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DOE OSTI2019

The Necessity for Iteration in the Application of Numerical Simulation to EGS: Examples from the EGS Collab Test Bed 1

The United States Department of Energy, Geothermal Technologies Office (GTO) is funding a collaborative investigation of enhanced geothermal systems (EGS) processes at the meso-scale. This study, referred to as the EGS Collab project, is a unique opportunity for scientists and engineers to investigate the creation of fracture networks and circulation of fluids across those networks under in-situ stress conditions. The EGS Collab project is envisioned to comprise three experiments and the site for the first experiment is on the 4850 Level in phyllite of the Precambrian Poorman formation, at the Sanford Underground Research Facility, located at the former Homestake Gold Mine, in Lead, South Dakota. Principal objectives of the project are to develop a number of intermediate-scale field sites and to conduct well-controlled in situ experiments focused on rock fracture behavior and permeability enhancement. Data generated during these experiments will be compared against predictions of a suite of computer codes specifically designed to solve problems involving coupled thermal, hydrological, geomechanical, and geochemical processes. Comparisons between experimental and numerical simulation results will provide code developers with direction for improvements and verification of process models, build confidence in the suite of available numerical tools, and ultimately identify critical future development needs for the geothermal modeling community. Moreover, conducting thorough comparisons of models, modelling approaches, measurement approaches and measured data, via the EGS Collab project, will serve to identify techniques that are most likely to succeed at the Frontier Observatory for Research in Geothermal Energy (FORGE), the GTO’s flagship EGS research effort. As noted, outcomes from the EGS Collab project experiments will serve as benchmarks for computer code verification, but numerical simulation additionally plays an essential role in designing these meso-scale experiments. This paper reviews specific numerical simulations supporting the design of experiments within Test Bed 1, a volume of phyllite rock under in-situ stress conditions off the western side of the West Access Drift on the 4850 Level, near Governor’s Corner. Numerical simulations were executed prior to the start of hydraulic stimulation activities within Test Bed 1 following standard practices, using best estimates of principal stress conditions, thermal conditions, and the rock petrophysical properties, including geomechanical properties. These simulations indicated notching of the borehole would promote the initiation of transverse fractures, seismic magnitudes during the hydraulic stimulation would be below 0.1 magnitude on the Richter scale, a rock thermal conductivity of 5.0 W/m K yielded agreement with kISMET borehole temperature logs, back pressure on the production borehole would increase circulation across the test bed, and the production borehole would serve to halt propagation of the hydraulic fracture to the drift. Pre-existing natural fractures, heterogeneities in the rock properties, monitoring boreholes, and overlooked mine elements have prompted a second look at numerically modeling stimulation, fluid circulation, tracer migration, and thermal breakthrough. Numerical simulation is an invaluable tool for providing insight and understanding to complex physical processes. The success of simulations, however, often depends on including all of the salient features of the system in the founding conceptual model. This paper takes a retrospective look at examples where the conceptual model and simulation was sufficient to provide accurate forecasts and those where elements were missing, necessitating rethinking of the simulation.

numerical simulation, EGS Collab, enhanced geother↗

DOE OSTI2023

Operational Focused Data Analytics for Optimizing Radiation Portal Monitor-Based Nuclear Smuggling Detection Systems at Global Ports of Entry

The National Nuclear Security Administration’s Office of Nuclear Smuggling Detection and Deterrence has deployed a fleet of radiation portal monitors (RPMs) across the world at global ports of entry including seaports, airports, and land border crossings. These RPMs are integrated into radiation detection systems (RDS) that also include fixed cameras, optical character recognition (OCR) systems, primary scanning systems (e.g., X-ray or gamma-ray), and secondary scanning systems (e.g., spectroscopic radiation portal monitors, portable radiation detection systems). The data from these sensing technologies is collected at the Central Alarm Station (CAS) where servers and computers reside to control and operate the system. Operators utilize the data collected by the CAS and declared cargo information to make decisions on how to respond to an alarm.This work explores the use of CAS-located data, looking at both the sensor data streams and operator inputs, to perform analysis which supports customs and border protection agencies to improve training capability and operational effectiveness. We focus on analyzing site level effectiveness and behavior by rolling up CAS-located data collected from individual occurrences. To-date, more than 15 sites (e.g., seaports, airports, border crossings) have been analyzed in this manner with the goal of understanding system operations to verify effectiveness and recommend potential improvements. This work first aims to provide background information on relevant CAS-located data sources and our current operational system analytics process including example results. After summarizing our current analytic techniques, we discuss how the future data analytics systems can provide key benefits to improving operational performance while minimizing the burden these detection systems place on operators.

