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At least 721 records · Page 40

A parallel in energy Krylov solution algorithm for the variational nodal method

To reduce the computational expense caused by the large number of energy groups in thermal and fast reactor calculations, we researched using parallelization in energy (i.e. group) of the multi-group response matrix equations derived from the Variational Nodal Method. This study focuses on solving steady-state eigenvalue problems in diffusion theory that are typically needed for depletion and reactivity coefficient calculations. To examine serial and parallel performance, GMRES, a Krylov algorithm, is applied to the multi-group system of equations at each fission source iteration. We also study the impact of using Wielandt acceleration on the eigenvalue/eigenvector problem. Numerical results based on a 72 group thermal and a 216 group fast reactor core problems are obtained for both serial and parallel calculations. The results show reduced CPU times when using GMRES and Wielandt acceleration in both serial and parallel calculations. (authors)

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

LMFR design and optimization methodology

This paper presents and applies a methodology for designing and optimizing Liquid Metal-cooled Fast Reactors (LMFRs). The methodology, called the Design and Optimization Methodology (DOM), achieves its goals by the effective exploration of a search space. The paper presents two case studies to demonstrate DOM. Both studies were based on the WEC long-life core LFR design. In the first study, DOM was used to explore the search space in the vicinity of the WEC (Westinghouse Electric Company LLC) long-life core LFR design trying to find a more optimized design. The objective of this optimization attempt was to reduce the fuel cycle cost. The WEC long-life core LFR design uses uranium mononitride (UN) fuel with natural nitrogen enrichment. In the second study, DOM was used to design a competitive UN fueled Lead-cooled Fast Reactor (LFR) which uses {sup 15}N enriched UN fuel. Based on the results from the second study, an estimation of the {sup 15}N enrichment cost required to obtain an economic core was performed. (authors)

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

MSFR TRU-burning potential and comparison with an SFR

The objective of this work is to evaluate the Molten Salt Fast Reactor (MSFR) potential benefits in terms of transuranics (TRU) burning through a comparative analysis with a sodium-cooled FR. The comparison is based on TRU- and MA-burning rates, as well as on the in-core evolution of radiotoxicity and decay heat. Solubility issues limit the TRU-burning rate to 1/3 that achievable in traditional low-CR FRs (low-Conversion-Ratio Fast Reactors). The softer spectrum also determines notable radiotoxicity and decay heat of the equilibrium actinide inventory. On the other hand, the liquid fuel suggests the possibility of using a Pu-free feed composed only of Th and MA (Minor Actinides), thus maximizing the MA burning rate. This is generally not possible in traditional low-CR FRs due to safety deterioration and decay heat of reprocessed fuel. In addition, the high specific power and the lack of out-of-core cooling times foster a quick transition toward equilibrium, which improves the MSFR capability to burn an initial fissile loading, and makes the MSFR a promising system for a quick (i.e., in a reactor lifetime) transition from the current U-based fuel cycle to a novel closed Th cycle. (authors)

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Validation Study in SAS4A Code in Simulated Mild TOP Condition

Model improvements and validation efforts for SAS4A code, which is the most advanced computer code for simulating the the primary phase of the Core Disruptive Accident (CDA) of MOX-fueled Sodium-cooled Fast Reactors, have been performed utilizing the experimental data from the CABRI programs by JAEA (Japan Atomic Energy Agency), IRSN (Institut de Radioprotection et de Surete Nucleaire), CEA (Commissariat a l'Energie Atomique et aux Energies Alternatives) and KIT (Karlsruhe Institute of Technology). In order to confirm validity of improved models of SAS4A, a systematic and comprehensive validation plan was defined. It was based on the PIRT (Phenomena Identification and Ranking Table) result for CDA of MOX-fueled fast reactors. The fuel failure position and time are the most important parameters, which dominate the analytical results in a reactor calculation. The failure position will affect the reactivity feedback due to the fuel distribution after failure and consequently would have an effect on the energy release in the initiating phase. This paper describes the preliminary result of validation study for SAS4A code in simulated Transient Over-Power (TOP) condition. (authors)

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Coupled 3D-neutronics / thermal-hydraulics analysis of an unprotected loss-of-flow accident for a 3600 MWth SFR core

