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At least 739 records · Page 41

Spin dynamics induced by ultrafast heating with ferromagnetic/antiferromagnetic interfacial exchange in perpendicularly magnetized hard/soft bilayers

The laser-induced spin dynamics of FeCo in perpendicularly magnetized L1{sub 0}-MnGa/FeCo bilayers with ferromagnetic and antiferromagnetic interfacial exchange coupling (IEC) are examined using the time-resolved magneto-optical Kerr effect. We found a precessional phase reversal of the FeCo layer as the IEC changes from ferromagnetic to antiferromagnetic. Moreover, a precession-suspension window was observed when the magnetic field was applied in a certain direction for the bilayer with ferromagnetic IEC. Our observations reveal that the spin dynamics modulation is strongly dependent on the IEC type within the Landau-Lifshitz-Gilbert depiction. The IEC dependence of the precessional phase and amplitude suggests the interesting method for magnetization dynamics modulation.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Spin Dynamics of Triple-𝐐 Magnetic Orderings in a Triangular Lattice: Implications for Multi-𝐐 Orderings in General Two-Dimensional Lattices

Multi-𝐐 magnetic structures on two-dimensional (2D) lattices provide a key route to realizing topological physics in 2D magnetism. A major experimental challenge is to unambiguously confirm their formation by excluding the possibility of topologically trivial multidomain single- or double-𝐐 magnetic orders, which cannot be distinguished using conventional diffraction techniques. Here, we propose that long-wavelength spin dynamics offers a universal diagnostic for triangular lattices: Triple-𝐐 orders that preserve rotational symmetry and single- or double-𝐐 orders that break it exhibit qualitatively distinct anisotropies in their Goldstone-mode velocities, stemming from fundamental differences in their underlying spin configurations. We validate this concept using the metallic triangular-lattice antiferromagnet Co 0.325 ⁢TaS 2 , which hosts both a stripe-type single-𝐐 state and a triple-𝐐 tetrahedral ordering at different temperatures. Using inelastic neutron-scattering and spin dynamics simulations, we first refine the spin Hamiltonian by fitting the paramagnetic excitation spectra, allowing us to develop an unbiased model independent of magnetic ordering. We then show that the observed velocity profiles of the Goldstone modes agree with the high-temperature model’s predictions: markedly anisotropic for the single-𝐐 phase and near isotropic for the triple-𝐐 phase. Importantly, this contrast persists across various exchange parameters, highlighting its model-independent nature and suggesting potential applicability to other 2D lattice systems. Beyond the long-wavelength regime, we present a substantial discrepancy between the measured and simulated magnon spectra exclusively in the triple-𝐐 phase. We attribute this discrepancy to magnon energy renormalization arising from order-of-magnitude-enhanced magnon-magnon interactions in the triple-𝐐 phase, due to its noncollinear configuration. This work provides universal insight into the dynamical properties of topological multi-𝐐 magnetic orderings in 2D lattice structures, offering a broadly applicable diagnostic to distinguishing them from topologically trivial single- or double-𝐐 counterparts. The unequivocal confirmation of the triple-𝐐 structure in Co 0.325 ⁢TaS 2 further establishes it as a prominent material platform for exploring topological spin textures in the genuine 2D limit.

Park, Pyeongjae [Oak Ridge National Laboratory (OR↗

N - V –Diamond Magnetic Microscopy Using a Double Quantum 4-Ramsey Protocol

We introduce a double quantum (DQ) 4-Ramsey measurement protocol that enables wide-field magnetic imaging using nitrogen-vacancy (N-V) centers in diamond, with enhanced homogeneity of the magnetic sensitivity relative to conventional single quantum (SQ) techniques. The DQ 4-Ramsey protocol employs microwave-phase alternation across four consecutive Ramsey (4-Ramsey) measurements to isolate the desired DQ magnetic signal from any residual SQ signal induced by microwave pulse errors. In a demonstration experiment employing a 1-μm-thick N-V layer in a macroscopic diamond chip, the DQ 4-Ramsey protocol provides a volume-normalized dc magnetic sensitivity of η V = 34nTHz –1/2 μm 3/2 across a 125 μm × 125 μm field of view, with about 5× less spatial variation in sensitivity across the field of view compared to a SQ measurement. Furthermore, the improved robustness and magnetic sensitivity homogeneity of the DQ 4-Ramsey protocol enables imaging of dynamic broadband magnetic sources such as integrated circuits and electrically active cells.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Conservation of angular momentum in ultrafast spin dynamics