Kuhn, Michael↗

DOE OSTI2019

GPLADD: Quantifying Trust in Government and Commercial Systems A Game-Theoretic Approach

Trust in a microelectronics-based system can be characterized as the level of confidence that a system is free of subversive alterations made during system development, or that the development process of a system has not been manipulated by a malicious adversary. Trust in systems has become an increasing concern over the past decade. This report introduces a novel game-theoretic framework, called GPLADD (Graph-based Probabilistic Learning Attacker and Dynamic Defender), for analyzing and quantifying system trustworthiness at the end of the development process, through the analysis of risk of development-time system manipulation. GPLADD represents attacks and attacker-defender contests over time. Here, time is an explicit constraint and allows incorporating the informational asymmetries between the attacker and defender into analysis. GPLADD includes an explicit representation of attack steps via multi-step attack graphs, attacker and defender strategies, and player actions at different times. GPLADD allows quantifying the attack success probability over time and the attacker and defender costs based on their capabilities and strategies. This ability to quantify different attacks provides an input for evaluation of trust in the development process. We demonstrate GPLADD on an example attack and its variants. We develop a method for representing success probability for arbitrary attacks and derive an explicit analytic characterization of success probability for a specific attack. We present a numeric Monte Carlo study of a small set of attacks, quantify attack success probabilities, attacker and defender costs, and illustrate the options the defender has for limiting the attack success and improving trust in the development process.

37 attack↗

DOE OSTI2020

Dynamic Optimal Dispatch of Energy Systems with Intermittent Renewables and Damage Model

With the increasing penetration of intermittent renewable energy sources into the grid, there is a growing need for process systems-based strategies that integrate dispatchable and variable energy systems for supplying the demand while maintaining grid reliability. The proposed framework corresponds to a dynamic mixed-integer linear programming optimization approach that integrates coal-fired and natural gas-fired power plants, NaS batteries for energy storage, and solar/wind energy to supply the demand. This optimization approach considers an economic goal and constraints to provide power balance while maintaining the overall damage of the natural gas combined cycle (NGCC) power plant drum under a maximum stress as well as avoiding the overheating of the NGCC superheater and reheater. Renewable curtailment levels are also retained at minimum levels. Case studies are analyzed considering different loads and renewable penetration levels. The results show that the demand was met for all cases. Grid flexibility was mostly provided by the NGCC, while the batteries were used sparingly. In addition, considering a CO 2 equivalent analysis, the environmental performance was intrinsically connected to grid flexibility and the level of renewable penetration. Stress analysis results reinforced the necessity for an equipment health-related constraint.

97 MATHEMATICS AND COMPUTING↗

DOE OSTI2017

Review—Practical Challenges Hindering the Development of Solid State Li Ion Batteries

Solid state electrolyte systems boasting Li+ conductivity of >10 mS cm -1 at room temperature have opened the potential for developing a solid state battery with power and energy densities that are competitive with conventional liquid electrolyte systems. The primary focus of this review is twofold. First, differences in Li penetration resistance in solid state systems are discussed, and kinetic limitations of the solid state interface are highlighted. Second, technological challenges associated with processing such systems in relevant form factors are elucidated, and architectures needed for cell level devices in the context of product development are reviewed. Specific research vectors that provide high value to advancing solid state batteries are outlined and discussed.

