numerically non-diffusive Eulerian transport algorithm, minVAR, was recently developed for preservation of correlations between interrelated tracers during advective transport. The present study extends this work by: (1) providing further investigation of several interesting geometric constructions found in contours of constant minVAR, short for minimum variance, through extension to three coordinate dimensions. These contours capture point-by-point representations of thousands of individual atmospheric aerosol and/or cloud particles as they evolve and are rendered on Eulerian grids at a level of sub-grid resolution limited only by numerical precision; and (2) exploration of geometric similarities between the Arakawa C-grid, used to obtain interpolated values of the wind field at grid scale and minVAR. In particular, we consider interpolation of the u and v horizontal components of wind velocity from grid to sub-grid scales. The last results are motivated by recent applications of the Weather Research and Forecasting (WRF) model applied in the coastal Houston region, where the recent TRacking Aerosol Convection Interactions ExpeRiment (TRACER) field campaign was organized. A unique and fully consistent mapping is obtained between particles moving along meteorological wind trajectories and the non-diffusive, non-dispersive representation of such trajectories on an Eulerian grid.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRS2012

The Cloud-Aerosol Transport System (CATS): A New Lidar for Aerosol and Cloud Profiling from the International Space Station

Spaceborne lidar profiling of aerosol and cloud layers has been successfully implemented during a number of prior missions, including LITE, ICESat, and CALIPSO. Each successive mission has added increased capability and further expanded the role of these unique measurements in wide variety of applications ranging from climate, to air quality, to special event monitoring (ie, volcanic plumes). Many researchers have come to rely on the availability of profile data from CALIPSO, especially data coincident with measurements from other A-Train sensors. The CALIOP lidar on CALIPSO continues to operate well as it enters its fifth year of operations. However, active instruments have more limited lifetimes than their passive counterparts, and we are faced with a potential gap in lidar profiling from space if the CALIOP lidar fails before a new mission is operational. The ATLID lidar on EarthCARE is not expected to launch until 2015 or later, and the lidar component of NASA's proposed Aerosols, Clouds, and Ecosystems (ACE) mission would not be until after 2020. Here we present a new aerosol and cloud lidar that was recently selected to provide profiling data from the International Space Station (ISS) starting in 2013. The Cloud-Aerosol Transport System (CATS) is a three wavelength (1064,532,355 nm) elastic backscatter lidar with HSRL capability at 532 nm. Depolarization measurements will be made at all wavelengths. The primary objective of CATS is to continue the CALIPSO aerosol and cloud profile data record, ideally with overlap between both missions and EarthCARE. In addition, the near real time (NRT) data capability ofthe ISS will enable CATS to support operational applications such as aerosol and air quality forecasting and special event monitoring. The HSRL channel will provide a demonstration of technology and a data testbed for direct extinction retrievals in support of ACE mission development. An overview of the instrument and mission will be provided, along with a summary of the science objectives and simulated data. Input from the ICAP community is desired to help plan our NRT mission goals and interactions with ICAP forecasters.

Welton, Ellsworth J.↗
NASA NTRS2020

Cloud-top pressure retrieval with DSCOVR EPIC oxygen A- and B-band observations

An analytic transfer inverse model for Earth Polychromatic Imaging Camera (EPIC) observations is proposed to retrieve the cloud-top pressure (CTP) with the consideration of in-cloud photon penetration. In this model, an analytic equation was developed to represent the reflection at the top of the atmosphere from above cloud, in cloud, and below cloud. The coefficients of this analytic equation can be derived from a series of EPIC simulations under different atmospheric conditions using a nonlinear regression algorithm. With estimated cloud pressure thickness, the CTP can be retrieved from EPIC observation data by solving the analytic equation. To simulate the EPIC measurements, a program package using the double-k approach was developed. Compared to line-by-line calculation, this approach can calculate high-accuracy results with a 100-fold computation time reduction. During the retrieval processes, two kinds of retrieval results, i.e., baseline CTP and retrieved CTP, are provided. The baseline CTP is derived without considering in-cloud photon penetration, and the retrieved CTP is derived by solving the analytic equation, taking into consideration in-cloud and below-cloud interactions. The retrieved CTPs for the oxygen A and B bands are smaller than their related baseline CTP. At the same time, both baseline CTP and retrieved CTP at the oxygen B band are larger than those at the oxygen A band. Compared to the difference in baseline CTP between the B band and A band, the difference in retrieved CTP between these two bands is generally reduced. Out of around 10 000 cases, in retrieved CTP between the A and B bands we found an average bias of 93 mb with a standard deviation of 81 mb. The cloud layer top pressure from Cloud–Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) measurements is used for validation. Under single-layer cloud situations, the retrieved CTPs for the oxygen A band agree well with the CTPs from CALIPSO, the mean difference of which within 5 mb in the case study. Under multiple-layer cloud situations, the CTPs derived from EPIC measurements may be larger than the CTPs of high-level thin clouds due to the effect of photon penetration.

