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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 757 records · Page 42

Broadband quadrature-squeezed vacuum and nonclassical photon number correlations from a nanophotonic device

We report demonstrations of both quadrature-squeezed vacuum and photon number difference squeezing generated in an integrated nanophotonic device. Squeezed light is generated via strongly driven spontaneous four-wave mixing below threshold in silicon nitride microring resonators. The generated light is characterized with both homodyne detection and direct measurements of photon statistics using photon number–resolving transition-edge sensors. We measure 1.0(1) decibels of broadband quadrature squeezing (~4 decibels inferred on-chip) and 1.5(3) decibels of photon number difference squeezing (~7 decibels inferred on-chip). Nearly single temporal mode operation is achieved, with measured raw unheralded second-order correlations g (2) as high as 1.95(1). Multiphoton events of over 10 photons are directly detected with rates exceeding any previous quantum optical demonstration using integrated nanophotonics. These results will have an enabling impact on scaling continuous variable quantum technology.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Application of Microwave Plasma Atomic Emission Spectrometry and Hydride Generation for Determination of Arsenic and Selenium in Mineral Water

The ability to determine arsenic and selenium at their maximum acceptable concentrations (MAC) in drinking water via microwave plasma atomic emission spectrometry (MP-AES) and hydride generation is shown in this study. The determination of these elements is possible even in samples with a high degree of mineralization (up to 12 g/L). To provide the required sensitivity of determination of both elements, certain operating modes of the spray chamber for hydride generation are chosen. The conditions for the determination of these elements in mineral and medical-table waters are proposed.

36 MATERIALS SCIENCE↗

Acousto-Optic Commutation of Fiber-Optic Channels

An acousto-optic commutator of fiber-optic channels based on a ТеО{sub 2} two-coordinate deflector has been proposed and realized. The commutator yields switching of optical radiation from a single output waveguide into a two-dimensional input matrix of waveguides, or vice versa, switching from any matrix waveguide into a single output one. The main interrelated parameters have been obtained. It has been established that the commutator has a short response time of 2–10 μs, yields up to several hundreds of switching channels, low insertion losses of 2–5 dB, and a considerable inter-channel isolation from –35 to –60 dB. Experiments were performed for the output matrix containing 19 waveguides. The channel multiplexing operating mode of this commutator has been demonstrated, which is simultaneous transmission of a signal from the output waveguide into a given number of waveguides of the input matrix.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

New results from the CUORE experiment

We report that the Cryogenic Underground Observatory for Rare Events (CUORE) is the first bolometric experiment searching for neutrino-less double-beta (0vββ) decay that has been able to reach the one-ton scale. The detector, located at the Laboratori Nazionali del Gran Sasso in Italy, consists of an array of 988 TeO 2 crystals arranged in a compact cylindrical structure of 19 towers. Following the completion of the detector construction in August 2016, CUORE began its first physics data run in 2017 at a base temperature of about 10 mK. Following multiple optimization campaigns in 2018, CUORE is currently in stable operating mode. In 2019, CUORE released its second result of the search for 0vββ corresponding to a TeO 2 exposure of 372.5 kg∙yr and a median exclusion sensitivity to a 130 Te 0vββ decay half-life of 1.7 ∙ 10 25 yr. We find no evidence for 0vββ decay and set a 90% C.I. Bayesian lower limit of 3.2 ∙ 10 25 yr on the 130 Te 0vββ decay half-life. We present the current status of CUORE’s search for 0vββ. We give an update of the CUORE background model and the measurement of the 130 Te two neutrino double-beta (2vββ) decay half-life. Eventually, we show the preliminary results on half-life limits from the analysis of 130 Te 0vββ and 2vββ decay to the first 0 + excited state of 130 Xe.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Automatic Differentiation of C++ Codes on Emerging Manycore Architectures with Sacado

