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Results for “Weak localization”

Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 721 records · Page 40
All sourcesNASA NTRSDOE OSTI
DOE OSTI2018

Spatial–temporal spectroscopy characterizations and electronic structure of methylammonium perovskites

Using time-resolved laser-scanning confocal microscopy and ultrafast optical pump/THz probe spectroscopy, we measure photoluminescence (PL) and THz-conductivity in perovskite micro-crystals and films. PL quenching and lifetime variations occur from local heterogeneity. Ultrafast THz-spectra measure sharp quantum transitions from excitonic Rydberg states, providing weakly bound excitons with a binding energy of ~13.5 meV at low temperatures. Ab-initio electronic structure calculations give a direct band gap of 1.64 eV, a dielectric constant of ~18, heavy electrons, and light holes, resulting in weakly bound excitons, consistent with the binding energies from the experiment. Here, the complementary spectroscopy and simulations reveal fundamental insights into perovskite light-matter interactions.

36 MATERIALS SCIENCE↗
DOE OSTI2013

F-18 Labeled Diabody-Luciferase Fusion Proteins for Optical-ImmunoPET

The goal of the proposed work is to develop novel dual-labeled molecular imaging probes for multimodality imaging. Based on small, engineered antibodies called diabodies, these probes will be radioactively tagged with Fluorine-18 for PET imaging, and fused to luciferases for optical (bioluminescence) detection. Performance will be evaluated and validated using a prototype integrated optical-PET imaging system, OPET. Multimodality probes for optical-PET imaging will be based on diabodies that are dually labeled with 18F for PET detection and fused to luciferases for optical imaging. 1) Two sets of fusion proteins will be built, targeting the cell surface markers CEA or HER2. Coelenterazine-based luciferases and variant forms will be evaluated in combination with native substrate and analogs, in order to obtain two distinct probes recognizing different targets with different spectral signatures. 2) Diabody-luciferase fusion proteins will be labeled with 18F using amine reactive [18F]-SFB produced using a novel microwave-assisted, one-pot method. 3) Sitespecific, chemoselective radiolabeling methods will be devised, to reduce the chance that radiolabeling will inactivate either the target-binding properties or the bioluminescence properties of the diabody-luciferase fusion proteins. 4) Combined optical and PET imaging of these dual modality probes will be evaluated and validated in vitro and in vivo using a prototype integrated optical-PET imaging system, OPET. Each imaging modality has its strengths and weaknesses. Development and use of dual modality probes allows optical imaging to benefit from the localization and quantitation offered by the PET mode, and enhances the PET imaging by enabling simultaneous detection of more than one probe.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗
NASA NTRS1974

A search for soft X-ray emission from red-giant coronae

Hills has pointed out that if red-giant coronae are weak sources of soft X-rays, then the problems of the identification of the local component of the soft X-ray background and the observed lack of gas in globular clusters may be simultaneously resolved. Using instrumentation aboard OAO Copernicus, we have searched unsuccessfully for emission in the 10-100 A band from four nearby red giants. In all cases, our upper limits are of the order of the minimum theoretically predicted fluxes.

Margon, B.↗
NASA NTRS1976

An implicit finite-difference algorithm for hyperbolic systems in conservation-law form

An implicit finite-difference scheme is developed for the efficient numerical solution of nonlinear hyperbolic systems in conservation-law form. The algorithm is second-order time-accurate, noniterative, and in a spatially factored form. Second- or fourth-order central and second-order one-sided spatial differencing are accommodated within the solution of a block tridiagonal system of equations. Significant conceptual and computational simplifications are made for systems whose flux vectors are homogeneous functions (of degree one), e.g., the Eulerian gasdynamic equations. Conservative hybrid schemes, which switch from central to one-sided spatial differencing whenever the local characteristic speeds are of the same sign, are constructed to improve the resolution of weak solutions. Numerical solutions are presented for a nonlinear scalar model equation and the two-dimensional Eulerian gasdynamic equations.

