ATR NATIONAL SCIENTIFIC USER FACILITY 2013 ANNUAL REPORT
Advanced Test Reactor National Scientific User Facility 2013 Annual Report
A. Ulrich, Julie↗
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Nuclear Fuels & Materials Spotlight Volume 4
As the nation's nuclear energy laboratory, Idaho National Laboratory brings together talented people and specialized nuclear research capability to accomplish our mission. This edition of the Nuclear Fuels and Materials Division Spotlight provides an overview of some of our recent accomplishments in research and capability development. These accomplishments include: • The first identification of silver and palladium migrating through the SiC layer in TRISO fuel • A description of irradiation assisted stress corrosion testing capabilities that support commercial light water reactor life extension • Results of high-temperature safety testing on coated particle fuels irradiated in the ATR • New methods for testing the integrity of irradiated plate-type reactor fuel • Description of a 'Smart Fuel' concept that wirelessly provides real time information about changes in nuclear fuel properties and operating conditions • Development and testing of ultrasonic transducers and real-time flux sensors for use inside reactor cores, and • An example of a capsule irradiation test. Throughout Spotlight, you'll find examples of productive partnerships with academia, industry, and government agencies that deliver high-impact outcomes. The work conducted at Idaho National Laboratory helps to spur innovation in nuclear energy applications that drive economic growth and energy security. We appreciate your interest in our work here at INL, and hope that you find this issue informative.
99 GENERAL AND MISCELLANEOUS↗
Preliminary Investigation of Zircaloy-4 as a Research Reactor Cladding Material
As part of a scoping study for the ATR fuel conversion project, an initial comparison of the material properties of Zircaloy-4 and Aluminum-6061 (T6 and O-temper) is performed to provide a preliminary evaluation of Zircaloy-4 for possible inclusion as a candidate cladding material for ATR fuel elements. The current fuel design for the ATR uses Aluminum 6061 (T6 and O temper) as a cladding and structural material in the fuel element and to date, no fuel failures have been reported. Based on this successful and longstanding operating history, Zircaloy-4 properties will be evaluated against the material properties for aluminum-6061. The preliminary investigation will focus on a comparison of density, oxidation rates, water chemistry requirements, mechanical properties, thermal properties, and neutronic properties.
22 GENERAL STUDIES OF NUCLEAR REACTORS↗
Summary of LWRS Research in Addressing RPV Research Gaps in NRC EMDA Report
Reactor Pressure Vessels (RPVs) are critical components in nuclear reactors, housing the reactor core and coolant under extreme conditions of temperature, pressure, and radiation. These harsh environments contribute to the degradation of RPV materials over time, presenting challenges for extending reactor operations beyond their original design lifespans. The NRC Expanded Materials Degradation Assessment (EMDA) report volume 3 have been instrumental in guiding research to support extending the operational life of light water reactors (LWRs) up to 80 years. It provides a comprehensive framework to address technical challenges related to aging and degradation mechanisms in RPVs. The LWRS program has played a key role in advancing this research, supporting projects such as the UCSB ATR-2 Experiment, material testing from Zion and Palisades reactors, and the development of advanced mini-compact tension testing techniques. These efforts have been crucial in identifying and addressing gaps in our understanding of RPV aging, contributing to the successful subsequent license renewals of eight LWR units in the U.S. The EMDA report volume 3, built on the Phenomena Identification and Ranking Table (PIRT) analysis from earlier versions of the EPRI Materials Degradation Matrix (MDM) and Issue Management Tables (IMTs), provides a detailed assessment of RPV degradation mechanisms. However, as EPRI has updated the MDM and IMT, it is important to revisit research priorities and methodologies to reflect these changes. The revised MDM and IMT may introduce new factors affecting long-term RPV performance and safety, highlighting the need for continued research and updated guidance to ensure the reliable and safe operation of reactors beyond 80 years.
22 GENERAL STUDIES OF NUCLEAR REACTORS↗
Initial Characterization of ATR End Box Samples
Aluminum samples taken from discarded irradiated Advanced Test Reactor fuel element end boxes (upper and lower adapter ) were characterized to determine the chemical composition and hydration state of the surface oxides. The samples were analyzed using scanning electron microscope imaging and chemical identification, x-ray diffraction to evaluate crystalline morphology, and thermogravitational analysis to determine mass loss by dehydration. The samples were acquired from the discarded fuel element components stored in the ATR fuel handling canal and transferred to the Materials and Fuels Complex for analysis. The measurements indicate that the samples have limited oxide thickness, indicating that little corrosion has occurred beyond the initial passive layer that was intentionally formed prior to irradiation. The presence of minimal aluminum oxyhydroxide suggests that there will be minimal risk to store these fuels in air with limited risk for alteration of the base passive layer. These observations will be compared against samples that will be taken of the same type of fuel that has been in dry storage for more than 10 years.