The total angular momentum of a closed system is a conserved quantity, which should remain constant in time for any excitation experiment once the pumping signal has been extinguished. Such conservation, however, is never satisfied in practice in any real-time first-principles description of the demagnetization process. Furthermore, there is growing experimental evidence that the same takes place in experiments. The missing angular momentum is usually associated to lattice vibrations, which are not measured experimentally and are never considered in real-time simulations. Here, in this study, we critically analyze the issue and conclude that current state-of-the-art simulations violate angular momentum conservation already at the electronic level of description. This shortcoming originates from an oversimplified description of the spin-orbit coupling, which includes atomic contributions but neglects completely that of itinerant electrons. We corroborate our findings with time-dependent simulations using model tight-binding Hamiltonians, and show that indeed such conservation can be reintroduced by an appropriate choice of spin-orbit coupling. The consequences of our findings on recent experiments are also discussed.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Magnetic and Elastic Vibrations in Manganese–Zinc Spinel Crystals as the Functions of Anisotropy Constant

The amplitudes of magnetic and elastic vibrations for Mn{sub 0.61}Zn{sub 0.35}Fe{sub 2.04}O{sub 4} spinel crystalline slab are calculated by solving the equations describing the magnetic and elastic dynamics. The anisotropy constants, magnetization, second-order elastic constants and magnetoelastic coupling constants for a studied crystal are expressed as the functions of temperature. The magnetization vector and elastic shear components are found as the functions of the first magnetic anisotropy constant at different values of an external constant magnetic field greater than a saturation field. The procession patterns for normally and tangentially magnetized slabs are displayed for two values of the first anisotropy constant. High absolute values of the first anisotropy constant are shown to refer to reorientation of the magnetization vector.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Supergranulation-driven Alfven waves in the solar chromosphere and related phenomena.

It has recently been recognized that Alfven waves frequently dominate the microstructure of the solar wind at the orbit of the earth. We seek a solar source for these waves, and consider here their excitation by the supergranular motions. The wave equation is solved in a horizontally stratified, bi-exponential solar atmosphere. The interaction of Alfven wave motions associated with adjacent supergranules is discussed qualitatively. The Alfven wave effectively conveys the supergranular motions to great heights in the chromosphere. These motions are oppositely directed above intersupergranule boundaries, and compress the magnetic field there. A naive calculation of the compression, based on balancing dynamic and magnetic pressures, leads to adequate agreement with observations of the chromospheric network. We find that the magnetic field is appreciably compressed only below about 1500 km, and on this basis we reject theories of spicule formation which require large vertical magnetic fields at the heights reached by spicules. We advance a theory for spicule formation, in which spicules form as a result of matter being squeezed upward, out of the compression region between adjacent supergranules.

Hollweg, J. V.↗

Spin-lattice coupling in uranium dioxide probed by magnetostriction measurements at high magnetic fields (P08358-E001-PF)

Our preliminary magnetostriction measurements have already shown a strong interplay of lattice dynamic and magnetism in both antiferromagnetic and paramagnetic states, and give unambiguous evidence of strong spin- phonon coupling in uranium dioxide. Further studies are planned to address the puzzling behavior of UO 2 in magnetic and paramagnetic states and details of the spin-phonon coupling.

36 MATERIALS SCIENCE↗

Numerical simulations of magnetized jets

The present axisymmetric numerical simulations of light hypersonic jets allow unmagnetized jets and jets carrying a dynamically important magnetic field to be contrasted. After decelerating a weakly magnetized jet through a series of weak, oblique shocks, a Mach disk and a strong annular shock are encountered near the outer edges of the contact discontinuity separating the shocked fluid from the shocked ambient gas. Upon passing the annular shock, the gas quickly expands and enters a backflowing cocoon surrounding the jet. The overall speed of advance of the jet is reduced; matter near the jet axis which passes through the terminal Mach disk accumulates in a plug, and gas is discharged into the cocoon by the intermittent shedding of vortices. When magnetic stresses dominate, however, the jet is rapidly decelerated via a Mach disk and strong annular shock.