DSCOVR↗
NASA NTRS2011

An Investigation of Interaction of Saharan Dust and Atlantic ITCZ Using Cloudsat-Calipso and A-Train Data

In this study, we investigate the radiative forcing of Saharan dust, its interactions with the Atlantic Intertropical Convergence Zone (ITCZ), through African easterly waves (AEW), African easterly jets (AEJ), and its impacts in short term numerical forecasts of tropical cyclogenesis using the GOCART-GEOS5 forecast system. Our approach is to develop and use an A-Train satellite simulator (ATSS) to constrain the observed aerosol index of refraction and particle size distribution by finding the values that simultaneously minimize the difference between observed CALIOP, CloudSat, OMI, and MODIS radiances and simulated radiances inverted from atmospheric model output using procedures and physical principles consistent with those used in corresponding retrieval algorithms. We use observations from the A-train and TRMM to determine relationships among the Saharan dust layer, transport by the AEW, and possible responses to dust radiative forcing in developing tropical cyclones in the A-ITCZ. Preliminary model results showing physical processes associated with the generation and transport of the Saharan dust layer, their interactions with the incipient moisture, clouds and rainfall in developing tropical cyclones will be presented. Also presented will be results of a case study of possible radiative impacts on AEW and AEJ during the NAMMA field campaign.

Lau, W.↗
NASA NTRS2012

The Aerosol-Monsoon Climate System of Asia

In Asian monsoon countries such as China and India, human health and safety problems caused by air-pollution are worsening due to the increased loading of atmospheric pollutants stemming from rising energy demand associated with the rapid pace of industrialization and modernization. Meanwhile, uneven distribution of monsoon rain associated with flash flood or prolonged drought, has caused major loss of human lives, and damages in crop and properties with devastating societal impacts on Asian countries. Historically, air-pollution and monsoon research are treated as separate problems. However a growing number of recent studies have suggested that the two problems may be intrinsically intertwined and need to be studied jointly. Because of complexity of the dynamics of the monsoon systems, aerosol impacts on monsoons and vice versa must be studied and understood in the context of aerosol forcing in relationship to changes in fundamental driving forces of the monsoon climate system (e.g. sea surface temperature, land-sea contrast etc.) on time scales from intraseasonal variability (~weeks) to climate change (~ multi-decades). Indeed, because of the large contributions of aerosols to the global and regional energy balance of the atmosphere and earth surface, and possible effects of the microphysics of clouds and precipitation, a better understanding of the response to climate change in Asian monsoon regions requires that aerosols be considered as an integral component of a fully coupled aerosol-monsoon system on all time scales. In this paper, using observations and results from climate modeling, we will discuss the coherent variability of the coupled aerosol-monsoon climate system in South Asia and East Asia, including aerosol distribution and types, with respect to rainfall, moisture, winds, land-sea thermal contrast, heat sources and sink distributions in the atmosphere in seasonal, interannual to climate change time scales. We will show examples of how elevated absorbing aerosols (dust and black carbon) may interact with monsoon dynamics to produce feedback effects on the atmospheric water cycle, leading to in accelerated melting of snowpacks over the Himalayas and Tibetan Plateau, and subsequent changes in evolution of the pre-monsoon and peak monsoon rainfall, moisture and wind distributions in South Asia and East Asia.

Lau, William K. M.↗
NASA NTRS2014

Stereoscopic Retrieval of Smoke Plume Heights and Motion from Space-Based Multi-Angle Imaging, Using the MISR INteractive eXplorer(MINX)