11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
At-power subcritical multiplication in the advanced test reactor
The degree to which a given physical subdivision of a critical reactor acts as a neutron source for other lobes is not analytically characterized for general application. ATR and ATRC both operate at power, and individual power-producing lobes rely on each other as neutron sources in order to maintain constant power, which in general requires either exactly critical multiplication within a reactor or an external neutron source. Here, this work shows that lobe powers in ATR or ATRC can be related with subcritical multiplication theory, demonstrating that the lobes are not individually critical. This explanation is significant for ATR due to the desire to irradiate a large variety of experiments simultaneously, each having its impact on the core neutron population. This work also establishes the lack of relationship between experiment reactivity worth and cross-sections calculated from fundamental nuclear data. For any physical subdivision of any other critical reactor, it is likewise true that the subdivision undergoes only subcritical multiplication.
21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗
EVALUATION OF CORE PHYSICS ANALYSIS METHODS FOR CONVERSION OF THE INL ADVANCED TEST REACTOR TO LOW-ENRICHMENT FUEL
Computational neutronics studies to support the possible conversion of the ATR to LEU are underway. Simultaneously, INL is engaged in a physics methods upgrade project to put into place modern computational neutronics tools for future support of ATR fuel cycle and experiment analysis. A number of experimental measurements have been performed in the ATRC in support of the methods upgrade project, and are being used to validate the new core physics methods. The current computational neutronics work is focused on performance of scoping calculations for the ATR core loaded with a candidate LEU fuel design. This will serve as independent confirmation of analyses that have been performed previously, and will evaluate some of the new computational methods for analysis of a candidate LEU fuel for ATR.
11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
Experimental quantification of the background neutron flux in the Advanced Test Reactor fuel storage canal - 25562
The Advanced Test Reactor at the Idaho National Laboratory is one of only a few high-power, versatile, research reactors of its type in the world. The ATR fuel storage canal features a gamma irradiation facility that has various uses as well. It is composed of a simple dry tube that extends down into one of the fuel storage rack positions. This tube is surrounded by used fuel elements that can be selected from the inventory to produce the desired gamma radiation level and, to some extent, spectrum within the dry tube. The gamma field within the dry tube is accompanied by a small background neutron flux, produced primarily by photoneutron production in the small fraction of heavy water (D{sub 2}O) that is naturally present in light water. Neutron activation spectrometry was employed to quantify the background neutron flux in the dry tube in a configuration where the gamma exposure rate was approximately 5x10{sup 6} Roentgens per hour. The measurement technique used is very sensitive and provided self-consistent results in terms of raw activation data quality. The background neutron fluxes in the gamma facility were very low, but still detectable. The total neutron flux in the energy region above 0.414 eV and the thermal neutron flux (below 0.414 eV) were estimated from the activation measurements to be 7.5x10{sup 2} and 1.0x10{sup 2} n/cm{sup 2}-s, respectively. High uncertainties (factors of approximately 20-30% in the above-thermal range and 100% in the thermal range) apply to these results. These high uncertainties are primarily due to the limited number of activation interactions that could be used to detect such small fluxes and the resulting propagation of uncertainties associated with the various input parameters involved in the spectral unfolding process. (authors)
11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
ATR Conversion Update for USHPRR Stakeholders Meeting
This presentation provides on update on the ATR Low Enriched Uranium (LEU) Fuel Development project to the United States High Performance Research Reactor (USHPRR) Program.
42 ENGINEERING↗
Evaluation of core physics analysis methods for conversion of the INL advanced test reactor to low-enrichment fuel
Computational neutronics studies to support the possible conversion of the ATR to LEU are underway. Simultaneously, INL is engaged in a physics methods upgrade project to put into place modern computational neutronics tools for future support of ATR fuel cycle and experiment analysis. A number of experimental measurements have been performed in the ATRC in support of the methods upgrade project, and are being used to validate the new core physics methods. The current computational neutronics work is focused on performance of scoping calculations for the ATR core loaded with a candidate LEU fuel design. This will serve as independent confirmation of analyses that have been performed previously, and will evaluate some of the new computational methods for analysis of a candidate LEU fuel for ATR. (authors)
11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
Westinghouse Accident Tolerant Fuel Program
The PowerPoint presentation includes a timeline for the program implementation, the technical approach taken, a summary of testing results, a status of task 2, what has been done to share the results so far, and a summary of upcoming work.
ATR, HIFR, advanced test reactor, high flux isotop↗
NuScale Physics ECAR and Hardware Pictures
NuScale is requesting information on their Consolidated Innovative Nuclear Research (CINR) experiment. The CINR was awarded through the Nuclear Science User Facilities. Photos include the NuScale basket, insert, and instrumentation holder.