The core behaviour of a large (3600 MWth) sodium-cooled fast reactor (SFR) is investigated in this paper with the use of a coupled TRACE/PARCS model. The SFR neutron spectrum is characterized by several performance advantages, but also leads to one dominating neutronics drawback - a positive sodium void reactivity. This implies a positive reactivity effect when sodium coolant is removed from the core. In order to evaluate such feedback in terms of the dynamics, a representative unprotected loss-of-flow (ULOF) transient, i.e. flow run-down without SCRAM in which sodium boiling occurs, is analyzed. Although analysis of a single transient cannot allow general conclusions to be drawn, it does allow better understanding of the underlying physics and can lead to proposals for improving the core response during such an accident. The starting point of this study is the reference core design considered in the framework of the Collaborative Project on the European Sodium Fast Reactor (CP-ESFR). To reduce the void effect, the core has been modified by introducing an upper sodium plenum (along with a boron layer) and by reducing the core height-to-diameter ratio. For the ULOF considered, a sharp increase in core power results in melting of the fuel in the case of the reference core. In the modified core, a large dryout leads to melting of the clad. It seems that, for the hypothetical event considered, fuel failure cannot be avoided with just improvement of the neutronics design; therefore, thermal-hydraulics optimization has been considered. An innovative assembly design is proposed to prevent sodium vapour blocking the fuel channel. This results in preventing a downward propagation of the sodium boiling to the core center, thus limiting it to the upper region. Such a void map introduces a negative coolant density reactivity feedback, which dominates the total reactivity change. As a result, the power level and the fuel temperature are effectively reduced, and a large dryout is prevented. As a next step, the classical sodium plenum is replaced by a fission gas plenum (with lower sodium fraction), thus improving flow stability. Stable boiling at a steady power level is achieved in this final configuration. (authors)

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

High Temperature Reactor (HTR) Deep Burn Core and Fuel Analysis: Design Selection for the Prismatic Block Reactor With Results from FY-2011 Activities

The Deep Burn (DB) Project is a U.S. Department of Energy sponsored feasibility study of Transuranic Management using high burnup fuel in the high temperature helium cooled reactor (HTR). The DB Project consists of seven tasks: project management, core and fuel analysis, spent fuel management, fuel cycle integration, TRU fuel modeling, TRU fuel qualification, and HTR fuel recycle. In the Phase II of the Project, we conducted nuclear analysis of TRU destruction/utilization in the HTR prismatic block design (Task 2.1), deep burn fuel/TRISO microanalysis (Task 2.3), and synergy with fast reactors (Task 4.2). The Task 2.1 covers the core physics design, thermo-hydraulic CFD analysis, and the thermofluid and safety analysis (low pressure conduction cooling, LPCC) of the HTR prismatic block design. The Task 2.3 covers the analysis of the structural behavior of TRISO fuel containing TRU at very high burnup level, i.e. exceeding 50% of FIMA. The Task 4.2 includes the self-cleaning HTR based on recycle of HTR-generated TRU in the same HTR. Chapter IV contains the design and analysis results of the 600MWth DB-HTR core physics with the cycle length, the average discharged burnup, heavy metal and plutonium consumptions, radial and axial power distributions, temperature reactivity coefficients. Also, it contains the analysis results of the 450MWth DB-HTR core physics and the analysis of the decay heat of a TRU loaded DB-HTR core. The evaluation of the hot spot fuel temperature of the fuel block in the DB-HTR (Deep-Burn High Temperature Reactor) core under full operating power conditions are described in Chapter V. The investigated designs are the 600MWth and 460MWth DB-HTRs. In Chapter VI, the thermo-fluid and safety of the 600MWth DB-HTRs has been analyzed to investigate a thermal-fluid design performance at the steady state and a passive safety performance during an LPCC event. Chapter VII describes the analysis results of the TRISO fuel microanalysis of the 600MWth and 450MWth DB-HTRs. The TRISO fuel microanalysis covers the gas pressure buildup in a coated fuel particle including helium production, the thermo-mechanical behavior of a CFP, the failure probabilities of CFPs, the temperature distribution in a CPF, and the fission product (FP) transport in a CFP and a graphite. In Chapter VIII, it contains the core design and analysis of sodium cooled fast reactor (SFR) with deep burn HTR reactor. It considers a synergistic combination of the DB-MHR and an SFR burner for a safe and efficient transmutation of the TRUs from LWRs. Chapter IX describes the design and analysis results of the self-cleaning (or self-recycling) HTR core. The analysis is considered zero and 5-year cooling time of the spent LWR fuels.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Proliferation resistance assessments during the design phase of a recycling facility as a means of reducing proliferation risks

