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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 775 records · Page 43

Instantaneous Photosynthetically Available Radiation (IPAR) prediction models based on Neural Network for ocean waters.

Instantaneous photosynthetically available radiation (IPAR) at the ocean surface and its vertical profile below the surface play a critical role in models to calculate net primary productivity of marine phytoplankton. In this work, we report two IPAR prediction models based on neural network (NN) approach, one for open ocean and the other for coastal waters. These models are trained, validated, and tested using a large volume of synthetic datasets for open ocean and coastal waters simulated by a radiative transfer model. Our NN models are designed to predict IPAR under a large range of atmospheric and oceanic conditions. The NN models can compute subsurface IPAR profile very accurately up to euphotic zone depth. The root mean square errors associated with the diffuse attenuation coefficient of IPAR are less than 0.011 𝑚−1 and 0.036 𝑚−1 for open ocean and coastal waters respectively. The performance of the NN models is better than presently available semi analytical models, with significant superiority in coastal waters.

PACE↗

Predicting Radiation-Induced Plutonium Redox Chemistry using Multi-scale Modeling Methods

Over the the last 70 years plutonium (Pu) has been integral in the development of several technologies that have changed the world, yet our fundamental understanding of its chemistry is still far from complete. This is a testament to this element’s unique and complex properties, such as its ability to coexist as multiple oxidation states in aqueous solution. Careful manipulation of plutonium oxidation states is essential in the study and utilization of its rich chemistry. To achieve this level of control, a comprehensive mechanistic understanding of radiation-induced plutonium redox chemistry is critical due to the unavoidable exposure of plutonium to ionizing radiation fields, both inherent and from in-process applications. For this reason, we have developed an experimentally evaluated multi-scale computer model for the prediction of gamma radiation-induced Pu(IV) redox chemistry in concentrated nitric acid solutions (1.0, 3.0, and 6.0 M). Under these acidic, aqueous solution conditions, cobalt-60 gamma irradiation afforded negligible net change in the steady-state oxidation state distribution of Pu(IV). Multi-scale calculations, which are in excellent agreement with experimental data, indicate that this observation is due to radiation-induced redox cycling between Pu(IV) and Pu(III), as achieved by the reduction of Pu(IV) by radiolytic nitrous acid and hydrogen peroxide, and the oxidation of Pu(III) by nitrate and hydroxyl radicals. These radiation-induced redox processes are augmented by plutonium’s inherent disproportionation reactions.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗

Integrative Analysis of Desert Dust Size and Abundance Suggests Less Dust Climate Cooling

Desert dust aerosols affect Earths global energy balance through interactions with radiation, clouds, and ecosystems. But the magnitudes of these effects are so uncertain that it remains unclear whether atmospheric dust has a net warming or cooling effect on global climate. Consequently, it is still uncertain whether large changes in atmospheric dust loading over the past century have slowed or accelerated anthropogenic climate change, and the climate impact of possible future alterations in dust loading is similarly disputed. Here we use an integrative analysis of dust aerosol sizes and abundance to constrain the climatic impact of dust through direct interactions with radiation. Using a combination of observational, experimental, and model data, we find that atmospheric dust is substantially coarser than represented in current climate models. Since coarse dust warms global climate, the dust direct radiative effect (DRE) is likely less cooling than the 0.4 W m superscript 2 estimated by models in a current ensemble. We constrain the dust DRE to -0.20 (-0.48 to +0.20) W m superscript 2, which suggests that the dust DRE produces only about half the cooling that current models estimate, and raises the possibility that dust DRE is actually net warming the planet.

Atmospheric chemistry↗

An economical net solar flux radiometer.

The theory and design of an economical solar flux radiometer readily adaptable to the conventional radiosonde system are presented in response to the need cited by the Atmospheric Radiation Working Group (1971) for the development of an inexpensive light-weight short-wave radiometer sonde. Prototype instrument tests and current modifications are discussed. It is shown that the basic instrument can be easily modified to measure separately the upward and downward directed flux components, in addition to the net flux.

Darkow, G. L.↗

Accomplishments of Thermal Neutron Scattering Research at North Carolina State University [Slides]

Thermal neutron scattering law (TSL) data evaluations have been completed and contributed to ENDF. New evaluations are underway. FLASSH is developing as a modern platform for thermal neutron data analysis featuring an enhanced user experience and low learning overhead. Advanced TSL techniques in combination with Doppler analysis have been developed, which were incorporated into FLASSH. ML/DL NeTS method development has been initiated. Experimental capabilities for validation have been developed at the PULSTAR reactor.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

The Development of a Nonequilibrium Radiative Heat Transfer Computational Model for High Altitude Entry Vehicle Flowfield Methods