Lind, Kevin R.↗

Image Quality of the Helioseismic and Magnetic Imager (HMI) Onboard the Solar Dynamics Observatory (SDO)

We describe the imaging quality of the Helioseismic and Magnetic Imager (HMI) onboard the Solar Dynamics Observatory (SDO) as measured during the ground calibration of the instrument. We describe the calibration techniques and report our results for the final configuration of HMI. We present the distortion, modulation transfer function, stray light,image shifts introduced by moving parts of the instrument, best focus, field curvature, and the relative alignment of the two cameras. We investigate the gain and linearity of the cameras, and present the measured flat field.

Solar Dynamics Observatory↗

Current induced magnetization switching in Co/Cu/Ni-Fe nanopillar with orange peel coupling

The impact of orange peel coupling on spin current induced magnetization switching in a Co/Cu/Ni-Fe nanopillar device is investigated by solving the switching dynamics of magnetization of the free layer governed by the Landau-Lifshitz-Gilbert-Slonczewski (LLGS) equation. The value of the critical current required to initiate the magnetization switching is calculated analytically by solving the LLGS equation and verified the same through numerical analysis. Results of numerical simulation of the LLGS equation using Runge-Kutta fourth order procedure shows that the presence of orange peel coupling between the spacer and the ferromagnetic layers reduces the switching time of the nanopillar device from 67 ps to 48 ps for an applied current density of 4 × 10{sup 12}Am{sup −2}. Also, the presence of orange peel coupling reduces the critical current required to initiate switching, and in this case, from 1.65 × 10{sup 12}Am{sup −2} to 1.39 × 10{sup 12}Am{sup −2}.

36 MATERIALS SCIENCE↗

Dynamics of a fractal set of first-order magnetic phase transitions in frustrated Lu 2 CoMnO 6

The axial next-nearest-neighbor Ising model predicts a fractal (infinite) set of phases with incommensurate wave vectors that are separated by first-order phase boundaries. This complexity results from a simple frustration condition between nearest- and next-nearest-neighbor interactions along a chain of Ising spins. Using x-ray photon correlation spectroscopy (XPCS), we investigate the surprising antiferromagnetic dynamics that emerge from such a complex phase diagram over a wide range of temperatures. In this work, we present XPCS measurements of the frustrated magnetic chain compound Lu 2 CoMnO 6 and Monte Carlo simulations. Incommensurate magnetic Bragg peaks slide towards commensurate “up-up-down-down” spin order with decreasing temperature and increasing time. Both simulation and experiment support a counterintuitive “upside-down” temperature dependence of the magnetic dynamics: at higher temperatures in the region of first-order phase boundaries, slower dynamics are observed where the speckle maintains its coherence. At the lowest temperatures, where part of the sample adopts commensurate order, the dynamics speed up and result in fast decoherence.

36 MATERIALS SCIENCE↗

Modified helix-like instability structure on imploding z-pinch liners that are pre-imposed with a uniform axial magnetic field

Recent experiments at the Sandia National Laboratories Z Facility have, for the first time, studied the implosion dynamics of magnetized liner inertial fusion (MagLIF) style liners that were pre-imposed with a uniform axial magnetic field. As reported [T. J. Awe et al., Phys. Rev. Lett. 111, 235005 (2013)] when premagnetized with a 7 or 10 T axial field, these liners developed 3D-helix-like hydrodynamic instabilities; such instabilities starkly contrast with the azimuthally correlated magneto-Rayleigh-Taylor (MRT) instabilities that have been consistently observed in many earlier non-premagnetized experiments. The helical structure persisted throughout the implosion, even though the azimuthal drive field greatly exceeded the expected axial field at the liner's outer wall for all but the earliest stages of the experiment. Whether this modified instability structure has practical importance for magneto-inertial fusion concepts depends primarily on whether the modified instability structure is more stable than standard azimuthally correlated MRT instabilities. In this manuscript, we discuss the evolution of the helix-like instability observed on premagnetized liners. While a first principles explanation of this observation remains elusive, recent 3D simulations suggest that if a small amplitude helical perturbation can be seeded on the liner's outer surface, no further influence from the axial field is required for the instability to grow.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Spin-glass dynamics in the presence of a magnetic field: exploration of microscopic properties