Beam, R. M.↗
NASA NTRS1988

Energy transfer in isotropic turbulence at low Reynolds numbers

Detailed measurements were made of energy transfer among the scales of motion in incompressible turbulent fields at low Reynolds numbers generated by direct numerical simulation. It was observed that although the transfer resulted from triad interactions that were non-local in k space, the energy always transferred locally. The results are consistent with the notion of non-uniform advection of small weak eddies by larger and stronger ones, similar to transfer processes in the far dissipation range at high Reynolds numbers.

Domaradzki, J. A.↗
NASA NTRS2000

High-Frequency Observations of Blazars

We report on the results of high-frequency VLBA observations of 42 gamma-ray bright blazars monitored at 22 and 43 GHz between 1993.9 and 1997.6. In 1997 the observations included polarization-sensitive imaging. The cores of gamma-ray blazars are only weakly polarized, with EVPAs (electric-vector position angles) usually within 40 deg of the local direction of the jet. The EVPAs of the jet components are usually within 20 deg of the local jet direction. The apparent speeds of the gamma-ray bright blazars are considerably faster than in the general population of bright compact radio sources. Two X-ray flares (observed with RXTE) of the quasar PKS 1510-089 appear to be related to radio flares, but with the radio leading the X-ray variations by about 2 weeks. This can be explained either by synchrotron self-Compton emission in a component whose variations are limited by light travel time or by the Mirror Compton model.

Marscher, A. P.↗
NASA NTRS2000

High-Frequency Observations of Blazars

We report on the results of high-frequency VLBA observations of 42 gamma ray bright blazars monitored at 22 and 43 GHz between 1993.9 and 1997-6. In 1997 the observations included polarization-sensitive imaging. The cores of gamma ray blazars are only weakly polarized, with EVPAs (electric-vector position angles) usually within 40 degrees of the local direction of the jet. The EVPAs of the jet components are usually within 20 degrees of the local jet direction. The apparent speeds of the gamma ray bright blazars are considerably faster than in the general population of bright compact radio sources. Two X-ray flares (observed with RXTE) of the quasar PKS 1510-089 appear to be related to radio flares, but with the radio leading the X-ray variations by about 2 weeks. This can be explained either by synchrotron self-Compton emission in a component whose variations are limited by light travel time or by the Mirror Compton model.

Marscher, A. P.↗
NASA NTRS2004

Tholins as Coloring Agents on Solar System Bodies

Pre-biotic organic materials appear to be common on many small bodies in the outer Solar System, as evidenced by the color properties of these objects. We report on our continuing study of color properties in connection with the presence of complex organic solids (tholins) among the planets and their satellites, the asteroids, and the trans- Neptunian objects (Kuiper Belt objects). Most small, icy bodies in the Solar System, whether they have high or low surface reflectance (albedo), show a pronounced downward slope in reflectance at wavelengths shorter than approx. 1 micron. This increasing absorption of sunlight toward shorter wavelengths is characteristic of pi-bonds in hydrocarbons having chains or rings of conjugated C atoms. Tholins, which contain polycyclic aromatic and aliphatic hydrocarbons, exhibit these color properties. Using the complex refractive indices of tholins in models of the reflectance spectra of icy bodies in the Solar System, we find that these complex organic materials satisfactorily account for the coloration so widely observed. The new results presented here show that the wide variety of colors of Kuiper Belt objects can be fit very well with tholins, as can the colors of Pluto and Triton. The implications of these fits of Kuiper Belt objects is that complex organic material is created on their surfaces by energetic particle bombardment of native ices, and also may be accreted from external sources. In the cases of Pluto and Triton, photochemistry of their weak N2 + CH4 + CO atmospheres produces complex organic molecules that precipitate to the surface, providing local color.

Cruikshank, D. P.↗
NASA NTRSDate not supplied

Evaluating the Performance of GPM IMERG Products for Extreme Precipitation Estimation in Volta River Basin of Ghana

The Volta River basin in West Africa, covering a substantial area of Ghana, faces significant water management challenges due to highly variable rainfall and limited availability of high temporal resolution rain gauges. This study, developed under the 2024 Global Precipitation Measurement (GPM) Mission mentorship program, evaluates precipitation in the Volta River basin using high-resolution satellite-derived data from the Integrated Multi-satellite Retrievals for GPM (IMERG). In the absence of sub-daily rainfall data, comparisons were made between daily, monthly, and seasonal precipitation from local gauges and IMERG V06 and V07 (early and final) runs. Results indicated a very weak correlation between daily precipitation estimates from IMERG and gauge data, but a significantly improved correlation for monthly and seasonal estimates. Additionally, IMERG data were used to identify heavy rainfall events and drought periods, which were compared to known occurrences in the region. By addressing these objectives, this study contributes to more accurate extreme precipitation estimation in the Volta River basin, thereby enhancing disaster risk management and climate resilience in Ghana.