This final report will attempt to concisely summarize the activities and accomplishments associated with NASA Grant and to include pertinent documents in an appendix. The project initially had one primary and several secondary objectives. The original primary objective was to couple into the NASA Johnson Space Center (JSC) nonequilibrium chemistry Euler equation entry vehicle flowfield code, INEQ3D, the Texas A&M University (TAMU) local thermodynamic nonequilibrium (LTNE) radiation model. This model had previously been developed and verified under NASA Langley and NASA Johnson sponsorship as part of a viscous shock layer entry vehicle flowfield code. The secondary objectives were: (1) to investigate the necessity of including the radiative flux term in the vibrational-electron-electronic (VEE) energy equation as well as in the global energy equation, (2) to determine the importance of including the small net change in electronic energy between products and reactants which occurs during a chemical reaction, and (3) to study the effect of atom-atom impact ionization reactions on entry vehicle nonequilibrium flowfield chemistry and radiation. For each, of these objectives, it was assumed that the code would be applicable to lunar return entry conditions, i.e. altitude above 75 km, velocity greater, than 11 km/sec, where nonequilibrium chemistry and radiative heating phenomena would be significant. In addition, it was tacitly assumed that as part of the project the code would be applied to a variety of flight conditions and geometries.

Carlson, Leland A.↗

Approach to Defect-Free Lifetime and High Electron Density in CdTe

Achieving simultaneously high carrier density and lifetime is crucial to II-VI semiconductor-based applications such as photovoltaics and infrared detectors; yet, it is a challenging task. In this work, high purity CdTe single crystals doped with indium (In) were grown by vertical Bridgman melt growth under carefully controlled stoichiometry. Two-photon excitation time-resolved photoluminescence was employed to measure bulk recombination lifetime by eliminating surface recombination effects. By adjusting stoichiometry with post growth annealing, high-net free carrier density approaching 10 18 cm -3 was attained simultaneously with lifetime approaching the radiative limit by suppressing non-radiative recombination centers.

14 SOLAR ENERGY↗

BTRIC Technical Support for Appalachia: FY 2024 Summary Report on Net Negative Carbon Building Demonstration with AgPod

This report investigates the effects of various concentrations of CO 2 on the photosynthesis and biomass accumulation of crops growing in an AgPod, using kale as the test crop. In the first year of the study, increasing the CO 2 concentration in the AgPod was found to promote higher photosynthetic rates in kale plants up to 1,300 ppm (the highest CO 2 concentration measured). An interesting finding was that net photosynthetic rates of kale leaves remain unsaturated until reaching unusually high levels of photosynthetically active radiation (PAR, > 1,200 µmol m -1 s -1 ) and CO 2 concentration (> 1,100 ppm). Such high levels of saturating PAR and CO 2 concentration values rarely occur under natural conditions, suggesting a promising potential for carbon capture via enriched controlled environment agriculture (ECEA). During the second year of the study, a second crop was planted to confirm the actual effects on growth with increased CO 2 concentrations. Our results suggest that growing kale plants in the AgPod system at higher CO 2 levels resulted in a successful and highly productive crop, up to three times the amount grown at 415 CO 2 . Further, the kale plants grown under higher CO 2 conditions (1000 ppm) are not CO 2 saturated and can potentially further improve yield at even higher CO 2 environments.

32 ENERGY CONSERVATION, CONSUMPTION, AND UTILIZATI↗

Multichannel spectrophotometry of stellar flares

Stellar flares have been observed using the 32 channel spectrophotometer on the 5 m telescope. Net flare fluxes in the region 3200-7000 A are presented. A simple model of blackbody radiation and hydrogen recombination emission appears to fit the continuum points well. Owing to vignetting problems, only the region between 4200 and 7000 A was used for a detailed fit to the Planck function to obtain apparent temperatures and effective areas. The rise of each flare was associated with an increase of the area, while the initial steep decline of the light was associated with a similar decrease of the blackbody temperature. The maximum temperatures, coincident with maximum light, were 7500-9500 K, similar to values for solar flares. The hydrogen line emission rose simultaneously with the continuum but declined more slowly. The ratio of H sub gamma to H sub alpha was about 1.5 at the peak, declining to about 1.0 after the peak.

Mochnacki, S. W.↗

Several features of the earthward and tailward streaming of energetic protons /0.29-0.5 MeV/ in the earth's plasma sheet

The reported investigation represents an extension of a study conducted by Lui and Krimigis (1981) who have examined the question of transport of energetic protons measured by the Charged Particle Measurements Experiment on IMP 7 and 8 in the magnetotail. It has been shown that there is a substantial net earthward transport of these particles, with fluxes seemingly capable of replenishing the losses of outer radiation belt protons. In the current investigation the earlier study is extended by reporting several features of the earthward and tailward streaming of these energetic protons. Attention is given to selection criteria and isolation of magnetospheric protons, the dawn-dusk reversal in streaming anisotropy, the amplitude of streaming anisotropy, and spectral hardness.