Automatic differentiation (AD) is a well-known technique for evaluating analytic derivatives of calculations implemented on a computer, with numerous software tools available for incorporating AD technology into complex applications. However, a growing challenge for AD is the efficient differentiation of parallel computations implemented on emerging manycore computing architectures such as multicore CPUs, GPUs, and accelerators as these devices become more pervasive. In this work, we explore forward mode, operator overloading-based differentiation of C++ codes on these architectures using the widely available Sacado AD software package. In particular, we leverage Kokkos, a C++ tool providing APIs for implementing parallel computations that is portable to a wide variety of emerging architectures. Here we describe the challenges that arise when differentiating code for these architectures using Kokkos, and two approaches for overcoming them that ensure optimal memory access patterns as well as expose additional dimensions of fine-grained parallelism in the derivative calculation. We describe the results of several computational experiments that demonstrate the performance of the approach on a few contemporary CPU and GPU architectures. We then conclude with applications of these techniques to the simulation of discretized systems of partial differential equations.

97 MATHEMATICS AND COMPUTING↗

Quantitative Scanning Transmission Electron Microscopy for Materials Science: Imaging, Diffraction, Spectroscopy, and Tomography

Scanning transmission electron microscopy (STEM) is one of the most powerful characterization tools in materials science research. Due to instrumentation developments such as highly coherent electron sources, aberration correctors, and direct electron detectors, STEM experiments can examine the structure and properties of materials at length scales of functional devices and materials down to single atoms. STEM encompasses a wide array of flexible operating modes, including imaging, diffraction, spectroscopy, and 3D tomography experiments. This review outlines many common STEM experimental methods with a focus on quantitative data analysis and simulation methods, especially those enabled by open source software. The hope is to introduce both classic and new experimental methods to materials scientists and summarize recent progress in STEM characterization. The review also discusses the strengths and weaknesses of the various STEM methodologies and briefly considers promising future directions for quantitative STEM research.

36 MATERIALS SCIENCE↗

Quantitative imaging of carbon dimer precursor for nanomaterial synthesis in the carbon arc

Delineating the dominant processes responsible for nanomaterial synthesis in a plasmaenvironment requires measurements of the precursor species contributing to the growth ofnanostructures. We performed comprehensive measurements of spatial and temporal profiles ofcarbon dimers in sub-atmospheric-pressure carbon arc by laser-induced fluorescence.Measured spatial profiles of carbon dimers coincide with the growth region of carbon nanotubes (Fang et al2016 Carbon 107 273-80) and vary depending on the arc operation mode, which is determinedby the discharge current and the ablation rate of the graphite anode. The carbon dimer density profileexhibits large spatial and time variations due to motion of the arc core. A comparison of theexperimental data with the 2D simulation results of self-consistent arc modeling shows a goodagreement. The model predicts well the main processes determining spatial profiles of carbondimers.

arc discharge↗

ELM-free and inter-ELM divertor heat flux broadening induced by Edge Harmonics Oscillation in NSTX

A new n=1 dominated Edge Harmonic Oscillation (EHO) has been found in NSTX. The new EHO, rotating toroidally in the counter-current direction and the opposite direction of the neutral beam, was observed during certain inter-ELM and ELM-free periods of H-mode operation. This EHO is associated with a significant broadening of the integral heat flux width (?_int) by up to 150%, and a decrease in the divertor peak heat flux by >60%. An EHO induced filament was also observed by the gas puff imaging diagnostic. The toroidal rotating filaments could change the edge magnetic topology resulting in toroidal rotating strike point splitting and heat flux broadening. Experimental result of the counter current rotation of strike points splitting is consistent with the counter-current EHO.

Divertor heat flux width↗

In-situ biogas upgrading during anaerobic digestion of food waste amended with walnut shell biochar at bench scale

Here, a modified version of an in-situ CO 2 removal process was applied during AD of food waste with two types of walnut shell biochar (WSB) at bench-scale under batch operating mode. Compared to the coarse WSB, the fine WSB has a higher ash content (43 vs. 36 wt%) and higher concentrations of calcium (31 vs. 19 wt% of ash), magnesium (8.4 vs. 5.6 wt% of ash) and sodium (23.4 vs. 0.3 wt% of ash), but a lower potassium concentration (0.2 vs. 40% wt% of ash). The 0.96 - 3.83 g biochar (g VS added ) -1 fine WSB amended digesters produced biogas with 77.5-98.1% CH 4 content by removing 40-96% of the CO 2 compared to the control digesters at mesophilic and thermophilic temperature conditions. In a direct comparison at 1.83 g biochar (g VS added ) -1 , the fine WSB amended digesters (85.7% CH 4 content and 61% CO 2 removal) outperformed the coarse WSB amended digesters (78.9% CH 4 content and 51% CO 2 removal). Biochar addition also increased alkalinity as CaCO3 from 2,800 mg L -1 in the control digesters to 4,800-6,800 mg L -1 providing process stability for food waste AD.