Jessica Sutton↗
DOE OSTI2020

Distinct behavior of localized and delocalized carriers in anatase TiO 2 (001) during reaction with O 2

Two-dimensional (2D) metallic states induced by oxygen vacancies $(V_{O}\text{s})$ at oxide surfaces and interfaces provide opportunities for the development of advanced applications, but the ability to control the behavior of these states is still limited. As such, we used angle resolved photoelectron spectroscopy combined with density-functional theory (DFT) to study the reactivity of $V_O$-induced states at the (001) surface of anatase TiO 2 , where both 2D metallic and deeper lying in-gap states (IGs) are observed. The 2D and IG states exhibit remarkably different evolutions when the surface is exposed to molecular O 2 : while IGs are almost completely quenched, the metallic states are only weakly affected. DFT calculations indeed show that the IGs originate from surface $V_{O}\text{s}$ and remain localized at the surface, where they can promptly react with O 2 . In contrast, the metallic states originate from subsurface vacancies whose migration to the surface for recombination with O 2 is kinetically hindered on anatase TiO 2 (001), thus making them much less sensitive to oxygen dosing.

36 MATERIALS SCIENCE↗
DOE OSTI2016

The Reynolds stress induced by weakly up-down asymmetric ion temperature gradient mode

A weakly up-down asymmetric ion temperature gradient (ITG) mode (formed in the up-down symmetric equilibrium), localized in the bad curvature region, may contribute dominantly to the nonlinear Reynolds stress because its growth rate is higher than the competing modes: the strongly up-down asymmetric modes, and other modes peaked (poloidally) away from the outboard mid-plane. Based on the fluid ITG model, the parameterized analytic wave function is constructed in the two dimensional (2D) Fourier-ballooning representation, and numerically verified by making use of the finite difference methods. Analytic expressions for the poloidal Reynolds stresses, defined on a rational surface, are given for both the weakly and the strongly up-down asymmetric ITG modes. It is shown here that the poloidal stresses of both modes can be interpreted as a superposition of a monopole and a dipole structure. For comparison with the experiment, the stresses are calculated for L-mode discharge parameters on five machines. Analytic expressions for the total parallel Reynolds stresses (contributed from all rational surfaces) are also derived for both modes: they are also exhibited, graphically, using a Gaussian wave intensity model.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2014

Evidence for Divisome Localization Mechanisms Independent of the Min System and SlmA in Escherichia coli

Cell division in Escherichia coli starts with assembly of FtsZ protofilaments into a ring-like structure, the Z-ring. Positioning of the Z-ring at midcell is thought to be coordinated by two regulatory systems, nucleoid occlusion and the Min system. In E. coli, nucleoid occlusion is mediated by the SlmA proteins. Here, we address the question of whether there are additional positioning systems that are capable of localizing the E. coli divisome with respect to the cell center. Using quantitative fluorescence imaging we show that slow growing cells lacking functional Min and SlmA nucleoid occlusion systems continue to divide preferentially at midcell. We find that the initial Z-ring assembly occurs over the center of the nucleoid instead of nucleoid-free regions under these conditions. We determine that Z-ring formation begins shortly after the arrival of the Ter macrodomain at the nucleoid center. Removal of either the MatP, ZapB, or ZapA proteins significantly affects the accuracy and precision of Z-ring positioning relative to the nucleoid center in these cells in accordance with the idea that these proteins link the Ter macrodomain and the Z-ring. Interestingly, even in the absence of Min, SlmA, and the putative Ter macrodomain – Z-ring link, there remains a weak midcell positioning bias for the Z-ring. Our work demonstrates that additional Z-ring localization systems are present in E. coli than are known currently. In particular, we identify that the Ter macrodomain acts as a landmark for the Z-ring in the presence of MatP, ZapB and ZapA proteins.