The synergy between experiment, theory, and simulations enables a microscopic analysis of spin-glass dynamics in a magnetic field in the vicinity of and below the spin-glass transition temperature T g . The spin-glass correlation length, ξ(t, t w ; T), is analysed both in experiments and in simulations in terms of the waiting time t w after the spin glass has been cooled down to a stabilised measuring temperature T < T g and of the time t after the magnetic field is changed. This correlation length is extracted experimentally for a CuMn 6 at. % single crystal, as well as for simulations on the Janus II special-purpose supercomputer, the latter with time and length scales comparable to experiment. The non-linear magnetic susceptibility is reported from experiment and simulations, using ξ(t, t w ; T) as the scaling variable. Previous experiments are reanalysed, and disagreements about the nature of the Zeeman energy are resolved. The growth of the spin-glass magnetisation in zero-field magnetisation experiments, M ZFC (t, t w ; T), is measured from simulations, verifying the scaling relationships in the dynamical or non-equilibrium regime. Lastly, our preliminary search for the de Almeida–Thouless line in D = 3 is discussed.

36 MATERIALS SCIENCE↗

Magnetic interactions in γ-Fe{sub 2}O{sub 3}@SiO{sub 2} nanocomposites

Structural and magnetic properties of γ-Fe{sub 2}O{sub 3} nanoparticles of 4 nm diameter, dispersed into silica SiO{sub 2} matrix with a wide range value of volume fraction (0.05 to 1), were investigated. Produced γ-Fe{sub 2}O{sub 3}@SiO{sub 2} nanocomposites consist of an assembly of very small single domain magnetic object (<10 nm) with a random distribution of both inter-particle distance and direction of particle magnetic moment. We focused on the determination of a magnetic percolation threshold, defined as the magnetic particles concentration value above which the magnetic properties of isolated particles vanished in favor of a magnetic collective behavior induced by magnetic interactions. A percolation threshold value of 0.63 was obtained by a local probe technique such as {sup 57}Fe Mössbauer spectrometry and confirmed by global magnetic measurements through zero-field cooled, field-cooled, and ac susceptibility data. Below this threshold, dynamic ac magnetization measurements show a thermally activated Arrhenius dependence of the blocking temperature of superparamagnetic nanoparticles and above this critical value, one observes a slowing down of their dynamic properties, which lead toward the establishment of a spin-glass like state.

36 MATERIALS SCIENCE↗

Dynamic spin localization and γ -magnets

Here, we explore an unusual type of quantum matter that can be realized by qubits having different physical origins. Interactions in this matter are described by essentially different coupling operators for all qubits. We show that the simplest such models, which can be realized with localized states in Dirac materials, satisfy integrability conditions that we use to describe pseudospin dynamics in a linearly time-dependent magnetic field. Generalizing to an arbitrary number of qubits, we construct a spin Hamiltonian, which we call the γ -magnet. This system does not conserve polarization of any spin and the net spin polarization. Nevertheless, for arbitrarily strong interactions, nonadiabatic dynamics, and any initial eigenstate, we find that quantum interference suppresses spin flips. This behavior resembles many-body localization but occurs in phase space of many spins rather than real space. This effect may not have a counterpart in classical physics and can be a signature of a new type of spin ordering, which is different from both disordered spin glasses and ordered phases of spin lattices.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Modeling of different scenarios of thin current sheet equilibria in the Earth’s magnetotail