Airborne particles desert dust, wildfire smoke, volcanic effluent, urban pollution affect Earth's climate as well as air quality and health. They are found in the atmosphere all over the planet, but vary immensely in amount and properties with season and location. Most aerosol particles are injected into the near-surface boundary layer, but some, especially wildfire smoke, desert dust and volcanic ash, can be injected higher into the atmosphere, where they can stay aloft longer, travel farther, produce larger climate effects, and possibly affect human and ecosystem health far downwind. So monitoring aerosol injection height globally can make important contributions to climate science and air quality studies. The Multi-angle Imaging Spectro-Radiometer (MISR) is a space borne instrument designed to study Earths clouds, aerosols, and surface. Since late February 2000 it has been retrieving aerosol particle amount and properties, as well as cloud height and wind data, globally, about once per week. The MINX visualization and analysis tool complements the operational MISR data products, enabling users to retrieve heights and winds locally for detailed studies of smoke plumes, at higher spatial resolution and with greater precision than the operational product and other space-based, passive remote sensing techniques. MINX software is being used to provide plume height statistics for climatological studies as well as to investigate the dynamics of individual plumes, and to provide parameterizations for climate modeling.

aerosols↗
NASA NTRS2019

Ocean Color Instrument Integration and Testing

This paper describes the plans, flows, key facilities, components and equipment necessary to fully integrate, functionally test, qualify and calibrate the Ocean Color Instrument (OCI) on the Plankton, Aerosols, Clouds, and oceans Ecosystem (PACE) observatory. PACE is currently in the design phase of mission development. It is scheduled to launch in 2022, extending and improving NASA's twenty-year record of satellite observations of global ocean biology, aerosols and clouds. PACE will advance the assessment of ocean health by measuring the distribution of phytoplankton, which are small plants and algae that sustain the marine food web. It will also continue systematic records of key atmospheric variables associated with air quality and the Earth's climate. PACE's primary sensor, the OCI, is a highly advanced optical spectrometer that will be used to measure properties of light over portions of the electromagnetic spectrum. It will enable continuous measurement of light at finer wavelength resolution than previous NASA satellite sensors, extending key system ocean color data records for climate studies. The color of the ocean is determined by the interaction of sunlight with substances or particles present in seawater such as chlorophyll. By monitoring global phytoplankton distribution and abundance with unprecedented detail, the OCI will contribute to a better understanding of the complex systems that drive ocean ecology and it's impacts on global fisheries. This paper will focus on the Integration and Test (I&T) activities for OCI while it is at the NASA Goddard Space Flight Center. The OCI integration consists of assembly and alignment of the rotating telescope, electronics box integration, fixed deck assembly integration, thermal systems integration and the final assembly and testing. This I&T phase will be followed by the OCI calibration and characterization, environmental tests which include electromagnetic interference (EMI)/electromagnetic compatibility (EMC), vibration with sine sweep, acoustics, shock, thermal balance, thermal vacuum, mass properties and center of gravity. This paper will briefly discuss OCI shipment and delivery to the spacecraft vendor for observatory level I&T as well as some launch preparation activities.

Petro, Susanna↗
NASA NTRS2022

Dynamical Perturbation of the Stratosphere by a Pyrocumulonimbus Injection of Carbonaceous Aerosols

The Pacific Northwest pyrocumulonimbus Event (PNE) took place in British Columbia during the evening and night-time hours between the 12th and 13th of August 2017. Several pyroconvective clouds erupted in this occasion, and released in the upper troposphere/lower stratosphere unprecedented amounts of carbonaceous aerosols (300 ktn). Only a few years later, an even larger pyroCb injection took place over Australia. This event, named the Australian New Year (ANY) event, injected up to 1100 ktn of aerosol between December 29th 2019 and January 4th 2020. Such large injections of carbonaceous aerosol modify the stratospheric radiative budgets, locally perturbing stratospheric temperatures and winds. In this study, we use the Goddard Earth Observing System Chemistry Climate Model (GEOS CCM) to study the pertubations on the stratospheric meteorology induced by an aerosol injection of the magnitude of the PNE. Our simulations include the radiative interactions of aerosols, so that their impact on temperatures and winds are explicitly simulated. We show how the presence of the carbonaceous aerosols from the pyroCb causes the formation and maintenance of a synoptic scale stratospheric anticyclone. We follow this disturbance considering the potential vorticity anomaly and the brown carbon aerosol loading and we describe its dynamical and thermodynamical structure and its evolution in time. The analysis presented here shows that the simulated anticyclone undergoes daily expansion-compression cycles governed by the radiative heating, which are directly related to the vertical motion of the plume, and that the aerosol radiative heating is essential in maintaining the anticyclone itself.