Lui, A. T. Y.↗

Absolute measurement of the extreme UV solar flux

A windowless rare-gas ionization chamber has been developed to measure the absolute value of the solar extreme UV flux in the 50-575-A region. Successful results were obtained on a solar-pointing sounding rocket. The ionization chamber, operated in total absorption, is an inherently stable absolute detector of ionizing UV radiation and was designed to be independent of effects from secondary ionization and gas effusion. The net error of the measurement is + or - 7.3 percent, which is primarily due to residual outgassing in the instrument, other errors such as multiple ionization, photoelectron collection, and extrapolation to the zero atmospheric optical depth being small in comparison. For the day of the flight, Aug. 10, 1982, the solar irradiance (50-575 A), normalized to unit solar distance, was found to be 5.71 + or - 0.42 x 10 to the 10th photons per sq cm sec.

Carlson, R. W.↗

On the sensitivity of a residual circulation model to differences in input temperature data

The residual mean circulation (RMC) formulation of zonally averaged transport in the middle atmosphere produces a circulation which depends on the distributions of net diabatic heating and temperature. Such circulations are from two temperature data sets, using the same radiative transfer code (Rosenfield et al. 1987). These circulations are then used to transport N2O in a photochemical model. The circulations and the resulting N2O distributions are notably different during the Northern Hemisphere winter, with that based on the NMC temperatures producing too much upward transport in the tropical stratosphere, as judged by comparison with the stratospheric and mesoscale sounder data. The experiment demonstrates that model calculations, in general, and perturbation assessments, in particular, are likely to be quite sensitive to the choice of input temperature data (where this is not computed self-consistently). It also reveals what appears to be a seasonally dependent bias in NMC zonally averaged temperatures with respect to those obtained from the LIMS instrument during 1978/1979.

Guthrie, Paul D.↗

Resonance transition radiation X-ray laser

A free electron laser is proposed using a periodic dielectric and helical magnetic field. Periodic synchronism between the electrons and the optical wave is obtained at the period of the dielectric and not at the period of the helical magnetic field. The synchronism condition and the gain of the new device are derived. The effects on the gain from dephasing and beam expansion due to elastic scattering of the electrons in the periodic medium are included in the gain calculation. Examples of the resonance transition radiation laser and klystron are given. Operation at photon energies between 2.5 and 3.5 keV with net gain up to 12 percent is feasible using high electron-beam energies of 3 and 5 GeV. Moderate (300-MeV) beam energy allows operation between 80 to 110 eV with up to 57 percent net gain using a klystron design. In both cases, rapid foil heating may limit operation to a single electron-beam pulse.

Reid, Max B.↗

Thermal and Driven Stochastic Growth of Langmuir Waves in the Solar Wind and Earth's Foreshock

Statistical distributions of Langmuir wave fields in the solar wind and the edge of Earth's foreshock are analyzed and compared with predictions for stochastic growth theory (SGT). SGT quantitatively explains the solar wind, edge, and deep foreshock data as pure thermal waves, driven thermal waves subject to net linear growth and stochastic effects, and as waves in a pure SGT state, respectively, plus radiation near the plasma frequency f(sub p). These changes are interpreted in terms of spatial variations in the beam instability's growth rate and evolution toward a pure SGT state. SGT analyses of field distributions are shown to provide a viable alternative to thermal noise spectroscopy for wave instruments with coarse frequency resolution, and to separate f(sub p) radiation from Langmuir waves.

Cairns, Iver H.↗

Progress on Pu-238 Production at Idaho National Laboratory From February 2022 to December 2022

Idaho National Laboratory (INL) has continued to qualify irradiation positions in the Advanced Test Reactor (ATR) for Pu-238 production to support NASA deep space missions. Over the past year, INL qualified Np-237 targets for ATR’s North East Flux Trap (NEFT), inner A, and H positions. Work has begun to requalify the South Flux Trap (SFT) and qualify the East Flux Trap (EFT) for the ATR GEN I target and is midway through the qualification process. This paper gives an overview of operational and technical activities from February 2022 to December 2022.