09 BIOMASS FUELS↗

Single-mode porous silicon waveguide interferometers with unity confinement factors for ultra-sensitive surface adlayer sensing

Guided wave-optics has emerged as a promising platform for label free biosensing. However, device sensitivity toward surface-bound small molecules is directly limited by the evanescent interaction and low confinement factor with the active sensing region. Here, we report a mesoporous silicon waveguide design and inverse fabrication technique that resolves the evanescent field interaction limitation while achieving maximal transverse confinement factors and preserving single-mode operation. The waveguide sensors are characterized in a Fabry-Perot interferometer configuration and the ultra-high sensitivity to small molecule adlayers is demonstrated. We also identify dispersion to be a promising degree of freedom for exceeding the sensitivity limits predicted by the conventional non-dispersive effective medium theory.

47 OTHER INSTRUMENTATION↗

Fugitive methane detection using open-path stand-off chirped laser dispersion spectroscopy

We report an open-path chirped laser dispersion spectrometer capable of detecting the atmospheric methane concentration above the background using both specular and diffusive reflective surfaces via two distinct operation modes in a stand-off detection configuration. The system is integrated with simultaneous ranging functionality, which enables average concentration measurements for varying optical pathlengths. The system was first tested for accuracy and characterized to achieve sensitivity of 2.9 p p m - m / H z 1 / 2 and pathlength precision of 0.2 m / H z 1 / 2 with a controlled release of methane outside the laboratory. The instrument was subsequently field-deployed in the proximity of a natural gas compressor station for fugitive methane detection. The instrument successfully detected methane plumes and narrowed down the location of the plume through multi-path measurement. The field measurements were verified by a co-located reference mobile methane sensor.

Chen, Yifeng↗

Metasurface quantum-cascade laser with electrically switchable polarization

Dynamic control of a laser’s output polarization state is desirable for applications in polarization sensitive imaging, spectroscopy, and ellipsometry. Using external elements to control the polarization state is a common approach. Less common and more challenging is directly switching the polarization state of a laser, which, however, has the potential to provide high switching speeds, compactness, and power efficiency. Here, we demonstrate a new approach to achieve direct and electrically controlled polarization switching of a semiconductor laser. This is enabled by integrating a polarization-sensitive metasurface with a semiconductor gain medium to selectively amplify a cavity mode with the designed polarization state, therefore leading to an output in the designed polarization. Here, the demonstration is for a terahertz quantum-cascade laser, which exhibits electrically controlled switching between two linear polarizations separated by 80°, while maintaining an excellent beam with a narrow divergence of ~3°×3° and a single-mode operation fixed at ~3.4 THz, combined with a peak power as high as 93 mW at a temperature of 77 K. The polarization-sensitive metasurface is composed of two interleaved arrays of surface-emitting antennas, all of which are loaded with quantum-cascade gain materials. Each array is designed to resonantly interact with one specific polarization; when electrical bias is selectively applied to the gain material in one array, selective amplification of one polarization occurs. The amplifying metasurface is used along with an output coupler reflector to build a vertical-external-cavity surface-emitting laser whose output polarization state can be switched solely electrically. In conclusion, this work demonstrates the potential of exploiting amplifying polarization-sensitive metasurfaces to create lasers with desirable polarization states—a concept which is applicable beyond the terahertz and can potentially be applied to shorter wavelengths.