Pyrocumulonimbus↗
NASA NTRS2011

Ground-Based Network and Supersite Observations to Complement and Enrich EOS Research

Since 1997 NASA has been successfully launching a series of satellites - the Earth Observing System (EOS) - to intensively study, and gain a better understanding of, the Earth as an integrated system. Space-borne remote sensing observations, however, are often plagued by contamination of surface signatures. Thus, ground-based in-situ and remote-sensing measurements, where signals come directly from atmospheric constituents, the sun, and/or the Earth-atmosphere interactions, provide additional information content for comparisons that confirm quantitatively the usefulness of the integrated surface, aircraft, and satellite datasets. Through numerous participations, particularly but not limited to the EOS remote-sensing/retrieval and validation projects over the years, NASA/GSFC has developed and continuously refined ground-based networks and mobile observatories that proved to be vital in providing high temporal measurements, which complement and enrich the satellite observations. These are: the AERO NET (AErosol RObotic NETwork) a federation of ground-based globally distributed network of spectral sun-sky photometers; the MPLNET (Micro-Pulse Lidar NETwork, a similarly organized network of micro-pulse lidar systems measuring aerosol and cloud vertical structure continuously; and the SMART-COMMIT (Surface-sensing Measurements for Atmospheric Radiative Transfer - Chemical, Optical & Microphysical Measurements of In-situ Troposphere, mobile observatories, a suite of spectral radiometers and in-situ probes acquiring supersite measurements. Most MPLNET sites are collocated with those of AERONET, and both networks always support the deployment of SMART-COMMIT worldwide. These data products follow the data structure of EOS conventions: Level-0, instrument archived raw data; Level-1 (or 1.5), real-time data with no (or limited) quality assurance; Level-2, not real high temporal and spectral resolutions. In this talk, we will present NASA/GSFC groundbased facilities, serving as network or supersite observations, which have been playing key roles in major international research projects over diverse aerosol regimes to complement and enrich the EOS scientific research.

Tsay, Si-Chee↗
NASA NTRS2022

The Future: Nasa’s Surface Biology and Geology Mission and the Dark (Aquatic) Side

With the release of NASA’s Earth System Observatory (ESO) measurement targets that includes studying the Earth’s Surface Biology and Geology (SBG), a global visible to shortwave infrared imaging spectrometer and a multispectral thermal infrared imager have been planned to launch in the late 2020s. This mission will enable unprecedented interdisciplinary science and applications relevant to studying the biology and geology of the Earth's surface. Measurement targets are directly aligned for studying coastal and inland waters ecosystems and water quality, including coralreef ecosystems, snow and ice, mineralogy, volcanology, biology, ecology, biodiversity, and components of radiative forcing from the surface such as greenhouse gas emissions. The observations not only have scientific value in studying feedbacks and interactions of surface processes (e.g., harmful algal blooms, domoic acid, oil spills, and other hazardous events), but also societal benefit – with the capacity to support real-world decision-making such as response to theseevents and inland water conservation, protection of drinking water quality for public and environmental health, and habitat conservation. The work presented here outlines the conducted mission and architecture study and the initiation of science performance trades (signal sensitivity; spectral, spatial, and temporal resolution; and atmospheric effects) informing the design of the SBG segment of the ESO providing the most value to myriad science and applications as possible. Science and applications synergies and algorithms with the Plankton, Aerosol, Cloud, and ocean Ecosystem (PACE) and the Geostationary Littoral Imaging and Monitoring Radiometer (GLIMR) is opportunistic for advancing aquatics research and applications.

THE FUTURE↗
DOE OSTI2026

High-Resolution LiDAR Observations for Coupled Effects of Dry-Air Entrainment and Haze-Cloud Interactions on Cloud Vertical Structure

This study demonstrates the high-resolution profiling of cloud microphysics in a laboratory chamber using Time-Correlated Single Photon Counting (TCSPC) LiDAR. We present a novel retrieval method to derive vertical extinction (𝜎) profiles, constrained by in situ measurements, to diagnose responses to dry-air entrainment. In clean clouds, the LiDAR signals and retrieved 𝜎 remain relatively uniform, with entrainment effects confined to the upper layer. In contrast, polluted clouds exhibit strong vertical variability and a transition to a water-vapor-limited state. Entrainment significantly enhances the haze number concentration (𝑁ℎ), particularly near the bottom, creating highly height-dependent extinction profiles for polluted clouds. Our results highlight the capability of high-resolution LiDAR in capturing fine-scale vertical inhomogeneities. This approach provides a robust framework for quantifying how aerosol loading modulates entrainment sensitivity, offering new insights into the transition between buffered and water-vapor-limited regimes.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRS1978

Some aspects of the interaction of radiation with the thermal and mass budgets of cloud droplets

It is shown that the effects of radiative heating or cooling can have a substantial influence on the mass budget of a cloud droplet and thus on the microphysical properties of a cloud as a whole. The radiative transfer equation, including all orders of multiple scattering, is solved for spectral windows of earth's atmosphere by adopting the Eddington approximation and assuming that the cloud is isothermal and illuminated by fluxes from both the ground and the sky. The results obtained for the 8-12-micron window indicate that radiative cooling can increase a droplet's growth rate and may also make the droplet cooler than the surrounding gas while water vapor is diffusing in, which would cause diffusiophoreisis and thermophoreisis to combine and increase the efficiency with which droplets would scavenge aerosols.

