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DOE OSTI2025

Photoelectron–residual-ion interaction in angle-resolved streaked shake-up ionization of helium

Streaked photoelectron emission spectra access the correlated dynamics of photoelectrons and residual target electrons with attosecond temporal resolution. Here, we calculated ab initio single-ionization spectra for photoemission from helium atoms by colinearly polarized ultrashort XUV and assisting few-femtosecond IR pulses. Distinguishing direct and shake-up ionization resulting in ground-state and excited (𝑛 = 2, 3) He + residual ions, respectively, we examined the effects of the correlated photoemission dynamics on the photoelectron phase accumulation as a function of the observable photoelectron detection direction and kinetic energy and XUV–IR pulse delay. We tracked the dynamical evolution of the residual ion in relative streaked photo- emission delays and found dominant contributions for shake-up emission from the residual-ion–photoelectron interaction. These are in very good and fair agreement, respectively, for 𝑛 = 2 and 𝑛 = 3 shake-up photoemission along the pulse-polarization directions, with previous experimental and theoretical investigations [Ossiander et al ., Nat. Phys. 13, 280 (2017)] and reveal a strong photoemission-direction dependence for shake-up ionization due to the coupling between the photoelectron and evolving residual-ion charge distribution in the IR-laser field.

Stark effect↗

DOE OSTI2023

Spectral and Spatial Properties of Amplified Radiation in High Gain Tapering Enhanced Stimulated Super-radiant Amplification Regime (Technical Report)

There is a wide convergence of scientific and industrial interests in understanding the physics of high efficiency conversion of relativistic electron beam power into coherent radiation. Improved understanding would open the door to ultrahigh intensity X-ray laser pulses (single shot coherent imaging and Schwingerfield physics), as well as at longer wavelength for fast throughput material processing (EUV-lithography). Modern particle accelerators can be extremely efficient (approaching 50 %) in terms of wall-plug energy use. State-of-the-art light sources on the other hand do not take advantage of all the available power and most of it is left in the beam and simply wasted on the beam dump. This proposal aimed at developing a program based on Tapered Enhanced Stimulated Superradiant Amplification to address the current limitation in electron-based coherent radiation generation exploiting the progress in high brightness beam generation and strong coupling with the electromagnetic field in a strongly tapered undulator system.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

NASA NTRS1984

HEAO 3 observations of the Crab pulsar

The Crab pulsar (PSR 0531+21) is the only pulsar which has been observed throughout almost the entire electromagnetic spectrum from 0.5 keV to over 2000 GeV. In general, the emission from the Crab nebula and its pulsar has been remarkably constant in time (except for the pulsations). However, several recent observations, especially of gamma-ray line emission, indicate possible time variations. The present investigation is concerned with the data obtained with the HEAO C-1 experiment. The data have been studied with the hope of finding information regarding a number of questions, taking into account the existence of line emission from the pulsar, the variation of the shape of the light curve with time, and the spectral variations as a function of pulsar phase. The spectrum of the total phase-averaged pulsed emission is found to be consistent with a single power-law spectrum from 50 keV to 10 MeV.

Mahoney, W. A.↗

NASA NTRS2012

Coincident Observation of Lightning using Spaceborne Spectrophotometer and Ground-Level Electromagnetic Sensors

The present study aims at assessing a possible new way to reveal the properties of lightning flash, using spectrophotometric data obtained by FORMOSAT-2/ISUAL which is the first spaceborne multicolor lightning detector. The ISUAL data was analyzed in conjunction with ground ]based electromagnetic data obtained by Duke magnetic field sensors, NLDN, North Alabama Lightning Mapping Array (LMA), and Kennedy Space Center (KSC) electric field antennas. We first classified the observed events into cloud ]to ]ground (CG) and intra ]cloud (IC) lightning based on the Duke and NLDN measurements and analyzed ISUAL data to clarify their optical characteristics. It was found that the ISUAL optical waveform of CG lightning was strongly correlated with the current moment waveform, suggesting that it is possible to evaluate the electrical properties of lightning from satellite optical measurement to some extent. The ISUAL data also indicated that the color of CG lightning turned to red at the time of return stroke while the color of IC pulses remained unchanged. Furthermore, in one CG event which was simultaneously detected by ISUAL and LMA, the observed optical emissions slowly turned red as the altitude of optical source gradually decreased. All of these results indicate that the color of lightning flash depends on the source altitude and suggest that spaceborne optical measurement could be a new tool to discriminate CG and IC lightning. In the presentation, we will also show results on the comparison between the ISUAL and KSC electric field data to clarify characteristics of each lightning process such as preliminary breakdown, return stroke, and subsequent upward illumination.