The sustainability criterion for Gen IV nuclear energy systems inherently presumes the availability of efficient fuel recycling capabilities. One area for research on advanced fuel recycling concerns safeguards aspects of this type of facilities. Since a recycling facility may be considered as sensitive from a non-proliferation perspective, it is important to address these issues early in the design process, according to the principle of Safeguards By Design. Presented in this paper is a mode of procedure, where assessments of the proliferation resistance (PR) of a recycling facility for fast reactor fuel have been performed so as to identify the weakest barriers to proliferation of nuclear material. Two supplementing established methodologies have been applied; TOPS (Technological Opportunities to increase Proliferation resistance of nuclear power Systems) and PR-PP (Proliferation Resistance and Physical Protection evaluation methodology). The chosen fuel recycling facility belongs to a small Gen IV lead-cooled fast reactor system that is under study in Sweden. A schematic design of the recycling facility, where actinides are separated using solvent extraction, has been examined. The PR assessment methodologies make it possible to pinpoint areas in which the facility can be improved in order to reduce the risk of diversion. The initial facility design may then be slightly modified and/or safeguards measures may be introduced to reduce the total identified proliferation risk. After each modification of design and/or safeguards implementation, a new PR assessment of the revised system can then be carried out. This way, each modification can be evaluated and new ways to further enhance the proliferation resistance can be identified. This type of iterative procedure may support Safeguards By Design in the planning of new recycling plants and other nuclear facilities. (authors)

98 NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL P↗

FY23 Status of Quality Assurance Plan for Out-of-Pile Test Data

The DOE Advanced Reactor Technology program has supported recovery and preservation of legacy metallic fuel data collected as part of the US fast reactor program, recognizing it as essential to development and licensing activities for advanced fast reactors. Databases were established as organized collections of experimental records and data generated from in-pile experiments at EBRII, FFTF, and TREAT as well as related out-of-pile examinations of irradiated fuels. The Out-of-Pile Transient Database (OPTD), includes records of over 150 out-of-pile furnace transient tests on metallic fuels conducted at Argonne’s Alpha-Gamma Hot Cell Facility to evaluate their transient performance and characterize fuel/cladding interaction. The database is accessible to registered users from US universities, laboratories, and nuclear industry. Because the data in OPTD has not been formally qualified, its applicability and ability to support licensing activities is limited. This report outlines progress and plans to quality assure data in OPTD, maximizing its impact for model validation and verification as well as qualification of fuels for safe and effective use in advanced reactor designs.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Validation study of sodium pool fire modeling efforts in $\mathrm{MELCOR}$ and $\mathrm{SPHINCS}$ codes

Discharge of sodium coolant into containment from a sodium-cooled fast reactor vessel can occur in the event of a pipe leak or break. In this situation, some of the liquid sodium droplets discharged from the coolant system will react with oxygen in the air before reaching the containment. This phase of the event is normally termed the sodium spray fire phase. Unreacted sodium droplets pool on the containment floor where continued reaction with containment atmospheric oxygen occurs. This phase of the event is normally termed the sodium pool fire phase. Both phases of these sodium-oxygen reactions (or fires) are important to model because of the heat addition and aerosol generation that occur. Any fission products trapped in the sodium coolant may also be released during this progression of events, which if released from containment could pose a health risk to workers and the public. The paper describes progress of an international collaborative research in the area of the sodium fire modeling in the sodium-cooled fast reactors between the United States and Japan under the framework of the Civil Nuclear Energy Research and Development Working Group. In this collaboration between Sandia National Laboratories and Japan Atomic Energy Agency, the validation basis for and modeling capabilities of sodium spray and pool fires in MELCOR of Sandia National Laboratories and SPHINCS of Japan Atomic Energy Agency are being enhanced. Here this study documents MELCOR and SPHINCS sodium pool fire model validation exercises against the JAEA’s sodium pool fire experiments, F7-1 and F7-2. The proposed enhancement of the sodium pool fire models in MELCOR through addition of thermal hydraulic and sodium spreading models that enable a better representation of experimental results is also described.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

FY26 Progress on Demonstration of a Multiphysics Steady State Capability for Modeling Core Radial Expansion in SFRs