25 ENERGY STORAGE↗

DOE OSTI2024

Enabling Capabilities and Resources: 2024 Principal Investigator Meeting Proceedings

As a major supporter of basic genome-enabled research, BER’s Biological Systems Science Division (BSSD) fosters scientific discovery by funding - fundamental biological research across disciplines in conjunction with enabling investigational tools and computational capabilities that include world-class user facilities. The overarching goal of BSSD is to provide the necessary fundamental science to understand, predict, manipulate, and design biological systems that underpin innovations for bioenergy and bioproduct production and enhance understanding of natural, DOE-relevant environmental processes (Biological Systems Science Division Strategic Plan, 2021). To accelerate the U.S. bioeconomy, BSSD pursues innovative science underpinning advances in sustainable biofuels and bioproducts and the development of next-generation technologies and computational resources for systems biology research. The 2024 BSSD Enabling Capabilities and Resources (ECR) Principal Investigator (PI) meeting brought together PIs across the BSSD ECR portfolio to confer on shared interests and opportunities. The meeting was held concurrently with the Genomic Science program (GSP) PI meeting to optimize collaboration on research to advance bioenergy and the bioeconomy. Rick Stevens of Argonne National Laboratory gave a keynote on How Generative Artificial Intelligence Can Impact Biological Research (see Keynote: How Generative Artificial Intelligence Can Impact Biological Research, this page). Plenary presentations included several joint sessions that illuminated the integration and understanding of the larger BSSD mission. GSP’s objective is to provide systems-level understanding of plants, microbes, and their communities through its Bioenergy Research, Biosystems Design, and Environmental Microbiome Research portfolios. The objective of the ECR portfolio is to support development of computational and instrumental platforms to advance fundamental GSP research—and BER more broadly— toward the overall goal of understanding the functional principles of living systems and their response to environmental challenges.

59 BASIC BIOLOGICAL SCIENCES↗

DOE OSTI2026

Persistent DynAMICS

Persistent DynAMICS is a lightweight software platform that enables distributed sensing systems to operate as a unified, responsive network. It integrates with existing sensors, data systems, and processing tools as an overlay, without requiring hardware replacement or increasing user burden. As data is collected, the system identifies situations that require additional attention and directs selected sensors to gather more information. For example, if a sensor detects an unusual condition along a pipeline, the system can task nearby sensors or different sensing modalities to confirm the event and focus data collection where it is needed. To support this, the platform forms temporary groups of sensors that work together to address specific objectives. Once complete, these groups are dissolved and resources are reassigned as needed. Communication is handled through an integrated messaging framework with client and server components, enabling reliable operation and data continuity even in low-bandwidth or intermittent connectivity environments.

97 MATHEMATICS AND COMPUTING↗

DOE OSTI2022

SRF Cavity Emulator for PIP-II LLRF Lab and Field Testing

There are many stages in the LLRF and RF system development process for any new accelerator that can take advantage of hardware emulation of the high-power RF system and RF cavities. LLRF development, bench testing, control system development and testing of installed systems must happen well before SRF cavities are available for test. The PIP-II Linac has three frequencies of SRF cavities, 162.5 MHz, 325 MHz and 650 MHz and a simple analog emulator design has been chosen that can meet the cavity bandwidth requirements, provide tuning errors to emulate Lorentz force detuning and microphonics for all cavity types. This emulator design utilizes a quartz crystal with a bandwidth of 65Hz at an IF of ~ 4 MHz, providing a Q of ~ 1.3 x 10^7 at 650MHz. This paper will discuss the design and test results of this emulator.