Adachi, Toru↗

DOE OSTI2023

Imaging electron angular distributions to assess a full-power petawatt-class laser focus

Here we present a technique to assess the focal volume of petawatt-class lasers at full power. Our approach exploits quantitative measurement of the angular distribution of electrons born in the focus via ionization of rarefied gas, which are accelerated forward and ejected ponderomotively by the field. We show that a bivariate (θ,Φ) angular distribution, which was obtained with image plates, not only enables the peak intensity to be extracted, but also reflects nonideality of the focal-spot intensity distribution. In our prototype demonstration at intensities of a few ×10 19 to a few ×10 20 W/cm 2 , an f/10 optic produced a focal spot in the paraxial regime. This allows a plane-wave parametrization of the peak intensity given by tanθ c =2/a 0 (a 0 being the normalized vector potential and θ c the minimum ejection angle) to be compared with our measurements. Qualitative agreement was found using an a 0 inferred from the pulse energy, pulse duration, and focal spot distribution with a modified parametrization, tanθ c =2η/a 0 ($η=2.02^{+0.26}_{–0.22}$). This highlights the need for (i) better understanding of intensity degradation due to focal-spot distortions and (ii) more robust modeling of the ejection dynamics. Using single-shot detection of electrons, we showed that while there is significant shot-to-shot variation in the number of electrons ejected at a given angular position, the average distribution scales with the pulse energy in a way that is consistent with that seen with the image plates. Finally, we note that the asymptotic behavior as θ→0° limits the usability of angular measurement. For 800 nm, this limit is at an intensity ~10 21 W/cm 2 .

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

DOE OSTI2021

Laser cooling of antihydrogen atoms

The photon—the quantum excitation of the electromagnetic field—is massless but carries momentum. A photon can therefore exert a force on an object upon collision 1 . Slowing the translational motion of atoms and ions by application of such a force 2,3 , known as laser cooling, was first demonstrated 40 years ago 4,5 . It revolutionized atomic physics over the following decades 6–8 , and it is now a workhorse in many fields, including studies on quantum degenerate gases, quantum information, atomic clocks and tests of fundamental physics. However, this technique has not yet been applied to antimatter. Here we demonstrate laser cooling of antihydrogen 9 , the antimatter atom consisting of an antiproton and a positron. By exciting the 1S–2P transition in antihydrogen with pulsed, narrow-linewidth, Lyman-α laser radiation 10,11 , we Doppler-cool a sample of magnetically trapped antihydrogen. Although we apply laser cooling in only one dimension, the trap couples the longitudinal and transverse motions of the anti-atoms, leading to cooling in all three dimensions. We observe a reduction in the median transverse energy by more than an order of magnitude—with a substantial fraction of the anti-atoms attaining submicroelectronvolt transverse kinetic energies. We also report the observation of the laser-driven 1S–2S transition in samples of laser-cooled antihydrogen atoms. The observed spectral line is approximately four times narrower than that obtained without laser cooling. The demonstration of laser cooling and its immediate application has far-reaching implications for antimatter studies. A more localized, denser and colder sample of antihydrogen will drastically improve spectroscopic 11–13 and gravitational 14 studies of antihydrogen in ongoing experiments. Furthermore, the demonstrated ability to manipulate the motion of antimatter atoms by laser light will potentially provide ground-breaking opportunities for future experiments, such as anti-atomic fountains, anti-atom interferometry and the creation of antimatter molecules.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

DOE OSTI2019

Electromagnetic backgrounds and potassium-42 activity in the DEAP-3600 dark matter detector

The DEAP-3600 experiment is searching for weakly interacting massive particles dark matter with a 3.3 × 10 3 kg single phase liquid argon (LAr) target, located 2.1 km underground at SNOLAB. The experimental signature of dark matter interactions is kilo electron volt–scale 40 Ar nuclear recoils producing 128 nm LAr scintillation photons observed by photomultiplier tubes. The largest backgrounds in DEAP-3600 are electronic recoils (ERs) induced by β and γ rays originating from internal and external radioactivity in the detector material. A background model of the ER interactions in DEAP-3600 was developed and is described in this work. The model is based on several components which are expected from radioisotopes in the LAr, from ex situ material assay measurements, and from dedicated independent in situ analyses. This prior information is used in a Bayesian fit of the ER components to a 247.2 d dataset to model the radioactivity in the surrounding detector materials. Pulse-shape discrimination separates ER and NR events. However, detailed knowledge of the ER background and activity of detector components sets valuable constraints on NR backgrounds including neutrons and alphas. In addition, the activity of 42 Ar in LAr in DEAP-3600 is determined by measuring the daughter decay of 42 K. Finally, this cosmogenically activated trace isotope is a relevant background at higher energies for other rare event searches using atmospheric argon, e.g., DarkSide-20k, GERDA, or LEGEND. The specific activity of 42 Ar in the atmosphere is found to be 40.4 ± 5.9 μ Bq/kg of argon.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2019