The Earth’s magnetosphere is an open dynamic system permanently interacting with the solar wind, i.e., the plasma flow from the Sun. Some plasma processes in the magnetosphere are of spontaneous explosive character, while others develop rather slowly as compared to the characteristic times of plasma particle motion in it. The large-scale current sheet in the magnetotail can be in an almost equilibrium state both in quiet periods and during geomagnetic perturbations, and its variations can be considered quasistatic. Thus, under some conditions, the magnetotail current sheet can be described as an equilibrium plasma system. Its state depends on various parameters, in particular, on those determining the dynamics of charged particles. Knowing the main governing parameters, one can study the structure and properties of the current sheet equilibrium. This work is devoted to the self-consistent modeling of the equilibrium thin current sheet (TCS) of the Earth’s magnetotail, the thickness of which is comparable with the ion gyroradius. The main objective of this work is to examine how the TCS structure depends on the parameters characterizing the particle dynamics and magnetic field geometry. A numerical hybrid self-consistent TCS model in which the tension of magnetic field lines is counterbalanced by the inertia of ions moving through the sheet is constructed. The ion dynamics is considered in the quasi-adiabatic approximation, while the electron motion, in the conductive fluid approximation. Depending on the values of the adiabaticity parameter κ (which determines the character of plasma particle motion) and the dimensionless normal component of the magnetic field b{sub z}, the following two scenarios are considered: (A) the adiabaticity parameter is proportional to the particle energy and b{sub z} = const and (B) the particle energy is fixed and the adiabaticity parameter is proportional to b{sub z}. The structure of the current sheet and particle dynamics in it are studied as functions of the parameters κ and b{sub z}. It is shown that, in scenario A, the current sheet thickness decreases with increasing adiabaticity parameter due to a decrease in the ion gyroradius. Accordingly, the radius of curvature of magnetic field lines decreases, which leads to an increase in the contribution of electron drift currents near the neutral plane z = 0. Numerical simulations demonstrate that current equilibria can exist if the adiabaticity parameter lies in the range 0.05 ≤ κ ≤ 0.7. At κ ∼ 0.7, the contribution of electron drift currents to the total current density is much larger than the contribution of ions and the ion motion becomes chaotic. At larger values of the adiabaticity parameter, no equilibrium solutions were found in the framework of the given one-dimensional model. Therefore, the value κ = 0.7 corresponds to the upper applicability limit of the quasi-adiabatic model of the current sheet. In scenario B, an increase in the parameter κ leads to the appearance of a large number of quasi-trapped ions in the current sheet, due to which the current sheet thickens and the amplitude of the current density decreases. As a result, equilibrium solutions exist in a much narrower range of the adiabaticity parameter, 0.05≤ κ ≤ 0.25. Consequences of the existence of parametric boundaries of equilibrium solutions for the TCS under actual geomagnetic conditions are discussed.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Energetics and dynamics of resonant and nonresonant scattering in strong magnetic fields

The energetics and the dynamics resulting from electron-photon resonant and nonresonant scattering in a plasma with magnetic field about 10 to the 12th G are studied in detail. Precise analytic results are obtained in the optically thin limit, and numerical results are presented for the optically thick case. For the latter, it is found that when the equilibrium temperature T(C) is determined by the cooling/heating balance due solely to cyclotron resonant scattering, the ratio of T(C) to the superstrong field B remains fairly constant for N(e) up to about 6 x 10 to the 21st electrons/sq cm. This line-dominated region comes to an end when the extra heating from the hard continuum photons becomes competitive with the line processes and drives T(C) well above the pure line value. For parameters characteristic of GB 880205, the thickness of the line-dominated region is determined to be between 10 to the 21st and 10 to the 22nd electrons/sq cm.

Lamb, Don Q.↗

Spin Transfer Torque Switching in Pentalayer Nanopillar with Biquadratic Coupling

The effect of biquadratic coupling on spin transfer torque-assisted magnetization switching in the pentalayer nanopillar device is studied by numerically solving the magnetization switching dynamics of the free layer governed by the Landau- Lifshitz-Gilbert-Slonczewski (LLGS) equation. Magnetization switching time in the absence of biquadratic coupling for an applied current density of 10 × 10{sup 11}Am{sup − 2} is 186 ps. Biquadratic coupling arises due to the uncorrelated roughness in the ferromagnetic layers and it reduces the switching time to 160 ps. Further, the impact of the period of roughness and spacer layer thickness on switching time are studied.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