43 PARTICLE ACCELERATORS↗

DOE OSTI2021

Impact of 2D–3D Heterointerface on Remote Epitaxial Interaction through Graphene

Remote epitaxy has drawn attention as it offers epitaxy of functional materials that can be released from the substrates with atomic precision, thus enabling production and heterointegration of flexible, transferrable, and stackable freestanding single-crystalline membranes. In addition, the remote interaction of atoms and adatoms through two-dimensional (2D) materials in remote epitaxy allows investigating and utilizing electrical/chemical/physical coupling of bulk (3D) materials via 2D materials (3D-2D-3D coupling). Here, we unveil the respective roles and impacts of the substrate material, graphene, substrate-graphene interface, and epitaxial material for electrostatic coupling of these materials, which governs cohesive ordering and can lead to single-crystal epitaxy in the overlying film. Further, we show that simply coating a graphene layer on wafers does not guarantee successful implementation of remote epitaxy, since atomically precise control of the graphene-coated interface is required, and provide key considerations for maximizing the remote electrostatic interaction between the substrate and adatoms. This was enabled by exploring various material systems and processing conditions, and we demonstrate that the rules of remote epitaxy vary significantly depending on the ionicity of material systems as well as the graphene-substrate interface and the epitaxy environment. The general rule of thumb discovered here enables expanding 3D material libraries that can be stacked in freestanding form.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

DOE OSTI2020

Hybrid magnonics: Physics, circuits, and applications for coherent information processing

Hybrid dynamic systems have recently gained interest with respect to both fundamental physics and device applications, particularly with their potential for coherent information processing. In this work, we will focus on the recent rapid developments of magnon-based hybrid systems, which seek to combine magnonic excitations with diverse excitations for transformative applications in devices, circuits, and information processing. Key to their promising potentials is that magnons are highly tunable excitations and can be easily engineered to couple with various dynamic media and platforms. The capability of reaching strong coupling with many different excitations has positioned magnons well for studying solid-state coherent dynamics and exploiting unique functionality. In addition, with their gigahertz frequency bandwidth and the ease of fabrication and miniaturization, magnonic devices and systems can be conveniently integrated into microwave circuits for mimicking a broad range of device concepts that have been applied in microwave electronics, photonics, and quantum information. We will discuss a few potential directions for advancing magnon hybrid systems, including on-chip geometry, novel coherent magnonic functionality, and coherent transduction between different platforms. As a future outlook, we will discuss the opportunities and challenges of magnonic hybrid systems for their applications in quantum information and magnonic logic.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

DOE OSTI2017

Analysis and improvement of input channel selection algorithm for reliability of control systems in nuclear power plants - 138

In most of non-safety NSSS (Nuclear Steam Supply System) control systems, a process input is composed of two channels for redundancy. In a normal situation, the average of both input channels is used in the control algorithm. If a failed channel is detected, the 'channel selection algorithm' chooses the remaining normal input channel. For a bumpless transition, many implemented control systems include the 'ramping rate' function, which makes it possible for the selected input to slowly approach the new input channel. However, it recently turned out that this function adopted for positive effects may result in unintended consequences for the related control system and the plant in certain cases. Due to a process transient in the plant according to a significant event, any related sensor input signal can rapidly change and finally exceed the pre-defined range for detecting an out-of-range event in a short time. During the process of channel conversion due to a rapid transient in the plant, the processed input from the redundant channels can be distorted if the ramping rate function is not properly implemented. As a result, it can result in a plant shutdown because the control system fails to perform the critical function to mitigate a plant transient. To solve these potential problems, we analyzed the overall causes and derived a proposed algorithm for improving reliability and performance of the control systems. (authors)

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

DOE OSTI2025

Contaminant Investigation and Pre‐Processing Opportunities for Textile‐To‐Textile Recycling