Experimental Study of the Rare Neutral-Kaon Decays at J-PARC (Final Technical Report)

Understanding the origin of CP violation is currently one of the most forefront issues in elementary particle physics. Together with a better understanding of quark mixing and neutrino mixing phenomena, it is one of the central goals of particle physics, and has been pursued vigorously in many experiments. The very rare decay $K_L \to \pi ^0 v\bar{v}$ provides one of the best probes for understanding the original of CP violation in the quark sector. Particularly, theoretical uncertainties are very small in the Standard Model (SM) calculations, and the value therefore most suitable to be tested for beyond SM contributions. J-PARC E14 (also known as KOTO) aims to reach Standard Model sensitivity and beyond with Stage-1 and Stage-2. KOTO acquired 100 hours beam data in May 2013 and the result has been accepted for publication. From 2015-16, KOTO increased the data set by a factor of twenty, which will allow a limit to be set at the Grossman-Nir bound. This bound is valid in virtually any extension of the Standard Model. By comparing this model-independent bound and SM prediction, it is clear that there is considerable room for new physics. Analysis on these collected data sets shows neutron interactions which mimic the two-photon signal could become a potential background. To discriminate neutron background from the photon signal, one important tool, as shown in current data, is to perform detailed waveform analysis of the signal from the phototubes. To fully capture the calorimeter pulse shape with best fidelity from 100 out of the 2700 channels of CsI, we built the 500 MSPS (Mega Samples Per Second) with 14-bit digitizers. With KOTO Stage-2 currently in the planning stages, we started R&D work on a full width, but length scalable photon veto barrel detector with detailed layout of active detector elements.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

NASA NTRS2002

Ion Dynamic Capture Experiments With The High Performance Antiproton Trap (HiPAT)

To take the first step towards using the energy produced from the matter-antimatter annihilation for propulsion applications, the NASA Marshall Space Flight Center (MSFC) Propulsion Research Center (PRC) has initiated a research activity examining the storage of low energy antiprotons. The High Performance Antiproton Trap (HiPAT) is an electromagnetic system (Penning-Malmberg design) consisting of a 4 Tesla superconductor, a high voltage electrode confinement system, and an ultra high vacuum test section. It has been designed with an ultimate goal of maintaining 10(exp 12) charged particles with a half-life of 18 days. Currently, this system is being evaluated experimentally using normal matter ions that are cheap to produce, relatively easy to handle, and provide a good indication of overall trap behavior (with the exception of assessing annihilation losses). The ions are produced via a positive hydrogen ion source and transported to HiPAT in a beam line equipped with electrostatic optics. The optics serve to both focus and gate the incoming ions, providing microsecond-timed beam pulses that are dynamically captured by cycling the HiPAT forward containment field like a "trap door". Initial dynamic capture experiments have been successfully performed with beam energy and currents set to 1.9 kV and 23 micro-amps, respectively. At these settings up to 2x10(exp 9) ions have been trapped during a single dynamic cycle.

Martin, James↗

DOE OSTI2025

Coherent frequency combs from electrons colliding with a laser pulse

Highly coherent and powerful light sources capable of generating soft x-ray frequency combs are essential for high precision measurements and rigorous tests of fundamental physics. In this work, we derive the analytical conditions required for the emission of coherent radiation from an electron beam colliding with a laser pulse, modeled as a plane wave. These conditions are applied in a series of numerical simulations, where we show that a soft x-ray frequency comb can be produced if the electrons are regularly-spaced and sufficiently monoenergetic. High quality beams of this kind may be produced in the near future from laser-plasma interactions or linear accelerators. Furthermore, we highlight the advantageous role of employing few-cycle laser pulses in relaxing the stringent monoenergeticity requirements for coherent emission. The conditions derived here can also be used to optimize coherent emission in other frequency ranges, such as the terahertz domain.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