Under the U.S. Department of Energy Office of Nuclear Energy Advanced Modeling and Simulation (NEAMS) Program, an integrated multiphysics approach is being developed to model the core bowing phenomena important to liquid metal-cooled fast reactors. Core bowing is an important passive safety mechanism in liquid metal-cooled fast reactors and involves multiphysics effects including radiation transport, fluid flow, heat transfer, and mechanical response to temperature and flux gradients. This report summarizes recent progress on developing a multiphysics, MOOSE-based workflow to predict core bowing and associated reactivity feedback. Significant new capabilities in the reactor physics code Griffin - sodium backfill and pin power reconstruction for deformed geometries - were applied in this effort. This year’s work included verification, code comparisons, sensitivity studies, and coupled demonstrations that advance the state of MOOSE-based core bowing workflow. Griffin’s sodium backfill capability was verified by demonstrating that its automated treatment of geometry expansion and material-density updates reproduces manual calculations exactly, confirming solid mass conservation and proper coolant backfilling in expanded geometries. Reconstructed pin powers were compared for Griffin’s ductheterogeneous and ring-heterogeneous treatments in single-, seven-, and nineteen-assembly cases, with best agreement observed in lower-leakage configurations and the duct-heterogeneous approach offering substantially lower computational cost. Thermal-hydraulic sensitivity sensitivities showed that MOOSE SCM, SAM, and CFD are expected to produce similar deformation predictions despite variances in their temperature predictions, and that explicit treatment of inter-assembly flow becomes increasingly important as gap flow rate increases. Finally, coupled demonstrations on small multi-assembly configurations using Griffin, MOOSE Solid Mechanics, MOOSE SCM, and Heat Conduction produced physically consistent reactivity feedback from thermal expansion and bowing. The coupled demonstrations simulated grid plate expansion as well as resultant core bowing at full power conditions. Simplifications were made in current workflow, namely the assumption of instantaneous full power conditions following hot zero power, and pre-expanding the Griffin geometry axially due to lack of an axial fuel pin expansion model and temperature feedback to Griffin.

Wozniak, Nicholas↗

THERMAL STRATIFICATION IN A POOL-TYPE GEOMETRY

Sodium fast reactors are poised to be a leading candidate for the next generation of commercial reactor deployment. Before licensing can be completed it is important that information be gathered which examines reactor transients during loss of flow accidents. During loss of flow accidents thermally stratified layers can form in the reactor pool. The formation of thermal stratification in the primary pool of a sodium fast reactor during a loss of flow accident can cause cyclic thermal fatigue on the reactor vessel potentially leading to crack formation and weld failure. Computational models have been built to analyze the formation and persistence of thermal stratification during accident transients, but are not currently validated by experimental data. A thermal stratification research facility has been developed and tested to research thermal stratification with loss of flow type conditions. Data from the experiments will be used to validate computational models. The facility can simulate both protected and unprotected loss of flow accident transients in the temperature range of 200-325 [C] with flow rates from 2 gpm to 20 gpm.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

SAS4A/SASSYS-1 Validation with the FFTF LOFWOS Tests #10-12

The FFTF liquid sodium cooled test reactor was built to assist the development and testing of advanced fuels and material for fast reactors. The goals of the FFTF Passive Safety Testing program included confirming the safety margins of FFTF as a liquid metal reactor, providing data for computer code validation, and demonstrating the inherent and passive safety benefits of its specific design features. The program included thirteen unprotected loss of flow without scram tests. The results of modeling and simulation of LOFWOS Tests #10, #11, and #12 are presented in this report to support validation of Argonne’s SAS4A/SASSYS-1 fast reactor safety analysis code. These three tests did not use the primary loop pony motors and thus transitioned to natural circulation flow rates from varying initial power levels. This validation activity leverages modeling and simulation efforts that originated under an International Atomic Energy Agency Coordinated Research Project (CRP) for benchmark analysis of the FFTF LOFWOS Test #13. The SAS4A/SASSYS-1 model originally developed for the CRP has been extended to include LOFWOS Tests #10-12 and modernized to utilize new code features and modeling practices. Predicted results from SAS4A/SASSYS-1 were compared to measured test data and differences were investigated. Overall, it was concluded that, for LOFWOS Tests #10-12, there was good agreement between the flow, power, and temperature predictions and the measured data.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Coupling Experiments and Simulations to Understand Metallic Fuel Behavior