Millions of metric tons of textiles are landfilled or incinerated each year in the United States, with less than 1% of textiles recycled into new clothing or fabrics. To counter this trend, a growing number of companies and researchers are exploring how a circular economy can be applied to support textile‐to‐textile recycling. A significant barrier they face comes down to quickly and efficiently extracting pure feedstock material from post‐consumer garments that feature a mix of natural and synthetic fibers. Textile recyclers prefer pure feedstocks, as working with mixed sources typically means lower throughput, higher risk of equipment failure, and diminished business margins. To facilitate a circular economy for textiles, methods, and technologies are needed that can efficiently separate out materials and contaminants from end‐of‐life textiles to increase the flow of pure feedstocks to recyclers. This paper summarizes findings from interviews with a cross section of textile recyclers and from a review of literature to define basic feedstock requirements. In addition to our qualitative research, we deconstruct a bale of post‐consumer textiles and analyze them using computer‐vision imaging, Fourier transform infrared spectroscopy (FTIR), and machine learning. The resulting data are used to set system‐level design inputs for an automated contaminant removal system to process post‐consumer clothing into appropriate feedstocks for recycling. To set the system's levels for automated real‐time near‐infrared analysis, we identify the minimum percentage of primary material that any single garment in a load of used clothing must contain for the average of the full output stream to meet the target purity levels of recyclers. Here, the envisioned automated system can also address undesirable trace materials that might contaminate the processed stream by using imaging cameras coupled with artificial intelligence to identify sections of clothing for de‐trimming. Proof‐of‐concept machine learning algorithms are evaluated to locate and identify trims or garment areas with hidden contaminant materials. Integrating these methods into automated textile cutting systems can provide a cost‐effective means for increasing feedstock purity from used clothing, which can advance circularity for textiles by helping recyclers to reach production volumes and quality targets that were not possible solely with manual dismantling operations.

Parsons, Ryan [Rochester Institute of Technology, ↗

DOE OSTI2021

Climate Change Impacts on the South American Monsoon System and Its Surface–Atmosphere Processes Through RegCM4 CORDEX-CORE Projections

Here, we evaluate projected changes in surface water and energy balances and surface–atmosphere coupling in the South American Monsoon System (SAMS) for the end of the century (2080–2099). The analyses are based on two ensemble datasets, which follow Representative Concentration Pathway 8.5 in the future period, and cover four subdomains (Northern and Southern—NAMZ and SAMZ—Amazon, La Plata Basin—LPB, and Southern Southeast Brazil—SSB). One ensemble consists of three Global Climate Models (HadGEM2-ES, MPI-ESM-MR and NorESM1-M), while the other consists of their dynamically downscaled version at 25 km horizontal grid spacing using Regional Climate Model version 4 (RegCM4). As both ensembles are able in reproducing the annual cycle of the components of the surface water and energy balances in the present climate, they can be used in the study of future climate. During the wet season (November–March), both ensembles project a decrease in precipitation over NAMZ and SAMZ (an exception is RegCM4 that projects a slight increase in SAMZ), and an increase across the LPB and SSB. These changes do not cause retreat or expansion of the monsoon area over the continent, which is similar to the present climate (1995–2014). For the wet season, the ensembles are in line with the presence of a strong surface–atmosphere coupling in LPB and SSB, weak coupling in SAMZ and very weak coupling in NAMZ. For future climate, the coupling is even weaker in NAMZ, which may be a driver for the negative changes in precipitation. For the other subdomains, while the ensembles project similar signals of precipitation changes, they disagree with the surface-atmosphere coupling highlighting the uncertainties in future climate.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2018

Crystalline Silicotitanate (CST) Ion Exchange Media Performance Evaluations in SRS Average Supernate Simulant and Tank 10H Waste Solution to Support TCCR

Savannah River Remediation (SRR) is deploying an “at-tank” ion exchange process to remove radioactive cesium from waste supernate which is referred to as the Tank Closure Cesium Removal (TCCR) system utilizing Crystalline Silicotitanate (CST) media. After being loaded with cesium, but before flushed and dried and sent to Interim Safe Storage (ISS), it is anticipated that the TCCR ion exchange columns will be taken off-line (stagnant) with the CST media still immersed in supernate. The currently designed columns include no active cooling system during processing (although no rmal process fluid flow through the column during operations provides significant cooling) or during off-line conditions and temperature increases are expected in the stagnant, loaded, and liquid-filled columns due to decay heat from the radionuclides absorbed to the CST. As a result, modification of the Tank 10H supernate composition has been considered through the addition of either NaOH or KOH reagents to decrease cesium loading.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