47 OTHER INSTRUMENTATION↗

ORBITAL ANGULAR MOMENTUM BEAMS RESEARCH USING A FREE-ELECTRON LASER OSCILLATOR

Orbital angular momentum (OAM) photon beams are excellent tools for non-contact optical manipulation of mat- ter in a broad photon energy range. A free-electron laser (FEL) oscillator is well-suited for studying OAM beams with various features including a wide spectral coverage, wavelength tunability, two-color lasing, polarization control, etc. Here, we report the first experimental demonstration of superposed OAM beams from an oscillator FEL. Lasing at around 458 nm, we have generated superposed OAM beams up to the fourth order as a superposition of two pure OAM modes with opposite helicities. These generated beams have a good beam quality, a high degree of circular polarization, and high power. Using external rf modulation with frequen- cies from 1 to 30 Hz, we also developed a pulsed mode operation of the OAM beams with a highly reproducible temporal structure. FEL operation showcased in this work can be extended to higher photon energies, e.g. using a future x-ray FEL oscillator. The operation of such an OAM FEL also paves the way for the generation of OAM gamma-ray beams via Compton scattering.

Liu, P.↗

Linac to BAR/RCS transfer line design for EIC electron injection system

A transfer line has been designed for the Electron-Ion Collider (EIC) to transport electron bunches from the linac to the Rapid Cycling Synchrotron (RCS). In its initial operational stage, the line accommodates 1 nC electron bunches directly from the linac. To support a future upgrade involving a Beam Accumulator Ring (BAR), which will stack individual bunches to form high-charge 28 nC bunches, the design incorporates two switching dipoles enabling injection into and extraction from the BAR. Additionally, a beam dump has been included for operational flexibility and safety. The final segment of the line interfaces with the RCS through a modified Penner bend, preserving beam quality while satisfying geometric constraints. This layout ensures compatibility with both current and future operational modes of the EIC injection system.

Accelerator Physics↗

New Improved Horizontal Electropolishing System for SRF Cavities

The best performance of niobium SRF accelerating cavities is obtained with surfaces smoothed with electropolishing chemical finishing. Jefferson Lab has recently specified, procured, installed, and commissioned a new versatile production electropolishing (EP) tool. Experience with EP research and operations at JLab as well as vendor interactions and experience guided development of the system specification. Detailed design and fabrication was awarded by contract to Semiconductor Process Equipment Corporation (SPEC). The delivered system was integrated into the JLab chemroom infrastructure and commissioned in 2020. The new EP tool provides much improved heat exchange from the circulating H₂SO₄/HF electrolyte and also the cavity via variable temperature external cooling water flow, resulting in quite uniform cavity wall temperature control and thus improved removal uniformity. With the JLab infrastructure, stabilized process temperature as low as 5 C is available. We describe the system and illustrate operational modes in this contribution.

Reece, C. E.↗

Introduction to IdentiFINDERs

These are slides from a presentation. The identiFINDER provides information on radiation levels. It can automatically identify isotopes in its library. It can save spectra for transfer to a computer, and has a 4-8 hour battery life. The following is covered: an overview, operating modes, getting started, finder mode, search, identification mode, dose & rate, warning & alarm, options (ultra LGH), options (identifinder2), and general procedure.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

CSTT Update: Fuel Quality Analyzer

These are slides from a presentation. The following topics are covered: project background (scope and approach), developing the prototype (timeline), update on intellectual property, analyzer comparisons (improving humidification, stabilizing the baseline, applying clean-up strategy, impact of ionomer content and improving clean-up), proposed operating mode, considerations for testing in real-world conditions (Gen 1 analyzer electronics development, testing partner identified, field trial planning), summary, and future work.

47 OTHER INSTRUMENTATION↗

Storage Ring Current Monitor

The storage ring current monitor is expected to be utilized for the following functions: measurement of the current circulating in the storage ring; measurement of the beam lifetime; measurement of the injection efficiency; provide the level of the circulating current for the equipment protection system; provide amount of charge required for the next injection cycle in the top-up mode operation. The current will be monitored with a parametric current transformer (DCCT) integrated into the vacuum system of the storage ring. The electronic module will convert the current reading into the corresponding voltage which will be measured with a digital voltmeter (DVM). The digitized data will be processed by the control system.

43 PARTICLE ACCELERATORS↗