The development of metal alloy fuels for minor actinide transmutation in fast reactor systems is of high importance. However, it faces numerous technical challenges such as: i) fuel behavior has to be benign during core off-normal events; ii) fuel has to maintain integrity to high burnup; iii) low minor actinide fabrication loss under remote handling conditions; and iv) fuel has to lend itself to low-loss recycling process. Limited experimental fuel performance data is currently available to support the selection of a fuel type for a transmutation system. Metallic fuels are being considered for application in fast reactor environment due to the high burn-up, high fissile and fertile density capability, inherent safety characteristics, favorable thermal response, and relatively easy recycling process. The uranium-plutonium-zirconium (U-Pu- Zr) based alloys are considered as one of the most promising metallic fuels for such application. In this work, we present results of microstructural characterization of Pu-Zr and U-Pu-Zr alloys and provide much needed linkage between thermal properties and microscopic scale observation. A firm understanding of microstructural evolution in reactor materials is imperative and will lead to deeper understanding of in-reactor degradation behavior, creating a new generation of radiation-resistant materials and fuels with the potential for significant increases in burn-up.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Irradiation dose and temperature dependence of fracture toughness in high dose HT9 steel from the fuel duct of FFTF

To expand the knowledge base for fast reactor core materials, fracture toughness has been evaluated for high dose HT9 steel using miniature disk compact tension (DCT) specimens. The HT9 steel DCT specimens were machined from the ACO-3 fuel duct of the Fast Flux Test Facility (FFTF), which achieved high doses in the range of 3–148 dpa at 378–504 C. The static fracture resistance (J-R) tests have been performed in a servohydraulic testing machine in vacuum at selected temperatures including room temperature, 200 C, and each irradiation temperature. Brittle fracture with a low toughness less than 50 MPa pm occurred in room temperature tests when irradiation temperature was below 400 C, while ductile fracture with stable crack growth was observed when irradiation temperature was higher. No fracture toughness less than 100 MPa pm was measured when the irradiation temperature was above 430 C. It was shown that the influence of irradiation temperature was dominant in fracture toughness while the irradiation dose has only limited influence over the wide dose range 3–148 dpa. A slow decrease of fracture toughness with test temperature above room temperature was observed for the nonirradiated and high temperature (>430 *C) irradiation cases, which indicates that the ductile–brittle transition temperatures (DBTTs) in those conditions are lower than room temperature. A comparison with the collection of existing data confirmed the dominance of irradiation temperature in the fracture toughness of HT9 steels.

Byun, Thak Sang↗

Generic Repository Concepts and Thermal Analysis for Advanced Fuel Cycles - 12477

A geologic disposal concept for spent nuclear fuel (SNF) or high-level waste (HLW) consists of three components: waste inventory, geologic setting, and concept of operations. A set of reference geologic disposal concepts has been developed by the U.S. Department of Energy (DOE), Used Fuel Disposition campaign. Reference concepts are identified for crystalline rock, clay/shale, bedded salt, and deep borehole (crystalline basement) geologic settings. These were analyzed for waste inventory cases representing a range of waste types that could be produced by advanced nuclear fuel cycles. Concepts of operation consisting of emplacement mode, repository layout, and engineered barrier descriptions, were selected based on international progress. All of these disposal concepts are enclosed emplacement modes, whereby waste packages are in direct contact with encapsulating engineered or natural materials. Enclosed modes have less capacity to dissipate heat than open modes such as that proposed for a repository at Yucca Mountain. Thermal analysis has identified important relationships between waste package size and capacity, and the duration of surface decay storage needed to meet temperature limits for different disposal concepts. For the crystalline rock and clay/shale repository concepts, a waste package surface temperature limit of 100 deg. C was assumed to prevent changes in clay-based buffer material or clay-rich host rock. Surface decay storage of 50 to 100 years is needed for disposal of high-burnup LWR SNF in 4-PWR packages, or disposal of HLW glass from reprocessing LWR uranium oxide (UOX) fuel. High-level waste (HLW) from reprocessing of metal fuel used in a fast reactor could be disposed after decay storage of 50 years or less. For disposal in salt the rock thermal conductivity is significantly greater, and higher temperatures (200 deg. C) can be tolerated at the waste package surface. Decay storage of 10 years or less is needed for high-burnup LWR SNF in 4-PWR packages, while 12-PWR packages could be emplaced after 40 years or less. HLW from reprocessing LWR UOX fuel or metal fuel from fast reactors, could be disposed of in salt after 10 to 50 years of decay storage depending on the specific composition and other factors. For the deep borehole disposal concept no near-field temperature limits are recognized because no performance credit is taken for waste form or waste package integrity, or containment by the near-field host rock. These results show the key differences in thermal management strategies available to the U.S. repository program, given the range of disposal concepts. A host medium such as salt with greater thermal conductivity and peak temperature tolerance could shorten decay storage by 50 years, or facilitate the use of larger waste packages. The LWR UOX SNF evaluated in this study represents that which could be produced in the coming decades. The existing, lower burnup used fuel that is presently in storage at many LWR locations across the U.S. is significantly cooler, and analyses of this type could be used to show that disposal is possible with less decay storage or larger waste packages. We note that while the temperature limits and waste package capacities used in this study are similar to those used internationally and in past U.S. studies, they might be increased as the result of ongoing research and development activities. This study selected enclosed emplacement modes to conform with disposal concepts developed internationally and previously in the U.S. Open modes (such as that proposed for a repository at Yucca Mountain) afford additional flexibility in waste management and the necessary investment, because the same facility serves both storage and disposal functions. Use of open modes, and combined analysis of storage, transportation, and disposal functions, are appropriate to consider in future studies of this type. (authors)