DOE OSTI2020

Pathways to excitation of atoms with bicircular laser pulses

We study the excitation of the hydrogen atom by bichromatic circularly polarized laser pulses using numerical solutions of the time-dependent Schrödinger equation. The results are in agreement with the selection rules for multiphoton processes in such fields, namely, excited states are populated in which orbital angular momentum and magnetic quantum numbers are either both odd or both even, independent of the relative helicity, peak intensity, and pulse duration of the pulses. For co-rotating pulses the results show that excitation predominantly proceeds to states with magnetic quantum number of the same helicity as the laser pulses. Besides pathways via direct photon absorption from the ground state our results indicate that a transfer of population among the Rydberg states occurs via Λ-type transitions. In the case of counter-rotating pulses the largest excitation probability is found for Rydberg states that differ in magnetic quantum number by Δm=±3. This pattern allows us to estimate how many photons from each of the two bichromatic fields have been absorbed. Finally, we confirm that a population in Rydberg states beyond a maximum orbital angular quantum number is unlikely.

74 ATOMIC AND MOLECULAR PHYSICS↗

DOE OSTI2024

Toward an integrated multi-gigahertz ionizing particle diagnostic

Needs arising at both current and future accelerator facilities call for the development of radiation-hardened position-sensing diagnostics that can operate with multi-GHz repetition rates. Such instruments are likely to also have applications in the diagnosis of rapid plasma behavior. Here, building on the recent work of our Advanced Accelerator Diagnostics Collaboration, we are exploring the development of integrated multi-GHz ionizing particle detection systems based on chemical-vapor deposition diamond sensors, with the initial goal of producing a quadrant detector that can determine the intensity and centroid position of a particle beam at a repetition rate between 5 and 10 GHz. Results from our initial high-speed characterization work are presented, including those from a single-channel sensor with a GHz response. Approaches to achieving multi-GHz (5–10 GHz) rate capability, including the design of a dedicated Application Specific Integrated Circuit and the use of 3D RF-solver computer aided design software, are presented and discussed in more detail. 3D RF simulations suggest clean pulses of duration less than 250 ps (FWHM less than 125 ps) can be achieved with the approaches developed by this work.

43 PARTICLE ACCELERATORS↗

DOE OSTI2024

Development of a high current density, high temperature superconducting cable for pulsed magnets

Abstract A low AC loss Rare Earth Barium Copper Oxide (REBCO) cable, based on the VIPER cable technology has been developed by Commonwealth Fusion Systems for use in high field, REBCO based tokamaks. The new cable is composed of partitioned and transposed copper ‘petals’ shaped to fit together in a circular pattern with each petal containing a REBCO tape stack and insulated from each other to reduce AC losses. A stainless steel jacket adds mechanical robustness—also serving as a vessel for solder impregnation—while a tube runs through the middle for cooling purposes. Additionally, fiber optic sensors are placed under the tape stacks for quench detection. To qualify this design, a series of experiments were conducted as part of the SPARC tokamak Central Solenoid Model Coil program—to retire the risks associated with full scale, fast ramping, high flux HTS Central Solenoid (CS) and Poloidal Field (PF) coils for tokamak fusion power plants and net energy demonstrators. These risk study and risk reduction experiments include (1) AC loss measurement and model validation in the range of ~5 T/s, (2) an IxB electromagnetic loading of over 850 kN/m at the cable level and up to 300 kN/m at the stack level, (3) a transverse compression resilience of over 350 MPa, (4) manufacturability at tokamak relevant speeds and scales, (5) cable to cable joint performance, (6) fiber optic based quench detection speed, accuracy, and feasibility, and (7) overall winding pack integration and magnet assembly. The result is a cable technology, now referred to as PIT VIPER, with AC losses that measure fifteen times lower (at ~5 T/s) than its predecessor technology; a 2% or lower degradation of critical current (Ic) at high IxB electromagnetic loads; no detectable Ic degradation up to 570 MPa of transverse compression on the cable unit cell; end to end magnet manufacturing, consistently producing Ic values within 7% of the model prediction; cable to cable joint resistances at 20 K on the order of ~15 nΩ; and fast, functional quench detection capabilities that do not involve voltage taps. This cable technology will be tested comprehensively in a Central Solenoid Model Coil to prove its readiness for compact, high field tokamak operation.