59 BASIC BIOLOGICAL SCIENCES↗
NASA NTRS2014

Diagenetic Features in Yellowknife Bay, Gale Crater, Mars: Implications for Substrate Rheology and Potential Gas Release

Multiple diagenetic features have been observed in clay­-bearing mudstone exposed within Yellowknife Bay, Gale Crater, Mars. These features occurred during at least two separate episodes: an early generation of spheroidal concretions that co-­occur with a dense networks of mineralized fractures, and a later generation of mineralized veins. Concretions consist of mm-sized spheroids (0.4 to 8.0 mm, mean diameter of 1.2 mm) that are distinctly more resistant than the encompassing mudstone. Dissected spheroids suggest an origin via compaction and incipient lithification of the substrate at the perimeter of syndepositional void space. Concretions are generally patchy in their distribution within clay-‐bearing mudstone, but in places can be the dominant fabric element. Locally dense networks of mineralized fractures occur in regions of low concretion abundance. These consist of short (< 50 cm), curvilinear to planar mineralized voids that occur across a range of orientations from vertical to subhorizontal. Fractures are filled by multi-phase cement consisting of two isopachous, erosionally resistant outer bands, and a central less resistant fill. Physical relationships suggests that original fractures may have formed as both interconnected voids and as discrete cross--cutting features. Co--occurrence of early diagenetic concretions and fracture networks suggests a common origin via gas release within a subaqueous, shallow substrate. We suggest that gas release within weakly cohesive subsurface sediments resulted in substrate dewatering and an increase in the cohesive strength of the substrate. Local differences in substrate strength and rate of gas production would have result in formation of either discrete voids or fracture networks. A second generation of mineralized veins is characterized by a regionally low spatial density, predominantly vertical or horizontal orientations, and a single phase of Ca-‐sulfate mineral fill. These veins cross-cut the early diagenetic elements and intersect a greater thickness of stratigraphy within Yellowknife Bay, suggesting a later-‐diagenetic origin via hydraulic fracturing.

Kah, L. C.↗
DOE OSTI2010

PROBING NEARBY COSMIC-RAY ACCELERATORS AND INTERSTELLAR MEDIUM TURBULENCE WITH MILAGRO HOT SPOTS

Both the acceleration of cosmic rays (CRs) in supernova remnant shocks and their subsequent propagation through the random magnetic field of the Galaxy are deemed to result in an almost isotropic CR spectrum. However, the MILAGRO TeV observatory discovered sharp ({approx}10{sup 0}) arrival anisotropies of CR nuclei. We suggest a mechanism for producing a weak and narrow CR beam which operates en route to the observer. The key assumption is that CRs are scattered by a strongly anisotropic Alfven wave spectrum formed by the turbulent cascade across the local field direction. The strongest pitch-angle scattering occurs for particles moving almost precisely along the field line. Partly because this direction is also the direction of the minimum of the large-scale CR angular distribution, the enhanced scattering results in a weak but narrow particle excess. The width, the fractional excess, and the maximum momentum of the beam are calculated from a systematic transport theory depending on a single scale l which can be associated with the longest Alfven wave, which efficiently scatters the beam. The best match to all three characteristics of the beam is achieved at l {approx} 1 pc. The distance to a possible source of the beam is estimated to be within a few 100 pc. Possible approaches to the determination of the scale l from the characteristics of the source are discussed. Alternative scenarios of drawing the beam from the galactic CR background are considered. The beam-related large-scale anisotropic CR component is found to be energy independent, which is also consistent with the observations.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2024

LoVoCCS. II. Weak Lensing Mass Distributions, Red-sequence Galaxy Distributions, and Their Alignment with the Brightest Cluster Galaxy in 58 Nearby X-Ray-luminous Galaxy Clusters