Barkstrom, B. R.↗
NASA NTRS2005

Improvement of Raman lidar algorithm for quantifying aerosol extinction

Aerosols are particles of different composition and origin and influence the formation of clouds which are important in atmospheric radiative balance. At the present there is high uncertainty on the effect of aerosols on climate and this is mainly due to the fact that aerosol presence in the atmosphere can be highly variable in space and time. Monitoring of the aerosols in the atmosphere is necessary to better understanding many of these uncertainties. A lidar (an instrument that uses light to detect the extent of atmospheric aerosol loading) can be particularly useful to monitor aerosols in the atmosphere since it is capable to record the scattered intensity as a function of altitude from molecules and aerosols. One lidar method (the Raman lidar) makes use of the different wavelength changes that occur when light interacts with the varying chemistry and structure of atmospheric aerosols. One quantity that is indicative of aerosol presence is the aerosol extinction which quantifies the amount of attenuation (removal of photons), due to scattering, that light undergoes when propagating in the atmosphere. It can be directly measured with a Raman lidar using the wavelength dependence of the received signal. In order to calculate aerosol extinction from Raman scattering data it is necessary to evaluate the rate of change (derivative) of a Raman signal with respect to altitude. Since derivatives are defined for continuous functions, they cannot be performed directly on the experimental data which are not continuous. The most popular technique to find the functional behavior of experimental data is the least-square fit. This procedure allows finding a polynomial function which better approximate the experimental data. The typical approach in the lidar community is to make an a priori assumption about the functional behavior of the data in order to calculate the derivative. It has been shown in previous work that the use of the chi-square technique to determine the most likely functional behavior of the data prior to actually calculating the derivative eliminates the need for making a priori assumptions. We note that the a priori choice of a model itself can lead to larger uncertainties as compared to the method that is validated here. In this manuscript, the chi-square technique that determines the most likely functional behavior is validated through numerical simulation and by application to a large body of Raman lidar measurements. In general, we show that the chi-square approach to evaluate aerosol extinction yields lower extinction uncertainty than the traditional technique. We also use the technique to study the feasibility of developing a general characterization of the extinction uncertainty that could permit the uncertainty in Raman lidar aerosol extinction measurements to be estimated accurately without the use of the chi-square technique.

Russo, Felicita↗
NASA NTRS2012

The View from the Top: CALIOP Ice Water Content in the Uppermost Layer of Tropical Cyclones

NASA's CALIPSO satellite carries both the Cloud and Aerosol Lidar with Orthogonal Polarization (CALIOP) and the Imaging Infrared Radiometer (IIR). The lidar is ideally suited to viewing the very top of tropical cyclones, and the IIR provides critical optical and microphysical information. The lidar and the IIR data work together to understand storm clouds since they are perfectly co-located, and big tropical cyclones provide an excellent complex target for comparing the observations. There is a lot of information from these case studies for understanding both the observations and the tropical cyclones, and we are just beginning to scratch the surface of what can be learned. Many tropical cyclone cloud particle measurements are focused on the middle and lower regions of storms, but characterization of cyclone interaction with the lowermost stratosphere at the upper storm boundary may be important for determining the total momentum and moisture transport budget, and perhaps for predicting storm intensity as well. A surprising amount of cloud ice is to be found at the very top of these big storms.