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Atmospheric pressure ionisation - mass spectrometry for argon online monitoring in ASTRID

Safety, operability, waste transmutation and mastered investment costs are key issues for the development of generation IV reactors, especially sodium cooled fast reactors. To achieve a development scheduled around 2040, the nuclear energy division of CEA, France, is studying a prototype called ASTRID (Advanced Sodium Technological Reactor for Industrial Demonstration) which is in its conceptual design phase. To achieve a high level of maturity, In Service Inspection and Repair is very important, in particular fuel cladding failure detection. If such a failure occurs, fission products Xenon and Krypton are released. Their fast and sensitive detection is a challenge. The use of a commercial API-MS is evaluated in this work. Detection limits below 10 ppt have been measured for Kr 84 and for Xe 132. (authors)

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Mechanical Properties of Aged A709

A709 plate is in the process of being developed and qualified through a collaboration by Argonne National Laboratory (ANL), Idaho National Laboratory (INL), and Oak Ridge National Laboratory (ORNL). The goal is to qualify A709 plate in Section III, Division 5 of the American Society of Mechanical Engineers (ASME) Boiler and Pressure Vessel Code (BPVC). This would permit the construction of A709 plate for fast-reactor structural applications. A tradeoff between creep and creep-fatigue properties was established in prior work. A processing route was identified as providing the optimal balance between creep-rupture and elevated-temperature cyclic properties for the solution annealed condition. This condition, however, resulted in a shorter than desired creep-rupture life. Aging is probed to evaluate its potential at further improving mechanical properties. Aging statically precipitates the solutes in solution prior to service. The processing routes identified as providing the best creep-rupture properties and best balance in mechanical properties are investigated. This report discloses the results from tensile, creep, and elevated-temperature cyclic testing performed at INL on the aged material. The aged properties are compared to solution annealed properties. A709 offers improvement in performance compared to 316H particularly at high temperatures; 316H is a material qualified in Section III, Division 5 of the ASME BPVC. For certain high-temperature fast-reactor design conditions, 316H cannot be used while A709 can.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Verification and Validation Tests of Gamma Library of MC2-3 for Coupled Neutron and Gamma Heating Calculation

For the accurate assessment of the heat generation rate in fast reactors, the gamma library of MC2 -3 and the MC2 -3 + GAMSOR procedure employing the coupled neutron and gamma heating calculation has been thoroughly verified against Monte Carlo results and validated using the ZPPR-15D gamma dose measurement data. NJOY outputs are post-processed in a consistent way with the NJOY procedure to avoid any missing data or double counting of data. Prompt heating for 379 out of 391 isotopes in the gamma library was verified against MCNP6.2 to within 1% relative error in total heating for most isotopes. For both a simple one-dimensional slab problem representing a sodium cooled fast reactor and the Experimental Breeder Reactor II (EBR-II) benchmark problem, the root-mean-square values of assembly power error were less than 0.5% for fuel assemblies, ~1% in blankets and ~1 to ~3% in reflectors compared to MCNP6.2 results. The most plausible cause for the 3% error in a reflector assembly is believed to be the error in the multigroup neutron cross sections for the reflector assembly. For validation, gamma doses measured with thermoluminiscent dosimeters (TLDs) in the ZPPR-15D experiment were calculated using GAMSOR. Due to the uncertainty in the TLD measurement with regards to the energy deposition of photons and neutrons, the validation data leads to a 12.7% uncertainty on the experimental measurement. With this uncertainty bound, the calculated doses all fell within one standard deviation of the measured value. Combined with the accurate calculation of reaction rate distributions and neutron spectrum measurements, these results indicate good agreement for the neutron and gamma heating calculations that were performed.

coupled neutron and gamma heating↗