11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
Overview of Experiment Process at the Advanced Test Reactor
PowerPoint presentation only for Idaho State University Nuclear Seminar Class
21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗
Improvements to In-Canal Assay of High Specific Activity 60Co at the ATR
Improvements to the quality of measurements in the assaying of High Specific Activity (HSA) cobalt 60 produced at the Advanced Test Reactor at the Idaho National Laboratory are presented. Such assays are conducted regularly between cycles at the ATR, and due to the radiological safety concerns, they are performed within the ATR canal. A standard ion chamber detector was placed in a collimated assay tube within the canal. Another tube, parallel to the detector, was used to position various cobalt 60 standards and targets. The collimated port between these tubes allows for the targets to be pulled across via a winch system. Previous measurements were performed at discrete 1.5-inch steps using a hand-cranked winch system. Charge was collected and integrated for 10 seconds at each discrete step during a scan. Two substantial improvements to the assay include an electronically controlled, motor-driven winch system and a software controlled continuous charge collection. Combined, these changes improved the quality of measurements as well as streamline the assay process. Further examination of these charge profiles indicated a reasonable amount of photon scattering, or shine, before a line-of-sight is established. This created inaccuracies in the reported activity of the cobalt targets. A series of MCNP-6.3 calculations were performed in an effort to quantify and correct for this shine effect. The results of the calculations and how they were employed to a create shine correction factor for the in-canal cobalt assay at the ATR are presented. The overall bias showed an overestimation of the HSA cobalt 60 activity by around 7-8%.
07 - ISOTOPES AND RADIATION SOURCES↗
2011 Annual Industrial Wastewater Reuse Report for the Idaho National Laboratory Site's Advanced Test Reactor Complex Cold Waste Pond
This report describes conditions, as required by the state of Idaho Industrial Wastewater Reuse Permit (LA 000161 01, Modification B), for the wastewater land application site at the Idaho National Laboratory Site's Advanced Test Reactor Complex Cold Waste Pond from November 1, 2010 through October 31, 2011. The report contains the following information: Facility and system description Permit required effluent monitoring data and loading rates Groundwater monitoring data Status of compliance activities Noncompliance and other issues Discussion of the facility's environmental impacts During the 2011 permit year, approximately 166 million gallons of wastewater were discharged to the Cold Waste Pond. This is well below the maximum annual permit limit of 375 million gallons. As shown by the groundwater sampling data, sulfate and total dissolved solids concentrations are highest near the Cold Waste Pond and decrease rapidly as the distance from the Cold Waste Pond increases. Although concentrations of sulfate and total dissolved solids are elevated near the Cold Waste Pond, both parameters were below the Ground Water Quality Rule Secondary Constituent Standards in the down gradient monitoring wells.
2011 Annual Industrial Wastewater Reuse Report↗
Conceptual Design Report for the Xe-6/7/8 Experiment in the NE Flux Trap
X energy, LLC has initiated conceptual design of a high-temperature, pebble-bed reactor and requested that Idaho National Laboratory evaluate the feasibility of irradiating several fuel pebbles in the Advanced Test Reactor. The proposed fuel for the X energy reactor utilizes the same tristructural-isotropic coated fuel particles as are used in the Department of Energy-sponsored Advanced Gas Reactor (AGR) fuel tests, which have been irradiated in the ATR since 2006. The X energy test has been denoted XE 6/7/8 based on nomenclature from the AGR fuel-test series. Three tests will be combined into one test train: XE 6 constitutes the fuel qualification test, whose aim is to demonstrate fuel performance at the upper end of prototypical reactor conditions; XE 7 is designated a “margin test,” and its purpose is to demonstrate fuel integrity at conditions substantially beyond reactor operating conditions; and XE 8 incorporates designed-to-fail particles in order to release fission products and help validate fission product release codes. The XE series of experiments would consist of multiple separate capsules that would be irradiated simultaneously. Each capsule would have its own inert sweep-gas atmosphere with individual on line temperature monitoring. The sweep-gas effluent from each capsule would also have online fission product monitoring to track performance of the fuel in each individual capsule during irradiation.
11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
Effects of ATR-2 Irradiation to High Fluence on Nine RPV Surveillance Materials
The reactor pressure vessel (RPV) in a light-water reactor (LWR) represents the first line of defense against a release of radiation in case of an accident. Thus, regulations that govern the operation of commercial nuclear power plants require conservative margins of fracture toughness, both during normal operation and under accident scenarios. In the unirradiated condition, the RPV has sufficient fracture toughness such that failure is implausible under any postulated condition, including pressurized thermal shock (PTS) in pressurized water reactors (PWR). In the irradiated condition, however, the fracture toughness of the RPV may be severely degraded, with the degree of toughness loss dependent on the radiation sensitivity of the materials. The available embrittlement predictive models and our present understanding of radiation damage are not fully quantitative, and do not treat all potentially significant variables and issues, particularly considering extension of operation to 80y.
22 GENERAL STUDIES OF NUCLEAR REACTORS↗
A Methodology for Loading the Advanced Test Reactor Driver Core for Experiment Analysis
In support of experiments in the ATR, a new methodology was devised for loading the ATR Driver Core. This methodology will replace the existing methodology used by the INL Neutronic Analysis group to analyze experiments. Studied in this paper was the as-run analysis for ATR Cycle 152B, specifically comparing measured lobe powers and eigenvalue calculations.
42 ENGINEERING↗