Sanabria, Charlie (ORCID:0000000150175309)↗

DOE OSTI2021

Transition metal dichalcogenide monolayers in an ultrashort optical pulse: Femtosecond currents and anisotropic electron dynamics

We theoretically study the interaction of an ultrafast intense linearly polarized optical pulse with monolayers of transition metal dichalcogenides (TMDCs). Such a strong pulse redistributes electrons between the bands and generates femtosecond currents during the pulse. Due to the large bandwidth of the incident pulse, this process is completely an off-resonant. While in TMDCs, the time-reversal symmetry is conserved, the inversion symmetry is broken, and these monolayers have axial symmetry along the armchair direction but not along with the zigzag one. The pulse, polarized along with asymmetric directions of TMDC monolayer, generates both longitudinal, i.e., along the direction of polarization, and transverse, i.e., in the perpendicular direction, currents. Such currents result in charge transfer through the system. Finally, we study different TMDC materials and show how the femtosecond transport in TMDC monolayers depend on their parameters, such as lattice constant and bandgap.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

NASA NTRS1991

Finite difference time domain calculation of transients in antennas with nonlinear loads

Determining transient electromagnetic fields in antennas with nonlinear loads is a challenging problem. Typical methods used involve calculating frequency domain parameters at a large number of different frequencies, then applying Fourier transform methods plus nonlinear equation solution techniques. If the antenna is simple enough so that the open circuit time domain voltage can be determined independently of the effects of the nonlinear load on the antennas current, time stepping methods can be applied in a straightforward way. Here, transient fields for antennas with more general geometries are calculated directly using Finite Difference Time Domain (FDTD) methods. In each FDTD cell which contains a nonlinear load, a nonlinear equation is solved at each time step. As a test case, the transient current in a long dipole antenna with a nonlinear load excited by a pulsed plane wave is computed using this approach. The results agree well with both calculated and measured results previously published. The approach given here extends the applicability of the FDTD method to problems involving scattering from targets, including nonlinear loads and materials, and to coupling between antennas containing nonlinear loads. It may also be extended to propagation through nonlinear materials.

Luebbers, Raymond J.↗

NASA NTRS2007

Coherence Phenomena in Coupled Optical Resonators

Quantum coherence effects in atomic media such as electromagnetically-induced transparency and absorption, lasing without inversion, super-radiance and gain-assisted superluminality have become well-known in atomic physics. But these effects are not unique to atoms, nor are they uniquely quantum in nature, but rather are fundamental to systems of coherently coupled oscillators. In this talk I will review a variety of analogous photonic coherence phenomena that can occur in passive and active coupled optical resonators. Specifically, I will examine the evolution of the response that can occur upon the addition of a second resonator, to a single resonator that is side-coupled to a waveguide, as the coupling is increased, and discuss the conditions for slow and fast light propagation, coupled-resonator-induced transparency and absorption, lasing without gain, and gain-assisted superluminal pulse propagation. Finally, I will discuss the application of these systems to laser stabilization and gyroscopy.

Smith, David D.↗

NASA NTRS2004

Liquid-Metal-Fed Pulsed Plasma Thrusters

A short document proposes liquid-metal-fed pulsed plasma thrusters for small spacecraft. The propellant liquid for such a thruster would be a low-melting-temperature metal that would be stored molten in an unpressurized, heated reservoir and would be pumped to the thruster by a magnetohydrodynamic coupler. The liquid would enter the thruster via a metal tube inside an electrically insulating ceramic tube. A capacitor would be connected between the outlet of the metal tube and the outer electrode of the thruster. The pumping would cause a drop of liquid to form at the outlet, eventually growing large enough to make contact with the outer electrode. Contact would close the circuit through the capacitor, causing the capacitor to discharge through the drop. The capacitor would have been charged with enough energy that the discharge would vaporize, ionize, and electromagnetically accelerate the contents of the metal drop. The resulting plasma would be ejected at a speed of about 50 km/s. The vaporization of the drop would reopen the circuit through the capacitor, enabling recharging of the capacitor. As pumping continued, a new drop would grow and the process would repeat.

Markusic, Thomas↗

DOE OSTI2017

A collision timing monitor for SuperKEKB

The analysis of beamstrahlung radiation, emitted from a beam of charged particles due to the electromagnetic interaction with a second beam of charged particles, provides a diagnostic tool that can be used to monitor beam–beam collisions in a e + e - storage ring. In this paper we show that the beamstrahlung time profile is related to the timing of the collisions and the length of the beams, and how its measurement can be used to monitor and optimize collisions at the interaction point of the SuperKEKB collider. The method has a unique passive monitor capability, since it allows to monitor the timing of the collision without disturbing (scanning) the beam–beam timing, which needs to be measured to unprecedented accuracy at SuperKEKB. To measure the time dependence of beamstrahlung, here we describe a method based on nonlinear frequency mixing in a nonlinear crystal of beamstrahlung radiation with photons from a pulsed laser. We demonstrate that the method allows to measure and optimize the relative timing and length of the colliding bunches with 3% accuracy.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