The Local Volume Complete Cluster Survey is an ongoing program to observe nearly a hundred low-redshift X-ray-luminous galaxy clusters (redshifts 0.03 < z < 0.12 and X-ray luminosities in the 0.1–2.4 keV band L X500c > 10 44 erg s −1 ) with the Dark Energy Camera, capturing data in the u, g, r, i, z bands with a 5σ point source depth of approximately 25th–26th AB magnitudes. Here, we map the aperture masses in 58 galaxy cluster fields using weak gravitational lensing. These clusters span a variety of dynamical states, from nearly relaxed to merging systems, and approximately half of them have not been subject to detailed weak lensing analysis before. In each cluster field, we analyze the alignment between the 2D mass distribution described by the aperture mass map, the 2D red-sequence (RS) galaxy distribution, and the brightest cluster galaxy (BCG). We find that the orientations of the BCG and the RS distribution are strongly aligned throughout the interiors of the clusters: the median misalignment angle is 19° within 2 Mpc. We also observe the alignment between the orientations of the RS distribution and the overall cluster mass distribution (by a median difference of 32° within 1 Mpc), although this is constrained by galaxy shape noise and the limitations of our cluster sample size. These types of alignment suggest long-term dynamical evolution within the clusters over cosmic timescales.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2016

Enhancing Quantum Yield via Local Symmetry Distortion in Lanthanide-Based Upconverting Nanoparticles

Lanthanide-based upconverting nanoparticles exhibit significant promise for solar energy generation, biological imaging, and security technologies but have not seen widespread adoption due to the prohibitively low efficiencies of current materials. Weak transition dipole moments between 4f orbitals hinder both photon absorption and emission. Here, we introduce a novel way to increase the radiative transition rates in Yb,Er-based upconverting nanoparticles based on local symmetry distortion. Beginning from a host matrix of the well-studied hexagonal (β)-phase NaYF 4 , we incrementally remove Y 3+ ions and cosubstitute for them a 1:1 mixture of Gd 3+ and Lu 3+ . These two ions act to expand and contract the lattice, respectively, inducing local-level distortion while maintaining the average host structure. We synthesize a range of β-NaY 0.8-2 x Gd x Lu x F 4 :Yb 0.18 Er 0.02 nanoparticles and experimentally confirm that particle size, phase, global structure, and Yb 3+ and Er 3+ concentrations remain constant as x is varied. Upconversion quantum yield is probed as the degree of cosubstitution is varied from x = 0 to x = 0.24. We achieve a maximum quantum yield value of 0.074% under 63 W/cm 2 of excitation power density, representing a 1.6× enhancement over the unmodified particles and the highest measured value for near-infrared-to-visible upconversion in sub-25 nm unshelled nanoparticles. We also investigate upconversion emission at the single-particle level and report record improvements in emission intensity for sub-50 nm particles. Radiative rate enhancements are confirmed by measuring excited-state lifetimes. The approach described herein can be used in combination with more established methods of efficiency improvement, such as adding passivating shells or coupling to plasmonic nanoattenas, to further boost the upconversion quantum yield.

36 MATERIALS SCIENCE↗
DOE OSTI2015

Weak interactions in Graphane/BN systems under static electric fields—A periodic ab-initio study

Ab-initio calculations via periodic Hartree-Fock (HF) and local second-order Møller-Plesset perturbation theory (LMP2) are used to investigate the adsorption properties of combined Graphane/boron nitride systems and their response to static electric fields. It is shown how the latter can be used to alter both structural as well as electronic properties of these systems.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2013

Anomalous dimensions and non-gaussianity

Here, we analyze the signatures of inflationary models that are coupled to interacting field theories, a basic class of multifield models also motivated by their role in providing dynamically small scales. Near the squeezed limit of the bispectrum, we find a simple scaling behavior determined by operator dimensions, which are constrained by the appropriate unitarity bounds. Specifically, we analyze two simple and calculable classes of examples: conformal field theories (CFTs), and large-N CFTs deformed by relevant time-dependent double-trace operators. Together these two classes of examples exhibit a wide range of scalings and shapes of the bispectrum, including nearly equilateral, orthogonal and local non-Gaussianity in different regimes. Along the way, we compare and contrast the shape and amplitude with previous results on weakly coupled fields coupled to inflation. This signature provides a precision test for strongly coupled sectors coupled to inflation via irrelevant operators suppressed by a high mass scale up to ~ 10 3 times the inflationary Hubble scale.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