07 ISOTOPE AND RADIATION SOURCES↗

Effect of Confinement of SIA Cluster Diffusion by Impurities on Radiation Defect Accumulation due to 14MeV neutrons in Tungsten

Impurities acting as traps, reduce the self-interstitial atom (SIA) cluster mobility, thereby increasing recombination and in turn enhancing radiation-resistance of polycrystalline materials. However, at elevated temperatures, depending on SIA-trap (impurity) binding energy, SIA clusters may trap and detrap (detach) numerous times. In tungsten, SIA clusters of all sizes glide one-dimensionally (1D) along their Burgers vector direction. Hence, detrapped SIAs would retrace their path, confining their 1D-glide between traps. However, small SIA clusters can change the direction of their 1D-glide by overcoming a rotation barrier. In addition, impurities or solutes are known to reduce this barrier. A lower rotation barrier can result in detrapped SIA clusters that diffuse in a random 1D direction, effectively leading to 3D (net-3D) diffusion. Here we investigate the effect of two cases of SIA diffusion, namely confined-1D diffusion and net-3D diffusion, on the damage accumulation in polycrystalline tungsten under 14 MeV neutron irradiation using the object kinetic Monte Carlo method. Simulations were performed using cascade debris obtained from molecular dynamics simulations with primary knock-on atom (PKA) energies corresponding to 14 MeV neutrons. In the simulations with net-3D diffusion, SIA clusters of all sizes diffuse in a random 1D direction after the clusters detrap. While for the confined 1D diffusion case, SIA clusters larger than size 5 retain their original direction of 1D-glide. In both types of simulations, trapped vacancies are assumed to be permanently immobilized. Unexpectedly, the damage accumulation was lower with confined 1D diffusion than that with net-3D. We present a systematic comparison of the influence of the two cases of SIA diffusion on the radiation damage accumulation as a function of dose rate, detrapping barrier, and impurity concentration at 1025 K.

Accumulation and recovery of lattice damage, tungs↗

Neural Thermal Scattering (NeTS) Modules for Graphite & Beryllium [Slides]

This presentation discusses the motivations behind the project, which include facilitating compact formulation for TSL data, extending AI knowledge, and providing advanced reactor simulation framework. It also discusses how the project accounts for beryllium and graphite complexity, including atomistic, dynamical, and neural. Additionally, new material-informed neural thermal scattering (NeTS) Modules are examined. The implications, conclusions, and plan future work for the project are also discussed.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

CERES ERBE-like Monthly Geographical Averages (ES-4) in HDF (CER_ES4_Terra-FM1_Edition1)

The ERBE-like Monthly Geographical Averages (ES-4) product contains a month of space and time averaged Clouds and the Earth's Radiant Energy System (CERES) data for a single scanner instrument. The ES-4 is also produced for combinations of scanner instruments. For each observed 2.5-degree spatial region, the daily average, the hourly average over the month, and the overall monthly average of shortwave and longwave fluxes at the Top-of-the-Atmosphere (TOA) from the CERES ES-9 product are spatially nested up from 2.5-degree regions to 5- and 10-degree regions, to 2.5-, 5-, and 10-degree zonal averages, and to global monthly averages. For each nested area, the albedo and net flux are given. For each region, the daily average flux is estimated from an algorithm that uses the available hourly data, scene identification data, and diurnal models. This algorithm is 'like' the algorithm used for the Earth Radiation Budget Experiment (ERBE). The following CERES ES4 data sets are currently available: CER_ES4_FM1+FM2_Edition1 CER_ES4_PFM+FM1+FM2_Edition1 CER_ES4_PFM+FM1+FM2_Edition2 CER_ES4_PFM+FM1_Edition1 CER_ES4_PFM+FM2_Edition1 CER_ES4_TRMM-PFM_Edition1 CER_ES4_TRMM-PFM_Edition2 CER_ES4_Terra-FM1_Edition1 CER_ES4_Terra-FM2_Edition1 CER_ES4_FM1+FM2_Edition2 CER_ES4_Terra-FM1_Edition2 CER_ES4_Terra-FM2_Edition2 CER_ES4_Aqua-FM3_Edition1 CER_ES4_Aqua-FM4_Edition1 CER_ES4_FM1+FM2+FM3+FM4_Edition1 CER_ES4_Aqua-FM3_Edition2 CER_ES4_Aqua-FM4_Edition2 CER_ES4_FM1+FM3_Edition2 CER_ES4_FM1+FM4_Edition2 CER_ES4_PFM+FM1_Edition2 CER_ES4_PFM+FM2_Edition2 CER_ES4_Aqua-FM3_Edition1-CV CER_ES4_Aqua-FM4_Edition1-CV CER_ES4_Terra-FM1_Edition1-CV CER_ES4_Terra-FM2_Edition1-CV. [Location=GLOBAL] [Temporal_Coverage: Start_Date=1998-01-01; Stop_Date=2005-10-31] [Spatial_Coverage: Southernmost_Latitude=-90; Northernmost_Latitude=90; Westernmost_Longitude=-180; Easternmost_Longitude=180] [Data_Resolution: Latitude_Resolution=2.5 degree; Longitude_Resolution=2.5 degree; Horizontal_Resolution_Range=250 km - < 500 km or approximately 2.5 degrees - < 5.0 degrees; Temporal_Resolution=1 month; Temporal_Resolution_Range=Monthly - < Annual].

CLEAR-SKY LONGWAVE FLUX↗