DOE OSTI2022

Impact of 2D-3D heterointerface on remote epitaxial interaction through graphene

Remote epitaxy has drawn attention as it offers epitaxy of functional materials that can be released from the substrates with atomic precision. The realization of remote epitaxy leads to profound impact on production and heterointegration of flexible, transferrable, and stackable freestanding single-crystalline membranes, which can be extremely useful in manufacturing next generation electronic and photonic devices. In addition, the remote interaction of atoms and adatoms through two-dimensional (2D) materials in remote epitaxy allows investigation and utilization of electrical/chemical/physical coupling of bulk (3D) materials via 2D materials (3D-2D-3D coupling). Here, we unveil the respective roles and impacts of the substrate material, graphene, substrate-graphene interface, and epitaxial material for electrostatic coupling of these materials. The coupling governs cohesive ordering and can lead to single-crystal epitaxy in the overlying film. We show that simply coating a graphene layer on wafers does not guarantee successful implementation of remote epitaxy, since atomically precise control of the graphene-coated interface is required. Also, it provides key considerations for maximizing the remote electrostatic interaction between the substrate and adatoms. This was enabled by exploring various material systems and processing conditions, and we demonstrate that the rules of remote epitaxy vary significantly depending on the ionicity of material systems as well as the graphene-substrate interface and the epitaxy environment. The general rule of thumb discovered here enables expanding 3D material libraries that can be stacked in freestanding form.

Lu, Kuangye↗

DOE OSTI2022

Impact of 2D-3D heterointerface on remote epitaxial interaction through graphene

Lu, KUANGYE↗

DOE OSTI2018

Computing erasure metadata and data layout prior to storage using a processing platform

Techniques are provided for computing data and metadata layout prior to storage in a storage system using a processing platform. An exemplary processing platform comprises one or more of a compute node and a burst buffer appliance. The processing platform communicates with a plurality of the compute nodes over a network, wherein a plurality of applications executing on the plurality of compute nodes generate a plurality of data objects; computes erasure metadata for one or more of the data objects on at least one of the compute nodes; and provides the erasure metadata with the corresponding one or more data objects to a storage system. The processing platform optionally determines a full set of the data objects to be stored and queries the storage system to determine an anticipated layout of the full set of the data objects to be stored. The anticipated layout allows special handling, for example, for small files and large files that are identified based on predefined criteria.

96 KNOWLEDGE MANAGEMENT AND PRESERVATION↗

DOE OSTI2021

A Markov framework for generalized post-event systems recovery modeling: From single to multihazards

State-dependent models can be used to represent the system recovery process as a series of stochastic transitions from lower to higher functional states. However, the applications of these models have been limited in scope and there is a lack of a generalized recovery modeling framework. A generalized framework would permit a robust forecasting of systems and system-of-systems recovery under multiple hazards, and more broadly, would contribute to community disaster preparedness. This paper develops a generalized post hazard-event recovery modeling framework based on state-dependent Markov-type processes. We then apply the proposed framework to solve a spectrum of problems that range from hind-casting single-system recovery following a single hazard event to forecasting post-event trajectories under multiple hazards and modeling the recovery of a system-of-systems. First, Markov chains are used to hind-cast the observed recovery for a portfolio of buildings affected by the 2014 South Napa, California, earthquake. Next, Markov processes are used to formulate a parametric post hazard-event recovery model, which can be updated using Bayesian statistics when relevant datasets become available. Semi-Markov processes are then used to develop a more general model of single hazard recovery, which accounts for the intensity of the loading and level of damage caused by the event. Semi-Markov processes with non-renewal features are then used to account for multihazard interactions in a post-event recovery model, and applied to a case study that involves a community in Charleston, South Carolina. Lastly, Markov-type processes are combined with Bayesian networks to model the recovery of residential, commercial, educational, and industrial buildings (system-of-systems) following a hazard event. Overall, these applications demonstrate the versatility of the Markov framework towards handling recovery problems with varying levels of complexity.

42 ENGINEERING↗