Avery, Melody A.↗
NASA NTRS2018

Pre-Aerosol, Clouds, and Ocean Ecosystem (PACE) Mission Science Definition Team Report: PACE Technical Report Series - Volume 2

We live in an era in which increasing climate variability is having measurable impact on marine ecosystems within our own lifespans. At the same time, an ever-growing human population requires increased access to and use of marine resources. To understand and be better prepared to respond to these challenges, we must expand our capabilities to investigate and monitor ecological and bio geo chemical processes in the oceans. In response to this imperative, the National Aeronautics and Space Administration (NASA) conceived the Pre-Aerosol, Clouds, and ocean Ecosystem (PACE) mission to provide new information for understanding the living ocean and for improving forecasts of Earth System variability. The PACE mission will achieve these objectives by making global ocean color measurements that are essential for understanding the carbon cycle and its inter-relationship with climate change, and by expanding our understanding about ocean ecology and biogeochemistry. PACE measurements will also extend ocean climate data records collected since the 1990s to document changes in the function of aquatic ecosystems as they respond to human activities and natural processes over short and long periods of time. These measurements are pivotal for differentiating natural variability from anthropogenic climate change effects and for understanding the interactions between these processes and various human uses of the ocean. PACE ocean science goals and measurement capabilities greatly exceed those of our heritage ocean color sensors, and are needed to address the many outstanding science questions developed by the oceanographic community over the past 40 years.

Cetinic, Ivona↗
NASA NTRS2023

Virus Infection of Phytoplankton Increases Average Molar Mass and Reduces Hygroscopicity of Aerosolized Organic Matter

Viral infection of phytoplankton is a pervasive mechanism of cell death and bloom termination, which leads to the production of dissolved and colloidal organic matter that can be aerosolized into the atmosphere. Earth-observing satellites can track the growth and death of phytoplankton blooms on weekly time scales but the impact of viral infection on the cloud forming potential of associated aerosols is largely unknown. Here, we determine the influence of viral-derived organic matter, purified viruses, and marine hydrogels on the cloud condensation nuclei activity of their aerosolized solutions, compared to organic exudates from healthy phytoplankton. Dissolved organic material derived from exponentially growing and infected cells of well-characterized eukaryotic phytoplankton host-virus systems, including viruses from diatoms, coccolithophores and chlorophytes, was concentrated, desalted, and nebulized to form aerosol particles composed of primarily of organic matter. Aerosols from infected phytoplankton cultures resulted in an increase in critical activation diameter and average molar mass in three out of five combinations evaluated, along with a decrease in organic kappa (hygroscopicity) compared to healthy cultures and seawater controls. The infected samples also displayed evidence of increased surface tension depression at realistic cloud water vapor supersaturations. Amending the samples with xanthan gum to simulate marine hydrogels increased variability in organic kappa and surface tension in aerosols with high organic to salt ratios. Our findings suggest that the pulses of increased dissolved organic matter associated with viral infection in surface waters may increase the molar mass of dissolved organic compounds relative to surface waters occupied by healthy phytoplankton or low phytoplankton biomass.

Atmospheric science↗
NASA NTRS2006

Workshop on the Impacts of Aviation on Climate Change

Projections indicate that demand for aviation transportation will increase by more than two fold over the next few decades. Timely action is needed to understand and quantify the potential climate impacts of aviation emissions particularly given the sustained lapse over the last several years in U.S. research activities in this area. In response to the stated needs, a group of international experts participated in the Workshop on the Impacts of Aviation on Climate Change during June 7-9, 2006 in Boston, MA. The workshop focus was on the impacts of subsonic aircraft emissions in the UT/LS region and on the potential response of the climate system. The goals of the workshop were to assess and document the present state of scientific knowledge, to identify the key underlying uncertainties and gaps, to identify ongoing and further research needed, to explore the development of climate impact metrics, and to help focus the scientific community on the aviation-climate change research needs. The workshop concluded that the major ways that aviation can affect climate, in agreement with the 1999 assessment by the Intergovernmental Panel on Climate Change (IPCC), are the direct climate effects from CO2 and water vapor emissions, the indirect forcing on climate resulting from changes in the distributions and concentrations of ozone and methane as a primary consequence of aircraft nitrogen oxide (NOx) emissions, the direct effects (and indirect effects on clouds) from emitted aerosols and aerosol precursors, and the climate effects associated with contrails and cirrus cloud formation. The workshop was organized in three subgroups: (1) Effects of aircraft emissions on the UT/LS chemical composition, (2) Effects of water and particle emissions on contrails and on cirrus clouds, and (3) Impacts on climate from aircraft emissions and identification of suitable metrics to measure these impacts. The workshop participants acknowledged the need for focused research specifically to address the uncertainties and gaps in our understanding of current and projected impacts of aviation on climate and to develop metrics to better characterize these impacts. This may entail coordination and/or expansion of existing and planned climate research programs, or new activities. Such efforts should include strong and continuing interactions among the science and aviation communities as well as policymakers to develop well-informed decisions.

Wuebbles, Don↗